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  <front>
    <journal-meta><journal-id journal-id-type="publisher">AMT</journal-id><journal-title-group>
    <journal-title>Atmospheric Measurement Techniques</journal-title>
    <abbrev-journal-title abbrev-type="publisher">AMT</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Meas. Tech.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1867-8548</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/amt-19-4367-2026</article-id><title-group><article-title>An ensemble machine-learning first-guess approach for physics-based retrieval of ice particle size distributions from multi-frequency radar, validated with CCREST-M aircraft observations</article-title><alt-title>An ensemble machine-learning first-guess approach</alt-title>
      </title-group>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1 aff2">
          <name><surname>Baran</surname><given-names>Anthony J.</given-names></name>
          <email>anthony.baran@metoffice.gov.uk</email>
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Fox</surname><given-names>Stuart</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-3110-872X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Cotton</surname><given-names>Richard</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff3">
          <name><surname>Delanoë</surname><given-names>Julien</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff4 aff5">
          <name><surname>Walden</surname><given-names>Christopher J.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-5718-466X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff6">
          <name><surname>McCusker</surname><given-names>Karina</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1886-5323</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff6">
          <name><surname>Westbrook</surname><given-names>Christopher D.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff4">
          <name><surname>Huggard</surname><given-names>Peter G.</given-names></name>
          
        </contrib>
        <aff id="aff1"><label>1</label><institution>Met Office, FitzRoy Road, Exeter, EX1 3PB, UK</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>School of Physics, Astronomy, and Mathematics, University of Hertfordshire, Hatfield, AL10 9AB, UK</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Laboratoire Atmosphère, Milieux et Observations Spatiales, IPSL, UVSQ Université Paris-Saclay, Sorbonne Université,  CNRS, Guyancourt, France</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>RAL Space, STFC Rutherford Appleton Laboratory, Didcot, OX11 OQX, UK</institution>
        </aff>
        <aff id="aff5"><label>5</label><institution>National Centre for Atmospheric Science, Leeds, UK</institution>
        </aff>
        <aff id="aff6"><label>6</label><institution>Department of Meteorology, University of Reading, Reading, UK</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Anthony J. Baran (anthony.baran@metoffice.gov.uk)</corresp></author-notes><pub-date><day>1</day><month>July</month><year>2026</year></pub-date>
      
      <volume>19</volume>
      <issue>12</issue>
      <fpage>4367</fpage><lpage>4392</lpage>
      <history>
        <date date-type="received"><day>10</day><month>February</month><year>2026</year></date>
           <date date-type="rev-request"><day>17</day><month>February</month><year>2026</year></date>
           <date date-type="rev-recd"><day>28</day><month>May</month><year>2026</year></date>
           <date date-type="accepted"><day>9</day><month>June</month><year>2026</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2026 Anthony J. Baran et al.</copyright-statement>
        <copyright-year>2026</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026.html">This article is available from https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026.html</self-uri><self-uri xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026.pdf">The full text article is available as a PDF file from https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d2e181">The Characterising CiRrus and icE cloud acrosS the specTrum-Microwave (CCREST-M) aircraft campaign (February–March 2024) was based around the Chilbolton Observatory, UK, using the Facility for Airborne Atmospheric Measurements (FAAM) BAe-146 aircraft together with ground-based multi-frequency radars to provide a testbed for ice-cloud scattering and radiative transfer models across the microwave and sub-millimetre spectrum.  Ice particle size distributions (PSDs) are retrieved from the ground-based zenith-pointing radars at the time of the radiometric overpasses, and the aircraft in-situ PSDs are used as an independent validation dataset.</p>

      <p id="d2e184">We present a novel hybrid retrieval framework for mid-latitude ice PSD parameters (slope <inline-formula><mml:math id="M1" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, intercept <inline-formula><mml:math id="M2" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and shape <inline-formula><mml:math id="M3" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> of the gamma size distribution) that combines a machine-learning (ML) ensemble with physics-based multi-frequency radar retrievals using 3, 35, and 94 <inline-formula><mml:math id="M4" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> reflectivities. An ensemble of ML models is trained on observations from the Parameterising Ice Clouds using Airborne ObServationS and triple-frequency dOppler radar (PICASSO) campaign, also centred on Chilbolton Observatory.  These models predict PSD moments from temperature, pressure, 3 <inline-formula><mml:math id="M5" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>-retrieved ice water content (IWC), and the mean mass-weighted dimension. The ML predictions are converted into first guess gamma-PSD parameters at each height. A subsequent deterministic optimisation then adjusts <inline-formula><mml:math id="M6" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M7" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, using a randomly oriented rosette-aggregate scattering model, to enforce simultaneous agreement with the observed 35 and 94 <inline-formula><mml:math id="M8" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> reflectivities.</p>

      <p id="d2e255">Application of the above method to three CCREST-M cases show that the ML ensemble reproduces PSD moments well for two cases but fails when extrapolating beyond its trained temperature range in the third case.  Retrieved IWCs from the 3 <inline-formula><mml:math id="M9" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar compare favourably with in-situ measurements of IWC, and exponential (<inline-formula><mml:math id="M10" display="inline"><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>) and gamma PSD assumptions show comparable performance overall. Retrieved mean PSDs show generally good agreement with in-situ PSDs as a function of temperature for two of the cases, with IWCs within about 50 % of the in-situ measured IWCs over much of the <inline-formula><mml:math id="M11" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M12" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M13" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula> temperature range. The systematic biases seen in one case are attributed to temporal cloud evolution between radar and in-situ sampling. Independent validation using 200 <inline-formula><mml:math id="M14" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivity profiles shows good agreement between the forward-modelled refllectivities and measurements above about 4.5 <inline-formula><mml:math id="M15" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>. Below 4.5 <inline-formula><mml:math id="M16" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> the agreement is more sparse owing to the likely presence of dendritic particles, which depart from the rosette-aggregate scattering assumption.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d2e342">Accurate representation of ice crystal scattering properties and PSDs in cirrus and ice clouds is fundamental to improving numerical weather prediction and climate modelling (Liou, 1986; Baran, 2009, 2012; Yang et al., 2015; Liou and Yang, 2016; Krämer et al., 2025), and data assimilation (Geer and Baordo, 2014; Geer et al., 2017; Geer et al., 2021). Moreover, satellite missions such as EarthCARE (Earth, Clouds, Aerosols and Radiation Explorer; Illingworth et al., 2015; Mason et al., 2024; Barker et al., 2025) and the forthcoming Ice Cloud Imager (ICI; Eriksson et al., 2020; May et al., 2024) further heighten the need for realistic forward operators linking cloud microphysics to radar and radiometric observables.</p>
      <p id="d2e345">The assimilation of radar reflectivity into weather prediction models has become increasingly important for improving convective precipitation forecasts, as radar reflectivity provides information on the vertical structure of hydrometeors, IWC and on cloud development. However, this requires accurate forward operators that link model state variables to radar observations (Janisková, 2015; Liu et al., 2024), placing stringent demands on ice crystal scattering representations. Earlier work by Baran et al. (2011) demonstrated that ensemble models of ice crystals could be used to simulate equivalent radar reflectivity at 94 <inline-formula><mml:math id="M17" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> with forward model errors generally within <inline-formula><mml:math id="M18" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M19" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. Subsequent studies have demonstrated that spheroidal approximations can bias retrieved water contents (Fontaine et al., 2017; Schrom and Kumjian, 2019), and studies that directly assimilate radar reflectivity from both rainwater and ice-phase species (i.e., snow and graupel) have shown that the ice species significantly improves the analysis of the vertical hydrometeor spatial distributions (Wang and Liu, 2019). Moreover, a study by Hong et al. (2025), building on the findings of Baran et al. (2011) and Wu et al. (2024), demonstrated that incorporating multiple ice habits in the retrieval of snowfall rate from passive microwave radiometers significantly improved retrieval accuracy compared to assuming single ice crystal habits. Polarimetric observations above 100 <inline-formula><mml:math id="M20" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> have suggested that mixtures of random and oriented ice crystals may be needed to represent natural variability within the ice cloud (Brath et al., 2020; McCusker et al., 2024).</p>
      <p id="d2e382">A further uncertainty in retrievals of ice cloud properties is the functional form of the PSD. Recent studies have shown contrasting results, with Bartolomé García et al. (2024) suggesting that bimodal PSDs may offer improved realism over monomodal representations, especially in complex cloud scenes. However, for larger particles – such as those found in snow, where radar reflectivity becomes more sensitive to the upper end of the size distribution – exponential forms are still widely used. For instance, Wood and L'Ecuyer (2021) argue for the adequacy of exponential PSDs in their W-band retrievals of snow properties based on observational evidence. Similarly, McCusker et al. (2024) adopted an exponential PSD assumption to retrieve the slope parameter while holding the intercept parameter fixed, to characterise PSDs in a frontal mid-latitude system using airborne 35 <inline-formula><mml:math id="M21" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar measurements. Their retrievals were able to replicate the polarisation dependent brightness temperature depressions observed at 243 <inline-formula><mml:math id="M22" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> using the International Sub-Millimetre Airborne Radiometer (ISMAR; Fox et al., 2017). Conversely, gamma distributions have been preferred in other studies. For instance, Heymsfield et al. (2023), analysing quadruple-frequency radar observations from the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) field campaign data, prefer gamma PSDs to characterise snowstorms.  Using the same dataset, Duffy and Posselt (2022) found that a gamma distribution with <inline-formula><mml:math id="M23" display="inline"><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.25</mml:mn></mml:mrow></mml:math></inline-formula> best represented the mass- and reflectivity-related moments of the observed PSDs. These differences highlight the need for retrieval frameworks that can flexibly accommodate both exponential and gamma PSDs while remaining physically constrained by realistic scattering models.</p>
      <p id="d2e415">Closure tests between ice-cloud scattering models and radiometric observations require a near one-to-one relationship between the PSDs used as input to the radiative transfer model and the radiometric measurements.  Since a single research aircraft cannot simultaneously perform above-cloud radiometric measurements and in-situ microphysics sampling within the same cloud volume, we must retrieve the PSDs from ground-based multi-frequency radars that are co-incident with the radiometric overpasses. The CCREST-M campaign was designed to address this challenge by combining the FAAM BAe-146 aircraft measurements with co-located ground-based multi-frequency radars. The PSDs are then retrieved from the zenith-pointing radars at the same time as the radiometric overpasses, and the in-situ measured PSDs serve as an independent validation dataset. In this paper, we present a novel retrieval framework that combines an ensemble of machine learning models with physical radar retrievals to estimate PSD gamma parameters and IWC from 3, 35 and 94 <inline-formula><mml:math id="M24" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar observations. The ML ensemble provides first-guess estimates of the PSD parameters from inputs of temperature, pressure, 3 <inline-formula><mml:math id="M25" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>-retrieved IWC and the mean mass-weighted dimension, where the latter is estimated from a temperature-dependent second order polynomial obtained from the PICASSO climatology. A physical optimisation, using the scattering properties of randomly oriented rosette aggregates, is then used to modify <inline-formula><mml:math id="M26" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, with <inline-formula><mml:math id="M28" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> kept as its first-guess profile values, at each height level so that simulated 35 and 94 <inline-formula><mml:math id="M29" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> reflectivities match the observed values.</p>
      <p id="d2e469">The retrieved PSDs are compared with the in-situ PSDs measured by the FAAM BAe-146 aircraft for three case studies, and the retrieval methodology is further evaluated using the G-band 200 <inline-formula><mml:math id="M30" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivity observations from the Chilbolton Observatory GRaCE radar (Courtier et al., 2022). The G-band radar has recently been used by McCusker et al. (2025) to demonstrate the usefulness of such high-frequency radars to directly retrieve the IWC and snow rate of deep frontal mid-latitude cloud. This paper is the first demonstration of an ML-ensemble-assisted, physics-based radar retrieval of ice cloud PSDs validated with aircraft data. Although the same PICASSO climatology could in principle be used to define Bayesian priors in a classical optimal-estimation framework, we instead employ a machine-learning-based first guess. This approach implicitly captures the joint distribution of the local climatology without requiring an explicit multivariate error covariance and vertical correlation structure for (<inline-formula><mml:math id="M31" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M32" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M33" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>) and keeps the subsequent physics-based optimisation computationally straightforward.</p>
      <p id="d2e505">The paper is organised as follows: Section 2 describes the CCREST-M campaign, radars, and aircraft data. Section 3 outlines the ice crystal scattering model used in the forward operator, which is also formally defined in this section. Section 4 details the retrieval methodology, including the ML-ensemble approach developed using the PICASSO dataset, and the optimisation method applied to retrieve the PSD parameters and IWC from the radar reflectivity observations. Section 5 presents the retrieval results for the PSDs using three CCREST-M case studies, with detailed comparisons against in-situ aircraft measurements and forward-modelled radar reflectivities, including their residuals. Section 6 summarises the main findings and provides the conclusions.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>The rationale of the CCREST-M campaign, instrumentation and data</title>
      <p id="d2e516">The CCREST-M campaign combined coordinated FAAM BAe-146 aircraft measurements with ground-based radars at the Chilbolton Observatory, UK (51.15° N, 1.44° W; 84 <inline-formula><mml:math id="M34" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> above mean sea level), to study the microphysical and mm-wave and sub-mm-wave radiative properties of mid-latitude ice clouds. Three radars operated near-synchronously: the 3 <inline-formula><mml:math id="M35" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> CAMRa (Naud et al., 2005), the 35 <inline-formula><mml:math id="M36" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> Kepler, and the 94 <inline-formula><mml:math id="M37" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> mini-BASTA (Delanoë et al., 2016), providing complementary sensitivity across the particle-size spectrum. Detailed specifications for the 35 <inline-formula><mml:math id="M38" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> Kepler radar are provided on the National Centre for Atmospheric Science Atmospheric Measurement and Observation Facility website: <uri>https://amof.ac.uk/instruments/mobile-cloud-radar/</uri> (last access: 26 June 2026).</p>
      <p id="d2e563">This campaign was explicitly designed to deliver multi-frequency active measurements together with near-simultaneous passive measurements extending into the sub-millimetre. In particular, Chilbolton Observatory hosted the multi-frequency radars, and for one of the cases the 200 <inline-formula><mml:math id="M39" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> G-band GRaCE radar, while the FAAM aircraft carried the mm-wave and sub-mm-wave radiometers as well as the in-situ instrumentation. This combination enables the probing of the bulk microphysics with the lower-frequency radars and tests ice crystal scattering and radiative transfer models using the higher frequency radiometers. Since only one aircraft platform was available, CCREST-M could not obtain in-situ microphysical sampling at the same time and location as the radiometric overpasses. High-level radiometric legs and in-situ sampling had to be flown sequentially, so by the time the aircraft descended into the cloud the cloud volume sampled had evolved. In CCREST-M, the strategy is therefore to retrieve the PSDs from the ground-based multi-frequency radars at the time of the radiometric overpasses, and to use the in-situ PSDs from dedicated sampling legs as an independent validation dataset for the retrieved PSDs. This design, with a near one-to-one relationship between the retrieved PSDs and radiometric measurements makes CCREST-M a particularly stringent testbed for ice crystal scattering and radiative transfer models.</p>
      <p id="d2e574">The CCREST-M strategy therefore differs from earlier campaigns such as the Cirrus Coupled Cloud-Radiation Experiment (CIRCCREX), the North Atlantic Waveguide and Downstream Impact Experiment (NAWDEX), and PIKNMIX-F, which have provided useful active and/or passive observations of ice cloud but suffered from inexact passive/active collocation or lacked in-situ observations. CCREST-M also builds upon the PICASSO campaign (Sephton, 2022), which collected in-situ bulk and microphysical properties of ice clouds using the FAAM BAe-146 aircraft, alongside co-located ground-based radar observations at 3, 35 and 94 <inline-formula><mml:math id="M40" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> from Chilbolton Observatory, but lacked radiometric mm-wave and sub-mm-wave measurements to complement the multi-frequency radar measurements.</p>

      <fig id="F1" specific-use="star"><label>Figure 1</label><caption><p id="d2e588">A typical CCREST-M flight track (shown as the grey, orange and blue colours) towards and over the Chilbolton-based triple-frequency radars. The figure-of-eight patterns (blue) were flown over Chilbolton when all the radars were pointing at zenith. The aircraft flew along a specific flight path, known as the Chilbolton radial (orange), which is set at an angle of 246 or 270°. Figure created by Stuart Fox.</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f01.png"/>

      </fig>

      <p id="d2e597">CCREST-M took place between the 6 February and 25 March 2024. Twelve science flights were conducted, three of which – C374 (28 February), C379 (19 March), and C382 (25 March) – included in-situ sampling of the bulk and microphysical properties of the cloud. The duration of each science flight was approximately 4 <inline-formula><mml:math id="M41" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> and each followed a common flight pattern designed to link the ground-based radars and the radiometers in a repeatable way. Figure 1 shows a typical flight pattern; these consisted of straight and level runs along a radial (270 or 246°) to and from the Chilbolton-based radars, followed by figure-of-eight patterns centred on the Chilbolton Observatory. The decision on which radial to fly along was made in real time as the aircraft approached the Chilbolton area, in coordination with the radar operator.  Range Height-Indicator (RHI) scans from mainly the 3 <inline-formula><mml:math id="M42" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> CAMRa radar were used to identify the azimuth containing the deepest and most strongly reflecting ice cloud to ensure a good radiometric signal, and this information was augmented by 15 <inline-formula><mml:math id="M43" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> 10 <inline-formula><mml:math id="M44" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> geostationary satellite imagery. During the radial legs the ground-based radars operated in RHI scanning mode, providing vertical profiles of cloud structure along the aircraft's flight path for radiometer sampling. During the figure-of-eight patterns the aircraft repeatedly flew over the Observatory while the radars were zenith pointing, yielding time–height reflectivity profiles directly beneath the aircraft, while the radiometers sampled the cloud in nadir pointing mode. During the high-level radiometric runs there were dropsonde releases from the aircraft above the cloud to obtain pressure and temperature profiles for use in the retrieval of the PSDs.</p>
      <p id="d2e634">After the high-level radiometric overpasses and figure-of-eight loiter, the aircraft descended into the cloud for in-situ microphysics and bulk IWC sampling. For C379 and C382 this took the form of stepped descents with straight-and-level runs of several minutes at successive levels, whereas for C374 the aircraft performed a continuous profiling descent through the depth of the cloud. In all three cases, these in-situ legs act as an independent validation data set for the retrieved PSDs, although they are not strictly co-located with the ground-based radar observations.</p>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>Aircraft instrumentation, data summary, in-situ cases and ice crystal habit descriptions</title>
      <p id="d2e644">The instrumentation on board the FAAM aircraft that is utilised in this paper is summarised below in Table 1. All the aircraft FAAM data listed in Table 1 is available on the Centre for Environmental Data Analysis (CEDA) website given here: <uri>https://www.ceda.ac.uk/</uri> (last access: 26 June 2026). For a description of the microphysics and bulk probes shown in Table 1, the CIP-15, CIP-100 and the Nevzorov probe see McFarquhar et al. (2017) and Cotton et al.  (2013), respectively. For each flight, the in-situ measurements are composited from the CIP-15 and CIP-100 instruments following Cotton et al.  (2013), yielding size distributions from approximately 15 <inline-formula><mml:math id="M45" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> to 6.4 <inline-formula><mml:math id="M46" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">mm</mml:mi></mml:mrow></mml:math></inline-formula>.  The microphysics data processing done here is not different to that applied to the PICASSO campaign. However, here ice crystals smaller than 100 <inline-formula><mml:math id="M47" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> were omitted since they contribute negligibly to radar reflectivity and brightness temperature depressions at mm-wave and sub-mm-wave frequencies as shown by McCusker et al. (2024). Some PSDs were excluded if the Nevzorov probe measured IWCs below 0.002 <inline-formula><mml:math id="M48" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">gm</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, which is the estimated sensitivity of the Nevzorov probe as determined by Abel et al. (2014). Probe shattering effects were minimised through modified inlet arms of the CIP probes and inter-arrival time filtering when compositing the PSDs.</p>

<table-wrap id="T1"><label>Table 1</label><caption><p id="d2e695">A summary of instrumentation on board the FAAM aircraft during the CCREST-M flights.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="2">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Instrument</oasis:entry>
         <oasis:entry colname="col2">Measurement</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">CIP-15</oasis:entry>
         <oasis:entry colname="col2">PSD 15–960 <inline-formula><mml:math id="M49" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CIP-100</oasis:entry>
         <oasis:entry colname="col2">PSD 100 <inline-formula><mml:math id="M50" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>–6.4 <inline-formula><mml:math id="M51" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">mm</mml:mi></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Nevzorov probe</oasis:entry>
         <oasis:entry colname="col2">Bulk ice liquid and water</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Dropsondes–profiles</oasis:entry>
         <oasis:entry colname="col2">Temperature and pressure</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d2e784">In this paper, the roles of the aircraft measurements are as follows. The composite in-situ PSDs are used as a validation dataset for the PSDs retrieved from the multi-frequency radars. The Nevzorov probe provides bulk IWC, which we compare directly to the IWCs derived from the retrieved PSDs.  The dropsonde profiles provide temperature and pressure, which are both used as inputs to the machine-learning first-guess, together with the 3 <inline-formula><mml:math id="M52" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>-retrieved IWC and mean mass-weighted dimension. Typically, two to four dropsondes were released from the aircraft above the cloud tops during each case, while the aircraft flew along one of the Chilbolton radials.</p>
<sec id="Ch1.S2.SS1.SSS1">
  <label>2.1.1</label><title>A data summary of the radar and atmospheric data</title>
      <p id="d2e803">The processing of the radar data used here was done by the Chilbolton Observatory staff for the CAMRa and Kepler radar data. The CAMRa and Kepler radar data used in this paper are also available on the CEDA website referenced above. The mini-BASTA and 200 <inline-formula><mml:math id="M53" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> GRaCE radar data were processed by the Laboratoire Atmosphère, Milieux, Observations, Spatiales (LATMOS) and the University of Reading, respectively. During the CCREST-M campaign, the radar measurements coincided with near-direct FAAM aircraft overpasses.  The CAMRa, Kepler and mini-BASTA radars were operated in either zenith mode or Range-Height Indicator (RHI) scan mode during the aircraft overpass. The core overpass dataset was constructed from figure-of-eight aircraft flight patterns, with the radars pointing vertically, and extended datasets which includes the RHI scans. In this paper, we consider only the zenith-pointing radar data.</p>
      <p id="d2e814">The data from the three main radars (CAMRa, Kepler and mini-BASTA) were interpolated to a common 25 <inline-formula><mml:math id="M54" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid extending to an altitude of 13 <inline-formula><mml:math id="M55" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, matching the resolution of the Kepler radar. Reflectivity, Doppler velocity, and spectral width were extracted from each radar system, with signal quality control based on native instrument masks and angular thresholds (e.g. within 0.1° for Kepler, 0.4° for mini-BASTA) to exclude off-zenith and edge-of-beam artefacts. To characterise the radar reflectivity statistics for each of the case studies, the mean, median and the standard deviation were computed within a 40 s window (<inline-formula><mml:math id="M56" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M57" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula>) centred on the aircraft nadir time for each of the radar frequencies. In the context of this study, these processed time–height fields provide the reflectivity profiles from which we retrieve the PSDs at the times of the aircraft radiometric overpasses for forthcoming radiative transfer studies that will be presented in a later paper. The 40 <inline-formula><mml:math id="M58" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> window is a pragmatic choice that balances the need for enough radar samples to obtain robust statistics and to accommodate small timing differences between aircraft and radar data. In a few instances where no valid radar profiles were available during the 40 <inline-formula><mml:math id="M59" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> window, we instead use the nearest available profiles in time, selected by visual inspection to ensure that the reflectivity structure was sufficiently similar to that during the overpass, and we only retained profiles with valid in-cloud returns.</p>
      <p id="d2e868">Atmospheric temperature, pressure, humidity, and ozone profiles were provided using a combination of Vaisala RD41 dropsondes (for altitudes below aircraft level) and a mid-latitude winter climatology (for levels above the aircraft and ozone). Temperature and pressure were linearly interpolated onto the radar grid, and relative humidity was computed with respect to liquid or ice depending on the ambient temperature.</p>
      <p id="d2e871">To account for liquid water cloud attenuation, cloud liquid water path (LWP) was retrieved from the Chilbolton HATPRO microwave radiometer (Walden, 2026a), with missing data interpolated over short time gaps. The HATPRO LWP provides a column integrated value and does not constrain the vertical distribution of liquid water. We therefore assume the liquid cloud to be a single layer, with a representative in-cloud temperature taken from the interpolated atmospheric profile, where the cloud top height was manually defined using the ceilometer (Walden, 2026b), lidar, and radar backscatter profiles. The specific liquid water absorption at each radar frequency was computed from the Ellison (2007) absorption model at this representative temperature and multiplied by the HATPRO LWP to give the one-way attenuation. Two-way attenuation by ice crystals at 35 and 94 <inline-formula><mml:math id="M60" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> is not accounted for in this paper. It was previously found by McCusker et al.  (2024) that for similar frontal iced-cloud conditions the two-way path integrated ice attenuation at these frequencies to be well below 1 <inline-formula><mml:math id="M61" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. This is consistent with the recent multi-campaign comparison by Li et al. (2026), who reported a median W-band path-integrated snow attenuation of 0.3 <inline-formula><mml:math id="M62" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dB</mml:mi></mml:mrow></mml:math></inline-formula> and a sub-dB spread between parametrisations. Therefore, ice attenuation is not corrected for explicitly in this paper. To account for gaseous attenuation by oxygen and water vapour on the radar reflectivities at 35 and 94 <inline-formula><mml:math id="M63" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, we computed the two-way partial-column gaseous attenuation from near-surface to each in-cloud retrieval gate using the aircraft dropsonde-derived profiles of temperature, pressure and water vapour volume mixing ratio released near the Chilbolton Observatory. A simplified gas absorption parametrisation was used, consisting of pressure-scaled oxygen absorption and humidity-scaled water vapour absorption, with coefficients providing representative specific attenuation values of 0.02, and 0.1 <inline-formula><mml:math id="M64" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dB</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">km</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> for oxygen, and 0.01, and 0.08 <inline-formula><mml:math id="M65" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dB</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">km</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> for water vapour at 35 and 94 <inline-formula><mml:math id="M66" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, respectively, under standard atmospheric conditions as recommended by ITU-R P676.13 (2022). The mean partial-column two-way attenuation at 94 <inline-formula><mml:math id="M67" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> reaches approximately 1.5 dB at 94 <inline-formula><mml:math id="M68" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> for C374, this is consistent with Hogan et al. (2000), who using co-located 35 and 94 <inline-formula><mml:math id="M69" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radars at Chilbolton Observatory reported a two-way gaseous attenuation at 94 <inline-formula><mml:math id="M70" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> of approximately 2 dB from near-surface to 10 <inline-formula><mml:math id="M71" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>. At 3 <inline-formula><mml:math id="M72" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, gaseous attenuation is negligible (specific attenuation values of order 0.001 <inline-formula><mml:math id="M73" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dB</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">km</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> for oxygen and zero for water vapour) and is not considered further.</p>
      <p id="d2e1016">This dataset enables the construction of well-collocated multi-frequency radar reflectivity profiles, corrected for atmospheric and liquid water attenuation, with matched atmospheric profiles needed for the retrievals and radiative transfer. Here, we utilise only the mean radar reflectivity radar profiles.</p>

      <fig id="F2" specific-use="star"><label>Figure 2</label><caption><p id="d2e1021">Time–height cross-sections of 35 <inline-formula><mml:math id="M74" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> Kepler radar reflectivity for the three CCREST-M cases: C374 (28 February 2024, top panel), C379 (19 March 2024, middle panel), and C382 (25 March 2024, bottom panel).  Colours show the radar reflectivity (dBZ) at the native time–height resolution of the complete (i.e., RHI and Zenith-pointing data) processed Kepler dataset, with white areas indicating the absence of cloud or values below the noise threshold. The time periods used for the aircraft radial legs, figure-of-eight manoeuvres, and in-situ sampling are indicated at the top of each panel. The 35 <inline-formula><mml:math id="M75" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar is shown here as it provides a good compromise between sensitivity to ice crystals and susceptibility to attenuation. The colour bar on the right-hand side provides the radar reflectivity scale.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f02.png"/>

          </fig>

</sec>
<sec id="Ch1.S2.SS1.SSS2">
  <label>2.1.2</label><title>Case summaries and predominant ice crystal habits</title>
      <p id="d2e1054">The synoptic environments of the three flights were typical of winter mid-latitude frontal systems over the UK, with non-precipitating cloud during the science flying for C374 and weakly precipitating ice clouds during the science flying for C379 and C382. Figure 2 summarises the temporal and vertical structure of the three CCREST-M cases using time–height plots of 35 <inline-formula><mml:math id="M76" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> Kepler radar reflectivity. For C374 (Fig. 2, top panel), a deep frontal ice cloud is observed, with radar reflectivities ranging from approximately <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M78" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">25</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M79" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula> between about 3 to 9 <inline-formula><mml:math id="M80" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> for over two hours. Above about 9 <inline-formula><mml:math id="M81" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, the radar detects weaker and more intermittent returns, consistent with sparse upper-level ice cloud. Scientific flying for this case concluded at around 11:45 UTC as significant precipitation began.  For C379 (Fig. 2, middle panel), the primary ice layer is located between about 5 and 9 <inline-formula><mml:math id="M82" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>. Below about 2 <inline-formula><mml:math id="M83" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, stronger and more variable reflectivities indicate the presence of an underlying liquid water cloud, which occasionally produced light precipitation of around 1 <inline-formula><mml:math id="M84" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">mm</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">h</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> at the surface, as recorded by the Observatory rain gauges. The C382 (Fig. 2, bottom panel) case exhibits a somewhat generally thinner main ice layer than in the other cases, extending from roughly 5 to 8 <inline-formula><mml:math id="M85" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>. A shallow cirrus layer is present just below approximately 9 <inline-formula><mml:math id="M86" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, with a thickness of less than 1 <inline-formula><mml:math id="M87" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, and occasional low level-level liquid water cloud is also detected by the Kepler radar. For the cases C374 and C382, the liquid water paths were typically below 0.2 <inline-formula><mml:math id="M88" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. Overall, these time–height cross-sections confirm that all three cases correspond to mid-latitude frontal ice cloud with relatively persistent vertical structure, making them well suited for the radiometric overpasses and radar-based PSD retrievals.</p>

      <fig id="F3" specific-use="star"><label>Figure 3</label><caption><p id="d2e1187">Representative CIP-15 imagery obtained during three distinct altitude levels. In each panel, the top three rectangular strips correspond to cloud top, followed by the next three representing the cloud mid-level, and the bottom three rectangular strips represent the cloud base during descent through the ice layer for cases <bold>(a)</bold> C374, <bold>(b)</bold> C379, and <bold>(c)</bold> C382. Each rectangular strip spans 64 pixels across the CIP-15 array, corresponding to a physical width of 960 <inline-formula><mml:math id="M89" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> at 15 <inline-formula><mml:math id="M90" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> per pixel.  The length of each strip is variable.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f03.png"/>

          </fig>

      <p id="d2e1225">The most detailed analysis of C374 has already been reported by McCusker et al. (2025), who also provide a detailed description of the observed ice crystal habits for that case. Consistent with that study, examination of CIP-15 imagery from all three flights shows rosettes and aggregates of rosettes as the dominant particle types, with occasional columns, plates, and aggregates of columns. Typical examples of the CIP-15 imagery from the three cases are presented in Fig. 3a–c, where the image files were manually examined to identify the predominant ice crystal shapes across different altitudes, and the imagery is taken from the mid-point of each profile. Across all the three cases, a similar vertical evolution of ice crystal habit was observed as shown in the figure. That is, near cloud top the habits consisted of small, pristine rosettes and some columns. At mid-level in the cloud, larger more complex rosette aggregates were observed and at near cloud base, extensive irregular rosette aggregates and occasional columns and column aggregates were observed.</p>
      <p id="d2e1229">Although the three ice cloud cases differ in altitude and temperature, their microphysical ice crystal shape characteristics were broadly consistent, making them ideal cases for testing the retrieval methodology under comparable mid-latitude conditions. The same rosette-aggregate habits observed here underpin the scattering assumptions described in Sect. 3.</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>The ice crystal scattering model and forward radar reflectivity model</title>
      <p id="d2e1242">The scattering properties assumed in this study are based on the randomly oriented rosette-aggregate model described in detail by Kleanthous et al.  (2024). The model represents an ensemble of rosette aggregates generated using the aggregation model of Westbrook et al. (2004) and constrained to follow the Cotton et al. (2013) mass–dimension relationship, given by <inline-formula><mml:math id="M91" display="inline"><mml:mrow><mml:mtext>mass</mml:mtext><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.0257</mml:mn><mml:msubsup><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M92" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the maximum dimension of the ice crystal expressed in SI units, consistent with the Met Office two-moment microphysics scheme, see for details Field et al. (2023). The aggregates are constructed from solid three-branched rosette monomers and are assumed to be randomly oriented in 3-D space.</p>
      <p id="d2e1275">The ensemble comprises of 65 rosette-aggregate realisations spanning maximum dimensions between 10 <inline-formula><mml:math id="M93" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> and approximately 1 <inline-formula><mml:math id="M94" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">cm</mml:mi></mml:mrow></mml:math></inline-formula>, representative of the dominant habits observed during CCREST-M, as previously discussed in Sect. 2.1.2, and consistent with the findings reported by Lawson et al. (2019) and Wagner et al. (2025) in the case of in-situ generated cirrus, typical of the mid-latitudes. Full details of the model generation, morphology, and mass– and area–dimension power laws are described by Kleanthous et al. (2024). Although referred to as the rosette-aggregate model, this representation does not correspond to a single ice type. As detailed in Kleanthous et al. (2024), the aggregates are composed of rosettes but evolve into different structural forms as they grow, with morphology varying systematically when mass scales with the square of their maximum dimension. For each of the rosette-aggregates, the backscattering cross section, <inline-formula><mml:math id="M95" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, is computed using the electromagnetic boundary element method (BEM) described by Kleanthous et al.  (2022). The rosette-aggregate scattering model has been shown by Baran et al. (2024) to reproduce triple-frequency radar reflectivity measurements at 9, 35 and 94 <inline-formula><mml:math id="M96" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> to within a few <inline-formula><mml:math id="M97" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula> for various mid-latitude and mixed-phase cloud systems that were observed off the north-east coast of the United States during the IMPACTS campaign. Therefore, the rosette-aggregate model is utilised in this paper as the representative ice crystal habit for the retrievals.</p>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>The forward radar reflectivity model</title>
      <p id="d2e1339">From the BEM calculations, solutions found for <inline-formula><mml:math id="M98" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are used to forward model the equivalent radar reflectivity factor, <inline-formula><mml:math id="M99" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, where the units of <inline-formula><mml:math id="M100" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are <inline-formula><mml:math id="M101" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">mm</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msup><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and are transformed into units of <inline-formula><mml:math id="M102" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula> via <inline-formula><mml:math id="M103" display="inline"><mml:mrow><mml:mn mathvariant="normal">10</mml:mn><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>Z</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M104" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Atlas et al., 1995; Hong et al., 2008; Baran et al., 2011, and references therein) is calculated following Eq. (<xref ref-type="disp-formula" rid="Ch1.E1"/>):

            <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M105" display="block"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">18</mml:mn></mml:msup><mml:mi>C</mml:mi><mml:msubsup><mml:mo>∫</mml:mo><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>min</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>max</mml:mtext></mml:msub></mml:mrow></mml:msubsup><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mi>n</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></disp-formula>

          The measured reflectivities from CAMRa, Kepler, mini-BASTA and GRaCE are provided as equivalent radar reflectivity factor <inline-formula><mml:math id="M106" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in <inline-formula><mml:math id="M107" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. These values are computed using the standard definition of water-equivalent reflectivity, i.e., assuming scattering from water spheres and using the same definition as Eq. (<xref ref-type="disp-formula" rid="Ch1.E1"/>). For our forward model, we adopt the same convention, with <inline-formula><mml:math id="M108" display="inline"><mml:mrow><mml:mi>C</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msup><mml:mi mathvariant="italic">λ</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:mo>|</mml:mo><mml:mi>K</mml:mi><mml:msup><mml:mo>|</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:msup><mml:mi mathvariant="italic">π</mml:mi><mml:mn mathvariant="normal">5</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M109" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> is the incident wavelength in <inline-formula><mml:math id="M110" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M111" display="inline"><mml:mrow><mml:mo>|</mml:mo><mml:mi>K</mml:mi><mml:msup><mml:mo>|</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> is the dielectric factor of liquid water. This dielectric factor is both frequency and temperature dependent as discussed by Hogan et al.  (2006) and in that paper <inline-formula><mml:math id="M112" display="inline"><mml:mrow><mml:mo>|</mml:mo><mml:mi>K</mml:mi><mml:msup><mml:mo>|</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> at <inline-formula><mml:math id="M113" display="inline"><mml:mrow><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">270</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M114" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:math></inline-formula> for 35 and 94 <inline-formula><mml:math id="M115" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> is 0.88 and 0.67, respectively. At 3 <inline-formula><mml:math id="M116" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, we use the value of 0.93, and at 200 <inline-formula><mml:math id="M117" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> we use the value used by McCusker et al. (2025) to be consistent with that paper, which was also 0.93. For the cases described by Baran et al. (2024), it was shown that the equivalent radar reflectivity factor has only a weak dependence on temperature and differences in radar reflectivity between the different temperatures was found to be <inline-formula><mml:math id="M118" display="inline"><mml:mrow><mml:mo>≪</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M119" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. The other terms used in Eq. (<xref ref-type="disp-formula" rid="Ch1.E1"/>) are the backscattering cross section, <inline-formula><mml:math id="M120" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, in units of <inline-formula><mml:math id="M121" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M122" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, the assumed PSD in units of <inline-formula><mml:math id="M123" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>. The complex refractive indices of ice for 3, 35, 94 and 200 <inline-formula><mml:math id="M124" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, assuming a temperature of 270 <inline-formula><mml:math id="M125" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:math></inline-formula>, have been determined from the tabulation due to Mätzler (2006). This set of refractive indices for ice has been previously recommended by Eriksson et al. (2018). In Eq. (<xref ref-type="disp-formula" rid="Ch1.E1"/>), the factor <inline-formula><mml:math id="M126" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">18</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> is required to convert the units of the integrand into the units of <inline-formula><mml:math id="M127" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. We next consider the PSD assumptions for <inline-formula><mml:math id="M128" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, the ML approach and retrieval methodology.</p>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>The PSD assumptions, machine learning approach, and retrieval methodology</title>
      <p id="d2e1797">In radar studies, the PSD models used to represent snow crystals or ice aggregates are most commonly gamma or exponential size distributions, see for instance the studies by Heymsfield et al. (2023), and Kozu and Nakamura (1991). The well-known gamma size distributions are calculated following Eq. (<xref ref-type="disp-formula" rid="Ch1.E2"/>):

          <disp-formula id="Ch1.E2" content-type="numbered"><label>2</label><mml:math id="M129" display="block"><mml:mrow><mml:mi>n</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:msubsup><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi><mml:mi mathvariant="italic">μ</mml:mi></mml:msubsup><mml:msup><mml:mi mathvariant="normal">e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:msup></mml:mrow></mml:math></disp-formula>

        where <inline-formula><mml:math id="M130" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M131" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M132" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> represent the intercept parameter, the slope, and the shape parameter of the size distribution, respectively. The units of <inline-formula><mml:math id="M133" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M134" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> are <inline-formula><mml:math id="M135" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M136" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, respectively. In Eq. (<xref ref-type="disp-formula" rid="Ch1.E2"/>), the exponential PSD is represented when <inline-formula><mml:math id="M137" display="inline"><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>. The PSD parameters <inline-formula><mml:math id="M138" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M139" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M140" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> can be estimated from the moments of the PSD, where the <inline-formula><mml:math id="M141" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula>th moment of the PSD, <inline-formula><mml:math id="M142" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, is calculated following Eq. (<xref ref-type="disp-formula" rid="Ch1.E3"/>):

          <disp-formula id="Ch1.E3" content-type="numbered"><label>3</label><mml:math id="M143" display="block"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msubsup><mml:mo>∫</mml:mo><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>min</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>max</mml:mtext></mml:msub></mml:mrow></mml:msubsup><mml:mi>N</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:msubsup><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi><mml:mi>n</mml:mi></mml:msubsup><mml:mi mathvariant="normal">d</mml:mi><mml:mi>D</mml:mi></mml:mrow></mml:math></disp-formula>

        It follows from Kozu and Nakamura (1991) that <inline-formula><mml:math id="M144" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M145" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M146" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> can be estimated from the PSD moments following Eqs. (4)–(6):

          <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M147" display="block"><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">11</mml:mn><mml:mi>F</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">8</mml:mn><mml:mo>+</mml:mo><mml:mo>√</mml:mo><mml:mi>F</mml:mi><mml:mo>(</mml:mo><mml:mi>F</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">8</mml:mn><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>F</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></disp-formula>

        where <inline-formula><mml:math id="M148" display="inline"><mml:mrow><mml:mi>F</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msubsup><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn><mml:mn mathvariant="normal">3</mml:mn></mml:msubsup></mml:mrow><mml:mrow><mml:msubsup><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></inline-formula>, and

          <disp-formula id="Ch1.E5" content-type="numbered"><label>5</label><mml:math id="M149" display="block"><mml:mrow><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">4</mml:mn><mml:mo>)</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

        and <inline-formula><mml:math id="M150" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is given by:

          <disp-formula id="Ch1.E6" content-type="numbered"><label>6</label><mml:math id="M151" display="block"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mfenced open="(" close=")"><mml:mrow><mml:msup><mml:mi mathvariant="italic">λ</mml:mi><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mfenced><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">4</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

        where <inline-formula><mml:math id="M152" display="inline"><mml:mi mathvariant="normal">Γ</mml:mi></mml:math></inline-formula> is the gamma function.</p>
      <p id="d2e2243">Another useful microphysical parameter to derive is the mean mass-weighted diameter (<inline-formula><mml:math id="M153" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>) given by the ratio of <inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> on the assumption that mass is proportional to the maximum dimension of the ice crystal raised to the power of two. Here, we consider ice aggregation at radar frequencies assuming the Cotton et al. (2013) mass–dimension power law and this relationship is consistent with our definition of <inline-formula><mml:math id="M155" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. From the PICASSO campaign that took place over the Chilbolton Observatory, from those measured PSDs, all three of the model PSD parameters can be estimated from Eqs. (4)–(6), and from these the PSDs can be generated from Eq. (<xref ref-type="disp-formula" rid="Ch1.E2"/>).  Therefore, here, we require to retrieve <inline-formula><mml:math id="M156" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M157" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M158" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> from the multi-frequency radar reflectivities measured during CCREST-M. Note also, that <inline-formula><mml:math id="M159" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula> from above is determined from <inline-formula><mml:math id="M160" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M161" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M162" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> for the assumption of ice aggregation is more related to the radar reflectivity since in this case the radar backscatter is proportional to the square of the mass and <inline-formula><mml:math id="M164" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> further enhances the contribution of larger particles that dominate the radar signal. This is the reason as to why we adopt the definitions of Kozu and Nakamura (1991) in this paper to retrieve the PSDs.</p>
      <p id="d2e2377">Here, we make use of the in-situ measured PSDs from the PICASSO campaign, which was also conducted over the Chilbolton Observatory, where data were collected from ten flights that we utilise in this paper. The approach adopted here is based on the meteorological principle that mid-latitude cirrus clouds observed over the same geographical location should exhibit similar microphysical characteristics when sampled across similar time periods, assuming no significant climate shifts. By constructing a moment climatology from the PICASSO dataset, we can establish a baseline of cloud properties specific to the Chilbolton region. This climatology should reasonably represent the cloud structures encountered during the CCREST-M period of flying, as both campaigns targeted similar cloud systems in the same geographical location under comparable synoptic conditions during a similar period. Therefore, the moment climatology derived from PICASSO should provide valid prior information for CCREST-M retrievals within the sampled temperature range of the PICASSO campaign.</p>
      <p id="d2e2380">To construct the moment climatology, we utilise nine PICASSO flights, which are C076, C082, C098, C155, C169, C170, C171, C172, and C174, available from the CEDA website. We use these flights to obtain the profile of moments <inline-formula><mml:math id="M165" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M167" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M168" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, – that is, the variation of these quantities as a function of altitude – as well as profiles of in-cloud temperature, <inline-formula><mml:math id="M169" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, pressure, <inline-formula><mml:math id="M170" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>, and bulk IWC from the Nevzorov probe.  Data from flight C081 is kept as the “unseen” data to evaluate our ML models, as this flight is broadly representative of the others in terms of temperature and IWC ranges. The ML regression-based approach adopted in this study is described in the following sub-section.</p>
<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>The ensemble of machine learning models and results</title>
      <p id="d2e2454">The ensemble of ML models we utilise are from Python's scikit-learn (Pedregosa et al., 2011), this ensemble approach is used to predict the moments of the PSD that will serve as first-guess inputs for the physical retrieval of IWC and the previously described PSD parameters. In this ML model, the feature vector, <inline-formula><mml:math id="M171" display="inline"><mml:mi mathvariant="bold-italic">x</mml:mi></mml:math></inline-formula>, consists of: <list list-type="custom"><list-item><label>(i)</label>
      <p id="d2e2466"><inline-formula><mml:math id="M172" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M173" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is in units of <inline-formula><mml:math id="M174" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>,</p></list-item><list-item><label>(ii)</label>
      <p id="d2e2510"><inline-formula><mml:math id="M175" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>(IWC), where IWC is in units of <inline-formula><mml:math id="M176" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>,</p></list-item><list-item><label>(iii)</label>
      <p id="d2e2541"><inline-formula><mml:math id="M177" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:mi>p</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M178" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> is in units of <inline-formula><mml:math id="M179" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">hPa</mml:mi></mml:mrow></mml:math></inline-formula>, and to be consistent with all other feature spaces,</p></list-item><list-item><label>(iv)</label>
      <p id="d2e2576"><inline-formula><mml:math id="M180" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M181" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is in units of Kelvin.</p></list-item></list></p>
      <p id="d2e2609">For each moment <inline-formula><mml:math id="M182" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> where <inline-formula><mml:math id="M183" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>∈</mml:mo><mml:mo mathvariant="italic">{</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">4</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">6</mml:mn><mml:mo mathvariant="italic">}</mml:mo></mml:mrow></mml:math></inline-formula>, we train a separate ML model, f<sub>n</sub>, such that:

            <disp-formula id="Ch1.E7" content-type="numbered"><label>7</label><mml:math id="M185" display="block"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>f</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi mathvariant="bold-italic">x</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mi>f</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mtext>, IWC,</mml:mtext><mml:mi>p</mml:mi><mml:mo>,</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:math></disp-formula>

          where in Eq. (<xref ref-type="disp-formula" rid="Ch1.E7"/>) the <inline-formula><mml:math id="M186" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> symbol has been dropped for reasons of clarity.</p>
      <p id="d2e2732">For training the ML models we use the PICASSO climatology described above using the nine flights. From these flights we diagnose vertical profiles of the PSD moments <inline-formula><mml:math id="M187" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M188" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M189" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M190" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M191" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M192" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>, bulk IWC from the Nevzorov probe, and <inline-formula><mml:math id="M193" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> as defined above. However, in the CCREST-M application, <inline-formula><mml:math id="M194" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is not directly observed and is instead estimated from the empirical <inline-formula><mml:math id="M195" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> relationship derived from the PICASSO dataset (see Sect. 4.2), so that the same set of predictors can be used. From the feature space given by Eq. (<xref ref-type="disp-formula" rid="Ch1.E7"/>), the targets of the ML models are the logarithms of the PSD moments, <inline-formula><mml:math id="M196" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> for <inline-formula><mml:math id="M197" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:math></inline-formula>, and 6. Although <inline-formula><mml:math id="M198" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is strongly correlated with <inline-formula><mml:math id="M199" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in the PICASSO climatology, it is not a deterministic function of <inline-formula><mml:math id="M200" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, since for a given <inline-formula><mml:math id="M201" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> there can be considerable variation in <inline-formula><mml:math id="M202" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. Including both <inline-formula><mml:math id="M203" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M204" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in vector <inline-formula><mml:math id="M205" display="inline"><mml:mi mathvariant="bold-italic">x</mml:mi></mml:math></inline-formula> provides the ML models with complementary information representing the thermodynamics through <inline-formula><mml:math id="M206" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M207" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> and the cloud physics through IWC and <inline-formula><mml:math id="M208" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>. For each target moment <inline-formula><mml:math id="M209" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, we train a separate regression model <inline-formula><mml:math id="M210" display="inline"><mml:mrow><mml:msub><mml:mi>f</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi mathvariant="bold-italic">x</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> using an ensemble of ML models using the default hyperparameter settings to maintain simplicity and reproducibility. The ML models in the ensemble are the random forest regressor, gradient boosting regressor, and support vector regression. For the random forest regressor the “shuffle” parameter is set to “false” as the dataset is a time series and by setting this parameter to “false” we ensure that data from the prediction dataset were not randomly selected to be a part of the training dataset. Therefore, in the presentation of results that follow, the prediction dataset in unseen in the training dataset. The resulting predictions from each of the ML models are simply arithmetically averaged to find the prediction of the ensemble. This approach allows us to predict <inline-formula><mml:math id="M211" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> given <inline-formula><mml:math id="M212" display="inline"><mml:mrow><mml:mi>f</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="bold-italic">x</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, required for the retrieval algorithm.</p>
      <p id="d2e3069">We first evaluate the ensemble approach using a standard <inline-formula><mml:math id="M213" display="inline"><mml:mrow><mml:mn mathvariant="normal">80</mml:mn><mml:mo>:</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> split of the PICASSO climatology dataset, where 80 % of the data are used for the training data, and the remaining 20 % are used for the validation dataset.  The ensemble predictions for each target moment <inline-formula><mml:math id="M214" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> are compared with the actual values in Fig. 4a–d. The hexagonally binned scatter plots show that the ensemble ML predictions cluster tightly about the <inline-formula><mml:math id="M215" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>:</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> line for all the four moments, which indicates excellent agreement between predicted and true values across the full range of values. The mean-squared errors found for <inline-formula><mml:math id="M216" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M217" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M218" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M219" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> are 0.016, 0.0006, 0.003, and 0.006, respectively, demonstrating that the ensemble of ML models reproduces the logarithmic moments of the PSD with high accuracy. For comparison, using the default random forest model alone resulted in substantially larger mean-squared errors for <inline-formula><mml:math id="M220" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M221" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M222" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M223" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> which were found to be 0.1, 0.103, 0.12, and 0.191, respectively. Clearly, from these results, the ensemble ML model is better to use for the prediction of the required moments than a single ML model. The full results of comparisons are not shown here for reasons of brevity.</p>

      <fig id="F4" specific-use="star"><label>Figure 4</label><caption><p id="d2e3280">Hexagonally binned scatter plots of predicted versus true <inline-formula><mml:math id="M224" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mi>n</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> from the ensemble of ML models for the PICASSO validation subset for <bold>(a)</bold> <inline-formula><mml:math id="M225" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M226" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M227" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:math></inline-formula>, and <bold>(d)</bold> <inline-formula><mml:math id="M228" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:math></inline-formula>. The colour scale shows the logarithm to the base 10 of the number of points in each of the hexagonal bins and the dashed line in each of the panels indicates the <inline-formula><mml:math id="M229" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>:</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> line.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f04.png"/>

        </fig>

      <p id="d2e3382">Given the results for testing and prediction, the moment predictions for the unseen data from the PICASSO case C081 using the ensemble ML model are presented in Fig. 5a–d. Here, rather than presenting statistical representations of how well the predicted moments match the actual moments for C081, we present the moment comparisons in physical space. The figure demonstrates that the predicted re-transformed moments back to physical space compare generally very well with the variability of the actual moments from C081 as a function of temperature. The results depicted in Fig. 5a–d do indeed suggest that ML can be applied to predict the moments of unseen data, and as such ML can provide a good first guess profile for the PSD parameters in a physical retrieval of the microphysics using observed radar reflectivities.</p>

      <fig id="F5" specific-use="star"><label>Figure 5</label><caption><p id="d2e3387">Comparison of the re-transformed observed (open red circles) moments from C081 and predicted moments (open blue circles) using the ensemble-averaged ML predictions plotted against the in-cloud temperature for <bold>(a)</bold> <inline-formula><mml:math id="M230" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M231" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M232" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <bold>(d)</bold> <inline-formula><mml:math id="M233" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The key to each of the panels is shown in the bottom-left corner of panel <bold>(a)</bold>.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f05.png"/>

        </fig>

      <p id="d2e3456">When applying the trained models to the CCREST-M cases, the same feature vector <inline-formula><mml:math id="M234" display="inline"><mml:mi mathvariant="bold-italic">x</mml:mi></mml:math></inline-formula> is constructed using profiles of <inline-formula><mml:math id="M235" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M236" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> from the dropsondes, together with profiles of IWC and <inline-formula><mml:math id="M237" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> derived from the 3 <inline-formula><mml:math id="M238" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivity and a separate temperature-based polynomial model, respectively. The prediction of <inline-formula><mml:math id="M239" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> from <inline-formula><mml:math id="M240" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is next described in Sect. 4.2 and the retrieval methodology in physical space is described in the Sect. 4.3. In Sect. 4.4, the retrieval of IWC from the 3 <inline-formula><mml:math id="M241" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar is then described. A schematic overview of the full retrieval framework, from PICASSO training to the CCREST-M multi-frequency radar retrieval, is depicted in Fig. 6.</p>

      <fig id="F6" specific-use="star"><label>Figure 6</label><caption><p id="d2e3536">A schematic overview of the retrieval framework.  Step 1: an ensemble ML model is trained on the PICASSO dataset using in-situ PSDs and the Nevzorov IWC to compute the PSD moments <inline-formula><mml:math id="M242" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M243" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M244" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M245" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and the mean mass-weighted diameter <inline-formula><mml:math id="M246" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. Step 2: for each CCREST-M case, profiles of <inline-formula><mml:math id="M247" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M248" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>, 3 <inline-formula><mml:math id="M249" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>-retrieved IWC and <inline-formula><mml:math id="M250" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> are passed through the ML ensemble to predict the moments, which are converted into first-guess gamma PSD parameters, with <inline-formula><mml:math id="M251" display="inline"><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mtext>first guess</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M252" display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> is the altitude, and corresponding <inline-formula><mml:math id="M253" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">λ</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:msup><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M254" display="inline"><mml:mrow><mml:msubsup><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:msubsup><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>. Step 3: a physics-based multi-frequency radar retrieval adjusts <inline-formula><mml:math id="M255" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M256" display="inline"><mml:mrow><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> using the same <inline-formula><mml:math id="M257" display="inline"><mml:mrow><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:mi>D</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and scattering model so that simulated reflectivities <inline-formula><mml:math id="M258" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mn mathvariant="normal">35</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M259" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mn mathvariant="normal">94</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> match the observations, yielding retrieved PSD parameters, PSDs and estimated IWCs, and forward-modelled reflectivities.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f06.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Estimating the profile of <inline-formula><mml:math id="M260" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d2e3841">To obtain a first-guess profile of <inline-formula><mml:math id="M261" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> we exploit the observed relationship between <inline-formula><mml:math id="M262" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and the in-cloud temperature <inline-formula><mml:math id="M263" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in the PICASSO dataset, where <inline-formula><mml:math id="M264" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. Since we use <inline-formula><mml:math id="M265" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> to be the only predicator for <inline-formula><mml:math id="M266" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, the underlying relationship is expected to be a smooth function of temperature rather than a highly structured one. Therefore, a low-order polynomial is fitted to the PICASSO <inline-formula><mml:math id="M267" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> dataset. Polynomials from degree 1 to degree 10 were tested and each fit was evaluated using the coefficient of determination, <inline-formula><mml:math id="M268" display="inline"><mml:mrow><mml:msup><mml:mi>R</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>, the root mean-square error, RMSE, and a <inline-formula><mml:math id="M269" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula>-fold cross-validation score. It was found that a low-order polynomial provided a good fit, with <inline-formula><mml:math id="M270" display="inline"><mml:mrow><mml:msup><mml:mi>R</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.40</mml:mn></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M271" display="inline"><mml:mrow><mml:mtext>RMSE</mml:mtext><mml:mo>=</mml:mo><mml:mn mathvariant="normal">475</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M272" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>, and positive cross-validation performance, while higher-degree polynomials yield only marginal improvements in RMSE and increasingly unstable cross-validation statistics indicative of overfitting. The resulting quadratic relation between <inline-formula><mml:math id="M273" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> (in <inline-formula><mml:math id="M274" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>) and <inline-formula><mml:math id="M275" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (in <inline-formula><mml:math id="M276" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>) is <inline-formula><mml:math id="M277" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1797.5</mml:mn><mml:mo>+</mml:mo><mml:mn mathvariant="normal">62.33</mml:mn><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.652</mml:mn><mml:msubsup><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d2e4088">Figure 7 depicts the best-fit curve overlaid on the observed PICASSO distribution of <inline-formula><mml:math id="M278" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> as a function of <inline-formula><mml:math id="M279" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. It can be seen from the figure that the fit captures the overall increase of <inline-formula><mml:math id="M280" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> with temperature, while the substantial scatter about the curve, especially at the warmer temperatures, reflects the differing cloud bulk and microphysical properties encountered during each of the PICASSO flights.</p>

      <fig id="F7"><label>Figure 7</label><caption><p id="d2e4126">Joint distribution of <inline-formula><mml:math id="M281" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and in-cloud temperature <inline-formula><mml:math id="M282" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for the PICASSO dataset. The coloured hexagons show a two-dimensional histogram of <inline-formula><mml:math id="M283" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> versus <inline-formula><mml:math id="M284" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, shaded by log10(count) as indicated by the colour bar on the right-side of the figure.  The red line shows the best-fit quadratic polynomial: <inline-formula><mml:math id="M285" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1797.5</mml:mn><mml:mo>+</mml:mo><mml:mn mathvariant="normal">62.33</mml:mn><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.652</mml:mn><mml:msubsup><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f07.png"/>

        </fig>

      <p id="d2e4225">In the CCREST-M retrievals, this quadratic relation is used to predict a deterministic first-guess profile of <inline-formula><mml:math id="M286" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> from the dropsonde temperatures. As with the 3 <inline-formula><mml:math id="M287" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> IWC retrieval, the role of <inline-formula><mml:math id="M288" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is to keep the ML-based PSD moment estimates close to representative values by providing a good starting point, while the subsequent multi-frequency optimisation adjusts the PSD parameters to match the observed reflectivities. We next describe the physically based dual-frequency retrieval of the PSD parameters given the ML first guess PSD parameter profiles.</p>
</sec>
<sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Retrieval methodology in physical space</title>
      <p id="d2e4266">For the dual-frequency retrieval methodology we utilise the <inline-formula><mml:math id="M289" display="inline"><mml:mrow><mml:mn mathvariant="normal">35</mml:mn><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M290" display="inline"><mml:mrow><mml:mn mathvariant="normal">94</mml:mn><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> GHz mean profile radar data and we employ a gamma size distribution model for the PSD as given by Eq. (<xref ref-type="disp-formula" rid="Ch1.E2"/>). The forward model F is given by Eq. (<xref ref-type="disp-formula" rid="Ch1.E1"/>).  Here, the retrieval process begins with an initial guess profile derived from the ensemble of ML moment predictions, which are transformed into the PSD parameters <inline-formula><mml:math id="M291" display="inline"><mml:mrow><mml:mi mathvariant="italic">μ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M292" display="inline"><mml:mrow><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M293" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> via Eqs. (4)–(6), respectively, to provide the starting values for the retrieval. The algorithm then retrieves optimal values of <inline-formula><mml:math id="M294" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M295" display="inline"><mml:mrow><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> by minimising the differences between the forward model predictions and the observed radar reflectivities at both 35 and 94 <inline-formula><mml:math id="M296" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> simultaneously.</p>
      <p id="d2e4386">The minimisation problem can be formally expressed as:

            <disp-formula id="Ch1.E8" content-type="numbered"><label>8</label><mml:math id="M297" display="block"><mml:mtable class="split" rowspacing="0.2ex" displaystyle="true" columnalign="right left"><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:msup><mml:mo>)</mml:mo><mml:mtext>retrieved</mml:mtext></mml:msup><mml:mo>=</mml:mo><mml:mi>arg⁡</mml:mi><mml:mo movablelimits="false">min⁡</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>,</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>∥</mml:mo><mml:mi>F</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>,</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>Z</mml:mi><mml:mtext>obs</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:mn mathvariant="normal">35</mml:mn><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>,</mml:mo><mml:mn mathvariant="normal">94</mml:mn><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow><mml:mo>)</mml:mo><mml:mo>∥</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>

          where <inline-formula><mml:math id="M298" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mtext>obs</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> represents the observed 35 and 94 <inline-formula><mml:math id="M299" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivities, and the retrieval results are only accepted when the difference between the forward model and observations satisfies the following condition:

            <disp-formula id="Ch1.E9" content-type="numbered"><label>9</label><mml:math id="M300" display="block"><mml:mrow><mml:mo>∥</mml:mo><mml:mi>F</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>,</mml:mo><mml:mi mathvariant="italic">λ</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>Z</mml:mi><mml:mtext>obs</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:mn mathvariant="normal">35</mml:mn><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>,</mml:mo><mml:mn mathvariant="normal">94</mml:mn><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow><mml:mo>)</mml:mo><mml:mo>∥</mml:mo><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:mrow></mml:math></disp-formula>

          To solve this minimisation problem, we implement the Nelder–Mead simplex algorithm, which is a derivative-free optimisation method. The Nelder–Mead approach, see Nelder and Mead (1965), iteratively refines a simplex (a geometric figure in <inline-formula><mml:math id="M301" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula>-dimensional space with <inline-formula><mml:math id="M302" display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> vertices) to find the minimum of our objective function. Also, the Nelder–Mead algorithm demonstrates robust performance in the presence of noise and other irregularities in the objective function, making this method appropriate for the retrievals where observational uncertainties are inherent. In the next sub-section, we describe the method to retrieve the IWC from the 3 <inline-formula><mml:math id="M303" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar using the optimisation presented here.</p>
</sec>
<sec id="Ch1.S4.SS4">
  <label>4.4</label><title>Retrieval of the IWC profiles</title>
      <p id="d2e4672">To retrieve the IWC, we utilise the 3 <inline-formula><mml:math id="M304" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivities, and for this retrieval the climatologically averaged PSD parameters found for <inline-formula><mml:math id="M305" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M306" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M307" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>, which have been derived from the PICASSO dataset are used to initialise the retrieval of <inline-formula><mml:math id="M308" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, where <inline-formula><mml:math id="M309" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> is set to its climatologically averaged value of 2.33 throughout the retrieval. In the case of <inline-formula><mml:math id="M310" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, this parameter is allowed to vary with temperature following Hogan et al. (2006), where we initialise and adjust <inline-formula><mml:math id="M311" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> according to the relationship <inline-formula><mml:math id="M312" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">14</mml:mn></mml:msup><mml:mi>exp⁡</mml:mi><mml:mo>(</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.122</mml:mn><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, and the numerical factor in the relationship is derived from the PICASSO climatology using the <inline-formula><mml:math id="M313" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> equation from Kozu and Nakamura (1991), <inline-formula><mml:math id="M314" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is in units of degree Celsius. This retrieval uses the same forward-model retrieval framework as the full multi-frequency retrieval described in Sect. 4.3, but in this case the radar observation consists solely of the 3 <inline-formula><mml:math id="M315" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivities. The retrieval of IWC here is to provide IWC profiles as an input feature to the ensemble of ML models.</p>
      <p id="d2e4813">The gradient <inline-formula><mml:math id="M316" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> is retrieved by minimising the difference between <inline-formula><mml:math id="M317" display="inline"><mml:mrow><mml:mo>∥</mml:mo><mml:mi>F</mml:mi><mml:mo>(</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>Z</mml:mi><mml:mtext>obs</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow><mml:mo>)</mml:mo><mml:mo>∥</mml:mo></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math id="M318" display="inline"><mml:mrow><mml:mi>F</mml:mi><mml:mo>(</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M319" display="inline"><mml:mrow><mml:msub><mml:mi>Z</mml:mi><mml:mtext>obs</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> are the forward model given by Eq. (<xref ref-type="disp-formula" rid="Ch1.E1"/>) and observed radar reflectivities at 3 <inline-formula><mml:math id="M320" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, respectively, with retrievals only being accepted when these differences are less than 1 <inline-formula><mml:math id="M321" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. Thus, using the retrieved <inline-formula><mml:math id="M322" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, estimated <inline-formula><mml:math id="M323" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and constant <inline-formula><mml:math id="M324" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>, we apply the gamma PSD to estimate the IWC using:

            <disp-formula id="Ch1.E10" content-type="numbered"><label>10</label><mml:math id="M325" display="block"><mml:mrow><mml:mtext>IWC</mml:mtext><mml:mo>=</mml:mo><mml:msubsup><mml:mo>∫</mml:mo><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>min</mml:mtext></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>max</mml:mtext></mml:msub></mml:mrow></mml:msubsup><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mi>n</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></disp-formula>

          where in Eq. (<xref ref-type="disp-formula" rid="Ch1.E10"/>), <inline-formula><mml:math id="M326" display="inline"><mml:mrow><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is the mass–dimension relationship from Cotton et al. (2013), i.e., <inline-formula><mml:math id="M327" display="inline"><mml:mrow><mml:mi>m</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.0257</mml:mn><mml:msubsup><mml:mi>D</mml:mi><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. This mass power law is the same as the mass power law used to construct the rosette aggregate model described in Sect. 3, and the rosette aggregate model is used to predict the backscattering coefficients at 3 <inline-formula><mml:math id="M328" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> using the well-known Rayleigh scattering, assuming the equivalent ice mass spherical radius.</p>
      <p id="d2e5057">To test our retrieval of IWC using the 3 <inline-formula><mml:math id="M329" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar data we use collocated radar and aircraft observations from the PICASSO flight C081. Figure 8 compares the hexagonally binned retrieved IWC with the in-situ IWC measured by the Nevzorov probe for all samples above 3200 <inline-formula><mml:math id="M330" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. We focus on altitudes greater than 3200 <inline-formula><mml:math id="M331" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> owing to the presence of a melting layer at lower altitudes. We specifically target retrievals outside of the melting layer because during CCREST-M we deliberately avoided this region, as it is too complex to simulate accurately assuming the rosette aggregate model. Moreover, the comparisons in Fig. 8 include only data points where radar observations were recorded within 36 <inline-formula><mml:math id="M332" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> of the aircraft position, within 50 <inline-formula><mml:math id="M333" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> of the aircraft altitude, and within the same distance from the Chilbolton Observatory site. The hexagonally binned scatter plot shows that most points lie close to the <inline-formula><mml:math id="M334" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>:</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> line, with a RMSE difference of 0.047 <inline-formula><mml:math id="M335" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and a negligible bias of just 0.004 <inline-formula><mml:math id="M336" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, but with a moderate <inline-formula><mml:math id="M337" display="inline"><mml:mrow><mml:mi>r</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.44</mml:mn></mml:mrow></mml:math></inline-formula>, the latter value is probably owing to the limited range of sampled IWC because of the choice of the minimum altitude. However, in absolute terms the 3 <inline-formula><mml:math id="M338" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> retrieval of IWC reproduces the Nevzorov-derived IWC with small errors over the ice layer of interest. Moreover, in the retrieval framework, the 3 <inline-formula><mml:math id="M339" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> retrieved IWC profile is used only as a constraint on the first-guess PSD moments for the multi-frequency optimisation described in Sect. 4.3, so the IWC profile does not need to be completely correct but rather provide a reasonable estimate of the profile of ice mass within the cloud, which the retrieval achieves as Fig. 8 depicts.</p>

      <fig id="F8"><label>Figure 8</label><caption><p id="d2e5178">Hexagonally binned scatter plots of retrieved IWC from the 3 <inline-formula><mml:math id="M340" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar plotted against in-situ Nevzorov-derived IWC for the PICASSO flight C081and for altitudes greater than 3200 <inline-formula><mml:math id="M341" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. The colour scale on the right-side shows the <inline-formula><mml:math id="M342" display="inline"><mml:mrow><mml:msub><mml:mi>log⁡</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> of the number collocated samples per bin, with the dashed line indicating a slope of unity. The correlation coefficient, <inline-formula><mml:math id="M343" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula>, the root mean square error (RMSE) and the bias are shown at the top of the figure.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f08.png"/>

        </fig>

      <p id="d2e5221">In the next section, the retrieval methodologies outlined in this section and sub-sections are applied to the three in-situ cases that were sampled during the CCREST-M campaign of flying.</p>
</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>The PSD parameter retrievals and comparisons with aircraft data</title>
      <p id="d2e5234">Here, the retrieval methodology outlined in Sect. 4 is applied to the zenith-pointing 3, 35 and 94 <inline-formula><mml:math id="M344" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> mean radar reflectivity profiles for the three CCREST-M cases (C374, C379, C382). For each of the flights, the zenith-pointing radar profiles are taken from periods when the FAAM BAe-146 aircraft executed figure-of-eight overpasses above cloud top while all three radars operated in zenith pointing mode.</p>
      <p id="d2e5245">For C374, these figure-of-eight overpasses occurred in three blocks between about 10:24–10:43, 11:29–11:33, and 11:37–11:42 UTC at altitudes near to 10 <inline-formula><mml:math id="M345" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>. After the third set of overpasses, the aircraft flew a single profile descent through the cloud as described in Sect. 2. For C379, the aircraft flew two blocks of figure-of-eight overpasses between approximately 16:10–16:26 and 17:07–17:28 UTC. These were followed by in-situ sampling along the 270° radial, which began at about 17:33 UTC and lasted until about 18:11 UTC, and consisted of stepped descents with straight-and-level runs of several minutes at successive levels. Finally, for C382, the aircraft first completed the figure-of-eight overpasses between about 15:00 and 15:26 UTC and again between 16:17 and 16:28 UTC while the radars were in Zenith mode. The subsequent in-situ sampling along the 246° radial began at 16:33 until about 17:09 UTC, following a similar pattern to C379.</p>
      <p id="d2e5256">As alluded to previously, only a single aircraft was available, and from the flight patterns and timings described above, the in-situ PSDs and the zenith-retrieved PSDs are not strictly collocated in time and space, instead they represent different realisations of the same frontal ice cloud systems.  The in-situ legs typically lag the initial zenith-dwell period by about 60 <inline-formula><mml:math id="M346" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> but closely follow the final zenith-dwell period by about 5 <inline-formula><mml:math id="M347" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula>.  Horizontally, each in-situ straight and level run lasts about 9 <inline-formula><mml:math id="M348" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> at an airspeed of about 100 <inline-formula><mml:math id="M349" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, corresponding to along-track distances of order 50–60 <inline-formula><mml:math id="M350" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> along the selected Chilbolton radial before the aircraft turns to begin the next leg. Thus, the in-situ sampling spans a substantial segment of the radar radial rather than a single point above the Chilbolton site. For each flight we therefore compare the retrieved PSDs statistically with the in-situ composited PSDs, rather than on a point-by-point basis, and retrievals that are below the IWC threshold of 0.002 <inline-formula><mml:math id="M351" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> are rejected for the reasons given in Sect. 2.1.  The following sub-sections present the ensemble ML moment predictions, retrieved PSDs, and their comparisons with the in-situ moments and PSDs for each case.</p>
<sec id="Ch1.S5.SS1">
  <label>5.1</label><title>The case C374</title>
      <p id="d2e5333">For C374, we begin by comparing the ensemble ML predictions of the target moments with those derived in-situ from the composite PSDs. Following this, the retrieved PSDs are evaluated against the in-situ composite PSDs as a function of temperature, the dual-frequency residuals are also examined along with comparisons of IWCs estimated from the retrieved PSDs with the Nevzorov-derived IWCs.</p>
<sec id="Ch1.S5.SS1.SSS1">
  <label>5.1.1</label><title>Moment estimations and comparisons with aircraft data</title>
      <p id="d2e5343">The ensemble ML model predictions of <inline-formula><mml:math id="M352" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M353" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M354" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M355" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> are compared with the derived in-situ estimated moments from the composite PSDs in Fig. 9a–d, the comparisons are shown as normalised probability density functions (PDFs), where the area under the curve equates to unity. Here the in-situ distributions are formed from all PSDs measured during the stepped-descent legs, while the ML distributions are formed from the ML predictions from the zenith-radar retrieval levels over about the same altitude range. To assess the sensitivity of the ML predictions to the assumed shape of the PSD in the 3 <inline-formula><mml:math id="M356" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> IWC retrieval, results are shown for both gamma and exponential PSD assumptions. We consider altitudes greater than 1 <inline-formula><mml:math id="M357" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, and in-cloud temperatures warmer than <inline-formula><mml:math id="M358" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M359" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d2e5427">Under the gamma PSD assumption, the ML ensemble predictions compare favourably with the in-situ moments, with similar distribution spreads, indicating that the ML captures to some extent the natural variability observed in the in-situ data. The central tendency is well captured for <inline-formula><mml:math id="M360" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M361" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> as shown in panels (a) and (d) but is slightly underestimated for <inline-formula><mml:math id="M362" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M363" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in panels (b) and (c). A systematic bias is nonetheless evident across all the parameters, for instance, for <inline-formula><mml:math id="M364" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> the in-situ mean is 941 <inline-formula><mml:math id="M365" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> compared with 734 <inline-formula><mml:math id="M366" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> for the ensemble ML model, and similar leftward shifts are apparent in panels (b)–(d).</p>
      <p id="d2e5506">For the case of the exponential PSD assumption, we see that this PSD assumption mitigates the previous negative biases for the higher-order moments. The central tendencies of the ML predictions for <inline-formula><mml:math id="M367" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M368" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M369" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> shift towards the in-situ values, and the distribution spreads improve correspondingly. For <inline-formula><mml:math id="M370" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, which is a ratio of moments, the change in PSD assumption has little impact as shown in panel (a). The improvement at the high-order moments is likely owing to the exponential distribution predicting a greater occurrence of larger particles than the gamma distribution.</p>

      <fig id="F9" specific-use="star"><label>Figure 9</label><caption><p id="d2e5556">The normalised PDFs of the logarithm (base 10) of the predicted and observed moments for case C374. In-situ size distributions derived from the composite PSDs are shown as solid blue lines and a blue shaded fill. The ML ensemble predictions are presented for the gamma and exponential PSD assumptions used in the retrieval of the 3 <inline-formula><mml:math id="M371" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> IWC. The gamma and exponential PSD assumptions are shown as the orange-dashed line with orange fill, and green-dashed line with green fill, respectively. Comparisons are presented for <bold>(a)</bold> <inline-formula><mml:math id="M372" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M373" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M374" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <bold>(d)</bold> <inline-formula><mml:math id="M375" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The key is shown in the top-left corner of each panel.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f09.png"/>

          </fig>

      <p id="d2e5630">The impact of changing the shape assumption of the PSD on the retrieval of IWC and how this manifests itself on the retrieved PSDs as a function of temperature will be examined in the next sub-section.</p>
</sec>
<sec id="Ch1.S5.SS1.SSS2">
  <label>5.1.2</label><title>Retrieval of the PSDs and comparisons with the in-situ composite PSDs</title>
      <p id="d2e5641">Now that we have derived the first-guess profiles for the PSD parameters from the profiles of IWC, <inline-formula><mml:math id="M376" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M377" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M378" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>, the PSD parameters, <inline-formula><mml:math id="M379" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M380" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M381" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> are input to the dual-frequency retrieval as described in Sect. 4.3, only varying <inline-formula><mml:math id="M382" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M383" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> while keeping the profile of <inline-formula><mml:math id="M384" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula> as the first guess. Figure 10a–e presents a comparison between retrieved and in-situ composite PSDs for the flight C374, as a function of temperature for maximum dimensions greater than 100 <inline-formula><mml:math id="M385" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>m. The retrieved PSDs assume gamma and exponential size distributions for the retrieval of the IWC profiles using the 3 <inline-formula><mml:math id="M386" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar and only include retrievals greater than 1 <inline-formula><mml:math id="M387" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> in altitude to focus on the primary iced regions of this frontal cloud system and IWCs greater than 0.002 <inline-formula><mml:math id="M388" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. To provide robust statistical comparisons, the analysis presents the mean and the in-situ interpercentile range (20th to 95th percentiles) for both sets of data across five temperature bins: <inline-formula><mml:math id="M389" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M390" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M391" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M392" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M393" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M394" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M395" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M396" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M397" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> to 0 <inline-formula><mml:math id="M398" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>. This choice of in-situ interpercentile range retains the bulk of the distribution while excluding the retrievals in the lowest tail, and a small number of very large values which may arise from occasional misfits. Thus, the 20th to 95th percentile range provides a clearer view of the central behaviour of the retrievals relative to the in-situ composites without being overly influenced by a small number of extremes. Also, the temperature stratification allows examination of retrieval performance as a function of temperature, and it is the temperature that chiefly determines the microphysics. Here, we focus on the PSDs themselves rather than plotting the corresponding moments of the retrieved PSDs after the 35 and 94 <inline-formula><mml:math id="M399" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> fitting. This is because the moments are effectively summarised by the PSD comparisons shown in Fig. 10a–e and so a moment-by-moment comparison would therefore be redundant.</p>

      <fig id="F10" specific-use="star"><label>Figure 10</label><caption><p id="d2e5878">Comparison of retrieved and in-situ composite PSDs for flight C374 as a function of temperature. Retrieved mean PSDs assuming the gamma and exponential PSDs for the retrieval of the 3 <inline-formula><mml:math id="M400" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> IWC are shown as red solid lines and green-dotted lines, respectively. The composite mean in-situ PSDs are shown as solid blue lines and the in-situ 20th and 95th percentiles are shown as the grey dashed lines.  Results are presented for the temperature bins <bold>(a)</bold> <inline-formula><mml:math id="M401" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M402" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M403" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M404" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M405" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M406" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M407" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M408" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M409" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>, <bold>(d)</bold> <inline-formula><mml:math id="M410" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M411" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M412" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>, and <bold>(e)</bold> <inline-formula><mml:math id="M413" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> to 0 <inline-formula><mml:math id="M414" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>. The key is shown in the upper-right of panel <bold>(a)</bold>.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f10.png"/>

          </fig>

      <p id="d2e6056">For the case of assuming the gamma size distribution for the retrieval of IWC at 3 <inline-formula><mml:math id="M415" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> the comparisons presented in Fig. 10a–e show generally good agreement between the retrieved and in-situ PSDs across most of the temperature bins. For instance, the mean retrieved PSD is largely within the interpercentile range of the in-situ PSDs for most of the considered temperatures. The most notable systematic overestimations of the retrieved number concentrations relative to the in-situ concentrations occur for the sizes of several hundred <inline-formula><mml:math id="M416" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> at the warmer temperatures, especially as seen in Fig. 10c–e. In general, the figure shows that across all temperature regimes there is considerable overlap in the variability captured by the retrieved and in-situ PSDs, suggesting that the retrieval method successfully represents the natural variability in PSD characteristics, even when absolute concentrations might be biased at some of the sizes.</p>
      <p id="d2e6078">In the case of the exponential PSD being assumed to retrieve the IWC at 3 <inline-formula><mml:math id="M417" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, the exponential size distribution assumption produces notable changes in representing smaller ice crystal number concentrations at the warmer temperature bins. Specifically, it tends to overestimate number concentrations for sizes less than about 1000 <inline-formula><mml:math id="M418" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> and above several thousand microns, as shown in panels (b, d, e).</p>
      <p id="d2e6099">To further evaluate the retrieved PSDs assuming the gamma or exponential PSD for the retrieval of IWC at 3 <inline-formula><mml:math id="M419" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, we compare the mean and standard deviation, <inline-formula><mml:math id="M420" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>, of the IWC computed from the retrieved PSDs, using Eq. (<xref ref-type="disp-formula" rid="Ch1.E10"/>) assuming the Cotton et al. (2013) mass–dimension power law, within each temperature bin, with corresponding in-situ IWC statistics measured by the Nevzorov probe. The results of these comparisons are presented in Table 2, along with the numbers of retrieved PSDs and in-situ measurements within the interpercentile range used in the calculation for each of the temperature bins.</p>

<table-wrap id="T2" specific-use="star"><label>Table 2</label><caption><p id="d2e6122">Comparison of retrieved (<inline-formula><mml:math id="M421" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>/</mml:mo><mml:mtext>exp</mml:mtext></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>) and in-situ (In) statistics for the mean and standard deviation of the IWC in each temperature bin, with the total number (num) of retrievals (num<sub>gamma/exp</sub>) and measurements filtered into each temperature bin.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="7">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="center"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Temp Bin (<inline-formula><mml:math id="M423" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">In-situ num</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M424" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> num<sub>gamma</sub></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M426" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> num<sub>exp</sub></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M428" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="italic">γ</mml:mi></mml:msub><mml:mover accent="true"><mml:mtext>IWC</mml:mtext><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>±</mml:mo><mml:mi mathvariant="italic">σ</mml:mi></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math id="M429" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M430" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mtext>exp</mml:mtext></mml:msub><mml:mover accent="true"><mml:mtext>IWC</mml:mtext><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>±</mml:mo><mml:mi mathvariant="italic">σ</mml:mi></mml:mrow></mml:math></inline-formula>  (<inline-formula><mml:math id="M431" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col7">In <inline-formula><mml:math id="M432" display="inline"><mml:mrow><mml:mover accent="true"><mml:mtext>IWC</mml:mtext><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>±</mml:mo><mml:mi mathvariant="italic">σ</mml:mi></mml:mrow></mml:math></inline-formula>  (<inline-formula><mml:math id="M433" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M434" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M435" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">124</oasis:entry>
         <oasis:entry colname="col3">56</oasis:entry>
         <oasis:entry colname="col4">49</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M436" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.011</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.005</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M437" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.015</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.006</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M438" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.016</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.004</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M439" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M440" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">315</oasis:entry>
         <oasis:entry colname="col3">99</oasis:entry>
         <oasis:entry colname="col4">96</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M441" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.021</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.011</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M442" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.025</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.015</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M443" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.03</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.007</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M444" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M445" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">238</oasis:entry>
         <oasis:entry colname="col3">114</oasis:entry>
         <oasis:entry colname="col4">110</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M446" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.070</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.02</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M447" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.064</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.02</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M448" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.049</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.015</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M449" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M450" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">661</oasis:entry>
         <oasis:entry colname="col3">129</oasis:entry>
         <oasis:entry colname="col4">143</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M451" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.098</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.027</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M452" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.096</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.027</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M453" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.059</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.019</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M454" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> to 0</oasis:entry>
         <oasis:entry colname="col2">540</oasis:entry>
         <oasis:entry colname="col3">163</oasis:entry>
         <oasis:entry colname="col4">157</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M455" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.148</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.034</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M456" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.181</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.046</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M457" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.084</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.037</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d2e6699">Under both the gamma and exponential PSD assumptions, Table 2 demonstrates that for the integral property IWC, the retrieved PSDs generally compare well with the in-situ Nevzorov measurements in the two coldest temperature ranges. At the warmer temperatures, both assumptions tend to overestimate the in-situ mean IWC values by varying amounts, although the differences remain within a factor of two. However, despite this, there is substantial statistical overlap between the retrieved and in-situ IWC ranges for both PSD assumptions. The only exception being the exponential PSD assumption at the warmest temperature bin. Figure 10 and Table 2 illustrate the trade-off at different temperature bins in selecting an optimal size distribution that performs well across the full range of ice cloud conditions.</p>
      <p id="d2e6702">To evaluate the consistency of the retrieval framework, it is instructive to examine how well the forward-modelled radar reflectivities at 35 and 94 <inline-formula><mml:math id="M458" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> compare with observations when using the retrieved PSDs and scattering model. Figure 11 (left–right panels) depicts the radar reflectivity profiles and their residuals, assuming the gamma PSD for the 3 <inline-formula><mml:math id="M459" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> retrieval of IWC, computed from Eqs. (<xref ref-type="disp-formula" rid="Ch1.E1"/>) and (<xref ref-type="disp-formula" rid="Ch1.E9"/>), for accepted retrievals as a function of altitude for two of the six coincident overpasses between the aircraft and zenith-pointing radars. In Fig. 11 (left–right panels), we show residuals for the first (10.49 <inline-formula><mml:math id="M460" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula>) and last (11.63 <inline-formula><mml:math id="M461" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula>) overpass times, as these are representative of all six overpass times.</p>

      <fig id="F11" specific-use="star"><label>Figure 11</label><caption><p id="d2e6745">Comparison of forward model simulations (blue lines and circles) and observations (orange lines and circles) with their corresponding residuals (red lines and circles) as a function of altitude for the 35 <bold>(a, b)</bold> and 94 <inline-formula><mml:math id="M462" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> <bold>(c, d)</bold> radars. Times correspond to coincident aircraft overpasses for 10.49 <inline-formula><mml:math id="M463" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> (left panels) and 11.63 <inline-formula><mml:math id="M464" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> (right panels). The key is shown in the top-right of each panel.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f11.png"/>

          </fig>

      <p id="d2e6784">The radar reflectivity comparisons demonstrate generally good agreement between the forward-modelled and observed reflectivities across most altitude levels. At both of the frequencies, the simulated reflectivities closely follow the observed profiles through the main parts of the ice cloud, with residuals typically well within <inline-formula><mml:math id="M465" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M466" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. This agreement shows that the retrieved PSDs and scattering model are appropriate for the bulk of the ice cloud. However, at the cloud top regions and on some occasions in the cloud bottom regions, in particular panel (d) at the time of 11.625 <inline-formula><mml:math id="M467" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula>, below about 5 <inline-formula><mml:math id="M468" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, residuals show increased variability and magnitude, with some approaching <inline-formula><mml:math id="M469" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M470" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula> in those regions. At the cloud top regions, the radars become less sensitive, owing to the smaller sizes and concentrations of ice crystals making retrievals in those regions more problematic. The consistency of this pattern across all of the six times suggests that the greater deviations of the residuals from near-zero are systematic rather than random, indicating the fundamental limitation of the dual-frequency retrievals in regions where the ice crystals are small and radar sensitivity is reduced. At cloud bottom, ice crystal type may also be changing causing the retrievals to become more problematic where this could be occurring. The computed and measurement residuals are not shown for the exponential PSD assumption as these are very similar to those already presented in Fig. 11.</p>
      <p id="d2e6840">One radar frequency operated during C374 but not used in any retrievals was the G-band GRaCE radar, providing an excellent independent validation of the retrieved PSDs and scattering model. The radar operation during C374 and applied attenuation corrections have been fully discussed by McCusker et al.  (2025), and so will not be repeated here. However, in this paper, the G-band reflectivities have been corrected for ice attenuation using the rosette aggregate model. The forward-modelled GRaCE radar reflectivity using the retrieved filtered PSDs and the randomly oriented rosette aggregate model is compared with the GRaCE observations in Fig. 12. The figure compares the forward-modelled 200 <inline-formula><mml:math id="M471" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivity, computed from the retrieved PSDs assuming both the gamma and exponential PSD assumptions, with the GRaCE radar observations. The comparisons show time-averaged mean profiles, the standard radar reflectivity measurement uncertainty of <inline-formula><mml:math id="M472" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M473" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>, and the interpercentile ranges for both the observations and simulations. The simulations were averaged using the thresholds of 0.1 decimal hours for time and 100 <inline-formula><mml:math id="M474" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> for the altitude to provide meaningful statistical comparisons.  The comparisons were further restricted to times before approximately 11:45 UTC, beyond which the cloud evolved down to 2 <inline-formula><mml:math id="M475" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, a complex configuration which resulted in precipitation at later times. Above approximately 4.5 <inline-formula><mml:math id="M476" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> the calculated reflectivities sit within or very close to the measured 10–90th percentile envelope, and the gamma and exponential assumptions produce very similar forward-modelled profiles. For the upper part of the cloud, this level of agreement provides strong support for the rosette-aggregate scattering model and retrieved PSDs. Indeed, Fig. 3a (upper panels), show the predominant habits to be rosettes and small rosette aggregates, providing further evidence for the choice of scattering model.  Below approximately 4.5 <inline-formula><mml:math id="M477" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, the calculated mean reflectivities trend higher than the measured mean, although the calculated 10–90th percentile envelopes continue to overlap the measured envelope just above 3 <inline-formula><mml:math id="M478" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>. These discrepancies as shown by Fig. 3a in the lower parts of the clouds, are likely owing to the presence of more irregular dendritic particles and snowflakes, which are not represented by the rosette-aggregate model used here. Also, the two PSD assumptions in the lower part of the cloud follow each other closely, indicating that this independent validation cannot discriminate between the two PSD shape assumptions.</p>

      <fig id="F12"><label>Figure 12</label><caption><p id="d2e6912">Comparison of the time-averaged forward model simulations (red, green lines, and shade) assuming the retrieved PSDs, assuming the gamma (red lines) and exponential (green lines) PSDs for the retrieval of IWC at 3 <inline-formula><mml:math id="M479" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> with the 200 <inline-formula><mml:math id="M480" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> GRaCE radar observations (blue lines and shade). The key is shown in the top-right of the figure.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f12.png"/>

          </fig>

</sec>
</sec>
<sec id="Ch1.S5.SS2">
  <label>5.2</label><title>The case C379</title>
      <p id="d2e6947">For C379, the 94 <inline-formula><mml:math id="M481" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar experienced severe attenuation owing to precipitation and collection of water on the radar dome that occurred at about 09:00 UTC. More prolonged precipitation occurred from about 17:00 UTC for the rest of the day of between about several to 1 <inline-formula><mml:math id="M482" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">mm</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">h</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, as measured by the drop counting rain gauge at Chilbolton (McCusker et al., 2025). There was no rain after 10:00 UTC until about 16:00 UTC, when more episodic precipitation was measured by the rain gauge. The occurrence of lower-level liquid water cloud can clearly be seen in Fig. 2 (middle panel). Since this precipitation after 16:00 UTC occurred during the figure-of-eight overpasses and the aircraft in-situ sampling period, dual-frequency retrievals were not possible. Consequently, only single-frequency retrievals using the 35 <inline-formula><mml:math id="M483" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar are employed for this case. We begin with ML to predict the PSD parameters and use these to generate the PSDs that are compared with the in-situ composite PSDs, following the same analysis as used in Sect. 5.1.</p>
<sec id="Ch1.S5.SS2.SSS1">
  <label>5.2.1</label><title>Moment estimations and comparisons with aircraft data for C379</title>
      <p id="d2e6990">Following the methodology for the case C374, we examine the ML performance in predicting the PSD moments for single-frequency retrievals. Consistent with C374, IWC was optimally retrieved using an exponential size distribution with the 3 <inline-formula><mml:math id="M484" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar as input to the ML.</p>
      <p id="d2e7001">Figure 13a–d depicts the normalised PDFs, comparing the ML-predicted moments with those derived from the in-situ PSDs for <inline-formula><mml:math id="M485" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M486" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M487" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M488" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The ML-predicted <inline-formula><mml:math id="M489" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> distribution exhibits a bimodal structure with the primary peak positioned close to the in-situ peak. For the higher-order moments <inline-formula><mml:math id="M490" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M491" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M492" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, the ML-predicted distribution spreads align very well with the in-situ derived moments, suggesting the relative variability patterns are very well captured by ML for this case.</p>

      <fig id="F13" specific-use="star"><label>Figure 13</label><caption><p id="d2e7095">Same as Fig. 9, but for the case C379 and using the exponential size distribution to retrieve IWC at 3 <inline-formula><mml:math id="M493" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f13.png"/>

          </fig>

</sec>
<sec id="Ch1.S5.SS2.SSS2">
  <label>5.2.2</label><title>Single-frequency retrievals of the PSDs and comparisons with the in-situ composite PSDs for C379</title>
      <p id="d2e7120">For case C379, we use the 35 <inline-formula><mml:math id="M494" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar to the retrieve one PSD parameter.  The IWC profile first-guess is retrieved from the 3 <inline-formula><mml:math id="M495" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar assuming the gamma size distribution. The ML provides first-guess profiles for <inline-formula><mml:math id="M496" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M497" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>, while the slope parameter <inline-formula><mml:math id="M498" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> is optimised using Eq. (<xref ref-type="disp-formula" rid="Ch1.E8"/>) to minimise differences between the forward model simulations and the 35 <inline-formula><mml:math id="M499" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar observations.</p>
      <p id="d2e7175">Figure 14a–d compares the single-frequency PSD retrievals with the in-situ measurements for four temperature bins (<inline-formula><mml:math id="M500" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M501" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M502" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M503" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M504" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M505" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M506" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M507" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M508" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>).</p>

      <fig id="F14" specific-use="star"><label>Figure 14</label><caption><p id="d2e7271">Same as Fig. 10, but for the single-frequency retrieval using the 35 <inline-formula><mml:math id="M509" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar and assuming the gamma size distribution for the retrieval of IWC at 3 <inline-formula><mml:math id="M510" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f14.png"/>

          </fig>

      <p id="d2e7297">In Fig. 14a–d, the statistical variability of the mean retrieved PSD using a single-frequency shows good overlap within interpercentile ranges, except for panel (d) where occurrences for particle sizes between several hundred and several thousand <inline-formula><mml:math id="M511" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> are overestimated. Table 3 shows that the estimated mean IWC for this temperature bin is about three times larger than the in-situ value. This table also shows that the mean estimated IWCs agree well with the in-situ mean values between the temperatures of <inline-formula><mml:math id="M512" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M513" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M514" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>.</p>

<table-wrap id="T3" specific-use="star"><label>Table 3</label><caption><p id="d2e7343">Comparison of retrieved (Ret) and in-situ (In) statistics for the mean and standard deviation of the IWC in each temperature bin, with the total number (num) of retrievals and measurements filtered into each temperature bin.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="5">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Temp Bin (<inline-formula><mml:math id="M515" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">In-situ num</oasis:entry>
         <oasis:entry colname="col3">Ret num</oasis:entry>
         <oasis:entry colname="col4">Ret <inline-formula><mml:math id="M516" display="inline"><mml:mrow><mml:mover accent="true"><mml:mtext>IWC</mml:mtext><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>±</mml:mo><mml:mi mathvariant="italic">σ</mml:mi></mml:mrow></mml:math></inline-formula>  (<inline-formula><mml:math id="M517" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col5">In <inline-formula><mml:math id="M518" display="inline"><mml:mrow><mml:mover accent="true"><mml:mtext>IWC</mml:mtext><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>±</mml:mo><mml:mi mathvariant="italic">σ</mml:mi></mml:mrow></mml:math></inline-formula>  (<inline-formula><mml:math id="M519" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M520" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M521" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">137</oasis:entry>
         <oasis:entry colname="col3">35</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M522" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.015</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.003</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M523" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.014</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.008</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M524" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M525" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">285</oasis:entry>
         <oasis:entry colname="col3">88</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M526" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.023</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.009</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M527" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.021</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.005</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M528" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M529" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">510</oasis:entry>
         <oasis:entry colname="col3">135</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M530" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.034</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.019</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M531" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.030</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.011</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M532" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M533" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">31</oasis:entry>
         <oasis:entry colname="col3">11</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M534" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.040</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.013</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M535" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.013</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.007</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d2e7684">Critically, the single-frequency retrievals agree well with the in-situ measured IWCs across the sampled temperature range. For this case, the differences between the forward-modelled radar reflectivities at 35 <inline-formula><mml:math id="M536" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> and the observations when using the retrieved PSDs and scattering model are like those already presented for C374 in Fig. 11, and so are not repeated here for reasons of brevity. Suffice to say that generally throughout the cloud layer, between about 5.5 and 8 <inline-formula><mml:math id="M537" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, the measurement residuals are generally <inline-formula><mml:math id="M538" display="inline"><mml:mrow><mml:mo>≪</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M539" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula> for all overpass times. Having studied C374 and C379, we now examine the final case C382.</p>
</sec>
</sec>
<sec id="Ch1.S5.SS3">
  <label>5.3</label><title>The case C382</title>
      <p id="d2e7730">Case C382 represents a test of the retrieval methodology for ice clouds that are geometrically thinner than the other two cases. To avoid precipitation contamination of approximately just over 1 <inline-formula><mml:math id="M540" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">mm</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">h</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> between 16:00 and 17:00 UTC, this analysis focusses on the radar profile at 15.117 <inline-formula><mml:math id="M541" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula>, allowing application of the full dual-frequency retrieval methodology to the 3, 35 and 94 <inline-formula><mml:math id="M542" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar profiles. For this case, the in-situ sampling began at 16.55 and continued until about 17.15 <inline-formula><mml:math id="M543" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula>, some 60–90 <inline-formula><mml:math id="M544" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> after the first figure-of-eight overpasses, which began at about 15.00 <inline-formula><mml:math id="M545" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> and ended at 15.43 <inline-formula><mml:math id="M546" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula>.</p>
<sec id="Ch1.S5.SS3.SSS1">
  <label>5.3.1</label><title>Moment estimations and comparisons with aircraft data for C382</title>
      <p id="d2e7806">Following the established methodology, we first examine the ML performance in predicting the PSD moments used in the dual-frequency retrievals. The IWC profile is retrieved at 3 <inline-formula><mml:math id="M547" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> assuming the exponential size distribution function. Figure 15a–d, reveals a failure of the ML model for this thinner and colder ice cloud case, with minimal overlap between predicted and observed distributions. The ML-predicted <inline-formula><mml:math id="M548" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mtext>mmw</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> peaks at approximately 470 <inline-formula><mml:math id="M549" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> compared to the in-situ peak near to 600 <inline-formula><mml:math id="M550" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>.  The higher-order moments show even larger systematic underestimation, with predicted distribution shapes differing significantly from the in-situ distributions.</p>

      <fig id="F15" specific-use="star"><label>Figure 15</label><caption><p id="d2e7850">As Fig. 13, but for C382.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f15.png"/>

          </fig>

      <p id="d2e7859">This ML failure likely occurs because C382 falls outside the model's training domain. The PICASSO campaign training dataset predominantly sampled lower-altitude warmer ice clouds. This underscores the importance of ensuring training datasets encompass the full range of atmospheric conditions expected in applications. This is also why the ML PSD profiles are generally used as the first guess estimates to aid physics-based multi-frequency radar retrievals of the PSDs. </p>
</sec>
<sec id="Ch1.S5.SS3.SSS2">
  <label>5.3.2</label><title>Dual-frequency retrievals of the PSDs and comparisons with the in-situ composite PSDs for C382</title>
      <p id="d2e7871">Using the dual-frequency retrieval method with the ML-predicted moments from Fig. 15, the retrieved PSDs are compared with the in-situ measurements as a function of in-cloud temperature in Fig. 16a–c, following the same procedures as the other cases. Results assume the exponential size distribution for the retrieval of IWC at 3 <inline-formula><mml:math id="M551" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> for altitudes greater than 5 <inline-formula><mml:math id="M552" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> and IWCs greater than 0.002 <inline-formula><mml:math id="M553" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. The ice cloud was situated between approximately 5.0 and 8 <inline-formula><mml:math id="M554" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, with the in-cloud temperatures stratified into three in-cloud temperature bins: <inline-formula><mml:math id="M555" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M556" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M557" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M558" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M559" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M560" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M561" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>.</p>

      <fig id="F16" specific-use="star"><label>Figure 16</label><caption><p id="d2e7988">As Fig. 14 but for C382 and temperature bins of <bold>(a)</bold> <inline-formula><mml:math id="M562" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M563" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M564" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M565" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M566" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M567" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>, and <bold>(c)</bold> <inline-formula><mml:math id="M568" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> to <inline-formula><mml:math id="M569" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M570" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">°</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f16.png"/>

          </fig>

      <fig id="F17" specific-use="star"><label>Figure 17</label><caption><p id="d2e8100">Same as Fig. 11, but for the case C382 at the time of 15.117 <inline-formula><mml:math id="M571" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> (left panel) and 15.559 <inline-formula><mml:math id="M572" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> (right panel). Effects of a thin cirrus layer detached from the main ice layer can be seen at altitudes between about 8.5 and 9 <inline-formula><mml:math id="M573" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> (left panel).</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4367/2026/amt-19-4367-2026-f17.png"/>

          </fig>

      <p id="d2e8134">Figure 16a–c reveals that the dual-frequency retrievals do not improve upon the first-guess profiles, with mean retrieved PSDs generally systematically underestimating the in-situ number concentrations across all particle sizes at the two coldest temperature bins and for sizes greater than several hundred microns at the warmest temperature bin. This systematic bias propagates to substantial underestimation of computed IWC by several factors (not shown here for reasons of brevity). The in-situ PSDs exhibit notably broad distributions even at the coldest temperatures, suggesting the presence of large ice crystals throughout the sample volume of the in-situ measurements. Moreover, changing to the gamma size distribution to retrieve the IWC at 3 <inline-formula><mml:math id="M574" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> does not fundamentally alter these results, indicating that the mismatch between ML predictions and the ice cloud conditions cannot be bridged by PSD parameter optimisation alone.</p>
      <p id="d2e8145">To investigate whether improved initial conditions could enhance performance, we replaced the ML model predictions with the in-situ derived gamma PSD parameters as the first guess estimates. The results of this investigation revealed that this substitution does not improve agreement between the retrieved and in-situ PSDs, the results being very similar to Fig. 16 and so are not reproduced here for reasons of brevity. Despite starting from nearly perfect conditions, the dual-frequency optimisation consistently drives the retrievals away from the in-situ measurements. This systematic divergence may suggest that the fundamental issue lies with a mismatch between the radar observations and the in-situ measurements themselves, most likely owing to temporal evolution of the ice cloud between radar sampling, which began at 15.117 <inline-formula><mml:math id="M575" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> and ended at 16.559 <inline-formula><mml:math id="M576" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula>, and the later in-situ aircraft measurements. The 90 <inline-formula><mml:math id="M577" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> interval between the beginning radar sampling time and the in-situ sampling that started after 16.559 <inline-formula><mml:math id="M578" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> allowed the cloud to evolve toward broader PSDs with larger ice crystals.</p>
      <p id="d2e8180">To test whether the assumed Cotton et al. (2013) mass–dimension relation used in the rosette-aggregate scattering model is consistent with the in-situ measurements for C382, the IWC was re-computed from the composite PSDs using the relation in Eq. (<xref ref-type="disp-formula" rid="Ch1.E10"/>) and compared with the IWC derived from the Nevzorov probe. The re-computed PSD IWCs show a strong correlation with the measured IWCs with the correlation coefficient, <inline-formula><mml:math id="M579" display="inline"><mml:mrow><mml:mi>r</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.88</mml:mn></mml:mrow></mml:math></inline-formula>, and root mean square error of 0.014 <inline-formula><mml:math id="M580" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, and bias of <inline-formula><mml:math id="M581" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.006</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M582" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. The very good agreement obtained between the re-computed IWCs and the measured IWCs indicates that the assumed mass–dimension used for the rosette-aggregate scattering model is consistent with the in-situ IWC and cannot explain the discrepancy between the retrieved and in-situ PSDs.</p>
      <p id="d2e8241">Figure 17 presents the measurement residual analysis for the dual-frequency radar retrievals at the beginning of the radar sampling time at 15.117 <inline-formula><mml:math id="M583" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> (left panel) and at the end time 16.559 <inline-formula><mml:math id="M584" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> (right panel). The 35 <inline-formula><mml:math id="M585" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> residuals at 15.117 <inline-formula><mml:math id="M586" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> are quite stable, with most retrieval residuals being well within <inline-formula><mml:math id="M587" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.25</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M588" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. At 94 <inline-formula><mml:math id="M589" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, the residuals demonstrate a systematic negative bias in the presence of very small residuals at the corresponding 35 <inline-formula><mml:math id="M590" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> altitudes, though most residuals are between zero and <inline-formula><mml:math id="M591" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M592" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula>. This asymmetry in the residual analysis is a result of the retrieval optimisation favouring the 35 <inline-formula><mml:math id="M593" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> match at the expense of the 94 <inline-formula><mml:math id="M594" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> match, which suggests that at the beginning of the radar sampling the scattering model might not be completely representative of ice habits at this time. However, both frequency residuals at the time of 16.559 <inline-formula><mml:math id="M595" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> are essentially zero, except for near the cloud top at 35 <inline-formula><mml:math id="M596" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>, and inspection of the other six radar-sampling times shows that the 94 <inline-formula><mml:math id="M597" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> residual structure becomes progressively less noisy from beginning to end. The progressive stabilisation of the 94 <inline-formula><mml:math id="M598" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> residual structure possibly suggests that the cloud evolves to ice habits that are more consistent with the scattering model used here, future radiative transfer studies will study this aspect further. Given the evolution of the 94 <inline-formula><mml:math id="M599" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> residuals that is represented by Fig. 17, the temporal-evolution hypothesis remains the most plausible explanation for the discrepancy between the in-situ and retrieved PSDs.</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <label>6</label><title>Summary and conclusions</title>
      <p id="d2e8396">In this paper, a new retrieval methodology has been presented for estimating mid-latitude PSD parameters using multi-frequency radar observations. The approach combines ensemble machine learning predictions of <inline-formula><mml:math id="M600" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M601" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M602" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M603" display="inline"><mml:mrow><mml:msub><mml:mi>M</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> moments of the PSD with dual-frequency optimised physical retrievals based on the randomly oriented rosette aggregate ice crystal scattering model. The ensemble ML model, trained on the PICASSO climatology, provides robust first guess profiles of the PSD parameters <inline-formula><mml:math id="M604" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M605" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M606" display="inline"><mml:mi mathvariant="italic">μ</mml:mi></mml:math></inline-formula>, where <inline-formula><mml:math id="M607" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M608" display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> are subsequently refined by the physical retrieval to achieve simultaneous agreement with the 35 and 94 <inline-formula><mml:math id="M609" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivities. The 3 <inline-formula><mml:math id="M610" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar data are used separately to retrieve the IWC profiles that enter the ML feature vector to ultimately inform the retrieval of the PSDs.</p>
      <p id="d2e8503">Application of this retrieval methodology to three of the CCREST-M case studies (i.e., C374, C379 and C382), supported by the FAAM aircraft in-situ measurements, demonstrates that for the combined ML–physics methodology yields PSDs that reproduce observed radar reflectivities to within typically <inline-formula><mml:math id="M611" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.25</mml:mn></mml:mrow></mml:math></inline-formula>–0.5 <inline-formula><mml:math id="M612" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">dBZ</mml:mi></mml:mrow></mml:math></inline-formula> for well-constrained cases such as C374. Comparisons with in-situ composite PSDs show that the retrievals capture the observed variability as a function of temperature, with generally good agreement in mean values of the number concentration with ice crystal maximum dimension.  The choice of PSD functional form (i.e., the exponential or gamma size distributions) also introduces some sensitivity when retrieving the IWC using the 3 <inline-formula><mml:math id="M613" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar profiles. For the case C374, the gamma size distribution assumption is largely within the interpercentile ranges of the in-situ PSDs and the estimated IWCs are statistically within the ranges of the in-situ measured IWC. The exponential size distribution could overestimate the number concentrations at the smaller and larger sizes, though were also largely within the in-situ ranges of the measured IWCs, apart from the warmest temperature bin. Independent validation with the 200 <inline-formula><mml:math id="M614" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar reflectivities confirms the applicability of the rosette aggregate ice crystal scattering model for the bulk of the ice cloud above approximately 4.5 <inline-formula><mml:math id="M615" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>, where the rosette aggregates were the predominant in-situ habit. In the lower cloud regions, the presence of other ice particle types was the likely cause of departures of the rosette aggregate model simulations from the measurements. The 200 <inline-formula><mml:math id="M616" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> validation could not distinguish between the two PSD assumptions, and so no one PSD assumption was found to be the better choice.</p>
      <p id="d2e8557">For C379, the 35 <inline-formula><mml:math id="M617" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> single-frequency retrievals of the PSDs achieved successful PSD retrievals when the ML first guess was also very good.  However, the retrieved PSDs using the physically based optimisation method improved the ML first guess estimates and agreed well with the in-situ measurements for most of the temperature bins, demonstrating that single-frequency optimisation can still refine physically realistic first guess profiles when the ML model estimate is good.</p>
      <p id="d2e8568">However, for the case C382, limitations of the retrieval methodology were evident, where the presented methodology degrades in colder, thinner clouds where ML predictions extrapolate beyond their training range. For instance, in the case of C374 and C379, the ML first guess normalised distributions of the moments were found to overlap well with the normalised distributions of the in-situ derived moments. Only in the case of C382 did the ML method fail owing to an extrapolation being required rather than an interpolation.  Case-to-case differences emphasise the need for diverse training datasets and capturing the temporal evolution of ice clouds for multi-frequency approaches to robustly characterise ice cloud microphysics. For C382, the optimised retrieval did produce converged retrievals with 35 <inline-formula><mml:math id="M618" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> residuals essentially being at zero for most of the cloud layer during the radar-sampling period. However, the 94 <inline-formula><mml:math id="M619" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> residuals revealed a small systematic negative bias at the beginning of the radar sampling but diminished and became essentially zero by the end of the sampling period.  The 90 <inline-formula><mml:math id="M620" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> time difference between the beginning of the radar sampling and in-situ sampling, combined with the evolution noted in the 94 <inline-formula><mml:math id="M621" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> measurement residuals, strongly supports temporal evolution as the primary cause of the in-situ versus retrieved PSD disagreement.</p>
      <p id="d2e8604">A paper in preparation will use the same rosette aggregate ice crystal scattering model, together with the retrieved PSDs for all three cases, to forward model radiative transfer simulations of brightness temperatures across the mm-wave and sub-mm-wave spectrum. This will allow us to assess the consistency between the radar-constrained retrievals and the suitability of the adopted scattering model, using collocated radiometer measurements, for forward modelling in the data assimilation process.</p>
</sec>

      
      </body>
    <back><notes notes-type="codeavailability"><title>Code availability</title>

      <p id="d2e8611">CCREST-M code is available upon request.</p>
  </notes><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d2e8617">The CCREST-M dropsonde, and aircraft in-situ measurements and the 3 (CAMRa), and 35 <inline-formula><mml:math id="M622" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> (Kepler) radar data are available from the CEDA website located here: for C374:  <uri>https://catalogue.ceda.ac.uk/uuid/7892db5c68104a0c9caf99bc59337647</uri> (Facility for Airborne Atmospheric Measurements, Natural Environment Research Council, 2024a),  for C379: <uri>https://catalogue.ceda.ac.uk/uuid/7892db5c68104a0c9caf99bc59337647</uri> (Facility for Airborne Atmospheric Measurements, Natural Environment Research Council, 2024b), and  for C382: <uri>https://catalogue.ceda.ac.uk/uuid/67911f14d0a24d7ea8866eaf4575e9f5</uri> (Facility for Airborne Atmospheric Measurements, Natural Environment Research Council, 2024c).</p>
  </notes><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d2e8640">AJB conceived the scientific objectives of the CCREST-M campaign, developed the retrieval methodology and its implementation, performed the retrieval and in-situ comparison analyses, and led the writing of the manuscript, including revisions. SF co-developed the scientific aims of the CCREST-M campaign, served as the principal lead for the aircraft flight operations, provided the atmospheric and radar datasets for the retrievals, and contributed to the manuscript review and preparation for submission. RC provided the in-situ PSD and Nevzorov data analyses, supplied the PICASSO PSD climatology, and contributed to manuscript proofing. JD provided the 94 <inline-formula><mml:math id="M623" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> mini-BASTA radar data and its processing and contributed to manuscript proofing. CJW operated the Chilbolton Observatory radars during the CCREST-M campaign, provided and processed the CAMRa (3 <inline-formula><mml:math id="M624" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>) and Kepler (35 <inline-formula><mml:math id="M625" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula>) radar datasets, and assisted with manuscript proofing. KM supplied the 200 <inline-formula><mml:math id="M626" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar data and applied the necessary corrections for ice crystals, liquid water, and atmospheric attenuation. CDW provided the C081 PICASSO 3 <inline-formula><mml:math id="M627" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> data, corrections for the near-antenna 3 <inline-formula><mml:math id="M628" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> CCREST-M data, 200 <inline-formula><mml:math id="M629" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> processed data, and assisted with manuscript proofing. PGH and the GRaCE team operated the 200 <inline-formula><mml:math id="M630" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar system, provided the datasets to KM and CDW and contributed to manuscript proofing.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d2e8711">The contact author has declared that none of the authors has any competing interests.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <p id="d2e8717">Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this paper. The authors bear the ultimate responsibility for providing appropriate place names. Views expressed in the text are those of the authors and do not necessarily reflect the views of the publisher.</p>
  </notes><ack><title>Acknowledgements</title><p id="d2e8723">The authors would like to thank the crew and personnel involved in the CCREST-M campaign and the Chilbolton Observatory and mini-BASTA radar operators, and the personnel involved in the operation of the 200 <inline-formula><mml:math id="M631" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar at Chilbolton Observatory. The BAe-146 research aircraft is operated by Airtask and Avalon and managed by FAAM. We further thank NCAS for the availability of the 35 <inline-formula><mml:math id="M632" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radar and CNRS, and the LATMOS for providing, operating, and delivering to the Chilbolton Observatory the mini-BASTA radar. Access to the 3 and 35 <inline-formula><mml:math id="M633" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">GHz</mml:mi></mml:mrow></mml:math></inline-formula> radars was provided through the Atmospheric Measurement and Observation Facility (AMOF), part of UKRI-NERC funded National Capability delivered by the National Centre for Atmospheric Science (NCAS).</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d2e8752">This research has been supported by the Met Office, Public Weather Service.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d2e8759">This paper was edited by Chao Liu and reviewed by Haoran Li and one anonymous referee.</p>
  </notes><ref-list>
    <title>References</title>

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