Articles | Volume 8, issue 8
https://doi.org/10.5194/amt-8-3537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-8-3537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
31 Aug 2015
Research article |
| 31 Aug 2015
Detailed characterizations of the new Mines Douai comparative reactivity method instrument via laboratory experiments and modeling
V. Michoud
CORRESPONDING AUTHOR
Mines Douai, SAGE, 59508 Douai, France
Université de Lille, Lille, France
R. F. Hansen
Mines Douai, SAGE, 59508 Douai, France
School of Public and Environmental Affairs, Indiana University, Bloomington, IN, USA
Department of chemistry, Indiana University, Bloomington, IN, USA
now at: School of chemistry, University of Leeds, Leeds, UK
N. Locoge
Mines Douai, SAGE, 59508 Douai, France
Université de Lille, Lille, France
P. S. Stevens
School of Public and Environmental Affairs, Indiana University, Bloomington, IN, USA
Department of chemistry, Indiana University, Bloomington, IN, USA
S. Dusanter
CORRESPONDING AUTHOR
Mines Douai, SAGE, 59508 Douai, France
School of Public and Environmental Affairs, Indiana University, Bloomington, IN, USA
Université de Lille, Lille, France
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Cited
29 citations as recorded by crossref.
- Intercomparison of two comparative reactivity method instruments inf the Mediterranean basin during summer 2013 N. Zannoni et al. 10.5194/amt-8-3851-2015
- Towards a quantitative understanding of total OH reactivity: A review Y. Yang et al. 10.1016/j.atmosenv.2016.03.010
- OH reactivity of the urban air in Helsinki, Finland, during winter A. Praplan et al. 10.1016/j.atmosenv.2017.09.013
- Variability of hydroxyl radical (OH) reactivity in the Landes maritime pine forest: results from the LANDEX campaign 2017 S. Bsaibes et al. 10.5194/acp-20-1277-2020
- Measurement of OH reactivity by laser flash photolysis coupled with laser-induced fluorescence spectroscopy D. Stone et al. 10.5194/amt-9-2827-2016
- Summertime OH reactivity from a receptor coastal site in the Mediterranean Basin N. Zannoni et al. 10.5194/acp-17-12645-2017
- Proton-Transfer-Reaction Mass Spectrometry: Applications in Atmospheric Sciences B. Yuan et al. 10.1021/acs.chemrev.7b00325
- Characterization of Total OH Reactivity in a Rapeseed Field: Results from the COV3ER Experiment in April 2017 S. Bsaibes et al. 10.3390/atmos11030261
- Global modelling of the total OH reactivity: investigations on the “missing” OH sink and its atmospheric implications V. Ferracci et al. 10.5194/acp-18-7109-2018
- Techniques for measuring indoor radicals and radical precursors E. Alvarez et al. 10.1080/05704928.2022.2087666
- Measurement report: Important contributions of oxygenated compounds to emissions and chemistry of volatile organic compounds in urban air C. Wu et al. 10.5194/acp-20-14769-2020
- The improved comparative reactivity method (ICRM): measurements of OH reactivity under high-NO<sub><i>x</i></sub> conditions in ambient air W. Wang et al. 10.5194/amt-14-2285-2021
- Total OH Reactivity of Emissions from Humans: In Situ Measurement and Budget Analysis N. Wang et al. 10.1021/acs.est.0c04206
- Fast measurement of OH reactivity utilizing laser photolysis-laser induced fluorescence system based on kOH-NLM algorithm Y. Wang et al. 10.1016/j.snb.2024.136798
- Total OH Reactivity Changes Over the Amazon Rainforest During an El Niño Event E. Pfannerstill et al. 10.3389/ffgc.2018.00012
- Exploring ozone pollution in Chengdu, southwestern China: A case study from radical chemistry to O3-VOC-NOx sensitivity Z. Tan et al. 10.1016/j.scitotenv.2018.04.286
- Comparison of OH reactivity measurements in the atmospheric simulation chamber SAPHIR H. Fuchs et al. 10.5194/amt-10-4023-2017
- Total OH Reactivity Measurements in a Suburban Site of Shanghai G. Yang et al. 10.1029/2021JD035981
- Simulation of Cluster Dynamics of Proton-Bound Water Clusters in a High Kinetic Energy Ion-Mobility Spectrometer D. Erdogdu et al. 10.1021/jasms.1c00140
- Effect of Ozone, Clothing, Temperature, and Humidity on the Total OH Reactivity Emitted from Humans N. Zannoni et al. 10.1021/acs.est.1c01831
- OH reactivity from the emissions of different tree species: investigating the missing reactivity in a boreal forest A. Praplan et al. 10.5194/bg-17-4681-2020
- Shipborne measurements of total OH reactivity around the Arabian Peninsula and its role in ozone chemistry E. Pfannerstill et al. 10.5194/acp-19-11501-2019
- Intercomparison of OH and OH reactivity measurements in a high isoprene and low NO environment during the Southern Oxidant and Aerosol Study (SOAS) D. Sanchez et al. 10.1016/j.atmosenv.2017.10.056
- The Indoor Chemical Human Emissions and Reactivity (ICHEAR) project: Overview of experimental methodology and preliminary results G. Bekö et al. 10.1111/ina.12687
- How the OH reactivity affects the ozone production efficiency: case studies in Beijing and Heshan, China Y. Yang et al. 10.5194/acp-17-7127-2017
- Intercomparison of the comparative reactivity method (CRM) and pump–probe technique for measuring total OH reactivity in an urban environment R. Hansen et al. 10.5194/amt-8-4243-2015
- Long-term total OH reactivity measurements in a boreal forest A. Praplan et al. 10.5194/acp-19-14431-2019
- Total OH reactivity over the Amazon rainforest: variability with temperature, wind, rain, altitude, time of day, season, and an overall budget closure E. Pfannerstill et al. 10.5194/acp-21-6231-2021
- Intercomparison of two Comparative Reactivity Method instruments in the Mediterranean basin during summer 2013 N. Zannoni et al. 10.5194/amtd-8-5065-2015
28 citations as recorded by crossref.
- Intercomparison of two comparative reactivity method instruments inf the Mediterranean basin during summer 2013 N. Zannoni et al. 10.5194/amt-8-3851-2015
- Towards a quantitative understanding of total OH reactivity: A review Y. Yang et al. 10.1016/j.atmosenv.2016.03.010
- OH reactivity of the urban air in Helsinki, Finland, during winter A. Praplan et al. 10.1016/j.atmosenv.2017.09.013
- Variability of hydroxyl radical (OH) reactivity in the Landes maritime pine forest: results from the LANDEX campaign 2017 S. Bsaibes et al. 10.5194/acp-20-1277-2020
- Measurement of OH reactivity by laser flash photolysis coupled with laser-induced fluorescence spectroscopy D. Stone et al. 10.5194/amt-9-2827-2016
- Summertime OH reactivity from a receptor coastal site in the Mediterranean Basin N. Zannoni et al. 10.5194/acp-17-12645-2017
- Proton-Transfer-Reaction Mass Spectrometry: Applications in Atmospheric Sciences B. Yuan et al. 10.1021/acs.chemrev.7b00325
- Characterization of Total OH Reactivity in a Rapeseed Field: Results from the COV3ER Experiment in April 2017 S. Bsaibes et al. 10.3390/atmos11030261
- Global modelling of the total OH reactivity: investigations on the “missing” OH sink and its atmospheric implications V. Ferracci et al. 10.5194/acp-18-7109-2018
- Techniques for measuring indoor radicals and radical precursors E. Alvarez et al. 10.1080/05704928.2022.2087666
- Measurement report: Important contributions of oxygenated compounds to emissions and chemistry of volatile organic compounds in urban air C. Wu et al. 10.5194/acp-20-14769-2020
- The improved comparative reactivity method (ICRM): measurements of OH reactivity under high-NO<sub><i>x</i></sub> conditions in ambient air W. Wang et al. 10.5194/amt-14-2285-2021
- Total OH Reactivity of Emissions from Humans: In Situ Measurement and Budget Analysis N. Wang et al. 10.1021/acs.est.0c04206
- Fast measurement of OH reactivity utilizing laser photolysis-laser induced fluorescence system based on kOH-NLM algorithm Y. Wang et al. 10.1016/j.snb.2024.136798
- Total OH Reactivity Changes Over the Amazon Rainforest During an El Niño Event E. Pfannerstill et al. 10.3389/ffgc.2018.00012
- Exploring ozone pollution in Chengdu, southwestern China: A case study from radical chemistry to O3-VOC-NOx sensitivity Z. Tan et al. 10.1016/j.scitotenv.2018.04.286
- Comparison of OH reactivity measurements in the atmospheric simulation chamber SAPHIR H. Fuchs et al. 10.5194/amt-10-4023-2017
- Total OH Reactivity Measurements in a Suburban Site of Shanghai G. Yang et al. 10.1029/2021JD035981
- Simulation of Cluster Dynamics of Proton-Bound Water Clusters in a High Kinetic Energy Ion-Mobility Spectrometer D. Erdogdu et al. 10.1021/jasms.1c00140
- Effect of Ozone, Clothing, Temperature, and Humidity on the Total OH Reactivity Emitted from Humans N. Zannoni et al. 10.1021/acs.est.1c01831
- OH reactivity from the emissions of different tree species: investigating the missing reactivity in a boreal forest A. Praplan et al. 10.5194/bg-17-4681-2020
- Shipborne measurements of total OH reactivity around the Arabian Peninsula and its role in ozone chemistry E. Pfannerstill et al. 10.5194/acp-19-11501-2019
- Intercomparison of OH and OH reactivity measurements in a high isoprene and low NO environment during the Southern Oxidant and Aerosol Study (SOAS) D. Sanchez et al. 10.1016/j.atmosenv.2017.10.056
- The Indoor Chemical Human Emissions and Reactivity (ICHEAR) project: Overview of experimental methodology and preliminary results G. Bekö et al. 10.1111/ina.12687
- How the OH reactivity affects the ozone production efficiency: case studies in Beijing and Heshan, China Y. Yang et al. 10.5194/acp-17-7127-2017
- Intercomparison of the comparative reactivity method (CRM) and pump–probe technique for measuring total OH reactivity in an urban environment R. Hansen et al. 10.5194/amt-8-4243-2015
- Long-term total OH reactivity measurements in a boreal forest A. Praplan et al. 10.5194/acp-19-14431-2019
- Total OH reactivity over the Amazon rainforest: variability with temperature, wind, rain, altitude, time of day, season, and an overall budget closure E. Pfannerstill et al. 10.5194/acp-21-6231-2021
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Latest update: 13 Dec 2024
Short summary
This study presents the results of an exhaustive characterization of a CRM instrument developed at Mines Douai to measure total OH reactivity in the troposphere. To do so, a suite of laboratory experiments was conducted to assess the different corrections that need to be applied during data processing. The results were then compared to simulations from a 0-D box model, including two different chemical mechanisms, leading to reasonable agreement.
This study presents the results of an exhaustive characterization of a CRM instrument developed...
