Articles | Volume 12, issue 3
https://doi.org/10.5194/amt-12-1619-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-12-1619-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Mar 2019
Research article |
| 12 Mar 2019
| 12 Mar 2019
Quantitative capabilities of STXM to measure spatially resolved organic volume fractions of mixed organic ∕ inorganic particles
Matthew Fraund
Department of Chemistry, University of the Pacific, Stockton, CA 95211, USA
Tim Park
Department of Chemistry, University of the Pacific, Stockton, CA 95211, USA
Lin Yao
Department of Chemistry, Beijing Normal University, Beijing, 100875,
China
Daniel Bonanno
Department of Chemistry, University of the Pacific, Stockton, CA 95211, USA
Don Q. Pham
Department of Chemistry, University of the Pacific, Stockton, CA 95211, USA
Department of Chemistry, University of the Pacific, Stockton, CA 95211, USA
current address: Sonoma Technology, Petaluma, CA 94954, USA
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Cited
22 citations as recorded by crossref.
- Recent advances in synchrotron-based spectroscopy for organic contaminant analysis G. Chandrakasan et al. https://doi.org/10.1016/j.trac.2025.118589
- Physicochemical and Molecular Insights into the Boundary Layer and Free Troposphere Aerosol Interactions over the Southern Great Plains X. Mansoura et al. https://doi.org/10.1021/acs.est.5c10903
- Impact of dry intrusion events on the composition and mixing state of particles during the winter Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA) J. Tomlin et al. https://doi.org/10.5194/acp-21-18123-2021
- Stratospheric aerosol perturbation by tropospheric biomass burning and deep convection X. Shen et al. https://doi.org/10.1038/s41561-025-01821-1
- A review of atmospheric individual particle analyses: Methodologies and applications in environmental research L. Shao et al. https://doi.org/10.1016/j.gr.2022.01.007
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. https://doi.org/10.5194/acp-23-8659-2023
- Ptychography at the carbon K-edge N. Mille et al. https://doi.org/10.1038/s43246-022-00232-8
- Chemical imaging of individual stratospheric particles sampled over North America S. Sharpe et al. https://doi.org/10.1039/D5EA00127G
- Chemical Imaging of Atmospheric Biomass Burning Particles from North American Wildfires F. Rivera-Adorno et al. https://doi.org/10.1021/acsestair.4c00242
- An automated size and time-resolved aerosol collector platform integrated with environmental sensors to study the vertical profile of aerosols Z. Cheng et al. https://doi.org/10.1039/D2EA00097K
- Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation N. Lata et al. https://doi.org/10.1021/acsearthspacechem.1c00315
- Chemical characterization of microplastic particles formed in airborne waste discharged from sewer pipe repairs B. Peterson et al. https://doi.org/10.1039/D3EM00193H
- Chemical Composition and Mixing State of Wintertime Aerosol from the European Arctic Site of Ny-Ålesund, Svalbard Z. Lai et al. https://doi.org/10.1021/acsearthspacechem.5c00175
- Optical properties and composition of viscous organic particles found in the Southern Great Plains M. Fraund et al. https://doi.org/10.5194/acp-20-11593-2020
- Chemical Insights into the Molecular Composition of Organic Aerosols in the Urban Region of Houston, Texas T. Gautam et al. https://doi.org/10.1021/acsestair.4c00141
- Multi-modal chemical characterization of highly viscous submicrometer organic particles A. Morales et al. https://doi.org/10.1080/02786826.2023.2266494
- Atmospheric micro- and nano- particles: characteristics, sources, and environmental behavior L. Shao et al. https://doi.org/10.1360/CSB-2025-0728
- Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic D. Knopf et al. https://doi.org/10.5194/acp-22-5377-2022
- On the use of soft X-ray STXM for organic-inorganic halide perovskite photovoltaic materials H. Jun et al. https://doi.org/10.1016/j.elspec.2023.147358
- Measurement report: Role of organic coating and chemical composition on ice nucleation potential of atmospheric particles in European Arctic N. Lata et al. https://doi.org/10.5194/acp-26-6611-2026
- Particle phase-state variability in the North Atlantic free troposphere during summertime is determined by atmospheric transport patterns and sources Z. Cheng et al. https://doi.org/10.5194/acp-22-9033-2022
- Chemical composition and morphological analysis of atmospheric particles from an intensive bonfire burning festival J. Tomlin et al. https://doi.org/10.1039/D2EA00037G
22 citations as recorded by crossref.
- Recent advances in synchrotron-based spectroscopy for organic contaminant analysis G. Chandrakasan et al. https://doi.org/10.1016/j.trac.2025.118589
- Physicochemical and Molecular Insights into the Boundary Layer and Free Troposphere Aerosol Interactions over the Southern Great Plains X. Mansoura et al. https://doi.org/10.1021/acs.est.5c10903
- Impact of dry intrusion events on the composition and mixing state of particles during the winter Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA) J. Tomlin et al. https://doi.org/10.5194/acp-21-18123-2021
- Stratospheric aerosol perturbation by tropospheric biomass burning and deep convection X. Shen et al. https://doi.org/10.1038/s41561-025-01821-1
- A review of atmospheric individual particle analyses: Methodologies and applications in environmental research L. Shao et al. https://doi.org/10.1016/j.gr.2022.01.007
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. https://doi.org/10.5194/acp-23-8659-2023
- Ptychography at the carbon K-edge N. Mille et al. https://doi.org/10.1038/s43246-022-00232-8
- Chemical imaging of individual stratospheric particles sampled over North America S. Sharpe et al. https://doi.org/10.1039/D5EA00127G
- Chemical Imaging of Atmospheric Biomass Burning Particles from North American Wildfires F. Rivera-Adorno et al. https://doi.org/10.1021/acsestair.4c00242
- An automated size and time-resolved aerosol collector platform integrated with environmental sensors to study the vertical profile of aerosols Z. Cheng et al. https://doi.org/10.1039/D2EA00097K
- Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation N. Lata et al. https://doi.org/10.1021/acsearthspacechem.1c00315
- Chemical characterization of microplastic particles formed in airborne waste discharged from sewer pipe repairs B. Peterson et al. https://doi.org/10.1039/D3EM00193H
- Chemical Composition and Mixing State of Wintertime Aerosol from the European Arctic Site of Ny-Ålesund, Svalbard Z. Lai et al. https://doi.org/10.1021/acsearthspacechem.5c00175
- Optical properties and composition of viscous organic particles found in the Southern Great Plains M. Fraund et al. https://doi.org/10.5194/acp-20-11593-2020
- Chemical Insights into the Molecular Composition of Organic Aerosols in the Urban Region of Houston, Texas T. Gautam et al. https://doi.org/10.1021/acsestair.4c00141
- Multi-modal chemical characterization of highly viscous submicrometer organic particles A. Morales et al. https://doi.org/10.1080/02786826.2023.2266494
- Atmospheric micro- and nano- particles: characteristics, sources, and environmental behavior L. Shao et al. https://doi.org/10.1360/CSB-2025-0728
- Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic D. Knopf et al. https://doi.org/10.5194/acp-22-5377-2022
- On the use of soft X-ray STXM for organic-inorganic halide perovskite photovoltaic materials H. Jun et al. https://doi.org/10.1016/j.elspec.2023.147358
- Measurement report: Role of organic coating and chemical composition on ice nucleation potential of atmospheric particles in European Arctic N. Lata et al. https://doi.org/10.5194/acp-26-6611-2026
- Particle phase-state variability in the North Atlantic free troposphere during summertime is determined by atmospheric transport patterns and sources Z. Cheng et al. https://doi.org/10.5194/acp-22-9033-2022
- Chemical composition and morphological analysis of atmospheric particles from an intensive bonfire burning festival J. Tomlin et al. https://doi.org/10.1039/D2EA00037G
Saved (final revised paper)
Latest update: 08 Jul 2026
Short summary
Scanning transmission X-ray microscopy (STXM) is a powerful tool which is able to determine the elemental and functional composition of aerosols on a subparticle level. The current work validates the use of STXM for quantitatively calculating the organic volume fraction of individual aerosols by applying the calculation to lab-prepared samples. The caveats and limitations for this calculation are shown as well.
Scanning transmission X-ray microscopy (STXM) is a powerful tool which is able to determine the...
