Articles | Volume 18, issue 8
https://doi.org/10.5194/amt-18-1717-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-18-1717-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
22 Apr 2025
Research article |
| 22 Apr 2025
| 22 Apr 2025
Revised methodology for CO2 and CH4 measurements at remote sites using a working standard-gas-saving system
Motoki Sasakawa
CORRESPONDING AUTHOR
Center for Global Environmental Research, Earth System Division, National Institute for Environmental Studies, Tsukuba, 305-8506, Japan
Noritsugu Tsuda
Global Environmental Forum, Tsukuba, 305-0061, Japan
Toshinobu Machida
Center for Global Environmental Research, Earth System Division, National Institute for Environmental Studies, Tsukuba, 305-8506, Japan
Mikhail Arshinov
V.E. Zuev Institute of Atmospheric Optics, Russian Academy of Sciences, Siberian Branch, Tomsk, Russia
Denis Davydov
V.E. Zuev Institute of Atmospheric Optics, Russian Academy of Sciences, Siberian Branch, Tomsk, Russia
Aleksandr Fofonov
V.E. Zuev Institute of Atmospheric Optics, Russian Academy of Sciences, Siberian Branch, Tomsk, Russia
Boris Belan
V.E. Zuev Institute of Atmospheric Optics, Russian Academy of Sciences, Siberian Branch, Tomsk, Russia
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Satellite remote sensing of atmospheric mixing ratios of greenhouse gases (GHGs) can provide information on the emissions of these GHGs. This study presents a novel method to use atmospheric column mixing ratios with a Lagrangian model of atmospheric transport to estimate GHG emissions. This method can reduce model errors resulting from how an observation is represented by an atmospheric model potentially reducing the errors in the GHG emissions derived.
Sophie Wittig, Antoine Berchet, Isabelle Pison, Marielle Saunois, Joël Thanwerdas, Adrien Martinez, Jean-Daniel Paris, Toshinobu Machida, Motoki Sasakawa, Douglas E. J. Worthy, Xin Lan, Rona L. Thompson, Espen Sollum, and Mikhail Arshinov
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Sourish Basu, Xin Lan, Edward Dlugokencky, Sylvia Michel, Stefan Schwietzke, John B. Miller, Lori Bruhwiler, Youmi Oh, Pieter P. Tans, Francesco Apadula, Luciana V. Gatti, Armin Jordan, Jaroslaw Necki, Motoki Sasakawa, Shinji Morimoto, Tatiana Di Iorio, Haeyoung Lee, Jgor Arduini, and Giovanni Manca
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Atmospheric methane (CH4) has been growing steadily since 2007 for reasons that are not well understood. Here we determine sources of methane using a technique informed by atmospheric measurements of CH4 and its isotopologue 13CH4. Measurements of 13CH4 provide for better separation of microbial, fossil, and fire sources of methane than CH4 measurements alone. Compared to previous assessments such as the Global Carbon Project, we find a larger microbial contribution to the post-2007 increase.
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James S. Wang, S. Randolph Kawa, G. James Collatz, Motoki Sasakawa, Luciana V. Gatti, Toshinobu Machida, Yuping Liu, and Michael E. Manyin
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Satellite remote sensing of atmospheric mixing ratios of greenhouse gases (GHGs) can provide information on the emissions of these GHGs. This study presents a novel method to use atmospheric column mixing ratios with a Lagrangian model of atmospheric transport to estimate GHG emissions. This method can reduce model errors resulting from how an observation is represented by an atmospheric model potentially reducing the errors in the GHG emissions derived.
Anastasia Lampilahti, Olga Garmash, Diego Aliaga, Mikhail Arshinov, Denis Davydov, Boris Belan, Janne Lampilahti, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Ekaterina Ezhova
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Chiranjit Das, Ravi Kumar Kunchala, Prabir K. Patra, Naveen Chandra, Kentaro Ishijima, and Toshinobu Machida
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Preprint archived
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Our study compares model CO2 with aircraft and OCO-2 data to identify transport model errors to better policy-related flux estimation. The model align better with aircraft data than satellite data, especially over oceans, but struggles near the surface due to inaccurate CO2 estimates. Over the Amazon and Asian megacities, differences arise from limited measurements and coarse model resolution, highlighting the need for improved monitoring and higher-resolution data to capture emissions better.
Astrid Müller, Hiroshi Tanimoto, Takafumi Sugita, Prabir K. Patra, Shin-ichiro Nakaoka, Toshinobu Machida, Isamu Morino, André Butz, and Kei Shiomi
Atmos. Meas. Tech., 17, 1297–1316, https://doi.org/10.5194/amt-17-1297-2024, https://doi.org/10.5194/amt-17-1297-2024, 2024
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Satellite CH4 observations with high accuracy are needed to understand changes in atmospheric CH4 concentrations. But over oceans, reference data are limited. We combine various ship and aircraft observations with the help of atmospheric chemistry models to derive observation-based column-averaged mixing ratios of CH4 (obs. XCH4). We discuss three different approaches and demonstrate the applicability of the new reference dataset for carbon cycle studies and satellite evaluation.
Sophie Wittig, Antoine Berchet, Isabelle Pison, Marielle Saunois, Joël Thanwerdas, Adrien Martinez, Jean-Daniel Paris, Toshinobu Machida, Motoki Sasakawa, Douglas E. J. Worthy, Xin Lan, Rona L. Thompson, Espen Sollum, and Mikhail Arshinov
Atmos. Chem. Phys., 23, 6457–6485, https://doi.org/10.5194/acp-23-6457-2023, https://doi.org/10.5194/acp-23-6457-2023, 2023
Short summary
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Here, an inverse modelling approach is applied to estimate CH4 sources and sinks in the Arctic from 2008 to 2019. We study the magnitude, seasonal patterns and trends from different sources during recent years. We also assess how the current observation network helps to constrain fluxes. We find that constraints are only significant for North America and, to a lesser extent, West Siberia, where the observation network is relatively dense. We find no clear trend over the period of inversion.
Clément Narbaud, Jean-Daniel Paris, Sophie Wittig, Antoine Berchet, Marielle Saunois, Philippe Nédélec, Boris D. Belan, Mikhail Y. Arshinov, Sergei B. Belan, Denis Davydov, Alexander Fofonov, and Artem Kozlov
Atmos. Chem. Phys., 23, 2293–2314, https://doi.org/10.5194/acp-23-2293-2023, https://doi.org/10.5194/acp-23-2293-2023, 2023
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We measured CH4 and CO2 from aircraft over the Russian Arctic. Analyzing our data with the Lagrangian model FLEXPART, we find a sharp east–west gradient in atmospheric composition. Western Siberia is influenced by strong wetland CH4 emissions, deep CO2 gradient from biospheric uptake, and long-range transport from Europe and North America. Eastern flights document less variability. Over the Arctic Ocean, we find a small influence from marine CH4 emissions compatible with reasonable inventories.
Sourish Basu, Xin Lan, Edward Dlugokencky, Sylvia Michel, Stefan Schwietzke, John B. Miller, Lori Bruhwiler, Youmi Oh, Pieter P. Tans, Francesco Apadula, Luciana V. Gatti, Armin Jordan, Jaroslaw Necki, Motoki Sasakawa, Shinji Morimoto, Tatiana Di Iorio, Haeyoung Lee, Jgor Arduini, and Giovanni Manca
Atmos. Chem. Phys., 22, 15351–15377, https://doi.org/10.5194/acp-22-15351-2022, https://doi.org/10.5194/acp-22-15351-2022, 2022
Short summary
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Atmospheric methane (CH4) has been growing steadily since 2007 for reasons that are not well understood. Here we determine sources of methane using a technique informed by atmospheric measurements of CH4 and its isotopologue 13CH4. Measurements of 13CH4 provide for better separation of microbial, fossil, and fire sources of methane than CH4 measurements alone. Compared to previous assessments such as the Global Carbon Project, we find a larger microbial contribution to the post-2007 increase.
Boris D. Belan, Gerard Ancellet, Irina S. Andreeva, Pavel N. Antokhin, Viktoria G. Arshinova, Mikhail Y. Arshinov, Yurii S. Balin, Vladimir E. Barsuk, Sergei B. Belan, Dmitry G. Chernov, Denis K. Davydov, Alexander V. Fofonov, Georgii A. Ivlev, Sergei N. Kotel'nikov, Alexander S. Kozlov, Artem V. Kozlov, Katharine Law, Andrey V. Mikhal'chishin, Igor A. Moseikin, Sergei V. Nasonov, Philippe Nédélec, Olesya V. Okhlopkova, Sergei E. Ol'kin, Mikhail V. Panchenko, Jean-Daniel Paris, Iogannes E. Penner, Igor V. Ptashnik, Tatyana M. Rasskazchikova, Irina K. Reznikova, Oleg A. Romanovskii, Alexander S. Safatov, Denis E. Savkin, Denis V. Simonenkov, Tatyana K. Sklyadneva, Gennadii N. Tolmachev, Semyon V. Yakovlev, and Polina N. Zenkova
Atmos. Meas. Tech., 15, 3941–3967, https://doi.org/10.5194/amt-15-3941-2022, https://doi.org/10.5194/amt-15-3941-2022, 2022
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The change of the global climate is most pronounced in the Arctic, where the air temperature increases faster than the global average. This is associated with an increase in the concentration of greenhouse gases in the atmosphere. It is important to study how the air composition in the Arctic changes in the changing climate. Thus this integrated experiment was carried out to measure the composition of the troposphere in the Russian sector of the Arctic from on board the aircraft laboratory.
Hanna K. Lappalainen, Tuukka Petäjä, Timo Vihma, Jouni Räisänen, Alexander Baklanov, Sergey Chalov, Igor Esau, Ekaterina Ezhova, Matti Leppäranta, Dmitry Pozdnyakov, Jukka Pumpanen, Meinrat O. Andreae, Mikhail Arshinov, Eija Asmi, Jianhui Bai, Igor Bashmachnikov, Boris Belan, Federico Bianchi, Boris Biskaborn, Michael Boy, Jaana Bäck, Bin Cheng, Natalia Chubarova, Jonathan Duplissy, Egor Dyukarev, Konstantinos Eleftheriadis, Martin Forsius, Martin Heimann, Sirkku Juhola, Vladimir Konovalov, Igor Konovalov, Pavel Konstantinov, Kajar Köster, Elena Lapshina, Anna Lintunen, Alexander Mahura, Risto Makkonen, Svetlana Malkhazova, Ivan Mammarella, Stefano Mammola, Stephany Buenrostro Mazon, Outi Meinander, Eugene Mikhailov, Victoria Miles, Stanislav Myslenkov, Dmitry Orlov, Jean-Daniel Paris, Roberta Pirazzini, Olga Popovicheva, Jouni Pulliainen, Kimmo Rautiainen, Torsten Sachs, Vladimir Shevchenko, Andrey Skorokhod, Andreas Stohl, Elli Suhonen, Erik S. Thomson, Marina Tsidilina, Veli-Pekka Tynkkynen, Petteri Uotila, Aki Virkkula, Nadezhda Voropay, Tobias Wolf, Sayaka Yasunaka, Jiahua Zhang, Yubao Qiu, Aijun Ding, Huadong Guo, Valery Bondur, Nikolay Kasimov, Sergej Zilitinkevich, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 22, 4413–4469, https://doi.org/10.5194/acp-22-4413-2022, https://doi.org/10.5194/acp-22-4413-2022, 2022
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We summarize results during the last 5 years in the northern Eurasian region, especially from Russia, and introduce recent observations of the air quality in the urban environments in China. Although the scientific knowledge in these regions has increased, there are still gaps in our understanding of large-scale climate–Earth surface interactions and feedbacks. This arises from limitations in research infrastructures and integrative data analyses, hindering a comprehensive system analysis.
Shohei Nomura, Manish Naja, M. Kawser Ahmed, Hitoshi Mukai, Yukio Terao, Toshinobu Machida, Motoki Sasakawa, and Prabir K. Patra
Atmos. Chem. Phys., 21, 16427–16452, https://doi.org/10.5194/acp-21-16427-2021, https://doi.org/10.5194/acp-21-16427-2021, 2021
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Long-term measurements of greenhouse gases (GHGs) in India and Bangladesh unveiled specific characteristics in their variations in these regions. Plants including rice cultivated in winter and summer strongly affected seasonal variations and levels in CO2 and CH4. Long-term variability of GHGs showed quite different features in their growth rates from those in Mauna Loa. GHG trends in this region seemed to be hardly affected by El Niño–Southern Oscillation (ENSO).
Helmi Uusitalo, Jenni Kontkanen, Ilona Ylivinkka, Ekaterina Ezhova, Anastasiia Demakova, Mikhail Arshinov, Boris Denisovich Belan, Denis Davydov, Nan Ma, Tuukka Petäjä, Alfred Wiedensohler, Markku Kulmala, and Tuomo Nieminen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-530, https://doi.org/10.5194/acp-2021-530, 2021
Publication in ACP not foreseen
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Characteristics of formation of atmospheric aerosol at four boreal forest sites in Finland and Russian Siberia was analyzed. Our results provide information on the governing processes of atmospheric aerosol formation in the boreal forest area, which a substantial part of the continental biosphere. Aerosol formation was occurring less frequently at Siberian than in Finnish sites, which was affected by the lower particle growth rates and higher loss rates in Siberia.
Yosuke Niwa, Yousuke Sawa, Hideki Nara, Toshinobu Machida, Hidekazu Matsueda, Taku Umezawa, Akihiko Ito, Shin-Ichiro Nakaoka, Hiroshi Tanimoto, and Yasunori Tohjima
Atmos. Chem. Phys., 21, 9455–9473, https://doi.org/10.5194/acp-21-9455-2021, https://doi.org/10.5194/acp-21-9455-2021, 2021
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Fires in Equatorial Asia release a large amount of carbon into the atmosphere. Extensively using high-precision atmospheric carbon dioxide (CO2) data from a commercial aircraft observation project, we estimated fire carbon emissions in Equatorial Asia induced by the big El Niño event in 2015. Additional shipboard measurement data elucidated the validity of the analysis and the best estimate indicated 273 Tg C for fire emissions during September–October 2015.
Astrid Müller, Hiroshi Tanimoto, Takafumi Sugita, Toshinobu Machida, Shin-ichiro Nakaoka, Prabir K. Patra, Joshua Laughner, and David Crisp
Atmos. Chem. Phys., 21, 8255–8271, https://doi.org/10.5194/acp-21-8255-2021, https://doi.org/10.5194/acp-21-8255-2021, 2021
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Over oceans, high uncertainties in satellite CO2 retrievals exist due to limited reference data. We combine commercial ship and aircraft observations and, with the aid of model calculations, obtain column-averaged mixing ratios of CO2 (XCO2) data over the Pacific Ocean. This new dataset has great potential as a robust reference for XCO2 measured from space and can help to better understand changes in the carbon cycle in response to climate change using satellite observations.
Thomas Thorp, Stephen R. Arnold, Richard J. Pope, Dominick V. Spracklen, Luke Conibear, Christoph Knote, Mikhail Arshinov, Boris Belan, Eija Asmi, Tuomas Laurila, Andrei I. Skorokhod, Tuomo Nieminen, and Tuukka Petäjä
Atmos. Chem. Phys., 21, 4677–4697, https://doi.org/10.5194/acp-21-4677-2021, https://doi.org/10.5194/acp-21-4677-2021, 2021
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We compare modelled near-surface pollutants with surface and satellite observations to better understand the controls on the regional concentrations of pollution in western Siberia for late spring and summer in 2011. We find two commonly used emission inventories underestimate human emissions when compared to observations. Transport emissions are the main source of pollutants within the region during this period, whilst fire emissions peak during June and are only significant south of 60° N.
Shamil Maksyutov, Tomohiro Oda, Makoto Saito, Rajesh Janardanan, Dmitry Belikov, Johannes W. Kaiser, Ruslan Zhuravlev, Alexander Ganshin, Vinu K. Valsala, Arlyn Andrews, Lukasz Chmura, Edward Dlugokencky, László Haszpra, Ray L. Langenfelds, Toshinobu Machida, Takakiyo Nakazawa, Michel Ramonet, Colm Sweeney, and Douglas Worthy
Atmos. Chem. Phys., 21, 1245–1266, https://doi.org/10.5194/acp-21-1245-2021, https://doi.org/10.5194/acp-21-1245-2021, 2021
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In order to improve the top-down estimation of the anthropogenic greenhouse gas emissions, a high-resolution inverse modelling technique was developed for applications to global transport modelling of carbon dioxide and other greenhouse gases. A coupled Eulerian–Lagrangian transport model and its adjoint are combined with surface fluxes at 0.1° resolution to provide high-resolution forward simulation and inverse modelling of surface fluxes accounting for signals from emission hot spots.
Tuukka Petäjä, Ella-Maria Duplissy, Ksenia Tabakova, Julia Schmale, Barbara Altstädter, Gerard Ancellet, Mikhail Arshinov, Yurii Balin, Urs Baltensperger, Jens Bange, Alison Beamish, Boris Belan, Antoine Berchet, Rossana Bossi, Warren R. L. Cairns, Ralf Ebinghaus, Imad El Haddad, Beatriz Ferreira-Araujo, Anna Franck, Lin Huang, Antti Hyvärinen, Angelika Humbert, Athina-Cerise Kalogridis, Pavel Konstantinov, Astrid Lampert, Matthew MacLeod, Olivier Magand, Alexander Mahura, Louis Marelle, Vladimir Masloboev, Dmitri Moisseev, Vaios Moschos, Niklas Neckel, Tatsuo Onishi, Stefan Osterwalder, Aino Ovaska, Pauli Paasonen, Mikhail Panchenko, Fidel Pankratov, Jakob B. Pernov, Andreas Platis, Olga Popovicheva, Jean-Christophe Raut, Aurélie Riandet, Torsten Sachs, Rosamaria Salvatori, Roberto Salzano, Ludwig Schröder, Martin Schön, Vladimir Shevchenko, Henrik Skov, Jeroen E. Sonke, Andrea Spolaor, Vasileios K. Stathopoulos, Mikko Strahlendorff, Jennie L. Thomas, Vito Vitale, Sterios Vratolis, Carlo Barbante, Sabine Chabrillat, Aurélien Dommergue, Konstantinos Eleftheriadis, Jyri Heilimo, Kathy S. Law, Andreas Massling, Steffen M. Noe, Jean-Daniel Paris, André S. H. Prévôt, Ilona Riipinen, Birgit Wehner, Zhiyong Xie, and Hanna K. Lappalainen
Atmos. Chem. Phys., 20, 8551–8592, https://doi.org/10.5194/acp-20-8551-2020, https://doi.org/10.5194/acp-20-8551-2020, 2020
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The role of polar regions is increasing in terms of megatrends such as globalization, new transport routes, demography, and the use of natural resources with consequent effects on regional and transported pollutant concentrations. Here we summarize initial results from our integrative project exploring the Arctic environment and pollution to deliver data products, metrics, and indicators for stakeholders.
Marielle Saunois, Ann R. Stavert, Ben Poulter, Philippe Bousquet, Josep G. Canadell, Robert B. Jackson, Peter A. Raymond, Edward J. Dlugokencky, Sander Houweling, Prabir K. Patra, Philippe Ciais, Vivek K. Arora, David Bastviken, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Kimberly M. Carlson, Mark Carrol, Simona Castaldi, Naveen Chandra, Cyril Crevoisier, Patrick M. Crill, Kristofer Covey, Charles L. Curry, Giuseppe Etiope, Christian Frankenberg, Nicola Gedney, Michaela I. Hegglin, Lena Höglund-Isaksson, Gustaf Hugelius, Misa Ishizawa, Akihiko Ito, Greet Janssens-Maenhout, Katherine M. Jensen, Fortunat Joos, Thomas Kleinen, Paul B. Krummel, Ray L. Langenfelds, Goulven G. Laruelle, Licheng Liu, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Joe McNorton, Paul A. Miller, Joe R. Melton, Isamu Morino, Jurek Müller, Fabiola Murguia-Flores, Vaishali Naik, Yosuke Niwa, Sergio Noce, Simon O'Doherty, Robert J. Parker, Changhui Peng, Shushi Peng, Glen P. Peters, Catherine Prigent, Ronald Prinn, Michel Ramonet, Pierre Regnier, William J. Riley, Judith A. Rosentreter, Arjo Segers, Isobel J. Simpson, Hao Shi, Steven J. Smith, L. Paul Steele, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Francesco N. Tubiello, Aki Tsuruta, Nicolas Viovy, Apostolos Voulgarakis, Thomas S. Weber, Michiel van Weele, Guido R. van der Werf, Ray F. Weiss, Doug Worthy, Debra Wunch, Yi Yin, Yukio Yoshida, Wenxin Zhang, Zhen Zhang, Yuanhong Zhao, Bo Zheng, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Earth Syst. Sci. Data, 12, 1561–1623, https://doi.org/10.5194/essd-12-1561-2020, https://doi.org/10.5194/essd-12-1561-2020, 2020
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Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. We have established a consortium of multidisciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate new research aimed at improving and regularly updating the global methane budget. This is the second version of the review dedicated to the decadal methane budget, integrating results of top-down and bottom-up estimates.
Antonin Zabukovec, Gerard Ancellet, Iwan E. Penner, Mikhail Arshinov, Valery Kozlov, Jacques Pelon, Jean-Daniel Paris, Grigory Kokhanenko, Yuri S. Balin, Dmitry Chernov, and Boris D. Belan
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-195, https://doi.org/10.5194/acp-2020-195, 2020
Preprint withdrawn
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Description of two aircraft campaigns results carried out over Siberia in 2013 and 2017 to characterize aerosol emission. A methodology is proposed to derive the aerosol types using transport model and satellite observations. The extinction to backscatter ratio for each aerosol types is reported as it is a key parameter to constrain their radiative impact. These results are compared to previous work conducted in other regions and to aerosol data products observed by spaceborne lidars.
Mai Ouchi, Yutaka Matsumi, Tomoki Nakayama, Kensaku Shimizu, Takehiko Sawada, Toshinobu Machida, Hidekazu Matsueda, Yousuke Sawa, Isamu Morino, Osamu Uchino, Tomoaki Tanaka, and Ryoichi Imasu
Atmos. Meas. Tech., 12, 5639–5653, https://doi.org/10.5194/amt-12-5639-2019, https://doi.org/10.5194/amt-12-5639-2019, 2019
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A novel, practical observation system for measuring tropospheric carbon dioxide (CO2) concentrations carried by a small helium-filled balloon (CO2 sonde) has been developed for the first time. The low-cost CO2 sondes can potentially be used for frequent measurements of vertical profiles of CO2 in any parts of the world, providing useful information to understand the global and regional carbon budgets by replenishing the present sparse observation coverage.
Yasunori Tohjima, Hitoshi Mukai, Toshinobu Machida, Yu Hoshina, and Shin-Ichiro Nakaoka
Atmos. Chem. Phys., 19, 9269–9285, https://doi.org/10.5194/acp-19-9269-2019, https://doi.org/10.5194/acp-19-9269-2019, 2019
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The amount of fossil-fuel-derived carbon dioxide that was taken up by land biosphere and ocean was evaluated from atmospheric carbon dioxide and oxygen observations in the western Pacific over a 15-year period. The results showed that about 30 % and 17 % of the fossil-fuel-derived carbon dioxide emitted during a 17-year period (2000–2016) was taken up by the ocean and land sinks, respectively. Long-term trends of land and ocean sinks for the decadal period were also evaluated.
Yoichi Inai, Ryo Fujita, Toshinobu Machida, Hidekazu Matsueda, Yousuke Sawa, Kazuhiro Tsuboi, Keiichi Katsumata, Shinji Morimoto, Shuji Aoki, and Takakiyo Nakazawa
Atmos. Chem. Phys., 19, 7073–7103, https://doi.org/10.5194/acp-19-7073-2019, https://doi.org/10.5194/acp-19-7073-2019, 2019
Ekaterina Ezhova, Ilona Ylivinkka, Joel Kuusk, Kaupo Komsaare, Marko Vana, Alisa Krasnova, Steffen Noe, Mikhail Arshinov, Boris Belan, Sung-Bin Park, Jošt Valentin Lavrič, Martin Heimann, Tuukka Petäjä, Timo Vesala, Ivan Mammarella, Pasi Kolari, Jaana Bäck, Üllar Rannik, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 18, 17863–17881, https://doi.org/10.5194/acp-18-17863-2018, https://doi.org/10.5194/acp-18-17863-2018, 2018
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Understanding the connections between aerosols, solar radiation and photosynthesis in terrestrial ecosystems is important for estimates of the CO2 balance in the atmosphere. Atmospheric aerosols and clouds influence solar radiation. In this study, we quantify the aerosol effect on solar radiation in boreal forests and study forest ecosystems response to this change in the radiation conditions. The analysis is based on atmospheric observations from several remote stations in Eurasian forests.
Christine D. Groot Zwaaftink, Stephan Henne, Rona L. Thompson, Edward J. Dlugokencky, Toshinobu Machida, Jean-Daniel Paris, Motoki Sasakawa, Arjo Segers, Colm Sweeney, and Andreas Stohl
Geosci. Model Dev., 11, 4469–4487, https://doi.org/10.5194/gmd-11-4469-2018, https://doi.org/10.5194/gmd-11-4469-2018, 2018
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A Lagrangian particle dispersion model is used to simulate global fields of methane, constrained by observations through nudging. We show that this rather simple and computationally inexpensive method can give results similar to or as good as a computationally expensive Eulerian chemistry transport model with a data assimilation scheme. The three-dimensional methane fields are of interest to applications such as inverse modelling and satellite retrievals.
Igor B. Konovalov, Daria A. Lvova, Matthias Beekmann, Hiren Jethva, Eugene F. Mikhailov, Jean-Daniel Paris, Boris D. Belan, Valerii S. Kozlov, Philippe Ciais, and Meinrat O. Andreae
Atmos. Chem. Phys., 18, 14889–14924, https://doi.org/10.5194/acp-18-14889-2018, https://doi.org/10.5194/acp-18-14889-2018, 2018
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A good knowledge of black carbon (BC) emissions from open biomass burning (BB) is an important prerequisite for reliable climate predictions, especially in the Arctic. This paper introduces a method to constrain a regional budget of BB BC emissions using satellite measurements of the absorption and extinction optical depths and evaluates its potential application in a large Siberian region.
Taku Umezawa, Hidekazu Matsueda, Yousuke Sawa, Yosuke Niwa, Toshinobu Machida, and Lingxi Zhou
Atmos. Chem. Phys., 18, 14851–14866, https://doi.org/10.5194/acp-18-14851-2018, https://doi.org/10.5194/acp-18-14851-2018, 2018
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Distribution of atmospheric CO2 is key to estimate surface CO2 sources and sinks. We present extensive analysis of a unique 10-year three-dimensional dataset of atmospheric CO2 achieved by the CONTRAIL commercial airliner measurements over the Asia-Pacific region. Aided by model simulations, we identified the influence of anthropogenic and biospheric CO2 fluxes in the seasonal evolution of the spatial CO2 distributions under the seasonally varying meteorology (e.g., Asian summer monsoon)
Tuomo Nieminen, Veli-Matti Kerminen, Tuukka Petäjä, Pasi P. Aalto, Mikhail Arshinov, Eija Asmi, Urs Baltensperger, David C. S. Beddows, Johan Paul Beukes, Don Collins, Aijun Ding, Roy M. Harrison, Bas Henzing, Rakesh Hooda, Min Hu, Urmas Hõrrak, Niku Kivekäs, Kaupo Komsaare, Radovan Krejci, Adam Kristensson, Lauri Laakso, Ari Laaksonen, W. Richard Leaitch, Heikki Lihavainen, Nikolaos Mihalopoulos, Zoltán Németh, Wei Nie, Colin O'Dowd, Imre Salma, Karine Sellegri, Birgitta Svenningsson, Erik Swietlicki, Peter Tunved, Vidmantas Ulevicius, Ville Vakkari, Marko Vana, Alfred Wiedensohler, Zhijun Wu, Annele Virtanen, and Markku Kulmala
Atmos. Chem. Phys., 18, 14737–14756, https://doi.org/10.5194/acp-18-14737-2018, https://doi.org/10.5194/acp-18-14737-2018, 2018
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Atmospheric aerosols have diverse effects on air quality, human health, and global climate. One important source of aerosols is their formation via nucleation and growth in the atmosphere. We have analyzed long-term observations of regional new particle formation events around the globe and provide a comprehensive view on the characteristics of this phenomenon in diverse environments. The results are useful in developing more realistic representation of atmospheric aerosols in global models.
James S. Wang, S. Randolph Kawa, G. James Collatz, Motoki Sasakawa, Luciana V. Gatti, Toshinobu Machida, Yuping Liu, and Michael E. Manyin
Atmos. Chem. Phys., 18, 11097–11124, https://doi.org/10.5194/acp-18-11097-2018, https://doi.org/10.5194/acp-18-11097-2018, 2018
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We used measurements of CO2 in the atmosphere from the GOSAT satellite and from surface sites around the world, together with a transport model and a unique estimation technique, to quantify CO2 sources and removals over a recent period. We find that climate variations can strongly influence uptake by vegetation and release in decay and fires. However, regional gaps in observations and inaccuracies to which current satellite technology is susceptible result in important estimation biases.
Filippo Xausa, Pauli Paasonen, Risto Makkonen, Mikhail Arshinov, Aijun Ding, Hugo Denier Van Der Gon, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 18, 10039–10054, https://doi.org/10.5194/acp-18-10039-2018, https://doi.org/10.5194/acp-18-10039-2018, 2018
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Our project describes the feasibility of implementing particle number emissions taken from the GAINS model in global climate modeling through a simulation with the ECHAM-HAM global climate model. The results from the simulations have important implications regarding modeled particle number concentrations and future climate effects. Our findings represent an important starting point for further simulations concerning climate effects derived from anthropogenic particle emissions on a global scale.
Yu Hoshina, Yasunori Tohjima, Keiichi Katsumata, Toshinobu Machida, and Shin-ichiro Nakaoka
Atmos. Chem. Phys., 18, 9283–9295, https://doi.org/10.5194/acp-18-9283-2018, https://doi.org/10.5194/acp-18-9283-2018, 2018
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We installed a low flow rate measurement system on a cargo ship sailing between Japan and North America and started onboard continuous measurements for O2 and CO2. From the comparison between the in situ measurements and flask samples, we concluded that the uncertainties in the O2 and CO2 mole fraction for the in situ measurements are about 9 per meg and about 0.3 ppm, respectively.
Naoko Saitoh, Shuhei Kimoto, Ryo Sugimura, Ryoichi Imasu, Kei Shiomi, Akihiko Kuze, Yosuke Niwa, Toshinobu Machida, Yousuke Sawa, and Hidekazu Matsueda
Atmos. Meas. Tech., 10, 3877–3892, https://doi.org/10.5194/amt-10-3877-2017, https://doi.org/10.5194/amt-10-3877-2017, 2017
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This study evaluated biases in GOSAT/TANSO-FTS thermal infrared (TIR) V1 CO2 product on 736–287 hPa on the basis of comparisons with CONTRAIL CME CO2 data over airports. TIR V1 CO2 data had consistent negative biases of 1–1.5 %, with the largest negative biases at 541–398 hPa. Global comparisons between TIR CO2 data to which the bias-correction values were applied and CO2 data simulated by NICAM-TM confirmed the validity of the bias-correction values evaluated over airports in limited areas.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Ray Weiss, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Atmos. Chem. Phys., 17, 11135–11161, https://doi.org/10.5194/acp-17-11135-2017, https://doi.org/10.5194/acp-17-11135-2017, 2017
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Following the Global Methane Budget 2000–2012 published in Saunois et al. (2016), we use the same dataset of bottom-up and top-down approaches to discuss the variations in methane emissions over the period 2000–2012. The changes in emissions are discussed both in terms of trends and quasi-decadal changes. The ensemble gathered here allows us to synthesise the robust changes in terms of regional and sectorial contributions to the increasing methane emissions.
Yosuke Niwa, Hirofumi Tomita, Masaki Satoh, Ryoichi Imasu, Yousuke Sawa, Kazuhiro Tsuboi, Hidekazu Matsueda, Toshinobu Machida, Motoki Sasakawa, Boris Belan, and Nobuko Saigusa
Geosci. Model Dev., 10, 1157–1174, https://doi.org/10.5194/gmd-10-1157-2017, https://doi.org/10.5194/gmd-10-1157-2017, 2017
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We have developed forward and adjoint models based on NICAM-TM, as part of the 4D-Var system for atmospheric GHGs inversions. The models are computationally efficient enough to make the 4D-Var iterative calculation feasible. Trajectory analysis for high-CO2 concentration events are performed to test adjoint sensitivities; we also demonstrate the potential usefulness of our adjoint model for diagnosing tracer transport.
Rona L. Thompson, Motoki Sasakawa, Toshinobu Machida, Tuula Aalto, Doug Worthy, Jost V. Lavric, Cathrine Lund Myhre, and Andreas Stohl
Atmos. Chem. Phys., 17, 3553–3572, https://doi.org/10.5194/acp-17-3553-2017, https://doi.org/10.5194/acp-17-3553-2017, 2017
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Methane (CH4) fluxes were estimated for the high northern latitudes for 2005–2013 based on observations of atmospheric CH4 mixing ratios. Methane fluxes were found to be higher than prior estimates in northern Eurasia and Canada, especially in the Western Siberian Lowlands and the Canadian province Alberta. Significant inter-annual variations in the fluxes were found as well as a small positive trend. In Canada, the trend may be related to an increase in soil temperature over the study period.
Shohei Nomura, Hitoshi Mukai, Yukio Terao, Toshinobu Machida, and Yukihiro Nojiri
Atmos. Meas. Tech., 10, 667–680, https://doi.org/10.5194/amt-10-667-2017, https://doi.org/10.5194/amt-10-667-2017, 2017
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We developed a battery-powered CO2 measurement system for monitoring at the summit of Mt. Fuji, which experiences severe environmental conditions without access to gridded electricity for 10 months. Our measurement system used 100 batteries to run the measurement unit during these months. CO2 mole fractions at Mt. Fuji demonstrated clear seasonal variation. The trend and the variability of the CO2 growth rate observed at Mt. Fuji was very similar to that of the Mauna Loa Observatory.
Jinwoong Kim, Hyun Mee Kim, Chun-Ho Cho, Kyung-On Boo, Andrew R. Jacobson, Motoki Sasakawa, Toshinobu Machida, Mikhail Arshinov, and Nikolay Fedoseev
Atmos. Chem. Phys., 17, 2881–2899, https://doi.org/10.5194/acp-17-2881-2017, https://doi.org/10.5194/acp-17-2881-2017, 2017
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To investigate the effect of CO2 observations in Siberia on the surface CO2 flux analyses, two experiments using observation data sets with and without Siberian measurements were performed. While the magnitude of the optimized surface CO2 flux uptake in Siberia decreased, that in the other regions of the Northern Hemisphere increased for the experiment with Siberian observations. It is expected that the Siberian observations play an important role in estimating surface CO2 flux in the future.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Victor Brovkin, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Charles Curry, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Julia Marshall, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Catherine Prigent, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Paul Steele, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Michiel van Weele, Guido R. van der Werf, Ray Weiss, Christine Wiedinmyer, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Earth Syst. Sci. Data, 8, 697–751, https://doi.org/10.5194/essd-8-697-2016, https://doi.org/10.5194/essd-8-697-2016, 2016
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An accurate assessment of the methane budget is important to understand the atmospheric methane concentrations and trends and to provide realistic pathways for climate change mitigation. The various and diffuse sources of methane as well and its oxidation by a very short lifetime radical challenge this assessment. We quantify the methane sources and sinks as well as their uncertainties based on both bottom-up and top-down approaches provided by a broad international scientific community.
Hanna K. Lappalainen, Veli-Matti Kerminen, Tuukka Petäjä, Theo Kurten, Aleksander Baklanov, Anatoly Shvidenko, Jaana Bäck, Timo Vihma, Pavel Alekseychik, Meinrat O. Andreae, Stephen R. Arnold, Mikhail Arshinov, Eija Asmi, Boris Belan, Leonid Bobylev, Sergey Chalov, Yafang Cheng, Natalia Chubarova, Gerrit de Leeuw, Aijun Ding, Sergey Dobrolyubov, Sergei Dubtsov, Egor Dyukarev, Nikolai Elansky, Kostas Eleftheriadis, Igor Esau, Nikolay Filatov, Mikhail Flint, Congbin Fu, Olga Glezer, Aleksander Gliko, Martin Heimann, Albert A. M. Holtslag, Urmas Hõrrak, Juha Janhunen, Sirkku Juhola, Leena Järvi, Heikki Järvinen, Anna Kanukhina, Pavel Konstantinov, Vladimir Kotlyakov, Antti-Jussi Kieloaho, Alexander S. Komarov, Joni Kujansuu, Ilmo Kukkonen, Ella-Maria Duplissy, Ari Laaksonen, Tuomas Laurila, Heikki Lihavainen, Alexander Lisitzin, Alexsander Mahura, Alexander Makshtas, Evgeny Mareev, Stephany Mazon, Dmitry Matishov, Vladimir Melnikov, Eugene Mikhailov, Dmitri Moisseev, Robert Nigmatulin, Steffen M. Noe, Anne Ojala, Mari Pihlatie, Olga Popovicheva, Jukka Pumpanen, Tatjana Regerand, Irina Repina, Aleksei Shcherbinin, Vladimir Shevchenko, Mikko Sipilä, Andrey Skorokhod, Dominick V. Spracklen, Hang Su, Dmitry A. Subetto, Junying Sun, Arkady Y. Terzhevik, Yuri Timofeyev, Yuliya Troitskaya, Veli-Pekka Tynkkynen, Viacheslav I. Kharuk, Nina Zaytseva, Jiahua Zhang, Yrjö Viisanen, Timo Vesala, Pertti Hari, Hans Christen Hansson, Gennady G. Matvienko, Nikolai S. Kasimov, Huadong Guo, Valery Bondur, Sergej Zilitinkevich, and Markku Kulmala
Atmos. Chem. Phys., 16, 14421–14461, https://doi.org/10.5194/acp-16-14421-2016, https://doi.org/10.5194/acp-16-14421-2016, 2016
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After kick off in 2012, the Pan-Eurasian Experiment (PEEX) program has expanded fast and today the multi-disciplinary research community covers ca. 80 institutes and a network of ca. 500 scientists from Europe, Russia, and China. Here we introduce scientific topics relevant in this context. This is one of the first multi-disciplinary overviews crossing scientific boundaries, from atmospheric sciences to socio-economics and social sciences.
Zeli Tan, Qianlai Zhuang, Daven K. Henze, Christian Frankenberg, Ed Dlugokencky, Colm Sweeney, Alexander J. Turner, Motoki Sasakawa, and Toshinobu Machida
Atmos. Chem. Phys., 16, 12649–12666, https://doi.org/10.5194/acp-16-12649-2016, https://doi.org/10.5194/acp-16-12649-2016, 2016
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Methane emissions from the pan-Arctic could be important in understanding the global carbon cycle but are still poorly constrained to date. This study demonstrated that satellite retrievals can be used to reduce the uncertainty of the estimates of these emissions. We also provided additional evidence for the existence of large methane emissions from pan-Arctic lakes in the Siberian yedoma permafrost region. We found that biogeochemical models should be improved for better estimates.
Makoto Inoue, Isamu Morino, Osamu Uchino, Takahiro Nakatsuru, Yukio Yoshida, Tatsuya Yokota, Debra Wunch, Paul O. Wennberg, Coleen M. Roehl, David W. T. Griffith, Voltaire A. Velazco, Nicholas M. Deutscher, Thorsten Warneke, Justus Notholt, John Robinson, Vanessa Sherlock, Frank Hase, Thomas Blumenstock, Markus Rettinger, Ralf Sussmann, Esko Kyrö, Rigel Kivi, Kei Shiomi, Shuji Kawakami, Martine De Mazière, Sabrina G. Arnold, Dietrich G. Feist, Erica A. Barrow, James Barney, Manvendra Dubey, Matthias Schneider, Laura T. Iraci, James R. Podolske, Patrick W. Hillyard, Toshinobu Machida, Yousuke Sawa, Kazuhiro Tsuboi, Hidekazu Matsueda, Colm Sweeney, Pieter P. Tans, Arlyn E. Andrews, Sebastien C. Biraud, Yukio Fukuyama, Jasna V. Pittman, Eric A. Kort, and Tomoaki Tanaka
Atmos. Meas. Tech., 9, 3491–3512, https://doi.org/10.5194/amt-9-3491-2016, https://doi.org/10.5194/amt-9-3491-2016, 2016
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In this study, we correct the biases of GOSAT XCO2 and XCH4 using TCCON data. To evaluate the effectiveness of our correction method, uncorrected/corrected GOSAT data are compared to independent XCO2 and XCH4 data derived from aircraft measurements. Consequently, we suggest that this method is effective for reducing the biases of the GOSAT data. We consider that our work provides GOSAT data users with valuable information and contributes to the further development of studies on greenhouse gases.
Naoko Saitoh, Shuhei Kimoto, Ryo Sugimura, Ryoichi Imasu, Shuji Kawakami, Kei Shiomi, Akihiko Kuze, Toshinobu Machida, Yousuke Sawa, and Hidekazu Matsueda
Atmos. Meas. Tech., 9, 2119–2134, https://doi.org/10.5194/amt-9-2119-2016, https://doi.org/10.5194/amt-9-2119-2016, 2016
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This study compared GOSAT/TANSO-FTS thermal infrared (TIR) V1 and CONTRAIL CME CO2 data in the upper troposphere and lower stratosphere. The TIR CO2 averages agreed with the CME CO2 averages within 0.1 and 0.5 % in the Southern and Northern Hemisphere. At northern low and middle latitudes, their agreements were worse in spring and summer. The negative bias there made the maximum of TIR data being lower than that of CME data, which leads to underestimating the amplitude of CO2 seasonal variation.
Sudhanshu Pandey, Sander Houweling, Maarten Krol, Ilse Aben, Frédéric Chevallier, Edward J. Dlugokencky, Luciana V. Gatti, Emanuel Gloor, John B. Miller, Rob Detmers, Toshinobu Machida, and Thomas Röckmann
Atmos. Chem. Phys., 16, 5043–5062, https://doi.org/10.5194/acp-16-5043-2016, https://doi.org/10.5194/acp-16-5043-2016, 2016
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This study investigates the constraint provided by measurements of Xratio (XCH4/XCO2) from space on surface fluxes of CH4 and CO2. We apply the ratio inversion method described in Pandey et al. (2015) to Xratio retrievals from the GOSAT with the TM5-4DVAR inverse modeling system, to constrain the surface fluxes of CH4 and CO2 for 2009 and 2010. The results are compared to proxy CH4 inversions using model-derived-XCO2 mixing ratios from CarbonTracker and MACC.
G. G. Matvienko, B. D. Belan, M. V. Panchenko, O. A. Romanovskii, S. M. Sakerin, D. M. Kabanov, S. A. Turchinovich, Y. S. Turchinovich, T. A. Eremina, V. S. Kozlov, S. A. Terpugova, V. V. Pol'kin, E. P. Yausheva, D. G. Chernov, T. B. Zhuravleva, T. V. Bedareva, S. L. Odintsov, V. D. Burlakov, A. V. Nevzorov, M. Y. Arshinov, G. A. Ivlev, D. E. Savkin, A. V. Fofonov, V. A. Gladkikh, A. P. Kamardin, Y. S. Balin, G. P. Kokhanenko, I. E. Penner, S. V. Samoilova, P. N. Antokhin, V. G. Arshinova, D. K. Davydov, A. V. Kozlov, D. A. Pestunov, T. M. Rasskazchikova, D. V. Simonenkov, T. K. Sklyadneva, G. N. Tolmachev, S. B. Belan, V. P. Shmargunov, A. S. Kozlov, and S. B. Malyshkin
Atmos. Meas. Tech., 8, 4507–4520, https://doi.org/10.5194/amt-8-4507-2015, https://doi.org/10.5194/amt-8-4507-2015, 2015
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The primary objective of the Complex Aerosol Experiment was measurement of microphysical, chemical, and optical properties of aerosol particles in the surface air layer and free atmosphere. The measurement data were used to retrieve the whole set of aerosol optical parameters, necessary for radiation calculations. Three measurement cycles were performed within the experiment during 2013: in spring, summer (July), and in late summer/early autumn.
A. Berchet, I. Pison, F. Chevallier, J.-D. Paris, P. Bousquet, J.-L. Bonne, M. Y. Arshinov, B. D. Belan, C. Cressot, D. K. Davydov, E. J. Dlugokencky, A. V. Fofonov, A. Galanin, J. Lavrič, T. Machida, R. Parker, M. Sasakawa, R. Spahni, B. D. Stocker, and J. Winderlich
Biogeosciences, 12, 5393–5414, https://doi.org/10.5194/bg-12-5393-2015, https://doi.org/10.5194/bg-12-5393-2015, 2015
M. Reuter, M. Buchwitz, M. Hilker, J. Heymann, O. Schneising, D. Pillai, H. Bovensmann, J. P. Burrows, H. Bösch, R. Parker, A. Butz, O. Hasekamp, C. W. O'Dell, Y. Yoshida, C. Gerbig, T. Nehrkorn, N. M. Deutscher, T. Warneke, J. Notholt, F. Hase, R. Kivi, R. Sussmann, T. Machida, H. Matsueda, and Y. Sawa
Atmos. Chem. Phys., 14, 13739–13753, https://doi.org/10.5194/acp-14-13739-2014, https://doi.org/10.5194/acp-14-13739-2014, 2014
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Current knowledge about the European terrestrial biospheric carbon sink relies upon bottom-up and global surface flux inverse model estimates using in situ measurements. Our analysis of five satellite data sets comprises a regional inversion designed to be insensitive to potential retrieval biases and transport errors. We show that the satellite-derived sink is larger (1.0±0.3GtC/a) than previous estimates (0.4±0.4GtC/a).
F. Jiang, H. M. Wang, J. M. Chen, T. Machida, L. X. Zhou, W. M. Ju, H. Matsueda, and Y. Sawa
Atmos. Chem. Phys., 14, 10133–10144, https://doi.org/10.5194/acp-14-10133-2014, https://doi.org/10.5194/acp-14-10133-2014, 2014
M. Inoue, I. Morino, O. Uchino, Y. Miyamoto, T. Saeki, Y. Yoshida, T. Yokota, C. Sweeney, P. P. Tans, S. C. Biraud, T. Machida, J. V. Pittman, E. A. Kort, T. Tanaka, S. Kawakami, Y. Sawa, K. Tsuboi, and H. Matsueda
Atmos. Meas. Tech., 7, 2987–3005, https://doi.org/10.5194/amt-7-2987-2014, https://doi.org/10.5194/amt-7-2987-2014, 2014
Q. Zhu, Q. Zhuang, D. Henze, K. Bowman, M. Chen, Y. Liu, Y. He, H. Matsueda, T. Machida, Y. Sawa, and W. Oechel
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-22587-2014, https://doi.org/10.5194/acpd-14-22587-2014, 2014
Revised manuscript not accepted
H. F. Zhang, B. Z. Chen, I. T. van der Laan-Luijk, T. Machida, H. Matsueda, Y. Sawa, Y. Fukuyama, R. Langenfelds, M. van der Schoot, G. Xu, J. W. Yan, M. L. Cheng, L. X. Zhou, P. P. Tans, and W. Peters
Atmos. Chem. Phys., 14, 5807–5824, https://doi.org/10.5194/acp-14-5807-2014, https://doi.org/10.5194/acp-14-5807-2014, 2014
E. Saikawa, R. G. Prinn, E. Dlugokencky, K. Ishijima, G. S. Dutton, B. D. Hall, R. Langenfelds, Y. Tohjima, T. Machida, M. Manizza, M. Rigby, S. O'Doherty, P. K. Patra, C. M. Harth, R. F. Weiss, P. B. Krummel, M. van der Schoot, P. J. Fraser, L. P. Steele, S. Aoki, T. Nakazawa, and J. W. Elkins
Atmos. Chem. Phys., 14, 4617–4641, https://doi.org/10.5194/acp-14-4617-2014, https://doi.org/10.5194/acp-14-4617-2014, 2014
Y. Tohjima, M. Kubo, C. Minejima, H. Mukai, H. Tanimoto, A. Ganshin, S. Maksyutov, K. Katsumata, T. Machida, and K. Kita
Atmos. Chem. Phys., 14, 1663–1677, https://doi.org/10.5194/acp-14-1663-2014, https://doi.org/10.5194/acp-14-1663-2014, 2014
M. Inoue, I. Morino, O. Uchino, Y. Miyamoto, Y. Yoshida, T. Yokota, T. Machida, Y. Sawa, H. Matsueda, C. Sweeney, P. P. Tans, A. E. Andrews, S. C. Biraud, T. Tanaka, S. Kawakami, and P. K. Patra
Atmos. Chem. Phys., 13, 9771–9788, https://doi.org/10.5194/acp-13-9771-2013, https://doi.org/10.5194/acp-13-9771-2013, 2013
Y. Miyamoto, M. Inoue, I. Morino, O. Uchino, T. Yokota, T. Machida, Y. Sawa, H. Matsueda, C. Sweeney, P. P. Tans, A. E. Andrews, and P. K. Patra
Atmos. Chem. Phys., 13, 5265–5275, https://doi.org/10.5194/acp-13-5265-2013, https://doi.org/10.5194/acp-13-5265-2013, 2013
C. Crevoisier, D. Nobileau, R. Armante, L. Crépeau, T. Machida, Y. Sawa, H. Matsueda, T. Schuck, T. Thonat, J. Pernin, N. A. Scott, and A. Chédin
Atmos. Chem. Phys., 13, 4279–4289, https://doi.org/10.5194/acp-13-4279-2013, https://doi.org/10.5194/acp-13-4279-2013, 2013
Related subject area
Subject: Gases | Technique: In Situ Measurement | Topic: Data Processing and Information Retrieval
Comparison of methods for resolving the contributions of local emissions to measured concentrations
Gridded surface O3, NOx, and CO abundances for model metrics from the South Korean ground station network
Digitization and calibration of historical solar absorption infrared spectra from the Jungfraujoch site
Advancing N2O flux chamber measurement techniques in nutrient-poor ecosystems
Direct high-precision radon quantification for interpreting high-frequency greenhouse gas measurements
The Turbulent Enhancement Ratio as a novel Approach for Characterizing Local Emission Sources in Complex Environments
Intercomparison of fast airborne ozone instruments to measure eddy covariance fluxes: spatial variability in deposition at the ocean surface and evidence for cloud processing
Field assessments on the impact of CO2 concentration fluctuations along with complex-terrain flows on the estimation of the net ecosystem exchange of temperate forests
Multi-instrumental analysis of ozone vertical profiles and total columns in South America: comparison between subtropical and equatorial latitudes
Transferability of machine-learning-based global calibration models for NO2 and NO low-cost sensors
Detection and long-term quantification of methane emissions from an active landfill
Research of low-cost air quality monitoring models with different machine learning algorithms
New insights from the Jülich Ozone Sonde Intercomparison Experiment: calibration functions traceable to one ozone reference instrument
Identification of spikes in continuous ground-based in situ time series of CO2, CH4 and CO: an extended experiment within the European ICOS Atmosphere network
Data treatment and corrections for estimating H2O and CO2 isotope fluxes from high-frequency observations
Measurements of volatile organic compounds in ambient air by gas-chromatography and real-time Vocus PTR-TOF-MS: calibrations, instrument background corrections, and introducing a PTR Data Toolkit
Development of low-cost air quality stations for next-generation monitoring networks: calibration and validation of NO2 and O3 sensors
Detecting plumes in mobile air quality monitoring time series with density-based spatial clustering of applications with noise
Characterising the methane gas and environmental response of the Figaro Taguchi Gas Sensor (TGS) 2611-E00
Reducing errors on estimates of the carbon uptake period based on time series of atmospheric CO2
Generalized Kendrick analysis for improved visualization of atmospheric mass spectral data
Determination of NOx emission rates of inland ships from onshore measurements
Data quality enhancement for field experiments in atmospheric chemistry via sequential Monte Carlo filters
A flexible algorithm for network design based on information theory
Real-world wintertime CO, N2O, and CO2 emissions of a central European village
Evaluation of two common source estimation measurement strategies using large-eddy simulation of plume dispersion under neutral atmospheric conditions
Machine learning techniques to improve the field performance of low-cost air quality sensors
Estimation of sulfuric acid concentration using ambient ion composition and concentration data obtained with atmospheric pressure interface time-of-flight ion mass spectrometer
Importance of the Webb, Pearman, and Leuning (WPL) correction for the measurement of small CO2 fluxes
Unravelling a black box: an open-source methodology for the field calibration of small air quality sensors
An algorithm to detect non-background signals in greenhouse gas time series from European tall tower and mountain stations
Mobile atmospheric measurements and local-scale inverse estimation of the location and rates of brief CH4 and CO2 releases from point sources
SIBaR: a new method for background quantification and removal from mobile air pollution measurements
Machine learning calibration of low-cost NO2 and PM10 sensors: non-linear algorithms and their impact on site transferability
The high-frequency response correction of eddy covariance fluxes – Part 2: An experimental approach for analysing noisy measurements of small fluxes
The high-frequency response correction of eddy covariance fluxes – Part 1: An experimental approach and its interdependence with the time-lag estimation
Uncertainty of hourly-average concentration values derived from non-continuous measurements
Emissions relationships in western forest fire plumes – Part 1: Reducing the effect of mixing errors on emission factors
A new method to correct the electrochemical concentration cell (ECC) ozonesonde time response and its implications for “background current” and pump efficiency
Monitoring the compliance of sailing ships with fuel sulfur content regulations using unmanned aerial vehicle (UAV) measurements of ship emissions in open water
High-resolution mapping of urban air quality with heterogeneous observations: a new methodology and its application to Amsterdam
Towards standardized processing of eddy covariance flux measurements of carbonyl sulfide
Integration and calibration of non-dispersive infrared (NDIR) CO2 low-cost sensors and their operation in a sensor network covering Switzerland
Correcting the impact of the isotope composition on the mixing ratio dependency of water vapour isotope measurements with cavity ring-down spectrometers
Correcting high-frequency losses of reactive nitrogen flux measurements
Surface flux estimates derived from UAS-based mole fraction measurements by means of a nocturnal boundary layer budget approach
InnFLUX – an open-source code for conventional and disjunct eddy covariance analysis of trace gas measurements: an urban test case
Accurate measurements of atmospheric carbon dioxide and methane mole fractions at the Siberian coastal site Ambarchik
Traffic-related air pollution near roadways: discerning local impacts from background
Bayesian atmospheric tomography for detection and quantification of methane emissions: application to data from the 2015 Ginninderra release experiment
Taylor D. Edwards, Yee Ka Wong, Cheol-Heon Jeong, Jonathan M. Wang, Yushan Su, and Greg J. Evans
Atmos. Meas. Tech., 18, 2201–2240, https://doi.org/10.5194/amt-18-2201-2025, https://doi.org/10.5194/amt-18-2201-2025, 2025
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We tested a variety of scientific measurements and algorithms for distinguishing the amounts of air pollution that were emitted by a nearby polluter from background pollution that was already in the air. The results show that machine learning and other statistical algorithms produced accurate estimates of this background pollution. These findings help scientists and regulators to understand where pollution comes from and to improve measurements of pollution from sources like traffic.
Calum P. Wilson and Michael J. Prather
Atmos. Meas. Tech., 18, 1757–1769, https://doi.org/10.5194/amt-18-1757-2025, https://doi.org/10.5194/amt-18-1757-2025, 2025
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We evaluated how well we can infer air pollutant levels (ozone, carbon monoxide, and nitrogen oxides) between air quality stations throughout South Korea, finding good representation in most densely measured cities in spite of intense small-scale emission hotspots. Comparing observed air quality with gridded model output is desirable, and so we created gridded datasets over South Korea using air quality station measurements, which agreed with airborne measurements around Seoul.
Jamal Makkor, Mathias Palm, Matthias Buschmann, Emmanuel Mahieu, Martyn P. Chipperfield, and Justus Notholt
Atmos. Meas. Tech., 18, 1105–1114, https://doi.org/10.5194/amt-18-1105-2025, https://doi.org/10.5194/amt-18-1105-2025, 2025
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During the years 1950 and 1951, Marcel Migeotte took regular solar measurements in the form of paper rolls at the Jungfraujoch site. These historical spectra proved to be valuable for atmospheric research and needed to be saved for posterity. Therefore, a digitization method which used image-processing techniques was developed to extract them from the historical paper rolls. This allowed them to be saved in a machine-readable format that is easily accessible to the scientific community.
Nathalie Ylenia Triches, Jan Engel, Abdullah Bolek, Timo Vesala, Maija E. Marushchak, Anna-Maria Virkkala, Martin Heimann, and Mathias Göckede
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-203, https://doi.org/10.5194/amt-2024-203, 2025
Revised manuscript accepted for AMT
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This study explores nitrous oxide (N2O) fluxes from a nutrient-poor, sub-Arctic peatland. N2O is a potent greenhouse gas; understanding its fluxes is essential for addressing global warming. Using a new instrument and flux chambers, we introduce a system to reliably detect low N2O fluxes and provide recommendations on chamber closure times and flux calculation methods to better quantify N2O fluxes. We encourage researchers to further investigate N2O fluxes in low-nutrient environments.
Dafina Kikaj, Edward Chung, Alan D. Griffiths, Scott D. Chambers, Grant Forster, Angelina Wenger, Penelope Pickers, Chris Rennick, Simon O'Doherty, Joseph Pitt, Kieran Stanley, Dickon Young, Leigh S. Fleming, Karina Adcock, Emmal Safi, and Tim Arnold
Atmos. Meas. Tech., 18, 151–175, https://doi.org/10.5194/amt-18-151-2025, https://doi.org/10.5194/amt-18-151-2025, 2025
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We present a protocol to improve confidence in atmospheric radon measurements, enabling site comparisons and integration with greenhouse gas data. As a natural tracer, radon provides an independent check of transport model performance. This standardized method enhances radon’s use as a metric for model evaluation. Beyond UK observatories, it can support broader networks like ICOS and WMO/GAW, advancing global atmospheric research.
Christian Lamprecht, Martin Graus, Marcus Striednig, Michael Stichaner, Werner Jud, Andreas Held, and Thomas Karl
EGUsphere, https://doi.org/10.5194/egusphere-2024-2939, https://doi.org/10.5194/egusphere-2024-2939, 2024
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Air pollution management requires accurate determination of emissions and emission ratios of air pollutants. In this paper, we explore a new way to resolve excess mixing ratios in turbulent plumes, which allows aggregation of unbiased ensemble averages of air pollutant ratios that can be compared with emission models. The approach is tested in an urban environment and used to resolve emission patterns of nitrogen oxides and carbon dioxide.
Randall Chiu, Florian Obersteiner, Alessandro Franchin, Teresa Campos, Adriana Bailey, Christopher Webster, Andreas Zahn, and Rainer Volkamer
Atmos. Meas. Tech., 17, 5731–5746, https://doi.org/10.5194/amt-17-5731-2024, https://doi.org/10.5194/amt-17-5731-2024, 2024
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The ozone sink into oceans and marine clouds is seldom studied and highly uncertain. Calculations suggest O3 destruction at aqueous surfaces (ocean, droplets) may be strongly accelerated, but field evidence is missing. Here we compare three fast airborne O3 instruments to measure eddy covariance fluxes of O3 over the remote ocean, in clear and cloudy air. We find O3 fluxes below clouds are consistently directed into clouds, while O3 fluxes into oceans are much smaller and spatially variable.
Dexiong Teng, Jiaojun Zhu, Tian Gao, Fengyuan Yu, Yuan Zhu, Xinhua Zhou, and Bai Yang
Atmos. Meas. Tech., 17, 5581–5599, https://doi.org/10.5194/amt-17-5581-2024, https://doi.org/10.5194/amt-17-5581-2024, 2024
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Dense canopy weakens turbulent mixing, leading to significant CO2 storage (Fs), a key part of net ecosystem exchange (NEE) measured using eddy covariance. Gust-biased Fs measurements complicate NEE estimation in forests with complex terrain. We analyzed gust-induced CO2 fluctuations and their impact on Fs. Fs and its contribution to NEE can be explained by terrain complexity and turbulent mixing. This work highlights how gusts over complex terrain affect the Fs and NEE measurements.
Gabriela Dornelles Bittencourt, Hassan Bencherif, Damaris Kirsch Pinheiro, Nelson Begue, Lucas Vaz Peres, José Valentin Bageston, Douglas Lima de Bem, Francisco Raimundo da Silva, and Tristan Millet
Atmos. Meas. Tech., 17, 5201–5220, https://doi.org/10.5194/amt-17-5201-2024, https://doi.org/10.5194/amt-17-5201-2024, 2024
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The study examines the behavior of ozone at equatorial and subtropical latitudes in South America, in a multi-instrumental analysis. The methodology applied used ozonesondes (SHADOZ/NASA) and satellite data (TIMED/SABER), as well as analysis with ground-based and satellite instruments, allowing a more in-depth study at both latitudes. The main motivation is to understand how latitudinal differences in the observation of ozone content can interfere with the behavior of this trace gas.
Ayah Abu-Hani, Jia Chen, Vigneshkumar Balamurugan, Adrian Wenzel, and Alessandro Bigi
Atmos. Meas. Tech., 17, 3917–3931, https://doi.org/10.5194/amt-17-3917-2024, https://doi.org/10.5194/amt-17-3917-2024, 2024
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This study examined the transferability of machine learning calibration models among low-cost sensor units targeting NO2 and NO. The global models were evaluated under similar and different emission conditions. To counter cross-sensitivity, the study proposed integrating O3 measurements from nearby reference stations, in Switzerland. The models show substantial improvement when O3 measurements are incorporated, which is more pronounced when in regions with elevated O3 concentrations.
Pramod Kumar, Christopher Caldow, Grégoire Broquet, Adil Shah, Olivier Laurent, Camille Yver-Kwok, Sebastien Ars, Sara Defratyka, Susan Warao Gichuki, Luc Lienhardt, Mathis Lozano, Jean-Daniel Paris, Felix Vogel, Caroline Bouchet, Elisa Allegrini, Robert Kelly, Catherine Juery, and Philippe Ciais
Atmos. Meas. Tech., 17, 1229–1250, https://doi.org/10.5194/amt-17-1229-2024, https://doi.org/10.5194/amt-17-1229-2024, 2024
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This study presents a series of mobile measurement campaigns to monitor the CH4 emissions from an active landfill. These measurements are processed using a Gaussian plume model and atmospheric inversion techniques to quantify the landfill CH4 emissions. The methane emission estimates range between ~0.4 and ~7 t CH4 per day, and their variations are analyzed. The robustness of the estimates is assessed depending on the distance of the measurements from the potential sources in the landfill.
Gang Wang, Chunlai Yu, Kai Guo, Haisong Guo, and Yibo Wang
Atmos. Meas. Tech., 17, 181–196, https://doi.org/10.5194/amt-17-181-2024, https://doi.org/10.5194/amt-17-181-2024, 2024
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A low-cost multi-parameter air quality monitoring system (LCS) based on different machine learning algorithms is proposed. The LCS can measure particulate matter (PM) and gas pollutants simultaneously. The performance of the different algorithms (RF, MLR, KNN, BP, GA-BP) with the parameters such as R2 and RMSE are compared and discussed. These measurements indicate the LCS based on the machine learning algorithms can be used to predict the concentrations of PM and gas pollution.
Herman G. J. Smit, Deniz Poyraz, Roeland Van Malderen, Anne M. Thompson, David W. Tarasick, Ryan M. Stauffer, Bryan J. Johnson, and Debra E. Kollonige
Atmos. Meas. Tech., 17, 73–112, https://doi.org/10.5194/amt-17-73-2024, https://doi.org/10.5194/amt-17-73-2024, 2024
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This paper revisits fundamentals of ECC ozonesonde measurements to develop and characterize a methodology to correct for the fast and slow time responses using the JOSIE (Jülich Ozone Sonde Intercomparison Experiment) simulation chamber data. Comparing the new corrected ozonesonde profiles to an accurate ozone UV photometer (OPM) as reference allows us to evaluate the time response correction (TRC) method and to determine calibration functions traceable to one reference with 5 % uncertainty.
Paolo Cristofanelli, Cosimo Fratticioli, Lynn Hazan, Mali Chariot, Cedric Couret, Orestis Gazetas, Dagmar Kubistin, Antti Laitinen, Ari Leskinen, Tuomas Laurila, Matthias Lindauer, Giovanni Manca, Michel Ramonet, Pamela Trisolino, and Martin Steinbacher
Atmos. Meas. Tech., 16, 5977–5994, https://doi.org/10.5194/amt-16-5977-2023, https://doi.org/10.5194/amt-16-5977-2023, 2023
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We investigated the application of two automatic methods for detecting spikes due to local emissions in greenhouse gas (GHG) observations at a subset of sites from the ICOS Atmosphere network. We analysed the sensitivity to the spike frequency of using different methods and settings. We documented the impact of the de-spiking on different temporal aggregations (i.e. hourly, monthly and seasonal averages) of CO2, CH4 and CO 1 min time series.
Robbert P. J. Moonen, Getachew A. Adnew, Oscar K. Hartogensis, Jordi Vilà-Guerau de Arellano, David J. Bonell Fontas, and Thomas Röckmann
Atmos. Meas. Tech., 16, 5787–5810, https://doi.org/10.5194/amt-16-5787-2023, https://doi.org/10.5194/amt-16-5787-2023, 2023
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Isotope fluxes allow for net ecosystem gas exchange fluxes to be partitioned into sub-components like plant assimilation, respiration and transpiration, which can help us better understand the environmental drivers of each partial flux. We share the results of a field campaign isotope fluxes were derived using a combination of laser spectroscopy and eddy covariance. We found lag times and high frequency signal loss in the isotope fluxes we derived and present methods to correct for both.
Andrew R. Jensen, Abigail R. Koss, Ryder B. Hales, and Joost A. de Gouw
Atmos. Meas. Tech., 16, 5261–5285, https://doi.org/10.5194/amt-16-5261-2023, https://doi.org/10.5194/amt-16-5261-2023, 2023
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Quantification of a wide range of volatile organic compounds by proton-transfer-reaction mass spectrometry (PTR-MS) can be achieved with direct calibration of only a subset of compounds, characterization of instrument response, and simple reaction kinetics. We characterized our Vocus PTR-MS and developed a toolkit as a guide through this process. A catalytic zero air generator provided the lowest detection limits, and short, frequent calibrations informed variability in instrument response.
Alice Cavaliere, Lorenzo Brilli, Bianca Patrizia Andreini, Federico Carotenuto, Beniamino Gioli, Tommaso Giordano, Marco Stefanelli, Carolina Vagnoli, Alessandro Zaldei, and Giovanni Gualtieri
Atmos. Meas. Tech., 16, 4723–4740, https://doi.org/10.5194/amt-16-4723-2023, https://doi.org/10.5194/amt-16-4723-2023, 2023
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We assessed calibration models for two low-cost stations equipped with O3 and NO2 metal oxide sensors. Environmental parameters had improved accuracy in linear and black box models. Moreover, interpretability methods like SHapley Additive exPlanations helped identify the physical patterns and potential problems of these models in a field validation. Results showed both sensors performed well with the same linear model form, but unique coefficients were required for intersensor variability.
Blake Actkinson and Robert J. Griffin
Atmos. Meas. Tech., 16, 3547–3559, https://doi.org/10.5194/amt-16-3547-2023, https://doi.org/10.5194/amt-16-3547-2023, 2023
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Data collected using air quality instrumentation deployed on automobiles and driven repeatedly in Houston neighborhoods are analyzed using a novel machine learning technique. The aim is to separate large plumes from the rest of the data in order to identify the sources of the highest levels of the pollutants. The number and nature of these plumes are characterized spatially and can be linked to emissions from different types of motor vehicles.
Adil Shah, Olivier Laurent, Luc Lienhardt, Grégoire Broquet, Rodrigo Rivera Martinez, Elisa Allegrini, and Philippe Ciais
Atmos. Meas. Tech., 16, 3391–3419, https://doi.org/10.5194/amt-16-3391-2023, https://doi.org/10.5194/amt-16-3391-2023, 2023
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As methane (CH4) contributes to global warming, more CH4 measurements are required to better characterise source emissions. Hence, we tested a cheap CH4 sensor for 338 d of landfill sampling. We derived an excellent CH4 response model in a stable environment. However, different types of air with the same CH4 level had diverse sensor responses. We characterised temperature and water vapour response but could not replicate field sampling. Thus, other species may cause sensor interactions.
Theertha Kariyathan, Ana Bastos, Julia Marshall, Wouter Peters, Pieter Tans, and Markus Reichstein
Atmos. Meas. Tech., 16, 3299–3312, https://doi.org/10.5194/amt-16-3299-2023, https://doi.org/10.5194/amt-16-3299-2023, 2023
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The timing and duration of the carbon uptake period (CUP) are sensitive to the occurrence of major phenological events, which are influenced by recent climate change. This study presents an ensemble-based approach for quantifying the timing and duration of the CUP and their uncertainty when derived from atmospheric CO2 measurements with noise and gaps. The CUP metrics derived with the approach are more robust and have less uncertainty than when estimated with the conventional methods.
Mitchell W. Alton, Harald J. Stark, Manjula R. Canagaratna, and Eleanor C. Browne
Atmos. Meas. Tech., 16, 3273–3282, https://doi.org/10.5194/amt-16-3273-2023, https://doi.org/10.5194/amt-16-3273-2023, 2023
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Mass spectrometric measurements of atmospheric composition routinely detect hundreds of different ions of varying chemical composition, creating challenges for visualization and data interpretation. We present a new analysis technique to facilitate visualization, while providing greater chemical insight. Additionally, it can aid in identifying the chemical composition of ions. A graphical user interface for performing the analysis is introduced and freely available, enabling broad applications.
Kai Krause, Folkard Wittrock, Andreas Richter, Dieter Busch, Anton Bergen, John P. Burrows, Steffen Freitag, and Olesia Halbherr
Atmos. Meas. Tech., 16, 1767–1787, https://doi.org/10.5194/amt-16-1767-2023, https://doi.org/10.5194/amt-16-1767-2023, 2023
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Inland shipping is an important source of nitrogen oxides (NOx). The amount of emitted NOx depends on the characteristics of the individual vessels and the traffic density. Ship emissions are often characterised by the amount of emitted NOx per unit of burnt fuel, and further knowledge about fuel consumption is needed to quantify the total emissions caused by ship traffic. In this study, a new approach to derive absolute emission rates (in g s−1) from onshore measurements is presented.
Lenard L. Röder, Patrick Dewald, Clara M. Nussbaumer, Jan Schuladen, John N. Crowley, Jos Lelieveld, and Horst Fischer
Atmos. Meas. Tech., 16, 1167–1178, https://doi.org/10.5194/amt-16-1167-2023, https://doi.org/10.5194/amt-16-1167-2023, 2023
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Field experiments in atmospheric chemistry provide insights into chemical interactions of our atmosphere. However, high data coverage and accuracy are needed to enable further analysis. In this study, we explore a statistical method that combines knowledge about the chemical reactions with information from measurements to increase the quality of field experiment datasets. We test the algorithm for several applications and discuss limitations that depend on the specific variable and the dynamics.
Rona L. Thompson and Ignacio Pisso
Atmos. Meas. Tech., 16, 235–246, https://doi.org/10.5194/amt-16-235-2023, https://doi.org/10.5194/amt-16-235-2023, 2023
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Atmospheric networks are used for monitoring air quality and greenhouse gases and can provide essential information about the sources and sinks. The design of the network, specifically where to place the observations, is a critical question in order to maximize the information provided while minimizing the cost. Here, a novel method of designing atmospheric networks is presented with two examples, one on monitoring sources of methane and the second on monitoring fossil fuel emissions of CO2.
László Haszpra, Zoltán Barcza, Zita Ferenczi, Roland Hollós, Anikó Kern, and Natascha Kljun
Atmos. Meas. Tech., 15, 5019–5031, https://doi.org/10.5194/amt-15-5019-2022, https://doi.org/10.5194/amt-15-5019-2022, 2022
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A novel approach is used for the determination of greenhouse gas (GHG) emissions of small rural settlements, which may significantly differ from those of urban regions and have hardly been studied yet. Among other results, it turned out that wintertime nitrous oxide emission is significantly underestimated in the official emission inventories. Given the large number of such settlements, the underestimation may also distort the national total emission values reported to international databases.
Anja Ražnjević, Chiel van Heerwaarden, and Maarten Krol
Atmos. Meas. Tech., 15, 3611–3628, https://doi.org/10.5194/amt-15-3611-2022, https://doi.org/10.5194/amt-15-3611-2022, 2022
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We evaluate two widely used observational techniques (Other Test Method (OTM) 33A and car drive-bys) that estimate point source gas emissions. We performed our analysis on high-resolution plume dispersion simulation. For car drive-bys we found that at least 15 repeated measurements were needed to get within 40 % of the true emissions. OTM 33A produced large errors in estimation (50 %–200 %) due to its sensitivity to dispersion coefficients and underlying simplifying assumptions.
Tony Bush, Nick Papaioannou, Felix Leach, Francis D. Pope, Ajit Singh, G. Neil Thomas, Brian Stacey, and Suzanne Bartington
Atmos. Meas. Tech., 15, 3261–3278, https://doi.org/10.5194/amt-15-3261-2022, https://doi.org/10.5194/amt-15-3261-2022, 2022
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Poor air quality is a human health risk which demands high-spatiotemporal-resolution monitoring data to manage. Low-cost air quality sensors present a convenient pathway to delivering these needs, compared to traditional methods, but bring methodological challenges which can limit operational ability. In this study within Oxford, UK, we develop machine learning methods to improve the quality of low-cost sensors for NO2, PM10 (particulate matter) and PM2.5 and demonstrate their effectiveness.
Lisa J. Beck, Siegfried Schobesberger, Mikko Sipilä, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Meas. Tech., 15, 1957–1965, https://doi.org/10.5194/amt-15-1957-2022, https://doi.org/10.5194/amt-15-1957-2022, 2022
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Sulfuric acid is known to be a main compound in atmospheric new particle formation. Yet, its concentration is very low, which leads to challenges in detecting it. In our study, we derive the sulfuric acid concentration from measurements of ambient ions with a mass spectrometer. Our validation shows that the theoretical approach using the bisulfate ion and its clusters with H2SO4 captures the sulfuric acid concentration very well during daytime.
Katharina Jentzsch, Julia Boike, and Thomas Foken
Atmos. Meas. Tech., 14, 7291–7296, https://doi.org/10.5194/amt-14-7291-2021, https://doi.org/10.5194/amt-14-7291-2021, 2021
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Very small CO2 fluxes are measured at night in Arctic regions. If the sensible heat flux is not close to zero under these conditions, the WPL correction will take values on the order of the flux. A special quality control is proposed for these cases.
Seán Schmitz, Sherry Towers, Guillermo Villena, Alexandre Caseiro, Robert Wegener, Dieter Klemp, Ines Langer, Fred Meier, and Erika von Schneidemesser
Atmos. Meas. Tech., 14, 7221–7241, https://doi.org/10.5194/amt-14-7221-2021, https://doi.org/10.5194/amt-14-7221-2021, 2021
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The last 2 decades have seen substantial technological advances in the development of low-cost air pollution instruments. This study introduces a seven-step methodology for the field calibration of low-cost sensors with user-friendly guidelines, open-access code, and a discussion of common barriers. Our goal with this work is to push for standardized reporting of methods, make critical data processing steps clear for users, and encourage responsible use in the scientific community and beyond.
Alex Resovsky, Michel Ramonet, Leonard Rivier, Jerome Tarniewicz, Philippe Ciais, Martin Steinbacher, Ivan Mammarella, Meelis Mölder, Michal Heliasz, Dagmar Kubistin, Matthias Lindauer, Jennifer Müller-Williams, Sebastien Conil, and Richard Engelen
Atmos. Meas. Tech., 14, 6119–6135, https://doi.org/10.5194/amt-14-6119-2021, https://doi.org/10.5194/amt-14-6119-2021, 2021
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We present a technical description of a statistical methodology for extracting synoptic- and seasonal-length anomalies from greenhouse gas time series. The definition of what represents an anomalous signal is somewhat subjective, which we touch on throughout the paper. We show, however, that the method performs reasonably well in extracting portions of time series influenced by significant North Atlantic Oscillation weather episodes and continent-wide terrestrial biospheric aberrations.
Pramod Kumar, Grégoire Broquet, Camille Yver-Kwok, Olivier Laurent, Susan Gichuki, Christopher Caldow, Ford Cropley, Thomas Lauvaux, Michel Ramonet, Guillaume Berthe, Frédéric Martin, Olivier Duclaux, Catherine Juery, Caroline Bouchet, and Philippe Ciais
Atmos. Meas. Tech., 14, 5987–6003, https://doi.org/10.5194/amt-14-5987-2021, https://doi.org/10.5194/amt-14-5987-2021, 2021
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This study presents a simple atmospheric inversion modeling framework for the localization and quantification of unknown CH4 and CO2 emissions from point sources based on near-surface mobile concentration measurements and a Gaussian plume dispersion model. It is applied for the estimate of a series of brief controlled releases of CH4 and CO2 with a wide range of rates during the TOTAL TADI-2018 experiment. Results indicate a ~10 %–40 % average error on the estimate of the release rates.
Blake Actkinson, Katherine Ensor, and Robert J. Griffin
Atmos. Meas. Tech., 14, 5809–5821, https://doi.org/10.5194/amt-14-5809-2021, https://doi.org/10.5194/amt-14-5809-2021, 2021
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This paper describes the development of a new method used to estimate background from mobile monitoring time series. The method is tested on a previously published dataset, applied to an extensive mobile dataset, and compared with other previously published techniques used to estimate background. The results suggest that the method is a promising framework for background estimation.
Peer Nowack, Lev Konstantinovskiy, Hannah Gardiner, and John Cant
Atmos. Meas. Tech., 14, 5637–5655, https://doi.org/10.5194/amt-14-5637-2021, https://doi.org/10.5194/amt-14-5637-2021, 2021
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Machine learning (ML) calibration techniques could be an effective way to improve the performance of low-cost air pollution sensors. Here we provide novel insights from case studies within the urban area of London, UK, where we compared the performance of three ML techniques to calibrate low-cost measurements of NO2 and PM10. In particular, we highlight the key issue of the method-dependent robustness in maintaining calibration skill after transferring sensors to different measurement sites.
Toprak Aslan, Olli Peltola, Andreas Ibrom, Eiko Nemitz, Üllar Rannik, and Ivan Mammarella
Atmos. Meas. Tech., 14, 5089–5106, https://doi.org/10.5194/amt-14-5089-2021, https://doi.org/10.5194/amt-14-5089-2021, 2021
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Vertical turbulent fluxes of gases measured by the eddy covariance (EC) technique are subject to high-frequency losses. There are different methods used to describe this low-pass filtering effect and to correct the measured fluxes. In this study, we analysed the systematic uncertainty related to this correction for various attenuation and signal-to-noise ratios. A new and robust transfer function method is finally proposed.
Olli Peltola, Toprak Aslan, Andreas Ibrom, Eiko Nemitz, Üllar Rannik, and Ivan Mammarella
Atmos. Meas. Tech., 14, 5071–5088, https://doi.org/10.5194/amt-14-5071-2021, https://doi.org/10.5194/amt-14-5071-2021, 2021
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Gas fluxes measured by the eddy covariance (EC) technique are subject to filtering due to non-ideal instrumentation. For linear first-order systems this filtering causes also a time lag between vertical wind speed and gas signal which is additional to the gas travel time in the sampling line. The effect of this additional time lag on EC fluxes is ignored in current EC data processing routines. Here we show that this oversight biases EC fluxes and hence propose an approach to rectify this bias.
László Haszpra and Ernő Prácser
Atmos. Meas. Tech., 14, 3561–3571, https://doi.org/10.5194/amt-14-3561-2021, https://doi.org/10.5194/amt-14-3561-2021, 2021
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Most of the tall-tower greenhouse gas observatories apply a single gas analyzer for the sequential sampling of several intakes along the tower. The non-continuous sampling at each intake introduces excess uncertainty to the calculated hourly-average concentrations used in several applications. Based on real-world measurements, the paper systematically assesses this type of uncertainty.
Robert B. Chatfield, Meinrat O. Andreae, ARCTAS Science Team, and SEAC4RS Science Team
Atmos. Meas. Tech., 13, 7069–7096, https://doi.org/10.5194/amt-13-7069-2020, https://doi.org/10.5194/amt-13-7069-2020, 2020
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Forest burning affects air pollution and global climate. A NASA aircraft studied fire emissions including the Rim Fire near Yosemite. We found frequent confusions between the actual fire emission factors and other effects on the air samples. Effects on CO2 and CO can originate far upwind; the gases can mix variably into a smoke plume. We devised a theory of constant features in plumes. A statistical mixed-effects analysis of a co-emitted tracers model disentangles such mixing from fire effects.
Holger Vömel, Herman G. J. Smit, David Tarasick, Bryan Johnson, Samuel J. Oltmans, Henry Selkirk, Anne M. Thompson, Ryan M. Stauffer, Jacquelyn C. Witte, Jonathan Davies, Roeland van Malderen, Gary A. Morris, Tatsumi Nakano, and Rene Stübi
Atmos. Meas. Tech., 13, 5667–5680, https://doi.org/10.5194/amt-13-5667-2020, https://doi.org/10.5194/amt-13-5667-2020, 2020
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The time response of electrochemical concentration cell (ECC) ozonesondes points to at least two distinct reaction pathways with time constants of approximately 20 s and 25 min. Properly considering these time constants eliminates the need for a poorly defined "background" and allows reducing ad hoc corrections based on laboratory tests. This reduces the uncertainty of ECC ozonesonde measurements throughout the profile and especially in regions of low ozone and strong gradients of ozone.
Fan Zhou, Liwei Hou, Rui Zhong, Wei Chen, Xunpeng Ni, Shengda Pan, Ming Zhao, and Bowen An
Atmos. Meas. Tech., 13, 4899–4909, https://doi.org/10.5194/amt-13-4899-2020, https://doi.org/10.5194/amt-13-4899-2020, 2020
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On 15 July 2019, using an unmanned aerial vehicle (UAV), maritime authorities ferreted out a sailing ship whose fuel sulfur content (FSC) failed to meet Chinese regulations. This was the first time that a sailing ship had been caught for having failed the FSC regulations in China. The UAV system, method, and monitoring result utilized are discussed in this paper. We recommend that emissions from sailing ships be monitored more often in the open water in the future.
Bas Mijling
Atmos. Meas. Tech., 13, 4601–4617, https://doi.org/10.5194/amt-13-4601-2020, https://doi.org/10.5194/amt-13-4601-2020, 2020
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Many cities are experimenting with networks of low-cost sensors, complementary to their reference stations. Often the observations are published as dots on a map, as spatial interpolation is far from trivial. A new methodology to assimilate observations of different accuracy in a generic urban-air-quality model is introduced. It can be used for mapping local air quality based on reference measurements only or as a framework to integrate low-cost measurements next to official measurements.
Kukka-Maaria Kohonen, Pasi Kolari, Linda M. J. Kooijmans, Huilin Chen, Ulli Seibt, Wu Sun, and Ivan Mammarella
Atmos. Meas. Tech., 13, 3957–3975, https://doi.org/10.5194/amt-13-3957-2020, https://doi.org/10.5194/amt-13-3957-2020, 2020
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Biosphere–atmosphere gas exchange (flux) measurements of carbonyl sulfide (COS) are becoming popular for estimating biospheric photosynthesis. To compare COS flux measurements across different measurement sites, we need standardized protocols for data processing. We analyze how various data processing steps affect the calculated COS flux and how they differ from carbon dioxide (CO2) flux processing steps, and we aim to settle on a set of recommended protocols for COS flux calculation.
Michael Müller, Peter Graf, Jonas Meyer, Anastasia Pentina, Dominik Brunner, Fernando Perez-Cruz, Christoph Hüglin, and Lukas Emmenegger
Atmos. Meas. Tech., 13, 3815–3834, https://doi.org/10.5194/amt-13-3815-2020, https://doi.org/10.5194/amt-13-3815-2020, 2020
Yongbiao Weng, Alexandra Touzeau, and Harald Sodemann
Atmos. Meas. Tech., 13, 3167–3190, https://doi.org/10.5194/amt-13-3167-2020, https://doi.org/10.5194/amt-13-3167-2020, 2020
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We find that the known mixing ratio dependence of laser spectrometers for water vapour isotope measurements varies with isotope composition. We have developed a scheme to correct for this isotope-composition-dependent bias. The correction is most substantial at low mixing ratios. Stability tests indicate that the first-order dependency is a constant instrument characteristic. Water vapour isotope measurements at low mixing ratios can now be corrected by following our proposed procedure.
Pascal Wintjen, Christof Ammann, Frederik Schrader, and Christian Brümmer
Atmos. Meas. Tech., 13, 2923–2948, https://doi.org/10.5194/amt-13-2923-2020, https://doi.org/10.5194/amt-13-2923-2020, 2020
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With recent technological advances it is now possible to measure the exchange of trace gases between the land surface and the atmosphere. When using the so-called eddy-covariance method, certain corrections need to be applied to account for attenuation in the flux signal. These losses were found to be setup- and site-specific and can be up to 38 % for reactive nitrogen fluxes. We evaluated five different methods and recommend using an empirical version with locally measured cospectra.
Martin Kunz, Jost V. Lavric, Rainer Gasche, Christoph Gerbig, Richard H. Grant, Frank-Thomas Koch, Marcus Schumacher, Benjamin Wolf, and Matthias Zeeman
Atmos. Meas. Tech., 13, 1671–1692, https://doi.org/10.5194/amt-13-1671-2020, https://doi.org/10.5194/amt-13-1671-2020, 2020
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The nocturnal boundary layer (NBL) budget method enables the quantification of gas fluxes between ecosystems and the atmosphere under nocturnal stable stratification, a condition under which standard approaches struggle. However, up to now the application of the NBL method has been limited by difficulties in obtaining the required measurements. We show how an unmanned aircraft system (UAS) equipped with a carbon dioxide analyser can make this method more accessible.
Marcus Striednig, Martin Graus, Tilmann D. Märk, and Thomas G. Karl
Atmos. Meas. Tech., 13, 1447–1465, https://doi.org/10.5194/amt-13-1447-2020, https://doi.org/10.5194/amt-13-1447-2020, 2020
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The current work summarizes a long-term effort to provide an open-source code for the analysis of turbulent fluctuations of trace gases in the atmosphere by eddy covariance and disjunct eddy covariance, with a special focus on reactive gases that participate in atmospheric chemistry. The performance of the code is successfully evaluated based on measurements of minute fluxes of non-methane volatile organic compounds into the urban atmosphere.
Friedemann Reum, Mathias Göckede, Jost V. Lavric, Olaf Kolle, Sergey Zimov, Nikita Zimov, Martijn Pallandt, and Martin Heimann
Atmos. Meas. Tech., 12, 5717–5740, https://doi.org/10.5194/amt-12-5717-2019, https://doi.org/10.5194/amt-12-5717-2019, 2019
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We present continuous in situ measurements of atmospheric CO2 and CH4 mole fractions at the new station Ambarchik, located in northeastern Siberia. We describe the site, measurements and quality control, characterize the signals in comparison with data from Barrow, Alaska, and show which regions the measurements are sensitive to. Ambarchik data are available upon request.
Nathan Hilker, Jonathan M. Wang, Cheol-Heon Jeong, Robert M. Healy, Uwayemi Sofowote, Jerzy Debosz, Yushan Su, Michael Noble, Anthony Munoz, Geoff Doerksen, Luc White, Céline Audette, Dennis Herod, Jeffrey R. Brook, and Greg J. Evans
Atmos. Meas. Tech., 12, 5247–5261, https://doi.org/10.5194/amt-12-5247-2019, https://doi.org/10.5194/amt-12-5247-2019, 2019
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Increased interest in monitoring air quality near roadways, combined with traffic's often unclear contribution to elevated concentrations, has created a need for better interpretation of these data. Using 2 years of measurements collected during a near-road monitoring project in Canada, this paper contrasts three methods for estimating the fraction of roadside pollution resulting from on-road traffic. Robustness of these methods was compared with tandem measurements at background locations.
Laura Cartwright, Andrew Zammit-Mangion, Sangeeta Bhatia, Ivan Schroder, Frances Phillips, Trevor Coates, Karita Negandhi, Travis Naylor, Martin Kennedy, Steve Zegelin, Nick Wokker, Nicholas M. Deutscher, and Andrew Feitz
Atmos. Meas. Tech., 12, 4659–4676, https://doi.org/10.5194/amt-12-4659-2019, https://doi.org/10.5194/amt-12-4659-2019, 2019
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Despite extensive research, emission detection and quantification of greenhouse gases (GHGs) remain an open problem. This article presents a novel statistical framework for detecting and quantifying methane emissions and showcases its efficacy on data collected from different instruments in the 2015 Ginninderra controlled-release experiment. The developed techniques can be used to aid GHG emission reduction schemes by, for example, detecting and quantifying leaks from carbon storage facilities.
Cited articles
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Hall, B. D., Crotwell, A. M., Kitzis, D. R., Mefford, T., Miller, B. R., Schibig, M. F., and Tans, P. P.: Revision of the World Meteorological Organization Global Atmosphere Watch (WMO/GAW) CO2 calibration scale, Atmos. Meas. Tech., 14, 3015–3032, https://doi.org/10.5194/amt-14-3015-2021, 2021.
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Sasakawa, M., Machida, T., Tsuda, N., Arshinov, M., Davydov, D., Fofonov, A., and Krasnov, O.: Aircraft and tower measurements of CO2 concentration in the planetary boundary layer and the lower free troposphere over southern taiga in West Siberia: Long-term records from 2002 to 2011, J. Geophys. Res.-Atmos., 118, 9489–9498, https://doi.org/10.1002/jgrd.50755, 2013.
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Tohjima, Y., Katsumata, K., Morino, I., Mukai, H., Machida, T., Akama, I., Amari, T., and Tsunogai, U.: Theoretical and experimental evaluation of the isotope effect of NDIR analyzer on atmospheric CO2 measurement, J. Geophys. Res., 114, D13302, https://doi.org/10.1029/2009JD011734, 2009.
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Yver Kwok, C., Laurent, O., Guemri, A., Philippon, C., Wastine, B., Rella, C. W., Vuillemin, C., Truong, F., Delmotte, M., Kazan, V., Darding, M., Lebègue, B., Kaiser, C., Xueref-Rémy, I., and Ramonet, M.: Comprehensive laboratory and field testing of cavity ring-down spectroscopy analyzers measuring H2O, CO2, CH4 and CO, Atmos. Meas. Tech., 8, 3867–3892, https://doi.org/10.5194/amt-8-3867-2015, 2015.
Short summary
Standard gases are essential for accurate greenhouse gas measurements. However, exchanging cylinders at remote sites presents logistical challenges, requiring systems that minimize gas consumption. We developed methods for calculating greenhouse gas mole fractions and uncertainties using our original system designed to reduce standard gas use. We validated its long-term stability through instrument comparisons. The system has proven effective for maintaining observations at remote sites.
Standard gases are essential for accurate greenhouse gas measurements. However, exchanging...
