Articles | Volume 18, issue 12
https://doi.org/10.5194/amt-18-2659-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-18-2659-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Assimilation of volcanic sulfur dioxide products from IASI and TROPOMI into the chemical transport model MOCAGE: case study of the 2021 La Soufrière Saint Vincent eruption with the March 2022 version of MOCAGE
CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France
Jonathan Améric
CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France
Vincent Guidard
CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France
Related authors
Herizo Narivelo, Paul David Hamer, Virginie Marécal, Luke Surl, Tjarda Roberts, Sophie Pelletier, Béatrice Josse, Jonathan Guth, Mickaël Bacles, Simon Warnach, Thomas Wagner, Stefano Corradini, Giuseppe Salerno, and Lorenzo Guerrieri
Atmos. Chem. Phys., 23, 10533–10561, https://doi.org/10.5194/acp-23-10533-2023, https://doi.org/10.5194/acp-23-10533-2023, 2023
Short summary
Short summary
Volcanic emissions emit large quantities of gases and primary aerosols that can play an important role in atmospheric chemistry. We present a study of the fate of volcanic bromine emissions from the eruption of Mount Etna around Christmas 2018. Using a numerical model and satellite observations, we analyse the impact of the volcanic plume and how it modifies the composition of the air over the whole Mediterranean basin, in particular on tropospheric ozone through the bromine-explosion cycle.
Augustin Colette, Gaëlle Collin, François Besson, Etienne Blot, Vincent Guidard, Frédérik Meleux, Adrien Royer, Valentin Petiot, Claire Miller, Oihana Fermond, Alizé Jeant, Mario Adani, Joaquim Arteta, Anna Benedictow, Robert Bergström, Dene Bowdalo, Jorgen Brandt, Gino Briganti, Ana C. Carvalho, Jesper Heile Christensen, Florian Couvidat, Ilaria D'Elia, Massimo D'Isidoro, Hugo Denier van der Gon, Gaël Descombes, Enza Di Tomaso, John Douros, Jeronimo Escribano, Henk Eskes, Hilde Fagerli, Yalda Fatahi, Johannes Flemming, Elmar Friese, Lise Frohn, Michael Gauss, Camilla Geels, Guido Guarnieri, Marc Guevara, Antoine Guion, Jonathan Guth, Risto Hänninen, Kaj Hansen, Ulas Im, Ruud Janssen, Marine Jeoffrion, Mathieu Joly, Luke Jones, Oriol Jorba, Evgeni Kadantsev, Michael Kahnert, Jacek W. Kaminski, Rostislav Kouznetsov, Richard Kranenburg, Jeroen Kuenen, Anne Caroline Lange, Joachim Langner, Victor Lannuque, Francesca Macchia, Astrid Manders, Mihaela Mircea, Agnes Nyiri, Miriam Olid, Carlos Pérez García-Pando, Yuliia Palamarchuk, Antonio Piersanti, Blandine Raux, Miha Razinger, Lennard Robertson, Arjo Segers, Martijn Schaap, Pilvi Siljamo, David Simpson, Mikhail Sofiev, Anders Stangel, Joanna Struzewska, Carles Tena, Renske Timmermans, Thanos Tsikerdekis, Svetlana Tsyro, Svyatoslav Tyuryakov, Anthony Ung, Andreas Uppstu, Alvaro Valdebenito, Peter van Velthoven, Lina Vitali, Zhuyun Ye, Vincent-Henri Peuch, and Laurence Rouïl
Geosci. Model Dev., 18, 6835–6883, https://doi.org/10.5194/gmd-18-6835-2025, https://doi.org/10.5194/gmd-18-6835-2025, 2025
Short summary
Short summary
The Copernicus Atmosphere Monitoring Service – Regional Production delivers daily forecasts, analyses, and reanalyses of air quality in Europe. The service relies on a distributed modelling production by 11 leading European modelling teams following stringent requirements with an operational design that has no equivalent in the world. All the products are free, open, and quality-assured and disseminated with a high level of reliability.
Francesca Vittorioso, Vincent Guidard, and Nadia Fourrié
Atmos. Meas. Tech., 17, 5279–5299, https://doi.org/10.5194/amt-17-5279-2024, https://doi.org/10.5194/amt-17-5279-2024, 2024
Short summary
Short summary
The future Meteosat Third Generation Infrared Sounder (MTG-IRS) will represent a major innovation for the monitoring of the chemical state of the atmosphere. MTG-IRS will have the advantage of being based on a geostationary platform and acquiring data with a high temporal frequency. This work aims to evaluate its potential impact over Europe within a chemical transport model (MOCAGE). The results indicate that the assimilation of these data always has a positive impact on ozone analysis.
Safae Oumami, Joaquim Arteta, Vincent Guidard, Pierre Tulet, and Paul David Hamer
Geosci. Model Dev., 17, 3385–3408, https://doi.org/10.5194/gmd-17-3385-2024, https://doi.org/10.5194/gmd-17-3385-2024, 2024
Short summary
Short summary
In this paper, we coupled the SURFEX and MEGAN models. The aim of this coupling is to improve the estimation of biogenic fluxes by using the SURFEX canopy environment model. The coupled model results were validated and several sensitivity tests were performed. The coupled-model total annual isoprene flux is 442 Tg; this value is within the range of other isoprene estimates reported. The ultimate aim of this coupling is to predict the impact of climate change on biogenic emissions.
Herizo Narivelo, Paul David Hamer, Virginie Marécal, Luke Surl, Tjarda Roberts, Sophie Pelletier, Béatrice Josse, Jonathan Guth, Mickaël Bacles, Simon Warnach, Thomas Wagner, Stefano Corradini, Giuseppe Salerno, and Lorenzo Guerrieri
Atmos. Chem. Phys., 23, 10533–10561, https://doi.org/10.5194/acp-23-10533-2023, https://doi.org/10.5194/acp-23-10533-2023, 2023
Short summary
Short summary
Volcanic emissions emit large quantities of gases and primary aerosols that can play an important role in atmospheric chemistry. We present a study of the fate of volcanic bromine emissions from the eruption of Mount Etna around Christmas 2018. Using a numerical model and satellite observations, we analyse the impact of the volcanic plume and how it modifies the composition of the air over the whole Mediterranean basin, in particular on tropospheric ozone through the bromine-explosion cycle.
Antoine Perrot, Olivier Pannekoucke, and Vincent Guidard
Nonlin. Processes Geophys., 30, 139–166, https://doi.org/10.5194/npg-30-139-2023, https://doi.org/10.5194/npg-30-139-2023, 2023
Short summary
Short summary
This work is a theoretical contribution that provides equations for understanding uncertainty prediction applied in air quality where multiple chemical species can interact. A simplified minimal test bed is introduced that shows the ability of our equations to reproduce the statistics estimated from an ensemble of forecasts. While the latter estimation is the state of the art, solving equations is numerically less costly, depending on the number of chemical species, and motivates this research.
Mohammad El Aabaribaoune, Emanuele Emili, and Vincent Guidard
Atmos. Meas. Tech., 14, 2841–2856, https://doi.org/10.5194/amt-14-2841-2021, https://doi.org/10.5194/amt-14-2841-2021, 2021
Short summary
Short summary
This work aims to use correlated IASI errors in the ozone band within a chemical transport model assimilation. The validation of the results against ozone observations from ozonesondes, MLS, and OMI instruments has shown an improvement of the ozone distribution. The computational time was also highly reduced. The surface sea temperature was also improved. The work aims to improve the quality of the ozone prediction, which is important for air quality, climate, and meteorological applications.
Cited articles
Bennis, K. and Venzke, E.: Report on Soufriere St. Vincent (Saint Vincent and the Grenadines), Bulletin of the Global Volcanism Network, 46, https://doi.org/10.5479/si.GVP.BGVN202105-360150, 2021. a
Boichu, M., Menut, L., Khvorostyanov, D., Clarisse, L., Clerbaux, C., Turquety, S., and Coheur, P.-F.: Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case study, Atmos. Chem. Phys., 13, 8569–8584, https://doi.org/10.5194/acp-13-8569-2013, 2013. a
Bouyssel, F., Berre, L., Bénichou, H., Chambon, P., Girardot, N., Guidard, V., Loo, C., Mahfouf, J.-F., Moll, P., Payan, C., and Raspaud, D.: The 2020 Global Operational NWP Data Assimilation System at Météo-France, Springer International Publishing, 4, 645–664, https://doi.org/10.1007/978-3-030-77722-7_25, 2022. a
Brenot, H., Theys, N., Clarisse, L., van Geffen, J., van Gent, J., Van Roozendael, M., van der A, R., Hurtmans, D., Coheur, P.-F., Clerbaux, C., Valks, P., Hedelt, P., Prata, F., Rasson, O., Sievers, K., and Zehner, C.: Support to Aviation Control Service (SACS): an online service for near-real-time satellite monitoring of volcanic plumes, Nat. Hazards Earth Syst. Sci., 14, 1099–1123, https://doi.org/10.5194/nhess-14-1099-2014, 2014. a
Brenot, H., Theys, N., Clarisse, L., van Gent, J., Hurtmans, D. R., Vandenbussche, S., Papagiannopoulos, N., Mona, L., Virtanen, T., Uppstu, A., Sofiev, M., Bugliaro, L., Vázquez-Navarro, M., Hedelt, P., Parks, M. M., Barsotti, S., Coltelli, M., Moreland, W., Scollo, S., Salerno, G., Arnold-Arias, D., Hirtl, M., Peltonen, T., Lahtinen, J., Sievers, K., Lipok, F., Rüfenacht, R., Haefele, A., Hervo, M., Wagenaar, S., Som de Cerff, W., de Laat, J., Apituley, A., Stammes, P., Laffineur, Q., Delcloo, A., Lennart, R., Rokitansky, C.-H., Vargas, A., Kerschbaum, M., Resch, C., Zopp, R., Plu, M., Peuch, V.-H., Van Roozendael, M., and Wotawa, G.: EUNADICS-AV early warning system dedicated to supporting aviation in the case of a crisis from natural airborne hazards and radionuclide clouds, Nat. Hazards Earth Syst. Sci., 21, 3367–3405, https://doi.org/10.5194/nhess-21-3367-2021, 2021. a
Carn, S. A., Krueger, A. J., Krotkov, N. A., Yang, K., and Evans, K.: Tracking volcanic sulfur dioxide clouds for aviation hazard mitigation, Nat. Hazards, 51, 325–343, https://doi.org/10.1007/s11069-008-9228-4, 2009. a
Carn, S. A., Clarisse, L., and Prata, A. J.: Multi-decadal satellite measurements of global volcanic degassing, J. Volcanol. Geoth. Res., 311, 99–134, https://doi.org/10.1016/j.jvolgeores.2016.01.002, 2016. a
Clarisse, L., Hurtmans, D., Clerbaux, C., Hadji-Lazaro, J., Ngadi, Y., and Coheur, P.-F.: Retrieval of sulphur dioxide from the infrared atmospheric sounding interferometer (IASI), Atmos. Meas. Tech., 5, 581–594, https://doi.org/10.5194/amt-5-581-2012, 2012. a, b
Clarisse, L., Coheur, P.-F., Theys, N., Hurtmans, D., and Clerbaux, C.: The 2011 Nabro eruption, a SO2 plume height analysis using IASI measurements, Atmos. Chem. Phys., 14, 3095–3111, https://doi.org/10.5194/acp-14-3095-2014, 2014. a
Clerbaux, C., Boynard, A., Clarisse, L., George, M., Hadji-Lazaro, J., Herbin, H., Hurtmans, D., Pommier, M., Razavi, A., Turquety, S., Wespes, C., and Coheur, P.-F.: Monitoring of atmospheric composition using the thermal infrared IASI/MetOp sounder, Atmos. Chem. Phys., 9, 6041–6054, https://doi.org/10.5194/acp-9-6041-2009, 2009. a
Cornut, F., El Amraoui, L., Cuesta, J., Schmisser, R., Blanc, J., and Josse, B.: Assimilation of Aerosol Observations from the Future Spaceborne Lidar Onboard the AOS Mission into the MOCAGE Chemistry: Transport Model, in: Proceedings of the 30th International Laser Radar Conference, edited by: Sullivan, J. T., Leblanc, T., Tucker, S., Demoz, B., Eloranta, E., Hostetler, C., Ishii, S., Mona, L., Moshary, F., Papayannis, A., and Rupavatharam, K., Springer International Publishing, 645–651, https://doi.org/10.1007/978-3-031-37818-8_83, ISBN 978-3-031-37818-8, 2023. a
Courtier, P., Freydier, C., Geleyn, J.-F., and Rabier, F., and Rochas, M.: The Arpege project at Meteo France, ECMWF, II, 193–232, 1991. a
Cussac, M., Marécal, V., Thouret, V., Josse, B., and Sauvage, B.: The impact of biomass burning on upper tropospheric carbon monoxide: a study using MOCAGE global model and IAGOS airborne data, Atmos. Chem. Phys., 20, 9393–9417, https://doi.org/10.5194/acp-20-9393-2020, 2020. a
El Aabaribaoune, M., Emili, E., and Guidard, V.: Estimation of the error covariance matrix for IASI radiances and its impact on the assimilation of ozone in a chemistry transport model, Atmos. Meas. Tech., 14, 2841–2856, https://doi.org/10.5194/amt-14-2841-2021, 2021. a
El Amraoui, L., Sič, B., Piacentini, A., Marécal, V., Frebourg, N., and Attié, J.-L.: Aerosol data assimilation in the MOCAGE chemical transport model during the TRAQA/ChArMEx campaign: lidar observations, Atmos. Meas. Tech., 13, 4645–4667, https://doi.org/10.5194/amt-13-4645-2020, 2020. a, b
El Amraoui, L., Plu, M., Guidard, V., Cornut, F., and Bacles, M.: A Pre-Operational System Based on the Assimilation of MODIS Aerosol Optical Depth in the MOCAGE Chemical Transport Model, Remote Sens., 14, 1949, https://doi.org/10.3390/rs14081949, 2022. a, b
Emili, E., Barret, B., Massart, S., Le Flochmoen, E., Piacentini, A., El Amraoui, L., Pannekoucke, O., and Cariolle, D.: Combined assimilation of IASI and MLS observations to constrain tropospheric and stratospheric ozone in a global chemical transport model, Atmos. Chem. Phys., 14, 177–198, https://doi.org/10.5194/acp-14-177-2014, 2014. a
Esse, B., Burton, M., Hayer, C., Contreras-Arratia, R., Christopher, T., Joseph, E. P., Varnam, M., and Johnson, C.: SO2 emissions during the 2021 eruption of La Soufrière, St Vincent, revealed with back-trajectory analysis of TROPOMI imagery, Geological Society of London, Special Publications, 539, 231–244, https://doi.org/10.1144/SP539-2022-77, 2024. a
Feinberg, A., Sukhodolov, T., Luo, B.-P., Rozanov, E., Winkel, L. H. E., Peter, T., and Stenke, A.: Improved tropospheric and stratospheric sulfur cycle in the aerosol–chemistry–climate model SOCOL-AERv2, Geosci. Model Dev., 12, 3863–3887, https://doi.org/10.5194/gmd-12-3863-2019, 2019. a
Flemming, J. and Inness, A.: Volcanic sulfur dioxide plume forecasts based on UV satellite retrievals for the 2011 Grímsvötn and the 2010 Eyjafjallajökull eruption, J. Geophys. Res.-Atmos., 118, 10172–10189, https://doi.org/10.1002/jgrd.50753, 2013. a
Gouhier, M., Deslandes, M., Guéhenneux, Y., Hereil, P., Cacault, P., and Josse, B.: Operational Response to Volcanic Ash Risks Using HOTVOLC Satellite-Based System and MOCAGE-Accident Model at the Toulouse VAAC, Atmosphere, 11, 864, https://doi.org/10.3390/atmos11080864, 2020. a, b
Guth, J., Josse, B., Marécal, V., Joly, M., and Hamer, P.: First implementation of secondary inorganic aerosols in the MOCAGE version R2.15.0 chemistry transport model, Geosci. Model Dev., 9, 137–160, https://doi.org/10.5194/gmd-9-137-2016, 2016. a
Hedelt, P., Efremenko, D. S., Loyola, D. G., Spurr, R., and Clarisse, L.: Sulfur dioxide layer height retrieval from Sentinel-5 Precursor/TROPOMI using FP_ILM, Atmos. Meas. Tech., 12, 5503–5517, https://doi.org/10.5194/amt-12-5503-2019, 2019. a, b
Huijnen, V., Williams, J., van Weele, M., van Noije, T., Krol, M., Dentener, F., Segers, A., Houweling, S., Peters, W., de Laat, J., Boersma, F., Bergamaschi, P., van Velthoven, P., Le Sager, P., Eskes, H., Alkemade, F., Scheele, R., Nédélec, P., and Pätz, H.-W.: The global chemistry transport model TM5: description and evaluation of the tropospheric chemistry version 3.0, Geosci. Model Dev., 3, 445–473, https://doi.org/10.5194/gmd-3-445-2010, 2010. a
Inness, A., Ades, M., Balis, D., Efremenko, D., Flemming, J., Hedelt, P., Koukouli, M.-E., Loyola, D., and Ribas, R.: Evaluating the assimilation of S5P/TROPOMI near real-time SO2 columns and layer height data into the CAMS integrated forecasting system (CY47R1), based on a case study of the 2019 Raikoke eruption, Geosci. Model Dev., 15, 971–994, https://doi.org/10.5194/gmd-15-971-2022, 2022. a, b
Josse, B., Simon, P., and Peuch, V. H.: Radon global simulations with the multiscale chemistry and transport model MOCAGE, Tellus B, 56, 339–356, https://doi.org/10.3402/tellusb.v56i4.16448, 2004. a
Kaiser, J. W., Heil, A., Andreae, M. O., Benedetti, A., Chubarova, N., Jones, L., Morcrette, J.-J., Razinger, M., Schultz, M. G., Suttie, M., and van der Werf, G. R.: Biomass burning emissions estimated with a global fire assimilation system based on observed fire radiative power, Biogeosciences, 9, 527–554, https://doi.org/10.5194/bg-9-527-2012, 2012. a
Koukouli, M.-E., Michailidis, K., Hedelt, P., Taylor, I. A., Inness, A., Clarisse, L., Balis, D., Efremenko, D., Loyola, D., Grainger, R. G., and Retscher, C.: Volcanic SO2 layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations, Atmos. Chem. Phys., 22, 5665–5683, https://doi.org/10.5194/acp-22-5665-2022, 2022. a
Lamarque, J.-F., Bond, T. C., Eyring, V., Granier, C., Heil, A., Klimont, Z., Lee, D., Liousse, C., Mieville, A., Owen, B., Schultz, M. G., Shindell, D., Smith, S. J., Stehfest, E., Van Aardenne, J., Cooper, O. R., Kainuma, M., Mahowald, N., McConnell, J. R., Naik, V., Riahi, K., and van Vuuren, D. P.: Historical (1850–2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application, Atmos. Chem. Phys., 10, 7017–7039, https://doi.org/10.5194/acp-10-7017-2010, 2010. a, b
Lamotte, C., Guth, J., Marécal, V., Cussac, M., Hamer, P. D., Theys, N., and Schneider, P.: Modeling study of the impact of SO2 volcanic passive emissions on the tropospheric sulfur budget, Atmos. Chem. Phys., 21, 11379–11404, https://doi.org/10.5194/acp-21-11379-2021, 2021. a
Lechner, P., Tupper, A., Guffanti, M., Loughlin, S., and Casadevall, T.: Volcanic Ash and Aviation – The Challenges of Real-Time, Global Communication of a Natural Hazard, in: Observing the Volcano World: Volcano Crisis Communication, edited by: Fearnley, C. J., Bird, D. K., Haynes, K., McGuire, W. J., and Jolly, G., 51–64, https://doi.org/10.1007/11157_2016_49, ISBN 978-3-319-44097-2, 2018. a
Lefevre, F., Brasseur, G., Folkins, I., Smith, A., and Simon, P.: Chemistry of the 1991–1992 stratospheric winter: Three-dimensional model simulations, J. Geophys. Res.-Atmos., 99, 8183–8195, https://doi.org/10.1029/93JD03476, 1994. a
Li, C., Krotkov, N. A., Carn, S., Zhang, Y., Spurr, R. J. D., and Joiner, J.: New-generation NASA Aura Ozone Monitoring Instrument (OMI) volcanic SO2 dataset: algorithm description, initial results, and continuation with the Suomi-NPP Ozone Mapping and Profiler Suite (OMPS), Atmos. Meas. Tech., 10, 445–458, https://doi.org/10.5194/amt-10-445-2017, 2017. a
Marécal, V., Peuch, V.-H., Andersson, C., Andersson, S., Arteta, J., Beekmann, M., Benedictow, A., Bergström, R., Bessagnet, B., Cansado, A., Chéroux, F., Colette, A., Coman, A., Curier, R. L., Denier van der Gon, H. A. C., Drouin, A., Elbern, H., Emili, E., Engelen, R. J., Eskes, H. J., Foret, G., Friese, E., Gauss, M., Giannaros, C., Guth, J., Joly, M., Jaumouillé, E., Josse, B., Kadygrov, N., Kaiser, J. W., Krajsek, K., Kuenen, J., Kumar, U., Liora, N., Lopez, E., Malherbe, L., Martinez, I., Melas, D., Meleux, F., Menut, L., Moinat, P., Morales, T., Parmentier, J., Piacentini, A., Plu, M., Poupkou, A., Queguiner, S., Robertson, L., Rouïl, L., Schaap, M., Segers, A., Sofiev, M., Tarasson, L., Thomas, M., Timmermans, R., Valdebenito, Á., van Velthoven, P., van Versendaal, R., Vira, J., and Ung, A.: A regional air quality forecasting system over Europe: the MACC-II daily ensemble production, Geosci. Model Dev., 8, 2777–2813, https://doi.org/10.5194/gmd-8-2777-2015, 2015. a
Prata, A. J.: Satellite detection of hazardous volcanic clouds and the risk to global air traffic, Nat. Hazards, 51, 303–324, https://doi.org/10.1007/s11069-008-9273-z, 2009. a
Prata, F., Woodhouse, M., Huppert, H. E., Prata, A., Thordarson, T., and Carn, S.: Atmospheric processes affecting the separation of volcanic ash and SO2 in volcanic eruptions: inferences from the May 2011 Grímsvötn eruption, Atmos. Chem. Phys., 17, 10709–10732, https://doi.org/10.5194/acp-17-10709-2017, 2017. a
Price, C., Penner, J., and Prather, M.: NOx from lightning: 1. Global distribution based on lightning physics, J. Geophys. Res.-Atmos., 102, 5929–5941, https://doi.org/10.1029/96JD03504, 1997. a
Qu, Z., Henze, D. K., Li, C., Theys, N., Wang, Y., Wang, J., Wang, W., Han, J., Shim, C., Dickerson, R. R., and Ren, X.: SO2 Emission Estimates Using OMI SO2 Retrievals for 2005–2017, J. Geophys. Res.-Atmos., 124, 8336–8359, https://doi.org/10.1029/2019JD030243, 2019. a, b
Rodgers, C. D. and Connor, B. J.: Intercomparison of remote sounding instruments, J. Geophys. Res.-Atmos., 108, 4116, https://doi.org/10.1029/2002JD002299, 2003. a
Rouil, L., Honoré, C., Vautard, R., Beekmann, M., Bessagnet, B., Malherbe, L., Meleux, F., Dufour, A., Elichegaray, C., Flaud, J.-M., Menut, L., Martin, D., Peuch, A., Peuch, V.-H., and Poisson, N.: Prev'air: An Operational Forecasting and Mapping System for Air Quality in Europe, B. Am. Meteorol. Soc., 90, 73–84, https://doi.org/10.1175/2008BAMS2390.1, 2009. a
Schmidt, A., Witham, C. S., Theys, N., Richards, N. A. D., Thordarson, T., Szpek, K., Feng, W., Hort, M. C., Woolley, A. M., Jones, A. R., Redington, A. L., Johnson, B. T., Hayward, C. L., and Carslaw, K. S.: Assessing hazards to aviation from sulfur dioxide emitted by explosive Icelandic eruptions, J. Geophys. Res.-Atmos., 119, 14180–14196, https://doi.org/10.1002/2014JD022070, 2014. a
Schumann, U., Weinzierl, B., Reitebuch, O., Schlager, H., Minikin, A., Forster, C., Baumann, R., Sailer, T., Graf, K., Mannstein, H., Voigt, C., Rahm, S., Simmet, R., Scheibe, M., Lichtenstern, M., Stock, P., Rüba, H., Schäuble, D., Tafferner, A., Rautenhaus, M., Gerz, T., Ziereis, H., Krautstrunk, M., Mallaun, C., Gayet, J.-F., Lieke, K., Kandler, K., Ebert, M., Weinbruch, S., Stohl, A., Gasteiger, J., Groß, S., Freudenthaler, V., Wiegner, M., Ansmann, A., Tesche, M., Olafsson, H., and Sturm, K.: Airborne observations of the Eyjafjalla volcano ash cloud over Europe during air space closure in April and May 2010, Atmos. Chem. Phys., 11, 2245–2279, https://doi.org/10.5194/acp-11-2245-2011, 2011. a
Sears, T. M., Thomas, G. E., Carboni, E., A. Smith, A. J., and Grainger, R. G.: SO2 as a possible proxy for volcanic ash in aviation hazard avoidance, J. Geophys. Res.-Atmos., 5698–5709, https://doi.org/10.1002/jgrd.50505, 2013. a
Sellitto, P., Podglajen, A., Belhadji, R., Boichu, M., Carboni, E., Cuesta, J., Duchamp, C., Kloss, C., Siddans, R., Bègue, N., Blarel, L., Jegou, F., Khaykin, S., Renard, J.-B., and Legras, B.: The unexpected radiative impact of the Hunga Tonga eruption of 15th January 2022, Communications Earth & Environment, 3, 1–10, https://doi.org/10.1038/s43247-022-00618-z, 2022. a
Sindelarova, K., Granier, C., Bouarar, I., Guenther, A., Tilmes, S., Stavrakou, T., Müller, J.-F., Kuhn, U., Stefani, P., and Knorr, W.: Global data set of biogenic VOC emissions calculated by the MEGAN model over the last 30 years, Atmos. Chem. Phys., 14, 9317–9341, https://doi.org/10.5194/acp-14-9317-2014, 2014. a
Sič, B., El Amraoui, L., Marécal, V., Josse, B., Arteta, J., Guth, J., Joly, M., and Hamer, P. D.: Modelling of primary aerosols in the chemical transport model MOCAGE: development and evaluation of aerosol physical parameterizations, Geosci. Model Dev., 8, 381–408, https://doi.org/10.5194/gmd-8-381-2015, 2015. a
Sič, B., El Amraoui, L., Piacentini, A., Marécal, V., Emili, E., Cariolle, D., Prather, M., and Attié, J.-L.: Aerosol data assimilation in the chemical transport model MOCAGE during the TRAQA/ChArMEx campaign: aerosol optical depth, Atmos. Meas. Tech., 9, 5535–5554, https://doi.org/10.5194/amt-9-5535-2016, 2016. a
Spurr, R., de Haan, J., van Oss, R., and Vasilkov, A.: Discrete-ordinate radiative transfer in a stratified medium with first-order rotational Raman scattering, J. Quant. Spectrosc. Ra., 109, 404–425, https://doi.org/10.1016/j.jqsrt.2007.08.011, 2008. a
Stockwell, W. R., Kirchner, F., Kuhn, M., and Seefeld, S.: A new mechanism for regional atmospheric chemistry modeling, J. Geophys. Res.-Atmos., 102, 25847–25879, https://doi.org/10.1029/97JD00849, 1997. a
Theys, N.: S5P/TROPOMI SO2 ATBD, Tech. rep. 1.1.0, BIRA, https://sentinels.copernicus.eu/documents/247904/2476257/
Sentinel-5P-ATBD-SO2-TROPOMI/c3930dc9-16f6-4403-9049
-db768eca6ff9?version=1.1 (last access: 17 June 2025), 2018. a
Theys, N., De Smedt, I., Yu, H., Danckaert, T., van Gent, J., Hörmann, C., Wagner, T., Hedelt, P., Bauer, H., Romahn, F., Pedergnana, M., Loyola, D., and Van Roozendael, M.: Sulfur dioxide retrievals from TROPOMI onboard Sentinel-5 Precursor: algorithm theoretical basis, Atmos. Meas. Tech., 10, 119–153, https://doi.org/10.5194/amt-10-119-2017, 2017. a
Theys, N., Hedelt, P., De Smedt, I., Lerot, C., Yu, H., Vlietinck, J., Pedergnana, M., Arellano, S., Galle, B., Fernandez, D., Carlito, C. J. M., Barrington, C., Taisne, B., Delgado-Granados, H., Loyola, D., and Van Roozendael, M.: Global monitoring of volcanic SO2 degassing with unprecedented resolution from TROPOMI onboard Sentinel-5 Precursor, Scientific Reports, 9, 2643, https://doi.org/10.1038/s41598-019-39279-y, 2019. a
Thomas, H. E. and Prata, A. J.: Sulphur dioxide as a volcanic ash proxy during the April–May 2010 eruption of Eyjafjallajökull Volcano, Iceland, Atmos. Chem. Phys., 11, 6871–6880, https://doi.org/10.5194/acp-11-6871-2011, 2011. a
Veefkind, J. P., Aben, I., McMullan, K., Förster, H., de Vries, J., Otter, G., Claas, J., Eskes, H. J., de Haan, J. F., Kleipool, Q., van Weele, M., Hasekamp, O., Hoogeveen, R., Landgraf, J., Snel, R., Tol, P., Ingmann, P., Voors, R., Kruizinga, B., Vink, R., Visser, H., and Levelt, P. F.: TROPOMI on the ESA Sentinel-5 Precursor: A GMES mission for global observations of the atmospheric composition for climate, air quality and ozone layer applications, Remote Sens. Environ., 120, 70–83, https://doi.org/10.1016/j.rse.2011.09.027, 2012. a
Vittorioso, F., Guidard, V., and Fourrié, N.: Assessment of the contribution of the Meteosat Third Generation Infrared Sounder (MTG-IRS) for the characterisation of ozone over Europe, Atmos. Meas. Tech., 17, 5279–5299, https://doi.org/10.5194/amt-17-5279-2024, 2024. a
Webster, H. N. and Thomson, D. J.: Using ensemble meteorological data sets to treat meteorological uncertainties in a Bayesian volcanic ash inverse modeling system: A case study, Grímsvötn 2011, J. Geophys. Res.-Atmos., 127, e2022JD036469, https://doi.org/10.1029/2022JD036469, 2022. a
Witze, A.: Why the Tongan eruption will go down in the history of volcanology, Nature, 602, 376–378, https://doi.org/10.1038/d41586-022-00394-y, 2022. a
Short summary
Sulfur dioxide emitted during volcanic eruptions can be hazardous for aviation safety. A recent development aims at improving the forecasts of volcanic sulfur dioxide quantities made by the chemistry transport model developed at Météo-France by assimilated infrared and ultraviolet satellite instruments. We focus on the eruption event of the La Soufrière Saint Vincent volcano in April 2021. The combined assimilation of these observations always leads to better analyses and forecasts.
Sulfur dioxide emitted during volcanic eruptions can be hazardous for aviation safety. A recent...