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<article xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:oasis="http://docs.oasis-open.org/ns/oasis-exchange/table" dtd-version="3.0"><?xmltex \makeatother\@nolinetrue\makeatletter?>
  <front>
    <journal-meta>
<journal-id journal-id-type="publisher">AMT</journal-id>
<journal-title-group>
<journal-title>Atmospheric Measurement Techniques</journal-title>
<abbrev-journal-title abbrev-type="publisher">AMT</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Meas. Tech.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1867-8548</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>

    <article-meta>
      <article-id pub-id-type="doi">10.5194/amt-9-5119-2016</article-id><title-group><article-title>A polarimetric scattering database for non-spherical ice particles at microwave wavelengths</article-title>
      </title-group><?xmltex \runningtitle{A polarimetric scattering database for non-spherical ice particles}?><?xmltex \runningauthor{Y.~Lu et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff2 aff3">
          <name><surname>Lu</surname><given-names>Yinghui</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Jiang</surname><given-names>Zhiyuan</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="yes" rid="aff2">
          <name><surname>Aydin</surname><given-names>Kultegin</given-names></name>
          <email>aydin@engr.psu.edu</email>
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Verlinde</surname><given-names>Johannes</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Clothiaux</surname><given-names>Eugene E.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff2 aff4">
          <name><surname>Botta</surname><given-names>Giovanni</given-names></name>
          
        </contrib>
        <aff id="aff1"><label>1</label><institution>The Dept. of Meteorology and Atmospheric Science, The Pennsylvania State University, <?xmltex \hack{\newline}?> University Park, Pennsylvania, USA</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>The Dept. of Electrical Engineering, The Pennsylvania State University, University Park, <?xmltex \hack{\newline}?>  Pennsylvania, USA</institution>
        </aff>
        <aff id="aff3"><label>a</label><institution>now at: Climate and Ecosystem Sciences Division, Lawrence Berkeley National Laboratory, <?xmltex \hack{\newline}?>  Berkeley, California, USA</institution>
        </aff>
        <aff id="aff4"><label>b</label><institution>now at:  Google, New York,  USA</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Kultegin Aydin (aydin@engr.psu.edu)</corresp></author-notes><pub-date><day>19</day><month>October</month><year>2016</year></pub-date>
      
      <volume>9</volume>
      <issue>10</issue>
      <fpage>5119</fpage><lpage>5134</lpage>
      <history>
        <date date-type="received"><day>6</day><month>July</month><year>2016</year></date>
           <date date-type="rev-request"><day>13</day><month>July</month><year>2016</year></date>
           <date date-type="rev-recd"><day>24</day><month>September</month><year>2016</year></date>
           <date date-type="accepted"><day>26</day><month>September</month><year>2016</year></date>
      </history>
      <permissions>
<license license-type="open-access">
<license-p>This work is licensed under a Creative Commons Attribution 3.0 Unported License. To view a copy of this license, visit <ext-link ext-link-type="uri" xlink:href="http://creativecommons.org/licenses/by/3.0/">http://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions><self-uri xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016.html">This article is available from https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016.html</self-uri>
<self-uri xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016.pdf">The full text article is available as a PDF file from https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016.pdf</self-uri>


      <abstract>
    <p>The atmospheric science community has entered a period in which
electromagnetic scattering properties at microwave frequencies of
realistically constructed ice particles are necessary for making progress on
a number of fronts. One front includes retrieval of ice-particle properties
and signatures from ground-based, airborne, and satellite-based radar and
radiometer observations. Another front is evaluation of model microphysics by
application of forward operators to their outputs and comparison to
observations during case study periods. Yet a third front is data
assimilation, where again forward operators are applied to databases of
ice-particle scattering properties and the results compared to observations,
with their differences leading to corrections of the model state.</p>
    <p>Over the past decade investigators have developed databases of ice-particle
scattering properties at microwave frequencies and made them openly
available. Motivated by and complementing these earlier efforts, a database
containing polarimetric single-scattering properties of various types of ice
particles at millimeter to centimeter wavelengths is presented. While the
database presented here contains only single-scattering properties of ice
particles in a fixed orientation, ice-particle scattering properties are
computed for many different directions of the radiation incident on them.
These results are useful for understanding the dependence of ice-particle
scattering properties on ice-particle orientation with respect to the
incident radiation. For ice particles that are small compared to the wavelength, the
number of incident directions of the radiation is sufficient to compute
reasonable estimates of their (randomly) orientation-averaged scattering
properties.</p>
    <p>This database is complementary to earlier ones in that it contains
complete (polarimetric) scattering property information for each ice particle
– 44 plates, 30 columns, 405 branched planar crystals, 660 aggregates, and
640 conical graupel – and direction of incident radiation but is limited to
four frequencies (X-, Ku-, Ka-, and W-bands), does not include temperature
dependencies of the single-scattering properties, and does not include
scattering properties averaged over randomly oriented ice particles. Rules
for constructing the morphologies of ice particles from one database to the
next often differ; consequently, analyses that incorporate all of the
different databases will contain the most variability, while illuminating
important differences between them. Publication of this database is in
support of future analyses of this nature and comes with the hope that doing
so helps contribute to the development of a database standard for
ice-particle scattering properties, like the NetCDF (Network Common Data Form) CF (Climate and Forecast)
or NetCDF CF/Radial metadata conventions.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

      <?xmltex \hack{\newpage}?>
<sec id="Ch1.S1" sec-type="intro">
  <title>Introduction</title>
      <p>Cloud and precipitation processes are important components of the climate
system of Earth and have been gaining increased attention in recent years.
The importance of clouds and precipitation to climate and the uncertainties
clouds introduce into future climate projections have emerged as such
important topics that a new chapter in the most recent assessment of the
Intergovernmental Panel on Climate Change (IPCC) is now dedicated to clouds
and aerosols (IPCC, 2013; Chapter 7). As this chapter makes clear, amongst
the many outstanding issues related to clouds and precipitation are those
that result from ice-particle properties and processes, issues that must be
solved to reduce uncertainties related to clouds and precipitation in future
climate assessments.</p>
      <p>Passive and active microwave-based observations of cloud- and
precipitating-ice processes have an important role to play in improving our
understanding of them and their impacts. This includes, for example,
observational characterization of cloud and precipitation properties via the
core Global Precipitation Measurement (GPM) mission (e.g., Hou et al., 2014),
assimilation of cloud- and precipitation-affected microwave radiances in
operational numerical weather prediction schemes (e.g., Geer and Baordo,
2014), and assessment of cloud-ice microphysics parameterization performance (e.g., Galligani et al., 2015). As studies on these topics have advanced, so
has awareness of the importance of developing models of ice particles with
realistic shapes (e.g., Westbrook et al., 2004; Maruyama and Fujiyoshi 2005)
and radiative scattering properties (e.g., Kim, 2006; Liu, 2008; Petty and
Huang, 2010; Kulie et al., 2010; Johnson et al., 2012). As ice-particle
research has gained momentum, so has the importance of ice-particle
identification via remote sensing, leading to many studies on the value of
multiple frequencies  (e.g., Matrosov, 1998; Kneifel et al., 2011, 2015;
Leinonen et al., 2012, 2015; Battaglia et al., 2014; Kulie et al., 2014;
Stein et al., 2015; Leinonen and Moisseev, 2015), polarization (e.g., Straka
et al., 2000; Aydin and Singh, 2004; Chandrasekar et al., 2013; Kumjian,
2013), and the two combined (e.g., Tyynelä and Chandrasekhar, 2014) in their
identification. Polarimetric, multi-frequency measurements also provide one
path forward for quantitative estimation of ice water content (IWC). For
example, Aydin and Tang (1997), using 94  and 220 GHz radar frequencies;
Ryzhkov et al. (1998), using a 3 GHz radar frequency; and Lu et al. (2015),
using multiple radar frequencies, derived relationships between IWC and
polarimetric observables such as <italic>K</italic><inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">DP</mml:mi></mml:msub></mml:math></inline-formula> and
<italic>Z</italic><inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">DR</mml:mi></mml:msub></mml:math></inline-formula>.</p>
      <p>To develop ice-particle retrieval algorithms and forward radiative operators,
one must know the single-scattering properties (e.g., backscattering cross
section) of the ice particles in clouds and precipitation, which are quite
challenging to calculate because of their complex morphologies. Examples of
numerical methods capable of calculating single-scattering properties of ice
particles with arbitrary shapes are the discrete dipole approximation (DDA;
Purcell and Pennypacker, 1973; Draine and Flatau, 1994; Yurkin and Hoekstra,
2011), the finite-difference time domain method (FDTD; Yee, 1966; Tavlove and
Hagness, 2005), the pseudo-spectral time domain method (Liu et al., 2012),
the generalized multi-particle Mie method (GMM; Xu, 1995), and the recently
developed invariant embedding (Bi and Yang, 2014) and
superposition (Mackowski and Mishchenko, 1996; Mackowski, 2014) T-matrix
methods. Though accurate, these methods are often computationally expensive
and are not yet practical in running online calculations. Instead,
pre-calculated databases of ice-particle scattering properties at microwave
wavelengths are created and made publicly available, such as those published
by Kim (2006), Liu (2008), Nowell et al. (2013), Tyynelä and
Chandrasekar (2014), and Kuo et al. (2016) at microwave wavelengths. However,
these existing databases use randomly oriented ice particles, for which some
polarimetric information is lost, such as differential
reflectivity (<italic>Z</italic><inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">DR</mml:mi></mml:msub></mml:math></inline-formula>) and specific differential
phase (<italic>K</italic><inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">DP</mml:mi></mml:msub></mml:math></inline-formula>), and they are thus not suitable for all types of
polarimetric studies.</p>
      <p>In this work scattering calculations for ice aggregates (Botta et al., 2010,
2011), branched planar ice crystals (Botta et al., 2013; referred to as
“dendrites” in their paper), ice plates and columns (Lu et al., 2015), and
conical graupel (Oue et al., 2015) are assembled and synthesized into one
self-consistent set of scattering properties. The results are arranged into a
database containing single-scattering properties of ice particles at
frequencies of 9.4 GHz (X-band), 13.4 GHz (Ku-band), 35.6 GHz (Ka-band),
and 94.0 GHz (W-band) and for different orientations of the ice particles
relative to the incident radiation, which permits their use in all
polarimetric studies. The database
is now publically available for interested investigators. The remaining parts
of this paper describe the particle morphologies and the numerical methods
used in calculating the ice-particle single-scattering properties (Sect. 2),
the scattering geometry  (Sect. 3), the scattering properties
calculated (Sect. 4), the structure of the database (Sect. 5), and some
illuminative results from the database (Sect. 6), followed by a brief summary
and description of future refinements to the database (Sect. 7).</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><caption><p>Dielectric constants at 0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C for W-, Ka-, Ku-, and X-band
wavelengths of pure ice and of the tiny spheres used in the representations
of the plates, branched planar crystals, and columns after compensating for
the air gaps.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="6">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">

         <oasis:entry namest="col1" nameend="col2" align="center">Band (wavelength in mm) </oasis:entry>

         <oasis:entry colname="col3">W (3.19)</oasis:entry>

         <oasis:entry colname="col4">Ka (8.40)</oasis:entry>

         <oasis:entry colname="col5">Ku (22.4)</oasis:entry>

         <oasis:entry colname="col6">X (31.86)</oasis:entry>

       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>

         <oasis:entry rowsep="1" colname="col1" morerows="1">Pure ice</oasis:entry>

         <oasis:entry colname="col2">Real part</oasis:entry>

         <oasis:entry colname="col3">3.1682</oasis:entry>

         <oasis:entry colname="col4">3.1683</oasis:entry>

         <oasis:entry colname="col5">3.1686</oasis:entry>

         <oasis:entry colname="col6">3.1688</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col2">Imaginary part (10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>

         <oasis:entry colname="col3">3.2586</oasis:entry>

         <oasis:entry colname="col4">6.5053</oasis:entry>

         <oasis:entry colname="col5">13.044</oasis:entry>

         <oasis:entry colname="col6">16.777</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">Branched planar crystal/</oasis:entry>

         <oasis:entry colname="col2">Real part</oasis:entry>

         <oasis:entry colname="col3">5.6531</oasis:entry>

         <oasis:entry colname="col4">5.6536</oasis:entry>

         <oasis:entry colname="col5">5.6546</oasis:entry>

         <oasis:entry colname="col6">5.6552</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1">plate adjusted (69 %)</oasis:entry>

         <oasis:entry colname="col2">Imaginary part (10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>

         <oasis:entry colname="col3">10.356</oasis:entry>

         <oasis:entry colname="col4">20.676</oasis:entry>

         <oasis:entry colname="col5">41.462</oasis:entry>

         <oasis:entry colname="col6">53.332</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="1">Column adjusted (74 %)</oasis:entry>

         <oasis:entry colname="col2">Real part</oasis:entry>

         <oasis:entry colname="col3">4.9272</oasis:entry>

         <oasis:entry colname="col4">4.9275</oasis:entry>

         <oasis:entry colname="col5">4.9283</oasis:entry>

         <oasis:entry colname="col6">4.9288</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col2">Imaginary part (10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>

         <oasis:entry colname="col3">7.911</oasis:entry>

         <oasis:entry colname="col4">15.794</oasis:entry>

         <oasis:entry colname="col5">31.672</oasis:entry>

         <oasis:entry colname="col6">40.738</oasis:entry>

       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
<sec id="Ch1.S2">
  <title>Calculating single-scattering properties of individual ice particles</title>
      <p>The numerical methods we used to create the database are the GMM method
implemented by Xu (1995) and the DDA method implemented by Yurkin and
Hoekstra (2011). Both of these numerical methods have the flexibility to
model ice particles with arbitrary shapes. When using the GMM method, which
calculates scattering properties of clusters of non-overlapping spheres, the
ice particles are modeled using clusters of closely packed tiny (orders of
magnitude smaller than the wavelength) spheres that collectively resemble the
shape of the ice particles. Modeling ice aggregates using this approach is
convenient due to its flexibility in constructing arbitrary shapes using
clusters of spheres (Botta et al., 2010, 2011).</p>
      <p>The DDA method approximates an ice particle as a cluster of polarizable
points. This method calculates scattering properties of the cluster by
considering both the dipoles induced by the incident electric field at these
polarizable points and the interactions between these dipoles. Although not
required, the polarizable points are often arranged in cubic lattices to
accelerate calculations using the fast Fourier transform (Goodman et al.,
1991); thus the DDA method is suitable for calculating scattering properties
of compact particles such as ice columns and plates. A cubic lattice
arrangement for the polarizable points is less efficient computationally for
sparse particles because of the many gaps within the lattice (Petty and
Huang, 2010). As such, we do not use the DDA method to calculate scattering
properties of ice aggregates.</p>
      <p>Although the GMM and DDA methods provide scattering results with accuracies
specified in the calculations, they do not provide identical results because
they model ice particles in different ways (i.e., GMM as clusters of spheres
and DDA as dipoles). However, the shape differences between the two
representations of the same ice particle do not appear critical for
ice-particle scattering studies because of the variability in ice-particle
morphologies. Differences in the representation of a conical ice-particle
shape are overwhelmed by the differences of any conical shape with respect to
similarly shaped (but not identical) particles in nature. The morphologies of
the ice particles in the database and the methods used to represent them in
GMM and DDA calculations are now summarized.</p>
<sec id="Ch1.S2.SS1">
  <title>Aggregates</title>
      <p>The detailed algorithm for generating ice aggregates is described in Botta et
al. (2010, 2011). Only the GMM method was used for ice-aggregate scattering
calculations. Ice aggregates were constructed using ice columns (modeled as a
line of spheres) and stellar ice crystals (modeled as three identical lines
of spheres sharing a common central sphere). The dimensional relationship
used for the columns was
            <disp-formula id="Ch1.E1" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mi>d</mml:mi><mml:mo>=</mml:mo><mml:mn>3.527</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup><mml:msup><mml:mi>L</mml:mi><mml:mn>0.437</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <italic>d</italic> and <italic>L</italic> are, respectively, the width and length of the columns (in
centimeters) (Pruppacher and Klett, 1997, p. 51, Table 2.2b, N1e). The
dimensional relationship used for the stellar crystals was
            <disp-formula id="Ch1.E2" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mi>h</mml:mi><mml:mo>=</mml:mo><mml:mn>9.96</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:msup><mml:mi>d</mml:mi><mml:mn>0.415</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <italic>h</italic> and <italic>d</italic> are, respectively, the thickness and maximum dimension of
the stellar crystal (in centimeters) (Pruppacher and Klett, 1997, p. 51,
Table 2.2a, P1d). The dielectric constant of the spheres was set to that of
pure ice at 0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C (See Table 1).</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T2" specific-use="star"><caption><p>Species and size information for the ice particles in the database.
The number within parentheses below each ice-particle species is the total
number of ice particles of that species in the database. The numbers in
parentheses following the maximum dimensions of the aggregates (maximum
dimensions of the reference spheroids for the aggregates), branched planar
crystals, plates, and columns indicate the number of realizations (i.e.,
different ice particles) with that size. For conical graupel, with one
realization for each combination of density, cone angle, and
equal-volume-sphere radius, there are a total of 640 graupel particles in the
database.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="left" colsep="1"/>
     <oasis:colspec colnum="2" colname="col2" align="left" colsep="1"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="307.289764pt"/>
     <oasis:thead>
       <oasis:row rowsep="1">

         <oasis:entry rowsep="1" colname="col1" morerows="5">Aggregates (660)</oasis:entry>

         <oasis:entry rowsep="1" colname="col2">Type</oasis:entry>

         <oasis:entry rowsep="1" colname="col3">Maximum dimension of the reference spheroid (mm)</oasis:entry>

       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>

         <oasis:entry colname="col2">HD-N1e</oasis:entry>

         <oasis:entry colname="col3">0.58 (10), 0.85 (10), 1.26 (10), 1.86 (10), 2.76 (10), 4.01 (10), 5.88 (10), 8.69 (10), 12.67 (10), 18.42 (10)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col2">LD-N1e</oasis:entry>

         <oasis:entry colname="col3">0.46 (10), 0.65 (10), 0.92 (10), 1.31 (10), 1.87 (10), 2.63 (10), 3.76 (10), 5.32 (10), 7.58 (10), 10.77 (10), 15.41 (10), 21.73 (10), 31.22 (10), 44.17 (10)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col2">HD-P1d</oasis:entry>

         <oasis:entry colname="col3">0.38 (10), 0.58 (10), 0.86 (10), 1.27 (10), 1.87 (10), 2.75 (10), 4.01 (10), 5.95 (10), 8.69 (10), 12.77 (10), 18.85 (10), 27.84 (10), 40.46 (10)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col2">LD-P1d</oasis:entry>

         <oasis:entry colname="col3">0.45 (10), 0.63 (10), 0.91 (10), 1.30 (10), 1.85 (10), 2.64 (10), 3.76 (10), 5.31 (10), 7.58 (10), 10.65 (10), 15.23 (10), 21.66 (10), 30.71 (10), 43.78 (10), 62.58 (10)</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col2">LDt-P1d</oasis:entry>

         <oasis:entry colname="col3">0.46 (10), 0.65 (10), 0.92 (10), 1.30 (10), 1.87 (10), 2.63 (10), 3.76 (10), 5.33 (10), 7.59 (10), 10.78 (10), 15.43 (10), 21.84 (10), 31.09 (10), 44.67 (10)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"/>

         <oasis:entry colname="col2">Thickness</oasis:entry>

         <oasis:entry colname="col3">Maximum dimension (mm)</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"/>

         <oasis:entry colname="col2">ratio</oasis:entry>

         <oasis:entry colname="col3"/>

       </oasis:row>
       <oasis:row>

         <oasis:entry rowsep="1" colname="col1" morerows="1">Branched planar crystals   (405)</oasis:entry>

         <oasis:entry colname="col2">0.5</oasis:entry>

         <oasis:entry colname="col3">0.50 (1), 0.63 (1), 0.80 (1), 1.00 (2), 1.26 (4), 1.58 (9), 1.78 (13), 2.00 (10), 2.25 (10), 2.52 (9), 3.18 (6), 4.01 (5), 4.52 (5), 5.05 (4), 5.63 (4)</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col2">1.0</oasis:entry>

         <oasis:entry colname="col3">0.50 (1), 0.63 (1), 0.80 (1), 1.00 (1), 1.26 (4), 1.58 (9), 1.78 (15), 2.00 (17), 2.25 (21), 2.52 (27), 3.18 (35), 4.01 (46), 4.52 (49), 5.05 (49), 5.63 (45)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry rowsep="1" colname="col1" morerows="2">Plates (44)</oasis:entry>

         <oasis:entry colname="col2">0.5</oasis:entry>

         <oasis:entry colname="col3">0.10 (1), 0.12 (1), 0.16 (1), 0.20 (1), 0.26 (1), 0.32 (1), 0.40 (1), 0.50 (1), 0.64 (1), 0.80 (1), 1.00 (1), 1.28 (1), 1.61 (1), 2.02 (1), 2.52 (1)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col2">1.0</oasis:entry>

         <oasis:entry colname="col3">0.10 (1), 0.12 (1), 0.16 (1), 0.20 (1), 0.26 (1), 0.32 (1), 0.40 (1), 0.50 (1), 0.64 (1), 0.80 (1), 1.00 (1), 1.28 (1), 1.61 (1), 2.02 (1), 2.52 (1)</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col2">2.0</oasis:entry>

         <oasis:entry colname="col3">0.10 (1), 0.12 (1), 0.16 (1), 0.20 (1), 0.26 (1), 0.32 (1), 0.40 (1), 0.50 (1), 0.64 (1), 0.80 (1), 1.00 (1), 1.28 (1), 1.61 (1), 2.02 (1)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry rowsep="1" colname="col1" morerows="1">Columns (30)</oasis:entry>

         <oasis:entry colname="col2">1.0</oasis:entry>

         <oasis:entry colname="col3">0.18 (1), 0.22 (1), 0.28 (1), 0.35 (1), 0.44 (1), 0.54 (1), 0.69 (1), 0.86 (1), 1.07 (1), 1.35 (1), 1.68 (1), 2.12 (1), 2.65 (1), 3.34 (1), 4.17 (1)</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col2">2.0</oasis:entry>

         <oasis:entry colname="col3">0.18 (1), 0.24 (1), 0.30 (1), 0.36 (1), 0.46 (1), 0.58 (1), 0.70 (1), 0.88 (1), 1.13 (1), 1.40 (1), 1.77 (1), 2.15 (1), 2.76 (1), 3.42 (1), 4.31 (1)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="5">Conical graupel (640)</oasis:entry>

         <oasis:entry namest="col2" nameend="col3" align="center" colsep="0">Density (g cm<sup>-3</sup>) </oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry namest="col2" nameend="col3" align="center" colsep="0">0.05, 0.1, 0.2, 0.3, 0.4, 0.5, 0.6, 0.7, 0.8, 0.9 </oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry namest="col2" nameend="col3" align="center" colsep="0">Cone angle (degrees) </oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry namest="col2" nameend="col3" align="center" colsep="0">30, 40, 50, 60, 70, 80, 90, 100<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry namest="col2" nameend="col3" align="center" colsep="0">Equal-volume-sphere radius (mm) </oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry namest="col2" nameend="col3" align="center" colsep="0">0.20, 0.30, 0.40, 0.50, 1.00, 1.50, 2.00, 2.50 </oasis:entry>

       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p>The sizes and shapes of the ice aggregates were characterized by their
maximum dimensions (i.e., the maximum horizontal dimension of the cluster)
and their aspect ratios (i.e., the ratio between the maximum vertical and
horizontal dimensions). The ice-aggregate generation algorithm created each
ice-aggregate realization by first specifying a reference spheroid whose
maximum horizontal dimension and aspect ratio determined those of the
ice-aggregate realization. Then a column or stellar crystal monomer was added
to the aggregate one at a time, and the parts of the column or stellar crystal
that were outside of the reference spheroid were removed. This procedure was
repeated until the aggregate reached the desired mass within the specified
tolerance. Two mass-dimensional relationships (P1d and P1c in Mitchell, 1996)
were used to represent low-density (LD) and high-density (HD) aggregates. For
LDt-P1d aggregates in Table 2, the connecting point between the current
aggregate and the newly added stellar is randomly selected among the locations
at the tips, while for the remaining types of aggregates the connecting point is
randomly selected among all locations. For the ice aggregates in the database
the aspect ratios of the reference spheroids were set to 0.6. (The maximum
horizontal dimensions of the reference spheroids are listed in Table 2.)
However, the maximum dimensions and aspect ratios of the aggregates generated
in this manner were not necessarily those of the circumscribing spheroids.
For example, to build large aggregates with small amounts of mass, large
monomers have to be used, and the resulting aggregates are flat (Botta et al.,
2011).</p>
</sec>
<sec id="Ch1.S2.SS2">
  <title>Branched planar crystals and plates</title>
      <p>The morphologies of branched planar crystals in nature are characterized by
several features: their hexagonal core size (if present), branch widths,
sub-branch widths and locations, number of sub-branches, and spacing between
sub-branches. For the purpose of capturing different ice-crystal
morphologies, the properties of these different features must be varied to
obtain different realizations of branched planar crystals.</p>
      <p>Botta et al. (2013, their appendix A) describe the representations of branched
planar crystals used in the GMM calculations. To construct the database, the
maximum dimensions of the branched planar crystals in the database ranged
from 0.50
to 5.63 mm, equally spaced in logarithmic space. The thickness of a
branched planar crystal as a function of maximum dimension was given by the
dimensional relationship
            <disp-formula id="Ch1.E3" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mi>h</mml:mi><mml:mo>=</mml:mo><mml:mn>9.022</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:msup><mml:mi>d</mml:mi><mml:mn>0.377</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          <?xmltex \hack{\newpage}?><?xmltex \hack{\noindent}?>where <italic>h</italic> and <italic>d</italic> are the thickness and maximum dimension of
the branched planar crystal (in centimeters) (Pruppacher and Klett, 1997,
p. 51, Table 2.2b, P1e). To increase the variability of the branched planar
crystals in the database, a second thickness of the branched planar crystals
was obtained by multiplying the thickness <italic>h</italic> above by 0.5; therefore,
each branched planar crystal had one of two reference thickness variation
factors: 1.0 (the default thickness) and 0.5 (the halved thickness). There
were 405 different realizations of branched planar crystals whose
single-scattering properties were computed and are now included in the
database.</p>
      <p>For plates, i.e., planar crystals with no branches, maximum dimensions ranged from
0.10 to 2.52 mm, equally spaced in logarithmic space. The thicknesses of the
plates were given by the dimensional relationship
            <disp-formula id="Ch1.E4" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mi>h</mml:mi><mml:mo>=</mml:mo><mml:mn>1.41</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup><mml:msup><mml:mi>d</mml:mi><mml:mn>0.474</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <italic>h</italic> and <italic>d</italic> are the thickness and maximum dimension of
the plates (in centimeters) (Pruppacher and Klett, 1997, p. 51, Table 2.2a,
P1a). In the case of plates, thickness variation factors of 0.5, 1.0, and 2.0
were used to increase the range of variability of their properties. A total
of 44 realizations of plates are now included in the database.</p>
      <p>Representations of branched planar crystals and plates for GMM calculations
were as three layers of tiny spheres closely packed in the face-centered
cubic lattice (FCC), which achieves a maximum packing factor of 74 % for
an infinite lattice (Botta et al., 2013; Lu et al., 2013, 2014b). Thus the
radius of the tiny spheres was determined by the thickness of the planar ice
crystals. For branched planar crystals with the same maximum dimensions, the
crystals with half of the reference thickness needed significantly larger
numbers of tiny spheres to model than the ones with the reference thickness.
For some of the large, thin planar ice crystals with broad branches, the
numbers of tiny spheres used to represent them exceeded the capability of the
GMM code within our computational framework, and these realizations of planar
ice crystals were discarded. Because the largest planar crystals tend to grow
as open-structure crystals with thin branches, as opposed to broad
branches (Takahashi et al., 1991), the lack of this planar ice crystal type
from the database may not be detrimental.</p>
      <p>In Botta et al. (2013) and Lu et al. (2013) pure ice dielectric constants at
0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C were used for the tiny spheres in the GMM representations of
planar ice crystals. However, when considering the gaps between the tiny
spheres in the GMM representations of planar ice crystals, the ice crystals
were mixtures of the tiny spheres and the air gaps between them. Because of
this mixture of tiny spheres of pure ice and air, the dielectric constant of
the ice crystal (the “mixture”) was smaller than that of the pure ice in
the planar crystal. In order to match the effective dielectric constant of
the GMM representation of an ice crystal to that of pure ice at
0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C, the dielectric constants of the tiny spheres in this
representation were adjusted according to Lu et al. (2014a). In this approach
the effective dielectric constant of the mixture of tiny spheres and air gaps
in the GMM representation of an ice crystal was set to the dielectric
constant of pure ice at 0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C. Then the Maxwell–Garnett equation was
inverted to solve for the dielectric constant of the tiny spheres necessary
to achieve it:

                <disp-formula id="Ch1.E5" content-type="numbered"><mml:math display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϵ</mml:mi><mml:mi mathvariant="normal">spheres</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">ϵ</mml:mi><mml:mi mathvariant="normal">air</mml:mi></mml:msub><mml:mo>[</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mo>/</mml:mo><mml:mo>(</mml:mo><mml:mi>f</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">ϵ</mml:mi><mml:mi mathvariant="normal">ice</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:msub><mml:mi mathvariant="italic">ϵ</mml:mi><mml:mi mathvariant="normal">air</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>/</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">ϵ</mml:mi><mml:mi mathvariant="normal">ice</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">ϵ</mml:mi><mml:mi mathvariant="normal">air</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>)</mml:mo><mml:mo>]</mml:mo><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          where <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">ϵ</mml:mi></mml:math></inline-formula><sub>ice</sub> and <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">ϵ</mml:mi></mml:math></inline-formula><sub>air</sub> are the
dielectric constants of pure ice and air at 0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C, and <italic>f</italic> is
the volume fraction of the tiny spheres. Because the planar ice crystals were
modeled using three layers of tiny spheres, the volume fraction <italic>f</italic> of
the tiny spheres was set to 69 % (i.e., the volume fraction of spheres
closely packed into three layers infinite in extent), which is smaller than
74 % because two-thirds of the spheres were at the surface. The resulting
adjusted dielectric constant for the tiny spheres is listed in Table 1. After
realizing the limitations of the GMM method in computing the
single-scattering properties of pristine ice crystals, we performed DDA
calculations for pristine ice crystals as a supplement.</p>
      <p>The morphologies of the ice crystals used in the DDA calculations were
generated in the same way as those used in the GMM calculations. Most of the
planar ice crystals were modeled using 10 layers of dipoles, which was found
to be a reasonable balance between accuracy and computational time, while ice
crystals with aspect ratios close to unity were modeled using more layers of
dipoles for accuracy because the overall number of dipoles used to model them
was small. The dielectric constant of pure ice at 0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C was used in
all DDA representations of a planar ice crystal.</p>
</sec>
<sec id="Ch1.S2.SS3">
  <title>Columns</title>
      <p>The morphologies of columns were defined by their length (<italic>L</italic>) and
maximum dimension of their basal face (<italic>d</italic>), constrained by the
dimensional relationship
            <disp-formula id="Ch1.E6" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mi>d</mml:mi><mml:mo>=</mml:mo><mml:mn>3.0487</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup><mml:msup><mml:mi>L</mml:mi><mml:mn>0.61078</mml:mn></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <italic>d</italic> and <italic>L</italic> are in centimeters (Pruppacher and Klett,
1997, p. 51, Table 2.2b, N1a). Even though a needle model (N1a) was selected,
thickness (maximum dimension of the basal face) variation factors of 1.0 and
2.0 were used to increase the range of variability of their properties.
Therefore, we collectively call these crystals “columns” rather than
“needles” because they are representative of the class of columnar
crystals. In the GMM representation of ice columns, the columns have seven
spheres along the diagonal (i.e., maximum dimension) of their basal faces.
The ratio of the number of surface to interior tiny spheres was much lower
than for planar crystals; hence their volume fractions were considered to be
74 %. The dielectric constant of the tiny spheres was once again adjusted
so that the overall dielectric constant of the tiny sphere and air mixture
composing the ice column was that of pure ice (Table 1). For the DDA
calculations 16 dipoles were used along the diagonal of their basal faces.
The dielectric constant of pure ice at 0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C was used in all DDA
representations of an ice column.</p>
</sec>
<sec id="Ch1.S2.SS4">
  <title>Conical graupel</title>
      <p>The morphologies of conical graupel followed the sphere–cone–oblate–spheroid
particle morphologies in Aydin and Seliga (1984), which are
illustrated in their Fig. 1 and Fig. 1 here. The ratio of the
semi-minor (<italic>b</italic>) to semi-major (<italic>a</italic>) axis of the spheroidal
particle was set to <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>b</mml:mi><mml:mo>/</mml:mo><mml:mi>a</mml:mi><mml:mo>=</mml:mo><mml:mn>0.5</mml:mn></mml:mrow></mml:math></inline-formula>. The ratio of the radius <italic>c</italic> of
the sphere to the spheroidal semi-major axis was <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mi>a</mml:mi><mml:mo>=</mml:mo><mml:mn>0.2</mml:mn></mml:mrow></mml:math></inline-formula>. In this
framework the shape of conical graupel was determined by its cone angle
<inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula>, and its size was determined by the value of <italic>a</italic>. Cone angles
<inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> ranged from 30 to 100<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> in 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments. For each
cone angle, eight realizations of conical graupel were generated with
equal-volume-sphere radii of 0.2, 0.3, 0.4, 0.5, 1.0, 1.5, 2.0, and 2.5 mm.
For each realization of a conical graupel particle 10 calculations were
performed for particle densities of 0.05 g cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and from 0.1 to
0.9 g cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in 0.1 g cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> steps.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><caption><p>Two-dimensional slice through the axis of symmetry of a conical
graupel particle, with the solid line representing the outline of the particle
surface. The sphere with radius <italic>c</italic>, cone with apex angle <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> and
height <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>d</mml:mi><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">cos</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="italic">α</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula>), and spheroid with semi-major axis
<italic>a</italic> and semi-minor axis <italic>b</italic> used to build the conical graupel
particle are illustrated by shaded regions (within the particle) and dashed
lines. The line labeled <italic>d</italic> is tangent to both the sphere and
spheroid. In this work, like in Aydin and Seliga (1984), we assume the
constraints <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>b</mml:mi><mml:mo>/</mml:mo><mml:mi>a</mml:mi><mml:mo>=</mml:mo><mml:mn>0.5</mml:mn></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mi>a</mml:mi><mml:mo>=</mml:mo><mml:mn>0.2</mml:mn></mml:mrow></mml:math></inline-formula>. The
overall morphology of conical graupel in this representation is determined by
its cone angle <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula> and the spheroid semi-major axis <italic>a</italic>.</p></caption>
          <?xmltex \igopts{width=170.716535pt}?><graphic xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016-f01.png"/>

        </fig>

      <p>Because the DDA method has distinct advantages compared to GMM for computing
the single-scattering properties of compact ice particles, only the DDA
method was used to perform the calculations for conical graupel. The
dielectric constants of the conical graupel were calculated using the
Maxwell–Garnett formula (Bohren and Battan, 1980) with ice as the inclusion and air
as the matrix. Substituting the pure ice dielectric constants at
0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C and the ice volume fractions calculated based on the conical
graupel densities, effective dielectric constants were calculated and used in
the DDA calculations.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2" specific-use="star"><caption><p>Examples of <bold>(a)</bold>  an aggregate composed of stellar (color-coded)
monomers, <bold>(b)</bold> an aggregate composed of column (color-coded) monomers, <bold>(c)</bold> a
branched planar crystal, <bold>(d)</bold> a plate, <bold>(e)</bold> a column, and <bold>(f)</bold> a conical graupel
particle. In panels <bold>(a)</bold>–<bold>(e)</bold> the representations are for GMM calculations, and
the tiny spheres composing the representations are discernible. The conical
graupel particle in <bold>(f)</bold> is represented as a field of indiscernible polarizable
points on a rectangular lattice. Colors are used in <bold>(c)</bold>–<bold>(e)</bold> to distinguish
different layers of the tiny spheres that compose the ice particles. Note
that aggregate scattering properties are computed using GMM only, whereas
graupel particle scattering properties are computed using DDA only; all other
particle scattering properties are computed with both methods.</p></caption>
          <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016-f02.png"/>

        </fig>

</sec>
<sec id="Ch1.S2.SS5">
  <title>Summary of ice-particle types in the database</title>
      <p>Table 2 contains a summary of the important parameters that differentiate ice
particles within the aggregate, branched planar, plate, column, and conical
graupel types. And Fig. 2 provides an illustration of a single ice particle
within each type. All of this information is available within the Network Common Data Form
(NetCDF) files that compose the database.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><caption><p><bold>(a)</bold> The rotation angles, <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>, necessary to orient the scattering
coordinate system (<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>x</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup><mml:msup><mml:mi>y</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup><mml:msup><mml:mi>z</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>)
relative to the particle coordinate system (<inline-formula><mml:math display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mi>y</mml:mi><mml:mi>z</mml:mi></mml:mrow></mml:math></inline-formula>). <bold>(b)</bold> Orientation of the
scattered radiation, and hence the scattering plane, in the scattering
coordinate system.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016-f03.png"/>

        </fig>

</sec>
</sec>
<sec id="Ch1.S3">
  <title>Scattering geometry and reference frame</title>
      <p>Polarimetric radar observables are of value in ice-species classifications
and ice water content retrievals. In order to retain polarimetric information
for each ice-particle scattering calculation, we did not assume random
orientations for the ice particles as doing so leads to the loss of some
polarimetric information. Instead, the ice particles were fixed in
orientation, and their single-scattering properties calculated for different
directions of the incident radiation. For these calculations planar ice
crystals were oriented with their basal faces parallel to the <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:math></inline-formula> plane and
their maximum dimensions along the <inline-formula><mml:math display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> axis (Fig. 2). Ice columns had their
lengths parallel to the <inline-formula><mml:math display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> axis as well, with the diagonals (maximum
dimensions) of the basal faces aligned parallel to the <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:math></inline-formula> plane. For ice
aggregates the axis of symmetry of the circumscribing reference spheroid was
parallel to the <inline-formula><mml:math display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> axis, as was the axis of symmetry for conical graupel. We
used one right-handed <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mi>y</mml:mi><mml:mi>z</mml:mi></mml:mrow></mml:math></inline-formula> coordinate system, called the particle coordinate
system, to describe the orientations of the ice particles. A second
right-handed coordinate system was used to describe the direction of the
incident radiation and the scattering plane. The orientation of this second
coordinate system was obtained by first assuming it to be identical to the
particle coordinate system. Then, the <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:math></inline-formula> plane of this second coordinate
system was rotated by <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> about the <inline-formula><mml:math display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> axis,
with positive rotations representing a counterclockwise rotation when viewed
in the negative <inline-formula><mml:math display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> axis direction (Fig. 3a). The newly oriented coordinate
system, labeled with primes, was subsequently rotated by
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> about the <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>y</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> axis, to form the
coordinate system labeled with double primes, so that the <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>z</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> axis of this
coordinate system pointed in the direction of the incident radiation. For any
direction of the scattered radiation the plane containing the incident and
scattered radiation formed the scattering plane (Fig. 3b). The angle between
the directions of the incident and scattered radiation (i.e., the scattering
angle) was <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>, and the angle between the projection of the scattered
radiation onto the <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>x</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup><mml:msup><mml:mi>y</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> plane and the <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>x</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> axis was
<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> (Fig. 3b).</p>
      <p><?xmltex \hack{\newpage}?>Scattering properties associated with different incident angles were
calculated. The choice of the ranges and intervals of
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> were
based on the symmetry properties of the ice particles. The aggregates had no
symmetry axis, so <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> varied from 0 to
180<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive, in 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments, while
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> varied from 0 to 340<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive, in
20<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments. The ice crystal plates and branched planar crystals
had a six-fold symmetry about their symmetry axis perpendicular to their
basal faces, so <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> varied from 0 to
90<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive, in 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments, while
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> was set to 0 and 30<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>. The conical
graupel particles had rotational symmetry about their symmetry axis, so
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> varied from 0 to 180<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive,
in 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments, while <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> equaled
0<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>. The ice columns had reflection symmetry, so
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> varied from 0 to 90<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive,
in 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments, while <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> also varied
from 0 to 90<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive, in 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments. The orientation
of the diagonals of the basal faces of ice columns had only a small influence
on the single-scattering properties at the wavelengths investigated, so
rotations of the basal face diagonals outside of the <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:math></inline-formula> plane were not
considered.</p>
      <p>For some of the ice-particle sizes and radiation wavelengths used to
construct the database, lack of accurate interpolation from incident
radiation directions in the database to new directions of incident radiation
is by far its major limitation. This is true because some ice-particle
single-scattering properties changed by significant amounts, and nonlinearly,
over the angular intervals in <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> used to construct the database. Furthermore,
this makes averaging over canting angle problematic for these particular ice
particles. One possible means to accelerate the calculation of
orientation-averaged single-scattering properties over a range of
ice-particle orientations is use of the invariant embedding (Johnson, 1988;
Bi and Yang, 2014) or superposition (Mackowski and Mishchenko, 1996;
Mackowski, 2014) T-matrix methods. In these approaches the T-matrix for an
ice particle can be computed once and then used to calculate efficiently the
single-scattering properties averaged over a range of ice-particle
orientations.</p>
</sec>
<sec id="Ch1.S4">
  <title>Ice-particle single-scattering properties in the database</title>
      <p>In the far field, the amplitude scattering matrix can be used to describe the
relationship between the incident and scattered electric fields. Following
the convention in Bohren and Huffman (1983, Sect. 3.2),
          <disp-formula id="Ch1.E7" content-type="numbered"><mml:math display="block"><mml:mrow><?xmltex \hack{\hbox\bgroup\fontsize{8.8}{8.8}\selectfont$\displaystyle}?><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>∥</mml:mo><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>⟂</mml:mo><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">exp</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>(</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi><mml:mi>R</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi><mml:mi>R</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>∥</mml:mo><mml:mi mathvariant="normal">i</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>⟂</mml:mo><mml:mi mathvariant="normal">i</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>,</mml:mo><?xmltex \hack{$\egroup}?></mml:mrow></mml:math></disp-formula>
        where <italic>E</italic> is the electric field; the subscripts <inline-formula><mml:math display="inline"><mml:mo>∥</mml:mo></mml:math></inline-formula> and
<inline-formula><mml:math display="inline"><mml:mo>⟂</mml:mo></mml:math></inline-formula> indicate parallel and perpendicular to the scattering
plane (Fig. 3b); the subscripts s and i represent the scattered and incident
radiation; <italic>j</italic> is the square root of <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1; and <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>k</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">π</mml:mi><mml:mo>/</mml:mo><mml:mi mathvariant="italic">λ</mml:mi></mml:mrow></mml:math></inline-formula> is
the wave number, where <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> is the wavelength of the radiation,
<italic>R</italic> is the distance between the ice particle and an observation point
in the far field, and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi>n</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mrow><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:math></inline-formula>, or 4) are the elements of the
amplitude scattering matrix, which are dimensionless under this convention
and a function of the scattering polar angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> and
scattering azimuth angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>. For each triplet of a
realization of an ice particle, radiation frequency, and incident radiation
direction, the amplitude scattering matrices are computed and stored for
every 1<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> in <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> from 0 to 180<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>,
inclusive, and every 5<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> in <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> from 0 to
355<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive.</p>
      <p><?xmltex \hack{\newpage}?>Note that in the GMM output the amplitude scattering matrix is actually in
terms of <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mi>n</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> given by
          <disp-formula id="Ch1.E8" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>∥</mml:mo><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>⟂</mml:mo><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">exp</mml:mi><mml:mo>(</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi><mml:mi>R</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi><mml:mi>R</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">2</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">3</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">4</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">1</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mrow><mml:mo>∥</mml:mo><mml:mi mathvariant="normal">i</mml:mi></mml:mrow><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mrow><mml:mo>⟂</mml:mo><mml:mi mathvariant="normal">i</mml:mi></mml:mrow><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mrow><mml:mo>∥</mml:mo><mml:mi>i</mml:mi></mml:mrow><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mrow><mml:mo>⟂</mml:mo><mml:mi>i</mml:mi></mml:mrow><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> are defined with respect to
the <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>x</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup><mml:msup><mml:mi>z</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> plane
in Fig. 3b rather than the scattering plane, while
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>∥</mml:mo><mml:mi>s</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mrow><mml:mo>⟂</mml:mo><mml:mi>s</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> are still defined with respect to the scattering plane. The amplitude
scattering matrix elements <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mi>n</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> of the GMM output can be converted to the
convention of Bohren and Huffman (1983) via the transformation
          <disp-formula id="Ch1.E9" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mfenced open="[" close="]"><mml:mtable class="matrix" columnalign="center center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>=</mml:mo><mml:mfenced open="[" close="]"><mml:mtable class="matrix" columnalign="center center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">2</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">3</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">4</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mn mathvariant="normal">1</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mfenced open="[" close="]"><mml:mtable class="matrix" columnalign="center center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:mi mathvariant="normal">cos</mml:mi><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mi mathvariant="normal">sin</mml:mi><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="normal">sin</mml:mi><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mi mathvariant="normal">cos</mml:mi><mml:mo>(</mml:mo><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        The amplitude scattering matrix elements in the DDA output are of the same
convention as Bohren and Huffman (1983). In construction of the database we
adopted the convention of Bohren and Huffman (1983). The GMM output amplitude
scattering matrices are first transformed to the convention of Bohren and
Huffman (1983) before insertion into the database.</p>
      <p>Once the amplitude scattering matrices are computed, all of the
single-scattering properties follow. Because many of these single-scattering
properties are frequently used in applications, they are reported in the
database along with the amplitude scattering matrices. If a single-scattering
property was not provided directly by the GMM or DDA codes, it was computed
directly from the amplitude scattering matrices.</p>
      <p>In radar meteorology the electric fields are usually broken down into
components horizontal to the surface and perpendicular (vertical) to the
horizontal component. With this geometry the amplitude scattering matrix in
the forward-scatter alignment (FSA) convention of Bringi and
Chandrasekar (2001) is defined as
          <disp-formula id="Ch1.E10" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mi mathvariant="normal">h</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msubsup></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msubsup></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">exp</mml:mi><mml:mo>(</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi><mml:mi>R</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mi>R</mml:mi></mml:mfrac></mml:mstyle><mml:mfenced open="[" close="]"><mml:mtable class="matrix" columnalign="center center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">hh</mml:mi></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">hv</mml:mi></mml:msub></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">vh</mml:mi></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">vv</mml:mi></mml:msub></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mfenced close="]" open="["><mml:mtable class="matrix" columnalign="center" framespacing="0em"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mi mathvariant="normal">h</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msubsup></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>E</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msubsup></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where the subscripts h and v indicate horizontal and vertical polarizations,
and the superscripts s and i represent the scattered and incident radiation.
For the backward and forward scattering directions the scattering plane is
not uniquely defined. For these two directions we adopt the convention of
Bohren and Huffman (1983) in which the scattering plane rotates with
<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>. The scattering plane set by
<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>=</mml:mo><mml:mn>90</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> is the <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>y</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup><mml:msup><mml:mi>z</mml:mi><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> plane
in Fig. 3b. In this case <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>e</mml:mi><mml:mo stretchy="true" mathvariant="normal">^</mml:mo></mml:mover><mml:mo>∥</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula> is
always parallel to the horizontal polarization direction, and
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>e</mml:mi><mml:mo stretchy="true" mathvariant="normal">^</mml:mo></mml:mover><mml:mo>⟂</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula> is always parallel to the
vertical polarization direction no matter what the direction of the incident
radiation. Therefore, if  <inline-formula><mml:math display="inline"><mml:mover accent="true"><mml:mi>h</mml:mi><mml:mo mathvariant="normal" stretchy="true">^</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mover accent="true"><mml:mi>v</mml:mi><mml:mo stretchy="true" mathvariant="normal">^</mml:mo></mml:mover></mml:math></inline-formula>
represent horizontal and vertical polarization directions, then the wave
propagation direction is  <inline-formula><mml:math display="inline"><mml:mrow><mml:mover accent="true"><mml:mi>v</mml:mi><mml:mo mathvariant="normal" stretchy="true">^</mml:mo></mml:mover><mml:mo>×</mml:mo><mml:mover accent="true"><mml:mi>h</mml:mi><mml:mo mathvariant="normal" stretchy="true">^</mml:mo></mml:mover></mml:mrow></mml:math></inline-formula>, the
same as <inline-formula><mml:math display="inline"><mml:mrow><mml:mover accent="true"><mml:mi>e</mml:mi><mml:mo mathvariant="normal" stretchy="true">^</mml:mo></mml:mover><mml:mo>⟂</mml:mo><mml:mo>×</mml:mo><mml:msub><mml:mover accent="true"><mml:mi>e</mml:mi><mml:mo stretchy="true" mathvariant="normal">^</mml:mo></mml:mover><mml:mo>∥</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p>The <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">hh</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">vv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> amplitude
scattering matrix elements for backward and forward scattering can be
obtained from the dimensionless amplitude scattering matrix elements <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi>n</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
as

              <disp-formula specific-use="align" content-type="numbered"><mml:math display="block"><mml:mtable displaystyle="true"><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">hh</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mn>180</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mn>90</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>)</mml:mo><mml:mo>,</mml:mo><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">vv</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mn>180</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mn>90</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><?xmltex \hack{\hspace{0.8cm}}?><mml:mo>(</mml:mo><mml:mi mathvariant="normal">backward</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi mathvariant="normal">scattering</mml:mi><mml:mo>)</mml:mo><mml:mo>;</mml:mo></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">hh</mml:mi><mml:mi mathvariant="normal">f</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mn mathvariant="normal">0</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mn>90</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>)</mml:mo><mml:mo>,</mml:mo><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">vv</mml:mi><mml:mi mathvariant="normal">f</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mi>j</mml:mi><mml:mi>k</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:msub><mml:mi>S</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msup><mml:mn mathvariant="normal">0</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mn>90</mml:mn><mml:mo>∘</mml:mo></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:mtd></mml:mtr><mml:mlabeledtr id="Ch1.E11"><mml:mtd/><mml:mtd/><mml:mtd><mml:mrow><?xmltex \hack{\hspace{0.8cm}}?><mml:mo>(</mml:mo><mml:mi mathvariant="normal">forward</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi mathvariant="normal">scattering</mml:mi><mml:mo>)</mml:mo><mml:mo>.</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

          So the backscattering cross sections were computed as
          <disp-formula id="Ch1.E12" content-type="numbered"><mml:math display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">hh</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">4</mml:mn><mml:mi mathvariant="italic">π</mml:mi><mml:msup><mml:mfenced close="|" open="|"><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">hh</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msubsup></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>,</mml:mo><mml:mspace width="0.33em" linebreak="nobreak"/><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">vv</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">4</mml:mn><mml:mi mathvariant="italic">π</mml:mi><mml:msup><mml:mfenced close="|" open="|"><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">vv</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msubsup></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        And <italic>K</italic><inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">DP</mml:mi></mml:msub></mml:math></inline-formula> produced by some concentration <italic>n</italic> of a specific ice crystal can be computed
as
          <disp-formula id="Ch1.E13" content-type="numbered"><mml:math display="block"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi mathvariant="normal">DP</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn mathvariant="normal">3</mml:mn></mml:msup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn>180</mml:mn><mml:mi mathvariant="italic">π</mml:mi></mml:mfrac></mml:mstyle><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">π</mml:mi></mml:mrow><mml:mi>k</mml:mi></mml:mfrac></mml:mstyle><mml:mi>n</mml:mi><mml:mi mathvariant="normal">Re</mml:mi><mml:mo>(</mml:mo><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">hh</mml:mi><mml:mi mathvariant="normal">f</mml:mi></mml:msubsup><mml:mo>-</mml:mo><mml:msubsup><mml:mi>S</mml:mi><mml:mi mathvariant="normal">vv</mml:mi><mml:mi mathvariant="normal">f</mml:mi></mml:msubsup><mml:mo>)</mml:mo><mml:msup><mml:mo>[</mml:mo><mml:mo>∘</mml:mo></mml:msup><mml:mspace linebreak="nobreak" width="0.33em"/><mml:msup><mml:mi mathvariant="normal">km</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="italic">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>
</sec>
<sec id="Ch1.S5">
  <title>Structure of the database</title>
      <p>The database is stored in multiple NetCDF-formatted files for ease of use.
The name of each file contains an identifier indicating whether the GMM or
DDA method was used to produce the scattering properties that it contains.
Each file contains the scattering properties associated with one individual
ice particle at one frequency but for all directions of the incident and
scattered radiation. Because there are 181 scattering (polar)
angles (0  to 180<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive, in 1<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments) and
72 scattering azimuth angles (0  to 355<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive, in
5<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments) associated with the scattered radiation for each
direction of the incident radiation, there are 181 <inline-formula><mml:math display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 72, i.e., 13 032, sets
of amplitude scattering matrices associated with each direction of incident
radiation. Because aggregates have the greatest number of directions of the
incident radiation at 342, they lead to the largest files, containing 342 <inline-formula><mml:math display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 13 032 amplitude scattering matrices. Single-scattering properties that
have only one value for each calculation (e.g., extinction cross section,
absorption cross section, scattering cross section and backscattering cross
section) or are of particular interest (e.g., forward-scattered differential
phase) are extracted from each file and concatenated in a separate, much
smaller, file. This smaller file is indexed via the following parameters:
particle index indicating which particle is used in the calculation (e.g., 1
through 405 for branched planar crystals); frequency or wavelength indicators
of the incident radiation (i.e., W-, Ka-, Ku-, and X-bands for the
calculations currently in the database); polar angle
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> of the incident radiation (e.g.,
0  to 90<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, inclusive, in 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> increments for branched
planar crystals); and azimuth angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> of the
incident radiation (e.g., 0  and 30<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> for branched planar
crystals).</p>
      <p>Physical properties related to each ice-particle realization are stored in this smaller file as
variables with the particle index as the only dimension. These properties
include ice-particle maximum dimension, thickness, mass, and projected area
onto the <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:math></inline-formula> (horizontal) plane of the particle coordinate system. Detailed
information of the ice particles in the database, including the location and
radius of each tiny sphere used in the GMM representation of an ice particle
or the locations of the polarizable points in the DDA representation of an
ice particle, is provided in separate files for interested users. Finally,
images of the ice particles in the database are also available.</p>
      <p>The NetCDF files that compose the database are available through <ext-link xlink:href="http://dx.doi.org/10.5439/1258029" ext-link-type="DOI">10.5439/1258029</ext-link> (Aydin et al., 2016). The dimensions,
coordinate variables, geophysical variables, and file naming conventions for
the NetCDF files are summarized in Tables S1–S5.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4" specific-use="star"><caption><p>Horizontally (h)-polarized backscattering cross sections
<italic>C</italic><inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mrow><mml:mi mathvariant="normal">bsc</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">hh</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula> for all ice particles in the database for
side incident (<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn>90</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>,
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>) h-polarized radiation at (left
column) X-band and (right column) W-band wavelengths. The backscattering
cross sections are plotted vs.  <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="bold">a</mml:mi><mml:mn mathvariant="bold">1</mml:mn></mml:msub><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msub><mml:mi mathvariant="bold">b</mml:mi><mml:mn mathvariant="bold">1</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>   size
parameter,  <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="bold">a</mml:mi><mml:mn mathvariant="bold">2</mml:mn></mml:msub><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msub><mml:mi mathvariant="bold">b</mml:mi><mml:mn mathvariant="bold">2</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> maximum dimension, and
<inline-formula><mml:math display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="bold">a</mml:mi><mml:mn mathvariant="bold">3</mml:mn></mml:msub><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msub><mml:mi mathvariant="bold">b</mml:mi><mml:mn mathvariant="bold">3</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> mass. In <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="bold">a</mml:mi><mml:mn mathvariant="bold">1</mml:mn></mml:msub><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:msub><mml:mi mathvariant="bold">b</mml:mi><mml:mn mathvariant="bold">1</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> each backscattering cross section is
normalized by the cross sectional area of a solid (0.917 g cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) ice
sphere with mass equal to that of the ice particle;
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> represents the radius of this equal-mass solid
ice sphere.</p></caption>
        <?xmltex \igopts{width=369.885827pt}?><graphic xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016-f04.png"/>

      </fig>

</sec>
<sec id="Ch1.S6">
  <title>Some illuminative results from the database</title>
      <p>The backscattering cross sections of the ice particles in the database are
presented a number of different ways in Fig. 4. Focusing on the aggregates in
the database (all of whose scattering properties were computed with the GMM),
they range in mass from approximately <inline-formula><mml:math display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>   to 20 mg
with backscattering cross sections at W-band from approximately
<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>  to 10<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">1</mml:mn></mml:msup></mml:math></inline-formula> mm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> (Fig. 4b<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:math></inline-formula>). The aggregates in
Leinonen and Moisseev (2015) range in mass from approximately 5 <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> mg to just over 10 mg with W-band backscattering cross
sections from just below 1 <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> mm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>
to just above 2 <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn mathvariant="normal">0</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> mm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> (their Fig. 2). While these ranges are comparable to each other, there are differences
within them. For example, the drop in backscattering cross section that takes
place when particle dimensions along the direction of the radiation reach
about one-third of the wavelength (Fig. 4b<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:math></inline-formula>,b<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) occurs at smaller particle masses
here than in Leinonen and Moisseev (2015). We attribute these differences
between the two databases to the methods for building the aggregates and
differences in the orientations of the aggregates for the backscattering
calculations. The spacing in mass between ice particles is much smaller in
Leinonen and Moisseev (2015) as they needed small steps in mass for their
integrals of backscattering cross sections over aggregate size distributions.</p>
      <p>Upon inspection of the X-band backscattering cross sections in the database, only the
aggregates have maximum dimensions exceeding one-third the
wavelength (Fig. 4a<sub>2</sub>) and
hence exhibit the drop in cross section with increasing
size. For particles that are small compared to the wavelength, backscattering cross
sections generally increase with mass (Fig. 4a<sub>3</sub>) and its
proxy <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Fig. 4a<sub>1</sub>). The residual
spread about the best-fit line to the backscattering cross sections at X-band
wavelengths for ice-particle masses less than 1 mg, with the plates falling
slightly above the line and columns slightly below the line, is explained by
near-field interactions within the crystals (Lu et al., 2013). The ratio of
plate to column backscattering cross sections at 0.5 mg is about 4, or 6 dB,
which is quite close to the spread illustrated in Lu et al. (2013) for
electric fields parallel and perpendicular to the basal faces of dendritic
crystals.</p>
      <p>Finally, the spread in the backscattering cross sections of ice particles at
X-band wavelengths and at W-band wavelengths for side incident radiation of
each ice-particle type for a given mass (Fig. 4a<sub>3</sub>, b<sub>3</sub>) is due to variations in
morphologies for aggregate and branched planar particles, in thickness and
maximum dimension for plate and column particles, and in cone angle and density for
conical graupel. For branched planar, plate, and column particles, the
different numerical methods also contribute to the spread.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5" specific-use="star"><caption><p>Database branched planar
crystal  <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="bold">a</mml:mi><mml:mn mathvariant="bold">1</mml:mn></mml:msub><mml:mo>,</mml:mo><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msub><mml:mi mathvariant="bold">b</mml:mi><mml:mn mathvariant="bold">1</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> scattering cross sections,  <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="bold">a</mml:mi><mml:mn mathvariant="bold">2</mml:mn></mml:msub><mml:mo>,</mml:mo><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msub><mml:mi mathvariant="bold">b</mml:mi><mml:mn mathvariant="bold">2</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> backscattering
cross sections, and <inline-formula><mml:math display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="bold">a</mml:mi><mml:mn mathvariant="bold">3</mml:mn></mml:msub><mml:mo>,</mml:mo><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msub><mml:mi mathvariant="bold">b</mml:mi><mml:mn mathvariant="bold">3</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> asymmetry parameters for incident h-polarized radiation vs. size parameter
<inline-formula><mml:math display="inline"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi>r</mml:mi><mml:mi>e</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:mi mathvariant="italic">λ</mml:mi></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> is the
wavelength of the incident radiation and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the
radius of a solid (0.917 g cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) ice sphere with mass equal to that of
the crystal. GMM results are represented by open circles, whereas DDA results
are given by open squares. The solid lines represent the results for (blue)
sector snowflakes and (red) dendrite snowflakes from Liu (2008).</p></caption>
        <?xmltex \igopts{width=369.885827pt}?><graphic xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016-f05.png"/>

      </fig>

      <p>The database developed by Liu (2008) and Nowell et al. (2013) is
well documented and openly accessible. In Fig. 5 scattering cross sections,
backscattering cross sections, and asymmetry parameters computed via both DDA
and GMM for branched planar crystals in the current database are compared to
those of snowflakes in Liu (2008). Because Liu (2008) provides values
averaged over random orientations of each snowflake and has a single
snowflake for each maximum dimension (or mass represented by a single value
of <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, where <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the
radius of a solid (0.916 g cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) ice sphere with mass equal to that of
the crystal), values for the two snowflake types in Liu (2008) vs. size
parameter 2<inline-formula><mml:math display="inline"><mml:mrow><mml:mi mathvariant="italic">π</mml:mi><mml:msub><mml:mi>r</mml:mi><mml:mi mathvariant="normal">e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math display="inline"><mml:mo>/</mml:mo></mml:math></inline-formula> <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula>, where <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">λ</mml:mi></mml:math></inline-formula> is the
wavelength of the incident radiation, can be represented as lines. For the
current database the spread in values for fixed <italic>r<sub>e</sub></italic>
results from changes in ice-particle orientation with respect to the incident
radiation, changes in ice-particle morphology, and differences between the DDA
and GMM scattering methods.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6" specific-use="star"><caption><p><bold>(a)</bold> Morphology of the 361st branched planar crystal
in the database. <bold>(b)</bold>  The phase function <italic>p</italic> (grey dots) of the
361st branched planar crystal as a function of scattering
polar angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> for incident radiation with
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn>60</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>; for each scattering polar angle
<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> there are 72 grey dots, representing values for each
of the 72 different scattering azimuth angles <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>. The
phase function averaged over the 72 values of <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> is
represented by the solid red line. The dashed red and blue lines represent
the phase functions of the sector snowflake and dendrite snowflake from
Liu (2008) with a similar maximum dimension. <bold>(c)</bold> The phase function <italic>p</italic>
of the 361st branched planar crystal for (blue)
<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>=</mml:mo><mml:mn>60</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and (red) <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup><mml:mo>=</mml:mo><mml:mn>120</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> as
a function of scattering azimuth angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> for incident
radiation with <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn>60</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>. <bold>(d)</bold> The phase functions
<italic>p</italic> (averaged over scattering azimuth angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>) of
the 361st branched planar crystal as a function of
scattering polar angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> for radiation with incident
polar angles <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>, 30, 60, and 90<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>
and with incident azimuth angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>. The
results in <bold>(b)</bold>, <bold>(c)</bold>, and <bold>(d)</bold> were obtained from DDA calculations at the W-band
wavelength.</p></caption>
        <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://amt.copernicus.org/articles/9/5119/2016/amt-9-5119-2016-f06.png"/>

      </fig>

      <p>For branched planar crystals oriented such that the normal to their basal
planes is parallel to the incident radiation (<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>), incident radiation scattered
across the crystal constructively interferes in both the forward and backward
scattering directions, because the thickness of each crystal is much smaller
than the wavelength, resulting in induced dipoles that are all in phase. This,
together with symmetry in the phases of the waves scattered into the forward
and backward hemispheres, leads to asymmetry parameters that remain 0 for all
crystal sizes (Fig. 5a<sub>3</sub>, b<sub>3</sub>, dark blue
circles). At oblique incident radiation, there are both constructive and
destructive interferences for the scattered waves. As
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> increases towards 90<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, scattered waves in
the forward direction retain their constructive interference, whereas waves
scattered in other directions, including the backward direction, lose it.
This is especially true at the smaller W-band wavelength as the planar
crystals increase in maximum dimension. As this happens, forward scattering
dominates, with asymmetry parameters of the largest planar crystals at the
W-band wavelength reaching values near 0.9 at side
incidence (<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn>90</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>; Fig. 5b<sub>3</sub>, red circles). Though these tendencies are also apparent
at the X-band wavelength, they are much smaller because all branched planar
crystals in the database are small compared to (less than one-third of) the
wavelength. As a result, at the X-band wavelength the asymmetry parameters
never exceed 0.08.</p>
      <p>The loss in constructive interference in the backward scattering direction
for increasing incident polar angle <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> is
also reflected in drops in the backscattering cross sections, once again with
the drop increasing with branched planar crystal maximum dimension and with
it being significantly greater at the W-band wavelength compared to the
X-band wavelength (Fig.  5a<sub>2</sub>,b<sub>2</sub>).</p>
      <p>Carefully inspecting the backscattering cross sections at the X-band
wavelength near a size parameter of 0.13 (red oval in Fig. 5a<sub>2</sub>), one finds eight different particles contributing to
them. As expected, the backscattering cross sections for all eight particles
decrease with increasing incident polar angle. However, four of the particles
have significantly larger backscattering cross sections at
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> than the other four. These
differences result from the method (i.e., DDA vs. GMM) used to compute the
scattering properties. The four sets with the largest backscattering cross
sections were computed with DDA, whereas the four sets with the smallest
backscattering cross sections are for the same four branched planar crystals
but computed via GMM. The backscattering cross sections in
Fig. 5a<sub>2</sub> that fall below those for the sector and dendrite
snowflakes in Liu (2008) all result from GMM calculations, though many GMM
calculations also lie above them. That the Liu (2008) backscattering cross
sections split the difference between the DDA and some GMM results in the
current database was not by design. All of these same features are evident in
the scattering cross sections in Fig. 5a<sub>1</sub>, though the
decrease with increasing incident polar angle
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> is not as large because the scattering
cross sections are an integral quantity that includes contributions from
directions other than backward.</p>
      <p>Differences in the scattering cross sections at the W-band wavelength between
DDA and GMM are again evident (Fig. 5b<sub>1</sub>). However, for size
parameters larger than 0.75 the branched planar crystals are sufficiently
large that complicated patterns of constructive and destructive interference
vs. scattering angles (<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">sca</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula>)
take place for all incident polar angles <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>.
As a result, variability is driven by the incident polar angle, and the
scattering cross sections first increase and then decrease with incident
polar angle, reaching maximum values near <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn>50</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>.</p>
      <p>Richness in the directionality of the scattering for branched planar crystals
that are large compared to the W-band wavelength is illustrated in Fig. 6. Figure 6a
is a depiction of the branched planar crystal upon which the Fig. 6 results
are based; it has a maximum dimension greater than 5.5 mm and is nearly
twice the wavelength. For unpolarized radiation with an incident polar angle
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn>60</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and incident azimuth angle
<inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">ϕ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, the resulting scattering phase
function lacks azimuthal symmetry except for scattering angles close to the
forward and backward directions (Fig. 6b, grey dots; Fig. 6c, blue and red
lines). This lack of azimuthal symmetry is one motivating factor for not
reporting a scattering phase function in the database while retaining the
amplitude scattering matrices at 1<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> intervals in scattering polar angle and
5<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> intervals in scattering azimuth angle. The scattering phase function for
a specific direction can be calculated from the amplitude scattering matrices
following Bohren and Huffman (1983, pp. 71–72). Averaging the scattering
phase function over all azimuth angles for fixed scattering polar angle leads
to smooth dependence on scattering polar angle (Fig. 6b, solid red line)
with similar values in the forward scattering direction to the scattering
phase functions for randomly oriented snowflakes (Fig. 6b, dashed red and
blue lines; Liu, 2008).</p>
      <p>As Liu (2008) points out, when computing the scattering properties of a
randomly oriented ice particle, one must average over small changes in the
orientation of an ice particle, especially in order to compute accurate
backscattering cross sections. This being the case is evident in Fig. 6d,
where the scattering phase function does not depend strongly on the
orientation of the branched planar crystal for forward directions, where
constructive interference always occurs. In the backward direction the
scattering phase function is highly dependent on the ice-particle
orientation, dropping by 4 orders of magnitude as the incident polar angle
changes from <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, for which the
asymmetry parameter is 0, to <inline-formula><mml:math display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">P</mml:mi><mml:mi mathvariant="normal">inc</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mn>90</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, for
which the asymmetry parameter is much closer to 1.</p>
      <p>The imaginary part of the refractive index of ice is about 4 orders of
magnitude smaller than its real part at radar wavelengths (Table 1) and is
sensitive to the dielectric constant adjustment that we used to compensate
for the tiny sphere and air-gap mixture representation of ice particles in
the GMM scattering calculations. Moreover, the imaginary part can have large
relative changes over temperatures ranging from <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>40  to
0 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C (Mätzler, 2006). Because the current database incorporated
dielectric constants from Ray (1972), the imaginary parts of which are
significantly smaller than those of Mätzler (2006), and because we made
adjustments to them for the GMM calculations that may have substantially
altered their imaginary parts, the absorption cross sections in this database
should be used with caution.</p>
</sec>
<sec id="Ch1.S7" sec-type="conclusions">
  <title>Summary and future refinements</title>
      <p>A database of single-scattering properties of ice particles at millimeter to
centimeter wavelengths is presented to facilitate ground-based, airborne, and
satellite-based retrievals of ice cloud and ice precipitation properties.
Branched planar crystals, plates, columns, aggregates, and conical graupel
are generated, and their single-scattering properties calculated, using the GMM
and/or DDA methods for different directions of the incident radiation. In
addition to the scattering properties of each ice particle, including their
amplitude scattering matrices as a function of incident and scattered
directions, which provide full polarization information, the database also
contains the physical properties of each ice particle, including the location
of each ice-particle component (a tiny sphere in the GMM calculations and a
polarizable point in the DDA calculations), together with imagery of it. The
addition of new ice-particle realizations or new ice-particle species, such
as rimed or melting particles, will be incorporated into the database as they
become available and then subsequently documented.</p>
      <p>There are several limitations to the current database. First, the ice
particles in the database are just a small representation of the ice
particles that exist in nature. Direct observations of exact morphologies of
real ice particles, especially those in clouds, are limited. Improvements in
the observation of detailed ice-particle structures would serve as valuable
guidance in the future development of the database. Second, calculations at
high frequencies for more directions of the incident radiation will be
necessary to ensure accurate interpolation of ice-particle single-scattering
properties to other directions of the incident radiation. And finally, the
absorption cross sections in the database should be used with caution as they
are based on older dielectric constants (Ray, 1972), and in the case of the
GMM calculations may have errors in them as a result of adjustments made to
compensate for the air gaps in the tiny sphere representations of the ice
particles.</p>
</sec>
<sec id="Ch1.S8">
  <title>Data availability</title>
      <p>The database is available
through <ext-link xlink:href="http://dx.doi.org/10.5439/1258029" ext-link-type="DOI">10.5439/1258029</ext-link> (Aydin et al., 2016).</p>
</sec>

      
      </body>
    <back><app-group>
        <supplementary-material position="anchor"><p><bold>The Supplement related to this article is available online at <inline-supplementary-material xlink:href="http://dx.doi.org/10.5194/amt-9-5119-2016-supplement" xlink:title="pdf">doi:10.5194/amt-9-5119-2016-supplement</inline-supplementary-material>.</bold></p></supplementary-material>
        </app-group><ack><title>Acknowledgements</title><p>We would like to thank Giriprakash Palanisamy and Kathy Lazar for their
invaluable help in setting up the database as a Department of Energy (DOE)
Atmospheric Radiation Measurement (ARM) Program Principal Investigator Data
Product that comes with a DOI. Raymond McCord and Kenneth Kehoe, also of the
DOE ARM Program, provided many useful comments regarding the NetCDF4 files in
which the database is housed. Discussions with Stefan Kneifel, Ralf Bennartz,
Alan Geer, Pavlos Kollias, Ann Fridlind, Greg McFarquhar,
Christopher Williams, and Stephen Nesbit were helpful in framing the scope of the
database products and/or generating interest within the DOE ARM Program in
hosting it. Development of the database was supported primarily by NSF Grant
AGS-128180. Eugene E. Clothiaux's contributions to the database were
supported by DOE Grant DE-FG02-05ER64058. The authors would like to
acknowledge high-performance computing support from Yellowstone (ark:/85065/d7wd3xhc) provided by NCAR's Computational and Information
Systems Laboratory, sponsored by the National Science Foundation. Portions of
this research were conducted with Advanced Cyberinfrastructure computational
resources provided by the Institute for CyberScience at The Pennsylvania
State University (<uri>http://ics.psu.edu</uri>)<?xmltex \hack{\newline}?><?xmltex \hack{\newline}?>
Edited by:  M. Kulie<?xmltex \hack{\newline}?>
Reviewed by: two anonymous referees</p></ack><ref-list>
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    <!--<article-title-html>A polarimetric scattering database for non-spherical ice particles at microwave wavelengths</article-title-html>
<abstract-html><p class="p">The atmospheric science community has entered a period in which
electromagnetic scattering properties at microwave frequencies of
realistically constructed ice particles are necessary for making progress on
a number of fronts. One front includes retrieval of ice-particle properties
and signatures from ground-based, airborne, and satellite-based radar and
radiometer observations. Another front is evaluation of model microphysics by
application of forward operators to their outputs and comparison to
observations during case study periods. Yet a third front is data
assimilation, where again forward operators are applied to databases of
ice-particle scattering properties and the results compared to observations,
with their differences leading to corrections of the model state.</p><p class="p">Over the past decade investigators have developed databases of ice-particle
scattering properties at microwave frequencies and made them openly
available. Motivated by and complementing these earlier efforts, a database
containing polarimetric single-scattering properties of various types of ice
particles at millimeter to centimeter wavelengths is presented. While the
database presented here contains only single-scattering properties of ice
particles in a fixed orientation, ice-particle scattering properties are
computed for many different directions of the radiation incident on them.
These results are useful for understanding the dependence of ice-particle
scattering properties on ice-particle orientation with respect to the
incident radiation. For ice particles that are small compared to the wavelength, the
number of incident directions of the radiation is sufficient to compute
reasonable estimates of their (randomly) orientation-averaged scattering
properties.</p><p class="p">This database is complementary to earlier ones in that it contains
complete (polarimetric) scattering property information for each ice particle
– 44 plates, 30 columns, 405 branched planar crystals, 660 aggregates, and
640 conical graupel – and direction of incident radiation but is limited to
four frequencies (X-, Ku-, Ka-, and W-bands), does not include temperature
dependencies of the single-scattering properties, and does not include
scattering properties averaged over randomly oriented ice particles. Rules
for constructing the morphologies of ice particles from one database to the
next often differ; consequently, analyses that incorporate all of the
different databases will contain the most variability, while illuminating
important differences between them. Publication of this database is in
support of future analyses of this nature and comes with the hope that doing
so helps contribute to the development of a database standard for
ice-particle scattering properties, like the NetCDF (Network Common Data Form) CF (Climate and Forecast)
or NetCDF CF/Radial metadata conventions.</p></abstract-html>
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