Articles | Volume 17, issue 14
https://doi.org/10.5194/amt-17-4507-2024
© Author(s) 2024. This work is distributed under the Creative Commons Attribution 4.0 License.
A novel, balloon-borne UV–Vis spectrometer for direct sun measurements of stratospheric bromine
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- Final revised paper (published on 29 Jul 2024)
- Preprint (discussion started on 04 Jan 2024)
Interactive discussion
Status: closed
Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor
| : Report abuse
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RC1: 'Comment on egusphere-2023-2912', Anonymous Referee #1, 08 Feb 2024
- AC1: 'Reply on RC1', Karolin Voss, 16 May 2024
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RC2: 'Comment on egusphere-2023-2912', Anonymous Referee #2, 10 Apr 2024
- AC2: 'Reply on RC2', Karolin Voss, 16 May 2024
Peer review completion
AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Karolin Voss on behalf of the Authors (16 May 2024)
Author's response
Author's tracked changes
Manuscript
ED: Referee Nomination & Report Request started (17 May 2024) by Saulius Nevas
RR by Anonymous Referee #1 (17 May 2024)
RR by Anonymous Referee #2 (30 May 2024)
ED: Publish as is (04 Jun 2024) by Saulius Nevas
AR by Karolin Voss on behalf of the Authors (06 Jun 2024)
This is a well-written paper that presents the design and first results from a new balloon spectrometer for solar occultation measurements of BrO. The instrumentation is described in detail and the co-authors present improvements to the standard retrieval approach together with a convincing handling of instrumental artifacts. The inferred bromine load and its derived uncertainty shows the usefulness of these measurements for monitoring stratospheric bromine trends. The paper is a good fit for AMT and should be published after addressing these minor revisions:
The case that the 1-2 ppt difference quoted here is actually of scientific significance should be made. On the surface it seems small in light of the total budget of 20 ppt.
The system level descriptions of the solar tracker and the spectrometer units are well done, but would be greatly helped with schematic level drawings of the designs (in addition to the picture, which is a bit hard to follow for one not familiar with the instrument).
How big is the non-linearity correction in the processing step, even when the detector saturation is kept to 30-60%?
Something is missing the explanation of how the dependence of etalon optical density on SCD is used for the retrieval process. How is the extrapolation to the larger SCDs performed throughout the retrieval range beyond the high sun range used for the characterization of the dependence?
The significant difference in [BrO] for different polynomial degrees is somewhat concerning. Is there some level of non-orthogonality between the higher degree polynomials and the BrO cross section? If the residuals are the same, would it not make sense to take the result for the lowest degree polynomial as the most robust?
How will new CCD detectors avoid the contamination problem? It seems the cause is not well understood by the co-authors, so might it not happen again? Maybe it is from internal reflection in the focal plan array itself (this is a known phenomenon)?
Prolific use of brackets for parenthetical phrases and around quantities make the text a bit difficult to read. Check with the editor for guidance on correct typesetting.
Line 78: “correct for them”
Line 88: rephrase “all electronics threatened to overheat”
Line 155: rephrase “were more threatened”