Articles | Volume 13, issue 11
https://doi.org/10.5194/amt-13-6325-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-13-6325-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
An interlaboratory comparison of aerosol inorganic ion measurements by ion chromatography: implications for aerosol pH estimate
Jingsha Xu
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Shaojie Song
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA
Roy M. Harrison
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Department of Environmental Sciences/Center of Excellence in Environmental Studies, King Abdulaziz University, P.O. Box 80203, Jeddah, 21589, Saudi Arabia
Congbo Song
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Lianfang Wei
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China
Qiang Zhang
Institute of Surface-Earth System Science, Tianjin University, Tianjin, 300072, China
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China
Lu Lei
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China
Chao Zhang
Key Laboratory of Marine Environment and Ecology, Ministry of Education of China, and Frontiers Science Center for Deep Ocean Multispheres and Earth System, Ocean University of China, Qingdao 266100, China
Xiaohong Yao
Key Laboratory of Marine Environment and Ecology, Ministry of Education of China, and Frontiers Science Center for Deep Ocean Multispheres and Earth System, Ocean University of China, Qingdao 266100, China
Laboratory for Marine Ecology and Environmental Sciences, Qingdao National Laboratory for Marine Science and Technology, Qingdao, 266071, China
Dihui Chen
Key Laboratory of Marine Environment and Ecology, Ministry of Education of China, and Frontiers Science Center for Deep Ocean Multispheres and Earth System, Ocean University of China, Qingdao 266100, China
Weijun Li
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, 310027, China
Miaomiao Wu
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, 310027, China
Hezhong Tian
State Key Laboratory of Environmental Simulation and Pollution Control & Center for Atmospheric Environmental Studies, School of Environment, Beijing Normal University, Beijing 100875, China
Lining Luo
State Key Laboratory of Environmental Simulation and Pollution Control & Center for Atmospheric Environmental Studies, School of Environment, Beijing Normal University, Beijing 100875, China
Shengrui Tong
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China
Weiran Li
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China
Junling Wang
School of Environment, Tsinghua University, Beijing, 100084, China
Guoliang Shi
State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, Centre of Urban Transport Emission Research, College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China
Yanqi Huangfu
State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, Centre of Urban Transport Emission Research, College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China
Yingze Tian
State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, Centre of Urban Transport Emission Research, College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China
Baozhu Ge
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China
Shaoli Su
Research Center for Atmospheric Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing, 400714, China
Chao Peng
Research Center for Atmospheric Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing, 400714, China
Yang Chen
Research Center for Atmospheric Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing, 400714, China
Fumo Yang
Department of Environmental Science and Engineering, Sichuan University, Chengdu, 610065, China
Aleksandra Mihajlidi-Zelić
Centre of Excellence in Environmental Chemistry and Engineering – ICTM, University of Belgrade, Njegoševa 12 (Studentski trg 14–16), Belgrade, Serbia
Dragana Đorđević
Centre of Excellence in Environmental Chemistry and Engineering – ICTM, University of Belgrade, Njegoševa 12 (Studentski trg 14–16), Belgrade, Serbia
Stefan J. Swift
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UK
Imogen Andrews
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UK
Jacqueline F. Hamilton
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UK
Ye Sun
School of Space and Environment, Beihang University, Beijing, 100191, China
Agung Kramawijaya
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Jinxiu Han
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Supattarachai Saksakulkrai
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Clarissa Baldo
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Siqi Hou
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Feixue Zheng
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Kaspar R. Daellenbach
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Yongchun Liu
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Markku Kulmala
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Pingqing Fu
Institute of Surface-Earth System Science, Tianjin University, Tianjin, 300072, China
School of Geography Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
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- Final revised paper (published on 25 Nov 2020)
- Supplement to the final revised paper
- Preprint (discussion started on 04 May 2020)
Interactive discussion
Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
- Printer-friendly version
- Supplement
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RC1: 'Referee Report', Anonymous Referee #1, 19 May 2020
- AC2: 'point-by-point response', Jingsha Xu, 21 Aug 2020
- AC1: 'supplemental information', Jingsha Xu, 20 May 2020
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RC2: 'Comments on amt-2020-156', Anonymous Referee #2, 07 Jun 2020
- AC3: 'point-by-point response', Jingsha Xu, 21 Aug 2020
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RC3: 'Comments on amt-2020-156', Anonymous Referee #3, 24 Jun 2020
- AC4: 'point-by-point response', Jingsha Xu, 21 Aug 2020
Peer-review completion
AR: Author's response | RR: Referee report | ED: Editor decision
AR by Jingsha Xu on behalf of the Authors (26 Aug 2020)
Manuscript
ED: Referee Nomination & Report Request started (29 Aug 2020) by Mingjin Tang
RR by Anonymous Referee #3 (04 Sep 2020)
RR by Anonymous Referee #2 (12 Sep 2020)
ED: Publish subject to minor revisions (review by editor) (12 Sep 2020) by Mingjin Tang
AR by Jingsha Xu on behalf of the Authors (16 Sep 2020)
Author's response
Manuscript
ED: Publish as is (24 Sep 2020) by Mingjin Tang
AR by Jingsha Xu on behalf of the Authors (01 Oct 2020)
Manuscript
Short summary
An interlaboratory comparison was conducted for the first time to examine differences in water-soluble inorganic ions (WSIIs) measured by 10 labs using ion chromatography (IC) and by two online aerosol chemical speciation monitor (ACSM) methods. Major ions including SO42−, NO3− and NH4+ agreed well in 10 IC labs and correlated well with ACSM data. WSII interlab variability strongly affected aerosol acidity results based on ion balance, but aerosol pH computed by ISORROPIA II was very similar.
An interlaboratory comparison was conducted for the first time to examine differences in...