Articles | Volume 9, issue 12
https://doi.org/10.5194/amt-9-6117-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-9-6117-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
22 Dec 2016
Research article |
| 22 Dec 2016
Effect of secondary organic aerosol coating thickness on the real-time detection and characterization of biomass-burning soot by two particle mass spectrometers
Adam T. Ahern
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Ramachandran Subramanian
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Georges Saliba
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Eric M. Lipsky
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Penn State Greater Allegheny, 4000 University Drive, McKeesport,
Pennsylvania 15132, USA
Neil M. Donahue
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
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25 citations as recorded by crossref.
- Aerodynamic size-resolved composition and cloud condensation nuclei properties of aerosols in a Beijing suburban region C. Yu et al. 10.5194/acp-22-4375-2022
- Cloud droplet activation of black carbon particles coated with organic compounds of varying solubility M. Dalirian et al. 10.5194/acp-18-12477-2018
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- First Chemical Characterization of Refractory Black Carbon Aerosols and Associated Coatings over the Tibetan Plateau (4730 m a.s.l) J. Wang et al. 10.1021/acs.est.7b03973
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- Time-resolved analysis of primary volatile emissions and secondary aerosol formation potential from a small-scale pellet boiler H. Czech et al. 10.1016/j.atmosenv.2017.03.040
- A Review of Terminology Used to Describe Soot Formation and Evolution under Combustion and Pyrolytic Conditions H. Michelsen et al. 10.1021/acsnano.0c06226
- Mineralogy and mixing state of north African mineral dust by online single-particle mass spectrometry N. Marsden et al. 10.5194/acp-19-2259-2019
- Spatial Variability of Sources and Mixing State of Atmospheric Particles in a Metropolitan Area Q. Ye et al. 10.1021/acs.est.8b01011
- Concept for an electrostatic focusing device for continuous ambient pressure aerosol concentration J. Woo et al. 10.5194/amt-12-3395-2019
- Production of N2O5 and ClNO2 through Nocturnal Processing of Biomass-Burning Aerosol A. Ahern et al. 10.1021/acs.est.7b04386
- Trace Metals in Soot and PM2.5 from Heavy-Fuel-Oil Combustion in a Marine Engine J. Corbin et al. 10.1021/acs.est.8b01764
- Aerosol Measurements by Soot Particle Aerosol Mass Spectrometer: a Review Y. Zhang et al. 10.1007/s40726-020-00162-4
- Optical and Chemical Analysis of Absorption Enhancement by Mixed Carbonaceous Aerosols in the 2019 Woodbury, AZ, Fire Plume J. Lee et al. 10.1029/2020JD032399
- Response of the Reaction Probability of N2O5 with Authentic Biomass-Burning Aerosol to High Relative Humidity L. Jahl et al. 10.1021/acsearthspacechem.1c00227
- Characterization of submicron aerosol chemical composition and sources in the coastal area of Central Chile S. Saarikoski et al. 10.1016/j.atmosenv.2018.11.040
- Particle detection using the dual-vaporizer configuration of the soot particle Aerosol Mass Spectrometer (SP-AMS) A. Avery et al. 10.1080/02786826.2020.1844132
- Size-segregated water-soluble N-bearing species in the land-sea boundary zone of East China R. Li et al. 10.1016/j.atmosenv.2019.116990
- On-line determination of the chemical composition of single activated cloud condensation nuclei – a pilot study C. Dameto de España et al. 10.1080/02786826.2022.2069545
- Time-resolved analysis of particle emissions from residential biomass combustion – Emissions of refractory black carbon, PAHs and organic tracers I. Nielsen et al. 10.1016/j.atmosenv.2017.06.033
- Laser ablation aerosol particle time-of-flight mass spectrometer (LAAPTOF): performance, reference spectra and classification of atmospheric samples X. Shen et al. 10.5194/amt-11-2325-2018
- An inter-comparison of black-carbon-related instruments in a laboratory study of biomass burning aerosol A. Tasoglou et al. 10.1080/02786826.2018.1515473
- Investigating the dependence of light-absorption properties of combustion carbonaceous aerosols on combustion conditions Z. Cheng et al. 10.1080/02786826.2019.1566593
- Understanding atmospheric aerosol particles with improved particle identification and quantification by single-particle mass spectrometry X. Shen et al. 10.5194/amt-12-2219-2019
- N2O5reactive uptake kinetics and chlorine activation on authentic biomass-burning aerosol L. Goldberger et al. 10.1039/C9EM00330D
Latest update: 20 Nov 2024
Short summary
The SP-AMS exhibited a different sensitivity to black carbon vs. potassium as more SOA mass was condensed onto biomass burning particles. The SP-AMS's sensitivity to BC mass did not plateau following successive SOA coatings, despite achieving high OA : BC mass ratios > 9. A laser ablation single-particle mass spectrometer exhibited a positive correlation to the condensed SOA mass on individual soot particles, demonstrating its ability to obtain mass quantitative measurements from complex matrices.
The SP-AMS exhibited a different sensitivity to black carbon vs. potassium as more SOA mass was...
