Articles | Volume 17, issue 22
https://doi.org/10.5194/amt-17-6569-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-17-6569-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Nov 2024
Research article |
| 15 Nov 2024
| 15 Nov 2024
Design study for an airborne N2O lidar
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Andreas Fix
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Christian Fruck
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Gerhard Ehret
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
Martin Wirth
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 82234 Oberpfaffenhofen, Germany
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Georgios Dekoutsidis, Silke Groß, Martin Wirth, Martina Krämer, and Christian Rolf
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Dominik Brunner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys., 23, 2699–2728, https://doi.org/10.5194/acp-23-2699-2023, https://doi.org/10.5194/acp-23-2699-2023, 2023
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We evaluated six atmospheric transport models for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet (Carbon Dioxide and Methane Mission) campaign in 2018. The study analyzed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Ziming Wang, Luca Bugliaro, Tina Jurkat-Witschas, Romy Heller, Ulrike Burkhardt, Helmut Ziereis, Georgios Dekoutsidis, Martin Wirth, Silke Groß, Simon Kirschler, Stefan Kaufmann, and Christiane Voigt
Atmos. Chem. Phys., 23, 1941–1961, https://doi.org/10.5194/acp-23-1941-2023, https://doi.org/10.5194/acp-23-1941-2023, 2023
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Andreas Schäfler, Michael Sprenger, Heini Wernli, Andreas Fix, and Martin Wirth
Atmos. Chem. Phys., 23, 999–1018, https://doi.org/10.5194/acp-23-999-2023, https://doi.org/10.5194/acp-23-999-2023, 2023
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Justyna Swolkień, Andreas Fix, and Michał Gałkowski
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Determination of emissions from coal mines on a local scale requires instantaneous data. We analysed temporal emission data for ventilation shafts and factors influencing their variability. They were saturation of the seams with methane, the permeability of the rock mass, and coal output. The data for the verification should reflect the actual values of emissions from point sources. It is recommended to achieve this by using a standardised emission measurement system for all coal mines.
Konstantin Krüger, Andreas Schäfler, Martin Wirth, Martin Weissmann, and George C. Craig
Atmos. Chem. Phys., 22, 15559–15577, https://doi.org/10.5194/acp-22-15559-2022, https://doi.org/10.5194/acp-22-15559-2022, 2022
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A comprehensive data set of airborne lidar water vapour profiles is compared with ERA5 reanalyses for a robust characterization of the vertical structure of the mid-latitude lower-stratospheric moist bias. We confirm a moist bias of up to 55 % at 1.3 km altitude above the tropopause and uncover a decreasing bias beyond. Collocated O3 and H2O observations reveal a particularly strong bias in the mixing layer, indicating insufficiently modelled transport processes fostering the bias.
Manuel Gutleben, Silke Groß, Christian Heske, and Martin Wirth
Atmos. Chem. Phys., 22, 7319–7330, https://doi.org/10.5194/acp-22-7319-2022, https://doi.org/10.5194/acp-22-7319-2022, 2022
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Theresa Mieslinger, Bjorn Stevens, Tobias Kölling, Manfred Brath, Martin Wirth, and Stefan A. Buehler
Atmos. Chem. Phys., 22, 6879–6898, https://doi.org/10.5194/acp-22-6879-2022, https://doi.org/10.5194/acp-22-6879-2022, 2022
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The trades are home to a plethora of small cumulus clouds that are often barely visible to the human eye and difficult to detect with active and passive remote sensing methods. With the help of a new method and by means of high-resolution data we can detect small and particularly thin clouds. We find that optically thin clouds are a common phenomenon in the trades, covering a large area and influencing the radiative effect of clouds if they are undetected and contaminate the cloud-free signal.
Martin Hagen, Florian Ewald, Silke Groß, Lothar Oswald, David A. Farrell, Marvin Forde, Manuel Gutleben, Johann Heumos, Jens Reimann, Eleni Tetoni, Gregor Köcher, Eleni Marinou, Christoph Kiemle, Qiang Li, Rebecca Chewitt-Lucas, Alton Daley, Delando Grant, and Kashawn Hall
Earth Syst. Sci. Data, 13, 5899–5914, https://doi.org/10.5194/essd-13-5899-2021, https://doi.org/10.5194/essd-13-5899-2021, 2021
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The German polarimetric weather radar Poldirad was deployed for the international campaign EUREC4A on Barbados. The focus was monitoring clouds and precipitation in the trade wind region east of Barbados. Observations were with a temporal sequence of 5 min and a maximum range of 375 km. Examples of mesoscale precipitation patterns, rain rate accumulation, diurnal cycle, and vertical distribution show the potential for further studies on the life cycle of precipitating shallow cumulus clouds.
Sven Krautwurst, Konstantin Gerilowski, Jakob Borchardt, Norman Wildmann, Michał Gałkowski, Justyna Swolkień, Julia Marshall, Alina Fiehn, Anke Roiger, Thomas Ruhtz, Christoph Gerbig, Jaroslaw Necki, John P. Burrows, Andreas Fix, and Heinrich Bovensmann
Atmos. Chem. Phys., 21, 17345–17371, https://doi.org/10.5194/acp-21-17345-2021, https://doi.org/10.5194/acp-21-17345-2021, 2021
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Quantification of anthropogenic CH4 emissions remains challenging, but it is essential for near-term climate mitigation strategies. We use airborne remote sensing observations to assess bottom-up estimates of coal mining emissions from one of Europe's largest CH4 emission hot spots located in Poland. The analysis reveals that emissions from small groups of shafts can be disentangled, but caution is advised when comparing observations to commonly reported annual emissions.
Heike Konow, Florian Ewald, Geet George, Marek Jacob, Marcus Klingebiel, Tobias Kölling, Anna E. Luebke, Theresa Mieslinger, Veronika Pörtge, Jule Radtke, Michael Schäfer, Hauke Schulz, Raphaela Vogel, Martin Wirth, Sandrine Bony, Susanne Crewell, André Ehrlich, Linda Forster, Andreas Giez, Felix Gödde, Silke Groß, Manuel Gutleben, Martin Hagen, Lutz Hirsch, Friedhelm Jansen, Theresa Lang, Bernhard Mayer, Mario Mech, Marc Prange, Sabrina Schnitt, Jessica Vial, Andreas Walbröl, Manfred Wendisch, Kevin Wolf, Tobias Zinner, Martin Zöger, Felix Ament, and Bjorn Stevens
Earth Syst. Sci. Data, 13, 5545–5563, https://doi.org/10.5194/essd-13-5545-2021, https://doi.org/10.5194/essd-13-5545-2021, 2021
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The German research aircraft HALO took part in the research campaign EUREC4A in January and February 2020. The focus area was the tropical Atlantic east of the island of Barbados. We describe the characteristics of the 15 research flights, provide auxiliary information, derive combined cloud mask products from all instruments that observe clouds on board the aircraft, and provide code examples that help new users of the data to get started.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Florian Ewald, Silke Groß, Martin Wirth, Julien Delanoë, Stuart Fox, and Bernhard Mayer
Atmos. Meas. Tech., 14, 5029–5047, https://doi.org/10.5194/amt-14-5029-2021, https://doi.org/10.5194/amt-14-5029-2021, 2021
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In this study, we show how solar radiance observations can be used to validate and further constrain ice cloud microphysics retrieved from the synergy of radar–lidar measurements. Since most radar–lidar retrievals rely on a global assumption about the ice particle shape, ice water content and particle size biases are to be expected in individual cloud regimes. In this work, we identify and correct these biases by reconciling simulated and measured solar radiation reflected from these clouds.
Julian Kostinek, Anke Roiger, Maximilian Eckl, Alina Fiehn, Andreas Luther, Norman Wildmann, Theresa Klausner, Andreas Fix, Christoph Knote, Andreas Stohl, and André Butz
Atmos. Chem. Phys., 21, 8791–8807, https://doi.org/10.5194/acp-21-8791-2021, https://doi.org/10.5194/acp-21-8791-2021, 2021
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Abundant mining and industrial activities in the Upper Silesian Coal Basin lead to large emissions of the potent greenhouse gas methane. This study quantifies these emissions with continuous, high-precision airborne measurements and dispersion modeling. Our emission estimates are in line with values reported in the European Pollutant Release and Transfer Register (E-PRTR 2017) but significantly lower than values reported in the Emissions Database for Global Atmospheric Research (EDGAR v4.3.2).
Sebastian Wolff, Gerhard Ehret, Christoph Kiemle, Axel Amediek, Mathieu Quatrevalet, Martin Wirth, and Andreas Fix
Atmos. Meas. Tech., 14, 2717–2736, https://doi.org/10.5194/amt-14-2717-2021, https://doi.org/10.5194/amt-14-2717-2021, 2021
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We report on CO2 emissions of a coal-fired power plant derived from flight measurements performed with the IPDA lidar CHARM-F during the CoMet campaign in spring 2018. Despite the results being in broad agreement with reported emissions, we observe strong variations between successive flyovers. Using a high-resolution large eddy simulation, we identify strong atmospheric turbulence as the cause for the variations and recommend more favorable measurement conditions for future campaign planning.
Andreas Schäfler, Andreas Fix, and Martin Wirth
Atmos. Chem. Phys., 21, 5217–5234, https://doi.org/10.5194/acp-21-5217-2021, https://doi.org/10.5194/acp-21-5217-2021, 2021
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First-ever, collocated ozone and water vapor lidar observations across the tropopause are applied to investigate the extratropical transition layer (ExTL). The combined view of a quasi-instantaneous cross section and its tracer–tracer depiction allows us to analyze the ExTL shape and composition and the formation of mixing lines in relation to the dynamic situation. Such lidar data are relevant for future upper-tropospheric and lower-stratospheric investigations and model validations.
Mareike Heckl, Andreas Fix, Matthias Jirousek, Franz Schreier, Jian Xu, and Markus Rapp
Atmos. Meas. Tech., 14, 1689–1713, https://doi.org/10.5194/amt-14-1689-2021, https://doi.org/10.5194/amt-14-1689-2021, 2021
Michał Gałkowski, Armin Jordan, Michael Rothe, Julia Marshall, Frank-Thomas Koch, Jinxuan Chen, Anna Agusti-Panareda, Andreas Fix, and Christoph Gerbig
Atmos. Meas. Tech., 14, 1525–1544, https://doi.org/10.5194/amt-14-1525-2021, https://doi.org/10.5194/amt-14-1525-2021, 2021
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We present results of atmospheric measurements of greenhouse gases, performed over Europe in 2018 aboard German research aircraft HALO as part of the CoMet 1.0 (Carbon Dioxide and Methane Mission). In our analysis, we describe data quality, discuss observed mixing ratios and show an example of describing a regional methane source using stable isotopic composition based on the collected air samples. We also quantitatively compare our results to selected global atmospheric modelling systems.
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, Maria Tsichla, Ioanna Tsikoudi, and Dimitris Balis
Atmos. Chem. Phys., 20, 14005–14021, https://doi.org/10.5194/acp-20-14005-2020, https://doi.org/10.5194/acp-20-14005-2020, 2020
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Stratospheric smoke particles are found to significantly depolarize incident light, while this effect is also accompanied by a strong spectral dependence. We utilize scattering simulations to show that this behaviour can be attributed to the near-spherical shape of the particles. We also examine whether an extension of the current AERONET scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke associated with enhanced PLDR.
Alina Fiehn, Julian Kostinek, Maximilian Eckl, Theresa Klausner, Michał Gałkowski, Jinxuan Chen, Christoph Gerbig, Thomas Röckmann, Hossein Maazallahi, Martina Schmidt, Piotr Korbeń, Jarosław Neçki, Pawel Jagoda, Norman Wildmann, Christian Mallaun, Rostyslav Bun, Anna-Leah Nickl, Patrick Jöckel, Andreas Fix, and Anke Roiger
Atmos. Chem. Phys., 20, 12675–12695, https://doi.org/10.5194/acp-20-12675-2020, https://doi.org/10.5194/acp-20-12675-2020, 2020
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A severe reduction of greenhouse gas emissions is necessary to fulfill the Paris Agreement. We use aircraft- and ground-based in situ observations of trace gases and wind speed from two flights over the Upper Silesian Coal Basin, Poland, for independent emission estimation. The derived methane emission estimates are within the range of emission inventories, carbon dioxide estimates are in the lower range and carbon monoxide emission estimates are slightly higher than emission inventory values.
Manuel Gutleben, Silke Groß, Martin Wirth, and Bernhard Mayer
Atmos. Chem. Phys., 20, 12313–12327, https://doi.org/10.5194/acp-20-12313-2020, https://doi.org/10.5194/acp-20-12313-2020, 2020
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Airborne lidar measurements in the vicinity of Barbados are used to investigate radiative effects of long-range-transported Saharan air layers. Derived atmospheric heating rates indicate that observed enhanced water vapor concentrations inside these layers are the main drivers for dust vertical mixing inside the layers. Additionally, they may play a major role for the suppression of subjacent convective cloud development.
Ann Kristin Naumann and Christoph Kiemle
Atmos. Chem. Phys., 20, 6129–6145, https://doi.org/10.5194/acp-20-6129-2020, https://doi.org/10.5194/acp-20-6129-2020, 2020
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The interaction of water vapor and cloudiness poses challenges for weather and climate models. In this study we compare airborne lidar measurements from two field campaigns in the tropical Atlantic with high-resolution simulations. We find that at kilometer-scale grid spacing, the simulations show good skill in reproducing the water vapor distribution in the trades but struggle to capture the transition from cloud-free to low cloud fraction with increasing moisture.
Anna-Leah Nickl, Mariano Mertens, Anke Roiger, Andreas Fix, Axel Amediek, Alina Fiehn, Christoph Gerbig, Michal Galkowski, Astrid Kerkweg, Theresa Klausner, Maximilian Eckl, and Patrick Jöckel
Geosci. Model Dev., 13, 1925–1943, https://doi.org/10.5194/gmd-13-1925-2020, https://doi.org/10.5194/gmd-13-1925-2020, 2020
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Based on the global and regional chemistry–climate model system MECO(n), we implemented a forecast system to support the planning of measurement campaign research flights with chemical weather forecasts. We applied this system for the first time to provide 6 d forecasts in support of the CoMet 1.0
campaign targeting methane emitted from coal mining ventilation shafts in the Upper Silesian Coal Basin in Poland. We describe the new forecast system and evaluate its forecast skill.
Andreas Luther, Ralph Kleinschek, Leon Scheidweiler, Sara Defratyka, Mila Stanisavljevic, Andreas Forstmaier, Alexandru Dandocsi, Sebastian Wolff, Darko Dubravica, Norman Wildmann, Julian Kostinek, Patrick Jöckel, Anna-Leah Nickl, Theresa Klausner, Frank Hase, Matthias Frey, Jia Chen, Florian Dietrich, Jarosław Nȩcki, Justyna Swolkień, Andreas Fix, Anke Roiger, and André Butz
Atmos. Meas. Tech., 12, 5217–5230, https://doi.org/10.5194/amt-12-5217-2019, https://doi.org/10.5194/amt-12-5217-2019, 2019
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Methane ventilated from hard coal mines in the Upper Silesian
Coal Basin in Poland is measured with a mobile Fourier transform spectrometer EM27/SUN. The instrument was mounted on a truck driving in stop-and-go patterns downwind of the methane sources. The emissions are estimated with the cross-sectional flux method. Calculated emissions are in broad agreement with the E-PRTR database. Wind-related errors on the methane estimates dominate the error budget and typically amount to 20 %.
Manuel Gutleben, Silke Groß, and Martin Wirth
Atmos. Chem. Phys., 19, 10659–10673, https://doi.org/10.5194/acp-19-10659-2019, https://doi.org/10.5194/acp-19-10659-2019, 2019
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This study concentrates on airborne lidar measurements conducted during the NARVAL field experiments over the western subtropical North Atlantic Ocean to study differences between shallow marine cloud macro-physical properties (i.e. cloud fraction, cloud top height, cloud length, cloud gap length) in Saharan-dust-laden and dust-free trade wind regions. Cloud top heights, cloud fractions and cloud lengths are found to be lower and smaller in Saharan-dust-laden compared to dust-free regions.
Marek Jacob, Felix Ament, Manuel Gutleben, Heike Konow, Mario Mech, Martin Wirth, and Susanne Crewell
Atmos. Meas. Tech., 12, 3237–3254, https://doi.org/10.5194/amt-12-3237-2019, https://doi.org/10.5194/amt-12-3237-2019, 2019
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Tropical clouds are a key climate component but are still not fully understood. Therefore, we analyze airborne remote sensing measurements that were taken in the dry and wet seasons over the Atlantic east of Barbados. From these we derive sub-kilometer resolution data of vertically integrated atmospheric water vapor and liquid water. Results show that although the humidity is lower in the dry season, clouds are more frequent, contain more water, and produce more rain than in the wet season.
Kevin Wolf, André Ehrlich, Marek Jacob, Susanne Crewell, Martin Wirth, and Manfred Wendisch
Atmos. Meas. Tech., 12, 1635–1658, https://doi.org/10.5194/amt-12-1635-2019, https://doi.org/10.5194/amt-12-1635-2019, 2019
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Using passive spectral solar radiation and active lidar, radar, and microwave measurements with HALO during NARVAL-II, the cloud droplet number concentration of shallow trade wind cumulus is estimated. With stepwise inclusion of the different instruments into the retrieval, the benefits of the synergetic approach based on artificial measurements and two cloud cases are demonstrated. Significant improvement with the synergetic method compared to the solar-radiation-only method is reported.
Christiane Voigt, Andreas Dörnbrack, Martin Wirth, Silke M. Groß, Michael C. Pitts, Lamont R. Poole, Robert Baumann, Benedikt Ehard, Björn-Martin Sinnhuber, Wolfgang Woiwode, and Hermann Oelhaf
Atmos. Chem. Phys., 18, 15623–15641, https://doi.org/10.5194/acp-18-15623-2018, https://doi.org/10.5194/acp-18-15623-2018, 2018
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The 2015–2016 stratospheric winter was the coldest in the 36-year climatological data record. The extreme conditions promoted the formation of persistent Arctic polar stratospheric ice clouds. An extended ice PSC detected by airborne lidar in January 2016 shows a second mode with higher particle depolarization ratios. Back-trajectories from the high-depol ice matched to CALIOP PSC curtains provide evidence for ice nucleation on NAT. The novel data consolidate our understanding of PSC formation.
Yoann Tellier, Clémence Pierangelo, Martin Wirth, Fabien Gibert, and Fabien Marnas
Atmos. Meas. Tech., 11, 5865–5884, https://doi.org/10.5194/amt-11-5865-2018, https://doi.org/10.5194/amt-11-5865-2018, 2018
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The French and German space agencies (CNES, DLR) are currently developing MERLIN, a satellite that will measure atmospheric concentration of methane, a powerful greenhouse gas. To reach the desired precision, horizontally averaging the measurements along the satellite track is performed but leads to a processing bias due to non-linear equations. This article studies the processing biases for several averaging schemes and bias correction algorithms and recommends a best approach to limit biases.
Benedikt Urbanek, Silke Groß, Andreas Schäfler, and Martin Wirth
Atmos. Meas. Tech., 10, 1653–1664, https://doi.org/10.5194/amt-10-1653-2017, https://doi.org/10.5194/amt-10-1653-2017, 2017
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Cirrus evolution from nucleation to cloud breakup can be investigated with a novel classification scheme based on airborne lidar data. Applying it to a case study from the ML-CIRRUS campaign, we investigate the impact of large-scale dynamics and small-scale gravity lee waves on the detailed spatial distribution of evolution stages in individual clouds. Our scheme may help to gain more insights in optical and radiative properties of cirrus under various formation and life cycle conditions.
Kevin Wolf, André Ehrlich, Tilman Hüneke, Klaus Pfeilsticker, Frank Werner, Martin Wirth, and Manfred Wendisch
Atmos. Chem. Phys., 17, 4283–4303, https://doi.org/10.5194/acp-17-4283-2017, https://doi.org/10.5194/acp-17-4283-2017, 2017
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The potential of airborne radiance measurements in the sideward and nadir directions for cirrus remote sensing is investigated. Therefore radiative transfer simulations were used and the sensitivity of upward radiance with respect to optical thickness, effective radius, surface albedo, wavelength and viewing angle was studied. It was shown that sideward observations lead to more accurate retrieval results. Investigating a case study of ML-CIRRUS, these findings are confirmed.
Ulrich Schumann, Christoph Kiemle, Hans Schlager, Ralf Weigel, Stephan Borrmann, Francesco D'Amato, Martina Krämer, Renaud Matthey, Alain Protat, Christiane Voigt, and C. Michael Volk
Atmos. Chem. Phys., 17, 2311–2346, https://doi.org/10.5194/acp-17-2311-2017, https://doi.org/10.5194/acp-17-2311-2017, 2017
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A long-lived (1 h) contrail and overshooting convection were observed in the tropics, near Darwin, Australia. The data are used to study the contrail life cycle at low temperatures and cirrus from deep overturning convection in the lower tropical stratosphere. Airborne in situ, lidar, profiler, radar, and satellite data, as well as a photo, are used to distinguish contrail cirrus from convective cirrus and to study the origin of the observed ice and aerosol, up to 2.3 km above the tropopause.
Christiane Voigt, Andreas Dörnbrack, Martin Wirth, Silke M. Groß, Robert Baumann, Benedikt Ehard, Michael C. Pitts, Lamont R. Poole, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-1082, https://doi.org/10.5194/acp-2016-1082, 2016
Revised manuscript not accepted
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The letter describes unprecedented observations of widespread and persistent polar stratospheric ice clouds (ice PSCs) in the exceptionally cold Arctic stratospheric winter 2015/16. The unique observations are of global relevance because trends in Arctic ozone loss and in polar temperatures are highly uncertain. The new observations at cold conditions serve to enhance our knowledge on ice PSC formation, Arctic ozone loss and polar stratrospheric temperatures in a changing climate.
Manuel Gutleben, Silke Gross, Martin Wirth, and Andreas Schäfler
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-333, https://doi.org/10.5194/amt-2016-333, 2016
Revised manuscript not accepted
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Shallow marine cumulus convection over the Atlantic ocean is studied with observations by airborne and spaceborne lidar instruments. Cloud top height as well as cloud length and cloud gap length distributions are calculated by use of a newly developed algorithm. The distribution of cloud top heights during wintertime measurements shows a two-layer structure. However, significant differences in cloud top height distributions compared to summertime measurements are found.
Thomas Trickl, Hannes Vogelmann, Andreas Fix, Andreas Schäfler, Martin Wirth, Bertrand Calpini, Gilbert Levrat, Gonzague Romanens, Arnoud Apituley, Keith M. Wilson, Robert Begbie, Jens Reichardt, Holger Vömel, and Michael Sprenger
Atmos. Chem. Phys., 16, 8791–8815, https://doi.org/10.5194/acp-16-8791-2016, https://doi.org/10.5194/acp-16-8791-2016, 2016
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A rather homogeneous deep stratospheric intrusion event was mapped by vertical sounding over central Europe and by model calculations along the transport path. The very low minimum H2O mixing ratios demonstrate almost negligible mixing with tropospheric air during the downward transport. The vertical distributions of O3 and aerosol were transferred from the source region to Europe without major change. A rather shallow outflow from the stratosphere was found.
S. Groß, M. Wirth, A. Schäfler, A. Fix, S. Kaufmann, and C. Voigt
Atmos. Meas. Tech., 7, 2745–2755, https://doi.org/10.5194/amt-7-2745-2014, https://doi.org/10.5194/amt-7-2745-2014, 2014
C. Weaver, C. Kiemle, S. R. Kawa, T. Aalto, J. Necki, M. Steinbacher, J. Arduini, F. Apadula, H. Berkhout, and J. Hatakka
Atmos. Chem. Phys., 14, 2625–2637, https://doi.org/10.5194/acp-14-2625-2014, https://doi.org/10.5194/acp-14-2625-2014, 2014
G. Wetzel, H. Oelhaf, G. Berthet, A. Bracher, C. Cornacchia, D. G. Feist, H. Fischer, A. Fix, M. Iarlori, A. Kleinert, A. Lengel, M. Milz, L. Mona, S. C. Müller, J. Ovarlez, G. Pappalardo, C. Piccolo, P. Raspollini, J.-B. Renard, V. Rizi, S. Rohs, C. Schiller, G. Stiller, M. Weber, and G. Zhang
Atmos. Chem. Phys., 13, 5791–5811, https://doi.org/10.5194/acp-13-5791-2013, https://doi.org/10.5194/acp-13-5791-2013, 2013
S. Groß, M. Esselborn, B. Weinzierl, M. Wirth, A. Fix, and A. Petzold
Atmos. Chem. Phys., 13, 2487–2505, https://doi.org/10.5194/acp-13-2487-2013, https://doi.org/10.5194/acp-13-2487-2013, 2013
S. Groß, M. Esselborn, F. Abicht, M. Wirth, A. Fix, and A. Minikin
Atmos. Chem. Phys., 13, 2435–2444, https://doi.org/10.5194/acp-13-2435-2013, https://doi.org/10.5194/acp-13-2435-2013, 2013
Related subject area
Subject: Gases | Technique: Remote Sensing | Topic: Instruments and Platforms
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Measurement of the vertical atmospheric density profile from the X-ray Earth occultation of the Crab Nebula with Insight-HXMT
Quantification and mitigation of the instrument effects and uncertainties of the airborne limb imaging FTIR GLORIA
Improved calibration procedures for the EM27/SUN spectrometers of the COllaborative Carbon Column Observing Network (COCCON)
Ground-based Ku-band microwave observations of ozone in the polar middle atmosphere
Traceable total ozone column retrievals from direct solar spectral irradiance measurements in the ultraviolet
Far-ultraviolet airglow remote sensing measurements on Feng Yun 3-D meteorological satellite
The NO2 camera based on gas correlation spectroscopy
Total water vapour columns derived from Sentinel 5P using the AMC-DOAS method
Mobile and high-spectral-resolution Fabry–Pérot interferometer spectrographs for atmospheric remote sensing
Diurnal variability of stratospheric column NO2 measured using direct solar and lunar spectra over Table Mountain, California (34.38° N)
The “ideal” spectrograph for atmospheric observations
Differential absorption lidar for water vapor isotopologues in the 1.98 µm spectral region: sensitivity analysis with respect to regional atmospheric variability
Atmospheric carbon dioxide measurement from aircraft and comparison with OCO-2 and CarbonTracker model data
Prajjwal Rawat, James H. Crawford, Katherine R. Travis, Laura M. Judd, Mary Angelique G. Demetillo, Lukas C. Valin, James J. Szykman, Andrew Whitehill, Eric Baumann, and Thomas F. Hanisco
Atmos. Meas. Tech., 18, 2899–2917, https://doi.org/10.5194/amt-18-2899-2025, https://doi.org/10.5194/amt-18-2899-2025, 2025
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The Pandonia Global Network (PGN) consists of Pandora spectrometers that observe trace gases at a high time resolution to validate satellite observations and understand local air quality. To aid users, PGN assigns quality flags that assure scientifically valid data but eliminate large amounts of data appropriate for scientific applications. A new method based on contemporaneous data in two independent observation modes is proven using complementary ground-based and airborne observations.
Joel F. Campbell, Bing Lin, and Zhaoyan Liu
EGUsphere, https://doi.org/10.5194/egusphere-2025-1448, https://doi.org/10.5194/egusphere-2025-1448, 2025
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This is a reply to a recent article by Christoph Kiemle, regarding ranging measurements with cw lidar are discussed. Our methods and results are justified.
Harikrishnan Charuvil Asokan, Jochen Landgraf, Pepijn Veefkind, Stijn Dellaert, and André Butz
EGUsphere, https://doi.org/10.5194/egusphere-2025-1071, https://doi.org/10.5194/egusphere-2025-1071, 2025
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Greenhouse gases like CO2 and CH4 drive climate change. Satellites enable monitoring of these emissions from space. Our simulations show that the upcoming TANGO mission can detect about 500 targets per 4-day cycle under clear skies, but cloud cover reduces detection. Integrating cloud forecasts into TANGO’s maneuvering boosts detections, highlighting its potential for improving global emission monitoring.
Robert A. Stillwell, Adam Karboski, Matthew Hayman, and Scott M. Spuler
EGUsphere, https://doi.org/10.5194/egusphere-2025-1288, https://doi.org/10.5194/egusphere-2025-1288, 2025
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A method is introduced to expand the observational capability of a diode-laser-based lidar system. This method allows the lidar transmitter to change the laser pulse characteristics from one shot to the next. We use this capability to lower the minimum altitude of observation and also used it to observe clouds with higher range resolution.
Luis F. Millán, Matthew D. Lebsock, and Marcin J. Kurowski
EGUsphere, https://doi.org/10.5194/egusphere-2025-322, https://doi.org/10.5194/egusphere-2025-322, 2025
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This study explores the potential of a hypothetical spaceborne radar to observe water vapor within clouds.
Soohyun Ka and Jung Jin Oh
Atmos. Meas. Tech., 18, 1283–1299, https://doi.org/10.5194/amt-18-1283-2025, https://doi.org/10.5194/amt-18-1283-2025, 2025
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We developed a ground-based 110.836 GHz radiometer developed to measure the stratospheric ozone profile over Seoul, South Korea. To ensure precise measurements and correct the atmospheric spectrum, we employed hot–cold calibration along with continuous tipping curve calibration. Prior to the retrieval process, both pointing and frequency offsets were corrected. We provide stratospheric ozone profiles from 2016 to 2021, which are compared with collocated satellite observations.
Jiangman Xu, Ang Li, Zhaokun Hu, Hairong Zhang, and Min Qin
Atmos. Meas. Tech., 18, 865–879, https://doi.org/10.5194/amt-18-865-2025, https://doi.org/10.5194/amt-18-865-2025, 2025
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This article introduces an experimental system for rapidly acquiring trace gas profiles using multi-channel spectroscopy, significantly enhancing the time resolution of spectral collection. The fast synchronous multi-axis differential optical absorption spectroscopy (FS MAX-DOAS) successfully obtains gas profiles. This work can also be integrated with mobile platforms for navigational observation research, which is crucial for making mobile MAX-DOAS profile measurements.
Kåre Edvardsen, Matt Tully, and Steve Rhodes
EGUsphere, https://doi.org/10.5194/egusphere-2025-87, https://doi.org/10.5194/egusphere-2025-87, 2025
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A new, low-cost instrument for measuring total column ozone was tested against a MK III Brewer spectrophotometer for six months. Using the "Global Irradiance" method from the Norwegian GUV network, it showed ozone values matching Direct Sun Brewer measurements with a 1.8 % standard deviation. Despite temperature and cloud dependencies, the instrument is robust and easy to use. Fully coverage of the UV-A/B spectrum allows for further UV-radiation analysis. Total cost is less than EUR 3000.
Lorenzo Guerrieri, Stefano Corradini, Luca Merucci, Dario Stelitano, Fred Prata, Linda Lambertucci, Camilo Naranjo, and Riccardo Biondi
EGUsphere, https://doi.org/10.5194/egusphere-2025-63, https://doi.org/10.5194/egusphere-2025-63, 2025
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This work presents a new simplified ground based Thermal InfraRed (TIR) system capable to detect and retrieve volcanic emissions during both day and night. Knowing the location of the instrument and the crater, it is possible to compute the geometry (height and thickness) of a volcanic plume. Furthermore, thanks to a specific filter positioned in front of one of the TIR cameras, it is possible to compute the sulfur dioxide (SO2) content emitted by the volcano at a safe distance from the vent.
Guangqiang Fan, Yibin Fu, Juntao Huo, Yan Xiang, Tianshu Zhang, Wenqing Liu, and Zhi Ning
Atmos. Meas. Tech., 18, 443–453, https://doi.org/10.5194/amt-18-443-2025, https://doi.org/10.5194/amt-18-443-2025, 2025
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Our research introduces a differential absorption lidar system for monitoring tropospheric ozone, utilizing a single CO2 Raman cell. This technology enables the acquisition of high-resolution vertical ozone profiles from 0.3 to 4 km, essential for understanding air quality and climate impacts.
Fernando Chouza, Thierry Leblanc, Patrick Wang, Steven S. Brown, Kristen Zuraski, Wyndom Chace, Caroline C. Womack, Jeff Peischl, John Hair, Taylor Shingler, and John Sullivan
Atmos. Meas. Tech., 18, 405–419, https://doi.org/10.5194/amt-18-405-2025, https://doi.org/10.5194/amt-18-405-2025, 2025
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The JPL lidar group developed the SMOL (Small Mobile Ozone Lidar), an affordable ozone differential absorption lidar (DIAL) system covering all altitudes from 200 m to 10 km a.g.l. The comparison with airborne in situ and lidar measurements shows very good agreement. An additional comparison with nearby surface ozone measuring instruments indicates unbiased measurements by the SMOL lidars down to 200 m a.g.l.
Lara Noppen, Lieven Clarisse, Frederik Tack, Thomas Ruhtz, Martin Van Damme, Michel Van Roozendael, Dirk Schuettemeyer, and Pierre Coheur
EGUsphere, https://doi.org/10.5194/egusphere-2024-3455, https://doi.org/10.5194/egusphere-2024-3455, 2025
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Current infrared satellite sounders offer high spectral but low spatial resolution, limiting their ability to quantify atmospheric ammonia (NH3) at small scales. Through simulations and analysis of real data, we show that NH3 can be measured effectively from spectra with reduced resolution, either in a contiguous spectral range or in select well-chosen bands. This approach opens possibilities for the development of smaller dedicated instruments for observing NH3 at high spatial resolution.
Marie Lothon, François Gheusi, Fabienne Lohou, Véronique Pont, Serge Soula, Corinne Jambert, Solène Derrien, Yannick Bezombes, Emmanuel Leclerc, Gilles Athier, Antoine Vial, Alban Philibert, Bernard Campistron, Frédérique Saïd, Jeroen Sonke, Julien Amestoy, Erwan Bargain, Pierre Bosser, Damien Boulanger, Guillaume Bret, Renaud Bodichon, Laurent Cabanas, Guylaine Canut, Jean-Bernard Estrampes, Eric Gardrat, Zaida Gomez Kuri, Jérémy Gueffier, Fabienne Guesdon, Morgan Lopez, Olivier Masson, Pierre-Yves Meslin, Yves Meyerfeld, Nicolas Pascal, Eric Pique, Michel Ramonet, Felix Starck, and Romain Vidal
Atmos. Meas. Tech., 17, 6265–6300, https://doi.org/10.5194/amt-17-6265-2024, https://doi.org/10.5194/amt-17-6265-2024, 2024
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The Pyrenean Platform for Observation of the Atmosphere (P2OA) is a coupled plain–mountain instrumented platform in southwestern France for the monitoring of climate variables and the study of meteorological processes in a mountainous region. A comprehensive description of this platform is presented for the first time: its instrumentation, the associated dataset, and a meteorological characterization the site. The potential of the P2OA is illustrated through several examples of process studies.
Johannes Speidel, Hannes Vogelmann, Andreas Behrendt, Diego Lange, Matthias Mauder, Jens Reichardt, and Kevin Wolz
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-168, https://doi.org/10.5194/amt-2024-168, 2024
Revised manuscript accepted for AMT
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Humidity transport from the Earth's surface into the atmosphere is relevant for many processes. However, knowledge on the actual distribution of humidity concentrations is sparse – mainly due to technological limitations. With the herein presented lidar, it is possible to measure humidity concentrations and their vertical fluxes up to altitudes of >3 km with high spatio-temporal resolution, opening new possibilities for detailed process understanding and, ultimately, better model representation.
Karolin Voss, Philip Holzbeck, Klaus Pfeilsticker, Ralph Kleinschek, Gerald Wetzel, Blanca Fuentes Andrade, Michael Höpfner, Jörn Ungermann, Björn-Martin Sinnhuber, and André Butz
Atmos. Meas. Tech., 17, 4507–4528, https://doi.org/10.5194/amt-17-4507-2024, https://doi.org/10.5194/amt-17-4507-2024, 2024
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A novel balloon-borne instrument for direct sun and solar occultation measurements of several UV–Vis absorbing gases (e.g. O3, NO2, BrO, IO, and HONO) is described. Its major design features and performance during two stratospheric deployments are discussed. From the measured overhead BrO concentration and a suitable photochemical correction, total stratospheric bromine is inferred to (17.5 ± 2.2) ppt in air masses which entered the stratosphere around early 2017 ± 1 year.
Mark Weber
Atmos. Meas. Tech., 17, 3597–3604, https://doi.org/10.5194/amt-17-3597-2024, https://doi.org/10.5194/amt-17-3597-2024, 2024
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We investigate how stable the performance of a satellite instrument has to be to be useful for assessing long-term trends in stratospheric ozone. The stability of an instrument is specified in percent per decade and is also called instrument drift. Instrument drifts add to uncertainties of long-term trends. From simulated time series of ozone based on the Monte Carlo approach, we determine stability requirements that are needed to achieve the desired long-term trend uncertainty.
Zhaoyan Liu, Bing Lin, Joel F. Campbell, Jirong Yu, Jihong Geng, and Shibin Jiang
Atmos. Meas. Tech., 17, 2977–2990, https://doi.org/10.5194/amt-17-2977-2024, https://doi.org/10.5194/amt-17-2977-2024, 2024
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We introduce a concept utilizing a differential absorption barometric lidar operating within the 1.96 µm CO2 absorption band. Our focus is on a compact lidar configuration, featuring reduced telescope size and lower laser pulse energies towards minimizing costs for potential forthcoming Mars missions. The core measurement objectives encompass the determination of column CO2 absorption optical depth and abundance, surface air pressure, and vertical distributions of dust and cloud layers.
Jean-Philippe W. MacLean, Marianne Girard, Dylan Jervis, David Marshall, Jason McKeever, Antoine Ramier, Mathias Strupler, Ewan Tarrant, and David Young
Atmos. Meas. Tech., 17, 863–874, https://doi.org/10.5194/amt-17-863-2024, https://doi.org/10.5194/amt-17-863-2024, 2024
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We demonstrate the capabilities of the GHGSat satellite constellation to detect and quantify offshore methane emissions using a sun glint observation mode. Using this technique, we observe offshore methane emissions from space ranging from 180 kg h−1 to 84 000 kg h−1. We further assess the instrument performance in offshore environments, both empirically and using analytical modelling, and find that the detection limit varies with latitude and season.
Alexander Geddes, Ben Liley, Richard McKenzie, Michael Kotkamp, and Richard Querel
Atmos. Meas. Tech., 17, 827–838, https://doi.org/10.5194/amt-17-827-2024, https://doi.org/10.5194/amt-17-827-2024, 2024
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In this paper we describe a unique spectrometer that has been developed and tested over 10 years at Lauder, New Zealand. The spectrometer in question, UV2, makes alternating measurements of global UV and direct sun UV irradiance. After an assessment of the instrument performance, we compare the ozone and aerosol optical depth derived from UV2 to other independent measurements, finding excellent agreement suggesting that UV2 could supersede these measurements, particularly for ozone.
Haklim Choi, Xiong Liu, Ukkyo Jeong, Heesung Chong, Jhoon Kim, Myung Hwan Ahn, Dai Ho Ko, Dong-Won Lee, Kyung-Jung Moon, and Kwang-Mog Lee
Atmos. Meas. Tech., 17, 145–164, https://doi.org/10.5194/amt-17-145-2024, https://doi.org/10.5194/amt-17-145-2024, 2024
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GEMS is the first geostationary satellite to measure the UV--Vis region, and this paper reports the polarization characteristics of GEMS and an algorithm. We develop a polarization correction algorithm optimized for GEMS based on a look-up-table approach that simultaneously considers the polarization of incoming light and polarization sensitivity characteristics of the instrument. Pre-launch polarization error was adjusted close to zero across the spectral range after polarization correction.
Tobias D. Schmitt, Jonas Kuhn, Ralph Kleinschek, Benedikt A. Löw, Stefan Schmitt, William Cranton, Martina Schmidt, Sanam N. Vardag, Frank Hase, David W. T. Griffith, and André Butz
Atmos. Meas. Tech., 16, 6097–6110, https://doi.org/10.5194/amt-16-6097-2023, https://doi.org/10.5194/amt-16-6097-2023, 2023
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Our new observatory measures greenhouse gas concentrations of carbon dioxide (CO2) and methane (CH4) along a 1.55 km long light path over the city of Heidelberg, Germany. We compared our measurements with measurements that were taken at a single point at one end of our path. The two mostly agreed but show a significant difference for CO2 with certain wind directions. This is important when using greenhouse gas concentration measurements to observe greenhouse gas emissions of cities.
Kevin C. Cossel, Eleanor M. Waxman, Eli Hoenig, Daniel Hesselius, Christopher Chaote, Ian Coddington, and Nathan R. Newbury
Atmos. Meas. Tech., 16, 5697–5707, https://doi.org/10.5194/amt-16-5697-2023, https://doi.org/10.5194/amt-16-5697-2023, 2023
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Measurements of the emission rate of a gas or gases from point and area sources are important in a range of monitoring applications. We demonstrate a method for rapid quantification of the emission rate of multiple gases using a spatially scannable open-path sensor. The open-path spectrometer measures the total column density of gases between the spectrometer and a retroreflector mounted on an uncrewed aerial vehicle (UAV). By scanning the UAV altitude, we can determine the total gas emissions.
Benedikt A. Löw, Ralph Kleinschek, Vincent Enders, Stanley P. Sander, Thomas J. Pongetti, Tobias D. Schmitt, Frank Hase, Julian Kostinek, and André Butz
Atmos. Meas. Tech., 16, 5125–5144, https://doi.org/10.5194/amt-16-5125-2023, https://doi.org/10.5194/amt-16-5125-2023, 2023
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We developed a portable spectrometer (EM27/SCA) that remotely measures greenhouse gases in the lower atmosphere above a target region. The measurements can deliver insights into local emission patterns. To evaluate its performance, we set up the EM27/SCA above the Los Angeles Basin side by side with a similar non-portable instrument (CLARS-FTS). The precision is promising and the measurements are consistent with CLARS-FTS. In the future, we need to account for light scattering.
Daniel I. Herman, Griffin Mead, Fabrizio R. Giorgetta, Esther Baumann, Nathan A. Malarich, Brian R. Washburn, Nathan R. Newbury, Ian Coddington, and Kevin C. Cossel
Atmos. Meas. Tech., 16, 4053–4066, https://doi.org/10.5194/amt-16-4053-2023, https://doi.org/10.5194/amt-16-4053-2023, 2023
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Measurements of the isotope ratio of water vapor provide information about the sources and history of water vapor at a given location, which can be used to understand the impacts of climate change on global water use. Here, we demonstrate a new method for measuring isotope ratios over long open-air paths, which can reduce sampling bias and provide more spatial averaging than standard point sensor methods. We show that this new technique has high sensitivity and accuracy.
Luca Egli, Julian Gröbner, Herbert Schill, and Eliane Maillard Barras
Atmos. Meas. Tech., 16, 2889–2902, https://doi.org/10.5194/amt-16-2889-2023, https://doi.org/10.5194/amt-16-2889-2023, 2023
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This paper introduces a new method to retrieve total column ozone with spectral ground-based measurements from a novel array spectroradiometer. Total column ozone estimates using the small, cost-effective, and robust instrument and the new retrieval method are compared with other co-located total column ozone instruments. The comparison shows that the new system performs similarly to other well-established instruments, which require substantially more maintenance than the system introduced here.
Frank Werner, Nathaniel J. Livesey, Luis F. Millán, William G. Read, Michael J. Schwartz, Paul A. Wagner, William H. Daffer, Alyn Lambert, Sasha N. Tolstoff, and Michelle L. Santee
Atmos. Meas. Tech., 16, 2733–2751, https://doi.org/10.5194/amt-16-2733-2023, https://doi.org/10.5194/amt-16-2733-2023, 2023
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The algorithm that produces the near-real-time data products of the Aura Microwave Limb Sounder has been updated. The new algorithm is based on machine learning techniques and yields data products with much improved accuracy. It is shown that the new algorithm outperforms the previous versions, even when it is trained on only a few years of satellite observations. This confirms the potential of applying machine learning to the near-real-time efforts of other current and future mission concepts.
Xiaoyi Zhao, Vitali Fioletov, Alberto Redondas, Julian Gröbner, Luca Egli, Franz Zeilinger, Javier López-Solano, Alberto Berjón Arroyo, James Kerr, Eliane Maillard Barras, Herman Smit, Michael Brohart, Reno Sit, Akira Ogyu, Ihab Abboud, and Sum Chi Lee
Atmos. Meas. Tech., 16, 2273–2295, https://doi.org/10.5194/amt-16-2273-2023, https://doi.org/10.5194/amt-16-2273-2023, 2023
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The Brewer ozone spectrophotometer is one of the World Meteorological Organization (WMO) Global Atmosphere Watch (GAW)'s standard ozone monitoring instruments since the 1980s. This work is aimed at obtaining answers to (1) why Brewer primary calibration work can only be performed at certain sites (e.g., Izaña and MLO) and (2) what is needed to assure the equivalence of calibration quality from different sites.
Elion Daniel Hack, Theotonio Pauliquevis, Henrique Melo Jorge Barbosa, Marcia Akemi Yamasoe, Dimitri Klebe, and Alexandre Lima Correia
Atmos. Meas. Tech., 16, 1263–1278, https://doi.org/10.5194/amt-16-1263-2023, https://doi.org/10.5194/amt-16-1263-2023, 2023
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Water vapor is a key factor when seeking to understand fast-changing processes when clouds and storms form and develop. We show here how images from a calibrated infrared camera can be used to derive how much water vapor there is in the atmosphere at a given time. Comparing our results to an established technique, for a case of stable atmospheric conditions, we found an agreement within 2.8 %. Water vapor sky maps can be retrieved every few minutes, day or night, under partly cloudy skies.
Kai Wu, Paul I. Palmer, Dien Wu, Denis Jouglet, Liang Feng, and Tom Oda
Atmos. Meas. Tech., 16, 581–602, https://doi.org/10.5194/amt-16-581-2023, https://doi.org/10.5194/amt-16-581-2023, 2023
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We evaluate the theoretical ability of the upcoming MicroCarb satellite to estimate urban CO2 emissions over Paris and London. We explore the relative performance of alternative two-sweep and three-sweep city observing modes and take into account the impacts of cloud cover and urban biological CO2 fluxes. Our results find both the two-sweep and three-sweep observing modes are able to reduce prior flux errors by 20 %–40 % depending on the prevailing wind direction and cloud coverage.
Simon Leitner, Wendelin Feichtinger, Stefan Mayer, Florian Mayer, Dustin Krompetz, Rebecca Hood-Nowotny, and Andrea Watzinger
Atmos. Meas. Tech., 16, 513–527, https://doi.org/10.5194/amt-16-513-2023, https://doi.org/10.5194/amt-16-513-2023, 2023
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An increased social environmental awareness requires the monitoring of greenhouse gases (GHGs). We report on the development of two sampling devices (which can be mounted to a drone) and the subsequent measurement setup to analyse these gases. The functionality of the presented system was tested in the field, and the results emphasised the functionality of the sampling and measurement setup, demonstrating that it is a viable tool for monitoring GHGs and identifying their emission sources.
Sean Crowell, Tobias Haist, Michael Tscherpel, Jérôme Caron, Eric Burgh, and Berrien Moore III
Atmos. Meas. Tech., 16, 195–208, https://doi.org/10.5194/amt-16-195-2023, https://doi.org/10.5194/amt-16-195-2023, 2023
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Variations in brightness in radiance measurements cause errors that can be mitigated with hardware that scrambles the pattern of the incoming light. GeoCarb took this route to minimize this source of errors, but lab testing determined that the solution chosen was too sensitive to the the polarization of the incoming light. Modeling found that this was a predictable result of using gold coatings in the design, which is typical of spaceflight optical instruments.
Emily Bell, Christopher W. O'Dell, Thomas E. Taylor, Aronne Merrelli, Robert R. Nelson, Matthäus Kiel, Annmarie Eldering, Robert Rosenberg, and Brendan Fisher
Atmos. Meas. Tech., 16, 109–133, https://doi.org/10.5194/amt-16-109-2023, https://doi.org/10.5194/amt-16-109-2023, 2023
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A small percentage of data from the Orbiting Carbon Observatory-3 (OCO-3) instrument has been shown to have a geometry-related bias in the earliest public data release. This work shows that the bias is due to a complex interplay of aerosols and viewing geometry and is largely mitigated in the latest data version through improved bias correction and quality filtering.
Hiroshi Suto, Fumie Kataoka, Robert O. Knuteson, Kei Shiomi, Nobuhiro Kikuchi, and Akihiko Kuze
Atmos. Meas. Tech., 15, 5399–5413, https://doi.org/10.5194/amt-15-5399-2022, https://doi.org/10.5194/amt-15-5399-2022, 2022
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TANSO-FTS-2 onboard GOSAT-2 has operated nominally since February 2019, and the atmospheric radiance spectra it has acquired have been released to the public. This paper describes an updated model for spectral radiance calibration of TIR and its validation. The multi-satellite sensor and multi-angle comparison results suggest that the spectral radiance for TANSO-FTS-2 TIR, version v210210, is superior to that of the previous version in its consistency of multi-satellite sensor data.
Rory A. Barton-Grimley, Amin R. Nehrir, Susan A. Kooi, James E. Collins, David B. Harper, Anthony Notari, Joseph Lee, Joshua P. DiGangi, Yonghoon Choi, and Kenneth J. Davis
Atmos. Meas. Tech., 15, 4623–4650, https://doi.org/10.5194/amt-15-4623-2022, https://doi.org/10.5194/amt-15-4623-2022, 2022
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HALO is a multi-functional lidar that measures CH4 columns and profiles of H2O mixing ratio and aerosol/cloud optical properties. HALO supports carbon cycle, weather dynamics, and radiation science suborbital research and is a technology testbed for future space-based differential absorption lidar missions. In 2019 HALO collected CH4 columns and aerosol/cloud profiles during the ACT-America campaign. Here we assess HALO's CH4 accuracy and precision compared to co-located in situ observations.
Aaron Pearlman, Monica Cook, Boryana Efremova, Francis Padula, Lok Lamsal, Joel McCorkel, and Joanna Joiner
Atmos. Meas. Tech., 15, 4489–4501, https://doi.org/10.5194/amt-15-4489-2022, https://doi.org/10.5194/amt-15-4489-2022, 2022
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NOAA’s Geostationary Extended Observations (GeoXO) constellation is planned to consist of an atmospheric composition instrument (ACX) to support air quality forecasting and monitoring. As design trade-offs are being studied, we investigated one parameter, the polarization sensitivity, which has yet to be fully documented for NO2 retrievals. Our simulation study explores these impacts to inform the ACX’s development and better understand polarization’s role in trace gas retrievals.
Fernando Chouza, Thierry Leblanc, Mark Brewer, Patrick Wang, Giovanni Martucci, Alexander Haefele, Hélène Vérèmes, Valentin Duflot, Guillaume Payen, and Philippe Keckhut
Atmos. Meas. Tech., 15, 4241–4256, https://doi.org/10.5194/amt-15-4241-2022, https://doi.org/10.5194/amt-15-4241-2022, 2022
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The comparison of water vapor lidar measurements with co-located radiosondes and aerosol backscatter profiles indicates that laser-induced aerosol fluorescence in smoke layers injected into the stratosphere can introduce very large and chronic wet biases above 15 km, thus impacting the ability of these systems to accurately estimate long-term water vapor trends. The proposed correction method presented in this work is able to reduce this fluorescence-induced bias from 75 % to under 5 %.
Boris D. Belan, Gerard Ancellet, Irina S. Andreeva, Pavel N. Antokhin, Viktoria G. Arshinova, Mikhail Y. Arshinov, Yurii S. Balin, Vladimir E. Barsuk, Sergei B. Belan, Dmitry G. Chernov, Denis K. Davydov, Alexander V. Fofonov, Georgii A. Ivlev, Sergei N. Kotel'nikov, Alexander S. Kozlov, Artem V. Kozlov, Katharine Law, Andrey V. Mikhal'chishin, Igor A. Moseikin, Sergei V. Nasonov, Philippe Nédélec, Olesya V. Okhlopkova, Sergei E. Ol'kin, Mikhail V. Panchenko, Jean-Daniel Paris, Iogannes E. Penner, Igor V. Ptashnik, Tatyana M. Rasskazchikova, Irina K. Reznikova, Oleg A. Romanovskii, Alexander S. Safatov, Denis E. Savkin, Denis V. Simonenkov, Tatyana K. Sklyadneva, Gennadii N. Tolmachev, Semyon V. Yakovlev, and Polina N. Zenkova
Atmos. Meas. Tech., 15, 3941–3967, https://doi.org/10.5194/amt-15-3941-2022, https://doi.org/10.5194/amt-15-3941-2022, 2022
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The change of the global climate is most pronounced in the Arctic, where the air temperature increases faster than the global average. This is associated with an increase in the concentration of greenhouse gases in the atmosphere. It is important to study how the air composition in the Arctic changes in the changing climate. Thus this integrated experiment was carried out to measure the composition of the troposphere in the Russian sector of the Arctic from on board the aircraft laboratory.
Daochun Yu, Haitao Li, Baoquan Li, Mingyu Ge, Youli Tuo, Xiaobo Li, Wangchen Xue, Yaning Liu, Aoying Wang, Yajun Zhu, and Bingxian Luo
Atmos. Meas. Tech., 15, 3141–3159, https://doi.org/10.5194/amt-15-3141-2022, https://doi.org/10.5194/amt-15-3141-2022, 2022
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In this work, the measurement of vertical atmospheric density profiles using X-ray Earth occultation is investigated. The Earth’s density profile for the lower thermosphere is obtained with Insight-HXMT. It is shown that the Insight-HXMT X-ray satellite of China can be used as an X-ray atmospheric diagnostics instrument for the upper atmosphere. The Insight-HXMT satellite can, with other X-ray astronomical satellites in orbit, form a network for X-ray Earth occultation sounding in the future.
Jörn Ungermann, Anne Kleinert, Guido Maucher, Irene Bartolomé, Felix Friedl-Vallon, Sören Johansson, Lukas Krasauskas, and Tom Neubert
Atmos. Meas. Tech., 15, 2503–2530, https://doi.org/10.5194/amt-15-2503-2022, https://doi.org/10.5194/amt-15-2503-2022, 2022
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GLORIA is a 2-D infrared imaging spectrometer operated on two high-flying research aircraft. This paper details our instrument calibration and characterization efforts, which in particular leverage in-flight data almost exclusively and often exploit the novel 2-D nature of the measurements. We show that the instrument surpasses the original instrument specifications and conclude by analyzing how the derived errors affect temperature and ozone retrievals, two of our main derived quantities.
Carlos Alberti, Frank Hase, Matthias Frey, Darko Dubravica, Thomas Blumenstock, Angelika Dehn, Paolo Castracane, Gregor Surawicz, Roland Harig, Bianca C. Baier, Caroline Bès, Jianrong Bi, Hartmut Boesch, André Butz, Zhaonan Cai, Jia Chen, Sean M. Crowell, Nicholas M. Deutscher, Dragos Ene, Jonathan E. Franklin, Omaira García, David Griffith, Bruno Grouiez, Michel Grutter, Abdelhamid Hamdouni, Sander Houweling, Neil Humpage, Nicole Jacobs, Sujong Jeong, Lilian Joly, Nicholas B. Jones, Denis Jouglet, Rigel Kivi, Ralph Kleinschek, Morgan Lopez, Diogo J. Medeiros, Isamu Morino, Nasrin Mostafavipak, Astrid Müller, Hirofumi Ohyama, Paul I. Palmer, Mahesh Pathakoti, David F. Pollard, Uwe Raffalski, Michel Ramonet, Robbie Ramsay, Mahesh Kumar Sha, Kei Shiomi, William Simpson, Wolfgang Stremme, Youwen Sun, Hiroshi Tanimoto, Yao Té, Gizaw Mengistu Tsidu, Voltaire A. Velazco, Felix Vogel, Masataka Watanabe, Chong Wei, Debra Wunch, Marcia Yamasoe, Lu Zhang, and Johannes Orphal
Atmos. Meas. Tech., 15, 2433–2463, https://doi.org/10.5194/amt-15-2433-2022, https://doi.org/10.5194/amt-15-2433-2022, 2022
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Space-borne greenhouse gas missions require ground-based validation networks capable of providing fiducial reference measurements. Here, considerable refinements of the calibration procedures for the COllaborative Carbon Column Observing Network (COCCON) are presented. Laboratory and solar side-by-side procedures for the characterization of the spectrometers have been refined and extended. Revised calibration factors for XCO2, XCO and XCH4 are provided, incorporating 47 new spectrometers.
David A. Newnham, Mark A. Clilverd, William D. J. Clark, Michael Kosch, Pekka T. Verronen, and Alan E. E. Rogers
Atmos. Meas. Tech., 15, 2361–2376, https://doi.org/10.5194/amt-15-2361-2022, https://doi.org/10.5194/amt-15-2361-2022, 2022
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Ozone (O3) is an important trace gas in the mesosphere and lower thermosphere (MLT), affecting heating rates and chemistry. O3 profiles measured by the Ny-Ålesund Ozone in the Mesosphere Instrument agree with Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) for winter night-time, but autumn twilight SABER abundances are up to 50 % higher. O3 abundances in the MLT from two different SABER channels also show significant differences for both autumn twilight and summer daytime.
Luca Egli, Julian Gröbner, Gregor Hülsen, Herbert Schill, and René Stübi
Atmos. Meas. Tech., 15, 1917–1930, https://doi.org/10.5194/amt-15-1917-2022, https://doi.org/10.5194/amt-15-1917-2022, 2022
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This study presents traceable total column ozone retrievals from direct solar spectral irradiance measurements. The retrieved ozone does not require any field calibration with a reference instrument as it is required for other operational network instruments such as Brewer or Dobson. Total column ozone can be retrieved with a traceable overall standard uncertainty of less than 0.8 % indicating a benchmark uncertainty for total column ozone measurements.
Yungang Wang, Liping Fu, Fang Jiang, Xiuqing Hu, Chengbao Liu, Xiaoxin Zhang, Jiawei Li, Zhipeng Ren, Fei He, Lingfeng Sun, Ling Sun, Zhongdong Yang, Peng Zhang, Jingsong Wang, and Tian Mao
Atmos. Meas. Tech., 15, 1577–1586, https://doi.org/10.5194/amt-15-1577-2022, https://doi.org/10.5194/amt-15-1577-2022, 2022
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Far-ultraviolet (FUV) airglow radiation is particularly well suited for space-based remote sensing. The Ionospheric Photometer (IPM) instrument carried aboard the Feng Yun 3-D satellite measures the spectral radiance of the Earth FUV airglow. IPM is a tiny, highly sensitive, and robust remote sensing instrument. Initial results demonstrate that the performance of IPM meets the designed requirement and therefore can be used to study the thermosphere and ionosphere in the future.
Leon Kuhn, Jonas Kuhn, Thomas Wagner, and Ulrich Platt
Atmos. Meas. Tech., 15, 1395–1414, https://doi.org/10.5194/amt-15-1395-2022, https://doi.org/10.5194/amt-15-1395-2022, 2022
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We present a novel instrument for imaging measurements of NO2 with high spatiotemporal resolution based on gas correlation spectroscopy, called the GCS NO2 camera. The instrument works by placing two gas cells (cuvettes) in front of two photosensor arrays, one filled with air and one filled with a high concentration of NO2, acting as a non-dispersive spectral filter. NO2 images are then generated on the basis of the signal ratio of the two channels in the spectral region of 430–445 nm.
Tobias Küchler, Stefan Noël, Heinrich Bovensmann, John Philip Burrows, Thomas Wagner, Christian Borger, Tobias Borsdorff, and Andreas Schneider
Atmos. Meas. Tech., 15, 297–320, https://doi.org/10.5194/amt-15-297-2022, https://doi.org/10.5194/amt-15-297-2022, 2022
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We applied the air-mass-corrected differential optical absorption spectroscopy (AMC-DOAS) method to derive total column water vapour (TCWV) from Sentinel-5P measurements and compared it to independent data sets. The correlation coefficients of typically more than 0.9 and the small deviations up to 2.5 kg m−2 reveal good agreement between our data product and other TCWV data sets. In particular for the different Sentinel-5P water vapour products, the deviations are around 1 kg m−2.
Jonas Kuhn, Nicole Bobrowski, Thomas Wagner, and Ulrich Platt
Atmos. Meas. Tech., 14, 7873–7892, https://doi.org/10.5194/amt-14-7873-2021, https://doi.org/10.5194/amt-14-7873-2021, 2021
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We propose spectrograph implementations using Fabry–Pérot interferometers for atmospheric trace gas remote sensing. Compared with widely used grating spectrographs, we find substantial light throughput and mobility advantages for high resolving powers. Besides lowering detection limits and increasing the spatial and temporal resolution of many atmospheric trace gas measurements, this approach might enable remote sensing of further important gases such as tropospheric OH radicals.
King-Fai Li, Ryan Khoury, Thomas J. Pongetti, Stanley P. Sander, Franklin P. Mills, and Yuk L. Yung
Atmos. Meas. Tech., 14, 7495–7510, https://doi.org/10.5194/amt-14-7495-2021, https://doi.org/10.5194/amt-14-7495-2021, 2021
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Nitrogen dioxide (NO2) plays a dominant role in the stratospheric ozone-destroying catalytic cycle. We have retrieved the diurnal cycle of NO2 over Table Mountain in Southern California, USA, during a week in October 2018. Under clean conditions, we are able to predict the diurnal cycle using standard photochemistry. On a day with significant pollution, we see the effect of NO2 sources in the nearby Los Angeles Basin.
Ulrich Platt, Thomas Wagner, Jonas Kuhn, and Thomas Leisner
Atmos. Meas. Tech., 14, 6867–6883, https://doi.org/10.5194/amt-14-6867-2021, https://doi.org/10.5194/amt-14-6867-2021, 2021
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Absorption spectroscopy of scattered sunlight is extremely useful for the analysis of atmospheric trace gas distributions. A central parameter for the achievable sensitivity of spectroscopic instruments is the light throughput, which can be enhanced in a number of ways. We present new ideas and considerations of how instruments could be optimized. Particular emphasis is on arrays of massively parallel instruments. Such arrays can reduce the size and weight of instruments by orders of magnitude.
Jonas Hamperl, Clément Capitaine, Jean-Baptiste Dherbecourt, Myriam Raybaut, Patrick Chazette, Julien Totems, Bruno Grouiez, Laurence Régalia, Rosa Santagata, Corinne Evesque, Jean-Michel Melkonian, Antoine Godard, Andrew Seidl, Harald Sodemann, and Cyrille Flamant
Atmos. Meas. Tech., 14, 6675–6693, https://doi.org/10.5194/amt-14-6675-2021, https://doi.org/10.5194/amt-14-6675-2021, 2021
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Laser active remote sensing of tropospheric water vapor is a promising technology for enhancing our understanding of processes governing the global hydrological cycle. We investigate the potential of a ground-based lidar to monitor the main water vapor isotopes at high spatio-temporal resolutions in the lower troposphere. Using a realistic end-to-end simulator, we show that high-precision measurements can be achieved within a range of 1.5 km, in mid-latitude or tropical environments.
Qin Wang, Farhan Mustafa, Lingbing Bu, Shouzheng Zhu, Jiqiao Liu, and Weibiao Chen
Atmos. Meas. Tech., 14, 6601–6617, https://doi.org/10.5194/amt-14-6601-2021, https://doi.org/10.5194/amt-14-6601-2021, 2021
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In this work, an airborne experiment was carried out to validate a newly developed CO2 monitoring IPDA lidar against the in situ measurements obtained from a commercial CO2 monitoring instrument installed on an aircraft. The XCO2 values calculated with the IPDA lidar measurements were compared with the dry-air CO2 mole fraction measurements obtained from the in situ instruments, and the results showed a good agreement between the two datasets.
Cited articles
Abautret, J., Perez, J. P., Evirgen, A., Rothman, J., Cordat, A., and Christol, P.: Characterization of midwave infrared InSb avalanche photodiode, J. Appl. Phys., 117, 244502, https://doi.org/10.1063/1.4922977, 2015.
Alimi, Y., Pusino, V., Steer, M. J., and Cumming, D. R. S.: InSb Avalanche Photodiodes on GaAs Substrates for Mid-Infrared Detection, IEEE T. Electron Dev., 67, 179–184, https://doi.org/10.1109/TED.2019.2956283, 2020.
Amediek, A., Fix, A., Ehret, G., Caron, J., and Durand, Y.: Airborne lidar reflectance measurements at 1.57 µm in support of the A-SCOPE mission for atmospheric CO2, Atmos. Meas. Tech., 2, 755–772, https://doi.org/10.5194/amt-2-755-2009, 2009.
Amediek, A., Ehret, G., Fix, A., Wirth, M., Büdenbender, C., Quatrevalet, M., Kiemle, C., and Gerbig, C.: CHARM-F – a new airborne integrated-path differential-absorption lidar for carbon dioxide and methane observations: measurement performance and quantification of strong point source emissions, Appl. Optics, 56, 5182–5197, https://doi.org/10.1364/AO.56.005182, 2017.
Arias, P. A., Bellouin, N., Coppola, E., Jones, R. G., Krinner, G., Marotzke, J., Naik, V., Palmer, M. D., Plattner, G.-K., Rogelj, J., Rojas, M., Sillmann, J., Storelvmo, T., Thorne, P. W., and Trewin, B.: Technical Summary, in: Climate Change 2021: The Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, United Kingdom and New York, USA, 33–144, https://doi.org/10.1017/9781009157896.002, 2021.
Baldridge, A. M., Hook, S. J., Grove, C. I. and Rivera, G.: The ASTER Spectral Library Version 2.0, Remote Sens. Environ., 113, 711–715, 2009.
Barton-Grimley, R. A., Nehrir, A. R., Kooi, S. A., Collins, J. E., Harper, D. B., Notari, A., Lee, J., DiGangi, J. P., Choi, Y., and Davis, K. J.: Evaluation of the High Altitude Lidar Observatory (HALO) methane retrievals during the summer 2019 ACT-America campaign, Atmos. Meas. Tech., 15, 4623–4650, https://doi.org/10.5194/amt-15-4623-2022, 2022.
Campbell, J. F., Lin, B., Dobler, J., Pal, S., Davis, K., Obland, M. D., Erxleben, W., McGregor, D., O'Dell, C., Bell, E., Weir, B., Fan, T.-F., Kooi, S., Gordon, I., Corbett, A., and Kochanov, R.: Field evaluation of column CO2 retrievals from intensity-modulated continuous-wave differential absorption lidar measurements during the ACT-America campaign, Earth and Space Science, 7, e2019EA000847, https://doi.org/10.1029/2019EA000847, 2020.
Charaev, I., Bandurin, D. A., Bollinger, A. T., Phinney, I. Y., Drozdov, I., Colangelo, M., Butters, B. A., Taniguchi, T., Watanabe, K., He, X., Medeiros, O., Božović, I., Jarillo-Herrero, P., and Berggren, K. K.: Single-photon detection using high-temperature superconductors, Nat. Nanotechnol., 18, 343–349, 2023.
Chen, J., Chen, J., Li, X., He, J., Yang, L., Wang, J., Yu, F., Zhao, Z., Shen, C., Guo, H., Li, G., Chen, X., and Lu, W. High-performance HgCdTe avalanche photodetector enabled with suppression of band-to-band tunneling effect in mid-wavelength infrared, npj Quantum Materials, 6, 103, https://doi.org/10.1038/s41535-021-00409-3, 2021.
Eckl, M., Roiger, A., Kostinek, J., Fiehn, A., Huntrieser, H., Knote, C., Barkley, Z. R., Ogle, S., Baier, B. C. Sweeney, C., and Davis, K. J.: Quantifying nitrous oxide emissions in the U.S. Midwest: A top-down study using high resolution airborne in situ observations, Geophys. Res. Lett., 48, e2020GL091266, https://doi.org/10.1029/2020GL091266, 2021.
Ehret, G. and Kiemle, C.: Requirements Definition for Future DIAL Instruments, ESA Study Final Report, ESA-CR(P)-4513, ESA Contract no. 10880/03/NL/FF, 2005.
Ehret, G., Kiemle, C., Wirth, M., Amediek, A., Fix, A., and Houweling, S.: Space-borne remote sensing of CO2, CH4, and N2O by integrated path differential absorption lidar: a sensitivity analysis, Appl. Phys. B, 90, 593–608, 2008.
Gardiner, T., Helmore, J., Innocenti, F., and Robinson, R.: Field Validation of Remote Sensing Methane Emission Measurements, Remote Sens.-Basel, 9, 956, https://doi.org/10.3390/rs9090956, 2017.
Gong, Y., Bu, L., Yang, B., and Mustafa, F.: High Repetition Rate Mid-Infrared Differential Absorption Lidar for Atmospheric Pollution Detection, Sensors-Basel, 20, 2211, https://doi.org/10.3390/s20082211, 2020.
Gordon, I. E., Rothman, L. S., Hargreaves, R. J., et al.: The HITRAN2020 molecular spectroscopic database, J. Quant. Spectrosc. Ra., 277, 107949, https://doi.org/10.1016/j.jqsrt.2021.107949, 2022.
Hoegstedt, L., Fix, A., Wirth, M., Pedersen, C., and Tidemand-Lichtenberg, P.: Upconversion-based lidar measurements of atmospheric CO2, Opt. Express, 24, 5152–5161, https://doi.org/10.1364/OE.24.005152, 2016.
Jacob, J. C., Menzies, R. T. and Spiers G. D.: Data Processing and Analysis Approach to Retrieve Carbon Dioxide Weighted-Column Mixing Ratio and 2-μm Reflectance With an Airborne Laser Absorption Spectrometer, IEEE T. Geosci. Remote, 57, 958–971, https://doi.org/10.1109/TGRS.2018.2863711, 2019.
Kiemle, C., Quatrevalet, M., Ehret, G., Amediek, A., Fix, A., and Wirth, M.: Sensitivity studies for a space-based methane lidar mission, Atmos. Meas. Tech., 4, 2195–2211, https://doi.org/10.5194/amt-4-2195-2011, 2011.
Kiemle, C., Ehret, G., Amediek, A., Fix, A., Quatrevalet, M., and Wirth, M.: Potential of Spaceborne Lidar Measurements of Carbon Dioxide and Methane Emissions from Strong Point Sources, Remote Sens.-Basel, 9, 1137, https://doi.org/10.3390/rs9111137, 2017.
Koch, G. J., Beyon, J. Y., Gibert, F., Barnes, B. W., Ismail, S., Petros, M., Petzar, P. J., Yu, J., Modlin, E. A., Davis, K. J., and Singh, U. N.: Side-line tunable laser transmitter for differential absorption lidar measurements of CO2: design and application to atmospheric measurements, Appl. Optics, 47, 944–956, 2008.
Kochanov, R. V., Gordon, I. E., Rothman, L. S., Wcislo, P., Hill, C., and Wilzewski, J. S.: HITRAN Application Programming Interface (HAPI): A comprehensive approach to working with spectroscopic data, J. Quant. Spectrosc. Ra., 177, 15–30, 2016.
Loos, J., Birk, M., and Wagner, G.: Pressure broadening, -shift, speed dependence and line mixing in the ν3 rovibrational band of N2O, J. Quant. Spectrosc. Ra., 151, 300–309, 2015.
Mao, J., Abshire, J. B., Kawa, S. R., Sun, X., and Riris, H.: Airborne lidar measurements of atmospheric CO2 column concentrations to cloud tops made during the 2017 ASCENDS/ABoVE campaign, Atmos. Meas. Tech., 17, 1061–1074, https://doi.org/10.5194/amt-17-1061-2024, 2024.
Martyniuk, P., Wang, P., Rogalski, A., Gu, Y., Jiang, R., Wang, F., and Hu, W.: Infrared avalanche photodiodes from bulk to 2D materials, Light: Science & Applications, 12, 212, https://doi.org/10.1038/s41377-023-01259-3, 2023.
Meng, L., Fix, A., Wirth, M., Hoegstedt, L., Tidemand-Lichtenberg, P., Pedersen, C., and Rodrigo, P. J.: Upconversion detector for range-resolved DIAL measurement of atmospheric CH4, Opt. Express, 26, 3850-3860, 2018.
Meerdink, S. K., Hook, S. J., Roberts, D. A., and Abbott, E. A.: The ECOSTRESS spectral library version 1.0, Remote Sens. Environ., 230, 111196, https://doi.org/10.1016/j.rse.2019.05.015, 2019.
Medina, M. A., Piotrowski, M., Schellhorn, M., Wagner, F. R., Berrou, A., and Hildenbrand-Dhollande, A.: Beam quality and efficiency of ns-pulsed high-power mid-IR ZGP OPOs compared in linear and non-planar ring resonators, Opt. Express, 29, 21727–21737, https://doi.org/10.1364/OE.430717, 2021.
Nemtchinov, V., Sun, C., and Varanasi, P.: Measurements of Line Intensities and Line Widths in the ν3-fundamental Band of Nitrous Oxide at Atmospheric Temperatures, J. Quant. Spectrosc. Ra., 83, 267–284, 2004.
Ngo, N. H., Lisak, D., Tran, H., and Hartmann, J.-M.: An isolated line-shape model to go beyond the Voigt profile in spectroscopic databases and radiative transfer codes, J. Quant. Spectrosc. Ra., 129, 89–100, https://doi.org/10.1016/j.jqsrt.2013.05.034, 2013.
Ren, T., Wu, C., Yu, Y., Dai, T., Chen, F., and Pan, Q.: Development Progress of 3–5 µm Mid-Infrared Lasers: OPO, Solid-State and Fiber Laser, Appl. Sci., 11, 11451, https://doi.org/10.3390/app112311451, 2021.
Ricaud, P., Attié, J.-L., Chalinel, R., Pasternak, F., Léonard, J., Pison, I., Pattey, E., Thompson, R. L., Zelinger, Z., Lelieveld, J., Sciare, J., Saitoh, N., Warner, J., Fortems-Cheiney, A., Reynal, H., Vidot, J., Brooker, L., Berdeu, L., Saint-Pé, O., Patra, P. K., Dostál, M., Suchánek, J., Nevrlý, V., and Zwaaftink, C. G.: The Monitoring Nitrous Oxide Sources (MIN2OS) satellite project, Remote Sens. Environ., 266, 112688, https://doi.org/10.1016/j.rse.2021.112688, 2021.
Robinson, R., Gardiner, T., Innocenti, F., Woods, P., and Coleman, M.: Infrared differential absorption Lidar (DIAL) measurements of hydrocarbon emissions, J. Environ. Monitor., 13, 2213–2220, https://doi.org/10.1039/C0EM00312C, 2011.
Spiers, G. D., Menzies, R. T., Jacob, J., Christensen, L. E., Phillips, M. W., Choi, Y., and Browell, E. V.: Atmospheric CO2 measurements with a 2 µm airborne laser absorption spectrometer employing coherent detection, Appl. Optics, 50, 2098–2111, https://doi.org/10.1364/AO.50.002098, 2011.
Stull, R.: Practical Meteorology: An Algebra-based Survey of Atmospheric Science, version 1.02b, Univ. of British Columbia, 940 pp., ISBN 978-0-88865-283-6, 2017.
Sun, X., Abshire, J. B., Beck, J. D., Mitra, P., Reiff, K., and Yang, G.: HgCdTe avalanche photodiode detectors for airborne and spaceborne lidar at infrared wavelengths, Opt. Express, 25, 16589–16602, https://doi.org/10.1364/OE.25.016589, 2017.
Sun, X., Abshire, J. B., Ramanathan, A., Kawa, S. R., and Mao, J.: Retrieval algorithm for the column CO2 mixing ratio from pulsed multi-wavelength lidar measurements, Atmos. Meas. Tech., 14, 3909–3922, https://doi.org/10.5194/amt-14-3909-2021, 2021.
Tian, H., Pan, N., Thompson, R. L., Canadell, J. G., Suntharalingam, P., Regnier, P., Davidson, E. A., Prather, M., Ciais, P., Muntean, M., Pan, S., Winiwarter, W., Zaehle, S., Zhou, F., Jackson, R. B., Bange, H. W., Berthet, S., Bian, Z., Bianchi, D., Bouwman, A. F., Buitenhuis, E. T., Dutton, G., Hu, M., Ito, A., Jain, A. K., Jeltsch-Thömmes, A., Joos, F., Kou-Giesbrecht, S., Krummel, P. B., Lan, X., Landolfi, A., Lauerwald, R., Li, Y., Lu, C., Maavara, T., Manizza, M., Millet, D. B., Mühle, J., Patra, P. K., Peters, G. P., Qin, X., Raymond, P., Resplandy, L., Rosentreter, J. A., Shi, H., Sun, Q., Tonina, D., Tubiello, F. N., van der Werf, G. R., Vuichard, N., Wang, J., Wells, K. C., Western, L. M., Wilson, C., Yang, J., Yao, Y., You, Y., and Zhu, Q.: Global nitrous oxide budget (1980–2020), Earth Syst. Sci. Data, 16, 2543–2604, https://doi.org/10.5194/essd-16-2543-2024, 2024.
Vandenbussche, S., Langerock, B., Vigouroux, C., Buschmann, M., Deutscher, N. M., Feist, D. G., García, O., Hannigan, J. W., Hase, F., Kivi, R., Kumps, N., Makarova, M., Millet, D. B., Morino, I., Nagahama, T., Notholt, J., Ohyama, H., Ortega, I., Petri, C., Rettinger, M., Schneider, M., Servais, C. P., Sha, M. K., Shiomi, K., Smale, D., Strong, K., Sussmann, R., Té, Y., Velazco, V. A., Vrekoussis, M., Warneke, T., Wells, K. C., Wunch, D., Zhou, M., and De Mazière, M.: Nitrous Oxide Profiling from Infrared Radiances (NOPIR): Algorithm Description, Application to 10 Years of IASI Observations and Quality Assessment, Remote Sens.-Basel, 14, 1810. https://doi.org/10.3390/rs14081810, 2022.
Vaughan, J. M., Brown, D. W., Nash, C., Alejandro, S. B., and Koenig, G. G.: Atlantic Atmospheric Aerosol Studies: 2. Compendium of Airborne Backscatter Measurements at 10.6 µm, J. Geophys. Res.-Atmos., 100, 1043–1065, https://doi.org/10.1029/94JD01817, 1995.
Vaughan, J. M., Geddes, N. J., Flamant P. H., and Flesia, C.: Establishment of a backscatter coefficient and atmospheric database, DERA Report for ESA Contract no. 12510/97/NL/RE, DERA/EL/ISET/CR980139/1.0, 1998.
Vodopyanov, K. L.: Laser-Based Mid-infrared Sources and Applications, John Wiley & Sons, Incorporated, https://doi.org/10.1002/9781119074557, Print ISBN: 9781118301814, Online ISBN: 9781119074557, 2020.
Waldmann, P., Eckl, M., Gottschaldt, K.-D., Knez, L., Förster, E., Mallaun, C., Röckmann, T., Hutjes, R., Chen, H., Gerbig, C., Galkowski, M., Kiemle, C., and Roiger, A.: Quantifying agricultural CH4 and N2O emissions of the Netherlands using a novel airborne eddy-covariance measurements system: First results of the GHGMon campaign in June 2023, EGU General Assembly 2024, Vienna, Austria, 14–19 Apr 2024, EGU24-19467, https://doi.org/10.5194/egusphere-egu24-19467, 2024.
WMO: Global Greenhouse Gas Watch (G3W), https://wmo.int/activities/global-greenhouse-gas-watch-g3w (last access: 12 November 2024), 2024.
Yu, S., Guo, K., Li, S., Han, H., Zhang, Z., and Xia, H.: Three-dimensional detection of CO2 and wind using a 1.57 µm coherent differential absorption lidar, Opt. Express 32, 21134–21148, https://doi.org/10.1364/OE.523904, 2024.
Short summary
Nitrous oxide is the third most important greenhouse gas modified by human activities after carbon dioxide and methane. This study examines the feasibility of airborne differential absorption lidar to quantify emissions from agriculture, fossil fuel combustion, industry, and biomass burning. Simulations show that a technically realizable and affordable mid-infrared lidar system will be able to measure the nitrous oxide column concentration enhancements with sufficient precision.
Nitrous oxide is the third most important greenhouse gas modified by human activities after...
