<p>High-frequency parts of ocean wave spectra are strongly coupled to the local wind. Measurements of ocean wave spectra can be used to estimate sea surface winds. In this study, two deep neural networks (DNNs) were used to estimate the wind speed and direction from the first five Fourier coefficients from buoys. The DNNs were trained by wind and wave measurements from more than 100 meteorological buoys during 2014–2018. It is found that the wave measurements can best represent the wind information ~1 h ago, because the wave spectra contain wind information a short period before. The overall root-mean-square error (RMSE) of estimated wind speed is ~1.1 m/s, and the RMSE of wind direction is ~14° when wind speed is 7~25 m/s. This model can not only be used for the wind estimation for compact wave buoys but also for the quality control of wind and wave measurements from meteorological buoys.</p>