Articles | Volume 13, issue 9
Atmos. Meas. Tech., 13, 4973–4994, 2020
https://doi.org/10.5194/amt-13-4973-2020
Atmos. Meas. Tech., 13, 4973–4994, 2020
https://doi.org/10.5194/amt-13-4973-2020

Research article 23 Sep 2020

Research article | 23 Sep 2020

Multi-year ACSM measurements at the central European research station Melpitz (Germany) – Part 1: Instrument robustness, quality assurance, and impact of upper size cutoff diameter

Laurent Poulain et al.

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Cited articles

Aiken, A. C., DeCarlo, P. F., and Jimenez, J. L.: Elemental analysis of organic species with electron ionization high-resolution mass spectrometry, Anal. Chem., 79, 8350–8358, https://doi.org/10.1021/ac071150w, 2007. 
Allan, J. D., Delia, A. E., Coe, H., Bower, K. N., Alfarra, R. M., Jimenez, J. L., Middlebrook, A. M., Drewnick, F., Onasch, T. B., Canagaratna, M. R., Jayne, J. T., and Worsnop, D. R.: A generalised method for the extraction of chemically resolved mass spectra from Aerodyne aerosol mass spectrometer data, J. Aerosol Sci., 35, 909–922, https://doi.org/10.1016/j.jaerosci.2004.02.007, 2004. 
Allan, J. D., Alfarra, R. M., Bower, K. N., Williams, P. I., Gallagher, M. W., Jimenez, J. L., McDonald, A. G., Nemitz, E., Canagaratna, M. R., Jayne, J. T., Coe, H., and Worsnop, D. R.: Quantitative sampling using an Aerodyne aerosol mass spectrometer 2. Measurements of fine particulate chemical composition in two U.K. cities, J. Geophys. Res., 108, 4091, https://doi.org/10.1029/2002JD002358, 2003. 
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Short summary
The stability and the comparability between ACSM and collocated filter sampling and MPSS measurements was investigated in order to examine the instruments robustness for year-long measurements. Specific attention was paid to the influence of the upper size cutoff diameter to better understand how it might affect the data validation. Recommendations are provided for better on-site quality assurance and quality control of the ACSM, which would be useful for either long-term or intensive campaigns.