Articles | Volume 14, issue 3
https://doi.org/10.5194/amt-14-2237-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-14-2237-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Mar 2021
Research article |
| 23 Mar 2021
| 23 Mar 2021
Aerosol pH indicator and organosulfate detectability from aerosol mass spectrometry measurements
Melinda K. Schueneman
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Benjamin A. Nault
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
now at: Aerodyne Research, Inc., Billerica, MA, USA
Pedro Campuzano-Jost
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Duseong S. Jo
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Atmospheric Chemistry Observations and Modeling, National Center for Atmospheric Research, Boulder, CO 80301, USA
Douglas A. Day
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Jason C. Schroder
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
now at: Air Pollution Control Division, Colorado Department of Public Health and the Environment, Denver, CO, USA
Brett B. Palm
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Alma Hodzic
Atmospheric Chemistry Observations and Modeling, National Center for Atmospheric Research, Boulder, CO 80301, USA
Jack E. Dibb
Earth Systems Research Center, Institute for the Study of Earth, Oceans, and Space, University of New Hampshire, Durham, NH, USA
Jose L. Jimenez
CORRESPONDING AUTHOR
Department of Chemistry, and Cooperative Institute for Research in
Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
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Cited
14 citations as recorded by crossref.
- Modeling Indoor Inorganic Aerosol Concentrations During the ATHLETIC Campaign with IMAGES B. Berman et al. 10.1021/acsestair.4c00060
- Emission factors and evolution of SO2measured from biomass burning in wildfires and agricultural fires P. Rickly et al. 10.5194/acp-22-15603-2022
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Marine Submicron Aerosols from the Gulf of Mexico: Polluted and Acidic with Rapid Production of Sulfate and Organosulfates S. Zhou et al. 10.1021/acs.est.2c05469
- Contributions of Cleaning Solution Residues to Indoor Organic Surface Films R. O’Brien et al. 10.1021/acsestair.3c00053
- Quinaldine Red as a Fluorescent Probe for Particle Physicochemical Properties E. Rainone et al. 10.1021/acsearthspacechem.3c00286
- Trace H2S Promotes Organic Aerosol Production and Organosulfur Compound Formation in Archean Analog Haze Photochemistry Experiments N. Reed et al. 10.1029/2021GL097032
- Chemical transport models often underestimate inorganic aerosol acidity in remote regions of the atmosphere B. Nault et al. 10.1038/s43247-021-00164-0
- The Role of Indoor Surface pH in Controlling the Fate of Acids and Bases in an Unoccupied Residence J. Ditto et al. 10.1021/acsestair.4c00044
- Probing Atmospheric Aerosols by Multimodal Mass Spectrometry Techniques: Revealing Aging Characteristics of Its Individual Molecular Components K. Siemens et al. 10.1021/acsearthspacechem.3c00228
- Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations H. Bian et al. 10.5194/acp-24-1717-2024
- High-resolution physicochemical dataset of atmospheric aerosols over the Tibetan Plateau and its surroundings J. Xu et al. 10.5194/essd-16-1875-2024
- Probing the pH dependence of brown carbon formation: Insights from laboratory studies on aerosol particles and bulk phase solutions K. Jansen & M. Tolbert 10.1080/02786826.2023.2267649
- The importance of hydroxymethanesulfonate (HMS) in winter haze episodes in North China Plain C. Chen et al. 10.1016/j.envres.2022.113093
14 citations as recorded by crossref.
- Modeling Indoor Inorganic Aerosol Concentrations During the ATHLETIC Campaign with IMAGES B. Berman et al. 10.1021/acsestair.4c00060
- Emission factors and evolution of SO2measured from biomass burning in wildfires and agricultural fires P. Rickly et al. 10.5194/acp-22-15603-2022
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Marine Submicron Aerosols from the Gulf of Mexico: Polluted and Acidic with Rapid Production of Sulfate and Organosulfates S. Zhou et al. 10.1021/acs.est.2c05469
- Contributions of Cleaning Solution Residues to Indoor Organic Surface Films R. O’Brien et al. 10.1021/acsestair.3c00053
- Quinaldine Red as a Fluorescent Probe for Particle Physicochemical Properties E. Rainone et al. 10.1021/acsearthspacechem.3c00286
- Trace H2S Promotes Organic Aerosol Production and Organosulfur Compound Formation in Archean Analog Haze Photochemistry Experiments N. Reed et al. 10.1029/2021GL097032
- Chemical transport models often underestimate inorganic aerosol acidity in remote regions of the atmosphere B. Nault et al. 10.1038/s43247-021-00164-0
- The Role of Indoor Surface pH in Controlling the Fate of Acids and Bases in an Unoccupied Residence J. Ditto et al. 10.1021/acsestair.4c00044
- Probing Atmospheric Aerosols by Multimodal Mass Spectrometry Techniques: Revealing Aging Characteristics of Its Individual Molecular Components K. Siemens et al. 10.1021/acsearthspacechem.3c00228
- Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations H. Bian et al. 10.5194/acp-24-1717-2024
- High-resolution physicochemical dataset of atmospheric aerosols over the Tibetan Plateau and its surroundings J. Xu et al. 10.5194/essd-16-1875-2024
- Probing the pH dependence of brown carbon formation: Insights from laboratory studies on aerosol particles and bulk phase solutions K. Jansen & M. Tolbert 10.1080/02786826.2023.2267649
- The importance of hydroxymethanesulfonate (HMS) in winter haze episodes in North China Plain C. Chen et al. 10.1016/j.envres.2022.113093
Latest update: 06 Jan 2025
Short summary
This work focuses on two important properties of the aerosol, acidity, and sulfate composition, which is important for our understanding of aerosol health and environmental impacts. We explore different methods to understand the composition of the aerosol with measurements from a specific instrument and apply those methods to a large dataset. These measurements are confounded by other factors, making it challenging to predict aerosol sulfate composition; pH estimations, however, show promise.
This work focuses on two important properties of the aerosol, acidity, and sulfate composition,...
