Research article
11 Sep 2019
Research article
| 11 Sep 2019
An extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF) for online measurement of atmospheric aerosol particles
Felipe D. Lopez-Hilfiker et al.
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Cited
44 citations as recorded by crossref.
- A 1-year characterization of organic aerosol composition and sources using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF) L. Qi et al. 10.5194/acp-20-7875-2020
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- Chemical composition and sources of organic aerosol on the Adriatic coast in Croatia R. Casotto et al. 10.1016/j.aeaoa.2022.100159
- Experimental Study of OH-Initiated Heterogeneous Oxidation of Organophosphate Flame Retardants: Kinetics, Mechanism, and Toxicity Q. Liu et al. 10.1021/acs.est.9b05327
- On the fate of oxygenated organic molecules in atmospheric aerosol particles V. Pospisilova et al. 10.1126/sciadv.aax8922
- Analytical methods for organosulfate detection in aerosol particles: Current status and future perspectives K. Gao & T. Zhu 10.1016/j.scitotenv.2021.147244
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- Real-Time Detection of Aerosol Metals Using Online Extractive Electrospray Ionization Mass Spectrometry S. Giannoukos et al. 10.1021/acs.analchem.9b04480
- The fuel of atmospheric chemistry: Toward a complete description of reactive organic carbon C. Heald & J. Kroll 10.1126/sciadv.aay8967
- A review of microbial and chemical assessment of indoor surfaces V. Mihucz et al. 10.1080/05704928.2021.1995870
- Overestimation of Monoterpene Organosulfate Abundance in Aerosol Particles by Sampling in the Presence of SO2 M. Brüggemann et al. 10.1021/acs.estlett.0c00814
- HELIOS/SICRIT/mass spectrometry for analysis of aerosols in engine exhaust K. Thaler et al. 10.1080/02786826.2021.1909699
- Quantification of solid fuel combustion and aqueous chemistry contributions to secondary organic aerosol during wintertime haze events in Beijing Y. Tong et al. 10.5194/acp-21-9859-2021
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Online Aerosol Chemical Characterization by Extractive Electrospray Ionization–Ultrahigh-Resolution Mass Spectrometry (EESI-Orbitrap) C. Lee et al. 10.1021/acs.est.9b07090
- Real‐time organic aerosol chemical speciation in the indoor environment using extractive electrospray ionization mass spectrometry W. Brown et al. 10.1111/ina.12721
- Online Characterization of Organic Aerosol by Condensational Growth into Aqueous Droplets Coupled with Droplet-Assisted Ionization D. Kerecman et al. 10.1021/acs.analchem.0c03697
- Constraining the response factors of an extractive electrospray ionization mass spectrometer for near-molecular aerosol speciation D. Wang et al. 10.5194/amt-14-6955-2021
- Detection of trace metals in biogas using extractive electrospray ionization high-resolution mass spectrometry S. Giannoukos et al. 10.1016/j.renene.2021.01.047
- Large Emissions of Low-Volatility Siloxanes during Residential Oven Use E. Katz et al. 10.1021/acs.estlett.1c00433
- Uncovering global-scale risks from commercial chemicals in air Q. Liu et al. 10.1038/s41586-021-04134-6
- Large contribution to secondary organic aerosol from isoprene cloud chemistry H. Lamkaddam et al. 10.1126/sciadv.abe2952
- Evolution of Sea Spray Aerosol Particle Phase State Across a Phytoplankton Bloom P. Tumminello et al. 10.1021/acsearthspacechem.1c00186
- Resolving Ambient Organic Aerosol Formation and Aging Pathways with Simultaneous Molecular Composition and Volatility Observations B. Lee et al. 10.1021/acsearthspacechem.9b00302
- Effects of aerosol size and coating thickness on the molecular detection using extractive electrospray ionization C. Lee et al. 10.5194/amt-14-5913-2021
- Estimating mean molecular weight, carbon number, and OM∕OC with mid-infrared spectroscopy in organic particulate matter samples from a monitoring network A. Yazdani et al. 10.5194/amt-14-4805-2021
- Organic aerosol source apportionment in Zurich using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF-MS) – Part 1: Biogenic influences and day–night chemistry in summer G. Stefenelli et al. 10.5194/acp-19-14825-2019
- Composition of Ultrafine Particles in Urban Beijing: Measurement Using a Thermal Desorption Chemical Ionization Mass Spectrometer X. Li et al. 10.1021/acs.est.0c06053
- Measurement of atmospheric nanoparticles: Bridging the gap between gas-phase molecules and larger particles C. Peng et al. 10.1016/j.jes.2022.03.006
- The Sea Spray Chemistry and Particle Evolution study (SeaSCAPE): overview and experimental methods J. Sauer et al. 10.1039/D1EM00260K
- Photolytically induced changes in composition and volatility of biogenic secondary organic aerosol from nitrate radical oxidation during night-to-day transition C. Wu et al. 10.5194/acp-21-14907-2021
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- Mass spectrometry coupled with vacuum thermal desorption for enhanced volatile organic sample analysis Q. Yu et al. 10.1039/D0AY00175A
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al. 10.1021/acsearthspacechem.0c00346
- Comparison of five methodologies to apportion organic aerosol sources during a PM pollution event D. Srivastava et al. 10.1016/j.scitotenv.2020.143168
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- Photodegradation of α-Pinene Secondary Organic Aerosol Dominated by Moderately Oxidized Molecules V. Pospisilova et al. 10.1021/acs.est.0c06752
- Organosulfates in Ambient Aerosol: State of Knowledge and Future Research Directions on Formation, Abundance, Fate, and Importance M. Brüggemann et al. 10.1021/acs.est.9b06751
- Molecular characterization of ultrafine particles using extractive electrospray time-of-flight mass spectrometry M. Surdu et al. 10.1039/D1EA00050K
- Direct measurements of semi-volatile organic compound dynamics show near-unity mass accommodation coefficients for diverse aerosols X. Liu et al. 10.1038/s42004-019-0200-x
- Bulk Organic Aerosol Analysis by Proton-Transfer-Reaction Mass Spectrometry: An Improved Methodology for the Determination of Total Organic Mass, O:C and H:C Elemental Ratios, and the Average Molecular Formula J. Leglise et al. 10.1021/acs.analchem.9b02949
- Organic aerosol source apportionment in Zurich using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF-MS) – Part 2: Biomass burning influences in winter L. Qi et al. 10.5194/acp-19-8037-2019
- Aging Effects on Biomass Burning Aerosol Mass and Composition: A Critical Review of Field and Laboratory Studies A. Hodshire et al. 10.1021/acs.est.9b02588
40 citations as recorded by crossref.
- A 1-year characterization of organic aerosol composition and sources using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF) L. Qi et al. 10.5194/acp-20-7875-2020
- Evaluating Organic Aerosol Sources and Evolution with a Combined Molecular Composition and Volatility Framework Using the Filter Inlet for Gases and Aerosols (FIGAERO) J. Thornton et al. 10.1021/acs.accounts.0c00259
- Characterization of secondary organic aerosol from heated-cooking-oil emissions: evolution in composition and volatility M. Takhar et al. 10.5194/acp-21-5137-2021
- Chemical composition and sources of organic aerosol on the Adriatic coast in Croatia R. Casotto et al. 10.1016/j.aeaoa.2022.100159
- Experimental Study of OH-Initiated Heterogeneous Oxidation of Organophosphate Flame Retardants: Kinetics, Mechanism, and Toxicity Q. Liu et al. 10.1021/acs.est.9b05327
- On the fate of oxygenated organic molecules in atmospheric aerosol particles V. Pospisilova et al. 10.1126/sciadv.aax8922
- Analytical methods for organosulfate detection in aerosol particles: Current status and future perspectives K. Gao & T. Zhu 10.1016/j.scitotenv.2021.147244
- Airborne extractive electrospray mass spectrometry measurements of the chemical composition of organic aerosol D. Pagonis et al. 10.5194/amt-14-1545-2021
- Real-Time Detection of Aerosol Metals Using Online Extractive Electrospray Ionization Mass Spectrometry S. Giannoukos et al. 10.1021/acs.analchem.9b04480
- The fuel of atmospheric chemistry: Toward a complete description of reactive organic carbon C. Heald & J. Kroll 10.1126/sciadv.aay8967
- A review of microbial and chemical assessment of indoor surfaces V. Mihucz et al. 10.1080/05704928.2021.1995870
- Overestimation of Monoterpene Organosulfate Abundance in Aerosol Particles by Sampling in the Presence of SO2 M. Brüggemann et al. 10.1021/acs.estlett.0c00814
- HELIOS/SICRIT/mass spectrometry for analysis of aerosols in engine exhaust K. Thaler et al. 10.1080/02786826.2021.1909699
- Quantification of solid fuel combustion and aqueous chemistry contributions to secondary organic aerosol during wintertime haze events in Beijing Y. Tong et al. 10.5194/acp-21-9859-2021
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Online Aerosol Chemical Characterization by Extractive Electrospray Ionization–Ultrahigh-Resolution Mass Spectrometry (EESI-Orbitrap) C. Lee et al. 10.1021/acs.est.9b07090
- Real‐time organic aerosol chemical speciation in the indoor environment using extractive electrospray ionization mass spectrometry W. Brown et al. 10.1111/ina.12721
- Online Characterization of Organic Aerosol by Condensational Growth into Aqueous Droplets Coupled with Droplet-Assisted Ionization D. Kerecman et al. 10.1021/acs.analchem.0c03697
- Constraining the response factors of an extractive electrospray ionization mass spectrometer for near-molecular aerosol speciation D. Wang et al. 10.5194/amt-14-6955-2021
- Detection of trace metals in biogas using extractive electrospray ionization high-resolution mass spectrometry S. Giannoukos et al. 10.1016/j.renene.2021.01.047
- Large Emissions of Low-Volatility Siloxanes during Residential Oven Use E. Katz et al. 10.1021/acs.estlett.1c00433
- Uncovering global-scale risks from commercial chemicals in air Q. Liu et al. 10.1038/s41586-021-04134-6
- Large contribution to secondary organic aerosol from isoprene cloud chemistry H. Lamkaddam et al. 10.1126/sciadv.abe2952
- Evolution of Sea Spray Aerosol Particle Phase State Across a Phytoplankton Bloom P. Tumminello et al. 10.1021/acsearthspacechem.1c00186
- Resolving Ambient Organic Aerosol Formation and Aging Pathways with Simultaneous Molecular Composition and Volatility Observations B. Lee et al. 10.1021/acsearthspacechem.9b00302
- Effects of aerosol size and coating thickness on the molecular detection using extractive electrospray ionization C. Lee et al. 10.5194/amt-14-5913-2021
- Estimating mean molecular weight, carbon number, and OM∕OC with mid-infrared spectroscopy in organic particulate matter samples from a monitoring network A. Yazdani et al. 10.5194/amt-14-4805-2021
- Organic aerosol source apportionment in Zurich using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF-MS) – Part 1: Biogenic influences and day–night chemistry in summer G. Stefenelli et al. 10.5194/acp-19-14825-2019
- Composition of Ultrafine Particles in Urban Beijing: Measurement Using a Thermal Desorption Chemical Ionization Mass Spectrometer X. Li et al. 10.1021/acs.est.0c06053
- Measurement of atmospheric nanoparticles: Bridging the gap between gas-phase molecules and larger particles C. Peng et al. 10.1016/j.jes.2022.03.006
- The Sea Spray Chemistry and Particle Evolution study (SeaSCAPE): overview and experimental methods J. Sauer et al. 10.1039/D1EM00260K
- Photolytically induced changes in composition and volatility of biogenic secondary organic aerosol from nitrate radical oxidation during night-to-day transition C. Wu et al. 10.5194/acp-21-14907-2021
- Characteristics of wintertime VOCs in urban Beijing: Composition and source apportionment L. Wang et al. 10.1016/j.aeaoa.2020.100100
- Mass spectrometry coupled with vacuum thermal desorption for enhanced volatile organic sample analysis Q. Yu et al. 10.1039/D0AY00175A
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al. 10.1021/acsearthspacechem.0c00346
- Comparison of five methodologies to apportion organic aerosol sources during a PM pollution event D. Srivastava et al. 10.1016/j.scitotenv.2020.143168
- Atmospheric OH Oxidation Chemistry of Particulate Liquid Crystal Monomers: An Emerging Persistent Organic Pollutant in Air Q. Liu et al. 10.1021/acs.estlett.0c00447
- Photodegradation of α-Pinene Secondary Organic Aerosol Dominated by Moderately Oxidized Molecules V. Pospisilova et al. 10.1021/acs.est.0c06752
- Organosulfates in Ambient Aerosol: State of Knowledge and Future Research Directions on Formation, Abundance, Fate, and Importance M. Brüggemann et al. 10.1021/acs.est.9b06751
- Molecular characterization of ultrafine particles using extractive electrospray time-of-flight mass spectrometry M. Surdu et al. 10.1039/D1EA00050K
4 citations as recorded by crossref.
- Direct measurements of semi-volatile organic compound dynamics show near-unity mass accommodation coefficients for diverse aerosols X. Liu et al. 10.1038/s42004-019-0200-x
- Bulk Organic Aerosol Analysis by Proton-Transfer-Reaction Mass Spectrometry: An Improved Methodology for the Determination of Total Organic Mass, O:C and H:C Elemental Ratios, and the Average Molecular Formula J. Leglise et al. 10.1021/acs.analchem.9b02949
- Organic aerosol source apportionment in Zurich using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF-MS) – Part 2: Biomass burning influences in winter L. Qi et al. 10.5194/acp-19-8037-2019
- Aging Effects on Biomass Burning Aerosol Mass and Composition: A Critical Review of Field and Laboratory Studies A. Hodshire et al. 10.1021/acs.est.9b02588
Latest update: 29 Jan 2023
Short summary
We present a novel, field-deployable extractive electrospray time-of-flight mass spectrometer (EESI-TOF), which provides real-time, near-molecular measurements of organic aerosol at atmospherically relevant concentrations, addressing a critical gap in existing measurement capabilities. Successful deployments of the EESI-TOF for laboratory measurements, ground-based ambient sampling, and aboard a research aircraft highlight the versatility and potential of the EESI-TOF system.
We present a novel, field-deployable extractive electrospray time-of-flight mass spectrometer...