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Volume 10, issue 6
Atmos. Meas. Tech., 10, 2283–2298, 2017
https://doi.org/10.5194/amt-10-2283-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Meas. Tech., 10, 2283–2298, 2017
https://doi.org/10.5194/amt-10-2283-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 22 Jun 2017

Research article | 22 Jun 2017

Controlled nitric oxide production via O(1D)  + N2O reactions for use in oxidation flow reactor studies

Andrew Lambe et al.

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Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
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Peer review completion

AR: Author's response | RR: Referee report | ED: Editor decision
AR by Andrew Lambe on behalf of the Authors (20 Apr 2017)  Author's response    Manuscript
ED: Referee Nomination & Report Request started (01 May 2017) by Thomas F. Hanisco
RR by Anonymous Referee #2 (08 May 2017)
ED: Publish subject to minor revisions (Editor review) (09 May 2017) by Thomas F. Hanisco
AR by Andrew Lambe on behalf of the Authors (11 May 2017)  Author's response    Manuscript
ED: Publish as is (23 May 2017) by Thomas F. Hanisco
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Short summary
This work enables the study of NOx-influenced secondary organic aerosol formation chemistry in oxidation flow reactors to an extent that was not previously possible. The method uses reactions of exited oxygen O(1D) radicals (formed from ozone photolysis at 254 nm or nitrous oxide photolysis at 185 nm) with nitrous oxide (N2O) to produce NO. We demonstrate proof of concept using chemical ionization mass spectrometer measurements to detect gas-phase oxidation products of isoprene and α-pinene.
This work enables the study of NOx-influenced secondary organic aerosol formation chemistry in...
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