Articles | Volume 6, issue 12
https://doi.org/10.5194/amt-6-3425-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-6-3425-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
09 Dec 2013
Research article |
| 09 Dec 2013
Reporting the sensitivity of laser-induced fluorescence instruments used for HO2 detection to an interference from RO2 radicals and introducing a novel approach that enables HO2 and certain RO2 types to be selectively measured
L. K. Whalley
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Atmospheric Science, University of Leeds, Leeds, LS2 9JT, UK
M. A. Blitz
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Atmospheric Science, University of Leeds, Leeds, LS2 9JT, UK
M. Desservettaz
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
P. W. Seakins
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Atmospheric Science, University of Leeds, Leeds, LS2 9JT, UK
D. E. Heard
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Atmospheric Science, University of Leeds, Leeds, LS2 9JT, UK
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Cited
66 citations as recorded by crossref.
- Effect of the Alkoxy Radical Chemistry on the Ozone Formation from Anthropogenic Organic Compounds Investigated in Chamber Experiments M. Färber et al. 10.1021/acsestair.4c00064
- A new technique for the direct detection of HO<sub>2</sub> radicals using bromide chemical ionization mass spectrometry (Br-CIMS): initial characterization J. Sanchez et al. 10.5194/amt-9-3851-2016
- Wintertime photochemistry in Beijing: observations of RO<sub><i>x</i></sub> radical concentrations in the North China Plain during the BEST-ONE campaign Z. Tan et al. 10.5194/acp-18-12391-2018
- Observation and simulation of HOx radicals in an urban area in Shanghai, China G. Zhang et al. 10.1016/j.scitotenv.2021.152275
- Diurnal variability, photochemical production and loss processes of hydrogen peroxide in the boundary layer over Europe H. Fischer et al. 10.5194/acp-19-11953-2019
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- Exploring Oxidation in the Remote Free Troposphere: Insights From Atmospheric Tomography (ATom) W. Brune et al. 10.1029/2019JD031685
- Review of technologies and their applications for the speciated detection of RO2 radicals Y. Gao et al. 10.1016/j.jes.2022.09.028
- Impact of HO2 aerosol uptake on radical levels and O3 production during summertime in Beijing J. Dyson et al. 10.5194/acp-23-5679-2023
- Reactive indoor air chemistry and health—A workshop summary J. Wells et al. 10.1016/j.ijheh.2017.09.009
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- Measurements of hydroxyl and hydroperoxy radicals during CalNex‐LA: Model comparisons and radical budgets S. Griffith et al. 10.1002/2015JD024358
- Measurements of hydroperoxy radicals (HO<sub>2</sub>) at atmospheric concentrations using bromide chemical ionisation mass spectrometry S. Albrecht et al. 10.5194/amt-12-891-2019
- Intercomparison of measured and modelled photochemical ozone production rates: Suggestion of chemistry hypothesis regarding unmeasured VOCs J. Zhou et al. 10.1016/j.scitotenv.2024.175290
- Experimental budgets of OH, HO<sub>2</sub>, and RO<sub>2</sub> radicals and implications for ozone formation in the Pearl River Delta in China 2014 Z. Tan et al. 10.5194/acp-19-7129-2019
- Evaluating the sensitivity of radical chemistry and ozone formation to ambient VOCs and NO<sub><i>x</i></sub> in Beijing L. Whalley et al. 10.5194/acp-21-2125-2021
- The influence of clouds on radical concentrations: observations and modelling studies of HO<sub>x</sub> during the Hill Cap Cloud Thuringia (HCCT) campaign in 2010 L. Whalley et al. 10.5194/acp-15-3289-2015
- Measurement of interferences associated with the detection of the hydroperoxy radical in the atmosphere using laser-induced fluorescence M. Lew et al. 10.5194/amt-11-95-2018
- Comparison of temperature-dependent calibration methods of an instrument to measure OH and HO2 radicals using laser-induced fluorescence spectroscopy F. Winiberg et al. 10.5194/amt-16-4375-2023
- Experimental and theoretical study on the impact of a nitrate group on the chemistry of alkoxy radicals A. Novelli et al. 10.1039/D0CP05555G
- Techniques for measuring indoor radicals and radical precursors E. Alvarez et al. 10.1080/05704928.2022.2087666
- Radical chemistry at a rural site (Wangdu) in the North China Plain: observation and model calculations of OH, HO<sub>2</sub> and RO<sub>2</sub> radicals Z. Tan et al. 10.5194/acp-17-663-2017
- Understanding in situ ozone production in the summertime through radical observations and modelling studies during the Clean air for London project (ClearfLo) L. Whalley et al. 10.5194/acp-18-2547-2018
- A new method for atmospheric detection of the CH<sub>3</sub>O<sub>2</sub> radical L. Onel et al. 10.5194/amt-10-3985-2017
- Peroxy radical measurements by ethane – nitric oxide chemical amplification and laser-induced fluorescence during the IRRONIC field campaign in a forest in Indiana S. Kundu et al. 10.5194/acp-19-9563-2019
- An intercomparison of HO<sub>2</sub> measurements by fluorescence assay by gas expansion and cavity ring-down spectroscopy within HIRAC (Highly Instrumented Reactor for Atmospheric Chemistry) L. Onel et al. 10.5194/amt-10-4877-2017
- Missing peroxy radical sources within a summertime ponderosa pine forest G. Wolfe et al. 10.5194/acp-14-4715-2014
- Importance of isomerization reactions for OH radical regeneration from the photo-oxidation of isoprene investigated in the atmospheric simulation chamber SAPHIR A. Novelli et al. 10.5194/acp-20-3333-2020
- Speciated Monitoring of Gas-Phase Organic Peroxy Radicals by Chemical Ionization Mass Spectrometry: Cross-Reactions between CH3O2, CH3(CO)O2, (CH3)3CO2, and c-C6H11O2 B. Nozière & D. Hanson 10.1021/acs.jpca.7b06456
- The effect of viscosity and diffusion on the HO<sub>2</sub> uptake by sucrose and secondary organic aerosol particles P. Lakey et al. 10.5194/acp-16-13035-2016
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- Detailed budget analysis of HONO in central London reveals a missing daytime source J. Lee et al. 10.5194/acp-16-2747-2016
- New Instrument for Time-Resolved OH and HO2 Quantification in High-Pressure Laboratory Kinetics Studies L. Sheps & K. Au 10.1021/acs.jpca.4c00994
- Theoretical and experimental study of peroxy and alkoxy radicals in the NO3-initiated oxidation of isoprene L. Vereecken et al. 10.1039/D0CP06267G
- Dimeric Product of Peroxy Radical Self-Reaction Probed with VUV Photoionization Mass Spectrometry and Theoretical Calculations: The Case of C2H5OOC2H5 H. Yue et al. 10.3390/ijms24043731
- Impacts of bromine and iodine chemistry on tropospheric OH and HO<sub>2</sub>: comparing observations with box and global model perspectives D. Stone et al. 10.5194/acp-18-3541-2018
- Chemical Amplification - Cavity Attenuated Phase Shift Spectroscopy Measurements of Atmospheric Peroxy Radicals E. Wood & J. Charest 10.1021/ac502451m
- A hydroxyl radical detection system using gas expansion and fast gating laser-induced fluorescence techniques H. Chen et al. 10.1016/j.jes.2017.03.012
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- Significant OH production under surface cleaning and air cleaning conditions: Impact on indoor air quality N. Carslaw et al. 10.1111/ina.12394
- Rate constants of CH3O2 + NO2 CH3O2NO2 and C2H5O2 + NO2 C2H5O2NO2 reactions under atmospheric conditions N. Kohno et al. 10.1002/kin.21466
- Direct measurements of OH and other product yields from the HO<sub>2</sub> + CH<sub>3</sub>C(O)O<sub>2</sub> reaction F. Winiberg et al. 10.5194/acp-16-4023-2016
- Photooxidation of pinonaldehyde at ambient conditions investigated in the atmospheric simulation chamber SAPHIR M. Rolletter et al. 10.5194/acp-20-13701-2020
- Night-time measurements of HO<sub><i>x</i></sub> during the RONOCO project and analysis of the sources of HO<sub>2</sub> H. Walker et al. 10.5194/acp-15-8179-2015
- Investigation of the Cyclohexene Oxidation Mechanism Through the Direct Measurement of Organic Peroxy Radicals Y. Li et al. 10.1021/acs.est.4c06744
- Airborne measurement of peroxy radicals using chemical amplification coupled with cavity ring-down spectroscopy: the PeRCEAS instrument M. George et al. 10.5194/amt-13-2577-2020
- Measurements of Atmospheric HO2 Radicals Using Br-CIMS with Elimination of Potential Interferences from Ambient Peroxynitric Acid L. Wang et al. 10.1021/acs.analchem.4c01184
- The Molecular Identification of Organic Compounds in the Atmosphere: State of the Art and Challenges B. Nozière et al. 10.1021/cr5003485
- OH and HO<sub>2</sub> radical chemistry at a suburban site during the EXPLORE-YRD campaign in 2018 X. Ma et al. 10.5194/acp-22-7005-2022
- Improved laser-induced fluorescent instrument for online peroxy radical measurement: Consistency in high-sensitivity for detection G. Zhang et al. 10.1016/j.snb.2024.136774
- HONO measurement by differential photolysis C. Reed et al. 10.5194/amt-9-2483-2016
- Winter photochemistry in Beijing: Observation and model simulation of OH and HO2 radicals at an urban site X. Ma et al. 10.1016/j.scitotenv.2019.05.329
- Study of the Formation Dynamics of OH from the Photolysis of O3 by Ultrashort Laser Pulses J. Gao et al. 10.1021/acs.jpclett.0c01770
- Implementation of a chemical background method for atmospheric OH measurements by laser-induced fluorescence: characterisation and observations from the UK and China R. Woodward-Massey et al. 10.5194/amt-13-3119-2020
- Pressure-dependent calibration of the OH and HO<sub>2</sub> channels of a FAGE HO<sub>x</sub> instrument using the Highly Instrumented Reactor for Atmospheric Chemistry (HIRAC) F. Winiberg et al. 10.5194/amt-8-523-2015
- Testing Atmospheric Oxidation in an Alabama Forest P. Feiner et al. 10.1175/JAS-D-16-0044.1
- Measurement of tropospheric HO2 radical using fluorescence assay by gas expansion with low interferences Y. Wang et al. 10.1016/j.jes.2020.06.010
- Radical chemistry at night: comparisons between observed and modelled HO<sub>x</sub>, NO<sub>3</sub> and N<sub>2</sub>O<sub>5</sub> during the RONOCO project D. Stone et al. 10.5194/acp-14-1299-2014
- Evaluation of OH and HO<sub>2</sub> concentrations and their budgets during photooxidation of 2-methyl-3-butene-2-ol (MBO) in the atmospheric simulation chamber SAPHIR A. Novelli et al. 10.5194/acp-18-11409-2018
- A new instrument for time-resolved measurement of HO<sub>2</sub> radicals T. Speak et al. 10.5194/amt-13-839-2020
- An intercomparison of CH3O2 measurements by fluorescence assay by gas expansion and cavity ring-down spectroscopy within HIRAC (Highly Instrumented Reactor for Atmospheric Chemistry) L. Onel et al. 10.5194/amt-13-2441-2020
- Meteorology, Air Quality, and Health in London: The ClearfLo Project S. Bohnenstengel et al. 10.1175/BAMS-D-12-00245.1
- Observation and modelling of HO<sub>x</sub> radicals in a boreal forest K. Hens et al. 10.5194/acp-14-8723-2014
- Missing peroxy radical sources within a summertime ponderosa pine forest G. Wolfe et al. 10.5194/acp-14-4715-2014
63 citations as recorded by crossref.
- Effect of the Alkoxy Radical Chemistry on the Ozone Formation from Anthropogenic Organic Compounds Investigated in Chamber Experiments M. Färber et al. 10.1021/acsestair.4c00064
- A new technique for the direct detection of HO<sub>2</sub> radicals using bromide chemical ionization mass spectrometry (Br-CIMS): initial characterization J. Sanchez et al. 10.5194/amt-9-3851-2016
- Wintertime photochemistry in Beijing: observations of RO<sub><i>x</i></sub> radical concentrations in the North China Plain during the BEST-ONE campaign Z. Tan et al. 10.5194/acp-18-12391-2018
- Observation and simulation of HOx radicals in an urban area in Shanghai, China G. Zhang et al. 10.1016/j.scitotenv.2021.152275
- Diurnal variability, photochemical production and loss processes of hydrogen peroxide in the boundary layer over Europe H. Fischer et al. 10.5194/acp-19-11953-2019
- Radical chemistry and ozone production at a UK coastal receptor site R. Woodward-Massey et al. 10.5194/acp-23-14393-2023
- Exploring Oxidation in the Remote Free Troposphere: Insights From Atmospheric Tomography (ATom) W. Brune et al. 10.1029/2019JD031685
- Review of technologies and their applications for the speciated detection of RO2 radicals Y. Gao et al. 10.1016/j.jes.2022.09.028
- Impact of HO2 aerosol uptake on radical levels and O3 production during summertime in Beijing J. Dyson et al. 10.5194/acp-23-5679-2023
- Reactive indoor air chemistry and health—A workshop summary J. Wells et al. 10.1016/j.ijheh.2017.09.009
- Gas‐phase rate coefficients for a series of alkyl cyclohexanes with OH radicals and Cl atoms I. Bejan et al. 10.1002/kin.21179
- Measurements of hydroxyl and hydroperoxy radicals during CalNex‐LA: Model comparisons and radical budgets S. Griffith et al. 10.1002/2015JD024358
- Measurements of hydroperoxy radicals (HO<sub>2</sub>) at atmospheric concentrations using bromide chemical ionisation mass spectrometry S. Albrecht et al. 10.5194/amt-12-891-2019
- Intercomparison of measured and modelled photochemical ozone production rates: Suggestion of chemistry hypothesis regarding unmeasured VOCs J. Zhou et al. 10.1016/j.scitotenv.2024.175290
- Experimental budgets of OH, HO<sub>2</sub>, and RO<sub>2</sub> radicals and implications for ozone formation in the Pearl River Delta in China 2014 Z. Tan et al. 10.5194/acp-19-7129-2019
- Evaluating the sensitivity of radical chemistry and ozone formation to ambient VOCs and NO<sub><i>x</i></sub> in Beijing L. Whalley et al. 10.5194/acp-21-2125-2021
- The influence of clouds on radical concentrations: observations and modelling studies of HO<sub>x</sub> during the Hill Cap Cloud Thuringia (HCCT) campaign in 2010 L. Whalley et al. 10.5194/acp-15-3289-2015
- Measurement of interferences associated with the detection of the hydroperoxy radical in the atmosphere using laser-induced fluorescence M. Lew et al. 10.5194/amt-11-95-2018
- Comparison of temperature-dependent calibration methods of an instrument to measure OH and HO2 radicals using laser-induced fluorescence spectroscopy F. Winiberg et al. 10.5194/amt-16-4375-2023
- Experimental and theoretical study on the impact of a nitrate group on the chemistry of alkoxy radicals A. Novelli et al. 10.1039/D0CP05555G
- Techniques for measuring indoor radicals and radical precursors E. Alvarez et al. 10.1080/05704928.2022.2087666
- Radical chemistry at a rural site (Wangdu) in the North China Plain: observation and model calculations of OH, HO<sub>2</sub> and RO<sub>2</sub> radicals Z. Tan et al. 10.5194/acp-17-663-2017
- Understanding in situ ozone production in the summertime through radical observations and modelling studies during the Clean air for London project (ClearfLo) L. Whalley et al. 10.5194/acp-18-2547-2018
- A new method for atmospheric detection of the CH<sub>3</sub>O<sub>2</sub> radical L. Onel et al. 10.5194/amt-10-3985-2017
- Peroxy radical measurements by ethane – nitric oxide chemical amplification and laser-induced fluorescence during the IRRONIC field campaign in a forest in Indiana S. Kundu et al. 10.5194/acp-19-9563-2019
- An intercomparison of HO<sub>2</sub> measurements by fluorescence assay by gas expansion and cavity ring-down spectroscopy within HIRAC (Highly Instrumented Reactor for Atmospheric Chemistry) L. Onel et al. 10.5194/amt-10-4877-2017
- Missing peroxy radical sources within a summertime ponderosa pine forest G. Wolfe et al. 10.5194/acp-14-4715-2014
- Importance of isomerization reactions for OH radical regeneration from the photo-oxidation of isoprene investigated in the atmospheric simulation chamber SAPHIR A. Novelli et al. 10.5194/acp-20-3333-2020
- Speciated Monitoring of Gas-Phase Organic Peroxy Radicals by Chemical Ionization Mass Spectrometry: Cross-Reactions between CH3O2, CH3(CO)O2, (CH3)3CO2, and c-C6H11O2 B. Nozière & D. Hanson 10.1021/acs.jpca.7b06456
- The effect of viscosity and diffusion on the HO<sub>2</sub> uptake by sucrose and secondary organic aerosol particles P. Lakey et al. 10.5194/acp-16-13035-2016
- OH and HO<sub>2</sub> radical chemistry in a midlatitude forest: measurements and model comparisons M. Lew et al. 10.5194/acp-20-9209-2020
- Investigation of the oxidation of methyl vinyl ketone (MVK) by OH radicals in the atmospheric simulation chamber SAPHIR H. Fuchs et al. 10.5194/acp-18-8001-2018
- OH, HO2, and RO2 radical chemistry in a rural forest environment: measurements, model comparisons, and evidence of a missing radical sink B. Bottorff et al. 10.5194/acp-23-10287-2023
- Detailed budget analysis of HONO in central London reveals a missing daytime source J. Lee et al. 10.5194/acp-16-2747-2016
- New Instrument for Time-Resolved OH and HO2 Quantification in High-Pressure Laboratory Kinetics Studies L. Sheps & K. Au 10.1021/acs.jpca.4c00994
- Theoretical and experimental study of peroxy and alkoxy radicals in the NO3-initiated oxidation of isoprene L. Vereecken et al. 10.1039/D0CP06267G
- Dimeric Product of Peroxy Radical Self-Reaction Probed with VUV Photoionization Mass Spectrometry and Theoretical Calculations: The Case of C2H5OOC2H5 H. Yue et al. 10.3390/ijms24043731
- Impacts of bromine and iodine chemistry on tropospheric OH and HO<sub>2</sub>: comparing observations with box and global model perspectives D. Stone et al. 10.5194/acp-18-3541-2018
- Chemical Amplification - Cavity Attenuated Phase Shift Spectroscopy Measurements of Atmospheric Peroxy Radicals E. Wood & J. Charest 10.1021/ac502451m
- A hydroxyl radical detection system using gas expansion and fast gating laser-induced fluorescence techniques H. Chen et al. 10.1016/j.jes.2017.03.012
- Elevated levels of OH observed in haze events during wintertime in central Beijing E. Slater et al. 10.5194/acp-20-14847-2020
- Significant OH production under surface cleaning and air cleaning conditions: Impact on indoor air quality N. Carslaw et al. 10.1111/ina.12394
- Rate constants of CH3O2 + NO2 CH3O2NO2 and C2H5O2 + NO2 C2H5O2NO2 reactions under atmospheric conditions N. Kohno et al. 10.1002/kin.21466
- Direct measurements of OH and other product yields from the HO<sub>2</sub> + CH<sub>3</sub>C(O)O<sub>2</sub> reaction F. Winiberg et al. 10.5194/acp-16-4023-2016
- Photooxidation of pinonaldehyde at ambient conditions investigated in the atmospheric simulation chamber SAPHIR M. Rolletter et al. 10.5194/acp-20-13701-2020
- Night-time measurements of HO<sub><i>x</i></sub> during the RONOCO project and analysis of the sources of HO<sub>2</sub> H. Walker et al. 10.5194/acp-15-8179-2015
- Investigation of the Cyclohexene Oxidation Mechanism Through the Direct Measurement of Organic Peroxy Radicals Y. Li et al. 10.1021/acs.est.4c06744
- Airborne measurement of peroxy radicals using chemical amplification coupled with cavity ring-down spectroscopy: the PeRCEAS instrument M. George et al. 10.5194/amt-13-2577-2020
- Measurements of Atmospheric HO2 Radicals Using Br-CIMS with Elimination of Potential Interferences from Ambient Peroxynitric Acid L. Wang et al. 10.1021/acs.analchem.4c01184
- The Molecular Identification of Organic Compounds in the Atmosphere: State of the Art and Challenges B. Nozière et al. 10.1021/cr5003485
- OH and HO<sub>2</sub> radical chemistry at a suburban site during the EXPLORE-YRD campaign in 2018 X. Ma et al. 10.5194/acp-22-7005-2022
- Improved laser-induced fluorescent instrument for online peroxy radical measurement: Consistency in high-sensitivity for detection G. Zhang et al. 10.1016/j.snb.2024.136774
- HONO measurement by differential photolysis C. Reed et al. 10.5194/amt-9-2483-2016
- Winter photochemistry in Beijing: Observation and model simulation of OH and HO2 radicals at an urban site X. Ma et al. 10.1016/j.scitotenv.2019.05.329
- Study of the Formation Dynamics of OH from the Photolysis of O3 by Ultrashort Laser Pulses J. Gao et al. 10.1021/acs.jpclett.0c01770
- Implementation of a chemical background method for atmospheric OH measurements by laser-induced fluorescence: characterisation and observations from the UK and China R. Woodward-Massey et al. 10.5194/amt-13-3119-2020
- Pressure-dependent calibration of the OH and HO<sub>2</sub> channels of a FAGE HO<sub>x</sub> instrument using the Highly Instrumented Reactor for Atmospheric Chemistry (HIRAC) F. Winiberg et al. 10.5194/amt-8-523-2015
- Testing Atmospheric Oxidation in an Alabama Forest P. Feiner et al. 10.1175/JAS-D-16-0044.1
- Measurement of tropospheric HO2 radical using fluorescence assay by gas expansion with low interferences Y. Wang et al. 10.1016/j.jes.2020.06.010
- Radical chemistry at night: comparisons between observed and modelled HO<sub>x</sub>, NO<sub>3</sub> and N<sub>2</sub>O<sub>5</sub> during the RONOCO project D. Stone et al. 10.5194/acp-14-1299-2014
- Evaluation of OH and HO<sub>2</sub> concentrations and their budgets during photooxidation of 2-methyl-3-butene-2-ol (MBO) in the atmospheric simulation chamber SAPHIR A. Novelli et al. 10.5194/acp-18-11409-2018
- A new instrument for time-resolved measurement of HO<sub>2</sub> radicals T. Speak et al. 10.5194/amt-13-839-2020
- An intercomparison of CH3O2 measurements by fluorescence assay by gas expansion and cavity ring-down spectroscopy within HIRAC (Highly Instrumented Reactor for Atmospheric Chemistry) L. Onel et al. 10.5194/amt-13-2441-2020
3 citations as recorded by crossref.
- Meteorology, Air Quality, and Health in London: The ClearfLo Project S. Bohnenstengel et al. 10.1175/BAMS-D-12-00245.1
- Observation and modelling of HO<sub>x</sub> radicals in a boreal forest K. Hens et al. 10.5194/acp-14-8723-2014
- Missing peroxy radical sources within a summertime ponderosa pine forest G. Wolfe et al. 10.5194/acp-14-4715-2014
Saved (final revised paper)
Latest update: 13 Dec 2024
