Articles | Volume 12, issue 2
https://doi.org/10.5194/amt-12-1123-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-12-1123-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
22 Feb 2019
Research article |
| 22 Feb 2019
| 22 Feb 2019
An improved method for mobile characterisation of δ13CH4 source signatures and its application in Germany
Antje Hoheisel
CORRESPONDING AUTHOR
Institute of Environmental Physics, Heidelberg University, Heidelberg, Germany
Christiane Yeman
Institute of Environmental Physics, Heidelberg University, Heidelberg, Germany
now at: Laboratory of Ion Beam Physics, ETH Zurich, Zurich, Switzerland
Florian Dinger
Institute of Environmental Physics, Heidelberg University, Heidelberg, Germany
Max Planck Institute for Chemistry, Mainz, Germany
Henrik Eckhardt
Institute of Environmental Physics, Heidelberg University, Heidelberg, Germany
Martina Schmidt
Institute of Environmental Physics, Heidelberg University, Heidelberg, Germany
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25 citations as recorded by crossref.
- CH4 isotopic signatures of emissions from oil and gas extraction sites in Romania M. Menoud et al. 10.1525/elementa.2021.00092
- Detecting and sourcing GHGs and atmospheric trace gases in a municipal waste treatment plant using coupled chemistry and isotope compositions Y. Bezyk et al. 10.1016/j.wasman.2024.10.003
- Methane mapping, emission quantification, and attribution in two European cities: Utrecht (NL) and Hamburg (DE) H. Maazallahi et al. 10.5194/acp-20-14717-2020
- Advancing Scientific Understanding of the Global Methane Budget in Support of the Paris Agreement A. Ganesan et al. 10.1029/2018GB006065
- Methanogenic pathways and δ13C values from swine manure with a cavity ring‐down spectrometer: Ammonia cross‐interference and carbon isotope labeling F. Dalby et al. 10.1002/rcm.8628
- Stable isotopic signatures of methane from waste sources through atmospheric measurements S. Bakkaloglu et al. 10.1016/j.atmosenv.2022.119021
- Source apportionment of methane emissions from the Upper Silesian Coal Basin using isotopic signatures A. Fiehn et al. 10.5194/acp-23-15749-2023
- Analysis of regional CO2 contributions at the high Alpine observatory Jungfraujoch by means of atmospheric transport simulations and δ13C S. Pieber et al. 10.5194/acp-22-10721-2022
- Low Methane Emissions from the Natural Gas Distribution System Indicated by Mobile Measurements in a Chinese Megacity Hangzhou S. Zhao et al. 10.1021/acsestair.4c00068
- Methane (CH<sub>4</sub>) sources in Krakow, Poland: insights from isotope analysis M. Menoud et al. 10.5194/acp-21-13167-2021
- New contributions of measurements in Europe to the global inventory of the stable isotopic composition of methane M. Menoud et al. 10.5194/essd-14-4365-2022
- Methane emission mapping and quantification in two medium-sized cities in Germany: Heidelberg and Schwetzingen J. Wietzel & M. Schmidt 10.1016/j.aeaoa.2023.100228
- Mapping Urban Methane Sources in Paris, France S. Defratyka et al. 10.1021/acs.est.1c00859
- An open-path observatory for greenhouse gases based on near-infrared Fourier transform spectroscopy T. Schmitt et al. 10.5194/amt-16-6097-2023
- Six years of continuous carbon isotope composition measurements of methane in Heidelberg (Germany) – a study of source contributions and comparison to emission inventories A. Hoheisel & M. Schmidt 10.5194/acp-24-2951-2024
- Current-Modulated Cavity Ring-Down Spectroscopy for Mobile Monitoring of Natural Gas Leaks Z. Mo et al. 10.1109/JLT.2020.3003006
- Ethane measurement by Picarro CRDS G2201-i in laboratory and field conditions: potential and limitations S. Defratyka et al. 10.5194/amt-14-5049-2021
- CleanEx: A Versatile Automated Methane Preconcentration Device for High-Precision Analysis of 13CH4, 12CH3D, and 13CH3D I. Prokhorov & J. Mohn 10.1021/acs.analchem.2c01949
- Continuous CH<sub>4</sub> and <i>δ</i><sup>13</sup>CH<sub>4</sub> measurements in London demonstrate under-reported natural gas leakage E. Saboya et al. 10.5194/acp-22-3595-2022
- Quantification of methane oxidation measuring isotopic signal in 13C on Spanish landfills M. de la Fuente et al. 10.1016/j.apr.2024.102198
- Isotope composition of carbon dioxide and methane in a tropical urban atmosphere K. Carballo-Chaves et al. 10.1080/10256016.2020.1803855
- Methane, ethane, and propane production in Greenland ice core samples and a first isotopic characterization of excess methane M. Mühl et al. 10.5194/cp-19-999-2023
- Isotopic Signatures of Methane Emissions From Dairy Farms in California’s San Joaquin Valley V. Carranza et al. 10.1029/2021JG006675
- Isotopic signatures of major methane sources in the coal seam gas fields and adjacent agricultural districts, Queensland, Australia X. Lu et al. 10.5194/acp-21-10527-2021
- Carbon isotopic characterisation and oxidation of UK landfill methane emissions by atmospheric measurements S. Bakkaloglu et al. 10.1016/j.wasman.2021.07.012
25 citations as recorded by crossref.
- CH4 isotopic signatures of emissions from oil and gas extraction sites in Romania M. Menoud et al. 10.1525/elementa.2021.00092
- Detecting and sourcing GHGs and atmospheric trace gases in a municipal waste treatment plant using coupled chemistry and isotope compositions Y. Bezyk et al. 10.1016/j.wasman.2024.10.003
- Methane mapping, emission quantification, and attribution in two European cities: Utrecht (NL) and Hamburg (DE) H. Maazallahi et al. 10.5194/acp-20-14717-2020
- Advancing Scientific Understanding of the Global Methane Budget in Support of the Paris Agreement A. Ganesan et al. 10.1029/2018GB006065
- Methanogenic pathways and δ13C values from swine manure with a cavity ring‐down spectrometer: Ammonia cross‐interference and carbon isotope labeling F. Dalby et al. 10.1002/rcm.8628
- Stable isotopic signatures of methane from waste sources through atmospheric measurements S. Bakkaloglu et al. 10.1016/j.atmosenv.2022.119021
- Source apportionment of methane emissions from the Upper Silesian Coal Basin using isotopic signatures A. Fiehn et al. 10.5194/acp-23-15749-2023
- Analysis of regional CO2 contributions at the high Alpine observatory Jungfraujoch by means of atmospheric transport simulations and δ13C S. Pieber et al. 10.5194/acp-22-10721-2022
- Low Methane Emissions from the Natural Gas Distribution System Indicated by Mobile Measurements in a Chinese Megacity Hangzhou S. Zhao et al. 10.1021/acsestair.4c00068
- Methane (CH<sub>4</sub>) sources in Krakow, Poland: insights from isotope analysis M. Menoud et al. 10.5194/acp-21-13167-2021
- New contributions of measurements in Europe to the global inventory of the stable isotopic composition of methane M. Menoud et al. 10.5194/essd-14-4365-2022
- Methane emission mapping and quantification in two medium-sized cities in Germany: Heidelberg and Schwetzingen J. Wietzel & M. Schmidt 10.1016/j.aeaoa.2023.100228
- Mapping Urban Methane Sources in Paris, France S. Defratyka et al. 10.1021/acs.est.1c00859
- An open-path observatory for greenhouse gases based on near-infrared Fourier transform spectroscopy T. Schmitt et al. 10.5194/amt-16-6097-2023
- Six years of continuous carbon isotope composition measurements of methane in Heidelberg (Germany) – a study of source contributions and comparison to emission inventories A. Hoheisel & M. Schmidt 10.5194/acp-24-2951-2024
- Current-Modulated Cavity Ring-Down Spectroscopy for Mobile Monitoring of Natural Gas Leaks Z. Mo et al. 10.1109/JLT.2020.3003006
- Ethane measurement by Picarro CRDS G2201-i in laboratory and field conditions: potential and limitations S. Defratyka et al. 10.5194/amt-14-5049-2021
- CleanEx: A Versatile Automated Methane Preconcentration Device for High-Precision Analysis of 13CH4, 12CH3D, and 13CH3D I. Prokhorov & J. Mohn 10.1021/acs.analchem.2c01949
- Continuous CH<sub>4</sub> and <i>δ</i><sup>13</sup>CH<sub>4</sub> measurements in London demonstrate under-reported natural gas leakage E. Saboya et al. 10.5194/acp-22-3595-2022
- Quantification of methane oxidation measuring isotopic signal in 13C on Spanish landfills M. de la Fuente et al. 10.1016/j.apr.2024.102198
- Isotope composition of carbon dioxide and methane in a tropical urban atmosphere K. Carballo-Chaves et al. 10.1080/10256016.2020.1803855
- Methane, ethane, and propane production in Greenland ice core samples and a first isotopic characterization of excess methane M. Mühl et al. 10.5194/cp-19-999-2023
- Isotopic Signatures of Methane Emissions From Dairy Farms in California’s San Joaquin Valley V. Carranza et al. 10.1029/2021JG006675
- Isotopic signatures of major methane sources in the coal seam gas fields and adjacent agricultural districts, Queensland, Australia X. Lu et al. 10.5194/acp-21-10527-2021
- Carbon isotopic characterisation and oxidation of UK landfill methane emissions by atmospheric measurements S. Bakkaloglu et al. 10.1016/j.wasman.2021.07.012
Latest update: 14 Dec 2024
Short summary
In this study, we developed and applied a mobile instrument set-up to determine the carbon isotope source signature by measuring the plume of different methane sources. Therefore, we carefully characterised the analyser especially with regard to cross sensitivities of the gas matrix. During 21 field campaigns we determined mean carbon isotope values of three dairy farms, a biogas plant, a landfill, a wastewater treatment plant, an active deep coal mine and two natural gas facilities in Germany.
In this study, we developed and applied a mobile instrument set-up to determine the carbon...
