Articles | Volume 14, issue 2
https://doi.org/10.5194/amt-14-1319-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-14-1319-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Determination of equivalent black carbon mass concentration from aerosol light absorption using variable mass absorption cross section
Weilun Zhao
Department of Atmospheric and Oceanic Sciences, School of Physics,
Peking University, Beijing 100871, China
Wangshu Tan
Department of Atmospheric and Oceanic Sciences, School of Physics,
Peking University, Beijing 100871, China
School of Optics and Photonics, Beijing Institute of Technology,
Beijing 100081, China
Gang Zhao
Department of Atmospheric and Oceanic Sciences, School of Physics,
Peking University, Beijing 100871, China
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Chuanyang Shen
Department of Atmospheric and Oceanic Sciences, School of Physics,
Peking University, Beijing 100871, China
Yingli Yu
Economics & Technology Research Institute, China National Petroleum
Corporation, Beijing 100724, China
Department of Atmospheric and Oceanic Sciences, School of Physics,
Peking University, Beijing 100871, China
Chunsheng Zhao
CORRESPONDING AUTHOR
Department of Atmospheric and Oceanic Sciences, School of Physics,
Peking University, Beijing 100871, China
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Siying Chen, Rongzheng Cao, Yixuan Xie, Yinchao Zhang, Wangshu Tan, He Chen, Pan Guo, and Peitao Zhao
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Jie Qiu, Wangshu Tan, Gang Zhao, Yingli Yu, and Chunsheng Zhao
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Gang Zhao, Yishu Zhu, Zhijun Wu, Taomou Zong, Jingchuan Chen, Tianyi Tan, Haichao Wang, Xin Fang, Keding Lu, Chunsheng Zhao, and Min Hu
Atmos. Chem. Phys., 21, 9995–10004, https://doi.org/10.5194/acp-21-9995-2021, https://doi.org/10.5194/acp-21-9995-2021, 2021
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Tianyi Tan, Min Hu, Zhuofei Du, Gang Zhao, Dongjie Shang, Jing Zheng, Yanhong Qin, Mengren Li, Yusheng Wu, Limin Zeng, Song Guo, and Zhijun Wu
Atmos. Chem. Phys., 21, 8499–8510, https://doi.org/10.5194/acp-21-8499-2021, https://doi.org/10.5194/acp-21-8499-2021, 2021
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Chuanyang Shen, Gang Zhao, and Chunsheng Zhao
Atmos. Meas. Tech., 14, 1293–1301, https://doi.org/10.5194/amt-14-1293-2021, https://doi.org/10.5194/amt-14-1293-2021, 2021
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Aerosol hygroscopicity measured by the humidified tandem differential mobility analyzer (HTDMA) is affected by multiply charged particles from two aspects: (1) number contribution and (2) the weakening effect. An algorithm is proposed to do the multi-charge correction and applied to a field measurement. Results show that the difference between corrected and measured size-resolved κ can reach 0.05, highlighting that special attention needs to be paid to the multi-charge effect when using HTDMA.
Chuanyang Shen, Gang Zhao, Weilun Zhao, Ping Tian, and Chunsheng Zhao
Atmos. Chem. Phys., 21, 1375–1388, https://doi.org/10.5194/acp-21-1375-2021, https://doi.org/10.5194/acp-21-1375-2021, 2021
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Submicron particles larger than 300 nm dominate the aerosol light extinction and mass concentration in the urban environment. Aerosol hygroscopic properties extended to 600 nm were investigated at an urban site. Our results find that there exists a large fraction of a less hygroscopic group above 300 nm, and the hygroscopicity in this size range is enhanced significantly with the development of pollution levels. The hygroscopicity variation contributes greatly to the low visibility.
Martin J. Wolf, Megan Goodell, Eric Dong, Lilian A. Dove, Cuiqi Zhang, Lesly J. Franco, Chuanyang Shen, Emma G. Rutkowski, Domenic N. Narducci, Susan Mullen, Andrew R. Babbin, and Daniel J. Cziczo
Atmos. Chem. Phys., 20, 15341–15356, https://doi.org/10.5194/acp-20-15341-2020, https://doi.org/10.5194/acp-20-15341-2020, 2020
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Sea spray is the largest aerosol source on Earth. These aerosol particles can impact climate by inducing ice formation in clouds. The role that ocean biology plays in determining the composition and ice nucleation abilities of sea spray aerosol is unclarified. In this study, we demonstrate that atomized seawater from highly productive ocean regions is more effective at nucleating ice than seawater from lower-productivity regions.
Cuiqi Zhang, Yue Zhang, Martin J. Wolf, Leonid Nichman, Chuanyang Shen, Timothy B. Onasch, Longfei Chen, and Daniel J. Cziczo
Atmos. Chem. Phys., 20, 13957–13984, https://doi.org/10.5194/acp-20-13957-2020, https://doi.org/10.5194/acp-20-13957-2020, 2020
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Black carbon (BC) is considered the second most important global warming agent. However, the role of BC aerosol–cloud–climate interactions in the cirrus formation remains uncertain. Our study of selected BC types and sizes suggests that increases in diameter, compactness, and/or surface oxidation of BC particles lead to more efficient ice nucleation (IN) via pore condensation freezing (PCF) pathways,and that coatings of common secondary organic aerosol (SOA) materials can inhibit ice formation.
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