Articles | Volume 11, issue 4
https://doi.org/10.5194/amt-11-2313-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-11-2313-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
On the accuracy of aerosol photoacoustic spectrometer calibrations using absorption by ozone
Nicholas W. Davies
College of Engineering, Mathematics and Physical Sciences, University
of Exeter, Exeter, EX4 4QF, UK
Observation Based Research, Met Office, Exeter, EX1 3PB, UK
Michael I. Cotterell
College of Engineering, Mathematics and Physical Sciences, University
of Exeter, Exeter, EX4 4QF, UK
Observation Based Research, Met Office, Exeter, EX1 3PB, UK
Cathryn Fox
Observation Based Research, Met Office, Exeter, EX1 3PB, UK
Kate Szpek
Observation Based Research, Met Office, Exeter, EX1 3PB, UK
Jim M. Haywood
College of Engineering, Mathematics and Physical Sciences, University
of Exeter, Exeter, EX4 4QF, UK
Earth System and Mitigation Science, Met Office Hadley Centre, Exeter,
EX1 3PB, UK
Justin M. Langridge
CORRESPONDING AUTHOR
Observation Based Research, Met Office, Exeter, EX1 3PB, UK
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- Optimizing the performance of aerosol photoacoustic cells using a finite element model. Part 1: Method validation and application to single-resonator multipass cells M. Cotterell et al. 10.1080/02786826.2019.1650161
- Refractive Index of Engine‐Emitted Black Carbon and the Influence of Organic Coatings on Optical Properties D. Hu et al. 10.1029/2023JD039178
- Effect of relative humidity, NOx, and ammonia on the physical properties of naphthalene secondary organic aerosols A. Klodt et al. 10.1039/D3EA00033H
- Photoacoustic studies of energy transfer from ozone photoproducts to bath gases following Chappuis band photoexcitation M. Cotterell et al. 10.1039/D0CP05056C
- Physical and chemical properties of black carbon and organic matter from different combustion and photochemical sources using aerodynamic aerosol classification D. Hu et al. 10.5194/acp-21-16161-2021
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- Vertical variability of the properties of highly aged biomass burning aerosol transported over the southeast Atlantic during CLARIFY-2017 H. Wu et al. 10.5194/acp-20-12697-2020
- Rapid transformation of ambient absorbing aerosols from West African biomass burning H. Wu et al. 10.5194/acp-21-9417-2021
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- Cantilever-enhanced photoacoustic measurement of light-absorbing aerosols J. Karhu et al. 10.1080/02786826.2021.1998338
- The CLoud–Aerosol–Radiation Interaction and Forcing: Year 2017 (CLARIFY-2017) measurement campaign J. Haywood et al. 10.5194/acp-21-1049-2021
- A single-pass RGB differential photoacoustic spectrometer (RGB-DPAS) for aerosol absorption measurement at 473, 532, and 671 nm Z. Yu et al. 10.1080/02786826.2018.1551611
- Observation of absorbing aerosols above clouds over the south-east Atlantic Ocean from the geostationary satellite SEVIRI – Part 1: Method description and sensitivity F. Peers et al. 10.5194/acp-19-9595-2019
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- Observation of absorbing aerosols above clouds over the south-east Atlantic Ocean from the geostationary satellite SEVIRI – Part 2: Comparison with MODIS and aircraft measurements from the CLARIFY-2017 field campaign F. Peers et al. 10.5194/acp-21-3235-2021
- The impact of bath gas composition on the calibration of photoacoustic spectrometers with ozone at discrete visible wavelengths spanning the Chappuis band M. Cotterell et al. 10.5194/amt-12-2371-2019
- Optical and Chemical Analysis of Absorption Enhancement by Mixed Carbonaceous Aerosols in the 2019 Woodbury, AZ, Fire Plume J. Lee et al. 10.1029/2020JD032399
- Optimizing the performance of aerosol photoacoustic cells using a finite element model. Part 2: Application to a two-resonator cell M. Cotterell et al. 10.1080/02786826.2019.1648749
- Intercomparison of airborne and surface-based measurements during the CLARIFY, ORACLES and LASIC field experiments P. Barrett et al. 10.5194/amt-15-6329-2022
- A novel approach to calibrating a photoacoustic absorption spectrometer using polydisperse absorbing aerosol K. Foster et al. 10.5194/amt-12-3351-2019
- Metrological traceability of black carbon measurement based on optical methods and its challenges in China: A review Y. Liu et al. 10.1016/j.atmosres.2023.106854
- Accurate Measurement of the Optical Properties of Single Aerosol Particles Using Cavity Ring-Down Spectroscopy M. Cotterell et al. 10.1021/acs.jpca.2c01246
- Characterization and demonstration of a black carbon aerosol mimic for instrument evaluation C. Zangmeister et al. 10.1080/02786826.2019.1660302
- Cloud adjustments dominate the overall negative aerosol radiative effects of biomass burning aerosols in UKESM1 climate model simulations over the south-eastern Atlantic H. Che et al. 10.5194/acp-21-17-2021
- Can ozone be used to calibrate aerosol photoacoustic spectrometers? D. Fischer & G. Smith 10.5194/amt-11-6419-2018
- A 2-year intercomparison of three methods for measuring black carbon concentration at a high-altitude research station in Europe S. Tinorua et al. 10.5194/amt-17-3897-2024
- A single-beam photothermal interferometer for in situ measurements of aerosol light absorption B. Visser et al. 10.5194/amt-13-7097-2020
- Advanced instrumental approaches for chemical characterization of indoor particulate matter R. Duarte et al. 10.1080/05704928.2021.2018596
- A dual-wavelength photothermal aerosol absorption monitor: design, calibration and performance L. Drinovec et al. 10.5194/amt-15-3805-2022
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- Review of portable near infrared spectrometers: Current status and new techniques C. Zhu et al. 10.1177/09670335211030617
- Absorption closure in highly aged biomass burning smoke J. Taylor et al. 10.5194/acp-20-11201-2020
- Aerosol physical characterization: A review on the current state of aerosol documentary standards and calibration strategies K. Vasilatou et al. 10.1016/j.jaerosci.2024.106483
- Investigating Carbonaceous Aerosol and Its Absorption Properties From Fires in the Western United States (WE‐CAN) and Southern Africa (ORACLES and CLARIFY) T. Carter et al. 10.1029/2021JD034984
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Latest update: 11 Dec 2024
Short summary
The poorly characterised optical properties of atmospheric aerosols are one of the major uncertainties when modelling future climate change. Photoacoustic spectroscopy is an accurate and sensitive method for measurement of aerosol light absorption. Photoacoustic spectrometers require calibration; hence this study validates the use of ozone as a calibrant and simultaneously verifies the accuracy of the photoacoustic spectrometers in question.
The poorly characterised optical properties of atmospheric aerosols are one of the major...