Articles | Volume 9, issue 12
https://doi.org/10.5194/amt-9-6117-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-9-6117-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Effect of secondary organic aerosol coating thickness on the real-time detection and characterization of biomass-burning soot by two particle mass spectrometers
Adam T. Ahern
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Ramachandran Subramanian
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Georges Saliba
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Eric M. Lipsky
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Penn State Greater Allegheny, 4000 University Drive, McKeesport,
Pennsylvania 15132, USA
Neil M. Donahue
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, 15213, USA
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- An inter-comparison of black-carbon-related instruments in a laboratory study of biomass burning aerosol A. Tasoglou et al. 10.1080/02786826.2018.1515473
- Investigating the dependence of light-absorption properties of combustion carbonaceous aerosols on combustion conditions Z. Cheng et al. 10.1080/02786826.2019.1566593
- Understanding atmospheric aerosol particles with improved particle identification and quantification by single-particle mass spectrometry X. Shen et al. 10.5194/amt-12-2219-2019
- N2O5reactive uptake kinetics and chlorine activation on authentic biomass-burning aerosol L. Goldberger et al. 10.1039/C9EM00330D
Latest update: 14 Dec 2024
Short summary
The SP-AMS exhibited a different sensitivity to black carbon vs. potassium as more SOA mass was condensed onto biomass burning particles. The SP-AMS's sensitivity to BC mass did not plateau following successive SOA coatings, despite achieving high OA : BC mass ratios > 9. A laser ablation single-particle mass spectrometer exhibited a positive correlation to the condensed SOA mass on individual soot particles, demonstrating its ability to obtain mass quantitative measurements from complex matrices.
The SP-AMS exhibited a different sensitivity to black carbon vs. potassium as more SOA mass was...