Articles | Volume 10, issue 10
https://doi.org/10.5194/amt-10-3801-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-10-3801-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Single-particle measurements of bouncing particles and in situ collection efficiency from an airborne aerosol mass spectrometer (AMS) with light-scattering detection
Jin Liao
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado at Boulder, Boulder, CO 80309, USA
now at: Universities Space Research Association, Columbia, MD 21046, USA
now at: NASA Goddard Space Flight Center, Atmospheric Chemistry and Dynamic Laboratory, Greenbelt, MD 20771, USA
Charles A. Brock
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO 80305, USA
Daniel M. Murphy
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO 80305, USA
Donna T. Sueper
Aerodyne Research Inc., Billerica, MA 01821, USA
André Welti
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado at Boulder, Boulder, CO 80309, USA
now at: Leibniz Institute for Tropospheric Research, Department of Physics, Leipzig, 04318, Germany
Ann M. Middlebrook
CORRESPONDING AUTHOR
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO 80305, USA
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- Particle detection using the dual-vaporizer configuration of the soot particle Aerosol Mass Spectrometer (SP-AMS) A. Avery et al. 10.1080/02786826.2020.1844132
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- An Odd Oxygen Framework for Wintertime Ammonium Nitrate Aerosol Pollution in Urban Areas: NOx and VOC Control as Mitigation Strategies C. Womack et al. 10.1029/2019GL082028
- Evidence in biomass burning smoke for a light-absorbing aerosol with properties intermediate between brown and black carbon G. Adler et al. 10.1080/02786826.2019.1617832
- Airborne and ground-based observations of ammonium-nitrate-dominated aerosols in a shallow boundary layer during intense winter pollution episodes in northern Utah A. Franchin et al. 10.5194/acp-18-17259-2018
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11 citations as recorded by crossref.
- Measurement report: Evaluation of the TOF-ACSM-CV for PM1.0 and PM2.5 measurements during the RITA-2021 field campaign X. Liu et al. 10.5194/acp-24-3405-2024
- Limited impact of sulfate-driven chemistry on black carbon aerosol aging in power plant plumes M. Z. Markovic et al. 10.3934/environsci.2018.3.195
- Particle detection using the dual-vaporizer configuration of the soot particle Aerosol Mass Spectrometer (SP-AMS) A. Avery et al. 10.1080/02786826.2020.1844132
- Reactive nitrogen and total organic carbon calibration techniques for the Aerodyne aerosol mass spectrometer D. Price et al. 10.1080/02786826.2023.2218462
- Exploring the processes controlling secondary inorganic aerosol: evaluating the global GEOS-Chem simulation using a suite of aircraft campaigns O. Norman et al. 10.5194/acp-25-771-2025
- Molecular Properties of Brown Carbon Aerosol from Biomass Burning of Wildland Fuels at the Fire Sciences Laboratory L. Azzarello et al. 10.1021/acsestair.4c00264
- Evaluation of the new capture vaporizer for aerosol mass spectrometers: Characterization of organic aerosol mass spectra W. Hu et al. 10.1080/02786826.2018.1454584
- An Odd Oxygen Framework for Wintertime Ammonium Nitrate Aerosol Pollution in Urban Areas: NOx and VOC Control as Mitigation Strategies C. Womack et al. 10.1029/2019GL082028
- Evidence in biomass burning smoke for a light-absorbing aerosol with properties intermediate between brown and black carbon G. Adler et al. 10.1080/02786826.2019.1617832
- Airborne and ground-based observations of ammonium-nitrate-dominated aerosols in a shallow boundary layer during intense winter pollution episodes in northern Utah A. Franchin et al. 10.5194/acp-18-17259-2018
- Midlatitude Ozone Depletion and Air Quality Impacts from Industrial Halogen Emissions in the Great Salt Lake Basin C. Womack et al. 10.1021/acs.est.2c05376
Latest update: 30 Oct 2025
Short summary
The Aerodyne aerosol mass spectrometer (AMS) has emerged as a widely used method for measuring the real-time, submicron, nonrefractory aerosol composition. A large uncertainty in accurate measurements with the AMS (the collection efficiency due to particle bounce) is evaluated in this paper using in situ measurements of particle light scattering. Current calculations of the collection efficiency reasonably predict this effect in acidic environments, resulting in more confidence for AMS results.
The Aerodyne aerosol mass spectrometer (AMS) has emerged as a widely used method for measuring...