Articles | Volume 14, issue 3
https://doi.org/10.5194/amt-14-1893-2021
https://doi.org/10.5194/amt-14-1893-2021
Research article
 | 
09 Mar 2021
Research article |  | 09 Mar 2021

A new method to detect and classify polar stratospheric nitric acid trihydrate clouds derived from radiative transfer simulations and its first application to airborne infrared limb emission observations

Christoph Kalicinsky, Sabine Griessbach, and Reinhold Spang

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Cited articles

Achtert, P. and Tesche, M.: Assessing lidar-based classification schemes for polar stratospheric clouds based on 16 years of measurements at Esrange, Sweden, J. Geophys. Res., 119, 1386–1405, https://doi.org/10.1002/2013jd020355, 2014. a
Biermann, U. M.: Gefrier- und FTIR-Experimente zur Nukleation und Lebensdauer stratosphärischer Wolken, PhD thesis, Universität Bielefeld, Bielefeld, Germany, ISBN 3-89712-212-X, 1998. a, b
Biermann, U. M., Luo, B. P., and Peter, T.: Absorption spectra and optical constants of binary and ternary solutions of H2SO4, HNO3, and H2O in the mid infrared at atmospheric temperatures, J. Phys. Chem. A, 104, 783–793, https://doi.org/10.1021/jp992349i, 2000. a, b
Boone, C. D., Walker, K. A., and Bernath, P. F.: Version 3 Retrievals for the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS), in: The Atmospheric Chemistry Experiment ACE at 10: a solar occultation anthology, edited by: Bernath, P. F., A Deepak Publishing, Virginia, USA, 103–127, 2013. a, b, c, d
Bullister, J.: Atmospheric CFC-11, CFC-12, CFC-113, CCl4 and SF6 Histories, Tech. Rep., Carbon Dioxide Information Analysis Center, Oak Ridge National Laboratory, US Department of Energy, Oak Ridge, Tennessee, USA, 2011. a, b, c, d
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Short summary
For an airborne viewing geometry, radiative transfer simulations of infrared limb emission spectra in the presence of polar stratospheric clouds – nitric acid trihydrate (NAT), supercooled ternary solution, ice, and mixtures – were used to develop a size-sensitive NAT detection algorithm. Characteristic size-dependent spectral features in the 810–820 cm−1 region were exploited to subgroup the NAT into three size regimes: small NAT (≤ 1.0 μm), medium NAT (1.5–4.0 μm), and large NAT (≥ 3.5 μm).