Articles | Volume 16, issue 18
https://doi.org/10.5194/amt-16-4229-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-16-4229-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
21 Sep 2023
Research article |
| 21 Sep 2023
| 21 Sep 2023
Long-term airborne measurements of pollutants over the United Kingdom to support air quality model development and evaluation
Angela Mynard
CORRESPONDING AUTHOR
Met Office, Exeter, Devon, EX3 1PB, UK
Joss Kent
Met Office, Exeter, Devon, EX3 1PB, UK
Eleanor R. Smith
Met Office, Exeter, Devon, EX3 1PB, UK
Andy Wilson
Met Office, Exeter, Devon, EX3 1PB, UK
Kirsty Wivell
Met Office, Exeter, Devon, EX3 1PB, UK
Noel Nelson
Met Office, Exeter, Devon, EX3 1PB, UK
Matthew Hort
Met Office, Exeter, Devon, EX3 1PB, UK
James Bowles
Met Office, Exeter, Devon, EX3 1PB, UK
David Tiddeman
Met Office, Exeter, Devon, EX3 1PB, UK
Justin M. Langridge
Met Office, Exeter, Devon, EX3 1PB, UK
Benjamin Drummond
Met Office, Exeter, Devon, EX3 1PB, UK
Steven J. Abel
Met Office, Exeter, Devon, EX3 1PB, UK
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Erin N. Raif, Sarah L. Barr, Mark D. Tarn, James B. McQuaid, Martin I. Daily, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Paul R. Field, Kenneth S. Carslaw, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 14045–14072, https://doi.org/10.5194/acp-24-14045-2024, https://doi.org/10.5194/acp-24-14045-2024, 2024
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Ice-nucleating particles (INPs) allow ice to form in clouds at temperatures warmer than −35°C. We measured INP concentrations over the Norwegian and Barents seas in weather events where cold air is ejected from the Arctic. These concentrations were among the highest measured in the Arctic. It is likely that the INPs were transported to the Arctic from distant regions. These results show it is important to consider hemispheric-scale INP processes to understand INP concentrations in the Arctic.
Melody Sandells, Nick Rutter, Kirsty Wivell, Richard Essery, Stuart Fox, Chawn Harlow, Ghislain Picard, Alexandre Roy, Alain Royer, and Peter Toose
The Cryosphere, 18, 3971–3990, https://doi.org/10.5194/tc-18-3971-2024, https://doi.org/10.5194/tc-18-3971-2024, 2024
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Satellite microwave observations are used for weather forecasting. In Arctic regions this is complicated by natural emission from snow. By simulating airborne observations from in situ measurements of snow, this study shows how snow properties affect the signal within the atmosphere. Fresh snowfall between flights changed airborne measurements. Good knowledge of snow layering and structure can be used to account for the effects of snow and could unlock these data to improve forecasts.
Manfred Wendisch, Susanne Crewell, André Ehrlich, Andreas Herber, Benjamin Kirbus, Christof Lüpkes, Mario Mech, Steven J. Abel, Elisa F. Akansu, Felix Ament, Clémantyne Aubry, Sebastian Becker, Stephan Borrmann, Heiko Bozem, Marlen Brückner, Hans-Christian Clemen, Sandro Dahlke, Georgios Dekoutsidis, Julien Delanoë, Elena De La Torre Castro, Henning Dorff, Regis Dupuy, Oliver Eppers, Florian Ewald, Geet George, Irina V. Gorodetskaya, Sarah Grawe, Silke Groß, Jörg Hartmann, Silvia Henning, Lutz Hirsch, Evelyn Jäkel, Philipp Joppe, Olivier Jourdan, Zsofia Jurányi, Michail Karalis, Mona Kellermann, Marcus Klingebiel, Michael Lonardi, Johannes Lucke, Anna E. Luebke, Maximilian Maahn, Nina Maherndl, Marion Maturilli, Bernhard Mayer, Johanna Mayer, Stephan Mertes, Janosch Michaelis, Michel Michalkov, Guillaume Mioche, Manuel Moser, Hanno Müller, Roel Neggers, Davide Ori, Daria Paul, Fiona M. Paulus, Christian Pilz, Felix Pithan, Mira Pöhlker, Veronika Pörtge, Maximilian Ringel, Nils Risse, Gregory C. Roberts, Sophie Rosenburg, Johannes Röttenbacher, Janna Rückert, Michael Schäfer, Jonas Schaefer, Vera Schemann, Imke Schirmacher, Jörg Schmidt, Sebastian Schmidt, Johannes Schneider, Sabrina Schnitt, Anja Schwarz, Holger Siebert, Harald Sodemann, Tim Sperzel, Gunnar Spreen, Bjorn Stevens, Frank Stratmann, Gunilla Svensson, Christian Tatzelt, Thomas Tuch, Timo Vihma, Christiane Voigt, Lea Volkmer, Andreas Walbröl, Anna Weber, Birgit Wehner, Bruno Wetzel, Martin Wirth, and Tobias Zinner
Atmos. Chem. Phys., 24, 8865–8892, https://doi.org/10.5194/acp-24-8865-2024, https://doi.org/10.5194/acp-24-8865-2024, 2024
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The Arctic is warming faster than the rest of the globe. Warm-air intrusions (WAIs) into the Arctic may play an important role in explaining this phenomenon. Cold-air outbreaks (CAOs) out of the Arctic may link the Arctic climate changes to mid-latitude weather. In our article, we describe how to observe air mass transformations during CAOs and WAIs using three research aircraft instrumented with state-of-the-art remote-sensing and in situ measurement devices.
Declan L. Finney, Alan M. Blyth, Martin Gallagher, Huihui Wu, Graeme J. Nott, Michael I. Biggerstaff, Richard G. Sonnenfeld, Martin Daily, Dan Walker, David Dufton, Keith Bower, Steven Böing, Thomas Choularton, Jonathan Crosier, James Groves, Paul R. Field, Hugh Coe, Benjamin J. Murray, Gary Lloyd, Nicholas A. Marsden, Michael Flynn, Kezhen Hu, Navaneeth M. Thamban, Paul I. Williams, Paul J. Connolly, James B. McQuaid, Joseph Robinson, Zhiqiang Cui, Ralph R. Burton, Gordon Carrie, Robert Moore, Steven J. Abel, Dave Tiddeman, and Graydon Aulich
Earth Syst. Sci. Data, 16, 2141–2163, https://doi.org/10.5194/essd-16-2141-2024, https://doi.org/10.5194/essd-16-2141-2024, 2024
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The DCMEX (Deep Convective Microphysics Experiment) project undertook an aircraft- and ground-based measurement campaign of New Mexico deep convective clouds during July–August 2022. The campaign coordinated a broad range of instrumentation measuring aerosol, cloud physics, radar signals, thermodynamics, dynamics, electric fields, and weather. The project's objectives included the utilisation of these data with satellite observations to study the anvil cloud radiative effect.
Kirsty Wivell, Stuart Fox, Melody Sandells, Chawn Harlow, Richard Essery, and Nick Rutter
The Cryosphere, 17, 4325–4341, https://doi.org/10.5194/tc-17-4325-2023, https://doi.org/10.5194/tc-17-4325-2023, 2023
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Satellite microwave observations improve weather forecasts, but to use these observations in the Arctic, snow emission must be known. This study uses airborne and in situ snow observations to validate emissivity simulations for two- and three-layer snowpacks at key frequencies for weather prediction. We assess the impact of thickness, grain size and density in key snow layers, which will help inform development of physical snow models that provide snow profile input to emissivity simulations.
Andrew R. Jones, Susan J. Leadbetter, and Matthew C. Hort
Atmos. Chem. Phys., 23, 12477–12503, https://doi.org/10.5194/acp-23-12477-2023, https://doi.org/10.5194/acp-23-12477-2023, 2023
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The paper explores spread and calibration properties of ensemble atmospheric dispersion forecasts for hypothetical release events. Real-time forecasts from an ensemble weather prediction system were used to generate an ensemble of dispersion predictions and assessed against simulations produced using analysis meteorology. Results demonstrate good performance overall but highlight more skilful predictions for material released in the upper air compared with releases near the surface.
Danny McCulloch, Denis E. Sergeev, Nathan Mayne, Matthew Bate, James Manners, Ian Boutle, Benjamin Drummond, and Kristzian Kohary
Geosci. Model Dev., 16, 621–657, https://doi.org/10.5194/gmd-16-621-2023, https://doi.org/10.5194/gmd-16-621-2023, 2023
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We present results from the Met Office Unified Model (UM) to study the dry Martian climate. We describe our model set-up conditions and run two scenarios, with radiatively active/inactive dust. We compare both scenarios to results from an existing Mars climate model, the planetary climate model. We find good agreement in winds and air temperatures, but dust amounts differ between models. This study highlights the importance of using the UM for future Mars research.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Susan J. Leadbetter, Andrew R. Jones, and Matthew C. Hort
Atmos. Chem. Phys., 22, 577–596, https://doi.org/10.5194/acp-22-577-2022, https://doi.org/10.5194/acp-22-577-2022, 2022
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In this study we look at the ability of meteorological ensembles (multiple realisations of the meteorological data) to provide information about the uncertainty in the dispersion model predictions. Statistical measures are used to evaluate the model predictions, and these show that on average the ensemble predictions outperform the non-ensemble predictions.
Dawei Hu, M. Rami Alfarra, Kate Szpek, Justin M. Langridge, Michael I. Cotterell, Claire Belcher, Ian Rule, Zixia Liu, Chenjie Yu, Yunqi Shao, Aristeidis Voliotis, Mao Du, Brett Smith, Greg Smallwood, Prem Lobo, Dantong Liu, Jim M. Haywood, Hugh Coe, and James D. Allan
Atmos. Chem. Phys., 21, 16161–16182, https://doi.org/10.5194/acp-21-16161-2021, https://doi.org/10.5194/acp-21-16161-2021, 2021
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Here, we developed new techniques for investigating these properties in the laboratory and applied these to BC and BrC from different sources, including diesel exhaust, inverted propane flame and wood combustion. These have allowed us to quantify the changes in shape and chemical composition of different soots according to source and variables such as the moisture content of wood.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Huihui Wu, Jonathan W. Taylor, Justin M. Langridge, Chenjie Yu, James D. Allan, Kate Szpek, Michael I. Cotterell, Paul I. Williams, Michael Flynn, Patrick Barker, Cathryn Fox, Grant Allen, James Lee, and Hugh Coe
Atmos. Chem. Phys., 21, 9417–9440, https://doi.org/10.5194/acp-21-9417-2021, https://doi.org/10.5194/acp-21-9417-2021, 2021
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Seasonal biomass burning over West Africa is a globally significant source of carbonaceous particles in the atmosphere, which have important climate impacts but are poorly constrained. We conducted in situ airborne measurements to investigate the evolution of smoke aerosol properties in this region. We observed absorption enhancement for both black carbon and brown carbon after emission, which provides new field results and constraints on aerosol parameterizations for future climate models.
Fanny Peers, Peter Francis, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Michael I. Cotterell, Ian Crawford, Nicholas W. Davies, Cathryn Fox, Stuart Fox, Justin M. Langridge, Kerry G. Meyer, Steven E. Platnick, Kate Szpek, and Jim M. Haywood
Atmos. Chem. Phys., 21, 3235–3254, https://doi.org/10.5194/acp-21-3235-2021, https://doi.org/10.5194/acp-21-3235-2021, 2021
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Satellite observations at high temporal resolution are a valuable asset to monitor the transport of biomass burning plumes and the cloud diurnal cycle in the South Atlantic, but they need to be validated. Cloud and above-cloud aerosol properties retrieved from SEVIRI are compared against MODIS and measurements from the CLARIFY-2017 campaign. While some systematic differences are observed between SEVIRI and MODIS, the overall agreement in the cloud and aerosol properties is very satisfactory.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Huihui Wu, Jonathan W. Taylor, Kate Szpek, Justin M. Langridge, Paul I. Williams, Michael Flynn, James D. Allan, Steven J. Abel, Joseph Pitt, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 12697–12719, https://doi.org/10.5194/acp-20-12697-2020, https://doi.org/10.5194/acp-20-12697-2020, 2020
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Airborne measurements of highly aged biomass burning aerosols (BBAs) over the remote southeast Atlantic provide unique aerosol parameters for climate models. Our observations demonstrate the persistence of strongly absorbing BBAs across wide regions of the South Atlantic. We also found significant vertical variation in the single-scattering albedo of these BBAs, as a function of relative chemical composition and size. Aerosol properties in the marine BL are suggested to be separated from the FT.
Jonathan W. Taylor, Huihui Wu, Kate Szpek, Keith Bower, Ian Crawford, Michael J. Flynn, Paul I. Williams, James Dorsey, Justin M. Langridge, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim M. Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 11201–11221, https://doi.org/10.5194/acp-20-11201-2020, https://doi.org/10.5194/acp-20-11201-2020, 2020
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Every year, huge plumes of smoke hundreds of miles wide travel over the south Atlantic Ocean from fires in central and southern Africa. These plumes absorb the sun’s energy and warm the climate. We used airborne optical instrumentation to determine how absorbing the smoke was as well as the relative importance of black and brown carbon. We also tested different ways of simulating these properties that could be used in a climate model.
Hamish Gordon, Paul R. Field, Steven J. Abel, Paul Barrett, Keith Bower, Ian Crawford, Zhiqiang Cui, Daniel P. Grosvenor, Adrian A. Hill, Jonathan Taylor, Jonathan Wilkinson, Huihui Wu, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10997–11024, https://doi.org/10.5194/acp-20-10997-2020, https://doi.org/10.5194/acp-20-10997-2020, 2020
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The Met Office's Unified Model is widely used both for weather forecasting and climate prediction. We present the first version of the model in which both aerosol and cloud particle mass and number concentrations are allowed to evolve separately and independently, which is important for studying how aerosols affect weather and climate. We test the model against aircraft observations near Ascension Island in the Atlantic, focusing on how aerosols can "activate" to become cloud droplets.
Steven J. Abel, Paul A. Barrett, Paquita Zuidema, Jianhao Zhang, Matt Christensen, Fanny Peers, Jonathan W. Taylor, Ian Crawford, Keith N. Bower, and Michael Flynn
Atmos. Chem. Phys., 20, 4059–4084, https://doi.org/10.5194/acp-20-4059-2020, https://doi.org/10.5194/acp-20-4059-2020, 2020
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In situ measurements of a free-tropospheric (FT) biomass burning aerosol plume in contact with the boundary layer inversion overriding a pocket of open cells (POC) and surrounding stratiform cloud are presented. The data highlight the contrasting thermodynamic, aerosol and cloud properties in the two cloud regimes and further demonstrate that the cloud regime plays a key role in regulating the flow of FT aerosols into the boundary layer, which has implications for the aerosol indirect effect.
Paul A. Barrett, Alan Blyth, Philip R. A. Brown, and Steven J. Abel
Atmos. Chem. Phys., 20, 1921–1939, https://doi.org/10.5194/acp-20-1921-2020, https://doi.org/10.5194/acp-20-1921-2020, 2020
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Here we present new in situ observations from altocumulus clouds made with a research aircraft. By carefully measuring the cloud top height, we are able to study the turbulence and cloud properties in high vertical resolution, something not presented before. The clouds contain both ice particles and liquid drops, even though the temperature is −30 °C. These measurements will hopefully assist future developers of climate models to verify and assess the performance of simulations.
Fanny Peers, Peter Francis, Cathryn Fox, Steven J. Abel, Kate Szpek, Michael I. Cotterell, Nicholas W. Davies, Justin M. Langridge, Kerry G. Meyer, Steven E. Platnick, and Jim M. Haywood
Atmos. Chem. Phys., 19, 9595–9611, https://doi.org/10.5194/acp-19-9595-2019, https://doi.org/10.5194/acp-19-9595-2019, 2019
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The measurements from the geostationary satellite MSG/SEVIRI are used to retrieve the cloud and above-cloud aerosol properties over the South Atlantic. The technique relies on the spectral contrast and the magnitude of the signal in the visible to shortwave infrared region as well as the atmospheric correction based on forecasted water vapour profiles. The sensitivity analysis and the stability of the retrieval over time show great potential of the high-temporal-resolution observations.
Nicholas W. Davies, Cathryn Fox, Kate Szpek, Michael I. Cotterell, Jonathan W. Taylor, James D. Allan, Paul I. Williams, Jamie Trembath, Jim M. Haywood, and Justin M. Langridge
Atmos. Meas. Tech., 12, 3417–3434, https://doi.org/10.5194/amt-12-3417-2019, https://doi.org/10.5194/amt-12-3417-2019, 2019
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This research project assesses biases in traditional, filter-based, aerosol absorption measurements by comparison to state-of-the-art, non-filter-based, or in situ, measurements. We assess biases in traditional absorption measurements for three main aerosol types, including dust and fresh and aged biomass burning aerosols. The main results of this study are that the traditional and state-of-the-art absorption measurements are well correlated and that biases in the former are up to 45 %.
James Brooks, James D. Allan, Paul I. Williams, Dantong Liu, Cathryn Fox, Jim Haywood, Justin M. Langridge, Ellie J. Highwood, Sobhan K. Kompalli, Debbie O'Sullivan, Suresh S. Babu, Sreedharan K. Satheesh, Andrew G. Turner, and Hugh Coe
Atmos. Chem. Phys., 19, 5615–5634, https://doi.org/10.5194/acp-19-5615-2019, https://doi.org/10.5194/acp-19-5615-2019, 2019
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Our study, for the first time, presents measurements of aerosol chemical composition and physical characteristics across northern India in the pre-monsoon and monsoon seasons of 2016 using the FAAM BAe-146 UK research aircraft. Across northern India, an elevated aerosol layer dominated by sulfate aerosol exists that diminishes with monsoon arrival. The Indo-Gangetic Plain (IGP) boundary layer is dominated by organics, whereas outside the IGP sulfate dominates with increased scattering aerosol.
Ayoe Buus Hansen, Claire Suzanne Witham, Wei Ming Chong, Emma Kendall, Boon Ning Chew, Christopher Gan, Matthew Craig Hort, and Shao-Yi Lee
Atmos. Chem. Phys., 19, 5363–5385, https://doi.org/10.5194/acp-19-5363-2019, https://doi.org/10.5194/acp-19-5363-2019, 2019
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We have modelled biomass burning haze concentrations in Singapore between 2010 and 2015. The major contributing haze source regions at two monitoring stations located in the western and eastern part of Singapore, less than 30 km apart, show significant variation on seasonal and annual timescales, as well as between the stations. Our results show that haze concentrations in Singapore are driven by a combination of local and regional weather, climate, and the location of regional burning.
Michael I. Cotterell, Andrew J. Orr-Ewing, Kate Szpek, Jim M. Haywood, and Justin M. Langridge
Atmos. Meas. Tech., 12, 2371–2385, https://doi.org/10.5194/amt-12-2371-2019, https://doi.org/10.5194/amt-12-2371-2019, 2019
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Photoacoustic spectroscopy provides measurements of absorption coefficient for aerosol and gas samples but requires careful calibration, and researchers often use concentrations of ozone. Recent work has shown that the bath gas composition impacts the accuracy of this calibration at visible wavelengths. We explore further the role of bath gas, demonstrating that the calibration accuracy is optimal for a bath gas composed of 20 % oxygen and 80 % nitrogen at wavelengths of 405, 514 and 658 nm.
Gary Lloyd, Thomas W. Choularton, Keith N. Bower, Martin W. Gallagher, Jonathan Crosier, Sebastian O'Shea, Steven J. Abel, Stuart Fox, Richard Cotton, and Ian A. Boutle
Atmos. Chem. Phys., 18, 17191–17206, https://doi.org/10.5194/acp-18-17191-2018, https://doi.org/10.5194/acp-18-17191-2018, 2018
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The work deals with cold weather outbreaks at high latitudes that often bring severe weather such as heavy snow, lightning and high winds but are poorly forecast by weather models. Here we made measurements of these events and the clouds associated with them using a research aircraft. We found that the properties of these clouds were often very different to what the models predicted, and these results can potentially be used to bring significant improvement to the forecasting of these events.
Hamish Gordon, Paul R. Field, Steven J. Abel, Mohit Dalvi, Daniel P. Grosvenor, Adrian A. Hill, Ben T. Johnson, Annette K. Miltenberger, Masaru Yoshioka, and Ken S. Carslaw
Atmos. Chem. Phys., 18, 15261–15289, https://doi.org/10.5194/acp-18-15261-2018, https://doi.org/10.5194/acp-18-15261-2018, 2018
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Smoke from African fires is frequently transported across the Atlantic Ocean, where it interacts with clouds. We simulate the interaction of the smoke with the clouds, and the consequences of this for the solar radiation the clouds reflect. The simulations use a new regional configuration of the UK Met Office climate model. Our simulations indicate that the properties of the clouds, in particular their height and reflectivity, and the fractional cloud cover, are strongly affected by the smoke.
Nicholas W. Davies, Michael I. Cotterell, Cathryn Fox, Kate Szpek, Jim M. Haywood, and Justin M. Langridge
Atmos. Meas. Tech., 11, 2313–2324, https://doi.org/10.5194/amt-11-2313-2018, https://doi.org/10.5194/amt-11-2313-2018, 2018
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The poorly characterised optical properties of atmospheric aerosols are one of the major uncertainties when modelling future climate change. Photoacoustic spectroscopy is an accurate and sensitive method for measurement of aerosol light absorption. Photoacoustic spectrometers require calibration; hence this study validates the use of ozone as a calibrant and simultaneously verifies the accuracy of the photoacoustic spectrometers in question.
Rudra P. Pokhrel, Eric R. Beamesderfer, Nick L. Wagner, Justin M. Langridge, Daniel A. Lack, Thilina Jayarathne, Elizabeth A. Stone, Chelsea E. Stockwell, Robert J. Yokelson, and Shane M. Murphy
Atmos. Chem. Phys., 17, 5063–5078, https://doi.org/10.5194/acp-17-5063-2017, https://doi.org/10.5194/acp-17-5063-2017, 2017
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This study investigates enhancement of black carbon (BC) absorption in biomass burning emissions due to absorbing and non-absorbing coatings. The fraction of absorption due to BC, brown carbon (BrC), and lensing is estimated using different approaches. The similarities and differences between the results from these approaches are discussed. Absorption by BrC is shown to have good correlation with the elemental to organic carbon ratio (EC / OC) and AAE.
Ben T. Johnson, James M. Haywood, Justin M. Langridge, Eoghan Darbyshire, William T. Morgan, Kate Szpek, Jennifer K. Brooke, Franco Marenco, Hugh Coe, Paulo Artaxo, Karla M. Longo, Jane P. Mulcahy, Graham W. Mann, Mohit Dalvi, and Nicolas Bellouin
Atmos. Chem. Phys., 16, 14657–14685, https://doi.org/10.5194/acp-16-14657-2016, https://doi.org/10.5194/acp-16-14657-2016, 2016
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Biomass burning is a large source of carbonaceous aerosols, which scatter and absorb solar radiation, and modify cloud properties. We evaluate the simulation of biomass burning aerosol processes and properties in the HadGEM3 climate model using observations, including those from the South American Biomass Burning Analysis. We find that modelled aerosol optical depths are underestimated unless aerosol emissions (Global Fire Emission Database v3) are increased by a factor of 1.6–2.0.
Rudra P. Pokhrel, Nick L. Wagner, Justin M. Langridge, Daniel A. Lack, Thilina Jayarathne, Elizabeth A. Stone, Chelsea E. Stockwell, Robert J. Yokelson, and Shane M. Murphy
Atmos. Chem. Phys., 16, 9549–9561, https://doi.org/10.5194/acp-16-9549-2016, https://doi.org/10.5194/acp-16-9549-2016, 2016
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This paper gives first multi-wavelength estimates of SSA and AAE of emissions from combustion of Indonesian peat. In addition, it demonstrates that SSA of biomass burning emissions can be parameterized with EC / (EC+OC) and that this parameterization is quantitatively superior to previously published parameterizations based on MCE. It also shows that EC / (EC+OC) parameterization accurately predicts SSA during the first few hours of aging of a biomass burning plume.
Franco Marenco, Ben Johnson, Justin M. Langridge, Jane Mulcahy, Angela Benedetti, Samuel Remy, Luke Jones, Kate Szpek, Jim Haywood, Karla Longo, and Paulo Artaxo
Atmos. Chem. Phys., 16, 2155–2174, https://doi.org/10.5194/acp-16-2155-2016, https://doi.org/10.5194/acp-16-2155-2016, 2016
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A widespread and persistent smoke layer was observed in the Amazon
region during the biomass burning season, spanning a distance of 2200 km
and a period of 14 days. The larger smoke content was typically found
in elevated layers, from 1–1.5 km to 4–6 km.
Measurements have been compared to model predictions, and the latter
were able to reproduce the general features of the smoke layer, but
with some differences which are analysed and described in the paper.
C. L. Ryder, J. B. McQuaid, C. Flamant, P. D. Rosenberg, R. Washington, H. E. Brindley, E. J. Highwood, J. H. Marsham, D. J. Parker, M. C. Todd, J. R. Banks, J. K. Brooke, S. Engelstaedter, V. Estelles, P. Formenti, L. Garcia-Carreras, C. Kocha, F. Marenco, H. Sodemann, C. J. T. Allen, A. Bourdon, M. Bart, C. Cavazos-Guerra, S. Chevaillier, J. Crosier, E. Darbyshire, A. R. Dean, J. R. Dorsey, J. Kent, D. O'Sullivan, K. Schepanski, K. Szpek, J. Trembath, and A. Woolley
Atmos. Chem. Phys., 15, 8479–8520, https://doi.org/10.5194/acp-15-8479-2015, https://doi.org/10.5194/acp-15-8479-2015, 2015
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Measurements of the Saharan atmosphere and of atmospheric mineral dust are lacking but are vital to our understanding of the climate of this region and their impacts further afield. Novel observations were made by the Fennec climate programme during June 2011 and 2012 using ground-based, remote sensing and airborne platforms. Here we describe the airborne observations and the contributions they have made to furthering our understanding of the Saharan climate system.
A. K. Vance, S. J. Abel, R. J. Cotton, and A. M. Woolley
Atmos. Meas. Tech., 8, 1617–1625, https://doi.org/10.5194/amt-8-1617-2015, https://doi.org/10.5194/amt-8-1617-2015, 2015
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Comparisons on the FAAM BAe 146-301 aircraft show good agreement between chilled mirror hygrometers and a WVSS-II fed from a modified Rosemount inlet (wvssR) in coud-free conditions, but a WVSS-II fed from the standard flush inlet (wvssF) over-reads, except at higher humidities. Case studies in cloudy conditions show that wvssF is immune to liquid water and ice, whilst wvssR is susceptible to both. Both WVSS-II inlets respond much more rapidly than the chilled mirror devices, especially wvssF.
G. Allen, S. M. Illingworth, S. J. O'Shea, S. Newman, A. Vance, S. J.-B. Bauguitte, F. Marenco, J. Kent, K. Bower, M. W. Gallagher, J. Muller, C. J. Percival, C. Harlow, J. Lee, and J. P. Taylor
Atmos. Meas. Tech., 7, 4401–4416, https://doi.org/10.5194/amt-7-4401-2014, https://doi.org/10.5194/amt-7-4401-2014, 2014
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This paper presents a validated method and data set for new retrievals of trace gas concentrations and temperature from the ARIES infrared spectrometer instrument on the UK Atmospheric Research Aircraft (www.faam.ac.uk). This new capability for the aircraft will allow new science to be done because of the way it can sense information about the atmosphere without having to physically pass through it (remote sensing). This will allow us to better understand the make-up of the lower atmosphere.
S. J. Abel, R. J. Cotton, P. A. Barrett, and A. K. Vance
Atmos. Meas. Tech., 7, 3007–3022, https://doi.org/10.5194/amt-7-3007-2014, https://doi.org/10.5194/amt-7-3007-2014, 2014
D. A. Lack and J. M. Langridge
Atmos. Chem. Phys., 13, 10535–10543, https://doi.org/10.5194/acp-13-10535-2013, https://doi.org/10.5194/acp-13-10535-2013, 2013
Related subject area
Subject: Others (Wind, Precipitation, Temperature, etc.) | Technique: In Situ Measurement | Topic: Instruments and Platforms
Method development and application for the analysis of chiral organic marker species in ice-cores
High-resolution wind speed measurements with quadcopter uncrewed aerial systems: calibration and verification in a wind tunnel with an active grid
High-altitude balloon-launched uncrewed aircraft system measurements of atmospheric turbulence and qualitative comparison with infrasound microphone response
Evaluation of the hyperspectral radiometer (HSR1) at the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site
Cost-effective off-grid automatic precipitation samplers for pollutant and biogeochemical atmospheric deposition
The ratio of transverse to longitudinal turbulent velocity statistics for aircraft measurements
Modelling of cup anemometry and dynamic overspeeding in average wind speed measurements
Introducing the Video In Situ Snowfall Sensor (VISSS)
Quality evaluation for measurements of wind field and turbulent fluxes from a UAV-based eddy covariance system
A new reference-quality precipitation gauge wind shield
Acquiring high-resolution wind measurements by modifying radiosonde sounding procedures
A new accurate low-cost instrument for fast synchronized spatial measurements of light spectra
Drone-based meteorological observations up to the tropopause – a concept study
A new airborne broadband radiometer system and an efficient method to correct dynamic thermal offsets
Toward quantifying turbulent vertical airflow and sensible heat flux in tall forest canopies using fiber-optic distributed temperature sensing
A fiber-optic distributed temperature sensor for continuous in situ profiling up to 2 km beneath constant-altitude scientific balloons
New Absolute Cavity Pyrgeometer equation by application of Kirchhoff's law and adding a convection term
The DataHawk2 uncrewed aircraft system for atmospheric research
The measurement of mean wind, variances, and covariances from an instrumented mobile car in a rural environment
ICE-CAMERA: a flatbed scanner to study inland Antarctic polar precipitation
3D trajectories and velocities of rainfall drops in a multifractal turbulent wind field
Towards vertical wind and turbulent flux estimation with multicopter uncrewed aircraft systems
Instabilities, Dynamics, and Energetics accompanying Atmospheric Layering (IDEAL): high-resolution in situ observations and modeling in and above the nocturnal boundary layer
Infrasound measurement system for real-time in situ tornado measurements
Quantifying the coastal urban surface layer structure using distributed temperature sensing in Helsinki, Finland
On the quality of RS41 radiosonde descent data
Idealized simulation study of the relationship of disdrometer sampling statistics with the precision of precipitation rate measurement
Use of thermal signal for the investigation of near-surface turbulence
Drone measurements of surface-based winter temperature inversions in the High Arctic at Eureka
Ground mobile observation system for measuring multisurface microwave emissivity
A differential emissivity imaging technique for measuring hydrometeor mass and type
Effect of snow-covered ground albedo on the accuracy of air temperature measurements
Distributed wind measurements with multiple quadrotor unmanned aerial vehicles in the atmospheric boundary layer
The INFRA-EAR: a low-cost mobile multidisciplinary measurement platform for monitoring geophysical parameters
A dedicated robust instrument for water vapor generation at low humidity for use with a laser water isotope analyzer in cold and dry polar regions
Arctic observations and numerical simulations of surface wind effects on Multi-Angle Snowflake Camera measurements
The development of the “Storm Tracker” and its applications for atmospheric high-resolution upper-air observations
Use of automatic radiosonde launchers to measure temperature and humidity profiles from the GRUAN perspective
Using global reanalysis data to quantify and correct airflow distortion bias in shipborne wind speed measurements
The CopterSonde: an insight into the development of a smart unmanned aircraft system for atmospheric boundary layer research
Microphysical properties and fall speed measurements of snow ice crystals using the Dual Ice Crystal Imager (D-ICI)
The Disdrometer Verification Network (DiVeN): a UK network of laser precipitation instruments
The new BELUGA setup for collocated turbulence and radiation measurements using a tethered balloon: first applications in the cloudy Arctic boundary layer
Identification of platform exhaust on the RV Investigator
Evaluation of Windsond S1H2 performance in Kumasi during the 2016 DACCIWA field campaign
Recovery of the three-dimensional wind and sonic temperature data from a physically deformed sonic anemometer
Considerations for temperature sensor placement on rotary-wing unmanned aircraft systems
New calibration procedures for airborne turbulence measurements and accuracy of the methane fluxes during the AirMeth campaigns
Is it feasible to estimate radiosonde biases from interlaced measurements?
Vertical wind velocity measurements using a five-hole probe with remotely piloted aircraft to study aerosol–cloud interactions
Johanna Schäfer, Anja Beschnitt, François Burgay, Thomas Singer, Margit Schwikowski, and Thorsten Hoffmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-2243, https://doi.org/10.5194/egusphere-2024-2243, 2024
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Glaciers preserve organic compounds from atmospheric aerosols, which can serve as markers for emission sources. Most studies overlook the enantiomers of chiral compounds. We developed a 2-dimensional liquid chromatography method to determine the chiral ratios of monoterpene oxidation products cis-pinic acid and cis-pinonic acid in ice-core samples. Applied to samples from the Belukha glacier (1870–1970 CE), the method revealed fluctuating chiral ratios for the analytes.
Johannes Kistner, Lars Neuhaus, and Norman Wildmann
Atmos. Meas. Tech., 17, 4941–4955, https://doi.org/10.5194/amt-17-4941-2024, https://doi.org/10.5194/amt-17-4941-2024, 2024
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We use a fleet of multicopter drones to measure wind. To improve the accuracy of this wind measurement and to evaluate this improvement, we conducted experiments with the drones in a wind tunnel under various conditions. This wind tunnel can generate different kinds and intensities of wind. Here we measured with the drones and with other sensors as a reference and compared the results. We were able to improve our wind measurement and show how accurately it works in different situations.
Anisa N. Haghighi, Ryan D. Nolin, Gary D. Pundsack, Nick Craine, Aliaksei Stratsilatau, and Sean C. C. Bailey
Atmos. Meas. Tech., 17, 4863–4889, https://doi.org/10.5194/amt-17-4863-2024, https://doi.org/10.5194/amt-17-4863-2024, 2024
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This work summarizes measurements conducted in June 2021 using a small, uncrewed, stratospheric glider that was launched from a weather balloon to altitudes up to 30 km above sea level. The aircraft conducted measurements of wind speed and direction, pressure, temperature, and humidity during its descent as well as measurements of infrasonic sound levels. These data were used to evaluate the atmospheric turbulence observed during the descent phase of the flight.
Kelly A. Balmes, Laura D. Riihimaki, John Wood, Connor Flynn, Adam Theisen, Michael Ritsche, Lynn Ma, Gary B. Hodges, and Christian Herrera
Atmos. Meas. Tech., 17, 3783–3807, https://doi.org/10.5194/amt-17-3783-2024, https://doi.org/10.5194/amt-17-3783-2024, 2024
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A new hyperspectral radiometer (HSR1) was deployed and evaluated in the central United States (northern Oklahoma). The HSR1 total spectral irradiance agreed well with nearby existing instruments, but the diffuse spectral irradiance was slightly smaller. The HSR1-retrieved aerosol optical depth (AOD) also agreed well with other retrieved AODs. The HSR1 performance is encouraging: new hyperspectral knowledge is possible that could inform atmospheric process understanding and weather forecasting.
Alessia A. Colussi, Daniel Persaud, Melodie Lao, Bryan K. Place, Rachel F. Hems, Susan E. Ziegler, Kate A. Edwards, Cora J. Young, and Trevor C. VandenBoer
Atmos. Meas. Tech., 17, 3697–3718, https://doi.org/10.5194/amt-17-3697-2024, https://doi.org/10.5194/amt-17-3697-2024, 2024
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A new modular and affordable instrument was developed to automatically collect wet deposition continuously with an off-grid solar top-up power package. Monthly collections were performed across the Newfoundland and Labrador Boreal Ecosystem Latitudinal Transect of experimental forest sites from 2015 to 2016. The proof-of-concept systems were validated with baseline measurements of pH and conductivity and then applied to dissolved organic carbon as an analyte of emerging biogeochemical interest.
Jakub L. Nowak, Marie Lothon, Donald H. Lenschow, and Szymon P. Malinowski
EGUsphere, https://doi.org/10.5194/egusphere-2024-1366, https://doi.org/10.5194/egusphere-2024-1366, 2024
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According to a classical theory, the ratio of turbulence statistics corresponding to transverse and longitudinal wind velocity components equals 4/3 in the inertial range of scales. We analyze large amount of measurements obtained with three research aircraft during four field experiments in different locations and show the observed ratios are almost always significantly smaller. We discuss potential reasons of this disagreement but actual explanation remains to be determined.
Troels Friis Pedersen and Jan-Åke Dahlberg
Atmos. Meas. Tech., 17, 1441–1461, https://doi.org/10.5194/amt-17-1441-2024, https://doi.org/10.5194/amt-17-1441-2024, 2024
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Accuracy is important in wind speed measurements with cup anemometers. Dynamic overspeeding is historically considered an inherent and significant error, supported by a two-cup drag model. But lower (and even zero) overspeeding might be present for low-to-medium turbulence intensities for conical cups with short arms. A parabolic torque model reveals various dynamic overspeeding characteristics of cup anemometers, but modelling of actual cup anemometers is best made with tabulated data.
Maximilian Maahn, Dmitri Moisseev, Isabelle Steinke, Nina Maherndl, and Matthew D. Shupe
Atmos. Meas. Tech., 17, 899–919, https://doi.org/10.5194/amt-17-899-2024, https://doi.org/10.5194/amt-17-899-2024, 2024
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The open-source Video In Situ Snowfall Sensor (VISSS) is a novel instrument for characterizing particle shape, size, and sedimentation velocity in snowfall. It combines a large observation volume with relatively high resolution and a design that limits wind perturbations. The open-source nature of the VISSS hardware and software invites the community to contribute to the development of the instrument, which has many potential applications in atmospheric science and beyond.
Yibo Sun, Bilige Sude, Xingwen Lin, Bing Geng, Bo Liu, Shengnan Ji, Junping Jing, Zhiping Zhu, Ziwei Xu, Shaomin Liu, and Zhanjun Quan
Atmos. Meas. Tech., 16, 5659–5679, https://doi.org/10.5194/amt-16-5659-2023, https://doi.org/10.5194/amt-16-5659-2023, 2023
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Unoccupied aerial vehicles (UAVs) provide a versatile platform for eddy covariance (EC) flux measurements at regional scales with low cost, transport, and infrastructural requirements. This study evaluates the measurement performance in the wind field and turbulent flux of a UAV-based EC system based on the data from a set of calibration flights and standard operational flights and concludes that the system can measure the georeferenced wind vector and turbulent flux with sufficient precision.
John Kochendorfer, Tilden P. Meyers, Mark E. Hall, Scott D. Landolt, Justin Lentz, and Howard J. Diamond
Atmos. Meas. Tech., 16, 5647–5657, https://doi.org/10.5194/amt-16-5647-2023, https://doi.org/10.5194/amt-16-5647-2023, 2023
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A new wind shield has been designed to reduce the effects of precipitation gauge undercatch. Tested at three separate sites, it compared well to a well-established refence-quality precipitation wind shield. The new wind shield is smaller and more durable than other reference-quality shields, and it was designed for use in operational weather and climate networks.
Jens Faber, Michael Gerding, and Torsten Köpnick
Atmos. Meas. Tech., 16, 4183–4193, https://doi.org/10.5194/amt-16-4183-2023, https://doi.org/10.5194/amt-16-4183-2023, 2023
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Weather forecasters around the world use uncrewed balloons to measure wind and temperature for their weather models. In these measurements, wind is recorded from the shift of the balloon by the moving air. However, the balloons and the measurement devices also move by themselves in still air. This creates artificial wind measurements that are normally removed from the data. We show new techniques to avoid these movements and increase the altitude resolution of the wind measurement by 6 times.
Bert G. Heusinkveld, Wouter B. Mol, and Chiel C. van Heerwaarden
Atmos. Meas. Tech., 16, 3767–3785, https://doi.org/10.5194/amt-16-3767-2023, https://doi.org/10.5194/amt-16-3767-2023, 2023
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This paper presents a new instrument for fast measurements of solar irradiance in 18 wavebands (400–950 nm): GPS perfectly synchronizes 10 Hz measurement speed to universal time, low-cost (< EUR 200) complete standalone solution for realizing dense measurement grids to study cloud-shading dynamics, 940 nm waveband reveals atmospheric moisture column information, 11 wavebands to study photosynthetic active radiation and light interaction with vegetation, and good reflection spectra performance.
Konrad B. Bärfuss, Holger Schmithüsen, and Astrid Lampert
Atmos. Meas. Tech., 16, 3739–3765, https://doi.org/10.5194/amt-16-3739-2023, https://doi.org/10.5194/amt-16-3739-2023, 2023
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The first atmospheric soundings with an electrically powered small uncrewed aircraft system (UAS) up to an altitude of 10 km are presented and assessed for quality, revealing the potential to augment atmospheric observations and fill observation gaps for numerical weather prediction. This is significant because of the need for high-resolution meteorological data, in particular in remote areas with limited in situ measurements, and for reference data for satellite measurement calibration.
André Ehrlich, Martin Zöger, Andreas Giez, Vladyslav Nenakhov, Christian Mallaun, Rolf Maser, Timo Röschenthaler, Anna E. Luebke, Kevin Wolf, Bjorn Stevens, and Manfred Wendisch
Atmos. Meas. Tech., 16, 1563–1581, https://doi.org/10.5194/amt-16-1563-2023, https://doi.org/10.5194/amt-16-1563-2023, 2023
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Measurements of the broadband radiative energy budget from aircraft are needed to study the effect of clouds, aerosol particles, and surface conditions on the Earth's energy budget. However, the moving aircraft introduces challenges to the instrument performance and post-processing of the data. This study introduces a new radiometer package, outlines a greatly simplifying method to correct thermal offsets, and provides exemplary measurements of solar and thermal–infrared irradiance.
Mohammad Abdoli, Karl Lapo, Johann Schneider, Johannes Olesch, and Christoph K. Thomas
Atmos. Meas. Tech., 16, 809–824, https://doi.org/10.5194/amt-16-809-2023, https://doi.org/10.5194/amt-16-809-2023, 2023
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In this study, we compute the distributed sensible heat flux using a distributed temperature sensing technique, whose magnitude, sign, and temporal dynamics compare reasonably well to estimates from classical eddy covariance measurements from sonic anemometry. Despite the remaining uncertainty in computed fluxes, the results demonstrate the potential of the novel method to compute spatially resolving sensible heat flux measurement and encourage further research.
J. Douglas Goetz, Lars E. Kalnajs, Terry Deshler, Sean M. Davis, Martina Bramberger, and M. Joan Alexander
Atmos. Meas. Tech., 16, 791–807, https://doi.org/10.5194/amt-16-791-2023, https://doi.org/10.5194/amt-16-791-2023, 2023
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An instrument for in situ continuous 2 km vertical profiles of temperature below high-altitude balloons was developed for high-temporal-resolution measurements within the upper troposphere and lower stratosphere using fiber-optic distributed temperature sensing. The mechanical, electrical, and temperature calibration systems were validated from a short mid-latitude constant-altitude balloon flight within the lower stratosphere. The instrument observed small-scale and inertial gravity waves.
Bruce W. Forgan, Julian Gröbner, and Ibrahim Reda
Atmos. Meas. Tech., 16, 727–743, https://doi.org/10.5194/amt-16-727-2023, https://doi.org/10.5194/amt-16-727-2023, 2023
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This paper investigates the Absolute Cavity Pyrgeometer (ACP) and its use in measuring atmospheric terrestrial irradiances traceable to the standard system of units (SI). This work fits into the objective of the Expert Team on Radiation References, established by the World Meteorological Organization (WMO), to develop and validate instrumentation that can be used as reference instruments for terrestrial radiation measurements.
Jonathan Hamilton, Gijs de Boer, Abhiram Doddi, and Dale A. Lawrence
Atmos. Meas. Tech., 15, 6789–6806, https://doi.org/10.5194/amt-15-6789-2022, https://doi.org/10.5194/amt-15-6789-2022, 2022
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The DataHawk2 is a small, low-cost, rugged, uncrewed aircraft system (UAS) used to observe the thermodynamic and turbulence structures of the lower atmosphere, supporting an advanced understanding of the physical processes that regulate weather and climate. This paper discusses the development, performance, and sensing capabilities of the DataHawk2 using data collected during several recent field deployments.
Stefan J. Miller and Mark Gordon
Atmos. Meas. Tech., 15, 6563–6584, https://doi.org/10.5194/amt-15-6563-2022, https://doi.org/10.5194/amt-15-6563-2022, 2022
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This research investigates the measurement of atmospheric turbulence using a low-cost instrumented car that travels at near-highway speeds and is impacted by upwind obstructions and other on-road traffic. We show that our car design can successfully measure the mean flow and atmospheric turbulence near the surface. We outline a technique to isolate and remove the effects of sporadic passing traffic from car-measured velocity variances and discuss potential measurement uncertainties.
Massimo Del Guasta
Atmos. Meas. Tech., 15, 6521–6544, https://doi.org/10.5194/amt-15-6521-2022, https://doi.org/10.5194/amt-15-6521-2022, 2022
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Any instrument on the Antarctic plateau must cope with a harsh environment. Concordia station is a special place for testing new instruments. With low temperatures and weak winds, precipitation can be studied by simply collecting it on horizontal surfaces. This is typically done manually. ICE-CAMERA is intended as an automatic alternative. The combined construction of rugged equipment for taking photographs of particles and the adoption of machine learning techniques have served this purpose.
Auguste Gires, Ioulia Tchiguirinskaia, and Daniel Schertzer
Atmos. Meas. Tech., 15, 5861–5875, https://doi.org/10.5194/amt-15-5861-2022, https://doi.org/10.5194/amt-15-5861-2022, 2022
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Weather radars measure rainfall in altitude whereas hydro-meteorologists are mainly interested in rainfall at ground level. During their fall, drops are advected by the wind which affects the location of the measured field. Governing equation linking acceleration, gravity, buoyancy, and drag force is updated to account for oblateness of drops. Then multifractal wind is used as input to explore velocities and trajectories of drops. Finally consequence on radar rainfall estimation is discussed.
Norman Wildmann and Tamino Wetz
Atmos. Meas. Tech., 15, 5465–5477, https://doi.org/10.5194/amt-15-5465-2022, https://doi.org/10.5194/amt-15-5465-2022, 2022
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Multicopter uncrewed aerial systems (UAS, also known as drones) are very easy to use systems for collecting data in the lowest part of the atmosphere. Wind and turbulence are parameters that are particularly important for understanding the dynamics in the atmosphere. Only with three-dimensional measurements of the wind can a full understanding can be achieved. In this study, we show how even the vertical wind through the UAS can be measured with good accuracy.
Abhiram Doddi, Dale Lawrence, David Fritts, Ling Wang, Thomas Lund, William Brown, Dragan Zajic, and Lakshmi Kantha
Atmos. Meas. Tech., 15, 4023–4045, https://doi.org/10.5194/amt-15-4023-2022, https://doi.org/10.5194/amt-15-4023-2022, 2022
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Small-scale turbulent structures are ubiquitous in the atmosphere, yet our understanding of their structure and dynamics is vastly incomplete. IDEAL aimed to improve our understanding of small-scale turbulent flow features in the lower atmosphere. A small, unmanned, fixed-wing aircraft was employed to make targeted observations of atmospheric columns. Measured data were used to guide atmospheric model simulations designed to describe the structure and dynamics of small-scale turbulence.
Brandon C. White, Brian R. Elbing, and Imraan A. Faruque
Atmos. Meas. Tech., 15, 2923–2938, https://doi.org/10.5194/amt-15-2923-2022, https://doi.org/10.5194/amt-15-2923-2022, 2022
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Tornadic storms have been hypothesized to emit sound at frequencies below human hearing which animals and certain microphones can detect. This study covers the design, fabrication, and deployment of a specialized microphone that can be carried by first responders and storm chasers. The study also presents real-time processing methods, analyzes several recorded severe weather events including a tornado, and introduces a real-time web interface to allow for live monitoring of the mobile sensor.
Sasu Karttunen, Ewan O'Connor, Olli Peltola, and Leena Järvi
Atmos. Meas. Tech., 15, 2417–2432, https://doi.org/10.5194/amt-15-2417-2022, https://doi.org/10.5194/amt-15-2417-2022, 2022
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To study the complex structure of the lowest tens of metres of atmosphere in urban areas, measurement methods with great spatial and temporal coverage are needed. In our study, we analyse measurements with a promising and relatively new method, distributed temperature sensing, capable of providing detailed information on the near-surface atmosphere. We present multiple ways to utilise these kinds of measurements, as well as important considerations for planning new studies using the method.
Bruce Ingleby, Martin Motl, Graeme Marlton, David Edwards, Michael Sommer, Christoph von Rohden, Holger Vömel, and Hannu Jauhiainen
Atmos. Meas. Tech., 15, 165–183, https://doi.org/10.5194/amt-15-165-2022, https://doi.org/10.5194/amt-15-165-2022, 2022
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Radiosonde descent data could provide extra profiles of the atmosphere for forecasting and other uses. Descent data from Vaisala RS41 radiosondes have been compared with the ascent profiles and with ECMWF short-range forecasts. The agreement is mostly good. The descent rate is very variable and high descent rates cause temperature biases, especially at upper levels. Ascent winds are affected by pendulum motion; on average, the descent winds are smoother.
Karlie N. Rees and Timothy J. Garrett
Atmos. Meas. Tech., 14, 7681–7691, https://doi.org/10.5194/amt-14-7681-2021, https://doi.org/10.5194/amt-14-7681-2021, 2021
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Monte Carlo simulations are used to establish baseline precipitation measurement uncertainties according to World Meteorological Organization standards. Measurement accuracy depends on instrument sampling area, time interval, and precipitation rate. Simulations are compared with field measurements taken by an emerging hotplate precipitation sensor. We find that the current collection area is sufficient for light rain, but a larger collection area is required to detect moderate to heavy rain.
Matthias Zeeman
Atmos. Meas. Tech., 14, 7475–7493, https://doi.org/10.5194/amt-14-7475-2021, https://doi.org/10.5194/amt-14-7475-2021, 2021
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Understanding turbulence near the surface is important for many applications. In this work, methods for observing and analysing temperature structures in a near-surface volume were explored. Experiments were conducted to identify modes of organised motion. These help explain interactions between the vegetation and the atmosphere that are not currently well understood. Techniques used include fibre-optic sensing, thermal infrared imaging, signal decomposition, and machine learning.
Alexey B. Tikhomirov, Glen Lesins, and James R. Drummond
Atmos. Meas. Tech., 14, 7123–7145, https://doi.org/10.5194/amt-14-7123-2021, https://doi.org/10.5194/amt-14-7123-2021, 2021
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Two commercial quadcopters (DJI Matrice 100 and M210 RTK) were equipped with an air temperature measurement system. They were flown at the Polar Environment Atmospheric Research Laboratory, Eureka, Nunavut, Canada, at 80° N latitude to study surface-based temperature inversion during February–March field campaigns in 2017 and 2020. It was demonstrated that the drones can be effectively used in the High Arctic to measure vertical temperature profiles up to 75 m off the ground.
Wenying He, Hongbin Chen, Yuejian Xuan, Jun Li, Minzheng Duan, and Weidong Nan
Atmos. Meas. Tech., 14, 7069–7078, https://doi.org/10.5194/amt-14-7069-2021, https://doi.org/10.5194/amt-14-7069-2021, 2021
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Large microwave surface emissivities (ε) cause difficulties in widely using satellite microwave data over land. Usually, ground-based radiometers are fixed to a scan field to obtain the temporal evolution of ε over a single land-cover area. To obtain the long-term temporal evolution of ε over different land-cover surfaces simultaneously, we developed a ground mobile observation system to enhance in situ ε observations and presented some preliminary results.
Dhiraj K. Singh, Spencer Donovan, Eric R. Pardyjak, and Timothy J. Garrett
Atmos. Meas. Tech., 14, 6973–6990, https://doi.org/10.5194/amt-14-6973-2021, https://doi.org/10.5194/amt-14-6973-2021, 2021
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This paper describes a new instrument for quantifying the physical characteristics of hydrometeors such as snow and rain. The device can measure the mass, size, density and type of individual hydrometeors as well as their bulk properties. The instrument is called the Differential Emissivity Imaging Disdrometer (DEID) and is composed of a thermal camera and hotplate. The DEID measures hydrometeors at sampling frequencies up to 1 Hz with masses and effective diameters greater than 1 µg and 200 µm.
Chiara Musacchio, Graziano Coppa, Gaber Begeš, Christina Hofstätter-Mohler, Laura Massano, Guido Nigrelli, Francesca Sanna, and Andrea Merlone
Atmos. Meas. Tech., 14, 6195–6212, https://doi.org/10.5194/amt-14-6195-2021, https://doi.org/10.5194/amt-14-6195-2021, 2021
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In the context of the overhaul of the WMO/CIMO guide (no. 8) on instruments and methods of observation, we performed an experiment to quantify uncertainties in air temperature measurements due to reflected solar radiation from a snow-covered surface. Coupled sensors with different radiation shields were put under different ground conditions (grass vs. snow) for a whole winter. Results show that different shields may reduce the influence of backward radiation, which can produce errors up to 3 °C.
Tamino Wetz, Norman Wildmann, and Frank Beyrich
Atmos. Meas. Tech., 14, 3795–3814, https://doi.org/10.5194/amt-14-3795-2021, https://doi.org/10.5194/amt-14-3795-2021, 2021
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A fleet of quadrotors is presented as a system to measure the spatial distribution of atmospheric boundary layer flow. The big advantage of this approach is that multiple and flexible measurement points in space can be sampled synchronously. The algorithm to calculate the horizontal wind is based on the principle of aerodynamic drag and the related quadrotor dynamics. The validation reveals that an average accuracy of < 0.3 m s−1 for the wind speed and < 8° for the wind direction was achieved.
Olivier F. C. den Ouden, Jelle D. Assink, Cornelis D. Oudshoorn, Dominique Filippi, and Läslo G. Evers
Atmos. Meas. Tech., 14, 3301–3317, https://doi.org/10.5194/amt-14-3301-2021, https://doi.org/10.5194/amt-14-3301-2021, 2021
Christophe Leroy-Dos Santos, Mathieu Casado, Frédéric Prié, Olivier Jossoud, Erik Kerstel, Morgane Farradèche, Samir Kassi, Elise Fourré, and Amaëlle Landais
Atmos. Meas. Tech., 14, 2907–2918, https://doi.org/10.5194/amt-14-2907-2021, https://doi.org/10.5194/amt-14-2907-2021, 2021
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We developed an instrument that can generate water vapor at low humidity at a very stable level. This instrument was conceived to calibrate water vapor isotopic records obtained in very dry places such as central Antarctica. Here, we provide details on the instrument as well as results obtained for correcting water isotopic records for diurnal variability during a long field season at the Concordia station in East Antarctica.
Kyle E. Fitch, Chaoxun Hang, Ahmad Talaei, and Timothy J. Garrett
Atmos. Meas. Tech., 14, 1127–1142, https://doi.org/10.5194/amt-14-1127-2021, https://doi.org/10.5194/amt-14-1127-2021, 2021
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Snow measurements are very sensitive to wind. Here, we compare airflow and snowfall simulations to Arctic observations for a Multi-Angle Snowflake Camera to show that measurements of fall speed, orientation, and size are accurate only with a double wind fence and winds below 5 m s−1. In this case, snowflakes tend to fall with a nearly horizontal orientation; the largest flakes are as much as 5 times more likely to be observed. Adjustments are needed for snow falling in naturally turbulent air.
Wei-Chun Hwang, Po-Hsiung Lin, and Hungjui Yu
Atmos. Meas. Tech., 13, 5395–5406, https://doi.org/10.5194/amt-13-5395-2020, https://doi.org/10.5194/amt-13-5395-2020, 2020
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We have developed a small, light-weight (radiosonde of 20 g with battery), low-cost, and easy-to-use upper-air radiosonde system: the Storm Tracker. With the ability to receive multiple radiosondes simultaneously, the system enables high temporal and spatial resolution atmospheric observations. In the 2018 field campaign, the accuracy of the Storm tracker was tested using co-launched data with Vaisala RS41-SGP radiosondes, and the measurements show an overall good agreement.
Fabio Madonna, Rigel Kivi, Jean-Charles Dupont, Bruce Ingleby, Masatomo Fujiwara, Gonzague Romanens, Miguel Hernandez, Xavier Calbet, Marco Rosoldi, Aldo Giunta, Tomi Karppinen, Masami Iwabuchi, Shunsuke Hoshino, Christoph von Rohden, and Peter William Thorne
Atmos. Meas. Tech., 13, 3621–3649, https://doi.org/10.5194/amt-13-3621-2020, https://doi.org/10.5194/amt-13-3621-2020, 2020
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Radiosondes are one of the primary sources of upper-air data for weather and climate monitoring. In the last two decades, technological progress made available automated radiosonde launchers (ARLs), which are able to replace measurements typically performed manually. This work presents a comparative analysis of the technical performance of the ARLs currently available on the market and contribute to define a strategy to achieve the full traceability of the ARL products.
Sebastian Landwehr, Iris Thurnherr, Nicolas Cassar, Martin Gysel-Beer, and Julia Schmale
Atmos. Meas. Tech., 13, 3487–3506, https://doi.org/10.5194/amt-13-3487-2020, https://doi.org/10.5194/amt-13-3487-2020, 2020
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Shipborne wind speed measurements are relevant for field studies of air–sea interaction processes. Distortion of the airflow by the ship’s structure can, however, lead to errors. We estimate the flow distortion bias by comparing the observations to ERA-5 reanalysis data. The underlying assumptions are that the bias depends only on the relative orientation of the ship to the wind direction and that the ERA-5 wind speeds are (on average) representative of the true wind speed.
Antonio R. Segales, Brian R. Greene, Tyler M. Bell, William Doyle, Joshua J. Martin, Elizabeth A. Pillar-Little, and Phillip B. Chilson
Atmos. Meas. Tech., 13, 2833–2848, https://doi.org/10.5194/amt-13-2833-2020, https://doi.org/10.5194/amt-13-2833-2020, 2020
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The CopterSonde is an unmanned aircraft system designed with the purpose of sampling thermodynamic and kinematic parameters of the lower Earth's atmosphere, with a focus on vertical profiles in the planetary boundary layer. By incorporating adaptive sampling techniques and optimizing the sensor placement, our study shows that CopterSonde can provide similar information as a radiosonde, but with more control of its sampling location at much higher temporal and spatial resolution.
Thomas Kuhn and Sandra Vázquez-Martín
Atmos. Meas. Tech., 13, 1273–1285, https://doi.org/10.5194/amt-13-1273-2020, https://doi.org/10.5194/amt-13-1273-2020, 2020
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Directly measured shape and fall speed are two important parameters needed for models and remote sensing. This can be done by the new Dual Ice Crystal Imager (D-ICI) instrument, which takes two high-resolution pictures of falling snow crystals from two different angles. Fall speed is measured by doubly exposing the side-view picture. Size and shape are determined from the second picture providing the top view of the snow crystal. D-ICI has been tested on the ground in Kiruna, northern Sweden.
Ben S. Pickering, Ryan R. Neely III, and Dawn Harrison
Atmos. Meas. Tech., 12, 5845–5861, https://doi.org/10.5194/amt-12-5845-2019, https://doi.org/10.5194/amt-12-5845-2019, 2019
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A new network of precipitation instruments has been established for the UK. The instruments are capable of detecting the fall velocity and diameter of each particle that falls through a laser beam. The particle characteristics are derived from the duration and amount of decrease in beam brightness as perceived by a receiving diode. A total of 14 instruments make up the network and all instruments upload 60 s frequency data in near-real time to a publicly available website with plots.
Ulrike Egerer, Matthias Gottschalk, Holger Siebert, André Ehrlich, and Manfred Wendisch
Atmos. Meas. Tech., 12, 4019–4038, https://doi.org/10.5194/amt-12-4019-2019, https://doi.org/10.5194/amt-12-4019-2019, 2019
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In this study, we introduce the new tethered balloon system BELUGA, which includes different modular instrument packages for measuring turbulence and radiation in the atmospheric boundary layer. BELUGA was deployed in an Arctic field campaign in 2017, providing details of boundary layer processes in combination with low-level clouds. Those processes are still not fully understood and in situ measurements in the Arctic improve our understanding of the Arctic response in terms of global warming.
Ruhi S. Humphries, Ian M. McRobert, Will A. Ponsonby, Jason P. Ward, Melita D. Keywood, Zoe M. Loh, Paul B. Krummel, and James Harnwell
Atmos. Meas. Tech., 12, 3019–3038, https://doi.org/10.5194/amt-12-3019-2019, https://doi.org/10.5194/amt-12-3019-2019, 2019
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Undertaking atmospheric observations from ships provides important data in regions where measurements are impossible by other means. However, making measurements so close to a diesel exhaust plume is difficult. In this paper, we describe an algorithm that utilises ongoing measurements of aerosol number concentrations, black carbon mass concentrations, and mixing ratios of carbon monoxide and carbon dioxide to accurately distinguish between exhaust and background data periods.
Geoffrey Elie Quentin Bessardon, Kwabena Fosu-Amankwah, Anders Petersson, and Barbara Jane Brooks
Atmos. Meas. Tech., 12, 1311–1324, https://doi.org/10.5194/amt-12-1311-2019, https://doi.org/10.5194/amt-12-1311-2019, 2019
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This paper presents the first performance assessment during a field campaign of a new reusable radiosonde: the Windsond S1H2. The reuse feature of the S1H2 requires evaluation of the data alteration due to sonde reuse in addition to performance and reproducibility assessments. A comparison with the Vaisala RS41-SG, a well-proven system, shows the potential of the S1H2, with no major performance degradation arising from S1H2 sonde reuse but shows the need for improving the S1H2 GPS system.
Xinhua Zhou, Qinghua Yang, Xiaojie Zhen, Yubin Li, Guanghua Hao, Hui Shen, Tian Gao, Yirong Sun, and Ning Zheng
Atmos. Meas. Tech., 11, 5981–6002, https://doi.org/10.5194/amt-11-5981-2018, https://doi.org/10.5194/amt-11-5981-2018, 2018
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The three-dimensional wind and sonic temperature data from a physically deformed sonic anemometer was successfully recovered by developing equations, algorithms, and related software. Using two sets of geometry data from production calibration and return re-calibration, this algorithm can recover wind with/without transducer shadow correction and sonic temperature with crosswind correction, and then obtain fluxes at quality as expected. This study is applicable as a reference for related topics.
Brian R. Greene, Antonio R. Segales, Sean Waugh, Simon Duthoit, and Phillip B. Chilson
Atmos. Meas. Tech., 11, 5519–5530, https://doi.org/10.5194/amt-11-5519-2018, https://doi.org/10.5194/amt-11-5519-2018, 2018
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With the recent commercial availability of rotary-wing unmanned aircraft systems (rwUAS), their ability to collect observations in the lower atmosphere is quickly being realized. However, integrating sensors with an rwUAS can introduce errors if not sited properly. This study discusses an objective method of determining some of these error sources in temperature, including improper airflow and rotary motor heating. Errors can be mitigated by mounting thermistors under propellers near the tips.
Jörg Hartmann, Martin Gehrmann, Katrin Kohnert, Stefan Metzger, and Torsten Sachs
Atmos. Meas. Tech., 11, 4567–4581, https://doi.org/10.5194/amt-11-4567-2018, https://doi.org/10.5194/amt-11-4567-2018, 2018
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We present new in-flight calibration procedures for airborne turbulence measurements that exploit suitable regular flight legs without the need for dedicated calibration patterns. Furthermore we estimate the accuracy of the airborne wind measurement and of the turbulent fluxes of the traces gases methane and carbon dioxide.
Stefanie Kremser, Jordis S. Tradowsky, Henning W. Rust, and Greg E. Bodeker
Atmos. Meas. Tech., 11, 3021–3029, https://doi.org/10.5194/amt-11-3021-2018, https://doi.org/10.5194/amt-11-3021-2018, 2018
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We investigate the feasibility of quantifying the difference in biases of two instrument types (i.e. radiosondes) by flying the old and new instruments on alternating days, so-called interlacing, to statistically derive the systematic biases between the instruments. While it is in principle possible to estimate the difference between two instrument biases from interlaced measurements, the number of required interlaced flights is very large for reasonable autocorrelation coefficient values.
Radiance Calmer, Gregory C. Roberts, Jana Preissler, Kevin J. Sanchez, Solène Derrien, and Colin O'Dowd
Atmos. Meas. Tech., 11, 2583–2599, https://doi.org/10.5194/amt-11-2583-2018, https://doi.org/10.5194/amt-11-2583-2018, 2018
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Remotely piloted aircraft systems (RPAS), commonly called UAVs, are used in atmospheric science for in situ measurements. The presented work shows wind measurements from a five-hole probe on an RPAS. Comparisons with other instruments (sonic anemometer and cloud radar) show good agreement, validating the RPAS measurements. In situ vertical wind measurements at cloud base are highlighted because they are a major parameter needed for simulating aerosol–cloud interactions, though rarely collected.
Cited articles
Air Quality Expert Group: Fine Particulate Matter (PM2.5) in the United
Kingdom, Department for Environment Food and Rural Affairs (DEFRA), https://uk-air.defra.gov.uk/assets/documents/reports/cat11/1212141150_AQEG_Fine_Particulate_Matter_in_the_UK.pdf (last access: 15 February 2021), 2012.
Air Quality Expert Group: Estimation of changes in air pollution emissions,
concentrations and exposure during the COVID-19 outbreak in the UK, UK Air
Inf. Resour., 1–57, https://uk-air.defra.gov.uk/assets/documents/reports/cat09/2007010844_Estimation_of_Changes_in_Air_Pollution_During_COVID-19_outbreak_in_the_UK.pdf (last access: 6 January 2021), 2020.
Bates, K. H. and Jacob, D. J.: An Expanded Definition of the Odd Oxygen
Family for Tropospheric Ozone Budgets: Implications for Ozone Lifetime and
Stratospheric In fl uence Geophysical Research Letters, Geophys. Res. Lett.,
47, e2019GL084486, https://doi.org/10.1029/2019GL084486, 2019.
Beecken, J., Mellqvist, J., Salo, K., Ekholm, J., and Jalkanen, J.-P.: Airborne emission measurements of SO2, NOx and particles from individual ships using a sniffer technique, Atmos. Meas. Tech., 7, 1957–1968, https://doi.org/10.5194/amt-7-1957-2014, 2014.
Bond, T. C. and Bergstrom, R. W.: Light absorption by carbonaceous
particles: An investigative review, Aerosol Sci. Tech., 40, 27–67,
https://doi.org/10.1080/02786820500421521, 2006.
Bond, T. C., Anderson, T. L., and Campbell, D.: Calibration and
Intercomparison of Filter-Based Measurements of Visible Light Absorption by
Aerosols, Aerosol Sci. Tech., 30, 582–600,
https://doi.org/10.1080/027868299304435, 1999.
Brechtel Manufacturing Inc: Model 1200 Isokinetic Aerosol Inlet System
Manual ver. 8.0, manual, 2011.
Crilley, L. R., Singh, A., Kramer, L. J., Shaw, M. D., Alam, M. S., Apte, J. S., Bloss, W. J., Hildebrandt Ruiz, L., Fu, P., Fu, W., Gani, S., Gatari, M., Ilyinskaya, E., Lewis, A. C., Ng'ang'a, D., Sun, Y., Whitty, R. C. W., Yue, S., Young, S., and Pope, F. D.: Effect of aerosol composition on the performance of low-cost optical particle counter correction factors, Atmos. Meas. Tech., 13, 1181–1193, https://doi.org/10.5194/amt-13-1181-2020, 2020.
Dassios, K. G. and Pandis, S. N.: The mass accommodation coefficient of
ammonium nitrate aerosol, Atmos. Environ., 33, 2993–3003,
https://doi.org/10.1016/S1352-2310(99)00079-5, 1999.
Davies, N. W., Fox, C., Szpek, K., Cotterell, M. I., Taylor, J. W., Allan, J. D., Williams, P. I., Trembath, J., Haywood, J. M., and Langridge, J. M.: Evaluating biases in filter-based aerosol absorption measurements using photoacoustic spectroscopy, Atmos. Meas. Tech., 12, 3417–3434, https://doi.org/10.5194/amt-12-3417-2019, 2019.
DEFRA: Clean air strategy 2019, DEFRA, https://www.gov.uk/government/publications/clean-air-strategy-2019 (last access: 12 June 2020), 2019.
Denby, B., Cassiani, M., De Smet, P., De Leeuw, F., and Horálek, J.:
Sub-grid variability and its impact on European wide air quality exposure
assessment, Atmos. Environ., 45, 4220–4229,
https://doi.org/10.1016/j.atmosenv.2011.05.007, 2011.
Dewline: DewLine™, Dewline, https://twobtech.com/dewline.html, last access: 15 May 2020.
Ecotech: Aurora3000 Integrating Nephelometer with backscatter, user manual
v1.3, Ecotech, 2009.
El-Harbawi, M.: Air quality modelling, simulation, and computational
methods: a review, Environ. Rev., 21, 149–179, https://doi.org/10.1139/er-2012-0056, 2013.
Environment Agency: Automatic Urban and Rural Network (AURN) LSO Manual, Version 1.2, Environment Agency, https://uk-air.defra.gov.uk/assets/documents/reports/empire/lsoman/lsoman.html (last access: 13 September 2023), 2022.
Fleming, R. J.: The use of commercial aircraft as platforms for environmental measurements, B. Amer. Meteorol. Soc., 77, 2229–2242, 1996.
Frie, A. L. and Bahreini, R.: Refractive index confidence explorer (RICE): A
tool for propagating uncertainties through complex refractive index
retrievals from aerosol particles, Aerosol Sci. Tech., 55, 703–717,
https://doi.org/10.1080/02786826.2021.1895428, 2021.
Fuchs, N. A. and Sutugin, A. G.: High-dispersed aerosols, in: International Reviews in Aerosol Physics and Chemistry, Topics in Current Aerosol Research,
edited by: Hidy, G. M. and Brock, J. R., Pergamon, https://doi.org/10.1016/B978-0-08-016674-2.50006-6, 1971.
Gao, R. S., Telg, H., McLaughlin, R. J., Ciciora, S. J., Watts, L. A.,
Richardson, M. S., Schwarz, J. P., Perring, A. E., Thornberry, T. D.,
Rollins, A. W., Markovic, M. Z., Bates, T. S., Johnson, J. E., and Fahey, D.
W.: A light-weight, high-sensitivity particle spectrometer for PM2.5 aerosol measurements, Aerosol Sci. Tech., 50, 88–99,
https://doi.org/10.1080/02786826.2015.1131809, 2016.
Grange, S. K., Lee, J. D., Drysdale, W. S., Lewis, A. C., Hueglin, C., Emmenegger, L., and Carslaw, D. C.: COVID-19 lockdowns highlight a risk of increasing ozone pollution in European urban areas, Atmos. Chem. Phys., 21, 4169–4185, https://doi.org/10.5194/acp-21-4169-2021, 2021.
Hagan, D. H. and Kroll, J. H.: Assessing the accuracy of low-cost optical particle sensors using a physics-based approach, Atmos. Meas. Tech., 13, 6343–6355, https://doi.org/10.5194/amt-13-6343-2020, 2020.
Harrison, R. M., Jones, A. M., and Lawrence, R. G.: Major component
composition of PM10 and PM2.5 from roadside and urban background sites, Atmos. Environ., 38, 4531–4538, https://doi.org/10.1016/j.atmosenv.2004.05.022,
2004.
Haywood, J.: Prediction of visibility and aerosol within the operational Met Office Unified Model.II: Validation of model performance using observational data, Q. J. Roy. Meteor. Soc., 134, 1817–1832, https://doi.org/10.1002/qj.275, 2008.
Hinds, W. C.: Aerosol technology: properties, behavior, and measurement of airborne particles, John Wiley & Sons, ISBN 978-0-471-19410-1, 1999.
Hoon Jung, C., Jung Shin, H., Yi Lee, J., Pyo Kim, Y., Pitari, G., and Curci,
G.: Sensitivity and Contribution of Organic Aerosols to Aerosol Optical
Properties Based on Their Refractive Index and Hygroscopicity, Atmosphere, 7, 65, https://doi.org/10.3390/atmos7050065, 2016.
Kebabian, P. L., Herndon, S. C., and Freedman, A.: Detection of nitrogen
dioxide by cavity attenuated phase shift spectroscopy, Anal. Chem., 77,
724–728, https://doi.org/10.1021/ac048715y, 2005.
Lafon, S., Sokolik, I. N., Rajot, J. L., Caquincau, S., and Gaudichet, A.:
Characterization of iron oxides in mineral dust aerosols: Implications for
light absorption, J. Geophys. Res.-Atmos., 111, 1–19,
https://doi.org/10.1029/2005JD007016, 2006.
Langridge, J. M., Ball, S. M., Shillings, A. J. L., and Jones, R. L.: A
broadband absorption spectrometer using light emitting diodes for
ultrasensitive, in situ trace gas detection, Rev. Sci. Instrum., 79, 121310,
https://doi.org/10.1063/1.3046282, 2008.
Langridge, J. M., Lack, D., Brock, C. A., Bahreini, R., Middlebrook, A. M.,
Neuman, J. A., Nowak, J. B., Perring, A. E., Schwarz, J. P., Spackman, J.
R., Holloway, J. S., Pollack, I. B., Ryerson, T. B., Roberts, J. M.,
Warneke, C., De Gouw, J. A., Trainer, M. K., and Murphy, D. M.: Evolution of
aerosol properties impacting visibility and direct climate forcing in an
ammonia-rich urban environment, J. Geophys. Res.-Atmos., 117, 1–17,
https://doi.org/10.1029/2011JD017116, 2012.
Liu, X., Chance, K., Sioris, C. E., Spurr, R. J. D., Kurosu, T. P., Martin,
R. V., and Newchurch, M. J.: Ozone profile and tropospheric ozone retrievals
from the Global Ozone Monitoring Experiment: Algorithm description and
validation, J. Geophys. Res.-Atmos., 110, 1–19,
https://doi.org/10.1029/2005JD006240, 2005.
Liu, Y. and Daum, P. H.: The effect of refractive index on size
distributions and light scattering coefficients derived from optical
particle counters, J. Aerosol Sci., 31, 945–957,
https://doi.org/10.1016/S0021-8502(99)00573-X, 2000.
Lock, A. P., Martin, G. M., Bush, M. R., Brown, A. R., and Smith, R. N. B.: A
new boundary layer mixing scheme part I: Tests in climate and mesoscale
models, Mon. Weather Rev., 128, 3200–3217,
https://doi.org/10.1175/1520-0493(2000)128<3200:ANBLMS>2.0.CO;2, 2000.
Manisalidis, I., Stavropoulou, E., Stavropoulos, A., and Bezirtzoglou, E.:
Environmental and Health Impacts of Air Pollution: A Review, Front. Publ.
Heal., 8, 1–13, https://doi.org/10.3389/fpubh.2020.00014, 2020.
McMeeking, G. R., Morgan, W. T., Flynn, M., Highwood, E. J., Turnbull, K., Haywood, J., and Coe, H.: Black carbon aerosol mixing state, organic aerosols and aerosol optical properties over the United Kingdom, Atmos. Chem. Phys., 11, 9037–9052, https://doi.org/10.5194/acp-11-9037-2011, 2011.
McMeeking, G. R., Bart, M., Chazette, P., Haywood, J. M., Hopkins, J. R., McQuaid, J. B., Morgan, W. T., Raut, J.-C., Ryder, C. L., Savage, N., Turnbull, K., and Coe, H.: Airborne measurements of trace gases and aerosols over the London metropolitan region, Atmos. Chem. Phys., 12, 5163–5187, https://doi.org/10.5194/acp-12-5163-2012, 2012.
Met Office and Mynard, A.: MOASA Clean Air Project: airborne atmospheric measurements collection, NERC EDS Centre for Environmental Data Analysis [data set], https://doi.org/10.5285/0aa1ec0cf18e4065bdae8ae39260fe7d, 2023.
Molina, M. J. and Molina, L. T.: Megacities and atmospheric pollution, J.
Air Waste Manag. Assoc., 54, 644–680, https://doi.org/10.1080/10473289.2004.10470936, 2004.
Morgan, W. T., Allan, J. D., Bower, K. N., Esselborn, M., Harris, B., Henzing, J. S., Highwood, E. J., Kiendler-Scharr, A., McMeeking, G. R., Mensah, A. A., Northway, M. J., Osborne, S., Williams, P. I., Krejci, R., and Coe, H.: Enhancement of the aerosol direct radiative effect by semi-volatile aerosol components: airborne measurements in North-Western Europe, Atmos. Chem. Phys., 10, 8151–8171, https://doi.org/10.5194/acp-10-8151-2010, 2010.
Müller, T., Laborde, M., Kassell, G., and Wiedensohler, A.: Design and performance of a three-wavelength LED-based total scatter and backscatter integrating nephelometer, Atmos. Meas. Tech., 4, 1291–1303, https://doi.org/10.5194/amt-4-1291-2011, 2011.
Müller, T., Virkkula, A., and Ogren, J. A.: Constrained two-stream algorithm for calculating aerosol light absorption coefficient from the Particle Soot Absorption Photometer, Atmos. Meas. Tech., 7, 4049–4070, https://doi.org/10.5194/amt-7-4049-2014, 2014.
National Center for Biotechnology Information: PubChem Annotation Record for CALCIUM SULFATE, Hazardous Substances Data Bank (HSDB), https://pubchem.ncbi.nlm.nih.gov/compound/24497 (last access: 15 September 2023), 2023.
National Meteorological Library: Daily weather summary,
September 2020, National Meteorological Library and Archive, https://digital.nmla.metoffice.gov.uk/IO_00cfff7c-7099-4583-ac85-a9adca963bb5/ (last access: 21 October 2021), 2020.
Neal, L. S., Agnew, P., Moseley, S., Ordóñez, C., Savage, N. H., and
Tilbee, M.: Application of a statistical post-processing technique to a
gridded, operational, air quality forecast, Atmos. Environ., 98, 385–393,
https://doi.org/10.1016/j.atmosenv.2014.09.004, 2014.
Neal, L. S., Dalvi, M., Folberth, G., McInnes, R. N., Agnew, P., O'Connor, F. M., Savage, N. H., and Tilbee, M.: A description and evaluation of an air quality model nested within global and regional composition-climate models using MetUM, Geosci. Model Dev., 10, 3941–3962, https://doi.org/10.5194/gmd-10-3941-2017, 2017.
NOAA: CAMEO Chemicals, CAMEO Chem. version 2.7.1 rev 3, NOAA, https://cameochemicals.noaa.gov/chemical/25006, last access: 23 November 2021.
Nowak, J. B., Neuman, J. A., Bahreini, R., Brock, C. A., Middlebrook, A. M.,
Wollny, A. G., Holloway, J. S., Peischl, J., Ryerson, T. B., and Fehsenfeld,
F. C.: Airborne observations of ammonia and ammonium nitrate formation over
Houston, Texas, J. Geophys. Res.-Atmos., 115, 1–12,
https://doi.org/10.1029/2010JD014195, 2010.
Ogren, J. A., Wendell, J., Andrews, E., and Sheridan, P. J.: Continuous light absorption photometer for long-term studies, Atmos. Meas. Tech., 10, 4805–4818, https://doi.org/10.5194/amt-10-4805-2017, 2017.
OSCA: http://www.ukcleanair.org (last access: 1 December 2021), 2020.
Peers, F., Francis, P., Fox, C., Abel, S. J., Szpek, K., Cotterell, M. I., Davies, N. W., Langridge, J. M., Meyer, K. G., Platnick, S. E., and Haywood, J. M.: Observation of absorbing aerosols above clouds over the south-east Atlantic Ocean from the geostationary satellite SEVIRI – Part 1: Method description and sensitivity, Atmos. Chem. Phys., 19, 9595–9611, https://doi.org/10.5194/acp-19-9595-2019, 2019.
Perim de Faria, J., Bundke, U., Freedman, A., Onasch, T. B., and Petzold, A.: Laboratory validation of a compact single-scattering albedo (SSA) monitor, Atmos. Meas. Tech., 14, 1635–1653, https://doi.org/10.5194/amt-14-1635-2021, 2021.
Petzold, A., Thouret, V., Gerbig, C., Zahn, A., Brenninkmeijer, C. A. M.,
Gallagher, M., Hermann, M., Pontaud, M., Ziereis, H., Boulanger, D.,
Marshall, J., NéDélec, P., Smit, H. G. J., Friess, U., Flaud, J. M.,
Wahner, A., Cammas, J. P., Volz-Thomas, A., Thomas, K., Rohs, S., Bundke,
U., Neis, P., Berkes, F., Houben, N., Berg, M., Tappertzhofen, M., Blomel,
T., Pätz, W., Filges, A., Boschetti, F., Verma, S., Baum, S., Athier,
G., Cousin, J. M., Sauvage, B., Blot, R., Clark, H., Gaudel, A., Gressent,
A., Auby, A., Fontaine, A., Gautron, B., Bennouna, Y., Petetin, H., Karcher,
F., Abonnel, C., Dandin, P., Beswick, K., Wang, K. Y., Rauthe-Schöch,
A., Baker, A. K., Riede, H., Gromov, S., Zimmermann, P., Thorenz, U.,
Scharffe, D., Koeppel, C., Slemr, F., Schuck, T. J., Umezawa, T., Ditas, J.,
Cheng, Y., Schneider, J., Williams, J., Neumaier, M., Christner, E.,
Fischbeck, G., Safadi, L., Petrelli, A., Gehrlein, T., Heger, S., Dyroff,
C., Weber, S., Assmann, D., Rubach, F., Weigelt, A., Stratmann, G., Stock,
P., Penth, L., Walter, D., Heue, K. P., Allouche, Y., Marizy, C., Hermira,
J., Bringtown, S., Saueressig, G., Seidel, N., Huf, M., Waibel, A., Franke,
H., Klaus, C., Stosius, R., Baumgardner, D., Braathen, G., Paulin, M., and
Garnett, N.: Global-scale atmosphere monitoring by in-service aircraft –
current achievements and future prospects of the European Research
Infrastructure IAGOS, Tellus B, 6, 1–24, https://doi.org/10.3402/tellusb.v67.28452, 2015.
Qian, Y., Gustafson Jr., W. I., and Fast, J. D.: An investigation of the sub-grid variability of trace gases and aerosols for global climate modeling, Atmos. Chem. Phys., 10, 6917–6946, https://doi.org/10.5194/acp-10-6917-2010, 2010.
Rosenberg, P. D., Dean, A. R., Williams, P. I., Dorsey, J. R., Minikin, A., Pickering, M. A., and Petzold, A.: Particle sizing calibration with refractive index correction for light scattering optical particle counters and impacts upon PCASP and CDP data collected during the Fennec campaign, Atmos. Meas. Tech., 5, 1147–1163, https://doi.org/10.5194/amt-5-1147-2012, 2012.
Savage, N. H., Agnew, P., Davis, L. S., Ordóñez, C., Thorpe, R., Johnson, C. E., O'Connor, F. M., and Dalvi, M.: Air quality modelling using the Met Office Unified Model (AQUM OS24-26): model description and initial evaluation, Geosci. Model Dev., 6, 353–372, https://doi.org/10.5194/gmd-6-353-2013, 2013.
Solazzo, E., Bianconi, R., Pirovano, G., Moran, M. D., Vautard, R., Hogrefe, C., Appel, K. W., Matthias, V., Grossi, P., Bessagnet, B., Brandt, J., Chemel, C., Christensen, J. H., Forkel, R., Francis, X. V., Hansen, A. B., McKeen, S., Nopmongcol, U., Prank, M., Sartelet, K. N., Segers, A., Silver, J. D., Yarwood, G., Werhahn, J., Zhang, J., Rao, S. T., and Galmarini, S.: Evaluating the capability of regional-scale air quality models to capture the vertical distribution of pollutants, Geosci. Model Dev., 6, 791–818, https://doi.org/10.5194/gmd-6-791-2013, 2013.
Tang, W., Edwards, D. P., Emmons, L. K., Worden, H. M., Judd, L. M., Lamsal, L. N., Al-Saadi, J. A., Janz, S. J., Crawford, J. H., Deeter, M. N., Pfister, G., Buchholz, R. R., Gaubert, B., and Nowlan, C. R.: Assessing sub-grid variability within satellite pixels over urban regions using airborne mapping spectrometer measurements, Atmos. Meas. Tech., 14, 4639–4655, https://doi.org/10.5194/amt-14-4639-2021, 2021.
Thermo Scientific: Thermo Scientific Model 43 i Sulfur Dioxide Analyzer –
pulsed fluorescence gas analyzer, Thermo Fisher Scientific Inc., https://assets.thermofisher.com/TFS-Assets%2FLSG%2FSpecification-Sheets%2FEPM-43i-Datasheet.pdf,
last access: 24 May 2023.
UKRI: Integrated Research Observation System for Clean Air (OSCA), UK Research and Innovation, https://gtr.ukri.org/projects?ref=NE%2FT001984%2F1 (last access: 2 November 2021), 2021.
Veefkind, J. P., Aben, I., McMullan, K., Förster, H., de Vries, J.,
Otter, G., Claas, J., Eskes, H. J., de Haan, J. F., Kleipool, Q., van Weele,
M., Hasekamp, O., Hoogeveen, R., Landgraf, J., Snel, R., Tol, P., Ingmann,
P., Voors, R., Kruizinga, B., Vink, R., Visser, H., and Levelt, P. F.:
TROPOMI on the ESA Sentinel-5 Precursor: A GMES mission for global
observations of the atmospheric composition for climate, air quality and
ozone layer applications, Remote Sens. Environ., 120, 70–83,
https://doi.org/10.1016/j.rse.2011.09.027, 2012.
Virkkula, A.: Calibration of the 3-wavelength particle soot absorption
photometer (3λ PSAP), Aerosol Sci. Tech., 44, 706–712, https://doi.org/10.1080/02786826.2010.482110, 2010.
von der Weiden, S.-L., Drewnick, F., and Borrmann, S.: Particle Loss Calculator – a new software tool for the assessment of the performance of aerosol inlet systems, Atmos. Meas. Tech., 2, 479–494, https://doi.org/10.5194/amt-2-479-2009, 2009.
Williams, M. L., Beevers, S., Kitwiroon, N., Dajnak, D., Walton, H., Lott,
M. C., Pye, S., Fecht, D., Toledano, M. B., and Holland, M.: Public health
air pollution impacts of pathway options to meet the 2050 UK Climate Change
Act target: a modelling study, Publ. Heal. Res., 6, 1–124,
https://doi.org/10.3310/phr06070, 2018.
Wilson, K. L. and Birks, J. W.: Mechanism and elimination of a water vapor
interference in the measurement of ozone by UV absorbance, Environ. Sci.
Technol., 40, 6361–6367, https://doi.org/10.1021/es052590c, 2006.
World Health Organization: Evolution of WHO air quality guidelines: past, present and future, WHO Regional Office for Europe, Copenhagen, Denmark, ISBN 9789289052306, 2017.
Wyche, K. P., Nichols, M., Parfitt, H., Beckett, P., Gregg, D. J.,
Smallbone, K. L., and Monks, P. S.: Changes in ambient air quality and
atmospheric composition and reactivity in the South East of the UK as a
result of the COVID-19 lockdown, Sci. Total Environ., 755, 142526,
https://doi.org/10.1016/j.scitotenv.2020.142526, 2021.
Short summary
Air quality models are key in understanding complex air pollution processes and assist in developing strategies to mitigate the impacts of air pollution. The ability of regional air quality models to skilfully represent pollutant distributions aloft is important to enabling their skilful prediction at the surface. To assist in model development and evaluation, a long-term, quality-assured dataset of the 3-D distribution of key pollutants was collected over the United Kingdom (2019–2022).
Air quality models are key in understanding complex air pollution processes and assist in...
