Articles | Volume 10, issue 3
https://doi.org/10.5194/amt-10-839-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-10-839-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
The Caltech Photooxidation Flow Tube reactor: design, fluid dynamics and characterization
Yuanlong Huang
Department of Environmental Science and Engineering, California Institute of Technology, Pasadena, CA, USA
Matthew M. Coggon
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA, USA
now at: CIRES, University of Colorado, and NOAA Earth System Research Laboratory, Boulder, CO, USA
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA, USA
Hanna Lignell
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA, USA
now at: South Coast Air Quality Management District, Diamond Bar, CA, USA
Michael U. Bauer
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA, USA
Richard C. Flagan
Department of Environmental Science and Engineering, California Institute of Technology, Pasadena, CA, USA
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA, USA
Department of Environmental Science and Engineering, California Institute of Technology, Pasadena, CA, USA
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA, USA
Viewed
Total article views: 4,861 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 22 Sep 2016)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
2,825 | 1,878 | 158 | 4,861 | 130 | 177 |
- HTML: 2,825
- PDF: 1,878
- XML: 158
- Total: 4,861
- BibTeX: 130
- EndNote: 177
Total article views: 4,162 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 09 Mar 2017)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
2,445 | 1,567 | 150 | 4,162 | 121 | 165 |
- HTML: 2,445
- PDF: 1,567
- XML: 150
- Total: 4,162
- BibTeX: 121
- EndNote: 165
Total article views: 699 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 22 Sep 2016)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
380 | 311 | 8 | 699 | 9 | 12 |
- HTML: 380
- PDF: 311
- XML: 8
- Total: 699
- BibTeX: 9
- EndNote: 12
Viewed (geographical distribution)
Total article views: 4,861 (including HTML, PDF, and XML)
Thereof 4,694 with geography defined
and 167 with unknown origin.
Total article views: 4,162 (including HTML, PDF, and XML)
Thereof 4,022 with geography defined
and 140 with unknown origin.
Total article views: 699 (including HTML, PDF, and XML)
Thereof 672 with geography defined
and 27 with unknown origin.
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Cited
43 citations as recorded by crossref.
- Growth of Aitken mode ammonium sulfate particles by α-pinene ozonolysis J. Krasnomowitz et al. 10.1080/02786826.2019.1568381
- Aging aerosol in a well-mixed continuous-flow tank reactor: an introduction of the activation time distribution F. Friebel & A. Mensah 10.5194/amt-12-2647-2019
- Temperature error‐correction method for surface air temperature data J. Yang et al. 10.1002/met.1972
- Understanding balloon-borne frost point hygrometer measurements after contamination by mixed-phase clouds T. Jorge et al. 10.5194/amt-14-239-2021
- The Chamber Wall Index for Gas–Wall Interactions in Atmospheric Environmental Enclosures W. Brune 10.1021/acs.est.8b06260
- A Spherical Temperature Sensor Array Design for Near-Surface Atmospheric Temperature Studies J. Yang et al. 10.1175/JTECH-D-19-0188.1
- HOx and NOx production in oxidation flow reactors via photolysis of isopropyl nitrite, isopropyl nitrite-d7, and 1,3-propyl dinitrite at λ = 254, 350, and 369 nm A. Lambe et al. 10.5194/amt-12-299-2019
- Technical Note: Effect of varying the λ = 185 and 254 nm photon flux ratio on radical generation in oxidation flow reactors J. Rowe et al. 10.5194/acp-20-13417-2020
- Characterization of a new Teflon chamber and on-line analysis of isomeric multifunctional photooxidation products F. Löher et al. 10.5194/amt-17-4553-2024
- A new oxidation flow reactor for the measurements of secondary aerosol formation: Characterisation and a case study C. Wu et al. 10.1016/j.atmosenv.2023.119886
- Rapid Aqueous-Phase Hydrolysis of Ester Hydroperoxides Arising from Criegee Intermediates and Organic Acids R. Zhao et al. 10.1021/acs.jpca.8b02195
- Measurement of ambient NO<sub>3</sub> reactivity: design, characterization and first deployment of a new instrument J. Liebmann et al. 10.5194/amt-10-1241-2017
- An oxidation flow reactor for simulating and accelerating secondary aerosol formation in aerosol liquid water and cloud droplets N. Xu et al. 10.5194/amt-17-4227-2024
- A note on flow behavior in axially-dispersed plug flow reactors with step input of tracer Y. Huang & J. Seinfeld 10.1016/j.aeaoa.2019.100006
- Effect of experimental conditions on secondary organic aerosol formation in an oxidation flow reactor R. Zhao et al. 10.1016/j.apr.2021.01.011
- Mechanism of heterogeneous reaction between gaseous elemental mercury and H2O2 on Fe3O4 (1 1 0) surface C. Zhou et al. 10.1016/j.comptc.2017.11.003
- Iodometry-Assisted Liquid Chromatography Electrospray Ionization Mass Spectrometry for Analysis of Organic Peroxides: An Application to Atmospheric Secondary Organic Aerosol R. Zhao et al. 10.1021/acs.est.7b04863
- Secondary organic aerosol formation from the oxidation of decamethylcyclopentasiloxane at atmospherically relevant OH concentrations S. Charan et al. 10.5194/acp-22-917-2022
- Insights Into Formation and Aging of Secondary Organic Aerosol From Oxidation Flow Reactors: A Review Z. Zhang et al. 10.1007/s40726-024-00309-7
- Coupling Filter-Based Thermal Desorption Chemical Ionization Mass Spectrometry with Liquid Chromatography/Electrospray Ionization Mass Spectrometry for Molecular Analysis of Secondary Organic Aerosol Y. Huang et al. 10.1021/acs.est.0c01779
- Design and Experiments of a Naturally-Ventilated Radiation Shield for Ground Temperature Measurement Q. Liu et al. 10.3390/atmos14030523
- Mechanism study of enhanced interaction between gaseous elemental mercury and hydroxylated UIO-66 C. Zhou et al. 10.1007/s11356-020-08415-x
- Mathematical Description of the Aerodynamic Characteristics of Stationary Flows in a Vertical Conical Diffuser When Air Is Supplied through Various Tube Configurations L. Plotnikov 10.3390/axioms12030244
- Design and characterization of a new oxidation flow reactor for laboratory and long-term ambient studies N. Xu & D. Collins 10.5194/amt-14-2891-2021
- Molecular-level insight into uptake of dimethylamine on hydrated nitric acid clusters A. Pysanenko et al. 10.1039/D2EA00094F
- Overview of ICARUS─A Curated, Open Access, Online Repository for Atmospheric Simulation Chamber Data T. Nguyen et al. 10.1021/acsearthspacechem.3c00043
- A vacuum ultraviolet ion source (VUV-IS) for iodide–chemical ionization mass spectrometry: a substitute for radioactive ion sources Y. Ji et al. 10.5194/amt-13-3683-2020
- Development of an atmospheric boundary layer detection system based on a rotary-wing unmanned aerial vehicle G. You et al. 10.1063/5.0227462
- Secondary Organic Aerosol Formation from Ambient Air at an Urban Site in Beijing: Effects of OH Exposure and Precursor Concentrations J. Liu et al. 10.1021/acs.est.7b05701
- Evaluation of the Oxidation Flow Reactor for particulate matter emission limit certification J. Cao et al. 10.1016/j.atmosenv.2019.117086
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Physical simulation of aerodynamic flow characteristics in a vertical diffuser with air supply through different pipe configurations L. Plotnikov et al. 10.30724/1998-9903-2023-25-2-187-200
- Secondary organic aerosols from OH oxidation of cyclic volatile methyl siloxanes as an important Si source in the atmosphere C. Han et al. 10.5194/acp-22-10827-2022
- Direct measurement of N2O5 heterogeneous uptake coefficients on ambient aerosols via an aerosol flow tube system: design, characterization and performance X. Chen et al. 10.5194/amt-15-7019-2022
- Secondary organic aerosol formation from <i>α</i>-pinene, alkanes, and oil-sands-related precursors in a new oxidation flow reactor K. Li et al. 10.5194/acp-19-9715-2019
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Design of a temperature error correction method used for meteorology and climate research J. Yang et al. 10.1016/j.atmosres.2021.105817
- A new oxidation flow reactor for measuring secondary aerosol formation of rapidly changing emission sources P. Simonen et al. 10.5194/amt-10-1519-2017
- Microcapillary film reactor outperforms single-bore mesocapillary reactors in continuous flow chemical reactions K. Gill et al. 10.1016/j.cej.2020.127860
- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
- Assessing the degree of plug flow in oxidation flow reactors (OFRs): a study on a potential aerosol mass (PAM) reactor D. Mitroo et al. 10.5194/amt-11-1741-2018
- Understanding the Impact of High-NOx Conditions on the Formation of Secondary Organic Aerosol in the Photooxidation of Oil Sand-Related Precursors K. Li et al. 10.1021/acs.est.9b05404
- A new aerosol flow reactor to study secondary organic aerosol K. Pereira et al. 10.5194/amt-12-4519-2019
43 citations as recorded by crossref.
- Growth of Aitken mode ammonium sulfate particles by α-pinene ozonolysis J. Krasnomowitz et al. 10.1080/02786826.2019.1568381
- Aging aerosol in a well-mixed continuous-flow tank reactor: an introduction of the activation time distribution F. Friebel & A. Mensah 10.5194/amt-12-2647-2019
- Temperature error‐correction method for surface air temperature data J. Yang et al. 10.1002/met.1972
- Understanding balloon-borne frost point hygrometer measurements after contamination by mixed-phase clouds T. Jorge et al. 10.5194/amt-14-239-2021
- The Chamber Wall Index for Gas–Wall Interactions in Atmospheric Environmental Enclosures W. Brune 10.1021/acs.est.8b06260
- A Spherical Temperature Sensor Array Design for Near-Surface Atmospheric Temperature Studies J. Yang et al. 10.1175/JTECH-D-19-0188.1
- HOx and NOx production in oxidation flow reactors via photolysis of isopropyl nitrite, isopropyl nitrite-d7, and 1,3-propyl dinitrite at λ = 254, 350, and 369 nm A. Lambe et al. 10.5194/amt-12-299-2019
- Technical Note: Effect of varying the λ = 185 and 254 nm photon flux ratio on radical generation in oxidation flow reactors J. Rowe et al. 10.5194/acp-20-13417-2020
- Characterization of a new Teflon chamber and on-line analysis of isomeric multifunctional photooxidation products F. Löher et al. 10.5194/amt-17-4553-2024
- A new oxidation flow reactor for the measurements of secondary aerosol formation: Characterisation and a case study C. Wu et al. 10.1016/j.atmosenv.2023.119886
- Rapid Aqueous-Phase Hydrolysis of Ester Hydroperoxides Arising from Criegee Intermediates and Organic Acids R. Zhao et al. 10.1021/acs.jpca.8b02195
- Measurement of ambient NO<sub>3</sub> reactivity: design, characterization and first deployment of a new instrument J. Liebmann et al. 10.5194/amt-10-1241-2017
- An oxidation flow reactor for simulating and accelerating secondary aerosol formation in aerosol liquid water and cloud droplets N. Xu et al. 10.5194/amt-17-4227-2024
- A note on flow behavior in axially-dispersed plug flow reactors with step input of tracer Y. Huang & J. Seinfeld 10.1016/j.aeaoa.2019.100006
- Effect of experimental conditions on secondary organic aerosol formation in an oxidation flow reactor R. Zhao et al. 10.1016/j.apr.2021.01.011
- Mechanism of heterogeneous reaction between gaseous elemental mercury and H2O2 on Fe3O4 (1 1 0) surface C. Zhou et al. 10.1016/j.comptc.2017.11.003
- Iodometry-Assisted Liquid Chromatography Electrospray Ionization Mass Spectrometry for Analysis of Organic Peroxides: An Application to Atmospheric Secondary Organic Aerosol R. Zhao et al. 10.1021/acs.est.7b04863
- Secondary organic aerosol formation from the oxidation of decamethylcyclopentasiloxane at atmospherically relevant OH concentrations S. Charan et al. 10.5194/acp-22-917-2022
- Insights Into Formation and Aging of Secondary Organic Aerosol From Oxidation Flow Reactors: A Review Z. Zhang et al. 10.1007/s40726-024-00309-7
- Coupling Filter-Based Thermal Desorption Chemical Ionization Mass Spectrometry with Liquid Chromatography/Electrospray Ionization Mass Spectrometry for Molecular Analysis of Secondary Organic Aerosol Y. Huang et al. 10.1021/acs.est.0c01779
- Design and Experiments of a Naturally-Ventilated Radiation Shield for Ground Temperature Measurement Q. Liu et al. 10.3390/atmos14030523
- Mechanism study of enhanced interaction between gaseous elemental mercury and hydroxylated UIO-66 C. Zhou et al. 10.1007/s11356-020-08415-x
- Mathematical Description of the Aerodynamic Characteristics of Stationary Flows in a Vertical Conical Diffuser When Air Is Supplied through Various Tube Configurations L. Plotnikov 10.3390/axioms12030244
- Design and characterization of a new oxidation flow reactor for laboratory and long-term ambient studies N. Xu & D. Collins 10.5194/amt-14-2891-2021
- Molecular-level insight into uptake of dimethylamine on hydrated nitric acid clusters A. Pysanenko et al. 10.1039/D2EA00094F
- Overview of ICARUS─A Curated, Open Access, Online Repository for Atmospheric Simulation Chamber Data T. Nguyen et al. 10.1021/acsearthspacechem.3c00043
- A vacuum ultraviolet ion source (VUV-IS) for iodide–chemical ionization mass spectrometry: a substitute for radioactive ion sources Y. Ji et al. 10.5194/amt-13-3683-2020
- Development of an atmospheric boundary layer detection system based on a rotary-wing unmanned aerial vehicle G. You et al. 10.1063/5.0227462
- Secondary Organic Aerosol Formation from Ambient Air at an Urban Site in Beijing: Effects of OH Exposure and Precursor Concentrations J. Liu et al. 10.1021/acs.est.7b05701
- Evaluation of the Oxidation Flow Reactor for particulate matter emission limit certification J. Cao et al. 10.1016/j.atmosenv.2019.117086
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Physical simulation of aerodynamic flow characteristics in a vertical diffuser with air supply through different pipe configurations L. Plotnikov et al. 10.30724/1998-9903-2023-25-2-187-200
- Secondary organic aerosols from OH oxidation of cyclic volatile methyl siloxanes as an important Si source in the atmosphere C. Han et al. 10.5194/acp-22-10827-2022
- Direct measurement of N2O5 heterogeneous uptake coefficients on ambient aerosols via an aerosol flow tube system: design, characterization and performance X. Chen et al. 10.5194/amt-15-7019-2022
- Secondary organic aerosol formation from <i>α</i>-pinene, alkanes, and oil-sands-related precursors in a new oxidation flow reactor K. Li et al. 10.5194/acp-19-9715-2019
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Design of a temperature error correction method used for meteorology and climate research J. Yang et al. 10.1016/j.atmosres.2021.105817
- A new oxidation flow reactor for measuring secondary aerosol formation of rapidly changing emission sources P. Simonen et al. 10.5194/amt-10-1519-2017
- Microcapillary film reactor outperforms single-bore mesocapillary reactors in continuous flow chemical reactions K. Gill et al. 10.1016/j.cej.2020.127860
- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
- Assessing the degree of plug flow in oxidation flow reactors (OFRs): a study on a potential aerosol mass (PAM) reactor D. Mitroo et al. 10.5194/amt-11-1741-2018
- Understanding the Impact of High-NOx Conditions on the Formation of Secondary Organic Aerosol in the Photooxidation of Oil Sand-Related Precursors K. Li et al. 10.1021/acs.est.9b05404
- A new aerosol flow reactor to study secondary organic aerosol K. Pereira et al. 10.5194/amt-12-4519-2019
Latest update: 14 Dec 2024
Short summary
We report on the development of a new laminar flow tube reactor for the study of gas-phase atmospheric chemistry and secondary organic aerosol formation. The present paper is devoted to the design and fluid dynamical characterization of the reactor. The results of gas and particle residence time distribution experiments in the reactor, together with an evaluation of the effect of non-isothermal conditions, are reported.
We report on the development of a new laminar flow tube reactor for the study of gas-phase...