Articles | Volume 11, issue 10
https://doi.org/10.5194/amt-11-5767-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-11-5767-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Oct 2018
Research article |
| 19 Oct 2018
| 19 Oct 2018
Development and field testing of an online instrument for measuring the real-time oxidative potential of ambient particulate matter based on dithiothreitol assay
Joseph V. Puthussery
Department of Civil and Environmental Engineering, University of Illinois at
Urbana-Champaign, Urbana, 61801, USA
Chen Zhang
Department of Civil and Environmental Engineering, University of Illinois at
Urbana-Champaign, Urbana, 61801, USA
Vishal Verma
CORRESPONDING AUTHOR
Department of Civil and Environmental Engineering, University of Illinois at
Urbana-Champaign, Urbana, 61801, USA
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Cited
37 citations as recorded by crossref.
- Chemical characteristics and oxidative potential of indoor and outdoor PM2.5 in densely populated urban slums A. Anand et al. 10.1016/j.envres.2022.113562
- Particulate matter-induced oxidative stress – Mechanistic insights and antioxidant approaches reported in in vitro studies V. Vilas-Boas et al. 10.1016/j.etap.2024.104529
- Use of Dithiothreitol Assay to Evaluate the Oxidative Potential of Atmospheric Aerosols H. Jiang et al. 10.3390/atmos10100571
- Emerging applications of microfluidic techniques for in vitro toxicity studies of atmospheric particulate matter F. Liu et al. 10.1080/02786826.2021.1879373
- Indoor–Outdoor Oxidative Potential of PM2.5 in Wintertime Fairbanks, Alaska: Impact of Air Infiltration and Indoor Activities Y. Yang et al. 10.1021/acsestair.3c00067
- Review of in vitro studies evaluating respiratory toxicity of aerosols: impact of cell types, chemical composition, and atmospheric processing S. Salana & V. Verma 10.1039/D4EM00475B
- Oxidative potential of ambient PM2.5 from São Paulo, Brazil: Variations, associations with chemical components and source apportionment E. Serafeim et al. 10.1016/j.atmosenv.2023.119593
- Effects of operating conditions on PM oxidative potential assays M. Frezzini et al. 10.1016/j.atmosenv.2021.118802
- High-throughput, semi-automated dithiothreitol (DTT) assays for oxidative potential of fine particulate matter K. Berg et al. 10.1016/j.atmosenv.2019.117132
- A semi-automated instrument for cellular oxidative potential evaluation (SCOPE) of water-soluble extracts of ambient particulate matter S. Salana et al. 10.5194/amt-14-7579-2021
- Development and application of a mass closure PM<sub>2.5</sub> composition online monitoring system C. Su et al. 10.5194/amt-13-5407-2020
- Oxidative potential of solvent-extractable organic matter of ambient total suspended particulate in Bangkok, Thailand J. Wang et al. 10.1039/D1EM00414J
- Development, characterization, and application of an improved online reactive oxygen species analyzer based on the Monitor for AeRosols and Gases in ambient Air (MARGA) J. Wu et al. 10.5194/amt-15-2623-2022
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- Airborne Aerosols and Human Health: Leapfrogging from Mass Concentration to Oxidative Potential C. Molina et al. 10.3390/atmos11090917
- Light absorption and source apportionment of water soluble humic-like substances (HULIS) in PM2.5 at Nanjing, China M. Bao et al. 10.1016/j.envres.2021.112554
- Size-Resolved Redox Activity and Cytotoxicity of Water-Soluble Urban Atmospheric Particulate Matter: Assessing Contributions from Chemical Components A. Besis et al. 10.3390/toxics11010059
- Real-Time Measurements of PM2.5 Oxidative Potential Using a Dithiothreitol Assay in Delhi, India J. Puthussery et al. 10.1021/acs.estlett.0c00342
- The oxidative potential of particulate matter (PM) in different regions around the world and its relation to air pollution sources V. Farahani et al. 10.1039/D2EA00043A
- Toxicological Effects of Secondary Air Pollutants W. Xiang et al. 10.1007/s40242-023-3050-0
- Chemical and oxidative properties of fine particulate matter from near-road traffic sources N. Raparthi et al. 10.1016/j.envpol.2023.122514
- Diurnal profiles of particle-bound ROS of PM2.5 in urban environment of Hong Kong and their association with PM2.5, black carbon, ozone and PAHs S. Stevanovic et al. 10.1016/j.atmosenv.2019.117023
- A semi-automated multi-endpoint reactive oxygen species activity analyzer (SAMERA) for measuring the oxidative potential of ambient PM2.5aqueous extracts H. Yu et al. 10.1080/02786826.2019.1693492
- Remarkably High Oxidative Potential of Atmospheric PM2.5Coming from a Large-Scale Paddy-Residue Burning over the Northwestern Indo-Gangetic Plain A. Patel et al. 10.1021/acsearthspacechem.1c00125
- Major source categories of PM2.5 oxidative potential in wintertime Beijing and surroundings based on online dithiothreitol-based field measurements R. Cheung et al. 10.1016/j.scitotenv.2024.172345
- An instrument for the rapid quantification of PM-bound ROS: the Particle Into Nitroxide Quencher (PINQ) R. Brown et al. 10.5194/amt-12-2387-2019
- Development of a Physiologically Relevant Online Chemical Assay To Quantify Aerosol Oxidative Potential S. Campbell et al. 10.1021/acs.analchem.9b03282
- Effect of Biomass Burning, Diwali Fireworks, and Polluted Fog Events on the Oxidative Potential of Fine Ambient Particulate Matter in Delhi, India J. Puthussery et al. 10.1021/acs.est.2c02730
- Sources of acellular oxidative potential of water-soluble fine ambient particulate matter in the midwestern United States H. Yu et al. 10.1016/j.jhazmat.2024.134763
- Comparison of indoor and outdoor oxidative potential of PM2.5: pollution levels, temporal patterns, and key constituents F. Yang et al. 10.1016/j.envint.2021.106684
- High time resolution quantification of PM2.5 oxidative potential at a Central London Roadside Supersite S. Campbell et al. 10.1016/j.envint.2024.109102
- Key toxic components and sources affecting oxidative potential of atmospheric particulate matter using interpretable machine learning: Insights from fog episodes R. Li et al. 10.1016/j.jhazmat.2023.133175
- An Overview of the Automated and On-Line Systems to Assess the Oxidative Potential of Particulate Matter A. Carlino et al. 10.3390/atmos14020256
- Continuous measurement of reactive oxygen species inside and outside of a residential house during summer A. Eftekhari et al. 10.1111/ina.12789
- Particle lung deposited surface area (LDSAal) size distributions in different urban environments and geographical regions: Towards understanding of the PM2.5 dose–response T. Lepistö et al. 10.1016/j.envint.2023.108224
- Dynamic changes in the characteristics of fine particles and their oxidative potential in the city of Taj (Agra, India): the untold story of fireworks display I. Goyal et al. 10.1007/s11869-023-01402-4
- Spatiotemporal variability in the oxidative potential of ambient fine particulate matter in the Midwestern United States H. Yu et al. 10.5194/acp-21-16363-2021
37 citations as recorded by crossref.
- Chemical characteristics and oxidative potential of indoor and outdoor PM2.5 in densely populated urban slums A. Anand et al. 10.1016/j.envres.2022.113562
- Particulate matter-induced oxidative stress – Mechanistic insights and antioxidant approaches reported in in vitro studies V. Vilas-Boas et al. 10.1016/j.etap.2024.104529
- Use of Dithiothreitol Assay to Evaluate the Oxidative Potential of Atmospheric Aerosols H. Jiang et al. 10.3390/atmos10100571
- Emerging applications of microfluidic techniques for in vitro toxicity studies of atmospheric particulate matter F. Liu et al. 10.1080/02786826.2021.1879373
- Indoor–Outdoor Oxidative Potential of PM2.5 in Wintertime Fairbanks, Alaska: Impact of Air Infiltration and Indoor Activities Y. Yang et al. 10.1021/acsestair.3c00067
- Review of in vitro studies evaluating respiratory toxicity of aerosols: impact of cell types, chemical composition, and atmospheric processing S. Salana & V. Verma 10.1039/D4EM00475B
- Oxidative potential of ambient PM2.5 from São Paulo, Brazil: Variations, associations with chemical components and source apportionment E. Serafeim et al. 10.1016/j.atmosenv.2023.119593
- Effects of operating conditions on PM oxidative potential assays M. Frezzini et al. 10.1016/j.atmosenv.2021.118802
- High-throughput, semi-automated dithiothreitol (DTT) assays for oxidative potential of fine particulate matter K. Berg et al. 10.1016/j.atmosenv.2019.117132
- A semi-automated instrument for cellular oxidative potential evaluation (SCOPE) of water-soluble extracts of ambient particulate matter S. Salana et al. 10.5194/amt-14-7579-2021
- Development and application of a mass closure PM<sub>2.5</sub> composition online monitoring system C. Su et al. 10.5194/amt-13-5407-2020
- Oxidative potential of solvent-extractable organic matter of ambient total suspended particulate in Bangkok, Thailand J. Wang et al. 10.1039/D1EM00414J
- Development, characterization, and application of an improved online reactive oxygen species analyzer based on the Monitor for AeRosols and Gases in ambient Air (MARGA) J. Wu et al. 10.5194/amt-15-2623-2022
- The characteristics and size of lung-depositing particles vary significantly between high and low pollution traffic environments L. Salo et al. 10.1016/j.atmosenv.2021.118421
- Airborne Aerosols and Human Health: Leapfrogging from Mass Concentration to Oxidative Potential C. Molina et al. 10.3390/atmos11090917
- Light absorption and source apportionment of water soluble humic-like substances (HULIS) in PM2.5 at Nanjing, China M. Bao et al. 10.1016/j.envres.2021.112554
- Size-Resolved Redox Activity and Cytotoxicity of Water-Soluble Urban Atmospheric Particulate Matter: Assessing Contributions from Chemical Components A. Besis et al. 10.3390/toxics11010059
- Real-Time Measurements of PM2.5 Oxidative Potential Using a Dithiothreitol Assay in Delhi, India J. Puthussery et al. 10.1021/acs.estlett.0c00342
- The oxidative potential of particulate matter (PM) in different regions around the world and its relation to air pollution sources V. Farahani et al. 10.1039/D2EA00043A
- Toxicological Effects of Secondary Air Pollutants W. Xiang et al. 10.1007/s40242-023-3050-0
- Chemical and oxidative properties of fine particulate matter from near-road traffic sources N. Raparthi et al. 10.1016/j.envpol.2023.122514
- Diurnal profiles of particle-bound ROS of PM2.5 in urban environment of Hong Kong and their association with PM2.5, black carbon, ozone and PAHs S. Stevanovic et al. 10.1016/j.atmosenv.2019.117023
- A semi-automated multi-endpoint reactive oxygen species activity analyzer (SAMERA) for measuring the oxidative potential of ambient PM2.5aqueous extracts H. Yu et al. 10.1080/02786826.2019.1693492
- Remarkably High Oxidative Potential of Atmospheric PM2.5Coming from a Large-Scale Paddy-Residue Burning over the Northwestern Indo-Gangetic Plain A. Patel et al. 10.1021/acsearthspacechem.1c00125
- Major source categories of PM2.5 oxidative potential in wintertime Beijing and surroundings based on online dithiothreitol-based field measurements R. Cheung et al. 10.1016/j.scitotenv.2024.172345
- An instrument for the rapid quantification of PM-bound ROS: the Particle Into Nitroxide Quencher (PINQ) R. Brown et al. 10.5194/amt-12-2387-2019
- Development of a Physiologically Relevant Online Chemical Assay To Quantify Aerosol Oxidative Potential S. Campbell et al. 10.1021/acs.analchem.9b03282
- Effect of Biomass Burning, Diwali Fireworks, and Polluted Fog Events on the Oxidative Potential of Fine Ambient Particulate Matter in Delhi, India J. Puthussery et al. 10.1021/acs.est.2c02730
- Sources of acellular oxidative potential of water-soluble fine ambient particulate matter in the midwestern United States H. Yu et al. 10.1016/j.jhazmat.2024.134763
- Comparison of indoor and outdoor oxidative potential of PM2.5: pollution levels, temporal patterns, and key constituents F. Yang et al. 10.1016/j.envint.2021.106684
- High time resolution quantification of PM2.5 oxidative potential at a Central London Roadside Supersite S. Campbell et al. 10.1016/j.envint.2024.109102
- Key toxic components and sources affecting oxidative potential of atmospheric particulate matter using interpretable machine learning: Insights from fog episodes R. Li et al. 10.1016/j.jhazmat.2023.133175
- An Overview of the Automated and On-Line Systems to Assess the Oxidative Potential of Particulate Matter A. Carlino et al. 10.3390/atmos14020256
- Continuous measurement of reactive oxygen species inside and outside of a residential house during summer A. Eftekhari et al. 10.1111/ina.12789
- Particle lung deposited surface area (LDSAal) size distributions in different urban environments and geographical regions: Towards understanding of the PM2.5 dose–response T. Lepistö et al. 10.1016/j.envint.2023.108224
- Dynamic changes in the characteristics of fine particles and their oxidative potential in the city of Taj (Agra, India): the untold story of fireworks display I. Goyal et al. 10.1007/s11869-023-01402-4
- Spatiotemporal variability in the oxidative potential of ambient fine particulate matter in the Midwestern United States H. Yu et al. 10.5194/acp-21-16363-2021
Latest update: 03 Nov 2024
Short summary
The oxidative potential (OP) of ambient particulate matter (PM) has recently gained attention as an alternative metric for assessing the ambient PM toxicity. However, a major constraint in measuring the OP is its labor-intensive protocol. Here, we developed a new online instrument by coupling a mist chamber to an automated analytical system which can measure the real-time OP of ambient PM. We also report for the first time, the hourly averaged diurnal profile of ambient PM OP at an urban site.
The oxidative potential (OP) of ambient particulate matter (PM) has recently gained attention as...
