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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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https://doi.org/10.5194/amt-2020-127
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-2020-127
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

  04 May 2020

04 May 2020

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A revised version of this preprint was accepted for the journal AMT and is expected to appear here in due course.

Ground-based FTIR O3 retrievals from the 3040 cm−1 spectral range at Xianghe, China

Minqiang Zhou1, Pucai Wang2,3,4, Bavo Langerock1, Corinne Vigouroux1, Christian Hermans1, Nicolas Kumps1, Ting Wang2, Yang Yang2, Denghui Ji2, Liang Ran2, Jinqiang Zhang2, Yuejian Xuan2, Hongbin Chen2,3,4, Françoise Posny5, Valentin Duflot5,6, Jean-Marc Metzger6, and Martine De Mazière1 Minqiang Zhou et al.
  • 1Royal Belgian Institute for Space Aeronomy (BIRA-IASB), Brussels, 1180, Belgium
  • 2Key Laboratory of Middle Atmosphere and Global Environment Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
  • 3University of Chinese Academy of Sciences, Beijing, China
  • 4Xianghe Observatory of Whole Atmosphere, Institute of Atmospheric Physics, Chinese Academy of Sciences, Xianghe, China
  • 5LACy, Laboratoire de l’Atmosphère et des Cyclones, UMR8105 (CNRS, Université de La Réunion, Météo-France), Saint-Denis, Réunion, France
  • 6UMS 3365 – OSU Réunion, Université de La Réunion, Saint-Denis, Réunion, France

Abstract. In this study, we present O3 retrievals from ground-based Fourier-transform infrared (FTIR) solar absorption measurements between June 2018 and December 2019 at Xianghe, China (39.75° N, 116.96° E). The FTIR spectrometer at Xianghe is operated with indium gallium arsenide (InGaAs) and indium antimonide (InSb) detectors, recording the spectra between 1800 and 11000 cm−1. As the harmonized FTIR O3 retrieval strategy (Vigouroux et al., 2015) within the Network for the Detection of Atmospheric Composition Change (NDACC) uses the 1000 cm−1 spectral range, we designed an alternative O3 retrieval strategy in the 3040 cm−1 spectral range at Xianghe.

The retrieved O3 profile is mainly sensitive to the vertical range between 5 and 40 km, and the degree of freedom for signal is 2.4 ± 0.3 (1σ), indicating that there are two individual pieces of information in partial columns between the surface and 20 km and between 20 and 40 km. According to the optimal estimation method, the systematic and random uncertainties of the FTIR O3 total columns are about 13.6 % and 1.4 %, respectively. The random uncertainty is consistent with the observed daily standard deviation of the FTIR retrievals.

To validate the FTIR O3 total and partial columns, we apply the same O3 retrieval strategy at Maïdo, Reunion Island (21.08° N, 55.38° E). The FTIR O3 (3040 cm−1) measurements at Xianghe and Maïdo are then compared with the nearby ozonesondes at Beijing (39.81° N, 116.47° E) and at Gillot (20.89° S, 55.53° E), respectively, as well as with co-located TROPOspheric Monitoring Instrument (TROPOMI) satellite measurements at both sites. In addition, at Maïdo, we compare the FTIR O3 (3040 cm−1) retrievals with the standard NDACC FTIR O3 measurements using the 1000 cm−1 spectral range. It is found that the total columns retrieved from the FTIR O3 3040 cm−1 measurements are underestimated by 5.5–9.0 %, which is mainly due to the systematic uncertainty in the partial column between 20 and 40 km (about −10.4 %). The systematic uncertainty in the partial column between surface and 20 km is relatively small (within 2.4 %). By comparison with other measurements, it is found that the FTIR O3 (3040 cm−1) retrievals capture very well the seasonal and synoptic variations of the O3 total and two partial columns. Therefore, the ongoing FTIR measurements at Xianghe can provide useful information on the O3 variations and (in the future) long-term trends.

Minqiang Zhou et al.

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Minqiang Zhou et al.

Minqiang Zhou et al.

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Short summary
We study O3 retrievals in the 3040 cm−1 spectral range from FTIR measurements at Xianghe China (39.75N, 116.96E, 50 m a.s.l.) between June 2018 and December 2019. It is found that the FTIR O3 (3040 cm−1) retrievals capture very well the seasonal and synoptic variations of O3. The systematic and random uncertainties of FTIR O3 (3040 cm−1) total column are about 5.5–9.0 % and 1.4%, respectively. The DOF is 2.4±0.3 (1σ), with 2 individual pieces of information in surface-20 km and 20–40 km.
We study O3 retrievals in the 3040 cm−1 spectral range from FTIR measurements at Xianghe China...
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