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Atmospheric Measurement Techniques An interactive open-access journal of the European Geosciences Union
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https://doi.org/10.5194/amt-2020-438
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-2020-438
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

  03 Nov 2020

03 Nov 2020

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This preprint is currently under review for the journal AMT.

Modeled source apportionment of black carbon particles coated with a light-scattering shell

Aki Virkkula Aki Virkkula
  • Finnish Meteorological Institute, Helsinki, Finland

Abstract. The Aethalometer model been used widely for estimating the contributions of fossil fuel emissions and biomass burning to equivalent black carbon (eBC). The calculation is based on measured absorption Ångström exponents (αabs). The interpretation αabs is ambiguous since it is well-known that it not only depends on the dominant absorber but also on the size and internal structure of the particles, core size and shell thickness. In this work the uncertainties of the Aethalometer-model-derived apparent fractions of absorption by eBC from fossil fuel and biomass burning are evaluated with a core-shell Mie model. Biomass-burning fractions (BB(%)) were calculated for pure and coated single BC particles, for lognormal unimodal and bimodal size distributions of BC cores coated with ammonium sulfate, a scattering-only material. BB(%) was very seldom 0 % even though BC was the only absorbing material in the simulations. The shape of size distribution plays an important role. Narrow size distributions result in higher αabs and BB(%) values than wide size distributions. The sensitivity of αabs and BB(%) to variations in shell volume fractions is the highest for accumulation mode particles. This is important because that is where the largest aerosol mass is. For the interpretation of absorption Ångström exponents it would be very good to measure BC size distributions and shell thicknesses together with the wavelength dependency of absorption.

Aki Virkkula

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Aki Virkkula

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Short summary
The Aethalometer model is used widely for estimating the contributions of fossil fuel emissions and biomass burning to black carbon. The calculation is based on measured absorption Ångström exponents which is ambiguous since it not only depends on the dominant absorber but also on the size and internal structure of the particles, core size and shell thickness. The uncertainties of the fractions of absorption by eBC from fossil fuel and biomass burning are evaluated with a core-shell Mie model.
The Aethalometer model is used widely for estimating the contributions of fossil fuel emissions...
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