Articles | Volume 12, issue 4
https://doi.org/10.5194/amt-12-2287-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-12-2287-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Apr 2019
Research article |
| 12 Apr 2019
| 12 Apr 2019
Analysis of functional groups in atmospheric aerosols by infrared spectroscopy: systematic intercomparison of calibration methods for US measurement network samples
Matteo Reggente
ENAC/IIE Swiss Federal Institute of Technology Lausanne (EPFL), Lausanne, Switzerland
Ann M. Dillner
Air Quality Research Center, University of California Davis, Davis, CA 95616, USA
Satoshi Takahama
CORRESPONDING AUTHOR
ENAC/IIE Swiss Federal Institute of Technology Lausanne (EPFL), Lausanne, Switzerland
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Cited
18 citations as recorded by crossref.
- Infrared Ion Spectroscopy of Environmental Organic Mixtures: Probing the Composition of α-Pinene Secondary Organic Aerosol E. Walhout et al. 10.1021/acs.est.9b02077
- Comparison of methods of functional group analysis using results from laboratory and field aerosol measurements M. Claflin et al. 10.1080/02786826.2021.1918325
- Characterization of the organic functional group composition and sources of summertime aerosols in an eastern city of China K. Xia et al. 10.1016/j.atmosenv.2022.119078
- Variation in oxidative potential of fine particulate matter and its association with chemical constituents at a regional site in India S. Dubey et al. 10.1016/j.scitotenv.2024.176159
- Characterization of primary and aged wood burning and coal combustion organic aerosols in an environmental chamber and its implications for atmospheric aerosols A. Yazdani et al. 10.5194/acp-21-10273-2021
- Continuous observations from horizontally pointing lidar, weather parameters and PM2.5: a pre-deployment assessment for monitoring radioactive dust in Fukushima, Japan N. Lagrosas et al. 10.5194/amt-16-5937-2023
- Quantifying organic matter and functional groups in particulate matter filter samples from the southeastern United States – Part 2: Spatiotemporal trends A. Boris et al. 10.5194/amt-14-4355-2021
- Quantifying functional group compositions of household fuel-burning emissions E. Li et al. 10.5194/amt-17-2401-2024
- Quantification of major particulate matter species from a single filter type using infrared spectroscopy – application to a large-scale monitoring network B. Debus et al. 10.5194/amt-15-2685-2022
- An open platform for Aerosol InfraRed Spectroscopy analysis – AIRSpec M. Reggente et al. 10.5194/amt-12-2313-2019
- Secondary organic aerosol association with cardiorespiratory disease mortality in the United States H. Pye et al. 10.1038/s41467-021-27484-1
- Fragment ion–functional group relationships in organic aerosols using aerosol mass spectrometry and mid-infrared spectroscopy A. Yazdani et al. 10.5194/amt-15-2857-2022
- Organic acid evaporation kinetics from aqueous aerosols: implications for aerosol buffering capacity in the atmosphere K. Angle et al. 10.1039/D2EA00092J
- Analysis of functional groups in atmospheric aerosols by infrared spectroscopy: method development for probabilistic modeling of organic carbon and organic matter concentrations C. Bürki et al. 10.5194/amt-13-1517-2020
- Aging of atmospheric aerosols and the role of iron in catalyzing brown carbon formation H. Al-Abadleh 10.1039/D1EA00038A
- Chemical evolution of primary and secondary biomass burning aerosols during daytime and nighttime A. Yazdani et al. 10.5194/acp-23-7461-2023
- Quantifying organic matter and functional groups in particulate matter filter samples from the southeastern United States – Part 1: Methods A. Boris et al. 10.5194/amt-12-5391-2019
- Effects of Organic Matrices on Nucleophilic Aqueous Aerosol Chemistry: Yields and Mechanistic Insight for Brown Carbon Formation from Glyoxal and Ammonia G. Drozd et al. 10.1021/acsearthspacechem.2c00068
17 citations as recorded by crossref.
- Infrared Ion Spectroscopy of Environmental Organic Mixtures: Probing the Composition of α-Pinene Secondary Organic Aerosol E. Walhout et al. 10.1021/acs.est.9b02077
- Comparison of methods of functional group analysis using results from laboratory and field aerosol measurements M. Claflin et al. 10.1080/02786826.2021.1918325
- Characterization of the organic functional group composition and sources of summertime aerosols in an eastern city of China K. Xia et al. 10.1016/j.atmosenv.2022.119078
- Variation in oxidative potential of fine particulate matter and its association with chemical constituents at a regional site in India S. Dubey et al. 10.1016/j.scitotenv.2024.176159
- Characterization of primary and aged wood burning and coal combustion organic aerosols in an environmental chamber and its implications for atmospheric aerosols A. Yazdani et al. 10.5194/acp-21-10273-2021
- Continuous observations from horizontally pointing lidar, weather parameters and PM2.5: a pre-deployment assessment for monitoring radioactive dust in Fukushima, Japan N. Lagrosas et al. 10.5194/amt-16-5937-2023
- Quantifying organic matter and functional groups in particulate matter filter samples from the southeastern United States – Part 2: Spatiotemporal trends A. Boris et al. 10.5194/amt-14-4355-2021
- Quantifying functional group compositions of household fuel-burning emissions E. Li et al. 10.5194/amt-17-2401-2024
- Quantification of major particulate matter species from a single filter type using infrared spectroscopy – application to a large-scale monitoring network B. Debus et al. 10.5194/amt-15-2685-2022
- An open platform for Aerosol InfraRed Spectroscopy analysis – AIRSpec M. Reggente et al. 10.5194/amt-12-2313-2019
- Secondary organic aerosol association with cardiorespiratory disease mortality in the United States H. Pye et al. 10.1038/s41467-021-27484-1
- Fragment ion–functional group relationships in organic aerosols using aerosol mass spectrometry and mid-infrared spectroscopy A. Yazdani et al. 10.5194/amt-15-2857-2022
- Organic acid evaporation kinetics from aqueous aerosols: implications for aerosol buffering capacity in the atmosphere K. Angle et al. 10.1039/D2EA00092J
- Analysis of functional groups in atmospheric aerosols by infrared spectroscopy: method development for probabilistic modeling of organic carbon and organic matter concentrations C. Bürki et al. 10.5194/amt-13-1517-2020
- Aging of atmospheric aerosols and the role of iron in catalyzing brown carbon formation H. Al-Abadleh 10.1039/D1EA00038A
- Chemical evolution of primary and secondary biomass burning aerosols during daytime and nighttime A. Yazdani et al. 10.5194/acp-23-7461-2023
- Quantifying organic matter and functional groups in particulate matter filter samples from the southeastern United States – Part 1: Methods A. Boris et al. 10.5194/amt-12-5391-2019
Latest update: 20 Nov 2024
Short summary
We compare state-of-the-art models for predicting functional group composition in atmospheric particulate matter across urban and rural samples collected in a US monitoring network. While trends across models are consistent, absolute abundances can be sensitive to selection of calibration standards, spectral processing procedures, and calibration algorithms. Recommendations for further method development for reducing uncertainties are outlined.
We compare state-of-the-art models for predicting functional group composition in atmospheric...
