Articles | Volume 16, issue 17
https://doi.org/10.5194/amt-16-4115-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-16-4115-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Sep 2023
Research article |
| 12 Sep 2023
| 12 Sep 2023
Detection and analysis of Lhù'ààn Mân' (Kluane Lake) dust plumes using passive and active ground-based remote sensing supported by physical surface measurements
Seyed Ali Sayedain
CORRESPONDING AUTHOR
Centre d'Applications et de Recherches en Télédétection, Université de Sherbrooke, Sherbrooke, Canada
Norman T. O'Neill
Centre d'Applications et de Recherches en Télédétection, Université de Sherbrooke, Sherbrooke, Canada
James King
Département de géographie, Université de Montréal, Montréal, Canada
Patrick L. Hayes
Département de chimie, Université de Montréal, Montréal, Canada
Daniel Bellamy
Département de géographie, Université de Montréal, Montréal, Canada
Richard Washington
Department of Geography, University of Oxford, Oxford, United Kingdom
Sebastian Engelstaedter
Department of Geography, University of Oxford, Oxford, United Kingdom
Andy Vicente-Luis
Département de chimie, Université de Montréal, Montréal, Canada
Jill Bachelder
Département de chimie, Université de Montréal, Montréal, Canada
Malo Bernhard
Département de chimie, Université de Montréal, Montréal, Canada
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Norman T. O’Neill, Keyvan Ranjbar, Liviu Ivănescu, Yann Blanchard, Seyed Ali Sayedain, and Yasmin AboEl-Fetouh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1057, https://doi.org/10.5194/egusphere-2024-1057, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Dust from mid-latitude deserts or from local drainage basins is a weak component of atmospheric aerosols in the Arctic. Satellite-based dust estimates are often overestimated because dust and cloud measurements can be confused. Illustrations are given with an emphasis on the flawed claim that a classic indicator of dust (negative brightness temperature differences) is proof of the presence of airborne Arctic dust. Low altitude “warm” water plumes are the likely source of such negative values.
Norman T. O’Neill, Keyvan Ranjbar, Liviu Ivănescu, Yann Blanchard, Seyed Ali Sayedain, and Yasmin AboEl-Fetouh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1057, https://doi.org/10.5194/egusphere-2024-1057, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Dust from mid-latitude deserts or from local drainage basins is a weak component of atmospheric aerosols in the Arctic. Satellite-based dust estimates are often overestimated because dust and cloud measurements can be confused. Illustrations are given with an emphasis on the flawed claim that a classic indicator of dust (negative brightness temperature differences) is proof of the presence of airborne Arctic dust. Low altitude “warm” water plumes are the likely source of such negative values.
Nansi Fakhri, Robin Stevens, Arnold Downey, Konstantina Oikonomou, Jean Sciare, Charbel Afif, and Patrick L. Hayes
Atmos. Chem. Phys., 24, 1193–1212, https://doi.org/10.5194/acp-24-1193-2024, https://doi.org/10.5194/acp-24-1193-2024, 2024
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We investigated the chemical composition of atmospheric fine particles, their emission sources, and the potential human health risk associated with trace elements in particles for an urban site in Montréal over a 3-month period (August–November). This study represents the first time that such extensive composition measurements were included in an urban source apportionment study in Canada, and it provides greater resolution of fine-particle sources than has been previously achieved in Canada.
Liviu Ivănescu and Norman T. O'Neill
Atmos. Meas. Tech., 16, 6111–6121, https://doi.org/10.5194/amt-16-6111-2023, https://doi.org/10.5194/amt-16-6111-2023, 2023
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The starphotometers' complex infrastructure prohibits calibration campaigns. On-site calibration procedures appear as the only practical solution. A multi-star approach overcomes site-specific sky transparency stability problems. Star selection strategies were proposed for mitigating some sources of errors. Data processing strategies and instrument design improvements appear necessary.
Rosemary Huck, Robert G. Bryant, and James King
Atmos. Chem. Phys., 23, 6299–6318, https://doi.org/10.5194/acp-23-6299-2023, https://doi.org/10.5194/acp-23-6299-2023, 2023
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This study shows that mineral aerosol (dust) emission events in high-latitude areas are under-represented in both ground- and space-based detecting methods. This is done through a suite of ground-based data to prove that dust emissions from the proglacial area, Lhù’ààn Mân, occur almost daily but are not always recorded at different timescales. Dust has multiple effects on atmospheric processes; therefore, accurate quantification is important in the calibration and validation of climate models.
Norman T. O'Neill, Keyvan Ranjbar, Liviu Ivănescu, Thomas F. Eck, Jeffrey S. Reid, David M. Giles, Daniel Pérez-Ramírez, and Jai Prakash Chaubey
Atmos. Meas. Tech., 16, 1103–1120, https://doi.org/10.5194/amt-16-1103-2023, https://doi.org/10.5194/amt-16-1103-2023, 2023
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Aerosols are atmospheric particles that vary in size (radius) from a fraction of a micrometer (µm) to around 20 µm. They tend to be either smaller than 1 µm (like smoke or pollution) or larger than 1 µm (like dust or sea salt). Their optical effect (scattering and absorbing sunlight) can be divided into FM (fine-mode) and CM (coarse-mode) parts using a cutoff radius around 1 µm or a spectral (color) technique. We present and validate a theoretical link between the types of FM and CM divisions.
Outi Meinander, Pavla Dagsson-Waldhauserova, Pavel Amosov, Elena Aseyeva, Cliff Atkins, Alexander Baklanov, Clarissa Baldo, Sarah L. Barr, Barbara Barzycka, Liane G. Benning, Bojan Cvetkovic, Polina Enchilik, Denis Frolov, Santiago Gassó, Konrad Kandler, Nikolay Kasimov, Jan Kavan, James King, Tatyana Koroleva, Viktoria Krupskaya, Markku Kulmala, Monika Kusiak, Hanna K. Lappalainen, Michał Laska, Jerome Lasne, Marek Lewandowski, Bartłomiej Luks, James B. McQuaid, Beatrice Moroni, Benjamin Murray, Ottmar Möhler, Adam Nawrot, Slobodan Nickovic, Norman T. O’Neill, Goran Pejanovic, Olga Popovicheva, Keyvan Ranjbar, Manolis Romanias, Olga Samonova, Alberto Sanchez-Marroquin, Kerstin Schepanski, Ivan Semenkov, Anna Sharapova, Elena Shevnina, Zongbo Shi, Mikhail Sofiev, Frédéric Thevenet, Throstur Thorsteinsson, Mikhail Timofeev, Nsikanabasi Silas Umo, Andreas Uppstu, Darya Urupina, György Varga, Tomasz Werner, Olafur Arnalds, and Ana Vukovic Vimic
Atmos. Chem. Phys., 22, 11889–11930, https://doi.org/10.5194/acp-22-11889-2022, https://doi.org/10.5194/acp-22-11889-2022, 2022
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High-latitude dust (HLD) is a short-lived climate forcer, air pollutant, and nutrient source. Our results suggest a northern HLD belt at 50–58° N in Eurasia and 50–55° N in Canada and at >60° N in Eurasia and >58° N in Canada. Our addition to the previously identified global dust belt (GDB) provides crucially needed information on the extent of active HLD sources with both direct and indirect impacts on climate and environment in remote regions, which are often poorly understood and predicted.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Jeffrey S. Reid, Travis D. Toth, Blake Sorenson, Edward J. Hyer, James R. Campbell, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9949–9967, https://doi.org/10.5194/acp-22-9949-2022, https://doi.org/10.5194/acp-22-9949-2022, 2022
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The study provides a baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Keyvan Ranjbar, Norm T. O'Neill, and Yasmin Aboel-Fetouh
Atmos. Chem. Phys., 22, 1757–1760, https://doi.org/10.5194/acp-22-1757-2022, https://doi.org/10.5194/acp-22-1757-2022, 2022
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We argue that the illustration employed by Huang et al. (2015) to demonstrate the transport of Asian dust to the high Arctic was, in fact, largely a cloud event and that the actual impact of Asian dust was measurable but much weaker than what they proposed and had occurred a day earlier (in agreement with the transport model they had employed to predict the transport path to the high Arctic).
Liviu Ivănescu, Konstantin Baibakov, Norman T. O'Neill, Jean-Pierre Blanchet, and Karl-Heinz Schulz
Atmos. Meas. Tech., 14, 6561–6599, https://doi.org/10.5194/amt-14-6561-2021, https://doi.org/10.5194/amt-14-6561-2021, 2021
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Starphotometry seeks to provide accurate measures of nocturnal optical depth (OD). It is driven by a need to characterize aerosols and their radiative forcing effects during a very data-sparse period. A sub-0.01 OD error is required to adequately characterize key aerosol parameters. We found approaches for sufficiently mitigating errors to achieve the 0.01 standard. This renders starphotometry the equal of daytime techniques and opens the door to exploiting its distinct star-pointing advantages.
Benjamin A. Nault, Duseong S. Jo, Brian C. McDonald, Pedro Campuzano-Jost, Douglas A. Day, Weiwei Hu, Jason C. Schroder, James Allan, Donald R. Blake, Manjula R. Canagaratna, Hugh Coe, Matthew M. Coggon, Peter F. DeCarlo, Glenn S. Diskin, Rachel Dunmore, Frank Flocke, Alan Fried, Jessica B. Gilman, Georgios Gkatzelis, Jacqui F. Hamilton, Thomas F. Hanisco, Patrick L. Hayes, Daven K. Henze, Alma Hodzic, James Hopkins, Min Hu, L. Greggory Huey, B. Thomas Jobson, William C. Kuster, Alastair Lewis, Meng Li, Jin Liao, M. Omar Nawaz, Ilana B. Pollack, Jeffrey Peischl, Bernhard Rappenglück, Claire E. Reeves, Dirk Richter, James M. Roberts, Thomas B. Ryerson, Min Shao, Jacob M. Sommers, James Walega, Carsten Warneke, Petter Weibring, Glenn M. Wolfe, Dominique E. Young, Bin Yuan, Qiang Zhang, Joost A. de Gouw, and Jose L. Jimenez
Atmos. Chem. Phys., 21, 11201–11224, https://doi.org/10.5194/acp-21-11201-2021, https://doi.org/10.5194/acp-21-11201-2021, 2021
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Secondary organic aerosol (SOA) is an important aspect of poor air quality for urban regions around the world, where a large fraction of the population lives. However, there is still large uncertainty in predicting SOA in urban regions. Here, we used data from 11 urban campaigns and show that the variability in SOA production in these regions is predictable and is explained by key emissions. These results are used to estimate the premature mortality associated with SOA in urban regions.
Konstantin Baibakov, Samuel LeBlanc, Keyvan Ranjbar, Norman T. O'Neill, Mengistu Wolde, Jens Redemann, Kristina Pistone, Shao-Meng Li, John Liggio, Katherine Hayden, Tak W. Chan, Michael J. Wheeler, Leonid Nichman, Connor Flynn, and Roy Johnson
Atmos. Chem. Phys., 21, 10671–10687, https://doi.org/10.5194/acp-21-10671-2021, https://doi.org/10.5194/acp-21-10671-2021, 2021
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We find that the airborne measurements of the vertical extinction due to aerosols (aerosol optical depth, AOD) obtained in the Athabasca Oil Sands Region (AOSR) can significantly exceed ground-based values. This can have an effect on estimating the AOSR radiative impact and is relevant to satellite validation based on ground-based measurements. We also show that the AOD can marginally increase as the plumes are being transported away from the source and the new particles are being formed.
Phillipe Gauvin-Bourdon, James King, and Liliana Perez
Earth Surf. Dynam., 9, 29–45, https://doi.org/10.5194/esurf-9-29-2021, https://doi.org/10.5194/esurf-9-29-2021, 2021
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Arid ecosystem health is a complex interaction between vegetation and climate. Coupled with impacts from grazing, it can result in quick changes in vegetation cover. We present a wind erosion and vegetation health model with active grazers over 100-year tests to find the limits of arid environments for different levels of vegetation, rainfall, wind speed, and grazing. The model shows the resilience of grass landscapes to grazing and its role as an improved tool for managing arid landscapes.
Bing Pu, Paul Ginoux, Huan Guo, N. Christina Hsu, John Kimball, Beatrice Marticorena, Sergey Malyshev, Vaishali Naik, Norman T. O'Neill, Carlos Pérez García-Pando, Juliette Paireau, Joseph M. Prospero, Elena Shevliakova, and Ming Zhao
Atmos. Chem. Phys., 20, 55–81, https://doi.org/10.5194/acp-20-55-2020, https://doi.org/10.5194/acp-20-55-2020, 2020
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Dust emission initiates when surface wind velocities exceed a threshold depending on soil and surface characteristics and varying spatially and temporally. Climate models widely use wind erosion thresholds. The climatological monthly global distribution of the wind erosion threshold, Vthreshold, is retrieved using satellite and reanalysis products and improves the simulation of dust frequency, magnitude, and the seasonal cycle in the Geophysical Fluid Dynamics Laboratory land–atmosphere model.
Samantha Tremblay, Jean-Christophe Picard, Jill O. Bachelder, Erik Lutsch, Kimberly Strong, Pierre Fogal, W. Richard Leaitch, Sangeeta Sharma, Felicia Kolonjari, Christopher J. Cox, Rachel Y.-W. Chang, and Patrick L. Hayes
Atmos. Chem. Phys., 19, 5589–5604, https://doi.org/10.5194/acp-19-5589-2019, https://doi.org/10.5194/acp-19-5589-2019, 2019
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Atmospheric aerosols, tiny airborne particles, have an important impact on climate. However, a lack of understanding of the chemistry of aerosols is one of the largest contributors to uncertainty in predictions of climate change. Measurements of aerosols were carried out in the Arctic at Eureka Station, Canada, to better understand what role aerosols play in this fragile environment. It is found that organic aerosols, possibly originating from marine emissions, are ubiquitous during summertime.
Betty Croft, Randall V. Martin, W. Richard Leaitch, Julia Burkart, Rachel Y.-W. Chang, Douglas B. Collins, Patrick L. Hayes, Anna L. Hodshire, Lin Huang, John K. Kodros, Alexander Moravek, Emma L. Mungall, Jennifer G. Murphy, Sangeeta Sharma, Samantha Tremblay, Gregory R. Wentworth, Megan D. Willis, Jonathan P. D. Abbatt, and Jeffrey R. Pierce
Atmos. Chem. Phys., 19, 2787–2812, https://doi.org/10.5194/acp-19-2787-2019, https://doi.org/10.5194/acp-19-2787-2019, 2019
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Summertime Arctic atmospheric aerosols are strongly controlled by processes related to natural regional sources. We use a chemical transport model with size-resolved aerosol microphysics to interpret measurements made during summertime 2016 in the Canadian Arctic Archipelago. Our results explore the processes that control summertime aerosol size distributions and support a climate-relevant role for Arctic marine secondary organic aerosol formed from precursor vapors with Arctic marine sources.
Jonathan P. D. Abbatt, W. Richard Leaitch, Amir A. Aliabadi, Allan K. Bertram, Jean-Pierre Blanchet, Aude Boivin-Rioux, Heiko Bozem, Julia Burkart, Rachel Y. W. Chang, Joannie Charette, Jai P. Chaubey, Robert J. Christensen, Ana Cirisan, Douglas B. Collins, Betty Croft, Joelle Dionne, Greg J. Evans, Christopher G. Fletcher, Martí Galí, Roya Ghahreman, Eric Girard, Wanmin Gong, Michel Gosselin, Margaux Gourdal, Sarah J. Hanna, Hakase Hayashida, Andreas B. Herber, Sareh Hesaraki, Peter Hoor, Lin Huang, Rachel Hussherr, Victoria E. Irish, Setigui A. Keita, John K. Kodros, Franziska Köllner, Felicia Kolonjari, Daniel Kunkel, Luis A. Ladino, Kathy Law, Maurice Levasseur, Quentin Libois, John Liggio, Martine Lizotte, Katrina M. Macdonald, Rashed Mahmood, Randall V. Martin, Ryan H. Mason, Lisa A. Miller, Alexander Moravek, Eric Mortenson, Emma L. Mungall, Jennifer G. Murphy, Maryam Namazi, Ann-Lise Norman, Norman T. O'Neill, Jeffrey R. Pierce, Lynn M. Russell, Johannes Schneider, Hannes Schulz, Sangeeta Sharma, Meng Si, Ralf M. Staebler, Nadja S. Steiner, Jennie L. Thomas, Knut von Salzen, Jeremy J. B. Wentzell, Megan D. Willis, Gregory R. Wentworth, Jun-Wei Xu, and Jacqueline D. Yakobi-Hancock
Atmos. Chem. Phys., 19, 2527–2560, https://doi.org/10.5194/acp-19-2527-2019, https://doi.org/10.5194/acp-19-2527-2019, 2019
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The Arctic is experiencing considerable environmental change with climate warming, illustrated by the dramatic decrease in sea-ice extent. It is important to understand both the natural and perturbed Arctic systems to gain a better understanding of how they will change in the future. This paper summarizes new insights into the relationships between Arctic aerosol particles and climate, as learned over the past five or so years by a large Canadian research consortium, NETCARE.
Ian G. McKendry, Andreas Christen, Sung-Ching Lee, Madison Ferrara, Kevin B. Strawbridge, Norman O'Neill, and Andrew Black
Atmos. Chem. Phys., 19, 835–846, https://doi.org/10.5194/acp-19-835-2019, https://doi.org/10.5194/acp-19-835-2019, 2019
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Wildfire smoke in July 2015 had a significant impact on air quality, radiation, and energy budgets across British Columbia. With lighter smoke, a wetland and forested site showed enhanced photosynthetic activity (taking in carbon dioxide). However, with dense smoke the forested site became a strong source. These results suggest that smoke during the growing season potentially plays an important role in the carbon budget, and this effect will likely increase as climate changes.
Dean B. Atkinson, Mikhail Pekour, Duli Chand, James G. Radney, Katheryn R. Kolesar, Qi Zhang, Ari Setyan, Norman T. O'Neill, and Christopher D. Cappa
Atmos. Chem. Phys., 18, 5499–5514, https://doi.org/10.5194/acp-18-5499-2018, https://doi.org/10.5194/acp-18-5499-2018, 2018
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We use in situ measurements of particle light extinction to assess the performance of a typical aerosol remote retrieval method. The retrieved fine-mode fraction of extinction, a property commonly used to characterize the anthropogenic influence on the aerosol optical depth, compares well with the in situ measurements as does the retrieved effective fine-mode radius, which characterizes the average size of the particles that contribute most to scattering.
Adriana Rocha-Lima, J. Vanderlei Martins, Lorraine A. Remer, Martin Todd, John H. Marsham, Sebastian Engelstaedter, Claire L. Ryder, Carolina Cavazos-Guerra, Paulo Artaxo, Peter Colarco, and Richard Washington
Atmos. Chem. Phys., 18, 1023–1043, https://doi.org/10.5194/acp-18-1023-2018, https://doi.org/10.5194/acp-18-1023-2018, 2018
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We present results of ground-based measurements and subsequent laboratory analysis of Sahara dust samples collected in Algeria and Mauritania during the Fennec campaign in 2011. The results show that the sampled dust has low absorption characteristics and exhibits a distinct spectral bow-like shape. We find distinctive differences in the composition and optical characteristics of the dust from the two sites, corroborating with other studies that not all Saharan dust is the same.
Benjamin N. Murphy, Matthew C. Woody, Jose L. Jimenez, Ann Marie G. Carlton, Patrick L. Hayes, Shang Liu, Nga L. Ng, Lynn M. Russell, Ari Setyan, Lu Xu, Jeff Young, Rahul A. Zaveri, Qi Zhang, and Havala O. T. Pye
Atmos. Chem. Phys., 17, 11107–11133, https://doi.org/10.5194/acp-17-11107-2017, https://doi.org/10.5194/acp-17-11107-2017, 2017
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We incorporate recent findings about the behavior of organic pollutants in urban airsheds into the Community Multiscale Air Quality (CMAQ) model to refine predictions of organic particulate pollution in the United States. The new techniques, which account for the volatility and ongoing chemistry of airborne organic compounds, substantially reduce biases, particularly in the winter time and near emission sources.
Prettiny K. Ma, Yunliang Zhao, Allen L. Robinson, David R. Worton, Allen H. Goldstein, Amber M. Ortega, Jose L. Jimenez, Peter Zotter, André S. H. Prévôt, Sönke Szidat, and Patrick L. Hayes
Atmos. Chem. Phys., 17, 9237–9259, https://doi.org/10.5194/acp-17-9237-2017, https://doi.org/10.5194/acp-17-9237-2017, 2017
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Airborne particulate matter (PM) negatively impacts air quality in cities throughout the world. An important fraction of PM is organic aerosol. We have evaluated and developed several new models for secondary organic aerosol (SOA), which is formed from the chemical processing of gaseous precursors. Using our model results, we have quantified important SOA sources and precursors and also identified possible model parameterizations that could be used for air quality predictions.
Yann Blanchard, Alain Royer, Norman T. O'Neill, David D. Turner, and Edwin W. Eloranta
Atmos. Meas. Tech., 10, 2129–2147, https://doi.org/10.5194/amt-10-2129-2017, https://doi.org/10.5194/amt-10-2129-2017, 2017
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Multiband thermal measurements of zenith sky radiance were used in a retrieval algorithm, to estimate cloud optical depth and effective particle diameter of thin ice clouds in the Canadian High Arctic. The retrieval technique was validated using a synergy lidar and radar data. Inversions were performed across three polar winters and results showed a significant correlation (R2 = 0.95) for cloud optical depth retrievals and an overall accuracy of 83 % for the classification of thin ice clouds.
Hongyu Guo, Jiumeng Liu, Karl D. Froyd, James M. Roberts, Patrick R. Veres, Patrick L. Hayes, Jose L. Jimenez, Athanasios Nenes, and Rodney J. Weber
Atmos. Chem. Phys., 17, 5703–5719, https://doi.org/10.5194/acp-17-5703-2017, https://doi.org/10.5194/acp-17-5703-2017, 2017
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Fine particle pH is linked to many environmental impacts by affecting particle concentration and composition. Predicted Pasadena, CA (CalNex campaign), PM1 pH is 1.9 and PM2.5 pH 2.7, the latter higher due to sea salts. The model predicted gas–particle partitionings of HNO3–NO3−, NH3–NH4+, and HCl–Cl− are in good agreement, verifying the model predictions. A summary of contrasting locations in the US and eastern Mediterranean shows fine particles are generally highly acidic, with pH below 3.
Norman T. O'Neill, Konstantin Baibakov, Sareh Hesaraki, Liviu Ivanescu, Randall V. Martin, Chris Perro, Jai P. Chaubey, Andreas Herber, and Thomas J. Duck
Atmos. Chem. Phys., 16, 12753–12765, https://doi.org/10.5194/acp-16-12753-2016, https://doi.org/10.5194/acp-16-12753-2016, 2016
Amber M. Ortega, Patrick L. Hayes, Zhe Peng, Brett B. Palm, Weiwei Hu, Douglas A. Day, Rui Li, Michael J. Cubison, William H. Brune, Martin Graus, Carsten Warneke, Jessica B. Gilman, William C. Kuster, Joost de Gouw, Cándido Gutiérrez-Montes, and Jose L. Jimenez
Atmos. Chem. Phys., 16, 7411–7433, https://doi.org/10.5194/acp-16-7411-2016, https://doi.org/10.5194/acp-16-7411-2016, 2016
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An oxidation flow reactor (OFR) was deployed to study secondary organic aerosol (SOA) formation and aging of urban emissions at a wide range of OH exposures during the CalNex campaign in Pasadena, CA, in 2010. Results include linking SOA formation to short-lived reactive compounds, similar elemental composition of reactor-aged emissions to atmospheric aging, changes in OA mass due to condensation of oxidized gas-phase species and heterogeneous oxidation of particle-phase species.
K. Baibakov, N. T. O'Neill, L. Ivanescu, T. J. Duck, C. Perro, A. Herber, K.-H. Schulz, and O. Schrems
Atmos. Meas. Tech., 8, 3789–3809, https://doi.org/10.5194/amt-8-3789-2015, https://doi.org/10.5194/amt-8-3789-2015, 2015
C. L. Ryder, J. B. McQuaid, C. Flamant, P. D. Rosenberg, R. Washington, H. E. Brindley, E. J. Highwood, J. H. Marsham, D. J. Parker, M. C. Todd, J. R. Banks, J. K. Brooke, S. Engelstaedter, V. Estelles, P. Formenti, L. Garcia-Carreras, C. Kocha, F. Marenco, H. Sodemann, C. J. T. Allen, A. Bourdon, M. Bart, C. Cavazos-Guerra, S. Chevaillier, J. Crosier, E. Darbyshire, A. R. Dean, J. R. Dorsey, J. Kent, D. O'Sullivan, K. Schepanski, K. Szpek, J. Trembath, and A. Woolley
Atmos. Chem. Phys., 15, 8479–8520, https://doi.org/10.5194/acp-15-8479-2015, https://doi.org/10.5194/acp-15-8479-2015, 2015
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Measurements of the Saharan atmosphere and of atmospheric mineral dust are lacking but are vital to our understanding of the climate of this region and their impacts further afield. Novel observations were made by the Fennec climate programme during June 2011 and 2012 using ground-based, remote sensing and airborne platforms. Here we describe the airborne observations and the contributions they have made to furthering our understanding of the Saharan climate system.
P. L. Hayes, A. G. Carlton, K. R. Baker, R. Ahmadov, R. A. Washenfelder, S. Alvarez, B. Rappenglück, J. B. Gilman, W. C. Kuster, J. A. de Gouw, P. Zotter, A. S. H. Prévôt, S. Szidat, T. E. Kleindienst, J. H. Offenberg, P. K. Ma, and J. L. Jimenez
Atmos. Chem. Phys., 15, 5773–5801, https://doi.org/10.5194/acp-15-5773-2015, https://doi.org/10.5194/acp-15-5773-2015, 2015
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(1) Four different parameterizations for the formation and chemical evolution of secondary organic aerosol (SOA) are evaluated using a box model representing the Los Angeles region during the CalNex campaign.
(2) The SOA formed only from the oxidation of VOCs is insufficient to explain the observed SOA concentrations.
(3) The amount of SOA mass formed from diesel vehicle emissions is estimated to be 16-27%.
(4) Modeled SOA depends strongly on the P-S/IVOC volatility distribution.
K. C. Kaku, J. S. Reid, N. T. O'Neill, P. K. Quinn, D. J. Coffman, and T. F. Eck
Atmos. Meas. Tech., 7, 3399–3412, https://doi.org/10.5194/amt-7-3399-2014, https://doi.org/10.5194/amt-7-3399-2014, 2014
P. Cottle, K. Strawbridge, I. McKendry, N. O'Neill, and A. Saha
Atmos. Chem. Phys., 13, 4515–4527, https://doi.org/10.5194/acp-13-4515-2013, https://doi.org/10.5194/acp-13-4515-2013, 2013
Related subject area
Subject: Aerosols | Technique: Remote Sensing | Topic: Data Processing and Information Retrieval
Aerosol optical depth data fusion with Geostationary Korea Multi-Purpose Satellite (GEO-KOMPSAT-2) instruments GEMS, AMI, and GOCI-II: statistical and deep neural network methods
Stratospheric aerosol characteristics from SCIAMACHY limb observations: two-parameter retrieval
Retrieval and analysis of the composition of an aerosol mixture through Mie–Raman–fluorescence lidar observations
Transport of the Hunga volcanic aerosols inferred from Himawari-8/9 limb measurements
A near-global multiyear climate data record of the fine-mode and coarse-mode components of atmospheric pure dust
Innovative aerosol hygroscopic growth study from Mie–Raman–fluorescence lidar and microwave radiometer synergy
Evaluation of calibration performance of a low-cost particulate matter sensor using collocated and distant NO2
Geostationary aerosol retrievals of extreme biomass burning plumes during the 2019–2020 Australian bushfires
Multi-wavelength dataset of aerosol extinction profiles retrieved from GOMOS stellar occultation measurements
Deep-Pathfinder: a boundary layer height detection algorithm based on image segmentation
An iterative algorithm to simultaneously retrieve aerosol extinction and effective radius profiles using CALIOP
Cloud detection from multi-angular polarimetric satellite measurements using a neural network ensemble approach
Retrieving UV–Vis spectral single-scattering albedo of absorbing aerosols above clouds from synergy of ORACLES airborne and A-train sensors
Characterization of stratospheric particle size distribution uncertainties using SAGE II and SAGE III/ISS extinction spectra
Parameterizing spectral surface reflectance relationships for the Dark Target aerosol algorithm applied to a geostationary imager
Aerosol and cloud data processing and optical property retrieval algorithms for the spaceborne ACDL/DQ-1
Comparison of diurnal aerosol products retrieved from combinations of micro-pulse lidar and sun-photometer over KAUST observation site
Derivation of depolarization ratios of aerosol fluorescence and water vapor Raman backscatters from lidar measurements
Long-term aerosol particle depolarization ratio measurements with HALO Photonics Doppler lidar
HETEAC-Flex: an optimal estimation method for aerosol typing based on lidar-derived intensive optical properties
MAGARA: a Multi-Angle Geostationary Aerosol Retrieval Algorithm
Multi-section reference value for the analysis of horizontally scanning aerosol lidar observations
Retrieval of aerosol optical depth over the Arctic cryosphere during spring and summer using satellite observations
Post-process correction improves the accuracy of satellite PM2.5 retrievals
Quantifying particulate matter optical properties and flow rate in industrial stack plumes from the PRISMA hyperspectral imager
Aerosol retrieval over snow using the RemoTAP algorithm
Combined sun-photometer–lidar inversion: lessons learned during the EARLINET/ACTRIS COVID-19 campaign
Simultaneous retrieval of aerosol and ocean properties from PACE HARP2 with uncertainty assessment using cascading neural network radiative transfer models
Multi-angle aerosol optical depth retrieval method based on improved surface reflectance
First Atmospheric Aerosol Monitoring Results from Geostationary Environment Monitoring Spectrometer (GEMS) over Asia
Linear polarization signatures of atmospheric dust with the SolPol direct-sun polarimeter
Retrieval of aerosol properties from zenith sky radiance measurements
An ensemble method for improving the estimation of planetary boundary layer height from radiosonde data
Cloud top heights and aerosol layer properties from EarthCARE lidar observations: the A-CTH and A-ALD products
Influence of electromagnetic interference on the evaluation of lidar-derived aerosol properties from Ny-Ålesund, Svalbard
Global 3-D distribution of aerosol composition by synergistic use of CALIOP and MODIS observations
Aerosol optical depth retrieval from the EarthCARE Multi-Spectral Imager: the M-AOT product
Evaluating the effects of columnar NO2 on the accuracy of aerosol optical properties retrievals
An explicit formulation for the retrieval of the overlap function in an elastic and Raman aerosol lidar
The classification of atmospheric hydrometeors and aerosols from the EarthCARE radar and lidar: the A-TC, C-TC and AC-TC products
SAGE III/ISS aerosol/cloud categorization and its impact on GloSSAC
Exploring geometrical stereoscopic aerosol top height retrieval from geostationary satellite imagery in East Asia
Sensitivity studies of nighttime top-of-atmosphere radiances from artificial light sources using a 3-D radiative transfer model for nighttime aerosol retrievals
Instantaneous aerosol and surface retrieval using satellites in geostationary orbit (iAERUS-GEO) – estimation of 15 min aerosol optical depth from MSG/SEVIRI and evaluation with reference data
HETEAC – the Hybrid End-To-End Aerosol Classification model for EarthCARE
DeLiAn – a growing collection of depolarization ratio, lidar ratio and Ångström exponent for different aerosol types and mixtures from ground-based lidar observations
The impact and estimation of uncertainty correlation for multi-angle polarimetric remote sensing of aerosols and ocean color
POLIPHON conversion factors for retrieving dust-related cloud condensation nuclei and ice-nucleating particle concentration profiles at oceanic sites
Ground-based remote sensing of aerosol properties using high-resolution infrared emission and lidar observations in the High Arctic
The CALIPSO version 4.5 stratospheric aerosol subtyping algorithm
Minseok Kim, Jhoon Kim, Hyunkwang Lim, Seoyoung Lee, Yeseul Cho, Yun-Gon Lee, Sujung Go, and Kyunghwa Lee
Atmos. Meas. Tech., 17, 4317–4335, https://doi.org/10.5194/amt-17-4317-2024, https://doi.org/10.5194/amt-17-4317-2024, 2024
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Information about aerosol loading in the atmosphere can be collected from various satellite instruments. Aerosol products from various satellite instruments have their own error characteristics. This study statistically merged aerosol optical depth datasets from multiple instruments aboard geostationary satellites considering uncertainties. Also, a deep neural network technique is adopted for aerosol data merging.
Christine Pohl, Felix Wrana, Alexei Rozanov, Terry Deshler, Elizaveta Malinina, Christian von Savigny, Landon A. Rieger, Adam E. Bourassa, and John P. Burrows
Atmos. Meas. Tech., 17, 4153–4181, https://doi.org/10.5194/amt-17-4153-2024, https://doi.org/10.5194/amt-17-4153-2024, 2024
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Knowledge of stratospheric aerosol characteristics is important for understanding chemical and climate aerosol feedbacks. Two particle size distribution parameters, the aerosol extinction coefficient and the effective radius, are obtained from SCIAMACHY limb observations. The aerosol characteristics show good agreement with independent data sets from balloon-borne and satellite observations. This data set expands the limited knowledge of stratospheric aerosol characteristics.
Igor Veselovskii, Boris Barchunov, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, Mikhail Korenskii, Gaël Dubois, William Boissiere, and Nikita Kasianik
Atmos. Meas. Tech., 17, 4137–4152, https://doi.org/10.5194/amt-17-4137-2024, https://doi.org/10.5194/amt-17-4137-2024, 2024
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The paper presents a new method that categorizes atmospheric aerosols by analyzing their optical properties with a Mie–Raman–fluorescence lidar. The research specifically looks into understanding the presence of smoke, urban, and dust aerosols in the mixtures identified by this lidar. The reliability of the results is evaluated using the Monte Carlo technique. The effectiveness of this approach is successfully demonstrated through testing in ATOLL, an observatory influenced by diverse aerosols.
Fred Prata
Atmos. Meas. Tech., 17, 3751–3764, https://doi.org/10.5194/amt-17-3751-2024, https://doi.org/10.5194/amt-17-3751-2024, 2024
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Geostationary satellite data have been used to measure the stratospheric aerosols from the explosive Hunga volcanic eruption by using the data in a novel way. The onboard imager views part of the Earth's limb and data from this region were analysed to generate vertical cross-sections of aerosols high in the atmosphere. The analyses show the hemispheric spread of the aerosols and their vertical structure in layers from 22–28 km in the stratosphere.
Emmanouil Proestakis, Antonis Gkikas, Thanasis Georgiou, Anna Kampouri, Eleni Drakaki, Claire L. Ryder, Franco Marenco, Eleni Marinou, and Vassilis Amiridis
Atmos. Meas. Tech., 17, 3625–3667, https://doi.org/10.5194/amt-17-3625-2024, https://doi.org/10.5194/amt-17-3625-2024, 2024
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A new four-dimensional, multiyear, and near-global climate data record of the fine-mode (submicrometer diameter) and coarse-mode (supermicrometer diameter) components of atmospheric pure dust is presented. The dataset is considered unique with respect to a wide range of potential applications, including climatological, time series, and trend analysis over extensive geographical domains and temporal periods, validation of atmospheric dust models and datasets, and air quality.
Robin Miri, Olivier Pujol, Qiaoyun Hu, Philippe Goloub, Igor Veselovskii, Thierry Podvin, and Fabrice Ducos
Atmos. Meas. Tech., 17, 3367–3375, https://doi.org/10.5194/amt-17-3367-2024, https://doi.org/10.5194/amt-17-3367-2024, 2024
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This paper focuses on the use of fluorescence to study aerosols with lidar. An innovative method for aerosol hygroscopic growth study using fluorescence is presented. The paper presents case studies to showcase the effectiveness and potential of the proposed approach. These advancements will contribute to better understanding the interactions between aerosols and water vapor, with future work expected to be dedicated to aerosol–cloud interaction.
Kabseok Ko, Seokheon Cho, and Ramesh R. Rao
Atmos. Meas. Tech., 17, 3303–3322, https://doi.org/10.5194/amt-17-3303-2024, https://doi.org/10.5194/amt-17-3303-2024, 2024
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In our study, we examined how NO2, temperature, and relative humidity influence the calibration of PurpleAir PA-II sensors. We found that incorporating NO2 data from collocated reliable instruments enhances PM2.5 calibration performance. Due to the impracticality of collocating reliable NO2 instruments with sensors, we suggest using distant NO2 data for calibration. We demonstrated that performance improves when distant NO2 correlates highly with collocated NO2 measurements.
Daniel J. V. Robbins, Caroline A. Poulsen, Steven T. Siems, Simon R. Proud, Andrew T. Prata, Roy G. Grainger, and Adam C. Povey
Atmos. Meas. Tech., 17, 3279–3302, https://doi.org/10.5194/amt-17-3279-2024, https://doi.org/10.5194/amt-17-3279-2024, 2024
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Extreme wildfire events are becoming more common with climate change. The smoke plumes associated with these wildfires are not captured by current operational satellite products due to their high optical thickness. We have developed a novel aerosol retrieval for the Advanced Himawari Imager to study these plumes. We find very high values of optical thickness not observed in other operational satellite products, suggesting these plumes have been missed in previous studies.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Didier Fussen, Christine Bingen, Filip Vanhellemont, Nina Mateshvili, Alexei Rozanov, and Christine Pohl
Atmos. Meas. Tech., 17, 3085–3101, https://doi.org/10.5194/amt-17-3085-2024, https://doi.org/10.5194/amt-17-3085-2024, 2024
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We have developed the new multi-wavelength dataset of aerosol extinction profiles, which are retrieved from the averaged transmittance spectra by the Global Ozone Monitoring by Occultation of Stars instrument aboard Envisat. The retrieved aerosol extinction profiles are provided in the altitude range 10–40 km at 400, 440, 452, 470, 500, 525, 550, 672 and 750 nm for the period 2002–2012. FMI-GOMOSaero aerosol profiles have improved quality; they are in good agreement with other datasets.
Jasper S. Wijnands, Arnoud Apituley, Diego Alves Gouveia, and Jan Willem Noteboom
Atmos. Meas. Tech., 17, 3029–3045, https://doi.org/10.5194/amt-17-3029-2024, https://doi.org/10.5194/amt-17-3029-2024, 2024
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The mixing of air in the lower atmosphere influences the concentration of air pollutants and greenhouse gases. Our study developed a new method, Deep-Pathfinder, to estimate mixing layer height. Deep-Pathfinder analyses imagery with aerosol observations using artificial intelligence techniques for computer vision. Compared to existing methods, it improves temporal consistency and resolution and can be used in real time, which is valuable for aviation, forecasting, and air quality monitoring.
Liang Chang, Jing Li, Jingjing Ren, Changrui Xiong, and Lu Zhang
Atmos. Meas. Tech., 17, 2637–2648, https://doi.org/10.5194/amt-17-2637-2024, https://doi.org/10.5194/amt-17-2637-2024, 2024
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We described a modified lidar inversion algorithm to retrieve aerosol extinction and size distribution simultaneously from two-wavelength elastic lidar measurements. Its major advantage is that the lidar ratio of each layer is determined iteratively by a lidar ratio–Ångström exponent lookup table. The algorithm was applied to the Raman lidar and CALIOP measurements. The retrieved results by our method are in good agreement with those achieved by Raman method.
Zihao Yuan, Guangliang Fu, Bastiaan van Diedenhoven, Hai Xiang Lin, Jan Willem Erisman, and Otto P. Hasekamp
Atmos. Meas. Tech., 17, 2595–2610, https://doi.org/10.5194/amt-17-2595-2024, https://doi.org/10.5194/amt-17-2595-2024, 2024
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Currently, aerosol properties from spaceborne multi-angle polarimeter (MAP) instruments can only be retrieved in cloud-free areas or in areas where an aerosol layer is located above a cloud. Therefore, it is important to be able to identify cloud-free pixels for which an aerosol retrieval algorithm can provide meaningful output. The developed neural network cloud screening demonstrates that cloud masking for MAP aerosol retrieval can be based on the MAP measurements themselves.
Hiren T. Jethva, Omar Torres, Richard A. Ferrare, Sharon P. Burton, Anthony L. Cook, David B. Harper, Chris A. Hostetler, Jens Redemann, Vinay Kayetha, Samuel LeBlanc, Kristina Pistone, Logan Mitchell, and Connor J. Flynn
Atmos. Meas. Tech., 17, 2335–2366, https://doi.org/10.5194/amt-17-2335-2024, https://doi.org/10.5194/amt-17-2335-2024, 2024
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We introduce a novel synergy algorithm applied to ORALCES airborne measurements of above-cloud aerosol optical depth and UV–Vis satellite observations from OMI and MODIS to retrieve spectral aerosol single-scattering albedo of lofted layers of carbonaceous smoke aerosols over clouds. The development of the proposed aerosol–cloud algorithm implies a possible synergy of CALIOP and OMI–MODIS passive sensors to deduce a global product of AOD and SSA of absorbing aerosols above clouds.
Travis N. Knepp, Mahesh Kovilakam, Larry Thomason, and Stephen J. Miller
Atmos. Meas. Tech., 17, 2025–2054, https://doi.org/10.5194/amt-17-2025-2024, https://doi.org/10.5194/amt-17-2025-2024, 2024
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An algorithm is presented to derive a new SAGE III/ISS (Stratospheric Aerosol and Gas Experiment III on the International Space Station) Level-2 product: the size distribution of stratospheric particles. This is a significant improvement over previous techniques in that we now provide uncertainty estimates for all inferred parameters. We also evaluated the stability of this method in retrieving bimodal distribution parameters. We present a special application to the 2022 eruption of Hunga Tonga.
Mijin Kim, Robert C. Levy, Lorraine A. Remer, Shana Mattoo, and Pawan Gupta
Atmos. Meas. Tech., 17, 1913–1939, https://doi.org/10.5194/amt-17-1913-2024, https://doi.org/10.5194/amt-17-1913-2024, 2024
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The study focused on evaluating and modifying the surface reflectance parameterization (SRP) of the Dark Target (DT) algorithm for geostationary observation. When using the DT SRP with the ABIs sensor on GOES-R, artificial diurnal signatures were present in AOD retrieval. To overcome this issue, a new SRP was developed, incorporating solar zenith angle and land cover type. The revised SRP resulted in improved AOD retrieval, demonstrating reduced bias around local noon.
Guangyao Dai, Songhua Wu, Wenrui Long, Jiqiao Liu, Yuan Xie, Kangwen Sun, Fanqian Meng, Xiaoquan Song, Zhongwei Huang, and Weibiao Chen
Atmos. Meas. Tech., 17, 1879–1890, https://doi.org/10.5194/amt-17-1879-2024, https://doi.org/10.5194/amt-17-1879-2024, 2024
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An overview is given of the main algorithms applied to derive the aerosol and cloud optical property product of the Aerosol and Carbon Detection Lidar (ACDL), which is capable of globally profiling aerosol and cloud optical properties with high accuracy. The paper demonstrates the observational capabilities of ACDL for aerosol and cloud vertical structure and global distribution through two optical property product measurement cases and global aerosol optical depth profile observations.
Anton Lopatin, Oleg Dubovik, Georgiy Stenchikov, Ellsworth J. Welton, Illia Shevchenko, David Fuertes, Marcos Herreras-Giralda, Tatsiana Lapyonok, and Alexander Smirnov
EGUsphere, https://doi.org/10.5194/egusphere-2024-369, https://doi.org/10.5194/egusphere-2024-369, 2024
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This study compares aerosol properties over the KAUST campus using GRASP and MPLNET methods. It focuses on understanding the impact of different assumptions in aerosol retrieval methods on daytime and nighttime retrievals. The study analyses the seasonal variability of aerosol properties, aiding in understanding aerosol behavior and improving retrieval techniques. This is vital for enhancing our knowledge of aerosol distribution, which impacts climate and public health.
Igor Veselovskii, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, William Boissiere, Mikhail Korenskiy, Nikita Kasianik, Sergey Khaykyn, and Robin Miri
Atmos. Meas. Tech., 17, 1023–1036, https://doi.org/10.5194/amt-17-1023-2024, https://doi.org/10.5194/amt-17-1023-2024, 2024
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Measurements of transported smoke layers were performed with a lidar in Lille and a five-channel fluorescence lidar in Moscow. Results show the peak of fluorescence in the boundary layer is at 438 nm, while in the smoke layer it shifts to longer wavelengths. The fluorescence depolarization is 45 % to 55 %. The depolarization ratio of the water vapor channel is low (2 ± 0.5 %) in the absence of fluorescence and can be used to evaluate the contribution of fluorescence to water vapor signal.
Viet Le, Hannah Lobo, Ewan J. O'Connor, and Ville Vakkari
Atmos. Meas. Tech., 17, 921–941, https://doi.org/10.5194/amt-17-921-2024, https://doi.org/10.5194/amt-17-921-2024, 2024
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This study offers a long-term overview of aerosol particle depolarization ratio at the wavelength of 1565 nm obtained from vertical profiling measurements by Halo Doppler lidars during 4 years at four different locations across Finland. Our observations support the long-term usage of Halo Doppler lidar depolarization ratio such as the detection of aerosols that may pose a safety risk for aviation. Long-range Saharan dust transport and pollen transport are also showcased here.
Athena Augusta Floutsi, Holger Baars, and Ulla Wandinger
Atmos. Meas. Tech., 17, 693–714, https://doi.org/10.5194/amt-17-693-2024, https://doi.org/10.5194/amt-17-693-2024, 2024
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We introduce an aerosol-typing scheme (HETEAC-Flex) based on lidar-derived intensive optical properties and applicable to ground-based and spaceborne lidars. HETEAC-Flex utilizes the optimal estimation method and enables the identification of up to four different aerosol components, as well as the determination of their contribution to the aerosol mixture in terms of relative volume. The aerosol components represent common aerosol types such as dust, sea salt, smoke and pollution.
James A. Limbacher, Ralph A. Kahn, Mariel D. Friberg, Jaehwa Lee, Tyler Summers, and Hai Zhang
Atmos. Meas. Tech., 17, 471–498, https://doi.org/10.5194/amt-17-471-2024, https://doi.org/10.5194/amt-17-471-2024, 2024
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We present the new Multi-Angle Geostationary Aerosol Retrieval Algorithm (MAGARA) that fuses observations from GOES-16 and GOES-17 to retrieve information about aerosol loading (at 10–15 min cadence) and aerosol particle properties (daily), all at pixel-level resolution. We present MAGARA results for three case studies: the 2018 California Camp Fire, the 2019 Williams Flats Fire, and the 2019 Kincade Fire. We also compare MAGARA aerosol loading and particle properties with AERONET.
Juseon Shin, Gahyeong Kim, Dukhyeon Kim, Matthias Tesche, Gahyeon Park, and Youngmin Noh
Atmos. Meas. Tech., 17, 397–406, https://doi.org/10.5194/amt-17-397-2024, https://doi.org/10.5194/amt-17-397-2024, 2024
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We introduce the multi-section method, a novel approach for stable extinction coefficient retrievals in horizontally scanning aerosol lidar measurements, in this study. Our method effectively removes signal–noise-induced irregular peaks and derives a reference extinction coefficient, αref, from multiple scans, resulting in a strong correlation (>0.74) with PM2.5 mass concentrations. Case studies demonstrate its utility in retrieving spatio-temporal aerosol distributions and PM2.5 concentrations.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Soheila Jafariserajehlou, Sachin S. Gunthe, Andreas Herber, Christoph Ritter, Hartmut Bösch, and John P. Burrows
Atmos. Meas. Tech., 17, 359–375, https://doi.org/10.5194/amt-17-359-2024, https://doi.org/10.5194/amt-17-359-2024, 2024
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Aerosols are suspensions of particles dispersed in the air. In this study, we use a novel retrieval of satellite data to investigate an optical property of aerosols, the aerosol optical depth, in the high Arctic to assess their direct and indirect roles in climate change. This study demonstrates that the presented approach shows good quality and very promising potential.
Andrea Porcheddu, Ville Kolehmainen, Timo Lähivaara, and Antti Lipponen
EGUsphere, https://doi.org/10.5194/egusphere-2023-2635, https://doi.org/10.5194/egusphere-2023-2635, 2024
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This study focuses on improving the accuracy of satellite-based PM2.5 retrieval, crucial for monitoring air quality and its impact on health. It employs machine learning to correct the AOD-to-PM2.5 conversion ratio using various data sources. The approach produces high-resolution PM2.5 estimates with improved accuracy. The method is flexible and can incorporate additional training data from different sources, making it a valuable tool for air quality monitoring and epidemiological studies.
Gabriel Calassou, Pierre-Yves Foucher, and Jean-François Léon
Atmos. Meas. Tech., 17, 57–71, https://doi.org/10.5194/amt-17-57-2024, https://doi.org/10.5194/amt-17-57-2024, 2024
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We propose analyzing the aerosol composition of plumes emitted by different industrial stacks using PRISMA satellite hyperspectral observations. Three industrial sites have been observed: a coal-fired power plant in South Africa, a steel plant in China, and gas flaring at an oil extraction site in Algeria. Aerosol optical thickness and particle radius are retrieved within the plumes. The mass flow rate of particulate matter is estimated in the plume using the integrated mass enhancement method.
Zihan Zhang, Guangliang Fu, and Otto Hasekamp
Atmos. Meas. Tech., 16, 6051–6063, https://doi.org/10.5194/amt-16-6051-2023, https://doi.org/10.5194/amt-16-6051-2023, 2023
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In order to conduct accurate aerosol retrieval over snow, the Remote Sensing of Trace Gases and Aerosol Products (RemoTAP) algorithm is extended with a bi-directional reflection distribution function for snow surfaces. The experiments with both synthetic and real data show that the extended RemoTAP maintains capability for snow-free pixels and has obvious advantages in accuracy and the fraction of successful retrievals for retrieval over snow, especially over surfaces with snow cover > 75 %.
Alexandra Tsekeri, Anna Gialitaki, Marco Di Paolantonio, Davide Dionisi, Gian Luigi Liberti, Alnilam Fernandes, Artur Szkop, Aleksander Pietruczuk, Daniel Pérez-Ramírez, Maria J. Granados Muñoz, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Diego Bermejo Pantaleón, Juan Antonio Bravo-Aranda, Anna Kampouri, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Salvatore Romano, Maria Rita Perrone, Xiaoxia Shang, Mika Komppula, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Diofantos Hadjimitsis, Francisco Navas-Guzmán, Alexander Haefele, Dominika Szczepanik, Artur Tomczak, Iwona S. Stachlewska, Livio Belegante, Doina Nicolae, Kalliopi Artemis Voudouri, Dimitris Balis, Athena A. Floutsi, Holger Baars, Linda Miladi, Nicolas Pascal, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 16, 6025–6050, https://doi.org/10.5194/amt-16-6025-2023, https://doi.org/10.5194/amt-16-6025-2023, 2023
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EARLINET/ACTRIS organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. The work presented herein focuses on deriving a common methodology for applying a synergistic retrieval that utilizes the network's ground-based passive and active remote sensing measurements and deriving the aerosols from anthropogenic activities over Europe.
Meng Gao, Bryan A. Franz, Peng-Wang Zhai, Kirk Knobelspiesse, Andrew M. Sayer, Xiaoguang Xu, J. Vanderlei Martins, Brian Cairns, Patricia Castellanos, Guangliang Fu, Neranga Hannadige, Otto Hasekamp, Yongxiang Hu, Amir Ibrahim, Frederick Patt, Anin Puthukkudy, and P. Jeremy Werdell
Atmos. Meas. Tech., 16, 5863–5881, https://doi.org/10.5194/amt-16-5863-2023, https://doi.org/10.5194/amt-16-5863-2023, 2023
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This study evaluated the retrievability and uncertainty of aerosol and ocean properties from PACE's HARP2 instrument using enhanced neural network models with the FastMAPOL algorithm. A cascading retrieval method is developed to improve retrieval performance. A global set of simulated HARP2 data is generated and used for uncertainty evaluations. The performance assessment demonstrates that the FastMAPOL algorithm is a viable approach for operational application to HARP2 data after PACE launch.
Lijuan Chen, Ren Wang, Ying Fei, Peng Fang, Yong Zha, and Haishan Chen
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-204, https://doi.org/10.5194/amt-2023-204, 2023
Revised manuscript accepted for AMT
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This study explores the problems of surface reflectance estimation from previous MISR satellite remote sensing images and develops an error correction model to invert and obtain a higher precision AOD product. High-accuracy AOD is important not only for the daily monitoring of air pollution, but also for the study of energy exchange between land and atmosphere. The study will help to further improve the retrieval accuracy of multi-angle AOD on large spatial scales and long time series.
Yeseul Cho, Jhoon Kim, Sujung Go, Mijin Kim, Seoyoung Lee, Minseok Kim, Heesung Chong, Won-Jin Lee, Dong-Won Lee, Omar Torres, and Sang Seo Park
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-221, https://doi.org/10.5194/amt-2023-221, 2023
Revised manuscript accepted for AMT
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Aerosol optical properties have been provided from the Geostationary Environment Monitoring Spectrometer (GEMS). It is the world’s first geostationary earth orbit (GEO) satellite instrument designed for atmospheric environmental monitoring. This study describes improvements to the GEMS aerosol retrieval algorithm (AERAOD) and its validation results. These enhancements are aimed at providing more accurate and reliable aerosol monitoring results for Asia.
Vasiliki Daskalopoulou, Panagiotis I. Raptis, Alexandra Tsekeri, Vassilis Amiridis, Stelios Kazadzis, Zbigniew Ulanowski, Vassilis Charmandaris, Konstantinos Tassis, and William Martin
Atmos. Meas. Tech., 16, 4529–4550, https://doi.org/10.5194/amt-16-4529-2023, https://doi.org/10.5194/amt-16-4529-2023, 2023
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Atmospheric dust particles may present a preferential alignment due to their shape on long range transport. Since dust is abundant and plays a key role to global climate, the elusive observation of orientation will be a game changer to existing measurement techniques and the representation of particles in climate models. We utilize a specifically designed instrument, SolPol, and target the Sun from the ground for large polarization values under dusty conditions, a clear sign of orientation.
Sara Herrero-Anta, Roberto Román, David Mateos, Ramiro González, Juan Carlos Antuña-Sánchez, Marcos Herreras-Giralda, Antonio Fernando Almansa, Daniel González-Fernández, Celia Herrero del Barrio, Carlos Toledano, Victoria E. Cachorro, and Ángel M. de Frutos
Atmos. Meas. Tech., 16, 4423–4443, https://doi.org/10.5194/amt-16-4423-2023, https://doi.org/10.5194/amt-16-4423-2023, 2023
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This paper shows the potential of a simple radiometer like the ZEN-R52 as a possible alternative for aerosol property retrieval in remote areas. A calibration method based on radiative transfer simulations together with an inversion methodology using the GRASP code is proposed here. The results demonstrate that this methodology is useful for the retrieval of aerosol extensive properties like aerosol optical depth (AOD) and aerosol volume concentration for total, fine and coarse modes.
Xi Chen, Ting Yang, Zifa Wang, Futing Wang, and Haibo Wang
Atmos. Meas. Tech., 16, 4289–4302, https://doi.org/10.5194/amt-16-4289-2023, https://doi.org/10.5194/amt-16-4289-2023, 2023
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Uncertainties remain great in the planetary boundary layer height (PBLH) determination from radiosonde, especially during the transition period of different PBL regimes. We combine seven existing methods along with statistical modification on gradient-based methods. We find that the ensemble method can eliminate the overestimation of PBLH and reduce the inconsistency between individual methods. The ensemble method improves the effectiveness of PBLH determination to 62.6 %.
Ulla Wandinger, Moritz Haarig, Holger Baars, David Donovan, and Gerd-Jan van Zadelhoff
Atmos. Meas. Tech., 16, 4031–4052, https://doi.org/10.5194/amt-16-4031-2023, https://doi.org/10.5194/amt-16-4031-2023, 2023
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We introduce the algorithms that have been developed to derive cloud top height and aerosol layer products from observations with the Atmospheric Lidar (ATLID) onboard the Earth Cloud, Aerosol and Radiation Explorer (EarthCARE). The products provide information on the uppermost cloud and geometrical and optical properties of aerosol layers in an atmospheric column. They can be used individually but also serve as input for algorithms that combine observations with EarthCARE’s lidar and imager.
Tim Poguntke and Christoph Ritter
Atmos. Meas. Tech., 16, 4009–4014, https://doi.org/10.5194/amt-16-4009-2023, https://doi.org/10.5194/amt-16-4009-2023, 2023
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In this work we analyze the impact of electromagnetic interference on an aerosol lidar. We found that aging transient recorders may produce a noise with fixed frequency that can be removed a posteriori.
Rei Kudo, Akiko Higurashi, Eiji Oikawa, Masahiro Fujikawa, Hiroshi Ishimoto, and Tomoaki Nishizawa
Atmos. Meas. Tech., 16, 3835–3863, https://doi.org/10.5194/amt-16-3835-2023, https://doi.org/10.5194/amt-16-3835-2023, 2023
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A synergistic retrieval method of aerosol components (water-soluble, light-absorbing, dust, and sea salt particles) from CALIOP and MODIS observations was developed. The total global 3-D distributions and those for each component showed good consistency with the CALIOP and MODIS official products and previous studies. The shortwave direct radiative effects of each component at the top and bottom of the atmosphere and for the heating rate were also consistent with previous studies.
Nicole Docter, Rene Preusker, Florian Filipitsch, Lena Kritten, Franziska Schmidt, and Jürgen Fischer
Atmos. Meas. Tech., 16, 3437–3457, https://doi.org/10.5194/amt-16-3437-2023, https://doi.org/10.5194/amt-16-3437-2023, 2023
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We describe the stand-alone retrieval algorithm used to derive aerosol properties relying on measurements of the Multi-Spectral Imager (MSI) aboard the upcoming Earth Clouds, Aerosols and Radiation Explorer (EarthCARE) satellite. This aerosol data product will be available as M-AOT after the launch of EarthCARE. Additionally, we applied the algorithm to simulated EarthCARE MSI and Moderate Resolution Imaging Spectroradiometer (MODIS) data for prelaunch algorithm verification.
Theano Drosoglou, Ioannis-Panagiotis Raptis, Massimo Valeri, Stefano Casadio, Francesca Barnaba, Marcos Herreras-Giralda, Anton Lopatin, Oleg Dubovik, Gabriele Brizzi, Fabrizio Niro, Monica Campanelli, and Stelios Kazadzis
Atmos. Meas. Tech., 16, 2989–3014, https://doi.org/10.5194/amt-16-2989-2023, https://doi.org/10.5194/amt-16-2989-2023, 2023
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Aerosol optical properties derived from sun photometers depend on the optical depth of trace gases absorbing solar radiation at specific spectral ranges. Various networks use satellite-based climatologies to account for this or neglect their effect. In this work, we evaluate the effect of NO2 absorption in aerosol retrievals from AERONET and SKYNET over two stations in Rome, Italy, with relatively high NO2 spatiotemporal variations, using NO2 data from the Pandora network and the TROPOMI sensor.
Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Michaël Sicard, Federico Dios, Cristina Gil-Díaz, Daniel Camilo Fortunato dos Santos Oliveira, and Francesc Rocadenbosch
Atmos. Meas. Tech., 16, 3015–3025, https://doi.org/10.5194/amt-16-3015-2023, https://doi.org/10.5194/amt-16-3015-2023, 2023
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We derive an explicit (i.e., non-iterative) formula for the retrieval of the overlap function in an aerosol lidar with both elastic and Raman N2 and/or O2 channels used for independent measurements of aerosol backscatter and extinction coefficients. The formula requires only the measured, range-corrected elastic and the corresponding Raman signals, plus an assumed lidar ratio. We assess the influence of the lidar ratio error in the overlap function retrieval and present retrieval examples.
Abdanour Irbah, Julien Delanoë, Gerd-Jan van Zadelhoff, David P. Donovan, Pavlos Kollias, Bernat Puigdomènech Treserras, Shannon Mason, Robin J. Hogan, and Aleksandra Tatarevic
Atmos. Meas. Tech., 16, 2795–2820, https://doi.org/10.5194/amt-16-2795-2023, https://doi.org/10.5194/amt-16-2795-2023, 2023
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The Cloud Profiling Radar (CPR) and ATmospheric LIDar (ATLID) aboard the EarthCARE satellite are used to probe the Earth's atmosphere by measuring cloud and aerosol profiles. ATLID is sensitive to aerosols and small cloud particles and CPR to large ice particles, snowflakes and raindrops. It is the synergy of the measurements of these two instruments that allows a better classification of the atmospheric targets and the description of the associated products, which are the subject of this paper.
Mahesh Kovilakam, Larry Thomason, and Travis Knepp
Atmos. Meas. Tech., 16, 2709–2731, https://doi.org/10.5194/amt-16-2709-2023, https://doi.org/10.5194/amt-16-2709-2023, 2023
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The paper describes SAGE III/ISS aerosol/cloud categorization and its implications on Global Space-based Stratospheric Aerosol Climatology (GloSSAC). The presence of data from the SAGE type of multi-wavelength measurements is important in GloSSAC. The new aerosol/cloud categorization method described in this paper will help retain more measurements, particularly in the lower stratosphere during and following a volcanic event and other processes.
Minseok Kim, Jhoon Kim, Hyunkwang Lim, Seoyoung Lee, Yeseul Cho, Huidong Yeo, and Sang-Woo Kim
Atmos. Meas. Tech., 16, 2673–2690, https://doi.org/10.5194/amt-16-2673-2023, https://doi.org/10.5194/amt-16-2673-2023, 2023
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Aerosol height information is important when seeking an understanding of the vertical structure of the aerosol layer and long-range transport. In this study, a geometrical aerosol top height (ATH) retrieval using a parallax of two geostationary satellites is investigated. With sufficient longitudinal separation between the two satellites, a decent ATH product could be retrieved.
Jianglong Zhang, Jeffrey S. Reid, Steven D. Miller, Miguel Román, Zhuosen Wang, Robert J. D. Spurr, and Shawn Jaker
Atmos. Meas. Tech., 16, 2531–2546, https://doi.org/10.5194/amt-16-2531-2023, https://doi.org/10.5194/amt-16-2531-2023, 2023
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We adapted the spherical harmonics discrete ordinate method 3-dimentional radiative transfer model (3-D RTM) and developed a nighttime 3-D RTM capability for simulating top-of-atmosphere radiances from artificial light sources for aerosol retrievals. Our study suggests that both aerosol optical depth and aerosol plume height can be effectively retrieved using nighttime observations over artificial light sources, through the newly developed radiative transfer modeling capability.
Xavier Ceamanos, Bruno Six, Suman Moparthy, Dominique Carrer, Adèle Georgeot, Josef Gasteiger, Jérôme Riedi, Jean-Luc Attié, Alexei Lyapustin, and Iosif Katsev
Atmos. Meas. Tech., 16, 2575–2599, https://doi.org/10.5194/amt-16-2575-2023, https://doi.org/10.5194/amt-16-2575-2023, 2023
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A new algorithm to retrieve the diurnal evolution of aerosol optical depth over land and ocean from geostationary meteorological satellites is proposed and successfully evaluated with reference ground-based and satellite data. The high-temporal-resolution aerosol observations that are obtained from the EUMETSAT Meteosat Second Generation mission are unprecedented and open the door to studies that cannot be conducted with the once-a-day observations available from low-Earth-orbit satellites.
Ulla Wandinger, Athena Augusta Floutsi, Holger Baars, Moritz Haarig, Albert Ansmann, Anja Hünerbein, Nicole Docter, David Donovan, Gerd-Jan van Zadelhoff, Shannon Mason, and Jason Cole
Atmos. Meas. Tech., 16, 2485–2510, https://doi.org/10.5194/amt-16-2485-2023, https://doi.org/10.5194/amt-16-2485-2023, 2023
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We introduce an aerosol classification model that has been developed for the Earth Clouds, Aerosols and Radiation Explorer (EarthCARE). The model provides a consistent description of microphysical, optical, and radiative properties of common aerosol types such as dust, sea salt, pollution, and smoke. It is used for aerosol classification and assessment of radiation effects based on the synergy of active and passive observations with lidar, imager, and radiometer of the multi-instrument platform.
Athena Augusta Floutsi, Holger Baars, Ronny Engelmann, Dietrich Althausen, Albert Ansmann, Stephanie Bohlmann, Birgit Heese, Julian Hofer, Thomas Kanitz, Moritz Haarig, Kevin Ohneiser, Martin Radenz, Patric Seifert, Annett Skupin, Zhenping Yin, Sabur F. Abdullaev, Mika Komppula, Maria Filioglou, Elina Giannakaki, Iwona S. Stachlewska, Lucja Janicka, Daniele Bortoli, Eleni Marinou, Vassilis Amiridis, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Boris Barja, and Ulla Wandinger
Atmos. Meas. Tech., 16, 2353–2379, https://doi.org/10.5194/amt-16-2353-2023, https://doi.org/10.5194/amt-16-2353-2023, 2023
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DeLiAn is a collection of lidar-derived aerosol intensive optical properties for several aerosol types, namely the particle linear depolarization ratio, the extinction-to-backscatter ratio (lidar ratio) and the Ångström exponent. The data collection is based on globally distributed, long-term, ground-based, multiwavelength, Raman and polarization lidar measurements and currently covers two wavelengths, 355 and 532 nm, for 13 aerosol categories ranging from basic aerosol types to mixtures.
Meng Gao, Kirk Knobelspiesse, Bryan A. Franz, Peng-Wang Zhai, Brian Cairns, Xiaoguang Xu, and J. Vanderlei Martins
Atmos. Meas. Tech., 16, 2067–2087, https://doi.org/10.5194/amt-16-2067-2023, https://doi.org/10.5194/amt-16-2067-2023, 2023
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Multi-angle polarimetric measurements have been shown to greatly improve the remote sensing capability of aerosols and help atmospheric correction for ocean color retrievals. However, the uncertainty correlations among different measurement angles have not been well characterized. In this work, we provided a practical framework to evaluate the impact of the angular uncertainty correlation in retrieval results and a method to directly estimate correlation strength from retrieval residuals.
Yun He, Zhenping Yin, Albert Ansmann, Fuchao Liu, Longlong Wang, Dongzhe Jing, and Huijia Shen
Atmos. Meas. Tech., 16, 1951–1970, https://doi.org/10.5194/amt-16-1951-2023, https://doi.org/10.5194/amt-16-1951-2023, 2023
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With the AERONET database, this study derives dust-related conversion factors at oceanic sites used in the POLIPHON method, which can convert lidar-retrieved dust extinction to ice-nucleating particle (INP)- and cloud condensation nuclei (CCN)-relevant parameters. The particle linear depolarization ratio in the AERONET aerosol inversion product is used to identify dust data points. The derived conversion factors can be applied to inverse 3-D global distributions of dust-related INPCs and CCNCs.
Denghui Ji, Mathias Palm, Christoph Ritter, Philipp Richter, Xiaoyu Sun, Matthias Buschmann, and Justus Notholt
Atmos. Meas. Tech., 16, 1865–1879, https://doi.org/10.5194/amt-16-1865-2023, https://doi.org/10.5194/amt-16-1865-2023, 2023
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To measuring aerosol components, a Fourier transform infrared spectrometer (FTIS) and a lidar are operated in Ny-Ålesund, Spitsbergen (78° N, 11° E). Using the FTIS, a retrieval algorithm is developed for dust, sea salt, black carbon, and sulfate. The distribution of aerosols or clouds is provided by lidar and used as an indicator for aerosol or cloud retrieval with the FTS. Thus, a two-instrument joint-observation scheme is designed and is used on the data measured from 2019 to the present.
Jason L. Tackett, Jayanta Kar, Mark A. Vaughan, Brian J. Getzewich, Man-Hae Kim, Jean-Paul Vernier, Ali H. Omar, Brian E. Magill, Michael C. Pitts, and David M. Winker
Atmos. Meas. Tech., 16, 745–768, https://doi.org/10.5194/amt-16-745-2023, https://doi.org/10.5194/amt-16-745-2023, 2023
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The accurate identification of aerosol types in the stratosphere is important to characterize their impacts on the Earth climate system. The space-borne lidar on board CALIPSO is well-posed to identify aerosols in the stratosphere from volcanic eruptions and major wildfire events. This paper describes improvements implemented in the version 4.5 CALIPSO data release to more accurately discriminate between volcanic ash, sulfate, and smoke within the stratosphere.
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Parks, M. M., and Finger, D. C.: Monitoring dust events using doppler lidar
and ceilometer in Iceland, Atmosphere, 11, 1–23,
https://doi.org/10.3390/atmos11121294, 2020.
Short summary
We used (columnar) ground-based remote sensing (RS) tools and surface measurements to characterize local (drainage-basin) dust plumes at a site in the Yukon. Plume height, particle size, and column-to-surface ratios enabled insights into how satellite RS could be used to analyze Arctic-wide dust transport. This helps modelers refine dust impacts in their climate change simulations. It is an important step since local dust is a key source of dust deposition on snow in the sensitive Arctic region.
We used (columnar) ground-based remote sensing (RS) tools and surface measurements to...
