Articles | Volume 19, issue 20
https://doi.org/10.5194/amt-19-6517-2026
© Author(s) 2026. This work is distributed under the Creative Commons Attribution 4.0 License.
Classification-constrained retrieval of PM2.5 vertical profiles from fluorescence-raman-mie polarization lidar
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- Final revised paper (published on 16 Oct 2026)
- Supplement to the final revised paper
- Preprint (discussion started on 03 Aug 2026)
- Supplement to the preprint
Interactive discussion
Status: closed
Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor
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RC1: 'Comment on egusphere-2026-2485', Anonymous Referee #1, 21 Aug 2026
- AC1: 'Reply on RC1', Pan Guo, 20 Sep 2026
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RC2: 'Comment on egusphere-2026-2485', Anonymous Referee #2, 11 Sep 2026
- AC2: 'Reply on RC2', Pan Guo, 20 Sep 2026
Peer review completion
AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Pan Guo on behalf of the Authors (20 Sep 2026)
Author's response
Author's tracked changes
Manuscript
ED: Publish as is (22 Sep 2026) by Vassilis Amiridis
AR by Pan Guo on behalf of the Authors (24 Sep 2026)
Manuscript
The authors have substantially revised the manuscript and have addressed most of the concerns raised in my previous review. In particular, the revised manuscript now includes date-separated quantitative validation using 411 hourly near-surface samples, comparison of the classification-constrained retrieval with unconstrained and PDR-only models, sensitivity analyses of aerosol classification end-member parameters and aerosol-type-dependent lidar ratios, and a more comprehensive uncertainty analysis including model-parameter uncertainty. The discussion of aerosol chemical composition, seasonal applicability, and model generalizability has also been substantially improved.
The quantitative comparison is particularly useful. The combined PDR–Gf classification model achieves substantially lower RMSE, MAE, and bias than the model without aerosol-type constraints and the PDR-only model. These results provide much stronger quantitative evidence for the benefit of the proposed classification constraint than was available in the previous version.
The revised treatment of the extinction-partitioning assumption is also satisfactory. The authors now explicitly recognize that different aerosol components may have different lidar ratios, formulate the corresponding aerosol-type-dependent extinction partitioning, and quantify the sensitivity of the retrieved PM₂.₅ to plausible lidar-ratio variations. Similarly, the Monte Carlo analysis of PDR and fluorescence end-member parameters provides a useful assessment of the sensitivity of the retrieval to classification assumptions.
I have only a few remaining comments:
The new near-surface comparison provides important quantitative validation of the empirical retrieval model, but it should be clearly distinguished from independent validation of the complete vertical PM₂.₅ profiles. As the authors appropriately acknowledge in the Conclusions, direct vertically resolved PM₂.₅ observations from UAVs, tethered balloons, or aircraft are not available. Please ensure that the terminology used throughout the Abstract, Results, and Conclusions does not imply that the full vertical profiles have been independently validated.
The uncertainty analysis based on perturbations of the PDR and Gf end-member parameters represents sensitivity to the assumed classification parameters rather than instrument-level measurement uncertainties in PDR and Gf. The manuscript recognizes this distinction in Methods. I suggest maintaining this distinction explicitly when discussing “classification uncertainty” elsewhere in the manuscript.
I still encourage the authors to improve the data and code availability statement. At present, the lidar data, processed datasets, and analysis scripts are available upon reasonable request. If possible, the processed datasets underlying the principal figures and validation analysis, together with the relevant analysis code, should be deposited in a public repository with a persistent DOI. This would substantially improve reproducibility.
Overall, I believe that the authors have responded constructively to the major concerns of the previous review and that the methodological support for the conclusions is now considerably stronger. The remaining issues are primarily matters of clarification, terminology, and reproducibility rather than fundamental methodological concerns.