Articles | Volume 10, issue 6
https://doi.org/10.5194/amt-10-2283-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-10-2283-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
22 Jun 2017
Research article |
| 22 Jun 2017
Controlled nitric oxide production via O(1D) + N2O reactions for use in oxidation flow reactor studies
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Chemistry Department, Boston College, Chestnut Hill, Massachusetts, USA
Paola Massoli
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Xuan Zhang
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Current address: Atmospheric Chemistry Observations & Modeling Laboratory, National Center for Atmospheric Research, Boulder, Colorado, USA
Manjula Canagaratna
Aerodyne Research, Inc., Billerica, Massachusetts, USA
John Nowak
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Current address: Chemistry and Dynamics Branch, NASA Langley Research Center, Hampton, Virginia, USA
Conner Daube
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Physics Department, University of Helsinki, Helsinki, Finland
Wei Nie
Joint International Research Laboratory of Atmospheric and Earth System Sciences, School of Atmospheric Sciences, Nanjing University, Nanjing, China
Physics Department, University of Helsinki, Helsinki, Finland
Timothy Onasch
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Chemistry Department, Boston College, Chestnut Hill, Massachusetts, USA
John Jayne
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Charles Kolb
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Paul Davidovits
Chemistry Department, Boston College, Chestnut Hill, Massachusetts, USA
Douglas Worsnop
Aerodyne Research, Inc., Billerica, Massachusetts, USA
Physics Department, University of Helsinki, Helsinki, Finland
Department of Meteorology and Atmospheric Sciences, The Pennsylvania State University, University Park, Pennsylvania, USA
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- Secondary Organic Aerosol Formation of Fleet Vehicle Emissions in China: Potential Seasonality of Spatial Distributions K. Liao et al. 10.1021/acs.est.0c08591
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- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
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- Molecular characterization of alkyl nitrates in atmospheric aerosols by ion mobility mass spectrometry X. Zhang et al. 10.5194/amt-12-5535-2019
- Evolution of Atmospheric Total Organic Carbon from Petrochemical Mixtures K. Li et al. 10.1021/acs.est.1c02620
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- Molecular Analysis of Secondary Brown Carbon Produced from the Photooxidation of Naphthalene K. Siemens et al. 10.1021/acs.est.1c03135
- Insights Into Formation and Aging of Secondary Organic Aerosol From Oxidation Flow Reactors: A Review Z. Zhang et al. 10.1007/s40726-024-00309-7
- Evaluation of the chemical composition of gas- and particle-phase products of aromatic oxidation A. Mehra et al. 10.5194/acp-20-9783-2020
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- Can we achieve atmospheric chemical environments in the laboratory? An integrated model-measurement approach to chamber SOA studies H. Kenagy et al. 10.1126/sciadv.ado1482
- Model Evaluation of New Techniques for Maintaining High-NO Conditions in Oxidation Flow Reactors for the Study of OH-Initiated Atmospheric Chemistry Z. Peng et al. 10.1021/acsearthspacechem.7b00070
- Molecular characterization of oxidized organic nitrogen in the polluted urban atmosphere of Beijing L. Liu et al. 10.1016/j.scitotenv.2024.177109
45 citations as recorded by crossref.
- Evolution of the Complex Refractive Index of Secondary Organic Aerosols during Atmospheric Aging Q. He et al. 10.1021/acs.est.7b05742
- Oxygenated organic molecules produced by low-NOx photooxidation of aromatic compounds: contributions to secondary organic aerosol and steric hindrance X. Cheng et al. 10.5194/acp-24-2099-2024
- Nitrate radical generation via continuous generation of dinitrogen pentoxide in a laminar flow reactor coupled to an oxidation flow reactor A. Lambe et al. 10.5194/amt-13-2397-2020
- Connecting the Oxidative Potential of Secondary Organic Aerosols with Reactive Oxygen Species in Exposed Lung Cells P. Chowdhury et al. 10.1021/acs.est.9b04449
- Modeling of the chemistry in oxidation flow reactors with high initial NO Z. Peng & J. Jimenez 10.5194/acp-17-11991-2017
- Gas-phase composition and secondary organic aerosol formation from standard and particle filter-retrofitted gasoline direct injection vehicles investigated in a batch and flow reactor S. Pieber et al. 10.5194/acp-18-9929-2018
- Oxidized organic molecules in the tropical free troposphere over Amazonia Q. Zha et al. 10.1093/nsr/nwad138
- A steady-state continuous flow chamber for the study of daytime and nighttime chemistry under atmospherically relevant NO levels X. Zhang et al. 10.5194/amt-11-2537-2018
- Characterization of products formed from the oxidation of toluene and m-xylene with varying NOx and OH exposure D. Srivastava et al. 10.1016/j.chemosphere.2023.139002
- Oxygenated products formed from OH-initiated reactions of trimethylbenzene: autoxidation and accretion Y. Wang et al. 10.5194/acp-20-9563-2020
- Secondary Organic Aerosol Formation from the Photooxidation of Aromatic Ketone Intermediate Volatile Organic Compounds C. Liang et al. 10.1021/acs.est.4c05384
- Optical Properties of Secondary Organic Aerosol Produced by Photooxidation of Naphthalene under NOx Condition Q. He et al. 10.1021/acs.est.1c07328
- Secondary Organic Aerosol Formation of Fleet Vehicle Emissions in China: Potential Seasonality of Spatial Distributions K. Liao et al. 10.1021/acs.est.0c08591
- A large contribution of anthropogenic organo-nitrates to secondary organic aerosol in the Alberta oil sands A. Lee et al. 10.5194/acp-19-12209-2019
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Computational Comparison of Different Reagent Ions in the Chemical Ionization of Oxidized Multifunctional Compounds N. Hyttinen et al. 10.1021/acs.jpca.7b10015
- Assessing the degree of plug flow in oxidation flow reactors (OFRs): a study on a potential aerosol mass (PAM) reactor D. Mitroo et al. 10.5194/amt-11-1741-2018
- Secondary organic aerosol formation from <i>α</i>-pinene, alkanes, and oil-sands-related precursors in a new oxidation flow reactor K. Li et al. 10.5194/acp-19-9715-2019
- The Chemical Characteristics and Formation of Potential Secondary Aerosol (PSA) using an Oxidation Flow Reactor (OFR) in the Summer: Focus on the Residential Area, Suwon G. Park et al. 10.5572/KOSAE.2019.35.6.786
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Constraining nucleation, condensation, and chemistry in oxidation flow reactors using size-distribution measurements and aerosol microphysical modeling A. Hodshire et al. 10.5194/acp-18-12433-2018
- Secondary organic aerosols from OH oxidation of cyclic volatile methyl siloxanes as an important Si source in the atmosphere C. Han et al. 10.5194/acp-22-10827-2022
- Dynamic changes in optical and chemical properties of tar ball aerosols by atmospheric photochemical aging C. Li et al. 10.5194/acp-19-139-2019
- Highly oxygenated organic molecules produced by the oxidation of benzene and toluene in a wide range of OH exposure and NO<sub><i>x</i></sub> conditions X. Cheng et al. 10.5194/acp-21-12005-2021
- HOx and NOx production in oxidation flow reactors via photolysis of isopropyl nitrite, isopropyl nitrite-d7, and 1,3-propyl dinitrite at λ = 254, 350, and 369 nm A. Lambe et al. 10.5194/amt-12-299-2019
- Molecular characterization of alkyl nitrates in atmospheric aerosols by ion mobility mass spectrometry X. Zhang et al. 10.5194/amt-12-5535-2019
- Evolution of Atmospheric Total Organic Carbon from Petrochemical Mixtures K. Li et al. 10.1021/acs.est.1c02620
- Oligomer and highly oxygenated organic molecule formation from oxidation of oxygenated monoterpenes emitted by California sage plants A. Mehra et al. 10.5194/acp-20-10953-2020
- Theoretical Investigations on the Possibility of Prebiotic HCN Formation via O-Addition Reactions S. Ghoshal et al. 10.1021/acs.jpca.0c02538
- Formation of condensable organic vapors from anthropogenic and biogenic volatile organic compounds (VOCs) is strongly perturbed by NO<sub><i>x</i></sub> in eastern China Y. Liu et al. 10.5194/acp-21-14789-2021
- Reactive Uptake of Isoprene Epoxydiols Increases the Viscosity of the Core of Phase-Separated Aerosol Particles N. Olson et al. 10.1021/acsearthspacechem.9b00138
- Characterization of anthropogenic organic aerosols by TOF-ACSM with the new capture vaporizer Y. Zheng et al. 10.5194/amt-13-2457-2020
- Secondary reactions of aromatics-derived oxygenated organic molecules lead to plentiful highly oxygenated organic molecules within an intraday OH exposure Y. Wang et al. 10.5194/acp-24-7961-2024
- Organic peroxy radical chemistry in oxidation flow reactors and environmental chambers and their atmospheric relevance Z. Peng et al. 10.5194/acp-19-813-2019
- Isothermal evaporation of α-pinene secondary organic aerosol particles formed under low NOx and high NOx conditions Z. Li et al. 10.5194/acp-23-203-2023
- Ambient Measurements of Highly Oxidized Gas-Phase Molecules during the Southern Oxidant and Aerosol Study (SOAS) 2013 P. Massoli et al. 10.1021/acsearthspacechem.8b00028
- Oxidation Flow Reactor Results in a Chinese Megacity Emphasize the Important Contribution of S/IVOCs to Ambient SOA Formation W. Hu et al. 10.1021/acs.est.1c03155
- Molecular Analysis of Secondary Brown Carbon Produced from the Photooxidation of Naphthalene K. Siemens et al. 10.1021/acs.est.1c03135
- Insights Into Formation and Aging of Secondary Organic Aerosol From Oxidation Flow Reactors: A Review Z. Zhang et al. 10.1007/s40726-024-00309-7
- Evaluation of the chemical composition of gas- and particle-phase products of aromatic oxidation A. Mehra et al. 10.5194/acp-20-9783-2020
- Correcting micro-aethalometer absorption measurements for brown carbon aerosol C. Li et al. 10.1016/j.scitotenv.2021.146143
- Light absorption and scattering properties of indole secondary organic aerosol prepared under various oxidant and relative humidity conditions V. Baboomian et al. 10.1080/02786826.2023.2193235
- Can we achieve atmospheric chemical environments in the laboratory? An integrated model-measurement approach to chamber SOA studies H. Kenagy et al. 10.1126/sciadv.ado1482
- Model Evaluation of New Techniques for Maintaining High-NO Conditions in Oxidation Flow Reactors for the Study of OH-Initiated Atmospheric Chemistry Z. Peng et al. 10.1021/acsearthspacechem.7b00070
- Molecular characterization of oxidized organic nitrogen in the polluted urban atmosphere of Beijing L. Liu et al. 10.1016/j.scitotenv.2024.177109
Latest update: 20 Nov 2024
Short summary
This work enables the study of NOx-influenced secondary organic aerosol formation chemistry in oxidation flow reactors to an extent that was not previously possible. The method uses reactions of exited oxygen O(1D) radicals (formed from ozone photolysis at 254 nm or nitrous oxide photolysis at 185 nm) with nitrous oxide (N2O) to produce NO. We demonstrate proof of concept using chemical ionization mass spectrometer measurements to detect gas-phase oxidation products of isoprene and α -pinene.
This work enables the study of NOx-influenced secondary organic aerosol formation chemistry in...
