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<article xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:oasis="http://docs.oasis-open.org/ns/oasis-exchange/table" xml:lang="en" dtd-version="3.0" article-type="research-article">
  <front>
    <journal-meta><journal-id journal-id-type="publisher">AMT</journal-id><journal-title-group>
    <journal-title>Atmospheric Measurement Techniques</journal-title>
    <abbrev-journal-title abbrev-type="publisher">AMT</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Meas. Tech.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1867-8548</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/amt-19-4923-2026</article-id><title-group><article-title>Operational performance of the Vaisala CL61 ceilometer for atmospheric profiling</article-title><alt-title>Operational performance of the Vaisala CL61 for atmospheric profiling</alt-title>
      </title-group>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1">
          <name><surname>Le</surname><given-names>Viet</given-names></name>
          <email>viet.le@fmi.fi</email>
        <ext-link>https://orcid.org/0000-0002-9437-1966</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>O'Connor</surname><given-names>Ewan J.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-9834-5100</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Filioglou</surname><given-names>Maria</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-7375-1492</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff3">
          <name><surname>Vakkari</surname><given-names>Ville</given-names></name>
          
        </contrib>
        <aff id="aff1"><label>1</label><institution>Finnish Meteorological Institute, Helsinki, 00101, Finland</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, Kuopio, 70211, Finland</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Atmospheric Chemistry Research Group, Chemical Resource Beneficiation, North-West University, Potchefstroom, 2520, South Africa</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Viet Le (viet.le@fmi.fi)</corresp></author-notes><pub-date><day>30</day><month>July</month><year>2026</year></pub-date>
      
      <volume>19</volume>
      <issue>14</issue>
      <fpage>4923</fpage><lpage>4941</lpage>
      <history>
        <date date-type="received"><day>18</day><month>December</month><year>2025</year></date>
           <date date-type="rev-request"><day>4</day><month>January</month><year>2026</year></date>
           <date date-type="rev-recd"><day>16</day><month>July</month><year>2026</year></date>
           <date date-type="accepted"><day>17</day><month>July</month><year>2026</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2026 Viet Le et al.</copyright-statement>
        <copyright-year>2026</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026.html">This article is available from https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026.html</self-uri><self-uri xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026.pdf">The full text article is available as a PDF file from https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d2e123">The Vaisala CL61 is a new generation elastic backscatter lidar that extends the capabilities of conventional automatic low-power lidars and ceilometers by providing depolarization ratio measurements. Reliable use of these measurements, however, requires thorough evaluation and characterization of the instrument performance and subsequent corrections applied. In this study, performance of multiple CL61 instruments across different sites over 3-year period has been assessed. Results indicate some differences between instruments, with most of these early production units exhibiting a pronounced decrease in laser power over time, accompanied by an increase in background noise likely due to weaker return signals. Normally, the instrument scales the internal calibration factor to compensate for changes in laser power and thus provide consistent attenuated backscatter coefficient values from profile to profile over time. However, for the instrument at the Lindenberg site, by performing manual calibration with atmospheric targets, it is noted that once the laser power dropped below 40 % there is no further compensation in the internal calibration factor.</p>

      <p id="d2e126">The instrumental background noise and bias, characterized using the termination hood, are found to vary with temperature. A method has been developed for correcting the instrumental bias and for estimating the associated uncertainty. Additionally, an approach to estimate the uncertainty of volume and particle backscatter and linear depolarization ratio is presented. In a case study representing low aerosol load conditions in Finland, correcting for the instrumental bias changes the volume linear depolarization ratio by up to 0.005 relative to the instrument-provided values. On the other hand, the difference between volume linear depolarization ratio and particle linear depolarization ratio reached up to 0.1. These findings demonstrate that the CL61 firmware effectively removes the majority of the mean background bias, whereas accounting for the molecular contribution is important for quantitative interpretations of aerosol measurements at CL61's wavelength of 910.55 nm. Finally, signal loss in one unit has been traced to fogging of the inside surface of the window, and attributed to insufficient internal heating linked to the instrument's firmware behavior.</p>
  </abstract>
    
<funding-group>
<award-group id="gs1">
<funding-source>Magnus Ehrnroothin Säätiö</funding-source>
<award-id>n/a</award-id>
</award-group>
<award-group id="gs2">
<funding-source>Research Council of Finland</funding-source>
<award-id>337552</award-id>
<award-id>343359</award-id>
</award-group>
</funding-group>
</article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d2e138">Automatic low-power lidars and ceilometers (ALC) are ground-based elastic backscatter lidars originally developed for the automated detection of cloud base height to support aviation and meteorological operations. Over the past 2 decades, advancements in both hardware and data processing have greatly enhanced their capabilities <xref ref-type="bibr" rid="bib1.bibx10" id="paren.1"/>. Notably, improvements in signal quality, particularly in signal-to-noise ratio, now enable ALC to provide profiles of attenuated backscatter coefficient with sufficient dynamic range to permit the observation of a wide range of atmospheric phenomena, including rainfall <xref ref-type="bibr" rid="bib1.bibx37 bib1.bibx38" id="paren.2"><named-content content-type="pre">e.g.</named-content></xref>, fog <xref ref-type="bibr" rid="bib1.bibx18 bib1.bibx36" id="paren.3"><named-content content-type="pre">e.g.</named-content></xref>, icing <xref ref-type="bibr" rid="bib1.bibx22" id="paren.4"><named-content content-type="pre">e.g.</named-content></xref>, and even the quantitative estimation of aerosol concentrations <xref ref-type="bibr" rid="bib1.bibx40 bib1.bibx14" id="paren.5"><named-content content-type="pre">e.g.</named-content></xref>. ALC data are also increasingly used to estimate atmospheric boundary layer height <xref ref-type="bibr" rid="bib1.bibx27" id="paren.6"><named-content content-type="pre">e.g.</named-content></xref>, which is a critical parameter for numerical weather prediction and air quality models <xref ref-type="bibr" rid="bib1.bibx43 bib1.bibx3" id="paren.7"><named-content content-type="pre">e.g.</named-content></xref>. Their ability to operate autonomously and reliably in challenging environmental conditions, as well as being eye-safe, makes them well-suited for long-term monitoring and integration into operational networks of national meteorological services and research institutions <xref ref-type="bibr" rid="bib1.bibx20" id="paren.8"><named-content content-type="pre">e.g.</named-content></xref>. Many such organizations are actively investigating the use of ALC profile data to improve forecast model performance <xref ref-type="bibr" rid="bib1.bibx46 bib1.bibx24" id="paren.9"><named-content content-type="pre">e.g.</named-content></xref>.</p>
      <p id="d2e185">Vaisala has recently introduced the CL61 ceilometer, which is an ALC with the capability of measuring the volume linear depolarization ratio <inline-formula><mml:math id="M1" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. It is the ratio of the perpendicular to the parallel component of the backscattered signal relative to the emitted polarization. This ratio provides insight into particle sphericity <xref ref-type="bibr" rid="bib1.bibx7 bib1.bibx30 bib1.bibx2" id="paren.10"><named-content content-type="pre">e.g.</named-content></xref> and is essential for distinguishing various aerosol types <xref ref-type="bibr" rid="bib1.bibx23 bib1.bibx33 bib1.bibx15 bib1.bibx13 bib1.bibx28" id="paren.11"><named-content content-type="pre">e.g.</named-content></xref> such as pollen, smoke, dust, marine, and volcanic ash. It is also utilized in determining cloud phase <xref ref-type="bibr" rid="bib1.bibx39" id="paren.12"/> and in the retrieval of cloud microphysical properties <xref ref-type="bibr" rid="bib1.bibx11" id="paren.13"/>.</p>
      <p id="d2e215">To fully leverage the broad range of applications enabled by the CL61, including its new capability to measure <inline-formula><mml:math id="M2" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, careful quality control of the backscattered signal from both polarizations is essential. Environmental conditions, such as temperature and relative humidity, can influence lidar performance <xref ref-type="bibr" rid="bib1.bibx8" id="paren.14"/>, making it necessary to assess their impact on data quality. For instance, <xref ref-type="bibr" rid="bib1.bibx19" id="text.15"/> identified and corrected a temperature-dependent effect on the overlap function of a Lufft CHM15K ceilometer, which arises from temperature-induced changes in the laser as well as in the instrument's optical and electronic components. Similarly, the older Vaisala CL31 ceilometer has been known to have backscatter artifacts below approximately 70 m <xref ref-type="bibr" rid="bib1.bibx44 bib1.bibx31 bib1.bibx42" id="paren.16"/>, prompting many studies to omit these near-surface measurements. Identifying and correcting such artifacts in the CL61 would enable reliable observations extending down to heights that overlap with surface-based observations. This capability is especially valuable for studying near-surface meteorological phenomena such as fog, haze, and emissions from ground-level aerosol sources.</p>
      <p id="d2e238">In this study, we present a long-term evaluation of the CL61 ceilometers conducted at four different ACTRIS cloud profiling sites in Finland and Germany. Our analysis focuses on the impact of laser power on signal quality, the temperature sensitivity of the instrumental background and methods for its correction. Additionally, we demonstrate our calculation of the uncertainty in the volume and particle linear depolarization ratio (<inline-formula><mml:math id="M3" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M4" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> respectively). Finally, we report instances of signal loss attributed to fogging of the inside surface of the window, observed in some of the CL61 units.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Instrument description</title>
      <p id="d2e271">The CL61 ceilometer, manufactured by Vaisala, is a coaxial ALC system operating at a wavelength of 910.55 nm and equipped with depolarization measurement capability. Its key technical specifications are summarized in Table <xref ref-type="table" rid="T1"/>. In brief, the CL61 utilizes an InGaAs diode laser that emits linearly polarized pulses with an energy of 3.9 <inline-formula><mml:math id="M5" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">J</mml:mi></mml:mrow></mml:math></inline-formula> at a repetition rate of 9.5 kHz. The instrument features a single-lens optical design and performs depolarization measurements using a single-receiver with an avalanche photodiode (APD) detector that switches between two polarizing filters (one perpendicular and one parallel to the polarization of the transmitted pulses) in the same coaxial optical path. The CL61 alternates the acquisition of each polarization every 0.2 s, while using the same receiver module for both channels. Consequently, receiver sensitivity calibration is not required. The maximum detection range of CL61 is 15.4 km.</p>

<table-wrap id="T1" specific-use="star"><label>Table 1</label><caption><p id="d2e289">Specifications of the CL61 (CL61 User Guide: <uri>https://docs.vaisala.com/r/M212475EN-E/en-US</uri>, last access: 21 July 2025).</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="2">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Specification</oasis:entry>
         <oasis:entry colname="col2">Values</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">Laser wavelength</oasis:entry>
         <oasis:entry colname="col2">910.55 nm</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Laser</oasis:entry>
         <oasis:entry colname="col2">InGaAs diode</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Beam divergence</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M6" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.2</mml:mn></mml:mrow></mml:math></inline-formula> mrad <inline-formula><mml:math id="M7" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M8" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.35</mml:mn></mml:mrow></mml:math></inline-formula> mrad</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Receiver field-of-view</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M9" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.56</mml:mn></mml:mrow></mml:math></inline-formula> mrad</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Measurement maximum range</oasis:entry>
         <oasis:entry colname="col2">15 400 m</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Reporting range resolution</oasis:entry>
         <oasis:entry colname="col2">4.8 m</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Measurement interval</oasis:entry>
         <oasis:entry colname="col2">5 s</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Pulse duration</oasis:entry>
         <oasis:entry colname="col2">160 ns (at Full Width Half Maximum)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Pulse frequency</oasis:entry>
         <oasis:entry colname="col2">9.5 kHz</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Maximum pulse energy</oasis:entry>
         <oasis:entry colname="col2">4.7 <inline-formula><mml:math id="M10" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">J</mml:mi></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Height of complete overlap</oasis:entry>
         <oasis:entry colname="col2">250 m (in Kenttärova) and 550 m (in Vehmasmäki and Hyytiälä)</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d2e463">The overlap functions reported by the manufacturer are shown in Fig. S1 in the Supplement. Full overlap between the transmitted laser beam and the receiver field of view is achieved at approximately 250 m range for the instrument at Kenttärova. The instruments at Vehmasmäki and Hyytiälä have different overlap functions, with approximately 95 % overlap at 250 m range and complete overlap at approximately 550 m range. The overlap function is reported only in the new firmware (version 1.2.7), and no overlap function has been reported for the instrument at Lindenberg. Although the overlap function might change during operation, for example due to temperature variations <xref ref-type="bibr" rid="bib1.bibx19" id="paren.17"/>, the overlap correction applied to the data reported by the CL61 remains constant.</p>
      <p id="d2e470">Data collected up to December 2024 from four CL61 deployed at four different ACTRIS Cloudnet sites were analyzed. Three of these instruments are situated in Finland: Hyytiälä, Vehmasmäki, and Kenttärova, while the fourth is located in Lindenberg, Germany. The firmware versions of the instruments (i.e., 1.1.10 and 1.2.7), along with their respective periods of validity, are presented in Table <xref ref-type="table" rid="T2"/>. The data from this study were obtained from the ACTRIS Cloudnet data portal <xref ref-type="bibr" rid="bib1.bibx17" id="paren.18"/>.</p>

<table-wrap id="T2"><label>Table 2</label><caption><p id="d2e481">Firmware version of the CL61 across all the site locations.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:thead>
       <oasis:row>

         <oasis:entry colname="col1">Site and coordinate</oasis:entry>

         <oasis:entry colname="col2">Time</oasis:entry>

         <oasis:entry colname="col3">Firmware</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"/>

         <oasis:entry colname="col2"/>

         <oasis:entry colname="col3">version</oasis:entry>

       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>

         <oasis:entry colname="col1">Vehmasmäki</oasis:entry>

         <oasis:entry colname="col2">2022-01-01 to 2022-06-14</oasis:entry>

         <oasis:entry colname="col3">not stated</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">62.738° N, 27.543° E</oasis:entry>

         <oasis:entry colname="col2">2022-06-15 to 2023-04-27</oasis:entry>

         <oasis:entry colname="col3">1.1.10</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"/>

         <oasis:entry colname="col2">2023-04-28 to 2024-12-31</oasis:entry>

         <oasis:entry colname="col3">1.2.7</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">Hyytiälä</oasis:entry>

         <oasis:entry colname="col2">2022-01-01 to 2022-11-20</oasis:entry>

         <oasis:entry colname="col3">not stated</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">61.844° N, 24.287° E</oasis:entry>

         <oasis:entry colname="col2">2022-11-21 to 2023-11-22</oasis:entry>

         <oasis:entry colname="col3">1.1.10</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"/>

         <oasis:entry colname="col2">2023-11-23 to 2024-12-31</oasis:entry>

         <oasis:entry colname="col3">1.2.7</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">Kenttärova</oasis:entry>

         <oasis:entry colname="col2">2022-01-01 to 2022-06-20</oasis:entry>

         <oasis:entry colname="col3">not stated</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1">67.987° N, 24.243° E</oasis:entry>

         <oasis:entry colname="col2">2022-06-21 to 2024-12-31</oasis:entry>

         <oasis:entry colname="col3">1.2.7</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">Lindenberg</oasis:entry>

         <oasis:entry colname="col2" morerows="1">2024-03-01 to 2024-12-31</oasis:entry>

         <oasis:entry colname="col3" morerows="1">1.1.10</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">52.208° N, 14.118° E</oasis:entry>

       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d2e636">The CL61 is equipped with an internal heater to stabilize the temperatures of the laser and optical components. It includes a window heater and blower to maintain stable window conditions, as the window's transmission efficiency significantly affects the backscattered signal (see Sect. 4.3). The instrument's firmware continuously monitors and reports various housekeeping variables, such as internal temperature, laser temperature, window condition (calculated internally on a scale from 0 % for a fully obstructed window to 100 % for a clean window), and the status of the window blower heater. The quantity and type of variables reported may differ based on the firmware version.</p>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Methods</title>
      <p id="d2e648">The CL61 operates by emitting pulses of linear polarized laser light into the atmosphere and recording the backscattered signal. The received power per laser pulse is described by the lidar equation <xref ref-type="bibr" rid="bib1.bibx45" id="paren.19"/>:

          <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M11" display="block"><mml:mrow><mml:mi>P</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="italic">β</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:msubsup><mml:mo>∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi>r</mml:mi></mml:msubsup><mml:mi mathvariant="italic">α</mml:mi><mml:mo>(</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>)</mml:mo><mml:mi mathvariant="normal">d</mml:mi><mml:msup><mml:mi>r</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msup><mml:mo>+</mml:mo><mml:mi>B</mml:mi><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

        Here, <inline-formula><mml:math id="M12" display="inline"><mml:mrow><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is the overlap function that is unique to each instrument and is provided by the manufacturer. The coefficients <inline-formula><mml:math id="M13" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M14" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula> represent atmospheric extinction and backscatter, respectively, <inline-formula><mml:math id="M15" display="inline"><mml:mi>B</mml:mi></mml:math></inline-formula> is the background signal, and <inline-formula><mml:math id="M16" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> represents the lidar constant. This constant encapsulates the system-specific characteristics of the lidar, such as its receiver optics and laser properties. It is initially determined and provided by the manufacturer, but it may drift over time as the instrument ages and its performance changes. Although the internal firmware attempts to monitor and compensate for these changes, additional calibration, such as absolute calibration using stratocumulus clouds <xref ref-type="bibr" rid="bib1.bibx35 bib1.bibx21" id="paren.20"/>, is still necessary.</p>
      <p id="d2e791">The instrument provides two main output signals, ppol and xpol, in arbitrary units [a.u.], as they are reported prior to absolute calibration. These paremters represent the estimated normalized and background-, range- and overlap-corrected parallel- and cross-polarized components of the attenuated backscattered signal (<inline-formula><mml:math id="M17" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M18" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> respectively). They can be defined as:

              <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M19" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E2"><mml:mtd><mml:mtext>2</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mtext>ppol</mml:mtext><mml:msup><mml:mo>=</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>(</mml:mo><mml:mi>P</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">estimated</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo>=</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E3"><mml:mtd><mml:mtext>3</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mtext>xpol</mml:mtext><mml:msup><mml:mo>=</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mfenced open="(" close=")"><mml:mrow><mml:mi>P</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">estimated</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo>=</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

        where <inline-formula><mml:math id="M20" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">estimated</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the internally estimated background signal by the instrument. The instrument also provides the total attenuated backscatter signal, which is the sum of the attenuated backscatter from all polarizations:

          <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M21" display="block"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msup><mml:mo>=</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msup><mml:mo>+</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

        and the volume linear depolarization ratio being:

          <disp-formula id="Ch1.E5" content-type="numbered"><label>5</label><mml:math id="M22" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>Residual background signal</title>
      <p id="d2e1051">The observed backscattered signal detected by a lidar consists of the true atmospheric signal and the background signal <xref ref-type="bibr" rid="bib1.bibx9" id="paren.21"/>. The true atmospheric signal consists of backscattered contributions from particles (<inline-formula><mml:math id="M23" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and molecular scattering (<inline-formula><mml:math id="M24" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">mol</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), whilst the background signal includes contributions from both atmospheric background signal <inline-formula><mml:math id="M25" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (such as solar radiation, moonlight, or artificial light) and instrumental background <inline-formula><mml:math id="M26" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> signal (dark signal). Although the instrument already determines and performs the background correction internally, residual background components may still remain in the measured signal, such as the dark signal observed during termination hood measurements (see Sect. 3.1.1). Therefore, we extend Eqs. (2) and (3) to account for the residual background signal (hereafter referred to as the background signal), <inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, that is not removed by the internal correction:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M28" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E6"><mml:mtd><mml:mtext>6</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mtable rowspacing="0.2ex" class="split" displaystyle="true" columnalign="right left"><mml:mtr><mml:mtd><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msup><mml:mo>=</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>(</mml:mo><mml:mi>P</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">estimated</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo>+</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msup><mml:mo>=</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:msup><mml:mo>+</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E7"><mml:mtd><mml:mtext>7</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mtable class="split" rowspacing="0.2ex" displaystyle="true" columnalign="right left"><mml:mtr><mml:mtd><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msup><mml:mo>=</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>(</mml:mo><mml:mi>P</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">estimated</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo>+</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msup><mml:mo>=</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:msup><mml:mo>+</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

          To eliminate the range dependence from the background terms, we divide each expression by <inline-formula><mml:math id="M29" display="inline"><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>, yielding:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M30" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E8"><mml:mtd><mml:mtext>8</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo>+</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E9"><mml:mtd><mml:mtext>9</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo>+</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

          For simplicity, we define the background terms as:

            <disp-formula id="Ch1.E10" content-type="numbered"><label>10</label><mml:math id="M31" display="block"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mo>≡</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          where <inline-formula><mml:math id="M32" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M33" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M34" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo><mml:mo>+</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d2e1730">To derive the <inline-formula><mml:math id="M35" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>, the background signals need to be quantified. Since the measured <inline-formula><mml:math id="M36" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> signals include contributions from background signal in their respective polarization channels, it is necessary to estimate the background signal separately for each polarization (<inline-formula><mml:math id="M38" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M39" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). To achieve this, a background identification methodology has been developed. It identifies regions within the dataset that are free of aerosols and hydrometeors, where the <inline-formula><mml:math id="M40" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle></mml:math></inline-formula> and <inline-formula><mml:math id="M41" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle></mml:math></inline-formula> values are assumed to predominantly represent background signal.</p>
      <p id="d2e1853">The methodology proceeds as follows. First, the data is averaged over 5 min intervals. The <inline-formula><mml:math id="M42" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle></mml:math></inline-formula> and <inline-formula><mml:math id="M43" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle></mml:math></inline-formula> profiles are then decomposed using the stationary wavelet transform (SWT) with the bior.1 wavelet, implemented via PyWavelets <xref ref-type="bibr" rid="bib1.bibx32 bib1.bibx29" id="paren.22"/>. Subsequently, the background signal variance is reduced by applying a hard-threshold shrinkage function to the approximation and detail coefficients from levels <inline-formula><mml:math id="M44" display="inline"><mml:mn mathvariant="normal">1</mml:mn></mml:math></inline-formula> through <inline-formula><mml:math id="M45" display="inline"><mml:mn mathvariant="normal">7</mml:mn></mml:math></inline-formula>, using minimax thresholding <xref ref-type="bibr" rid="bib1.bibx32" id="paren.23"/>. The profile is reconstructed via the inverse stationary wavelet transform. Finally, the background range gates are identified as regions with values below half of the previously computed minimax threshold. The mean and variance of the background are computed from the original, non-averaged data with the identified background range gates using 5 min time intervals and 2 km range-bin intervals.</p>
      <p id="d2e1923">An example of this methodology applied to data in Kenttärova on 28 March 2024 is illustrated in Fig. <xref ref-type="fig" rid="F1"/>. During daylight hours, solar radiation significantly increases the variance (<inline-formula><mml:math id="M46" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M47" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>) of the background signal, resulting in a daytime variance much higher than that observed at night, as shown in panels (g) and (h). Above the aerosol and cloud layers, both the mean (<inline-formula><mml:math id="M48" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M49" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>) and variance of the background signals in both polarizations remain relatively stable with range, or at least exhibit considerably smaller variations compared to the diurnal fluctuations.</p>

      <fig id="F1" specific-use="star"><label>Figure 1</label><caption><p id="d2e2012">Time series from Kenttärova on 28 March 2024 showing: <bold>(a)</bold> <inline-formula><mml:math id="M50" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M51" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> background <inline-formula><mml:math id="M52" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, and <bold>(d)</bold> background <inline-formula><mml:math id="M53" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>. Panels <bold>(e)</bold> to <bold>(h)</bold> display the background at different range bins from 4000 to 6000, 6000 to 8000, 8000 to 10 000, 10 000 to 12 000, and 12 000 to 14 000 m, with color indicating the range bin: <bold>(e)</bold> <inline-formula><mml:math id="M54" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(f)</bold> <inline-formula><mml:math id="M55" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(g)</bold> <inline-formula><mml:math id="M56" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, and <bold>(h)</bold> <inline-formula><mml:math id="M57" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. These parameters are computed at a 10 s temporal resolution using all data within each range bin.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f01.png"/>

        </fig>

      <p id="d2e2194">By applying this methodology to the full dataset, we obtained the time series of <inline-formula><mml:math id="M58" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for all instruments in both polarizations. Comparing these background signals with other housekeeping parameters, such as laser power, enables us to evaluate the operational performance of each instrument. Moreover, since each background component is quantified independently, we can correct the signal and estimate its uncertainty in both polarizations <inline-formula><mml:math id="M59" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M60" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> and, consequently, in the derived linear depolarization ratio.</p>
<sec id="Ch1.S3.SS1.SSS1">
  <label>3.1.1</label><title>Instrumental background signal</title>
      <p id="d2e2245">To obtain the instrumental background signal, a termination hood (Vaisala CL61TERMHOOD) was placed over the window of each ceilometer located in Finland (Fig. <xref ref-type="fig" rid="F2"/>). The hood was applied without modifying the instrument's internal operating parameters, ensuring that all measurements reflected normal operational conditions. The hood's material and design totally attenuate the outgoing laser beam, preventing any backscatter signal from reaching the detector. As a result, the measured signal can be attributed entirely to the instrumental background signal adjusted by the overlap correction. Although the overlap correction remains constant for each instrument, it was reverted to accurately interpret the instrumental background signal in the near range <inline-formula><mml:math id="M61" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>.</p>

      <fig id="F2"><label>Figure 2</label><caption><p id="d2e2271">A termination hood (Vaisala CL61TERMHOOD) place on top of the CL61 in Hyytiälä.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f02.jpg"/>

          </fig>

      <p id="d2e2280">Figure <xref ref-type="fig" rid="F3"/> presents example profiles of <inline-formula><mml:math id="M62" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> both before and during the termination hood measurements. Before the termination hood was applied, the <inline-formula><mml:math id="M64" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> profiles in the aerosol and hydrometeor-free region above 5 km closely follow the theoretical molecular attenuated backscatter coefficient <inline-formula><mml:math id="M66" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">mol</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> (Fig. <xref ref-type="fig" rid="F3"/>b and c), indicating that the CL61 is sensitive to molecular scattering. The <inline-formula><mml:math id="M67" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">mol</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> profile was calculated following the method described by <xref ref-type="bibr" rid="bib1.bibx6" id="text.24"/> using meteorological input data from a numerical weather prediction model available from the ACTRIS Cloudnet data portal <xref ref-type="bibr" rid="bib1.bibx34" id="paren.25"/>. At ranges above 10 km, however, the molecular signal becomes indistinguishable from noise. The variance profiles, <inline-formula><mml:math id="M68" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>/</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M69" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>/</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, also remain relatively constant in this region (Fig. <xref ref-type="fig" rid="F3"/>f and g).</p>

      <fig id="F3" specific-use="star"><label>Figure 3</label><caption><p id="d2e2450">Measurements at Kenttärova on 5 March 2024. <bold>(a)</bold> The time series of <inline-formula><mml:math id="M70" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>. Panels <bold>(b)</bold>, <bold>(c)</bold>, <bold>(f)</bold>, and <bold>(g)</bold> display the averaged profiles in time at each range gate before the termination hood measurement (from 11:00 to 13:00 UTC): <bold>(b)</bold> <inline-formula><mml:math id="M71" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M72" display="inline"><mml:mrow><mml:mo>∥</mml:mo><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">mol</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M73" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M74" display="inline"><mml:mrow><mml:mo>⟂</mml:mo><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">mol</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(f)</bold> <inline-formula><mml:math id="M75" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>/</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(g)</bold> <inline-formula><mml:math id="M76" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>/</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. Panels <bold>(d)</bold>, <bold>(e)</bold>, <bold>(h)</bold> and <bold>(i)</bold> display the averaged profiles in time at each range gate during the termination hood measurement at 19 °C (from 14:00 to 15:00 UTC): <bold>(d)</bold> <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(e)</bold> <inline-formula><mml:math id="M78" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(h)</bold> <inline-formula><mml:math id="M79" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(i)</bold> <inline-formula><mml:math id="M80" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f03.png"/>

          </fig>

      <p id="d2e2765">During the termination hood measurement, <inline-formula><mml:math id="M81" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> from both polarizations remains relatively stable above 1.2 km, but increases significantly below this range (Fig. <xref ref-type="fig" rid="F3"/>d, e). This increase suggests the presence of a signal bias at lower ranges that has not been corrected by the firmware and will be investigated in this study. Additionally, a reduction in the signal variance of both polarization channels is observed during the termination hood measurement (Fig. <xref ref-type="fig" rid="F3"/>h, i) compared to the previous period above the complete overlap range. This reduction is attributed to the absence of solar influence during the termination hood measurement.</p>
      <p id="d2e2795">In principle, the nighttime measurements could be used to estimate <inline-formula><mml:math id="M82" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. However, only the portion of the <inline-formula><mml:math id="M83" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> profile at higher ranges, where clouds and aerosols are absent, can be reliably estimated. An example is shown in Fig. S2, where <inline-formula><mml:math id="M84" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>/</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> agrees well between the hood termination and nighttime measurements only at ranges above approximately 2 km. This agreement is observed only under clear-sky conditions, as cloud layers at lower ranges can increase the measured background values.</p>
      <p id="d2e2848">Since the CL61 is a coaxial lidar, it is prone to the afterpulsing effect, such as those caused by internal reflections of the outgoing laser beam that reach the detector <xref ref-type="bibr" rid="bib1.bibx8 bib1.bibx47" id="paren.26"/>. <xref ref-type="bibr" rid="bib1.bibx19" id="text.27"/> demonstrated that the overlap function for a ceilometer made by another manufacturer (Lufft CHM15k) was sensitive to the instrument internal temperature, <inline-formula><mml:math id="M85" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>, mainly due to temperature-induced changes in its optical components. It is likely that the observed bias is temperature-dependent and is caused by variations in instrumental background associated with afterpulsing, dark signal, and optical components under different temperature conditions. To quantify the effect of temperature, the termination hood measurement was repeated over a range of internal temperatures <inline-formula><mml:math id="M86" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>, reported as <monospace>internal_temperature</monospace> in the instrument housekeeping data, across a two-year period. Hence, the instrumental background signal mean (bias) and its variance (noise) from both polarizations with respect to internal temperature can be determined.</p>
</sec>
<sec id="Ch1.S3.SS1.SSS2">
  <label>3.1.2</label><title>Atmospheric background signal</title>
      <p id="d2e2882">For an accurate estimation of the background signal, the contribution from the atmospheric background signal, <inline-formula><mml:math id="M87" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, must be taken into account. As noted by <xref ref-type="bibr" rid="bib1.bibx26" id="text.28"/>, earlier instruments such as the CL31 incorporate a zero-bias level that compensates for temporal fluctuations in solar radiation. This is also evident in CL61 as shown in Fig. <xref ref-type="fig" rid="F3"/>b and c, where the <inline-formula><mml:math id="M88" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M89" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> values above 5 km closely follow <inline-formula><mml:math id="M90" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">mol</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, confirming the zero-mean solar radiation noise. Therefore, the firmware must have corrected the atmospheric background signal to a zero mean, leaving only its variance (noise) contributing to the background signal, which will be addressed in this study.</p>
      <p id="d2e2951">The solar noise variance can be seen from the diurnal pattern in Fig. <xref ref-type="fig" rid="F1"/>g and h; and the difference between the <inline-formula><mml:math id="M91" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">σ</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> profiles before (Fig. <xref ref-type="fig" rid="F3"/>f and g) and during (Fig. <xref ref-type="fig" rid="F3"/>h and i) the termination hood measurement. Since this difference remains approximately constant at all ranges above the aerosol layer near the ground, we assume that the atmospheric background variance from both polarizations, <inline-formula><mml:math id="M92" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, is also uniform down to the near range. Then, <inline-formula><mml:math id="M93" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> is calculated by computing the difference between the variance of the background signal <inline-formula><mml:math id="M94" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> (obtained between 10 and 12 km using the background identification methodology) and the variance of the instrumental background signal <inline-formula><mml:math id="M95" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> (obtained at the same range and temperature from the termination hood measurement):

              <disp-formula id="Ch1.E11" content-type="numbered"><label>11</label><mml:math id="M96" display="block"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">res</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mo>-</mml:mo><mml:mn mathvariant="normal">12</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>-</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mo>-</mml:mo><mml:mn mathvariant="normal">12</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

            Here, <inline-formula><mml:math id="M97" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> is independent of the range and is obtained separately for each polarization in each individual profile.</p>
</sec>
<sec id="Ch1.S3.SS1.SSS3">
  <label>3.1.3</label><title>Correction for systematic bias</title>
      <p id="d2e3151">After measuring <inline-formula><mml:math id="M98" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> across a range of <inline-formula><mml:math id="M99" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> during the termination hood measurements, the results are stored as a lookup table containing <inline-formula><mml:math id="M100" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> profiles at each <inline-formula><mml:math id="M101" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>. The attenuated backscatter coefficient for each polarization can be corrected by applying the <inline-formula><mml:math id="M102" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> value corresponding to the instrument's current internal temperature as follows:

                  <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M103" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E12"><mml:mtd><mml:mtext>12</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:msup><mml:mo>=</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E13"><mml:mtd><mml:mtext>13</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:msup><mml:mo>=</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            and their corresponding uncertainties are given by:

                  <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M104" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E14"><mml:mtd><mml:mtext>14</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>+</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:mfenced><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E15"><mml:mtd><mml:mtext>15</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:mo>(</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>+</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>)</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula></p>
      <p id="d2e3517">The bias-corrected attenuated backscatter coefficient and volume linear depolarization ratio are then calculated as:

                  <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M105" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E16"><mml:mtd><mml:mtext>16</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:msup><mml:mo>=</mml:mo><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:msup><mml:mo>+</mml:mo><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E17"><mml:mtd><mml:mtext>17</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            and their associated uncertainty, given by

                  <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M106" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E18"><mml:mtd><mml:mtext>18</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>+</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E19"><mml:mtd><mml:mtext>19</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:msup><mml:mi mathvariant="italic">δ</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>+</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mfenced><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula></p>
</sec>
</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>Calibration</title>
      <p id="d2e3783">To ensure the CL61 produces a consistent and accurate backscatter signal, the ceilometer signal must be manually calibrated in addition to its internal calibration. This involves calibrating the backscatter signal from the CL61 using a reference target with known backscatter characteristics. Two commonly used calibration methods for deriving <inline-formula><mml:math id="M107" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are based on different types of reference targets: atmospheric molecules (Rayleigh calibration) and liquid clouds (liquid cloud calibration).</p>
      <p id="d2e3797">The Rayleigh calibration <xref ref-type="bibr" rid="bib1.bibx12 bib1.bibx25 bib1.bibx5 bib1.bibx48 bib1.bibx1" id="paren.29"/>, often referred to as the backward inversion approach, is the standard method to derive the particle backscatter coefficient (<inline-formula><mml:math id="M108" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for most research aerosol lidars due to their sensitivity to molecular signal <xref ref-type="bibr" rid="bib1.bibx49" id="paren.30"/>. As illustrated in Fig. <xref ref-type="fig" rid="F3"/>b, the attenuated backscatter coefficient profile from CL61 closely follows the attenuated molecular backscatter coefficient above the aerosol layer at 4 km. This indicates a significant contribution of molecular scattering to the total CL61 signal, especially in aerosol- and hydrometeor-free regions. Therefore, the Rayleigh calibration can be applied to the CL61, provided a sufficiently long averaging time (more than 2 h) is used.</p>
      <p id="d2e3819">The Rayleigh calibration method requires an assumed lidar ratio for aerosol particles (<inline-formula><mml:math id="M109" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). At sites equipped with a sun photometer, <inline-formula><mml:math id="M110" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> can be constrained <xref ref-type="bibr" rid="bib1.bibx48" id="paren.31"/>; otherwise, a value of 50 sr was used. The first 50 m range has been discarded due to unreliable data (see Sect. 4.5), and it has been demonstrated that the resulting loss in optical depth for ignoring near range gates is negligible <xref ref-type="bibr" rid="bib1.bibx48" id="paren.32"/>. After the <inline-formula><mml:math id="M111" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> profile is derived, the lidar constant <inline-formula><mml:math id="M112" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> can be determined from the lidar equation <xref ref-type="bibr" rid="bib1.bibx48" id="paren.33"/>.</p>
      <p id="d2e3876">The liquid cloud calibration <xref ref-type="bibr" rid="bib1.bibx35 bib1.bibx21" id="paren.34"/> relies on the fact that the lidar ratio for liquid water clouds at the ceilometer wavelength is known. This method involves calculating the integrated attenuated backscatter coefficient for fully attenuated liquid water clouds, including the contribution from multiple scattering. The theoretical contribution from multiple scattering is computed for droplet diameters ranging from 8 to 20 <inline-formula><mml:math id="M113" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>, taking into account the CL61 beam divergence and receiver field of view. The integrated backscatter coefficient is then scaled to fit within the expected theoretical values. This scaling factor is the calibration factor <inline-formula><mml:math id="M114" display="inline"><mml:mi>C</mml:mi></mml:math></inline-formula>, which is the reciprocal of the lidar constant <inline-formula><mml:math id="M115" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">L</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The primary advantage of this approach over Rayleigh calibration is the substantially higher signal-to-noise ratio of the backscatter from water clouds compared to the molecular backscatter. As a result, it eliminates the need for long nighttime averaging periods required to obtain a reliable molecular signal.</p>
      <p id="d2e3911">A methodology was developed to identify suitable liquid cloud profiles. First, a representative liquid cloud profile containing a single liquid cloud layer and exhibiting complete signal attenuation approximately 200 m above the cloud base was selected as the reference profile. Each <inline-formula><mml:math id="M116" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> profile in the dataset was then cross-correlated with this reference to quantify their similarity. For each time step, the height corresponding to the maximum cross-correlation value was identified as the most similar location and treated as a pseudo in-cloud height. Next, the ratio of total in-cloud <inline-formula><mml:math id="M117" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, calculated over a 150 m layer centered at the pseudo in-cloud height, to the integrated <inline-formula><mml:math id="M118" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> of the entire profile was computed. A profile was classified as containing a liquid cloud if this ratio exceeded 90 %, ensuring that the integrated <inline-formula><mml:math id="M119" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> was not significantly influenced by strong aerosol loading or precipitation. Additionally, the cross-correlation value at the identified height was required to exceed 5 <inline-formula><mml:math id="M120" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<sup>−7</sup>. This threshold was selected to ensure that at least 1000 valid data points were available for each month.</p>
      <p id="d2e3978">To ensure robust data fitting, the cloud calibration is performed monthly using all suitable liquid cloud observations detected from the methodology. To validate the cloud calibration results, Rayleigh calibration was also computed occasionally when possible. Data from a co-located sun photometer was used to constrain the lidar ratio for Rayleigh calibration. If no sun photometer data is available, a lidar ratio of 50 sr is used.</p>
      <p id="d2e3981">The calibrated volume attenuated backscatter coefficient and its uncertainty can then be determined as follows, assuming the cloud calibration factor has an uncertainty of approximately 10 % <xref ref-type="bibr" rid="bib1.bibx21" id="paren.35"/>:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M122" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E20"><mml:mtd><mml:mtext>20</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>=</mml:mo><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>⋅</mml:mo><mml:mi>C</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E21"><mml:mtd><mml:mtext>21</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:mfenced open="(" close=")"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.01</mml:mn><mml:mo>⋅</mml:mo><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:mfenced><mml:mo>⋅</mml:mo><mml:msup><mml:mi>C</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula></p>
      <p id="d2e4083">For those instruments where termination hood measurements are not available:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M123" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E22"><mml:mtd><mml:mtext>22</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>=</mml:mo><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>⋅</mml:mo><mml:mi>C</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E23"><mml:mtd><mml:mtext>23</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mtable rowspacing="0.2ex" class="split" displaystyle="true" columnalign="right left"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>=</mml:mo><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.01</mml:mn><mml:mo>⋅</mml:mo><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mfenced><mml:mo>⋅</mml:mo><mml:msup><mml:mi>C</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>=</mml:mo><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>+</mml:mo><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">atmosphere</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.01</mml:mn><mml:mo>⋅</mml:mo><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mfenced><mml:mo>⋅</mml:mo><mml:msup><mml:mi>C</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula></p>
      <p id="d2e4245">The calibration is assumed to affect both polarization channels equally. Hence, <inline-formula><mml:math id="M124" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> remains unchanged.</p>
</sec>
<sec id="Ch1.S3.SS3">
  <label>3.3</label><title>Aerosol particle inversion</title>
      <p id="d2e4268">The particle backscatter coefficient profile (<inline-formula><mml:math id="M125" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is retrieved using the forward Klett solution <xref ref-type="bibr" rid="bib1.bibx25" id="paren.36"/> after applying the previously derived cloud calibration factor and assuming that the instrument does not undergo significant degradation within a one-month period. Similar to the previous section, the first <inline-formula><mml:math id="M126" display="inline"><mml:mrow><mml:mn mathvariant="normal">50</mml:mn><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> range has been discarded. The cloud calibration factor is estimated to have an uncertainty of approximately 10 % <xref ref-type="bibr" rid="bib1.bibx21" id="paren.37"/>. The forward inversion does not require extensive temporal averaging. When available, sun photometer observations are used to constrain the lidar ratio <inline-formula><mml:math id="M127" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; otherwise, a constant value of 50 sr is applied to all aerosol layers in the retrieval.</p>
      <p id="d2e4310">Let <inline-formula><mml:math id="M128" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>f</mml:mi><mml:mo>(</mml:mo><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>,</mml:mo><mml:mi>C</mml:mi><mml:mo>,</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> represent the inversion function; then the uncertainty of <inline-formula><mml:math id="M129" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is calculated as

            <disp-formula id="Ch1.E24" content-type="numbered"><label>24</label><mml:math id="M130" display="block"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>f</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>f</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>C</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi>C</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>f</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>S</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>
      <p id="d2e4469">The partial derivatives can be approximated using central differences:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M131" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E25"><mml:mtd><mml:mtext>25</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>f</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:msub><mml:mo>≈</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi>f</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:msub><mml:mo>,</mml:mo><mml:mi>C</mml:mi><mml:mo>,</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mfenced open="(" close=")"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:msub><mml:mo>,</mml:mo><mml:mi>C</mml:mi><mml:mo>,</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E26"><mml:mtd><mml:mtext>26</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>f</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>C</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi>C</mml:mi></mml:msub><mml:mo>≈</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi>f</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>,</mml:mo><mml:msub><mml:mi>C</mml:mi><mml:mo>max⁡</mml:mo></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mfenced open="(" close=")"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>,</mml:mo><mml:msub><mml:mi>C</mml:mi><mml:mo>min⁡</mml:mo></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E27"><mml:mtd><mml:mtext>27</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>f</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>S</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:msub><mml:mo>≈</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi>f</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>,</mml:mo><mml:mi>C</mml:mi><mml:mo>,</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mrow><mml:mi mathvariant="normal">p</mml:mi><mml:mo>,</mml:mo><mml:mo>max⁡</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:mfenced><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup><mml:mo>,</mml:mo><mml:mi>C</mml:mi><mml:mo>,</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mrow><mml:mi mathvariant="normal">p</mml:mi><mml:mo>,</mml:mo><mml:mo>min⁡</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:mfenced></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

          with <inline-formula><mml:math id="M132" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mo>min⁡</mml:mo></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.9</mml:mn><mml:mo>⋅</mml:mo><mml:mi>C</mml:mi></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M133" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mo>max⁡</mml:mo></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1.1</mml:mn><mml:mo>⋅</mml:mo><mml:mi>C</mml:mi></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M134" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mrow><mml:mi mathvariant="normal">p</mml:mi><mml:mo>,</mml:mo><mml:mo>min⁡</mml:mo></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M135" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mrow><mml:mi mathvariant="normal">p</mml:mi><mml:mo>,</mml:mo><mml:mo>min⁡</mml:mo></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula></p>
      <p id="d2e4858">Following <xref ref-type="bibr" rid="bib1.bibx4 bib1.bibx16" id="paren.38"/>, the particle linear depolarization ratio (<inline-formula><mml:math id="M136" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is then obtained as

            <disp-formula id="Ch1.E28" content-type="numbered"><label>28</label><mml:math id="M137" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mfenced close=")" open="("><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mi>R</mml:mi><mml:mo>-</mml:mo><mml:mfenced close=")" open="("><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mi>R</mml:mi><mml:mo>-</mml:mo><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          where the backscatter ratio <inline-formula><mml:math id="M138" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> is defined as

            <disp-formula id="Ch1.E29" content-type="numbered"><label>29</label><mml:math id="M139" display="block"><mml:mrow><mml:mi>R</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          and <inline-formula><mml:math id="M140" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the volume linear depolarization ratio, which is <inline-formula><mml:math id="M141" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">corrected</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in Eq. (17), or <inline-formula><mml:math id="M142" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:mfrac></mml:mstyle></mml:math></inline-formula> for instruments lacking termination hood measurements.</p>
      <p id="d2e5047">The molecular depolarization ratio (<inline-formula><mml:math id="M143" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is estimated following <xref ref-type="bibr" rid="bib1.bibx41" id="text.39"/>, accounting for major atmospheric gases and the influence of water vapor. The input data for these calculations are taken from a numerical weather prediction model (ECMWF IFS forecast) provided via the ACTRIS Cloudnet data portal <xref ref-type="bibr" rid="bib1.bibx34" id="paren.40"/>.</p>
      <p id="d2e5067">The uncertainty of <inline-formula><mml:math id="M144" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> can be determined using partial derivatives

            <disp-formula id="Ch1.E30" content-type="numbered"><label>30</label><mml:math id="M145" display="block"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>=</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>R</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi>R</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>
      <p id="d2e5194">Assuming <inline-formula><mml:math id="M146" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M147" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> are negligible and approximating <inline-formula><mml:math id="M148" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi>R</mml:mi></mml:msub><mml:mo>≈</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></inline-formula>, this reduces to

            <disp-formula id="Ch1.E31" content-type="numbered"><label>31</label><mml:math id="M149" display="block"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>≈</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>R</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>
      <p id="d2e5350">The partial derivatives are calculated as:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M150" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E32"><mml:mtd><mml:mtext>32</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mi>R</mml:mi><mml:mo>(</mml:mo><mml:mi>R</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mfenced close=")" open="("><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mi>R</mml:mi><mml:mo>-</mml:mo><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E33"><mml:mtd><mml:mtext>33</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>R</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mfenced close=")" open="("><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mi>R</mml:mi><mml:mo>-</mml:mo><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula></p>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Results and discussion</title>
<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Background noise</title>
      <p id="d2e5559">Figure <xref ref-type="fig" rid="F4"/> shows the time series of background noise (variance of the background signal), normalized by integration time assuming Poisson statistics (<inline-formula><mml:math id="M151" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>/</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>×</mml:mo><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">intergration</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), alongside the laser power. Most instruments (except for Vehmasmäki) exhibit a gradual decline in laser power, accompanied by corresponding increases in background noise, likely due to weaker return signal. These changes often occur in discrete steps rather than as a continuous trend. Notably, fluctuations in background noise are consistently related to changes in laser power. Periods of restored laser power and decreased background noise align with documented hardware interventions, such as transmitter replacements at Vehmasmäki (December 2022; Fig. <xref ref-type="fig" rid="F4"/>a) and Hyytiälä (February 2024; Fig. <xref ref-type="fig" rid="F4"/>b).</p>

      <fig id="F4" specific-use="star"><label>Figure 4</label><caption><p id="d2e5605">Time series of nighttime background signal variance normalized by the integration time (<inline-formula><mml:math id="M152" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>/</mml:mo><mml:msup><mml:mi>r</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:mo>×</mml:mo><mml:msub><mml:mi>t</mml:mi><mml:mi mathvariant="normal">intergration</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and the laser power are shown for <bold>(a)</bold> Vehmasmäki, <bold>(b)</bold> Hyytiälä, <bold>(c)</bold> Kenttärova, and <bold>(d)</bold> Lindenberg. Shaded regions denote different firmware versions; unshaded areas represent periods with no recorded firmware version and laser power.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f04.png"/>

        </fig>

      <p id="d2e5661">At Hyytiälä and Kenttärova, laser power gradually decreases from 100 % to around 40 % over 2 years. In contrast, the CL61 at Vehmasmäki maintains a consistently high laser power, ranging between 90 % and 100 % throughout the same period, with only a slight decrease during the summer, likely to regulate the internal temperature to prevent overheating. Meanwhile, the CL61 at Lindenberg experienced a sharp decline in laser power, from 80 % to below 10 % within just 1 year of operation. We also found that changes in the firmware version do not appear to have any noticeable effect on background noise levels.</p>
      <p id="d2e5665">The relationship between background noise, normalized by integration time, and laser power across several instruments is illustrated in Fig. <xref ref-type="fig" rid="F5"/>. Nighttime measurements (23:00 to 01:00 local time; LT), shown in blue, are unaffected by solar radiation, while all-day measurements are displayed in grey. It is important to note that the selected nighttime window is arbitrary and used solely for this analysis; for instance, locations such as Kenttärova experience no true nighttime during summer. The nighttime data clearly indicate that a decrease in laser power leads to an increase in background noise across all instruments. Daytime background noise is generally higher due to solar radiation, which varies with factors such as solar angle, cloud height, and surface albedo, making direct comparisons more complex. Nevertheless, the figure suggests that lower laser power also contributes to increased noise levels during daytime conditions.</p>

      <fig id="F5" specific-use="star"><label>Figure 5</label><caption><p id="d2e5672">Variance of background noise as a function of laser power percentage, normalized by integration time, at the following locations: <bold>(a)</bold> Vehmasmäki, <bold>(b)</bold> Hyytiälä, <bold>(c)</bold> Kenttärova, and <bold>(d)</bold> Lindenberg. Blue points represent data collected during nighttime hours (23:00–01:00 LT), while grey points include all available data.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f05.png"/>

        </fig>

      <p id="d2e5693">An increase in background noise can significantly reduce an instrument's ability to detect weak aerosol signals. This effect is clearly illustrated in Fig. S3. On 7 March 2024, an elevated aerosol layer was observed above 3 km in Lindenberg, indicated by enhanced attenuated backscatter coefficient values compared to those at lower altitudes between 1 and 3 km (Fig. S3a, c). However, by 2 December 2024, a reduction in laser power led to a higher noise floor, which meant that if a similar aerosol layer were present, it would no longer be distinguishable from the background noise (Fig. S3b, c).</p>
</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Instrumental background</title>
      <p id="d2e5704">In this section, we examine how the instrumental background bias (<inline-formula><mml:math id="M153" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>) and noise (<inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>) with the overlap correction reverted, vary with temperature and over time. The termination hood measurement was deployed multiple times at Vehmasmäki, Hyytiälä, and Kenttärova. Figure <xref ref-type="fig" rid="F6"/> presents the instrumental background profiles recorded during these termination hood measurement periods, which have been averaged and grouped according to the instruments' internal temperatures.</p>

      <fig id="F6" specific-use="star"><label>Figure 6</label><caption><p id="d2e5759">Termination hood profiles at various internal temperatures (color-coded) across different sites. In Vehmasmäki: <bold>(a)</bold> <inline-formula><mml:math id="M155" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M156" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M157" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, and <bold>(d)</bold> <inline-formula><mml:math id="M158" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. In Hyytiälä: <bold>(e)</bold> <inline-formula><mml:math id="M159" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(f)</bold> <inline-formula><mml:math id="M160" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(g)</bold> <inline-formula><mml:math id="M161" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, and <bold>(h)</bold> <inline-formula><mml:math id="M162" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. In Kenttärova: <bold>(i)</bold> <inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(j)</bold> <inline-formula><mml:math id="M164" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(k)</bold> <inline-formula><mml:math id="M165" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, and <bold>(l)</bold> <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f06.png"/>

        </fig>

      <p id="d2e6144">For the instruments located in Hyytiälä and Kenttärova, the <inline-formula><mml:math id="M167" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> profiles remain relatively stable around zero from the far range down to about 2 km, then increase sharply as the range decreases. On the other hand, in Vehmasmäki, it also remains near zero at far range, but <inline-formula><mml:math id="M168" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> begins to increase already at around 5 km and continues to rise toward shorter ranges. Meanwhile, the <inline-formula><mml:math id="M169" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> profiles for all three instruments remain near zero from the far range to about 2 km, after which they increase rapidly with decreasing range.</p>
      <p id="d2e6229">Overall, the internal temperature <inline-formula><mml:math id="M170" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> has a more pronounced effect on the <inline-formula><mml:math id="M171" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> profiles below 1 km than at higher ranges. In particular, the <inline-formula><mml:math id="M172" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> profiles in both polarizations deviate substantially from zero at below 200 m (see Fig. <xref ref-type="fig" rid="F7"/>) across all instruments. Notably, each instrument shows the same small peak in the instrumental background bias in both polarizations at approximately 150 m.</p>

      <fig id="F7" specific-use="star"><label>Figure 7</label><caption><p id="d2e6289">Termination hood profiles at various internal temperatures (color-coded) across different sites only up to 1000 m range. In Vehmasmäki: <bold>(a)</bold> <inline-formula><mml:math id="M173" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M174" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M175" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, and <bold>(d)</bold> <inline-formula><mml:math id="M176" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. In Hyytiälä: <bold>(e)</bold> <inline-formula><mml:math id="M177" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(f)</bold> <inline-formula><mml:math id="M178" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(g)</bold> <inline-formula><mml:math id="M179" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, and <bold>(h)</bold> <inline-formula><mml:math id="M180" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. In Kenttärova: <bold>(i)</bold> <inline-formula><mml:math id="M181" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(j)</bold> <inline-formula><mml:math id="M182" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(k)</bold> <inline-formula><mml:math id="M183" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, and <bold>(l)</bold> <inline-formula><mml:math id="M184" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f07.png"/>

        </fig>

      <p id="d2e6674">All instruments exhibit profiles of <inline-formula><mml:math id="M185" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> in both polarizations that remain constant above 500 m, followed by a sharp increase below this range. These instrumental background noise profiles show a pronounced sensitivity to internal temperature (from 4 to 38 °C). Notably, very low temperatures are associated with elevated instrumental background noise across the entire measurement range. This can be explained by the effect of the internal heater. As the internal temperature falls below an instrument-specific threshold (15 °C for Hyytiälä and Kenttärova), the internal heater is turned on. This leads to an increase in <inline-formula><mml:math id="M186" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, with the effect becoming more pronounced as the temperature decreases. When the internal temperature is high and the internal heater is off, internal temperature positively correlates with <inline-formula><mml:math id="M187" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">instrument</mml:mi></mml:msub><mml:mi>O</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d2e6752">Similar to Figs. <xref ref-type="fig" rid="F6"/>, <xref ref-type="fig" rid="F7"/>, S4 and S5 show the same profiles obtained during the termination hood measurements, but include range correction and the instrument-provided overlap correction. These profiles of <inline-formula><mml:math id="M188" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M189" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> provide a direct quantification of the impact of instrumental background bias and noise on the measurements and their dependence on temperature. For all CL61 instruments, the instrumental biases, <inline-formula><mml:math id="M190" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M191" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, remain below the order of <inline-formula><mml:math id="M192" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">7</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, while the noise terms, <inline-formula><mml:math id="M193" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M194" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, remain below the order of <inline-formula><mml:math id="M195" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">11</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. These biases are even smaller below 5 km. Below a range of 1 km, <inline-formula><mml:math id="M196" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> remains below 5 <inline-formula><mml:math id="M197" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<sup>−9</sup> and <inline-formula><mml:math id="M199" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> below 3 <inline-formula><mml:math id="M200" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<sup>−9</sup>. These small biases are usually negligible comparing to the typical atmospheric signal.</p>
      <p id="d2e6975">However, at very clean sites such as Kenttärova, the instrumental bias in <inline-formula><mml:math id="M202" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> can still affect the retrieved aerosol depolarization ratio, particularly under conditions of low depolarization. An example is shown in Fig. S6, which presents measurements from Kenttärova on 3 October 2023 under weakly depolarizing aerosol conditions. During this period, the <inline-formula><mml:math id="M203" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> profile below 400 m is on the order of <inline-formula><mml:math id="M204" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">9</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, while <inline-formula><mml:math id="M205" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> remains on the order of <inline-formula><mml:math id="M206" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. As a result, the instrumental bias becomes relatively significant for <inline-formula><mml:math id="M207" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, leading to a noticeable, although quantitatively small, reduction in <inline-formula><mml:math id="M208" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula> (from 0.002 to 0.001 at 200 m) after the bias correction is applied. Furthermore, the previously mentioned peak at 150 m is clearly visible in this case and is effectively mitigated after the removal of the instrumental bias. Overall, the impact of the bias correction is expected to be most pronounced under clean atmospheric conditions, such as in this case in Finland, where the <inline-formula><mml:math id="M209" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula> profile remains consistently low. The correction improves the overall shape of the profile, particularly around 150 m, by removing the artificial peak in <inline-formula><mml:math id="M210" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> at that height (Fig. S6). However, the change remains small in absolute terms.</p>
      <p id="d2e7097">For all instruments, the signal near the surface exhibits much more rapid fluctuations than at higher range gates. Figure S7 displays example profiles of <inline-formula><mml:math id="M211" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M212" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mo>⟂</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, and the instrument's internal temperature during a termination hood measurement at Kenttärova, revealing periodic variations in the signal below 50 m. To investigate this, the Fourier transforms of these signals were computed at each range gate over time and compared to that of the laser temperature recorded simultaneously. The results show that both the signals and the laser temperature exhibit a coincident spectral peak at approximately 0.0079 Hz (about 120 s), indicating a strong influence of laser temperature on the signals. Furthermore, additional distinct peaks in the signal spectra imply the presence of other instrument-related effects. Overall, these periodic variations appear sporadically across all instruments, with no consistent pattern indicating when they appear or disappear. Given the difficulty in developing a reliable correction method, we recommend excluding measurements below 50 m.</p>
      <p id="d2e7130">Figure <xref ref-type="fig" rid="F8"/> shows how the instrumental bias during the termination hood measurement at Vehmasmäki varies over time under consistent internal temperature conditions. Over a 6-month period, the calibration profiles at each temperature show only minor fluctuations. Therefore, we recommend performing termination hood checks at least once across the operating temperature range to determine the instrumental background bias and noise.</p>

      <fig id="F8" specific-use="star"><label>Figure 8</label><caption><p id="d2e7137">Termination hood profiles in Vehmasmäki at <bold>(a, b, e, f)</bold> 23 °C, and <bold>(c, d, g, h)</bold> 24 °C. These measurements were recorded at three different time points over a 6-month period in 2024. Panels <bold>(a)</bold>, <bold>(c)</bold>, <bold>(e)</bold>, and <bold>(g)</bold> display <inline-formula><mml:math id="M213" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, while panels <bold>(b)</bold>, <bold>(d)</bold>, <bold>(f)</bold>, and <bold>(h)</bold> display <inline-formula><mml:math id="M214" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msup><mml:mi/><mml:mo>∥</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f08.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Calibration</title>
      <p id="d2e7224">Figure <xref ref-type="fig" rid="F9"/> presents the time series of calibration factor from the cloud calibration and Rayleigh calibration methods for all the ceilometers. Detailed results of the cloud calibration factors derived from liquid cloud signals at each site are presented in Figs. S8–S11. Overall, the calibration factors obtained from the two methods agree well within their respective uncertainties, In Lindenberg, the calibration factor from the cloud calibration exhibits an approximate threefold decline over time, reflecting notable signal degradation. During this degradation period, Rayleigh calibration could not be performed because the elevated background-noise level (see Sect. 4.1) obscured the molecular return. In contrast, the other instruments show only short-term fluctuations without any clear long-term trend. Two periods with notable deviations in the calibration factor were also identified: June to October 2023 and November to December 2024 in Vehmasmäki. The issue in the CL61 at Vehmasmäki is due to the fogged window that attenuates the outgoing signal. This will be analyzed in more detail in the following section.</p>

      <fig id="F9" specific-use="star"><label>Figure 9</label><caption><p id="d2e7231">Time series of the calibration factor from cloud calibration, Rayleigh calibration and laser power at four sites: <bold>(a)</bold> Vehmasmäki, <bold>(b)</bold> Hyytiälä, <bold>(c)</bold> Kenttärova, and <bold>(d)</bold> Lindenberg. The dashed line indicates a calibration factor of <inline-formula><mml:math id="M215" display="inline"><mml:mi>c</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M216" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 1. Periods corresponding to different firmware versions are highlighted with shaded areas.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f09.png"/>

        </fig>

      <p id="d2e7267">Across all instruments, the calibration factor generally stays within the range of <inline-formula><mml:math id="M217" display="inline"><mml:mn mathvariant="normal">0.9</mml:mn></mml:math></inline-formula> to <inline-formula><mml:math id="M218" display="inline"><mml:mn mathvariant="normal">1.5</mml:mn></mml:math></inline-formula> as long as laser power remains above 40 %, aside from occasional deviations due to specific instrument issues. In Vehmasmäki, as the laser power remains above 90 %, the calibration factor fluctuates around <inline-formula><mml:math id="M219" display="inline"><mml:mn mathvariant="normal">1</mml:mn></mml:math></inline-formula> within 10 % fluctuation. In Hyytiälä, the highest changes in calibration factor is observed when the instrument's laser power is below 80 % with the firmware 1.1.10 and then below 60 % with the firmware 1.2.7. However, the calibration factor remains relatively stable at 1.25 even when the laser power drops from 100 % to 40 % with the firmware 1.2.7. In Kenttärova, laser power percentages were not recorded before June 2023, but the observed increase in the calibration factor is likely linked to a decrease in laser power. After a new transmitter was installed, the calibration factor returned to around <inline-formula><mml:math id="M220" display="inline"><mml:mn mathvariant="normal">1</mml:mn></mml:math></inline-formula>. In Lindenberg, a noticeable decline in the cloud calibration factor was observed as laser power dropped from 40 % to 10 %. It is still to be ascertained whether this trend also appears in instruments running the newer firmware version 1.2.7.</p>
      <p id="d2e7299">Figure S12 demonstrates the utility of cloud calibration for two cases; one with 80 % laser power on 3 March 2024 and another with just 10 % on 16 November 2024. This indicates that the method can still be used in situations with low laser power. Since the internal calibration value may not scale with low laser power values, regular cloud calibration is necessary to understand instrument performance and continue to provide profiles that can be used quantitatively, especially for laser power values below 40 %.</p>
</sec>
<sec id="Ch1.S4.SS4">
  <label>4.4</label><title>Signal correction and uncertainty estimation</title>
      <p id="d2e7310">After recording the termination hood profiles at different temperatures and determining the calibration factor, the correction and forward Klett inversion can be applied, and the associated uncertainty can be estimated using the method described in Sect. 3.3. Example results of this procedure are illustrated in Figs. <xref ref-type="fig" rid="F10"/> and <xref ref-type="fig" rid="F11"/> showcasing a typical Finnish low aerosol load condition in Kenttärova. During this period, the calibration factor was close to 1. On this date (Fig. <xref ref-type="fig" rid="F11"/>), aerosol was present below 1000 m within the boundary layer close to the ground, while several layers of clouds extended from 2 up to 3.5 km. Figure <xref ref-type="fig" rid="F10"/> presents the <inline-formula><mml:math id="M221" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M222" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula> and their associated uncertainties in the aerosol layer below 1000 m obtained from a measurement profile recorded at 13:01 UTC on the same day.</p>

      <fig id="F10" specific-use="star"><label>Figure 10</label><caption><p id="d2e7338">Example of uncorrected and corrected profiles in Kenttärova measured on 4 June 2024 at 13:01 UTC. <bold>(a)</bold> <inline-formula><mml:math id="M223" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> (instrument provided), <inline-formula><mml:math id="M224" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> (bias corrected and calibrated), <inline-formula><mml:math id="M225" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M226" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M227" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(c)</bold> <inline-formula><mml:math id="M228" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula> (instrument provided), <inline-formula><mml:math id="M229" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (bias corrected and calibrated), <inline-formula><mml:math id="M230" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(d)</bold> <inline-formula><mml:math id="M231" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M232" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. Error bars represent 1 standard deviation (<inline-formula><mml:math id="M233" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) of the measurements.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f10.png"/>

        </fig>

      <fig id="F11" specific-use="star"><label>Figure 11</label><caption><p id="d2e7504">An example of corrected and calibrated profile in Kenttärova on 4 June 2024 at 13:00–17:00 UTC (same day as Fig. <xref ref-type="fig" rid="F10"/>). <bold>(a)</bold> <inline-formula><mml:math id="M234" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> <inline-formula><mml:math id="M235" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> <bold>(c)</bold> <inline-formula><mml:math id="M236" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(d)</bold> <inline-formula><mml:math id="M237" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> <bold>(e)</bold> <inline-formula><mml:math id="M238" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(f)</bold> <inline-formula><mml:math id="M239" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <bold>(g)</bold> <inline-formula><mml:math id="M240" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and <bold>(h)</bold> <inline-formula><mml:math id="M241" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>. For particle properties in panels <bold>(e)</bold>–<bold>(h)</bold>, profiles are shown only up to 1 km range.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f11.png"/>

        </fig>

      <p id="d2e7665">At below 1000 m range, the corrected <inline-formula><mml:math id="M242" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> differs only slightly from the original uncorrected <inline-formula><mml:math id="M243" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, with the difference ranging from 1 <inline-formula><mml:math id="M244" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<sup>−9</sup> to 2.5 <inline-formula><mml:math id="M246" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<sup>−9</sup> sr<sup>−1</sup> m<sup>−1</sup> (Fig. <xref ref-type="fig" rid="F10"/>a). This difference is expected to be relatively smaller within the clouds, where the signal is stronger and the instrumental bias decreases with increasing range. In contrast, the particle backscatter coefficient <inline-formula><mml:math id="M250" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is substantially lower than <inline-formula><mml:math id="M251" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> by approximately 1.5 <inline-formula><mml:math id="M252" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<sup>−7</sup> sr<sup>−1</sup> m<sup>−1</sup>, indicating a significant contribution from molecular scattering. The <inline-formula><mml:math id="M256" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M257" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> profiles are relatively similar to each other, and they both increase exponentially with height (Fig. <xref ref-type="fig" rid="F10"/>b).</p>
      <p id="d2e7864">Similarly, the original uncorrected (<inline-formula><mml:math id="M258" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula>) and the corrected (<inline-formula><mml:math id="M259" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) profiles differ only slightly, by the difference is about 0.001 to 0.005 (Fig. <xref ref-type="fig" rid="F10"/>c) while <inline-formula><mml:math id="M260" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula> itself being around 0.07. In contrast, the particle linear depolarization ratio <inline-formula><mml:math id="M261" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is substantially higher, differing from the original <inline-formula><mml:math id="M262" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula> by approximately 0.1 with <inline-formula><mml:math id="M263" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> at around 0.1 to 0.15. For example, during pollen seasons in Finland, <inline-formula><mml:math id="M264" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> has been observed at 0.23 for pine and 0.26 for birch at this wavelength <xref ref-type="bibr" rid="bib1.bibx13" id="paren.41"/>. The variances (<inline-formula><mml:math id="M265" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M266" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>) are comparable below 200 m, but at higher ranges, <inline-formula><mml:math id="M267" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> becomes markedly larger.</p>
      <p id="d2e7990">Overall, the pronounced differences between <inline-formula><mml:math id="M268" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M269" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, as well as between <inline-formula><mml:math id="M270" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M271" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, highlight the importance of accounting for the molecular contribution when performing quantitative assessments of aerosol measurement with CL61 for low aerosol load conditions in Finland. While the difference between <inline-formula><mml:math id="M272" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M273" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> (and <inline-formula><mml:math id="M274" display="inline"><mml:mi mathvariant="italic">δ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M275" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) may be small, the termination hood remains important as it allows the estimation of measurement uncertainties. Averaging multiple profiles reduces the uncertainties, as illustrated in Fig. S13, which shows the profiles averaged over 10 min.</p>
      <p id="d2e8082">Figure <xref ref-type="fig" rid="F11"/> illustrates the time series of <inline-formula><mml:math id="M276" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M277" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M278" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M279" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> profiles, along with their corresponding variances on the same day. Similar to Fig. <xref ref-type="fig" rid="F10"/>, <inline-formula><mml:math id="M280" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> is higher than <inline-formula><mml:math id="M281" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, while <inline-formula><mml:math id="M282" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is lower than <inline-formula><mml:math id="M283" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in this period. The profiles of <inline-formula><mml:math id="M284" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M285" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> vary with time during this period, exhibiting an exponential increase with range. On the other hand, the <inline-formula><mml:math id="M286" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M287" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">σ</mml:mi><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula> profiles demonstrate a more pronounced dependence on the signal magnitude (Fig. <xref ref-type="fig" rid="F11"/>d and h), with stronger atmospheric signals resulting in smaller uncertainties.</p>
</sec>
<sec id="Ch1.S4.SS5">
  <label>4.5</label><title>Signal loss</title>
      <p id="d2e8264">As previously noted, abrupt changes in the cloud calibration factor at Vehmasmäki were observed from June to October 2023 and again from November to December 2024. Similar deviations are present during the same periods, as seen in the window condition housekeeping variable (Fig. S14). These patterns indicate that an obstruction, likely on the instrument window, was attenuating both outgoing and incoming laser beams.</p>

      <fig id="F12" specific-use="star"><label>Figure 12</label><caption><p id="d2e8269">Measurements from Vehmasmäki on 19 May 2023: <bold>(a)</bold> <inline-formula><mml:math id="M288" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">β</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> internal temperature, <bold>(c)</bold> window condition, <bold>(d)</bold> internal humidity, <bold>(e)</bold> window blower heater, and <bold>(f)</bold> calculated dew point and measured outside air temperature.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/4923/2026/amt-19-4923-2026-f12.png"/>

        </fig>

      <p id="d2e8308">Figure <xref ref-type="fig" rid="F12"/> illustrates a specific example from 19 May 2023. On this date, a sudden drop in the attenuated backscatter signal below 2000 m occurred just before 06:00 UTC. At the same time, the window condition value sharply declined from around 100 % to 70 %. This coincided with the automatic deactivation of the window blower heater. Housekeeping data, including internal temperature and relative humidity, were used to estimate the internal dew point, which was then compared to the external air temperature. When the window blower heater was off, the window cooled to match the outside air temperature. Once the window temperature dropped below the internal dew point, condensation began to form on the inside surface of the window and attenuated the signal. This occurred despite the measured internal relative humidity remaining below 70 %. This is because the measurement does not represent the relative humidity at the window surface, where the temperature is closer to ambient temperature.</p>
      <p id="d2e8314">Since condensation affects the entire signal profile and the degree of attenuation depends on its severity, it is not possible to precisely quantify the signal loss or reconstruct the original profile. This issue could be mitigated by keeping both the window blower and heater always on. However, at the time of this writing, this is not possible (personal communication with Vaisala). Additionally, hardware modifications may be required to maintain a sufficiently low internal dew point and prevent fogging.</p>
</sec>
</sec>
<sec id="Ch1.S5" sec-type="conclusions">
  <label>5</label><title>Conclusions</title>
      <p id="d2e8327">In this study, we investigate several characteristics of CL61 measurements across multiple sites over a 3-year period, using methodologies adapted from existing approaches.</p>
      <p id="d2e8330">First, we examine the temporal evolution of the background noise and its relationship with laser power. The background noise generally increases as the laser power decreases, which is particularly important because laser aging can substantially reduce the CL61's capability to detect weak aerosol signals. For most instruments, internal scaling of the calibration factor effectively compensates for changes in laser power. However, for the instrument at the Lindenberg site with an older firmware version (1.1.10), this compensation becomes insufficient when laser power drops below 40 %, resulting in a drift in the calibration factor. Therefore, regular cloud calibration is necessary to ensure quantitatively reliable profiles, especially when the laser power falls below 40 %. Additionally, some deviations in the calibration factor were linked to the fogging of the inside surface of the window.</p>
      <p id="d2e8333">Second, we performed termination hood measurements to characterize the instrumental residual background bias and noise profiles. The magnitude of the residual background bias for all instruments is generally small. In a case study in Kenttärova, the magnitude of the residual bias was approximately 1 %–2 % of the molecular backscatter. Nevertheless, the termination hood measurements remain crucial, as they allow the instrumental background to be quantified and subsequently used to estimate the uncertainties of the particle backscatter coefficient (<inline-formula><mml:math id="M289" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">β</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and the particle linear depolarization ratio (<inline-formula><mml:math id="M290" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), as presented in this study.</p>
      <p id="d2e8358">Third, we found that the instrumental residual background bias and noise profiles are sensitive to temperature and exhibit differences between parallel and perpendicular polarizations. We also recommend discarding the first 50 m of measurements, where periodic variations were frequently observed. Instrumental background profiles were obtained across a range of internal temperatures and were subsequently used to correct the bias and estimate its associated uncertainty. These profiles remained stable for at least one month for a given internal temperature, although small deviations appeared over a 6-month period. Consequently, we recommend making termination hood measurements at least once across the operating temperature range to characterize the instrumental background.</p>
      <p id="d2e8362">Fourth, we demonstrate that the molecular contribution to the measured depolarization ratio can be substantial, reaching approximately 0.1, whereas the impact of residual background bias is only around 0.005 in the same case study. This highlights the importance of accounting for the molecular contribution in CL61 depolarization ratio measurement under low aerosol load conditions.</p>
      <p id="d2e8365">Finally, we identify window fogging as an important issue affecting CL61 data quality. Fogging of the inside surface of the window was observed in some instruments and resulted in degraded measurements. Identifying and excluding such periods is therefore essential for ensuring the integrity of the dataset and the reliability of subsequent analyses.</p>
</sec>

      
      </body>
    <back><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d2e8372">The CL61 and model data used in this study are provided by the Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS) and are available respectively from the ACTRIS Data Centre using the following DOIs: <ext-link xlink:href="https://doi.org/10.60656/57adeb3f598243f2" ext-link-type="DOI">10.60656/57adeb3f598243f2</ext-link> <xref ref-type="bibr" rid="bib1.bibx34" id="paren.42"/>  and <ext-link xlink:href="https://doi.org/10.60656/d2626d9dd3454006" ext-link-type="DOI">10.60656/d2626d9dd3454006</ext-link> <xref ref-type="bibr" rid="bib1.bibx17" id="paren.43"/>. The CL61 raw data was obtained from the Cloudnet portal at <uri>https://cloudnet.fmi.fi</uri> (last access: 29 June 2026).</p>
  </notes><app-group>
        <supplementary-material position="anchor"><p id="d2e8390">The supplement related to this article is available online at <inline-supplementary-material xlink:href="https://doi.org/10.5194/amt-19-4923-2026-supplement" xlink:title="pdf">https://doi.org/10.5194/amt-19-4923-2026-supplement</inline-supplementary-material>.</p></supplementary-material>
        </app-group><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d2e8399">VL, EOC and MF performed the termination hood calibrations. VL prepared the manuscript. EOC, MF, VV contributed remarks and revisions on the manuscript.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d2e8405">The contact author has declared that none of the authors has any competing interests.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <p id="d2e8411">Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this paper. The authors bear the ultimate responsibility for providing appropriate place names. Views expressed in the text are those of the authors and do not necessarily reflect the views of the publisher.</p>
  </notes><ack><title>Acknowledgements</title><p id="d2e8418">The financial support of the Magnus Ehrnrooth Foundation, the Research Council of Finland, and Vaikuttavuussäätiö (the Finnish Research Impact Foundation) is gratefully acknowledged. We also acknowledge ACTRIS, the Finnish Meteorological Institute, and the Lindenberg Meteorological Observatory – Richard Assmann Observatory (MOL-RAO).</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d2e8423">This research has been supported by the Magnus Ehrnroothin Säätiö, the Research Council of Finland, Luonnontieteiden ja Tekniikan Tutkimuksen Toimikunta (grant nos. 337552 and 343359), Vaikuttavuussäätiö (the Finnish Research Impact Foundation) through the Tandem Industry Academia (TIA) program.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d2e8429">This paper was edited by Ulla Wandinger and reviewed by two anonymous referees.</p>
  </notes><ref-list>
    <title>References</title>

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