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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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Preprints
https://doi.org/10.5194/amt-2020-186
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-2020-186
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

  01 Jul 2020

01 Jul 2020

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A revised version of this preprint is currently under review for the journal AMT.

Version 2 Ozone Monitoring Instrument SO2 Product (OMSO2 V2): New Anthropogenic SO2 Vertical Column Density Dataset

Can Li1,2, Nickolay A. Krotkov2, Peter J. T. Leonard3,2, Simon Carn4, Joanna Joiner2, Robert J. D. Spurr5, and Alexander Vasilkov6 Can Li et al.
  • 1Earth System Science Interdisciplinary Center, University of Maryland, College Park, MD 20742, USA
  • 2NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA
  • 3ADNET Systems, Inc., Lanham, MD 20706, USA
  • 4Michigan Technological University, Houghton, MI 49931, USA
  • 5RT Solutions Inc., Cambridge, MA 02138, USA
  • 6Science Systems and Applications Inc., Lanham, MD 20706, USA

Abstract. The Ozone Monitoring Instrument (OMI) has been providing global observations of SO2 pollution since 2004. Here we introduce the new anthropogenic SO2 vertical column density (VCD) dataset in the version 2 OMI SO2 product (OMSO2 V2). As with the previous version (OMSO2 V1.3), the new dataset is generated with an algorithm based on principal component analysis of OMI radiances, but features several updates. The most important among those is the use of expanded lookup tables and model a priori profiles to estimate SO2 Jacobians for individual OMI pixels, in order to better characterize pixel-to-pixel variations in SO2 sensitivity, including over snow and ice. Additionally, new data screening and spectral fitting schemes have been implemented to improve the quality of the spectral fit. As compared with the planetary boundary layer SO2 dataset in OMSO2 V1.3, the new dataset has substantially better data quality, especially over areas that are relatively clean or affected by the south Atlantic anomaly. The updated retrievals over snow/ice yield more realistic seasonal changes in SO2 at high latitudes and offer enhanced sensitivity to sources during wintertime. An error analysis has been conducted to assess uncertainties in SO2 VCDs from both the spectral fit and Jacobian calculations. The uncertainties from spectral fitting are reflected in SO2 slant column densities (SCDs) and largely depend on the signal-to-noise ratio of the measured radiances, as implied by the generally smaller SCD uncertainties over clouds or for lower solar zenith angles. The SCD uncertainties for individual pixels are estimated to be ~ 0.15–0.3 DU (Dobson Units) between ~ 40° S and ~ 40° N and to be ~ 0.2–0.5 DU at higher latitudes. The uncertainties from the Jacobians are approximately ~ 50–100 % over polluted areas, and primarily attributed to errors in SO2 a priori profiles and cloud pressures, as well as the lack of explicit treatment for aerosols. Finally, the daily mean and median SCDs over the presumably SO2-free equatorial East Pacific have increased by only ~ 0.0035 DU and ~ 0.003 DU respectively over the entire 15-year OMI record; while the standard deviation of SCDs has grown by only ~ 0.02 DU or ~ 10 %. Such remarkable long-term stability makes the new dataset particularly suitable for detecting regional changes in SO2 pollution.

Can Li et al.

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Can Li et al.

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Short summary
Sulfur dioxide (SO2) is an important pollutant that causes haze and acid rain. The Ozone Monitoring Instrument (OMI) has been providing global observation of SO2 from space for over 15 years. In this paper, we introduce a new OMI SO2 dataset for global pollution monitoring. The dataset better accounts for the influences of different factors such as location, and sun and satellite angles, leading to improved data quality. The new OMI SO2 dataset is publicly available through NASA data center.
Sulfur dioxide (SO2) is an important pollutant that causes haze and acid rain. The Ozone...
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