Articles | Volume 8, issue 8
https://doi.org/10.5194/amt-8-3519-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-8-3519-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
27 Aug 2015
Research article |
| 27 Aug 2015
Probing ice-nucleation processes on the molecular level using second harmonic generation spectroscopy
Institute of Meteorology and Climate Research – Atmospheric Aerosol Research (IMKAAF), Karlsruhe Institute of Technology (KIT), 76344 Eggenstein-Leopoldshafen, Germany
J. Lützenkirchen
Institute of Nuclear Waste Disposal (INE), Karlsruhe Institute of Technology (KIT), 76344 Eggenstein-Leopoldshafen, Germany
T. Leisner
Institute of Meteorology and Climate Research – Atmospheric Aerosol Research (IMKAAF), Karlsruhe Institute of Technology (KIT), 76344 Eggenstein-Leopoldshafen, Germany
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31 citations as recorded by crossref.
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- Insights into Ice Formation via Immersion Freezing from Nonlinear Optical Spectroscopy K. Lovering & K. Chou https://doi.org/10.1007/s11244-018-0928-z
- Icephobicity of aluminium samples is not affected by pH-generated surface charge S. Apelt & U. Bergmann https://doi.org/10.1016/j.apsusc.2022.155039
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- Computationally efficient approach for the identification of ice-binding surfaces and how they bind ice P. Naullage et al. https://doi.org/10.1063/5.0021631
- Probing the Mineral–Water Interface with Nonlinear Optical Spectroscopy E. Backus et al. https://doi.org/10.1002/anie.202003085
- A set-up for simultaneous measurement of second harmonic generation and streaming potential and some test applications J. Lützenkirchen et al. https://doi.org/10.1016/j.jcis.2018.06.017
- Direct Observation of the Orientational Anisotropy of Buried Hydroxyl Groups inside Muscovite Mica A. Tuladhar et al. https://doi.org/10.1021/jacs.8b12483
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- Pre-ordering of interfacial water in the pathway of heterogeneous ice nucleation does not lead to a two-step crystallization mechanism L. Lupi et al. https://doi.org/10.1063/1.4961652
- Ice Nucleation at the Water–Sapphire Interface: Transient Sum-Frequency Response without Evidence for Transient Ice Phase A. Abdelmonem et al. https://doi.org/10.1021/acs.jpcc.8b07480
- The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review D. Knopf et al. https://doi.org/10.1021/acsearthspacechem.7b00120
- In Situ Chemical Analysis of the Gas–Aerosol Particle Interface Y. Qian et al. https://doi.org/10.1021/acs.analchem.8b02537
- Why α-Alumina Is an Effective Ice Nucleus A. Soni & G. Patey https://doi.org/10.1021/acs.jpcc.9b07973
- Efficient Enhancement of Second Harmonic Generation via Noninvasive Modulation L. Wu et al. https://doi.org/10.3390/app12083962
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- Transient Phase of Ice Observed by Sum Frequency Generation at the Water/Mineral Interface During Freezing K. Lovering et al. https://doi.org/10.1021/acs.jpclett.6b02920
- Single-Particle Time-of-Flight Mass Spectrometry Utilizing a Femtosecond Desorption and Ionization Laser M. Zawadowicz et al. https://doi.org/10.1021/acs.analchem.5b03158
- Modern methods to explore the dynamics between aerosols and convective precipitation: A critical review S. Metangley et al. https://doi.org/10.1016/j.dynatmoce.2024.101465
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- Confronting the Challenge of Modeling Cloud and Precipitation Microphysics H. Morrison et al. https://doi.org/10.1029/2019MS001689
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- Interactions at Aqueous Mineral Interfaces: Insights from Nonlinear Optical Spectroscopy and Atomic Force Microscopy T. Dickbreder & E. Backus https://doi.org/10.1146/annurev-physchem-082624-124821
- Effect of Surface Energy on Freezing Temperature of Water Y. Zhang et al. https://doi.org/10.1021/acsami.6b02094
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31 citations as recorded by crossref.
- Cloud history can change water–ice–surface interactions of oxide mineral aerosols: a case study on silica A. Abdelmonem et al. https://doi.org/10.5194/acp-20-1075-2020
- Interactions of Water with Mineral Dust Aerosol: Water Adsorption, Hygroscopicity, Cloud Condensation, and Ice Nucleation M. Tang et al. https://doi.org/10.1021/acs.chemrev.5b00529
- Insights into Ice Formation via Immersion Freezing from Nonlinear Optical Spectroscopy K. Lovering & K. Chou https://doi.org/10.1007/s11244-018-0928-z
- Icephobicity of aluminium samples is not affected by pH-generated surface charge S. Apelt & U. Bergmann https://doi.org/10.1016/j.apsusc.2022.155039
- Clay mineral mediated dynamics of CO2 hydrate formation and dissociation: Experimental insights for carbon sequestration M. Niu et al. https://doi.org/10.1016/j.energy.2024.133375
- Computationally efficient approach for the identification of ice-binding surfaces and how they bind ice P. Naullage et al. https://doi.org/10.1063/5.0021631
- Probing the Mineral–Water Interface with Nonlinear Optical Spectroscopy E. Backus et al. https://doi.org/10.1002/anie.202003085
- A set-up for simultaneous measurement of second harmonic generation and streaming potential and some test applications J. Lützenkirchen et al. https://doi.org/10.1016/j.jcis.2018.06.017
- Direct Observation of the Orientational Anisotropy of Buried Hydroxyl Groups inside Muscovite Mica A. Tuladhar et al. https://doi.org/10.1021/jacs.8b12483
- Heterogeneous ice nucleation on dust particles sourced from nine deserts worldwide – Part 1: Immersion freezing Y. Boose et al. https://doi.org/10.5194/acp-16-15075-2016
- Pre-ordering of interfacial water in the pathway of heterogeneous ice nucleation does not lead to a two-step crystallization mechanism L. Lupi et al. https://doi.org/10.1063/1.4961652
- Ice Nucleation at the Water–Sapphire Interface: Transient Sum-Frequency Response without Evidence for Transient Ice Phase A. Abdelmonem et al. https://doi.org/10.1021/acs.jpcc.8b07480
- The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review D. Knopf et al. https://doi.org/10.1021/acsearthspacechem.7b00120
- In Situ Chemical Analysis of the Gas–Aerosol Particle Interface Y. Qian et al. https://doi.org/10.1021/acs.analchem.8b02537
- Why α-Alumina Is an Effective Ice Nucleus A. Soni & G. Patey https://doi.org/10.1021/acs.jpcc.9b07973
- Efficient Enhancement of Second Harmonic Generation via Noninvasive Modulation L. Wu et al. https://doi.org/10.3390/app12083962
- Surface-charge-induced orientation of interfacial water suppresses heterogeneous ice nucleation on α-alumina (0001) A. Abdelmonem et al. https://doi.org/10.5194/acp-17-7827-2017
- Transient Phase of Ice Observed by Sum Frequency Generation at the Water/Mineral Interface During Freezing K. Lovering et al. https://doi.org/10.1021/acs.jpclett.6b02920
- Single-Particle Time-of-Flight Mass Spectrometry Utilizing a Femtosecond Desorption and Ionization Laser M. Zawadowicz et al. https://doi.org/10.1021/acs.analchem.5b03158
- Modern methods to explore the dynamics between aerosols and convective precipitation: A critical review S. Metangley et al. https://doi.org/10.1016/j.dynatmoce.2024.101465
- Untersuchung der Mineral‐Wasser‐Grenzschicht mit nicht‐linearer optischer Spektroskopie E. Backus et al. https://doi.org/10.1002/ange.202003085
- Is Ice Nucleation by Organic Crystals Nonclassical? An Assessment of the Monolayer Hypothesis of Ice Nucleation A. Metya & V. Molinero https://doi.org/10.1021/jacs.0c12012
- Ordered Hydrogen Bonding Structure of Water Molecules Adsorbed on Silver Iodide Particles under Subsaturated Conditions H. Yang et al. https://doi.org/10.1021/acs.jpcc.1c01767
- Confronting the Challenge of Modeling Cloud and Precipitation Microphysics H. Morrison et al. https://doi.org/10.1029/2019MS001689
- Direct molecular-level characterization of different heterogeneous freezing modes on mica – Part 1 A. Abdelmonem https://doi.org/10.5194/acp-17-10733-2017
- Ice Nucleation Efficiency of Hydroxylated Organic Surfaces Is Controlled by Their Structural Fluctuations and Mismatch to Ice Y. Qiu et al. https://doi.org/10.1021/jacs.6b12210
- Adsorption of CTAB on Sapphire-c at High pH: Surface and Zeta Potential Measurements Combined with Sum-Frequency and Second-Harmonic Generation A. Abdelmonem et al. https://doi.org/10.1021/acs.langmuir.1c03069
- Interactions at Aqueous Mineral Interfaces: Insights from Nonlinear Optical Spectroscopy and Atomic Force Microscopy T. Dickbreder & E. Backus https://doi.org/10.1146/annurev-physchem-082624-124821
- Effect of Surface Energy on Freezing Temperature of Water Y. Zhang et al. https://doi.org/10.1021/acsami.6b02094
- Unraveling the Mechanism of Ice Nucleation by Mica (001) Surfaces A. Soni & G. Patey https://doi.org/10.1021/acs.jpcc.1c08269
- The surface chemistry of sapphire-c: A literature review and a study on various factors influencing its IEP J. Lützenkirchen et al. https://doi.org/10.1016/j.cis.2017.12.004
Saved (final revised paper)
Latest update: 10 Aug 2026
Short summary
This manuscript belongs and is important to the environmental and atmospheric science, particularly cloud formation and cloud seeding, and presents a setup to apply Second Harmonic Generation spectroscopy to heterogeneous freezing research. We describe the setup and provide first results on temperature-dependent structural changes of water on the surfaces of two relevant atmospheric aerosol substances (sapphire and mica as poor and good ice nucleators, respectively).
This manuscript belongs and is important to the environmental and atmospheric science,...
