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  <front>
    <journal-meta><journal-id journal-id-type="publisher">AMT</journal-id><journal-title-group>
    <journal-title>Atmospheric Measurement Techniques</journal-title>
    <abbrev-journal-title abbrev-type="publisher">AMT</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Meas. Tech.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1867-8548</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/amt-19-935-2026</article-id><title-group><article-title>Seeking TOA SW flux closure over semi-synthetic 3D cloud fields: exploring the accuracy of two angular distribution models</article-title><alt-title>Seeking TOA SW flux closure over semi-synthetic 3D cloud fields</alt-title>
      </title-group>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1 aff2">
          <name><surname>Madenach</surname><given-names>Nils</given-names></name>
          <email>nils.madenach@tropos.de</email>
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff3 aff4">
          <name><surname>Tornow</surname><given-names>Florian</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-3664-6933</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff5">
          <name><surname>Barker</surname><given-names>Howard</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Preusker</surname><given-names>Rene</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2 aff6">
          <name><surname>Fischer</surname><given-names>Jürgen</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-6789-6062</ext-link></contrib>
        <aff id="aff1"><label>1</label><institution>Leibniz Institute for Tropospheric Research, Leipzig, Germany</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Freie Universität Berlin, Berlin, Germany</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Columbia University, New York, NY, USA</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>NASA Goddard Institute for Space Studies, New York, NY, USA</institution>
        </aff>
        <aff id="aff5"><label>5</label><institution>Environment and Climate Change Canada, Toronto, Ontario, Canada</institution>
        </aff>
        <aff id="aff6"><label>☆</label><institution>retired</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Nils Madenach (nils.madenach@tropos.de)</corresp></author-notes><pub-date><day>10</day><month>February</month><year>2026</year></pub-date>
      
      <volume>19</volume>
      <issue>3</issue>
      <fpage>935</fpage><lpage>947</lpage>
      <history>
        <date date-type="received"><day>26</day><month>March</month><year>2025</year></date>
           <date date-type="rev-request"><day>8</day><month>September</month><year>2025</year></date>
           <date date-type="rev-recd"><day>16</day><month>January</month><year>2026</year></date>
           <date date-type="accepted"><day>25</day><month>January</month><year>2026</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2026 Nils Madenach et al.</copyright-statement>
        <copyright-year>2026</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://amt.copernicus.org/articles/amt-19-935-2026.html">This article is available from https://amt.copernicus.org/articles/amt-19-935-2026.html</self-uri><self-uri xlink:href="https://amt.copernicus.org/articles/amt-19-935-2026.pdf">The full text article is available as a PDF file from https://amt.copernicus.org/articles/amt-19-935-2026.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d2e151">To accurately estimate outgoing top-of-atmosphere (TOA) shortwave (SW) fluxes from measurements of broadband radiances, angular distribution models (ADMs) are necessary. ADMs rely on radiance-predicting models that are trained on hemispherically-resolved CERES TOA radiance observations. The estimation of SW fluxes is particularly challenging for cloudy skies due to clouds' anisotropy, which substantially varies with their optical properties for any given sun-object-observer geometry. The aim of this study is to investigate the influence of micro- and macrophysical properties of liquid clouds on SW fluxes estimated by ADMs that are based on a semi-physical model and compare to operational ADMs. We hypothesize that a microphysically aware ADM performs better in observation angles influenced by single-scattering features.</p>

      <p id="d2e154">The semi-physical approach relies on a parameterized asymmetry parameter <inline-formula><mml:math id="M1" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>, which depends on the cloud effective radius and, after adjustments during training of the model, explicitly varies with sun–observer geometry. We link these adjustments to single scattering features, such as the shift of the cloud bow and glory with varying cloud droplet sizes.</p>

      <p id="d2e168">For the investigation, 125 3D cloud scenes are constructed based on observational data and theoretical assumptions. Using a Monte Carlo model, the TOA broadband SW radiances and fluxes of the semi-synthetic cloud scenes are simulated for different scenarios with varying viewing angles (<inline-formula><mml:math id="M2" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) along the principal plane and solar angles (<inline-formula><mml:math id="M3" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). Based on the resulting 20 000 scenarios, the sensitivity and accuracy of the two SW radiance-to-irradiance conversion approaches to cloud droplet size, spatial distribution of liquid water path, and mean optical thickness are quantified.</p>

      <p id="d2e193">The study emphasizes that explicitly including the liquid droplet effective radius in ADM generation can improve the accuracy of shortwave flux estimates. Particularly for viewing geometries that exhibit single scattering phenomena, such as cloud glory and cloud bow, flux estimates can benefit from microphysically aware ADMs. For the analyzed scenarios, we found that the errors of instantaneous TOA SW flux estimates could be reduced by up to 25 W m<sup>−2</sup>. For scenes with very large or small droplets, the median error was reduced by up to 7 W m<sup>−2</sup>.</p>
  </abstract>
    
<funding-group>
<award-group id="gs1">
<funding-source>European Space Agency</funding-source>
<award-id>4000112019/14/NL/CT</award-id>
<award-id>4000134661/21/NL/AD</award-id>
<award-id>4000133155/20/NL/FF/tfd</award-id>
</award-group>
</funding-group>
</article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d2e229">The Earth radiation budget (ERB) quantifies the overall balance of incoming solar radiation and outgoing reflected solar and emitted thermal radiation at the top of the atmosphere (TOA). Quantifying ERB is fundamental for understanding how the climate of Earth will change in the future. The main parameters influencing the ERB are the Earth's surface, clouds, aerosols, and atmospheric gases (e.g. <xref ref-type="bibr" rid="bib1.bibx10 bib1.bibx26 bib1.bibx27 bib1.bibx8" id="altparen.1"/>). TOA outgoing radiative fluxes are estimated using, e.g., radiance measurements of broadband (BB) radiometers aboard polar orbiting and geostationary satellites (e.g. <xref ref-type="bibr" rid="bib1.bibx24 bib1.bibx6 bib1.bibx22" id="altparen.2"/>).</p>
      <p id="d2e238">However, accurately estimating the flux leaving Earth's TOA using only one measurement at a single sun-observer geometry, as is the case for satellites, is challenging. In particular, the reflected solar radiation can be highly anisotropic, depending on the observed scene. For clouds, the dependency on sun–observer geometry is complex and governed by their macro- and microphysical properties. Over the past decades, a variety of radiance-predicting models have been developed and refined to estimate the anisotropy of observed cloud scenes (e.g., <xref ref-type="bibr" rid="bib1.bibx16 bib1.bibx11 bib1.bibx12 bib1.bibx17 bib1.bibx7 bib1.bibx21 bib1.bibx23" id="altparen.3"/>). Using these distribution models (ADMs) the radiance-to-irradiance (flux) conversion can be achieved from a single satellite observation. An overview of different SW ADM approaches is given in <xref ref-type="bibr" rid="bib1.bibx9" id="text.4"/>.</p>
      <p id="d2e247">In this study, we investigate TOA SW flux estimates for overcast marine liquid cloud scenes with varying macro- and microphysical properties. SW fluxes are estimated using two sets of ADMs: one based on the semi-physical log-linear model <xref ref-type="bibr" rid="bib1.bibx20 bib1.bibx21" id="paren.5"/> (semi-physical approach), and a second set derived using the state-of-the art sigmoidal approach <xref ref-type="bibr" rid="bib1.bibx17" id="paren.6"/>. The later is the currently operational approach used for SW flux estimates above clouds, for example, by the Clouds and the Earth's Radiant Energy System (CERES). The flux estimates from CERES are the input for the ANN (Artificial Neural Network) approach, used in the EarthCARE BMA-FLX processor <xref ref-type="bibr" rid="bib1.bibx23" id="paren.7"/>. To analyze the accuracy of the SW flux estimates and the sensitivity to micro- and macrophysical properties, we use 125 different semi-synthetic 3D cloud scenes to simulate TOA radiances and fluxes using a Monte Carlo model. The semi-physical approach explicitly incorporates the mean cloud top effective radius (<inline-formula><mml:math id="M6" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>) via the parameterized asymmetry parameter (<inline-formula><mml:math id="M7" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>; <xref ref-type="bibr" rid="bib1.bibx20" id="altparen.8"/>), which also depends on the sun-observer angular-bin (<sup>Δ</sup>). The study addresses the following main research questions: <list list-type="order"><list-item>
      <p id="d2e301">How sensitive is the accuracy of TOA SW flux estimates to variations in effective radius, cloud homogeneity and optical thickness?</p></list-item><list-item>
      <p id="d2e305">Can the explicit incorporation of cloud microphysics in a radiance-to-irradiance conversion approach improve the accuracy of SW flux estimates?</p></list-item><list-item>
      <p id="d2e309">Are the adjustments of the asymmetry parameter <inline-formula><mml:math id="M9" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> resulting from the optimization process physically plausible, and what are the underlying causes for this?</p></list-item></list> Section <xref ref-type="sec" rid="Ch1.S2"/> describes the theoretical basis of ADMs, the generation of 3D cloud scenes, and the configuration of the Monte Carlo model. In Sect. <xref ref-type="sec" rid="Ch1.S3"/>, the results are discussed, and in Sect. <xref ref-type="sec" rid="Ch1.S4"/>, the findings are summarized and concluded.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Theoretical Basis and Methodology</title>
      <p id="d2e338">ADMs describe the hemispherically resolved deviation of TOA angular-bin mean radiance <inline-formula><mml:math id="M10" display="inline"><mml:mrow><mml:mover accent="true"><mml:mi>I</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> from the isotropic case. The deviation is expressed through the anisotropic factor (<inline-formula><mml:math id="M11" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula>), where values greater than one indicate stronger reflection than the isotropic case, and values less than one indicate weaker reflection. Equation (<xref ref-type="disp-formula" rid="Ch1.E1"/>) describes how the anisotropic factor for a given solar zenith <inline-formula><mml:math id="M12" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, viewing zenith <inline-formula><mml:math id="M13" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and relative azimuth angle <inline-formula><mml:math id="M14" display="inline"><mml:mi mathvariant="italic">ϕ</mml:mi></mml:math></inline-formula> is calculated.

              <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M15" display="block"><mml:mtable rowspacing="5.690551pt" displaystyle="true"><mml:mlabeledtr id="Ch1.E1"><mml:mtd><mml:mtext>1</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi>R</mml:mi><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mover accent="true"><mml:mi>I</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:msubsup><mml:mo>∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">π</mml:mi></mml:mrow></mml:msubsup><mml:msubsup><mml:mo>∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msubsup><mml:mover accent="true"><mml:mi>I</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced><mml:mi>cos⁡</mml:mi><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mi>sin⁡</mml:mi><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">d</mml:mi><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E2"><mml:mtd><mml:mtext>2</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:mover accent="true"><mml:mi>I</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:mover accent="true"><mml:mi>F</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

        For a radiance observation <inline-formula><mml:math id="M16" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> at a given sun-observer geometry, the TOA flux estimates (<inline-formula><mml:math id="M17" display="inline"><mml:mrow><mml:mi>F</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>) are calculated using the anisotropic factor derived in Eq. (<xref ref-type="disp-formula" rid="Ch1.E1"/>), following Eq. (<xref ref-type="disp-formula" rid="Ch1.E3"/>).

          <disp-formula id="Ch1.E3" content-type="numbered"><label>3</label><mml:math id="M18" display="block"><mml:mrow><mml:mi>F</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:mi>R</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></disp-formula></p>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>Sigmoidal approach</title>
      <p id="d2e725">The currently operational approach to construct ADMs over marine clouds is described in, e.g., <xref ref-type="bibr" rid="bib1.bibx17" id="text.9"/> and is an extension of the approach from <xref ref-type="bibr" rid="bib1.bibx12" id="text.10"/>. For the approach, information of the CERES footprint average cloud optical depth <inline-formula><mml:math id="M19" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> (exponential of the average over logarithmic <inline-formula><mml:math id="M20" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> values) and the cloud fraction <inline-formula><mml:math id="M21" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula> (in %) is used to predict the hemispherical field of TOA SW radiances <inline-formula><mml:math id="M22" display="inline"><mml:mover accent="true"><mml:mi>I</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>. Per angular-bin a sigmoidal function (Eq. <xref ref-type="disp-formula" rid="Ch1.E4"/>) is fitted to the observed CERES radiance <inline-formula><mml:math id="M23" display="inline"><mml:mi>I</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M24" display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M25" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M26" display="inline"><mml:mrow><mml:mi>log⁡</mml:mi><mml:mfenced open="(" close=")"><mml:mrow><mml:mi>f</mml:mi><mml:mo>⋅</mml:mo><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mrow></mml:mfenced></mml:mrow></mml:math></inline-formula>. Where solar irradiance <inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> as well as <inline-formula><mml:math id="M28" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M29" display="inline"><mml:mi>b</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M30" display="inline"><mml:mi>c</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M31" display="inline"><mml:mrow><mml:msub><mml:mi>x</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> are free parameters in the model.

            <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M32" display="block"><mml:mrow><mml:mi>I</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mi>I</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>+</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mi>a</mml:mi><mml:mrow><mml:msup><mml:mfenced open="[" close="]"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mo>(</mml:mo><mml:mi>x</mml:mi><mml:mo>-</mml:mo><mml:msub><mml:mi>x</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>)</mml:mo><mml:mo>/</mml:mo><mml:mi>b</mml:mi></mml:mrow></mml:msup></mml:mrow></mml:mfenced><mml:mi>c</mml:mi></mml:msup></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></disp-formula></p>
</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Semi-physical approach</title>
      <p id="d2e916">As for the sigmoidal approach, the semi-physical approach uses CERES footprint average cloud optical depth <inline-formula><mml:math id="M33" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and the cloud fraction <inline-formula><mml:math id="M34" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula> (here not in % but as fraction). Additionally, the semi-physical approach includes information of the cloud microphysics in the form of the footprint averaged effective radius (<inline-formula><mml:math id="M35" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>) explicitly. Furthermore,  the water vapor load above the clouds (above cloud water vapor, ACWV) is taken into account.</p>
      <p id="d2e952">In <xref ref-type="bibr" rid="bib1.bibx18" id="text.11"/> the TOA SW anisotropy has been found to be sensitive to both <inline-formula><mml:math id="M36" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> and ACWV. In the case of effective radius, anisotropy differences  of up to 8 % were found. To incorporate these dependencies, a simple model (Eq. <xref ref-type="disp-formula" rid="Ch1.E5"/>) relating the outgoing radiance <inline-formula><mml:math id="M37" display="inline"><mml:mi>I</mml:mi></mml:math></inline-formula>, to the incoming solar irradiance (<inline-formula><mml:math id="M38" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) via a footprint albedo <inline-formula><mml:math id="M39" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> and a factor describing the attenuation due to water vapor above clouds (<inline-formula><mml:math id="M40" display="inline"><mml:mrow><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="normal">ACWV</mml:mi></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) has been formulated. The factor 2 arises from the fact that the light passes the water vapor layer twice before reaching the TOA. By using the logarithm (Eq. <xref ref-type="disp-formula" rid="Ch1.E6"/>) the model becomes linear and a simple first-degree polynomial function (Eq. <xref ref-type="disp-formula" rid="Ch1.E9"/>) can be fitted to the observations.

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M41" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E5"><mml:mtd><mml:mtext>5</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mi>I</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced><mml:mo>∼</mml:mo><mml:msub><mml:mi>I</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="italic">α</mml:mi><mml:mo>⋅</mml:mo><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">ACWV</mml:mi></mml:mrow></mml:msup></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E6"><mml:mtd><mml:mtext>6</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mi>log⁡</mml:mi><mml:mi>I</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi></mml:mrow></mml:mfenced><mml:mo>∼</mml:mo><mml:mi>log⁡</mml:mi><mml:msub><mml:mi>I</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>+</mml:mo><mml:mi>log⁡</mml:mi><mml:mi mathvariant="italic">α</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>⋅</mml:mo><mml:mtext>ACWV</mml:mtext></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

          The footprint albedo <inline-formula><mml:math id="M42" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> (Eq. <xref ref-type="disp-formula" rid="Ch1.E7"/>) is the sum of the clear sky portion of the scene (<inline-formula><mml:math id="M43" display="inline"><mml:mrow><mml:msub><mml:mi>f</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) multiplied with the clear sky albedo (<inline-formula><mml:math id="M44" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">cs</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>) and the cloud fraction (<inline-formula><mml:math id="M45" display="inline"><mml:mrow><mml:msub><mml:mi>f</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) multiplied with the two-stream albedo (<inline-formula><mml:math id="M46" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">ts</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, Eq. <xref ref-type="disp-formula" rid="Ch1.E8"/>). <inline-formula><mml:math id="M47" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">ts</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the Coakley–Chylek approximation <xref ref-type="bibr" rid="bib1.bibx4" id="paren.12"/> and depends on the footprint mean cloud optical thickness (<inline-formula><mml:math id="M48" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>) and the parameterized asymmetry parameter (<inline-formula><mml:math id="M49" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>) for the given sun-observer bin <sup>Δ</sup>.

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M51" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E7"><mml:mtd><mml:mtext>7</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi mathvariant="italic">α</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mi>f</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>⋅</mml:mo><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">cs</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>f</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub><mml:mo>⋅</mml:mo><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">ts</mml:mi></mml:msub></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E8"><mml:mtd><mml:mtext>8</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msub><mml:mi mathvariant="italic">α</mml:mi><mml:mi mathvariant="normal">ts</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo mathsize="1.5em">(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:mfenced><mml:mo mathsize="1.5em">)</mml:mo><mml:mo>⋅</mml:mo><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>/</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:mfenced close=")" open="("><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:mfenced></mml:mrow></mml:mfenced><mml:mo>⋅</mml:mo><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>/</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula></p>
<sec id="Ch1.S2.SS2.SSSx1" specific-use="unnumbered">
  <title>Parameterized asymmetry parameter</title>
      <p id="d2e1373">The asymmetry parameter <inline-formula><mml:math id="M52" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula> in the two-stream albedo describes the tendency of radiation to scatter in the forward or backward direction. Symmetric scattering corresponds to <inline-formula><mml:math id="M53" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M54" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 0, positive values (<inline-formula><mml:math id="M55" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M56" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> 0) to stronger forward scattering, and negative values (<inline-formula><mml:math id="M57" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M58" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 0) to stronger backward scattering. <inline-formula><mml:math id="M59" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula> is a function of cloud microphysics, represented in this study by the footprint-mean cloud-top effective radius (<inline-formula><mml:math id="M60" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>), and is for marine liquid clouds about 0.86. In the semi-physical approach, <inline-formula><mml:math id="M61" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula> is optimized during model training for each sun–observer geometry bin (<inline-formula><mml:math id="M62" display="inline"><mml:mi mathvariant="normal">Δ</mml:mi></mml:math></inline-formula>) to reduce residuals between the MODIS observations and the model <xref ref-type="bibr" rid="bib1.bibx20" id="paren.13"/>. Due to this bin-wise optimization, the parameterized <inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:mfenced></mml:mrow></mml:math></inline-formula> now also depends on the angular-bin <inline-formula><mml:math id="M64" display="inline"><mml:mi mathvariant="normal">Δ</mml:mi></mml:math></inline-formula> (see, e.g., Fig. <xref ref-type="fig" rid="F7"/>, lower panel). This optimization implicitly accounts for various 3D effects, as well as single-scattering features related to the underlying phase function, such as the broadening and forward shift of the cloud glory, and the shift of the cloud bow toward the backscatter direction for smaller <inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> (e.g., <xref ref-type="bibr" rid="bib1.bibx15" id="altparen.14"/>). With this new dependency, these single-scattering features become apparent in the radiances modeled using the  semi-physical approach (see, e.g., Figs. <xref ref-type="fig" rid="F1"/> and <xref ref-type="fig" rid="F6"/>).</p>

      <fig id="F1" specific-use="star"><label>Figure 1</label><caption><p id="d2e1525">Radiance (<inline-formula><mml:math id="M66" display="inline"><mml:mover accent="true"><mml:mi>I</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>) predicted for a <inline-formula><mml:math id="M67" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of 27° and an overcast scene over ocean with <inline-formula><mml:math id="M68" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> <inline-formula><mml:math id="M69" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 10. The three panels on the left show simulations using the semi-physical approach with variable <inline-formula><mml:math id="M70" display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and the right panel using the sigmoidal approach.</p></caption>
            <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f01.png"/>

          </fig>

      <p id="d2e1583">The semi-physical model is fitted to the observations using an ordinary-least-square method with the free parameters A, B, C (Eq. <xref ref-type="disp-formula" rid="Ch1.E9"/>).

              <disp-formula id="Ch1.E9" content-type="numbered"><label>9</label><mml:math id="M71" display="block"><mml:mrow><mml:mi>log⁡</mml:mi><mml:mi>I</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msubsup><mml:mo>,</mml:mo><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msubsup><mml:mo>,</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:mfenced><mml:mo>≈</mml:mo><mml:mtext>A</mml:mtext><mml:mo>+</mml:mo><mml:mtext>B</mml:mtext><mml:mo>⋅</mml:mo><mml:mi>log⁡</mml:mi><mml:mi mathvariant="italic">α</mml:mi><mml:mo>+</mml:mo><mml:mtext>C</mml:mtext><mml:mo>⋅</mml:mo><mml:mtext>ACWV</mml:mtext></mml:mrow></mml:math></disp-formula>

            Throughout this study, only overcast ocean scenes (<inline-formula><mml:math id="M72" display="inline"><mml:mrow><mml:msub><mml:mi>f</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M73" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 1) with a clear-sky fraction set to zero (<inline-formula><mml:math id="M74" display="inline"><mml:mrow><mml:msub><mml:mi>f</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M75" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 0) and no above cloud water vapor (ACWV <inline-formula><mml:math id="M76" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 0) are considered.</p>
      <p id="d2e1690">Figure <xref ref-type="fig" rid="F1"/> shows the predicted radiances using ADMs based on the sigmoidal approach (right panel) and on the semi-physical approach with varying <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> (three left panels) and illustrates the sensitivity of the semi-physical approach to cloud microphysics. In the figure, both approaches agree best for a <inline-formula><mml:math id="M78" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> of 10 <inline-formula><mml:math id="M79" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>, which is in the range of average values found in marine boundary layer stratocumulus clouds. For decreasing <inline-formula><mml:math id="M80" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> the broadening of cloud glory and bow becomes apparent.</p>
      <p id="d2e1754">A detailed explanation and further discussion of the semi-physical approach can be found in <xref ref-type="bibr" rid="bib1.bibx18 bib1.bibx20 bib1.bibx21" id="text.15"/>.</p>
      <p id="d2e1760">For the creation of both sets of ADMs, the same CERES Ed4SSF (Edition 4.0 Single Scanner Footprint) observations between 2000 and 2005 have been used. In this period, CERES aboard Aqua and Terra measured in the rotating azimuth plane scan mode, providing angular coverage for the ADM construction. The CERES Ed4SSF dataset of Aqua and Terra (described in <xref ref-type="bibr" rid="bib1.bibx17" id="altparen.16"/>) combines MODIS and CERES L2 data. The observations were grouped into sun–observer bins (<sup>Δ</sup>) spanning a 2° <inline-formula><mml:math id="M82" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2° hemispherical grid. Only observations with more than 95 % water surface, more than 0.1 % cloud fraction, and solar zenith angles between 0 and 82° have been used. In the case of <inline-formula><mml:math id="M83" display="inline"><mml:mrow><mml:mi>ln⁡</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi>f</mml:mi></mml:mrow></mml:mfenced></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M84" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 6 (where <inline-formula><mml:math id="M85" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula> is in %) a look-up table approach has been used instead of sigmoidal fit in sun glint affected geometries (sun glint angle <inline-formula><mml:math id="M86" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 20°). Further explanation on the selection of data and the methodology to fit the two approaches can be found in <xref ref-type="bibr" rid="bib1.bibx21" id="text.17"/>. By using two extra retrieved parameters (<inline-formula><mml:math id="M87" display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and ACWV), the semi-physical approach is affected by additional retrieval uncertainties.</p>
      <p id="d2e1835">To explore the research questions raised above, 125 semi-synthetical 30 <inline-formula><mml:math id="M88" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 30 km<sup>2</sup> 3D-cloud scenes with a horizontal resolution of 1 km and varying mean optical thicknesses (<inline-formula><mml:math id="M90" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>), homogeneities (<inline-formula><mml:math id="M91" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula>) and droplet number concentrations (<inline-formula><mml:math id="M92" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) are generated. The scenes are based on MODIS observations, and the vertical dimension is added using cloud adiabatic theory. The exact procedure is explained below.</p>
</sec>
</sec>
<sec id="Ch1.S2.SS3">
  <label>2.3</label><title>Brief Recap on Cloud Adiabatic Theory</title>
      <p id="d2e1891">Following the adiabatic theory described, for example, in <xref ref-type="bibr" rid="bib1.bibx3" id="text.18"/> and <xref ref-type="bibr" rid="bib1.bibx28" id="text.19"/>, the vertical profile of cloud liquid water content (LWC) can be approximated  by Eq. (<xref ref-type="disp-formula" rid="Ch1.E10"/>). The mean cloud volume radius (<inline-formula><mml:math id="M93" display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">vol</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for a given layer depends on the amount of liquid water in the layer LWC and the concentration of cloud droplets (<inline-formula><mml:math id="M94" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). The effective radius (<inline-formula><mml:math id="M95" display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is related to <inline-formula><mml:math id="M96" display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">vol</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> via the constant <inline-formula><mml:math id="M97" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> (see Eq. <xref ref-type="disp-formula" rid="Ch1.E12"/>).

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M98" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E10"><mml:mtd><mml:mtext>10</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mtext mathvariant="normal">LWC</mml:mtext><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo>⋅</mml:mo><mml:mi>z</mml:mi></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E11"><mml:mtd><mml:mtext>11</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">vol</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mo mathsize="1.5em">(</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">3</mml:mn><mml:mtext>LWC</mml:mtext></mml:mrow><mml:mrow><mml:mn mathvariant="normal">4</mml:mn><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo mathsize="1.5em">)</mml:mo><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E12"><mml:mtd><mml:mtext>12</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msup><mml:mi>k</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">vol</mml:mi></mml:msub></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

          where <inline-formula><mml:math id="M99" display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> [m] is the height from cloud base, <inline-formula><mml:math id="M100" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula> [1] the degree of adiabaticity, <inline-formula><mml:math id="M101" display="inline"><mml:mi mathvariant="normal">Γ</mml:mi></mml:math></inline-formula> [g m<sup>−3</sup> m<sup>−1</sup>] the adiabatic rate of increase of liquid water content, and <inline-formula><mml:math id="M104" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> [cm<sup>−3</sup>] the cloud droplet number concentration. Following the equations above, the optical thickness <inline-formula><mml:math id="M106" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> of the cloud depends only on the geometrical thickness <inline-formula><mml:math id="M107" display="inline"><mml:mi>h</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M108" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (see Eq. <xref ref-type="disp-formula" rid="Ch1.E13"/>).

            <disp-formula id="Ch1.E13" content-type="numbered"><label>13</label><mml:math id="M109" display="block"><mml:mrow><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>(</mml:mo><mml:mi>h</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mi mathvariant="normal">D</mml:mi><mml:mo>⋅</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Γ</mml:mi></mml:mrow></mml:mfenced><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mi>k</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mi>h</mml:mi><mml:mrow><mml:mn mathvariant="normal">5</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></disp-formula>

          where D is a constant. Following <xref ref-type="bibr" rid="bib1.bibx28" id="text.20"/>, the cloud top effective radius (<inline-formula><mml:math id="M110" display="inline"><mml:mrow><mml:msubsup><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>) has been calculated using:

            <disp-formula id="Ch1.E14" content-type="numbered"><label>14</label><mml:math id="M111" display="block"><mml:mrow><mml:msubsup><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup><mml:mo>(</mml:mo><mml:mi>h</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">3</mml:mn><mml:mn mathvariant="normal">4</mml:mn></mml:mfrac></mml:mstyle><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mi>f</mml:mi><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Γ</mml:mi></mml:mrow></mml:mfenced><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:mi>k</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mi>h</mml:mi><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></disp-formula>

          The values used for the parameters and constants are shown in Table <xref ref-type="table" rid="T1"/>.</p>

<table-wrap id="T1"><label>Table 1</label><caption><p id="d2e2359">Values used for the creation of cloud vertical profiles.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="center"/>
     <oasis:colspec colnum="2" colname="col2" align="center"/>
     <oasis:colspec colnum="3" colname="col3" align="center"/>
     <oasis:colspec colnum="4" colname="col4" align="center"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"><inline-formula><mml:math id="M112" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M113" display="inline"><mml:mi mathvariant="normal">Γ</mml:mi></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M114" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M115" display="inline"><mml:mi mathvariant="normal">D</mml:mi></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">1</oasis:entry>
         <oasis:entry colname="col2">1.5</oasis:entry>
         <oasis:entry colname="col3">0.8</oasis:entry>
         <oasis:entry colname="col4">0.0145</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
<sec id="Ch1.S2.SS4">
  <label>2.4</label><title>Creation of semi-Synthetic 3D-Cloud Scenes</title>
      <p id="d2e2441">The following is intended as a simplified approach to explore sensitivities. Despite its idealized nature, the implied relationship between optical depth and effective radius is assumed to be generally reasonable for the cloud cases investigated.</p>
      <p id="d2e2444">For the creation of the cloud scenes, we analyzed a MODIS frame from 5 September 2014, in the south-east Atlantic, covered by marine boundary layer stratocumulus clouds (Fig. <xref ref-type="fig" rid="F2"/>a). In order to obtain realistic ranges of mean cloud optical thickness <inline-formula><mml:math id="M116" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and homogeneities <inline-formula><mml:math id="M117" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> in marine boundary layer clouds, we separated the MODIS frame into 30 <inline-formula><mml:math id="M118" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 30 km<sup>2</sup> boxes, as shown in Fig. <xref ref-type="fig" rid="F2"/>a. For each box, we calculated <inline-formula><mml:math id="M120" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> following Eq. (<xref ref-type="disp-formula" rid="Ch1.E15"/>) and <inline-formula><mml:math id="M121" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> following Eq. (<xref ref-type="disp-formula" rid="Ch1.E16"/>).

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M122" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E15"><mml:mtd><mml:mtext>15</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>=</mml:mo><mml:mi>exp⁡</mml:mi><mml:mo>(</mml:mo><mml:mover accent="true"><mml:mrow><mml:mi>log⁡</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E16"><mml:mtd><mml:mtext>16</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi mathvariant="italic">ν</mml:mi><mml:mo>=</mml:mo><mml:mo mathsize="1.5em">(</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mrow><mml:mtext>SD</mml:mtext><mml:mo>(</mml:mo><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle><mml:msup><mml:mo mathsize="1.5em">)</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

          We found a value range of <inline-formula><mml:math id="M123" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> between 2.8 and 20.1 and of <inline-formula><mml:math id="M124" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> between 2 and 26.</p>

      <fig id="F2" specific-use="star"><label>Figure 2</label><caption><p id="d2e2598"><bold>(a)</bold> MODIS retrieved <inline-formula><mml:math id="M125" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> above south-east Atlantic on 5 September 2014. The frame is separated into 30 <inline-formula><mml:math id="M126" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 30 km<sup>2</sup> boxes. The blue dot denotes the location of St. Helena. <bold>(b)</bold> Example of a gamma distribution of <inline-formula><mml:math id="M128" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> (red line) following <xref ref-type="bibr" rid="bib1.bibx1" id="text.21"/> generated using <inline-formula><mml:math id="M129" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> <inline-formula><mml:math id="M130" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 12.6 and <inline-formula><mml:math id="M131" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M132" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 24.1 from a 30 <inline-formula><mml:math id="M133" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 30 km<sup>2</sup> box of the MODIS frame. In blue the histogram of the <inline-formula><mml:math id="M135" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> values within the box is displayed. <bold>(c)</bold> Vertical profiles of <inline-formula><mml:math id="M136" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>, relative humidity (RH) and H<sub>2</sub>O mixing ratio from radiosonde ascent at St. Helena from 5 September 2014 at 12:00 LT. The dashed black lines indicate the cloud base and the 50th and 95th percentile of cloud tops for all 125 scenes.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f02.png"/>

        </fig>

      <p id="d2e2721">For the creation of idealistic cloud scenes, gamma functions based on <xref ref-type="bibr" rid="bib1.bibx1" id="text.22"/> have been used to calculate PDFs of optical thickness values for the given <inline-formula><mml:math id="M138" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M139" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> pair of the scene (see Fig. <xref ref-type="fig" rid="F2"/>b). In total, 25 PDFs have been created based on five <inline-formula><mml:math id="M140" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> values (2.8, 4.5, 7.4, 12.2, 20.1) and five <inline-formula><mml:math id="M141" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> values between 2 and 26. In the next step, the idealistic range of <inline-formula><mml:math id="M142" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> values (<inline-formula><mml:math id="M143" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M144" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 0.001) for the given <inline-formula><mml:math id="M145" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M146" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> was extracted from each PDF, and the cloud geometrical thickness <inline-formula><mml:math id="M147" display="inline"><mml:mi>h</mml:mi></mml:math></inline-formula> was calculated using Eq. (<xref ref-type="disp-formula" rid="Ch1.E13"/>) for each <inline-formula><mml:math id="M148" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>-bin within the range.</p>
      <p id="d2e2819">Assuming a constant cloud base and <inline-formula><mml:math id="M149" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, the optical thickness <inline-formula><mml:math id="M150" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> depends only on the cloud top height (Eq. <xref ref-type="disp-formula" rid="Ch1.E13"/>). Using Eqs. (<xref ref-type="disp-formula" rid="Ch1.E10"/>) to (<xref ref-type="disp-formula" rid="Ch1.E12"/>) vertical profiles of LWC and <inline-formula><mml:math id="M151" display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are calculated for each <inline-formula><mml:math id="M152" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>-bin. The vertical resolution of the profiles is set to 25 m. For the stratocumulus deck of the MODIS frame (Fig. <xref ref-type="fig" rid="F2"/>a), a very similar cloud base is assumed. Using radiosonde measurements of <inline-formula><mml:math id="M153" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>, and water vapor at 12:00 LT in St. Helena, a cloud base of 761 m was assumed (see Fig. <xref ref-type="fig" rid="F2"/>c). To obtain a realistic spatial distribution of cloud profiles, we found for each scene, the MODIS box with the most similar <inline-formula><mml:math id="M154" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M155" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> values. The profiles are than allocated to the spatial distribution of the <inline-formula><mml:math id="M156" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> values within the box. Table <xref ref-type="table" rid="TA1"/> summarizes the pre-defined <inline-formula><mml:math id="M157" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M158" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of the scenes, as well as the calculated values (<inline-formula><mml:math id="M159" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>, <inline-formula><mml:math id="M160" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M161" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>) after assigning them to the MODIS boxes with the most similar values (<inline-formula><mml:math id="M162" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>).</p>
      <p id="d2e2987">Applying five different <inline-formula><mml:math id="M164" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>'s of 25, 50, 100, 200, and 400 [cm<sup>−3</sup>] resulted in 125 scenes with <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> values ranging from 5.1 to 22.1 <inline-formula><mml:math id="M167" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. Figures <xref ref-type="fig" rid="F3"/> and <xref ref-type="fig" rid="F4"/> display the results, showing the geometrical thickness <inline-formula><mml:math id="M168" display="inline"><mml:mi>h</mml:mi></mml:math></inline-formula> of the clouds for a range of <inline-formula><mml:math id="M169" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M170" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> and for a <inline-formula><mml:math id="M171" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of 25 and 400 [cm<sup>−3</sup>] respectively. The values in red represent the calculated <inline-formula><mml:math id="M173" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>, <inline-formula><mml:math id="M174" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M175" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> after assigning (see also Table <xref ref-type="table" rid="TA1"/>). Comparing Fig. <xref ref-type="fig" rid="F3"/> and Fig. <xref ref-type="fig" rid="F4"/>, we see that to reach the same <inline-formula><mml:math id="M176" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>, the cloud extend must be larger for larger cloud droplets (smaller <inline-formula><mml:math id="M177" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>).</p>

      <fig id="F3" specific-use="star"><label>Figure 3</label><caption><p id="d2e3152">Cloud geometrical thickness for the 25 scenes with varying <inline-formula><mml:math id="M178" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M179" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> and with the <inline-formula><mml:math id="M180" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> set to 25 [cm<sup>−3</sup>]. The numbers in red represent the scene-averaged values, calculated after assigning the generated profiles to the MODIS boxes.</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f03.png"/>

        </fig>

      <fig id="F4" specific-use="star"><label>Figure 4</label><caption><p id="d2e3203">Same as Fig. <xref ref-type="fig" rid="F3"/> but with <inline-formula><mml:math id="M182" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of 400 [cm<sup>−3</sup>].</p></caption>
          <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f04.png"/>

        </fig>

</sec>
<sec id="Ch1.S2.SS5">
  <label>2.5</label><title>Monte Carlos Simulations</title>
      <p id="d2e3245">The 125 semi-synthetic scenes of cloud fields are used as inputs for a Monte Carlo Model <xref ref-type="bibr" rid="bib1.bibx14 bib1.bibx2" id="paren.23"/> to simulate the SW TOA radiances and calculate TOA SW fluxes. For the simulations, cyclical boundary conditions are assumed. For each scene, simulations for 40 viewing zenith angles between <inline-formula><mml:math id="M184" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>77 to 77° along the principal plane and for solar zenith angles of 1, 27, 55, and 75° have been performed. In total, this resulted in 20 000 scenarios. For each simulation, <inline-formula><mml:math id="M185" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">7</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> photons have been used. The ocean surface is Lambertian with a wavelength independent albedo of 0.05. For the hydrometeors, Mie-phase functions with 1800 angular-bins are used. The spectrally-dependent optical properties are computed with the model used in EarthCARE’s ACM-RT product <xref ref-type="bibr" rid="bib1.bibx5" id="paren.24"/>.</p>
      <p id="d2e3272">In order to investigate the contribution of single scattering to the outgoing TOA radiance (research question 3), a histogram of the weighted fraction of the number of scattering events has been stored from the simulation for each scenario.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Results</title>
      <p id="d2e3285">In addition to flux estimates based on ADMs using the semi-physical approach (Sect. <xref ref-type="sec" rid="Ch1.S2.SS2"/>), fluxes based on the currently operational ADMs (Sect. <xref ref-type="sec" rid="Ch1.S2.SS1"/>), reconstructed in <xref ref-type="bibr" rid="bib1.bibx21" id="text.25"/> and based on <xref ref-type="bibr" rid="bib1.bibx17" id="text.26"/>, are estimated. In contrast to the semi-physical ADMs, the currently operational ADMs do not explicitly take into account the cloud droplet effective radius.</p>
      <p id="d2e3298">The estimated fluxes are compared against Monte Carlo simulations. Figure <xref ref-type="fig" rid="F5"/> illustrates Monte Carlo simulated radiances for all scenes with <inline-formula><mml:math id="M186" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M187" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 400 [cm<sup>−3</sup>] and for <inline-formula><mml:math id="M189" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M190" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M191" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>29° and <inline-formula><mml:math id="M192" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M193" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 27°.</p>

      <fig id="F5" specific-use="star"><label>Figure 5</label><caption><p id="d2e3379">Monte Carlo simulations of TOA radiances for scenes in Fig. <xref ref-type="fig" rid="F4"/> and for <inline-formula><mml:math id="M194" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M195" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M196" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>29° and <inline-formula><mml:math id="M197" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M198" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 27°.</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f05.png"/>

      </fig>

      <p id="d2e3435">Figure <xref ref-type="fig" rid="F6"/> displays the Monte Carlo simulated and scenario-averaged radiances <inline-formula><mml:math id="M199" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> (left panel) and corresponding anisotropies (right panel) at <inline-formula><mml:math id="M200" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M201" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 1° along the principal plane and for all scenes with <inline-formula><mml:math id="M202" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M203" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 2.8 and <inline-formula><mml:math id="M204" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M205" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 8 (see Table <xref ref-type="table" rid="TA1"/>) and for different <inline-formula><mml:math id="M206" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. We see the strong dependency of the reflected radiation from the mean cloud droplet size. We also observe single scattering features becoming apparent, such as the broadening of the cloud glory and the shift of the cloud bow towards the direct backscatter with decreasing droplet size (increasing <inline-formula><mml:math id="M207" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>).</p>

      <fig id="F6" specific-use="star"><label>Figure 6</label><caption><p id="d2e3555">Left panel: mean radiance of the MCS used as <inline-formula><mml:math id="M208" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> along <inline-formula><mml:math id="M209" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (principal plane) and for varying <inline-formula><mml:math id="M210" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. For a <inline-formula><mml:math id="M211" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M212" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 1° and for the scene with <inline-formula><mml:math id="M213" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M214" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 2.8 and <inline-formula><mml:math id="M215" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M216" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 8. The vertical lines indicate the location of single scattering phenomena as the cloud bow and cloud glory (around the direct backscatter). Yellow arrows indicate the shift of the cloud bow towards the direct backscatter and red arrows the broadening of the cloud glory with smaller droplets (higher <inline-formula><mml:math id="M217" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). Right panel: corresponding anisotropy values for the different <inline-formula><mml:math id="M218" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> but here expressed via the mean cloud top effective radius <inline-formula><mml:math id="M219" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> of the scene.</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f06.png"/>

      </fig>

      <p id="d2e3694">ADMs based on the sigmoidal and semi-physical approaches are constructed using the scene-averaged cloud parameters <inline-formula><mml:math id="M220" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> for the former, and additionally <inline-formula><mml:math id="M221" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> for latter (see Sect. <xref ref-type="sec" rid="Ch1.S2.SS1"/> and <xref ref-type="sec" rid="Ch1.S2.SS2"/>). All scenes are overcast (<inline-formula><mml:math id="M222" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M223" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 1) and have ACWV <inline-formula><mml:math id="M224" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 0. With the resulting anisotropies <inline-formula><mml:math id="M225" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula>, SW fluxes are estimated using the spatially averaged Monte Carlo simulated radiances <inline-formula><mml:math id="M226" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> (see Fig. <xref ref-type="fig" rid="F5"/>).</p>
      <p id="d2e3789">The upper panel of Fig. <xref ref-type="fig" rid="F7"/> shows the TOA SW fluxes across the principal plane for scenarios with a solar zenith angle of 1° and scenes with an optical thickness of <inline-formula><mml:math id="M227" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> <inline-formula><mml:math id="M228" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 7.4 and homogeneity of <inline-formula><mml:math id="M229" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M230" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 20. The solid lines show the “true” fluxes from the Monte Carlo simulations. The dashed lines represent the flux estimates based on the semi-physical approach (<inline-formula><mml:math id="M231" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mi mathvariant="normal">sp</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and the dotted lines flux estimates based on the sigmoidal approach (<inline-formula><mml:math id="M232" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mi mathvariant="normal">sig</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). The colors of the lines illustrate estimates for scenes with different cloud effective radii. In addition, the colored dots indicate the weighted fraction of photons of the scenario that experienced single scattering before reaching TOA. The lower panel illustrates the parameterized asymmetry parameter <inline-formula><mml:math id="M233" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> used for the semi-physical ADMs. The vertical lines show the location of the cloud bow and the direct backscatter, around which the cloud glory forms.</p>

      <fig id="F7"><label>Figure 7</label><caption><p id="d2e3861">Upper panel: flux estimates using ADM based on the semi-physical (dashed) and based on the sigmoidal (dotted) approach for different droplet number concentrations along the principal plain. The true flux of the Monte Carlo Simulations (MCS) is shown in the solid line. The colored dots represent for each scenario the fraction of photons that has been scattered only once. Lower panel: parameterized asymmetry parameter <inline-formula><mml:math id="M234" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> used for semi-physical approach.</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f07.png"/>

      </fig>

      <p id="d2e3882">The results show that a decrease of <inline-formula><mml:math id="M235" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from 16 to 5.3 <inline-formula><mml:math id="M236" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> produces up to 100 W m<sup>−2</sup> higher fluxes at TOA for the same <inline-formula><mml:math id="M238" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>.</p>
      <p id="d2e3931">Around the direct backscatter direction, where the cloud glory contributes to the observed radiance, the ADMs generated using the semi-physical approach result in flux estimates that are closer to the simulations. This is also the case at the cloud bow around <inline-formula><mml:math id="M239" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">40</mml:mn></mml:mrow></mml:math></inline-formula>°. Particularly for small droplet sizes (high droplet number concentrations), where the enhanced reflectance due to single scattering effects is largest, the currently operational approach underestimates the fluxes. Due to the bin-wise optimized asymmetry parameter (bottom panel), the semi-physical approach is able to capture single scattering features such as broadening and shift in the forward direction of the cloud glory, as well as the shift towards the direct backscatter of the cloud bow with decreasing <inline-formula><mml:math id="M240" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx21" id="paren.27"/>. The results illustrate that this leads to more accurate flux estimates in these geometries comparing to the sigmoidal approach.</p>
      <p id="d2e3961">For angles influenced by the cloud bow or cloud glory, an enhanced contribution of single scattering (colored dots) to the reflected radiance is clearly visible. Furthermore, the single scattering fraction increases with decreasing <inline-formula><mml:math id="M241" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. This underpins the hypothesis that the adjustments of <inline-formula><mml:math id="M242" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> (lower panel) during the bin-wise optimization procedure <xref ref-type="bibr" rid="bib1.bibx20" id="paren.28"/> are primarily attributable to perceived single scattering effects, such as the broadening and shift of the cloud glory and the shift of cloud bow.</p>
      <p id="d2e3992">Figure <xref ref-type="fig" rid="F8"/> shows the results for <inline-formula><mml:math id="M243" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for 27 and 55° with similar results. At geometries influenced by the cloud glory, the sigmoidal approach performs well under average microphysical conditions (e.g, <inline-formula><mml:math id="M244" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M245" display="inline"><mml:mo>≈</mml:mo></mml:math></inline-formula> 10 <inline-formula><mml:math id="M246" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>) but overestimates the fluxes at high and underestimates them at low <inline-formula><mml:math id="M247" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. This agrees with Fig. <xref ref-type="fig" rid="F1"/> where the predicted radiances using the sigmoidal approach (right panel) correspond well with the semi-physical approach using a typical mean effective radius of 10 <inline-formula><mml:math id="M248" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> (second panel) but are lower for small droplets (first panel) and higher for large droplets (third panel).</p>

      <fig id="F8"><label>Figure 8</label><caption><p id="d2e4068">As Fig. <xref ref-type="fig" rid="F7"/> upper panel but for a <inline-formula><mml:math id="M249" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of 27 and 55°.</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f08.png"/>

      </fig>

      <p id="d2e4091">At high and low <inline-formula><mml:math id="M250" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, both approaches struggle because fewer training data was available for these geometries. In sun-glint affected geometries both approaches have problems in estimate accurately the fluxes, but the semi-physical approach generally deviates even more. These findings are consistent with higher uncertainties of the models for these geometries found in <xref ref-type="bibr" rid="bib1.bibx20" id="text.29"/>.</p>
      <p id="d2e4108">In Fig. <xref ref-type="fig" rid="F9"/>, the flux deviations for scenes with a <inline-formula><mml:math id="M251" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of 400 cm<sup>−3</sup> and the corresponding highest homogeneity are illustrated for varying <inline-formula><mml:math id="M253" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M254" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The upper panel displays the deviation of the flux estimates using semi-physical (<inline-formula><mml:math id="M255" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>F</mml:mi><mml:mi mathvariant="normal">sp</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and the lower panel using sigmoidal based ADMs (<inline-formula><mml:math id="M256" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>F</mml:mi><mml:mi mathvariant="normal">sig</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). In the top of each panel, the average over all <inline-formula><mml:math id="M257" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> (black line) and the standard deviation (gray shadows) are shown. The doted isoline indicates areas where the differences exceed the EarthCARE mission goal of <inline-formula><mml:math id="M258" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> W m<sup>−2</sup>.</p>

      <fig id="F9" specific-use="star"><label>Figure 9</label><caption><p id="d2e4218">Deviation of fluxes estimated (<inline-formula><mml:math id="M260" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>F</mml:mi></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M261" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M262" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mi mathvariant="normal">MCS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M263" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M264" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mi mathvariant="normal">est</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) using ADM's based on the semi-physical approach (upper panel) and on the sigmoidal approach (lower panel) from the fluxes of MCS along the principal plane and for varying <inline-formula><mml:math id="M265" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M266" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>. The <inline-formula><mml:math id="M267" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of the scenes is 400 [cm<sup>−3</sup>] and for <inline-formula><mml:math id="M269" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> always the scene with the highest homogeneity is selected. The dotted blue and red lines represent the <inline-formula><mml:math id="M270" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>10 and 10 W m<sup>−2</sup> threshold. On top of each panel the deviation averaged over all optical thicknesses is shown. The shaded areas mark the 5th and 95th percentiles. The vertical lines indicate the direct backscatter and the cloud bow (<inline-formula><mml:math id="M272" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M273" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 40°).</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f09.png"/>

      </fig>

      <p id="d2e4363">In general, the semi-physical approach deviates less from the simulations, particularly in viewing geometries around the cloud glory and cloud bow. This is the case for all optical thicknesses and solar zenith angles, but for small <inline-formula><mml:math id="M274" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> the effect is more distinctive. The deviations in instantaneous flux estimates using the semi-physical approach compared to the currently operational approach can be reduced by up to 25 W m<sup>−2</sup> or even more. In the sun glint affected geometries, both approaches show large uncertainties. Both absolute and relative deviations (not shown) increase with smaller <inline-formula><mml:math id="M276" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> in this region. This indicates that even in overcast cases, with high optical thicknesses, the sun-glint significantly influences the TOA radiances. Figure <xref ref-type="fig" rid="F10"/> illustrates for each <inline-formula><mml:math id="M277" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> the box-whisker plots (<inline-formula><mml:math id="M278" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M279" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 500) of flux deviations (<inline-formula><mml:math id="M280" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>F</mml:mi></mml:mrow></mml:math></inline-formula>) for scenarios in the backward (left) and forward direction (right), and for different droplet number concentrations. Particularly at extreme <inline-formula><mml:math id="M281" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (e.g., 25 and 400 cm<sup>−3</sup>), the semi-physical approach deviates less from the simulations in the backward direction. For this cases the median deviation of the 5000 scenarios can be reduced by up to 7 W m<sup>−2</sup> (such as for <inline-formula><mml:math id="M284" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M285" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 55° and <inline-formula><mml:math id="M286" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). This can be explained by the fact that the sigmoidal  approach does not explicitly take <inline-formula><mml:math id="M287" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> into account. By using observations independently on their microphysics, the sigmoidal approach produces in the backward direction best estimates at average <inline-formula><mml:math id="M288" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> such as 50 and 100 cm<sup>−3</sup>, but is less accurate in extreme high or low <inline-formula><mml:math id="M290" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub><mml:mi>s</mml:mi></mml:mrow></mml:math></inline-formula>. For the forward direction where single scattering features are less important, the sigmoidal approach generally does not perform better. Table <xref ref-type="table" rid="T2"/> lists the probability of <inline-formula><mml:math id="M291" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>F</mml:mi></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M292" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> 10 W m<sup>−2</sup> for scenes with different <inline-formula><mml:math id="M294" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and for scenarios calculated for the backward, forward and nadir direction. For high <inline-formula><mml:math id="M295" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> the semi-physical approach can reduce the probability by up to 20 %. The mean absolute relative error was found to decrease with increasing <inline-formula><mml:math id="M296" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M297" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula>, and to increase with larger <inline-formula><mml:math id="M298" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and, particularly for the sigmoidal approach, with decreasing <inline-formula><mml:math id="M299" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> (increasing <inline-formula><mml:math id="M300" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) (not shown). In Fig. <xref ref-type="fig" rid="F11"/> the 30 <inline-formula><mml:math id="M301" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 30 km<sup>2</sup> scenes (<inline-formula><mml:math id="M303" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M304" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 55°) have been divided into subdomains with sizes of 25, 20, 15 and 10 km to explore the dependency of the flux estimates on domain size. The variability in <inline-formula><mml:math id="M305" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>F</mml:mi></mml:mrow></mml:math></inline-formula> increases with smaller domain sizes. As in the case of 30 km, the semi-physical approach produces better estimates in the backward direction and for domains with extremely high or low <inline-formula><mml:math id="M306" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math id="M307" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for all resolutions. For a domain size of 10 <inline-formula><mml:math id="M308" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10 km<sup>2</sup> both approaches show a positive bias. As EarthCARE's assessment domain has a size of 100 km<sup>2</sup>, the results might be of interest for the validation of the BMA-FLX product.</p>

      <fig id="F10" specific-use="star"><label>Figure 10</label><caption><p id="d2e4760">Box-Whisker plots showing flux deviations for the different <inline-formula><mml:math id="M311" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> using <inline-formula><mml:math id="M312" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M313" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 500 scenes of all <inline-formula><mml:math id="M314" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M315" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> and for the left side of each panel of <inline-formula><mml:math id="M316" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>77 <inline-formula><mml:math id="M317" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M318" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M319" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 0 and for the right side 0 <inline-formula><mml:math id="M320" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M321" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M322" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 77. The upper and lower limits represent the 95th and 5th percentiles.</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f10.png"/>

      </fig>

<table-wrap id="T2"><label>Table 2</label><caption><p id="d2e4874">Table showing the probability in % of <inline-formula><mml:math id="M323" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>F</mml:mi></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M324" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> 10 W m<sup>−2</sup>. Forward includes all scenarios of 0 <inline-formula><mml:math id="M326" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M327" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M328" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 77, backward of 0 <inline-formula><mml:math id="M329" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M330" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M331" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M332" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>77 and nadir of <inline-formula><mml:math id="M333" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1 <inline-formula><mml:math id="M334" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M335" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M336" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 1. The italic numbers are for the semi-physical approach and bold numbers for the sigmoidal approach.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="center"/>
     <oasis:colspec colnum="3" colname="col3" align="center"/>
     <oasis:colspec colnum="4" colname="col4" align="center"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"><inline-formula><mml:math id="M337" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Forward</oasis:entry>
         <oasis:entry colname="col3">Backward</oasis:entry>
         <oasis:entry colname="col4">Nadir</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">25</oasis:entry>
         <oasis:entry colname="col2"><italic>35.2</italic>/<bold>34.1</bold></oasis:entry>
         <oasis:entry colname="col3"><italic>23.0</italic>/<bold>31.5</bold></oasis:entry>
         <oasis:entry colname="col4"><italic>39.5</italic>/<bold>38.5</bold></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">50</oasis:entry>
         <oasis:entry colname="col2"><italic>33.7</italic>/<bold>31.0</bold></oasis:entry>
         <oasis:entry colname="col3"><italic>27.0</italic>/<bold>23.9</bold></oasis:entry>
         <oasis:entry colname="col4"><italic>41.0</italic>/<bold>33.0</bold></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">100</oasis:entry>
         <oasis:entry colname="col2"><italic>34.0</italic>/<bold>31.5</bold></oasis:entry>
         <oasis:entry colname="col3"><italic>27.1</italic>/<bold>24.3</bold></oasis:entry>
         <oasis:entry colname="col4"><italic>37.0</italic>/<bold>31.0</bold></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">200</oasis:entry>
         <oasis:entry colname="col2"><italic>36.7</italic>/<bold>42.8</bold></oasis:entry>
         <oasis:entry colname="col3"><italic>31.0</italic>/<bold>35.1</bold></oasis:entry>
         <oasis:entry colname="col4"><italic>38.0</italic>/<bold>43.5</bold></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">400</oasis:entry>
         <oasis:entry colname="col2"><italic>43.8</italic>/<bold>58.2</bold></oasis:entry>
         <oasis:entry colname="col3"><italic>41.0</italic>/<bold>55.8</bold></oasis:entry>
         <oasis:entry colname="col4"><italic>58.5</italic>/<bold>79.5</bold></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <fig id="F11" specific-use="star"><label>Figure 11</label><caption><p id="d2e5178">As Fig. <xref ref-type="fig" rid="F10"/> with <inline-formula><mml:math id="M338" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M339" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 55° but for domain sizes of 25, 20, 15 and 10 km.</p></caption>
        <graphic xlink:href="https://amt.copernicus.org/articles/19/935/2026/amt-19-935-2026-f11.png"/>

      </fig>

</sec>
<sec id="Ch1.S4" sec-type="conclusions">
  <label>4</label><title>Conclusion and Discussion</title>
      <p id="d2e5215">In this study, Top of Atmosphere (TOA) shortwave (SW) radiances are simulated along the principal plane for 125 semi-synthetic 3D scenes of marine boundary layer stratocumulus clouds with varying mean cloud optical thickness, cloud homogeneities, and mean effective radius. Seeking TOA SW flux closure above liquid clouds, two sets of ADMs based on the semi-physical <xref ref-type="bibr" rid="bib1.bibx21 bib1.bibx20" id="paren.30"/> and sigmoidal approach <xref ref-type="bibr" rid="bib1.bibx17" id="paren.31"/> are compared against the fluxes calculated using a Monte Carlo Model <xref ref-type="bibr" rid="bib1.bibx14 bib1.bibx2" id="paren.32"/>.</p>
      <p id="d2e5227">Averaged over all analyzed scenarios, the mean absolute relative error decreases with increasing <inline-formula><mml:math id="M340" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M341" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula>, and increases with increasing <inline-formula><mml:math id="M342" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and, particularly for the sigmoidal approach, with decreasing <inline-formula><mml:math id="M343" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> (Research question 1). Furthermore, the microphysically aware semi-physical approach reduces the errors in instantaneous flux estimates by up to 25 W m<sup>−2</sup> compared to the sigmoidal approach. The improvements are found to be largest for geometries in the backward direction and for scenes where microphysics deviated most from mean conditions, such as scenes with extremely high or low <inline-formula><mml:math id="M345" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math id="M346" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). The median deviation of these scenarios (backward direction and different <inline-formula><mml:math id="M347" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M348" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M349" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 500) is improved for all <inline-formula><mml:math id="M350" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M351" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> by up to 7 W m<sup>−2</sup>. Although this study only covers the principal plane, the results show the potential of improving SW flux estimates by explicitly incorporating cloud microphysics in ADMs. Similar results have been found in <xref ref-type="bibr" rid="bib1.bibx21" id="text.33"/>, where the two radiance-to-irradiance approaches have been compared using satellite data (Research question 2). Analyzing the Monte Carlo Simulations (MCS), the adjustments of the parameterized asymmetry parameter <inline-formula><mml:math id="M353" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> could be related to changes in the fraction of single scattering events contributing to the TOA radiance signal. The changes in the single scattering fraction are associated with phenomena such as cloud bow or cloud glory, which depend on cloud microphysical properties (Research question 3).</p>
      <p id="d2e5388">By explicitly incorporating cloud microphysical properties through the effective radius, the semi-physical approach substantially reduces flux estimation errors for the investigated scenarios, particularly for those affected by single-scattering phenomena such as the cloud glory and the cloud bow. As these phenomena are strongest in the backward direction, the improvements compared to the currently operational approach are most pronounced in scenarios with corresponding observational geometries. For sun glint affected geometries, the flux estimates show large variabilities, and any interpretation should be done with caution.</p>
      <p id="d2e5391">Using the optimized <inline-formula><mml:math id="M354" display="inline"><mml:mrow><mml:msup><mml:mi>g</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>, the semi-physical approach is able to capture the shift of the cloud bow and the broadening of the cloud glory with decreasing droplet size, explaining the more accurate estimates in these geometries.</p>
      <p id="d2e5406">The findings of this study encourage further research on microphysically aware ADMs. For the radiative closure experiment of the EarthCARE mission, launched in May 2024 <xref ref-type="bibr" rid="bib1.bibx25" id="paren.34"/>, the semi-physical approach shows potential to improve SW flux estimates. EarthCARE aims to achieve radiative closure by comparing simulated fluxes from active and passive instruments aboard the satellite with estimates from the broadband radiometer (BBR) <xref ref-type="bibr" rid="bib1.bibx23" id="paren.35"/>. Particularly for observational geometries in the backward-scattering direction, the semi-physical approach reduces potential misinterpretations of flux deviations that exceed the mission goal of 10 W m<sup>−2</sup>, but actually arise from uncertainties in the SW flux estimates. Although EarthCARE’s observational geometries lie outside the principal plane investigated in this study (e.g., <xref ref-type="bibr" rid="bib1.bibx19" id="altparen.36"/>), they are likewise influenced by variations in cloud microphysics and single-scattering phenomena.</p>
      <p id="d2e5430">When assessing radiative closure with EarthCARE, it is important to remember that BBR-based fluxes are estimates rather than direct measurements, and that their uncertainties depend on surface type, atmospheric conditions, and sun–satellite geometry. For low <inline-formula><mml:math id="M356" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> (high <inline-formula><mml:math id="M357" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), the semi-physical approach substantially reduces the probability of <inline-formula><mml:math id="M358" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>F</mml:mi></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M359" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> 10 W m<sup>−2</sup>. For both approaches, flux uncertainties increase with decreasing footprint size. Future work should further investigate the sensitivities to footprint size, retrieval errors (e.g., of above-cloud water vapor and <inline-formula><mml:math id="M361" display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), noise, and varying observational conditions.</p>
      <p id="d2e5501">Overall, the results highlight that explicitly incorporating cloud microphysical information into ADMs is a promising pathway for improving TOA SW flux estimates above clouds. Unlike previous Earth radiation budget missions that focused mainly on minimizing global flux biases, EarthCARE’s emphasis on radiative closure may particularly benefit from microphysically aware instantaneous flux estimates.</p>
</sec>

      
      </body>
    <back><app-group>

<app id="App1.Ch1.S1">
  <label>Appendix A</label><title/>

<table-wrap id="TA1"><label>Table A1</label><caption><p id="d2e5518">Table showing pre-selected <inline-formula><mml:math id="M362" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M363" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for the 25 scenes and the calculated <inline-formula><mml:math id="M364" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>, <inline-formula><mml:math id="M365" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M366" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> after assigning the profiles to the boxes of MODIS observations with the most similar <inline-formula><mml:math id="M367" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M368" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> values. The calculated values are for the scenes with <inline-formula><mml:math id="M369" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M370" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 25.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="5">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="center"/>
     <oasis:colspec colnum="3" colname="col3" align="center"/>
     <oasis:colspec colnum="4" colname="col4" align="center"/>
     <oasis:colspec colnum="5" colname="col5" align="center"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Scene</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M371" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M372" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">pre</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M373" display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M374" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ν</mml:mi><mml:mi mathvariant="normal">o</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M375" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">τ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>, <inline-formula><mml:math id="M376" display="inline"><mml:mi mathvariant="italic">ν</mml:mi></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M377" display="inline"><mml:mrow><mml:msubsup><mml:mover accent="true"><mml:mi>r</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">eff</mml:mi><mml:mi mathvariant="normal">ctop</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">1</oasis:entry>
         <oasis:entry colname="col2">2.8, 1.1</oasis:entry>
         <oasis:entry colname="col3">4.2, 1.5</oasis:entry>
         <oasis:entry colname="col4">4.2, 1.7</oasis:entry>
         <oasis:entry colname="col5">15.9</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2</oasis:entry>
         <oasis:entry colname="col2">2.8, 2.8</oasis:entry>
         <oasis:entry colname="col3">3.9, 2.7</oasis:entry>
         <oasis:entry colname="col4">3.8, 3.2</oasis:entry>
         <oasis:entry colname="col5">15.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">3</oasis:entry>
         <oasis:entry colname="col2">2.8, 4.6</oasis:entry>
         <oasis:entry colname="col3">3.6, 4.7</oasis:entry>
         <oasis:entry colname="col4">3.6, 5.3</oasis:entry>
         <oasis:entry colname="col5">15.4</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">4</oasis:entry>
         <oasis:entry colname="col2">2.8, 6.3</oasis:entry>
         <oasis:entry colname="col3">4.3, 7.8</oasis:entry>
         <oasis:entry colname="col4">4.3, 11.0</oasis:entry>
         <oasis:entry colname="col5">15.9</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">5</oasis:entry>
         <oasis:entry colname="col2">2.8, 8.0</oasis:entry>
         <oasis:entry colname="col3">4.4, 8.4</oasis:entry>
         <oasis:entry colname="col4">4.4, 8.7</oasis:entry>
         <oasis:entry colname="col5">16.0</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">6</oasis:entry>
         <oasis:entry colname="col2">4.5, 1.1</oasis:entry>
         <oasis:entry colname="col3">5.3, 1.1</oasis:entry>
         <oasis:entry colname="col4">5.2, 1.2</oasis:entry>
         <oasis:entry colname="col5">16.7</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">7</oasis:entry>
         <oasis:entry colname="col2">4.5, 4.6</oasis:entry>
         <oasis:entry colname="col3">4.4, 4.7</oasis:entry>
         <oasis:entry colname="col4">4.4, 4.9</oasis:entry>
         <oasis:entry colname="col5">16.0</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">8</oasis:entry>
         <oasis:entry colname="col2">4.5, 8.0</oasis:entry>
         <oasis:entry colname="col3">5.2, 7.8</oasis:entry>
         <oasis:entry colname="col4">5.2, 7.7</oasis:entry>
         <oasis:entry colname="col5">16.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">9</oasis:entry>
         <oasis:entry colname="col2">4.5, 11.5</oasis:entry>
         <oasis:entry colname="col3">4.4, 10.9</oasis:entry>
         <oasis:entry colname="col4">4.4, 10.5</oasis:entry>
         <oasis:entry colname="col5">16.0</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">10</oasis:entry>
         <oasis:entry colname="col2">4.5, 15.0</oasis:entry>
         <oasis:entry colname="col3">5.8, 15.5</oasis:entry>
         <oasis:entry colname="col4">5.8, 14.9</oasis:entry>
         <oasis:entry colname="col5">16.9</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">11</oasis:entry>
         <oasis:entry colname="col2">7.4, 1.1</oasis:entry>
         <oasis:entry colname="col3">7.8, 1.5</oasis:entry>
         <oasis:entry colname="col4">7.7, 1.5</oasis:entry>
         <oasis:entry colname="col5">18.0</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">12</oasis:entry>
         <oasis:entry colname="col2">7.4, 5.8</oasis:entry>
         <oasis:entry colname="col3">7.5, 5.8</oasis:entry>
         <oasis:entry colname="col4">7.5, 5.7</oasis:entry>
         <oasis:entry colname="col5">17.8</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">13</oasis:entry>
         <oasis:entry colname="col2">7.4, 10.5</oasis:entry>
         <oasis:entry colname="col3">7.4, 10.5</oasis:entry>
         <oasis:entry colname="col4">7.4, 10.5</oasis:entry>
         <oasis:entry colname="col5">17.8</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">14</oasis:entry>
         <oasis:entry colname="col2">7.4, 15.3</oasis:entry>
         <oasis:entry colname="col3">7.6, 15.1</oasis:entry>
         <oasis:entry colname="col4">7.6, 14.6</oasis:entry>
         <oasis:entry colname="col5">17.8</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">15</oasis:entry>
         <oasis:entry colname="col2">7.4, 20.0</oasis:entry>
         <oasis:entry colname="col3">6.6, 19.1</oasis:entry>
         <oasis:entry colname="col4">6.6, 19.0</oasis:entry>
         <oasis:entry colname="col5">17.4</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">16</oasis:entry>
         <oasis:entry colname="col2">12.2, 2.0</oasis:entry>
         <oasis:entry colname="col3">12.3, 2.3</oasis:entry>
         <oasis:entry colname="col4">12.3, 2.3</oasis:entry>
         <oasis:entry colname="col5">19.7</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">17</oasis:entry>
         <oasis:entry colname="col2">12.2, 7.8</oasis:entry>
         <oasis:entry colname="col3">12.0, 7.9</oasis:entry>
         <oasis:entry colname="col4">12.0, 7.8</oasis:entry>
         <oasis:entry colname="col5">19.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">18</oasis:entry>
         <oasis:entry colname="col2">12.2, 13.5</oasis:entry>
         <oasis:entry colname="col3">12.2, 13.6</oasis:entry>
         <oasis:entry colname="col4">12.2, 13.5</oasis:entry>
         <oasis:entry colname="col5">19.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">19</oasis:entry>
         <oasis:entry colname="col2">12.2, 19.2</oasis:entry>
         <oasis:entry colname="col3">11.9, 19.8</oasis:entry>
         <oasis:entry colname="col4">11.9, 19.3</oasis:entry>
         <oasis:entry colname="col5">19.5</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">20</oasis:entry>
         <oasis:entry colname="col2">12.2, 25.0</oasis:entry>
         <oasis:entry colname="col3">12.6, 24.1</oasis:entry>
         <oasis:entry colname="col4">12.6, 23.3</oasis:entry>
         <oasis:entry colname="col5">19.7</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">21</oasis:entry>
         <oasis:entry colname="col2">20.1, 5.0</oasis:entry>
         <oasis:entry colname="col3">18.8, 5.5</oasis:entry>
         <oasis:entry colname="col4">18.8, 5.5</oasis:entry>
         <oasis:entry colname="col5">21.4</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">22</oasis:entry>
         <oasis:entry colname="col2">20.1, 8.8</oasis:entry>
         <oasis:entry colname="col3">19.6, 9.1</oasis:entry>
         <oasis:entry colname="col4">19.6, 9.2</oasis:entry>
         <oasis:entry colname="col5">21.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">23</oasis:entry>
         <oasis:entry colname="col2">20.1, 12.5</oasis:entry>
         <oasis:entry colname="col3">21.5, 13.9</oasis:entry>
         <oasis:entry colname="col4">21.5, 14.0</oasis:entry>
         <oasis:entry colname="col5">22.0</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">24</oasis:entry>
         <oasis:entry colname="col2">20.1, 16.2</oasis:entry>
         <oasis:entry colname="col3">22.2, 14.6</oasis:entry>
         <oasis:entry colname="col4">22.2, 14.4</oasis:entry>
         <oasis:entry colname="col5">22.1</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">25</oasis:entry>
         <oasis:entry colname="col2">20.1, 20.0</oasis:entry>
         <oasis:entry colname="col3">20.3, 20.7</oasis:entry>
         <oasis:entry colname="col4">20.3, 20.3</oasis:entry>
         <oasis:entry colname="col5">21.7</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>


</app>
  </app-group><notes notes-type="codedataavailability"><title>Code and data availability</title>

      <p id="d2e6198">The analysis code and data products used to produce the figures and results presented in this manuscript are publicly available and can be accessed via the DOI: <ext-link xlink:href="https://doi.org/10.5281/zenodo.18460315" ext-link-type="DOI">10.5281/zenodo.18460315</ext-link> <xref ref-type="bibr" rid="bib1.bibx13" id="paren.37"/>.</p>
  </notes><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d2e6210">FT, NM and HB designed the study. NM created the input scenes, performed the analysis and wrote the paper. HB carried out the Monte Carlo Simulations. RP and JF supervised the work.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d2e6217">The contact author has declared that none of the authors has any competing interests.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <p id="d2e6224">Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this paper. The authors bear the ultimate responsibility for providing appropriate place names. Views expressed in the text are those of the authors and do not necessarily reflect the views of the publisher.</p>
  </notes><ack><title>Acknowledgements</title><p id="d2e6231">We thank the reviewers for their constructive and valuable feedback. Language refinement and grammar correction were assisted by AI-based tools. The authors are solely responsible for the scientific content and conclusions. This research has been supported by the European Space Agency (ESA; contract nos. 4000112019/14/NL/CT (CLARA), 4000134661/21/NL/AD (CARDINAL), and 4000133155/20/NL/FF/tfd (ICERAD)).</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d2e6237">This research has been supported by the European Space Agency (grant nos. 4000112019/14/NL/CT, 4000134661/21/NL/AD, and 4000133155/20/NL/FF/tfd).</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d2e6243">This paper was edited by Bernhard Mayer and reviewed by two anonymous referees.</p>
  </notes><ref-list>
    <title>References</title>

      <ref id="bib1.bibx1"><label>Barker et al.(1996)</label><mixed-citation>Barker, H. W., Wiellicki, B. A., and Parker, L.: A Parameterization for Computing Grid-Averaged Solar Fluxes for Inhomogeneous Marine Boundary Layer Clouds. Part II: Validation Using Satellite Data, J. Atmos. Sci., 53, 2304–2316, <ext-link xlink:href="https://doi.org/10.1175/1520-0469(1996)053&lt;2304:APFCGA&gt;2.0.CO;2" ext-link-type="DOI">10.1175/1520-0469(1996)053&lt;2304:APFCGA&gt;2.0.CO;2</ext-link>, 1996.</mixed-citation></ref>
      <ref id="bib1.bibx2"><label>Barker et al.(2003) </label><mixed-citation>Barker, H. W., Goldstein, R. K., and Stevens, D. E.: Monte Carlo Simulation of Solar Reflectances for Cloudy Atmospheres, J. Atmos. Sci., 60, 1881–1894, <ext-link xlink:href="https://doi.org/10.1175/1520-0469(2003)060&lt;1881:MCSOSR&gt;2.0.CO;2" ext-link-type="DOI">10.1175/1520-0469(2003)060&lt;1881:MCSOSR&gt;2.0.CO;2</ext-link>, 2003.</mixed-citation></ref>
      <ref id="bib1.bibx3"><label>Brenguier et al.(2000)</label><mixed-citation>Brenguier, J.-L., Pawlowska, H., Schüller, L., Preusker, R., Fischer, J., and  Fouquart, Y.: Radiative Properties of Boundary Layer Clouds: Droplet Effective Radius versus Number Concentration, J. Atmos. Sci., 57, 803–821,  <ext-link xlink:href="https://doi.org/10.1175/1520-0469(2000)057&lt;0803:RPOBLC&gt;2.0.CO;2" ext-link-type="DOI">10.1175/1520-0469(2000)057&lt;0803:RPOBLC&gt;2.0.CO;2</ext-link>, 2000.</mixed-citation></ref>
      <ref id="bib1.bibx4"><label>Coakley and Chylek(1975)</label><mixed-citation>Coakley, J. A. and Chylek, P.: The Two-Stream Approximation in Radiative  Transfer: Including the Angle of the Incident Radiation, J. Atmos. Sci., 32, 409–418, <ext-link xlink:href="https://doi.org/10.1175/1520-0469(1975)032&lt;0409:ttsair&gt;2.0.co;2" ext-link-type="DOI">10.1175/1520-0469(1975)032&lt;0409:ttsair&gt;2.0.co;2</ext-link>, 1975.</mixed-citation></ref>
      <ref id="bib1.bibx5"><label>Cole et al.(2023)</label><mixed-citation>Cole, J. N. S., Barker, H. W., Qu, Z., Villefranque, N., and Shephard, M. W.: Broadband radiative quantities for the EarthCARE mission: the ACM-COM and ACM-RT products, Atmos. Meas. Tech., 16, 4271–4288, <ext-link xlink:href="https://doi.org/10.5194/amt-16-4271-2023" ext-link-type="DOI">10.5194/amt-16-4271-2023</ext-link>, 2023.</mixed-citation></ref>
      <ref id="bib1.bibx6"><label>Dewitte et al.(2008)</label><mixed-citation>Dewitte, S., Gonzalez, L., Clerbaux, N., Ipe, A., Bertrand, C., and De Paepe,  B.: The Geostationary Earth Radiation Budget Edition 1 data processing  algorithms, Adv. Space Res., 41, 1906–1913,  <ext-link xlink:href="https://doi.org/10.1016/j.asr.2007.07.042" ext-link-type="DOI">10.1016/j.asr.2007.07.042</ext-link>, 2008. </mixed-citation></ref>
      <ref id="bib1.bibx7"><label>Domenech and Wehr(2011)</label><mixed-citation>Domenech, C. and Wehr, T.: Use of Artificial Neural Networks to Retrieve TOA SW Radiative Fluxes for the EarthCARE Mission, IEEE T. Geosci. Remote, 49, 1839–1849, <ext-link xlink:href="https://doi.org/10.1109/tgrs.2010.2102768" ext-link-type="DOI">10.1109/tgrs.2010.2102768</ext-link>, 2011.</mixed-citation></ref>
      <ref id="bib1.bibx8"><label>Forster et al.(2021)</label><mixed-citation>Forster, P., Storelvmo, T., Armour, K., Collins, W., Dufresne, J.-L., Frame,  D., Lunt, D. J., Mauritsen, T., Palmer, M. D., Watanabe, M., Wild, M., and  Zhang, H.: The Earth’s Energy Budget, Climate Feedbacks, and Climate  Sensitivity, in: Climate Change 2021: The Physical Science Basis.  Contribution of Working Group I to the Sixth Assessment Report of the  Intergovernmental Panel on Climate Change, edited by: Masson-Delmotte, V.,  Zhai, P., Pirani, A., Connors, S. L., Péan, C., Berger, S., Caud, N., Chen,  Y., Goldfarb, L., Gomis, M. I., Huang, M., Leitzell, K., Lonnoy, E.,  Matthews, J. B. R., Maycock, T. K., Waterfield, T., Yelekçi, O., Yu, R., and  Zhou, B., Cambridge University Press, Cambridge, United  Kingdom and New York, NY, USA, 923–1054, <ext-link xlink:href="https://doi.org/10.1017/9781009157896.009" ext-link-type="DOI">10.1017/9781009157896.009</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bibx9"><label>Gristey et al.(2021)</label><mixed-citation>Gristey, J. J., Su, W., Loeb, N. G., Vonder Haar, T. H., Tornow, F., Schmidt,  S. K., Hakuba, M. Z., Pilewskie, P., and Russell, J. E.: Shortwave radiance  to irradiance conversion for Earth radiation budget satellite observations: A  review, Remote Sensing, 13, 2640, <ext-link xlink:href="https://doi.org/10.3390/rs13132640" ext-link-type="DOI">10.3390/rs13132640</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bibx10"><label>Loeb and Manalo-Smith(2005)</label><mixed-citation>Loeb, N. G. and Manalo-Smith, N.: Top-of-Atmosphere Direct Radiative Effect of Aerosols over Global Oceans from Merged CERES and MODIS Observations, J. Climate, 18, 3506–3526, <ext-link xlink:href="https://doi.org/10.1175/jcli3504.1" ext-link-type="DOI">10.1175/jcli3504.1</ext-link>, 2005.</mixed-citation></ref>
      <ref id="bib1.bibx11"><label>Loeb et al.(2003)</label><mixed-citation>Loeb, N. G., Manalo-Smith, N., Kato, S., Miller, W. F., Gupta, S. K., Minnis,  P., and Wielicki, B. A.: Angular Distribution Models for Top-of-Atmosphere  Radiative Flux Estimation from the Clouds and the Earth’s Radiant Energy  System Instrument on the Tropical Rainfall Measuring Mission Satellite. Part I: Methodology, J. Appl. Meteorol., 42, 240–265,  <ext-link xlink:href="https://doi.org/10.1175/1520-0450(2003)042&lt;0240:ADMFTO&gt;2.0.CO;2" ext-link-type="DOI">10.1175/1520-0450(2003)042&lt;0240:ADMFTO&gt;2.0.CO;2</ext-link>, 2003.</mixed-citation></ref>
      <ref id="bib1.bibx12"><label>Loeb et al.(2005)</label><mixed-citation>Loeb, N. G., Kato, S., Loukachine, K., and Manalo-Smith, N.: Angular  Distribution Models for Top-of-Atmosphere Radiative Flux Estimation from the  Clouds and the Earth's Radiant Energy System Instrument on the <italic>Terra</italic>  Satellite. Part I: Methodology, J. Atmos. Ocean. Tech., 22, 338–351, <ext-link xlink:href="https://doi.org/10.1175/jtech1712.1" ext-link-type="DOI">10.1175/jtech1712.1</ext-link>, 2005.</mixed-citation></ref>
      <ref id="bib1.bibx13"><label>Madenach(2026)</label><mixed-citation>Madenach, N.: Seeking TOA SW flux closure over semi-synthetic 3D cloud fields Notebook, Version v1, Zenodo [data set/code], <ext-link xlink:href="https://doi.org/10.5281/zenodo.18460315" ext-link-type="DOI">10.5281/zenodo.18460315</ext-link>, 2026.</mixed-citation></ref>
      <ref id="bib1.bibx14"><label>Marchuk et al.(1980)</label><mixed-citation>Marchuk, G. I., Mikhailov, G. A., Nazaraliev, M. A., Darbinjan, R. A., Kargin, B. A., and Elepov, B. S.: Monte Carlo Methods in Atmospheric Optics, in: Optical Science Series, Springer Verlag, 12, 208 pp.,  <ext-link xlink:href="https://doi.org/10.1007/978-3-540-35237-2" ext-link-type="DOI">10.1007/978-3-540-35237-2</ext-link>, 1980.</mixed-citation></ref>
      <ref id="bib1.bibx15"><label>Mayer et al.(2004)</label><mixed-citation>Mayer, B., Schröder, M., Preusker, R., and Schüller, L.: Remote sensing of water cloud droplet size distributions using the backscatter glory: a case study, Atmos. Chem. Phys., 4, 1255–1263, <ext-link xlink:href="https://doi.org/10.5194/acp-4-1255-2004" ext-link-type="DOI">10.5194/acp-4-1255-2004</ext-link>, 2004.</mixed-citation></ref>
      <ref id="bib1.bibx16"><label>Smith et al.(1986)</label><mixed-citation>Smith, G. L., Green, R. N., Raschke, E., Avis, L. M., Suttles, J. T., Wielicki, B. A., and Davies, R.: Inversion methods for satellite studies of the Earth's Radiation Budget: Development of algorithms for the ERBE Mission,  Rev. Geophys., 24, 407–421, <ext-link xlink:href="https://doi.org/10.1029/rg024i002p00407" ext-link-type="DOI">10.1029/rg024i002p00407</ext-link>, 1986.</mixed-citation></ref>
      <ref id="bib1.bibx17"><label>Su et al.(2015)</label><mixed-citation>Su, W., Corbett, J., Eitzen, Z., and Liang, L.: Next-generation angular distribution models for top-of-atmosphere radiative flux calculation from CERES instruments: methodology, Atmos. Meas. Tech., 8, 611–632, <ext-link xlink:href="https://doi.org/10.5194/amt-8-611-2015" ext-link-type="DOI">10.5194/amt-8-611-2015</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bibx18"><label>Tornow et al.(2018)</label><mixed-citation>Tornow, F., Preusker, R., Domenech, C., Henken, C., and Testorp, S.:  Top-of-Atmosphere Shortwave Anisotropy over Liquid Clouds: Sensitivity to Clouds' Microphysical Structure and Cloud-Topped Moisture, Atmosphere, 9, <ext-link xlink:href="https://doi.org/10.3390/atmos9070256" ext-link-type="DOI">10.3390/atmos9070256</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bibx19"><label>Tornow et al.(2019)</label><mixed-citation>Tornow, F., Domenech, C., and Fischer, J.: On the Use of Geophysical Parameters for the Top-of-Atmosphere Shortwave Clear-Sky Radiance-to-Flux Conversion in EarthCARE, J. Atmos. Ocean. Tech., 36, 717–732,  <ext-link xlink:href="https://doi.org/10.1175/jtech-d-18-0087.1" ext-link-type="DOI">10.1175/jtech-d-18-0087.1</ext-link>, 2019.</mixed-citation></ref>
      <ref id="bib1.bibx20"><label>Tornow et al.(2020)</label><mixed-citation>Tornow, F., Domenech, C., Barker, H. W., Preusker, R., and Fischer, J.: Using two-stream theory to capture fluctuations of satellite-perceived TOA SW radiances reflected from clouds over ocean, Atmos. Meas. Tech., 13, 3909–3922, <ext-link xlink:href="https://doi.org/10.5194/amt-13-3909-2020" ext-link-type="DOI">10.5194/amt-13-3909-2020</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bibx21"><label>Tornow et al.(2021)</label><mixed-citation>Tornow, F., Domenech, C., Cole, J. N. S., Madenach, N., and Fischer, J.: Changes in TOA SW Fluxes over Marine Clouds When Estimated via Semiphysical Angular Distribution Models, J. Atmos. Ocean. Tech., 38, <ext-link xlink:href="https://doi.org/10.1175/JTECH-D-20-0107.1" ext-link-type="DOI">10.1175/JTECH-D-20-0107.1</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bibx22"><label>Velázquez Blázquez et al.(2024a)</label><mixed-citation>Velázquez Blázquez, A., Baudrez, E., Clerbaux, N., and Domenech, C.: Unfiltering of the EarthCARE Broadband Radiometer (BBR) observations: the BM-RAD product, Atmos. Meas. Tech., 17, 4245–4256, <ext-link xlink:href="https://doi.org/10.5194/amt-17-4245-2024" ext-link-type="DOI">10.5194/amt-17-4245-2024</ext-link>, 2024a.</mixed-citation></ref>
      <ref id="bib1.bibx23"><label>Velázquez Blázquez et al.(2024b)</label><mixed-citation>Velázquez Blázquez, A., Domenech, C., Baudrez, E., Clerbaux, N., Salas Molar, C., and Madenach, N.: Retrieval of top-of-atmosphere fluxes from combined EarthCARE lidar, imager, and broadband radiometer observations: the BMA-FLX product, Atmos. Meas. Tech., 17, 7007–7026, <ext-link xlink:href="https://doi.org/10.5194/amt-17-7007-2024" ext-link-type="DOI">10.5194/amt-17-7007-2024</ext-link>, 2024b.</mixed-citation></ref>
      <ref id="bib1.bibx24"><label>Viollier et al.(2009)</label><mixed-citation>Viollier, M., Standfuss, C., Chomette, O., and Quesney, A.: Top-of-Atmosphere  Radiance-to-Flux Conversion in the SW Domain for the ScaRaB-3 Instrument on  Megha-Tropiques, J. Atmos. Ocean. Tech., 26,  2161–2171, <ext-link xlink:href="https://doi.org/10.1175/2009jtecha1264.1" ext-link-type="DOI">10.1175/2009jtecha1264.1</ext-link>, 2009.</mixed-citation></ref>
      <ref id="bib1.bibx25"><label>Wehr et al.(2023)</label><mixed-citation>Wehr, T., Kubota, T., Tzeremes, G., Wallace, K., Nakatsuka, H., Ohno, Y., Koopman, R., Rusli, S., Kikuchi, M., Eisinger, M., Tanaka, T., Taga, M., Deghaye, P., Tomita, E., and Bernaerts, D.: The EarthCARE mission – science and system overview, Atmos. Meas. Tech., 16, 3581–3608, <ext-link xlink:href="https://doi.org/10.5194/amt-16-3581-2023" ext-link-type="DOI">10.5194/amt-16-3581-2023</ext-link>, 2023.</mixed-citation></ref>
      <ref id="bib1.bibx26"><label>Wild et al.(2014)</label><mixed-citation>Wild, M., Folini, D., Hakuba, M. Z., Schär, C., Seneviratne, S. I., Kato,  S., Rutan, D., Ammann, C., Wood, E. F., and König-Langlo, G.: The energy  balance over land and oceans: an assessment based on direct observations and  CMIP5 climate models, Clim. Dynam., 44, 3393–3429,  <ext-link xlink:href="https://doi.org/10.1007/s00382-014-2430-z" ext-link-type="DOI">10.1007/s00382-014-2430-z</ext-link>, 2014.</mixed-citation></ref>
      <ref id="bib1.bibx27"><label>Wild et al.(2018)</label><mixed-citation>Wild, M., Hakuba, M. Z., Folini, D., Dörig-Ott, P., Schär, C., Kato,  S., and Long, C. N.: The cloud-free global energy balance and inferred cloud  radiative effects: an assessment based on direct observations and climate  models, Clim. Dynam., 52, 4787–4812, <ext-link xlink:href="https://doi.org/10.1007/s00382-018-4413-y" ext-link-type="DOI">10.1007/s00382-018-4413-y</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bibx28"><label>Wood(2006)</label><mixed-citation>Wood, R.: Relationships between optical depth, liquid water path, droplet  concentration and effective radius in an adiabatic layer cloud, Tech. rep.,  <uri>https://atmos.uw.edu/~robwood/papers/chilean_plume/optical_depth_relations.pdf</uri> (last access: 3 February 2026), 2006.</mixed-citation></ref>

  </ref-list></back>
    <!--<article-title-html>Seeking TOA SW flux closure over semi-synthetic 3D cloud fields: exploring the accuracy of two angular distribution models</article-title-html>
<abstract-html/>
<ref-html id="bib1.bib1"><label>Barker et al.(1996)</label><mixed-citation>
      
Barker, H. W., Wiellicki, B. A., and Parker, L.: A Parameterization for Computing Grid-Averaged Solar Fluxes for Inhomogeneous Marine Boundary Layer Clouds. Part II: Validation Using Satellite Data, J. Atmos. Sci., 53, 2304–2316, <a href="https://doi.org/10.1175/1520-0469(1996)053&lt;2304:APFCGA&gt;2.0.CO;2" target="_blank">https://doi.org/10.1175/1520-0469(1996)053&lt;2304:APFCGA&gt;2.0.CO;2</a>, 1996.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib2"><label>Barker et al.(2003) </label><mixed-citation>
      
Barker, H. W., Goldstein, R. K., and Stevens, D. E.: Monte Carlo Simulation of Solar Reflectances for Cloudy Atmospheres, J. Atmos. Sci., 60, 1881–1894,
<a href="https://doi.org/10.1175/1520-0469(2003)060&lt;1881:MCSOSR&gt;2.0.CO;2" target="_blank">https://doi.org/10.1175/1520-0469(2003)060&lt;1881:MCSOSR&gt;2.0.CO;2</a>, 2003.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib3"><label>Brenguier et al.(2000)</label><mixed-citation>
      
Brenguier, J.-L., Pawlowska, H., Schüller, L., Preusker, R., Fischer, J., and  Fouquart, Y.: Radiative Properties of Boundary Layer Clouds: Droplet Effective Radius versus Number Concentration, J. Atmos. Sci., 57, 803–821,  <a href="https://doi.org/10.1175/1520-0469(2000)057&lt;0803:RPOBLC&gt;2.0.CO;2" target="_blank">https://doi.org/10.1175/1520-0469(2000)057&lt;0803:RPOBLC&gt;2.0.CO;2</a>, 2000.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib4"><label>Coakley and Chylek(1975)</label><mixed-citation>
      
Coakley, J. A. and Chylek, P.: The Two-Stream Approximation in Radiative  Transfer: Including the Angle of the Incident Radiation, J. Atmos. Sci., 32, 409–418, <a href="https://doi.org/10.1175/1520-0469(1975)032&lt;0409:ttsair&gt;2.0.co;2" target="_blank">https://doi.org/10.1175/1520-0469(1975)032&lt;0409:ttsair&gt;2.0.co;2</a>, 1975.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib5"><label>Cole et al.(2023)</label><mixed-citation>
      
Cole, J. N. S., Barker, H. W., Qu, Z., Villefranque, N., and Shephard, M. W.: Broadband radiative quantities for the EarthCARE mission: the ACM-COM and ACM-RT products, Atmos. Meas. Tech., 16, 4271–4288, <a href="https://doi.org/10.5194/amt-16-4271-2023" target="_blank">https://doi.org/10.5194/amt-16-4271-2023</a>, 2023.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib6"><label>Dewitte et al.(2008)</label><mixed-citation>
      
Dewitte, S., Gonzalez, L., Clerbaux, N., Ipe, A., Bertrand, C., and De Paepe,  B.: The Geostationary Earth Radiation Budget Edition 1 data processing  algorithms, Adv. Space Res., 41, 1906–1913,  <a href="https://doi.org/10.1016/j.asr.2007.07.042" target="_blank">https://doi.org/10.1016/j.asr.2007.07.042</a>, 2008.


    </mixed-citation></ref-html>
<ref-html id="bib1.bib7"><label>Domenech and Wehr(2011)</label><mixed-citation>
      
Domenech, C. and Wehr, T.: Use of Artificial Neural Networks to Retrieve TOA SW Radiative Fluxes for the EarthCARE Mission, IEEE T. Geosci. Remote, 49, 1839–1849, <a href="https://doi.org/10.1109/tgrs.2010.2102768" target="_blank">https://doi.org/10.1109/tgrs.2010.2102768</a>, 2011.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib8"><label>Forster et al.(2021)</label><mixed-citation>
      
Forster, P., Storelvmo, T., Armour, K., Collins, W., Dufresne, J.-L., Frame,  D., Lunt, D. J., Mauritsen, T., Palmer, M. D., Watanabe, M., Wild, M., and  Zhang, H.: The Earth’s Energy Budget, Climate Feedbacks, and Climate  Sensitivity, in: Climate Change 2021: The Physical Science Basis.  Contribution of Working Group I to the Sixth Assessment Report of the  Intergovernmental Panel on Climate Change, edited by: Masson-Delmotte, V.,  Zhai, P., Pirani, A., Connors, S. L., Péan, C., Berger, S., Caud, N., Chen,  Y., Goldfarb, L., Gomis, M. I., Huang, M., Leitzell, K., Lonnoy, E.,  Matthews, J. B. R., Maycock, T. K., Waterfield, T., Yelekçi, O., Yu, R., and  Zhou, B., Cambridge University Press, Cambridge, United  Kingdom and New York, NY, USA, 923–1054, <a href="https://doi.org/10.1017/9781009157896.009" target="_blank">https://doi.org/10.1017/9781009157896.009</a>, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib9"><label>Gristey et al.(2021)</label><mixed-citation>
      
Gristey, J. J., Su, W., Loeb, N. G., Vonder Haar, T. H., Tornow, F., Schmidt,  S. K., Hakuba, M. Z., Pilewskie, P., and Russell, J. E.: Shortwave radiance  to irradiance conversion for Earth radiation budget satellite observations: A  review, Remote Sensing, 13, 2640, <a href="https://doi.org/10.3390/rs13132640" target="_blank">https://doi.org/10.3390/rs13132640</a>, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib10"><label>Loeb and Manalo-Smith(2005)</label><mixed-citation>
      
Loeb, N. G. and Manalo-Smith, N.: Top-of-Atmosphere Direct Radiative Effect of Aerosols over Global Oceans from Merged CERES and MODIS Observations, J. Climate, 18, 3506–3526, <a href="https://doi.org/10.1175/jcli3504.1" target="_blank">https://doi.org/10.1175/jcli3504.1</a>, 2005.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib11"><label>Loeb et al.(2003)</label><mixed-citation>
      
Loeb, N. G., Manalo-Smith, N., Kato, S., Miller, W. F., Gupta, S. K., Minnis,  P., and Wielicki, B. A.: Angular Distribution Models for Top-of-Atmosphere  Radiative Flux Estimation from the Clouds and the Earth’s Radiant Energy  System Instrument on the Tropical Rainfall Measuring Mission Satellite. Part I: Methodology, J. Appl. Meteorol., 42, 240–265,  <a href="https://doi.org/10.1175/1520-0450(2003)042&lt;0240:ADMFTO&gt;2.0.CO;2" target="_blank">https://doi.org/10.1175/1520-0450(2003)042&lt;0240:ADMFTO&gt;2.0.CO;2</a>, 2003.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib12"><label>Loeb et al.(2005)</label><mixed-citation>
      
Loeb, N. G., Kato, S., Loukachine, K., and Manalo-Smith, N.: Angular  Distribution Models for Top-of-Atmosphere Radiative Flux Estimation from the  Clouds and the Earth's Radiant Energy System Instrument on the <i>Terra</i>  Satellite. Part I: Methodology, J. Atmos. Ocean. Tech., 22, 338–351, <a href="https://doi.org/10.1175/jtech1712.1" target="_blank">https://doi.org/10.1175/jtech1712.1</a>, 2005.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib13"><label>Madenach(2026)</label><mixed-citation>
      
Madenach, N.: Seeking TOA SW flux closure over semi-synthetic 3D cloud fields Notebook, Version v1, Zenodo [data set/code], <a href="https://doi.org/10.5281/zenodo.18460315" target="_blank">https://doi.org/10.5281/zenodo.18460315</a>, 2026.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib14"><label>Marchuk et al.(1980)</label><mixed-citation>
      
Marchuk, G. I., Mikhailov, G. A., Nazaraliev, M. A., Darbinjan, R. A., Kargin, B. A., and Elepov, B. S.: Monte Carlo Methods in Atmospheric Optics, in: Optical Science Series, Springer Verlag, 12, 208 pp.,  <a href="https://doi.org/10.1007/978-3-540-35237-2" target="_blank">https://doi.org/10.1007/978-3-540-35237-2</a>, 1980.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib15"><label>Mayer et al.(2004)</label><mixed-citation>
      
Mayer, B., Schröder, M., Preusker, R., and Schüller, L.: Remote sensing of water cloud droplet size distributions using the backscatter glory: a case study, Atmos. Chem. Phys., 4, 1255–1263, <a href="https://doi.org/10.5194/acp-4-1255-2004" target="_blank">https://doi.org/10.5194/acp-4-1255-2004</a>, 2004.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib16"><label>Smith et al.(1986)</label><mixed-citation>
      
Smith, G. L., Green, R. N., Raschke, E., Avis, L. M., Suttles, J. T., Wielicki, B. A., and Davies, R.: Inversion methods for satellite studies of the Earth's Radiation Budget: Development of algorithms for the ERBE Mission,  Rev. Geophys., 24, 407–421, <a href="https://doi.org/10.1029/rg024i002p00407" target="_blank">https://doi.org/10.1029/rg024i002p00407</a>, 1986.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib17"><label>Su et al.(2015)</label><mixed-citation>
      
Su, W., Corbett, J., Eitzen, Z., and Liang, L.: Next-generation angular distribution models for top-of-atmosphere radiative flux calculation from CERES instruments: methodology, Atmos. Meas. Tech., 8, 611–632, <a href="https://doi.org/10.5194/amt-8-611-2015" target="_blank">https://doi.org/10.5194/amt-8-611-2015</a>, 2015.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib18"><label>Tornow et al.(2018)</label><mixed-citation>
      
Tornow, F., Preusker, R., Domenech, C., Henken, C., and Testorp, S.:  Top-of-Atmosphere Shortwave Anisotropy over Liquid Clouds: Sensitivity to Clouds' Microphysical Structure and Cloud-Topped Moisture, Atmosphere, 9, <a href="https://doi.org/10.3390/atmos9070256" target="_blank">https://doi.org/10.3390/atmos9070256</a>, 2018.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib19"><label>Tornow et al.(2019)</label><mixed-citation>
      
Tornow, F., Domenech, C., and Fischer, J.: On the Use of Geophysical Parameters for the Top-of-Atmosphere Shortwave Clear-Sky Radiance-to-Flux Conversion in EarthCARE, J. Atmos. Ocean. Tech., 36, 717–732,  <a href="https://doi.org/10.1175/jtech-d-18-0087.1" target="_blank">https://doi.org/10.1175/jtech-d-18-0087.1</a>, 2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib20"><label>Tornow et al.(2020)</label><mixed-citation>
      
Tornow, F., Domenech, C., Barker, H. W., Preusker, R., and Fischer, J.: Using two-stream theory to capture fluctuations of satellite-perceived TOA SW radiances reflected from clouds over ocean, Atmos. Meas. Tech., 13, 3909–3922, <a href="https://doi.org/10.5194/amt-13-3909-2020" target="_blank">https://doi.org/10.5194/amt-13-3909-2020</a>, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib21"><label>Tornow et al.(2021)</label><mixed-citation>
      
Tornow, F., Domenech, C., Cole, J. N. S., Madenach, N., and Fischer, J.: Changes in TOA SW Fluxes over Marine Clouds When Estimated via Semiphysical Angular Distribution Models, J. Atmos. Ocean. Tech., 38, <a href="https://doi.org/10.1175/JTECH-D-20-0107.1" target="_blank">https://doi.org/10.1175/JTECH-D-20-0107.1</a>, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib22"><label>Velázquez Blázquez et al.(2024a)</label><mixed-citation>
      
Velázquez Blázquez, A., Baudrez, E., Clerbaux, N., and Domenech, C.: Unfiltering of the EarthCARE Broadband Radiometer (BBR) observations: the BM-RAD product, Atmos. Meas. Tech., 17, 4245–4256, <a href="https://doi.org/10.5194/amt-17-4245-2024" target="_blank">https://doi.org/10.5194/amt-17-4245-2024</a>, 2024a.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib23"><label>Velázquez Blázquez et al.(2024b)</label><mixed-citation>
      
Velázquez Blázquez, A., Domenech, C., Baudrez, E., Clerbaux, N., Salas Molar, C., and Madenach, N.: Retrieval of top-of-atmosphere fluxes from combined EarthCARE lidar, imager, and broadband radiometer observations: the BMA-FLX product, Atmos. Meas. Tech., 17, 7007–7026, <a href="https://doi.org/10.5194/amt-17-7007-2024" target="_blank">https://doi.org/10.5194/amt-17-7007-2024</a>, 2024b.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib24"><label>Viollier et al.(2009)</label><mixed-citation>
      
Viollier, M., Standfuss, C., Chomette, O., and Quesney, A.: Top-of-Atmosphere  Radiance-to-Flux Conversion in the SW Domain for the ScaRaB-3 Instrument on  Megha-Tropiques, J. Atmos. Ocean. Tech., 26,  2161–2171, <a href="https://doi.org/10.1175/2009jtecha1264.1" target="_blank">https://doi.org/10.1175/2009jtecha1264.1</a>, 2009.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib25"><label>Wehr et al.(2023)</label><mixed-citation>
      
Wehr, T., Kubota, T., Tzeremes, G., Wallace, K., Nakatsuka, H., Ohno, Y., Koopman, R., Rusli, S., Kikuchi, M., Eisinger, M., Tanaka, T., Taga, M., Deghaye, P., Tomita, E., and Bernaerts, D.: The EarthCARE mission – science and system overview, Atmos. Meas. Tech., 16, 3581–3608, <a href="https://doi.org/10.5194/amt-16-3581-2023" target="_blank">https://doi.org/10.5194/amt-16-3581-2023</a>, 2023.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib26"><label>Wild et al.(2014)</label><mixed-citation>
      
Wild, M., Folini, D., Hakuba, M. Z., Schär, C., Seneviratne, S. I., Kato,  S., Rutan, D., Ammann, C., Wood, E. F., and König-Langlo, G.: The energy  balance over land and oceans: an assessment based on direct observations and  CMIP5 climate models, Clim. Dynam., 44, 3393–3429,  <a href="https://doi.org/10.1007/s00382-014-2430-z" target="_blank">https://doi.org/10.1007/s00382-014-2430-z</a>, 2014.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib27"><label>Wild et al.(2018)</label><mixed-citation>
      
Wild, M., Hakuba, M. Z., Folini, D., Dörig-Ott, P., Schär, C., Kato,  S., and Long, C. N.: The cloud-free global energy balance and inferred cloud  radiative effects: an assessment based on direct observations and climate  models, Clim. Dynam., 52, 4787–4812, <a href="https://doi.org/10.1007/s00382-018-4413-y" target="_blank">https://doi.org/10.1007/s00382-018-4413-y</a>, 2018.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib28"><label>Wood(2006)</label><mixed-citation>
      
Wood, R.: Relationships between optical depth, liquid water path, droplet  concentration and effective radius in an adiabatic layer cloud, Tech. rep.,  <a href="https://atmos.uw.edu/~robwood/papers/chilean_plume/optical_depth_relations.pdf" target="_blank"/> (last access: 3 February 2026), 2006.

    </mixed-citation></ref-html>--></article>
