Articles | Volume 17, issue 3
https://doi.org/10.5194/amt-17-1037-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/amt-17-1037-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Feb 2024
Research article |
| 13 Feb 2024
| 13 Feb 2024
Development and characterization of a high-performance single-particle aerosol mass spectrometer (HP-SPAMS)
Xubing Du
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Qinhui Xie
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Qing Huang
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Xuan Li
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Junlin Yang
Guangzhou Hexin Analytical Instrument Limited Company, Guangzhou, 510530, China
Zhihui Hou
Guangzhou Hexin Analytical Instrument Limited Company, Guangzhou, 510530, China
Jingjing Wang
Guangzhou Hexin Analytical Instrument Limited Company, Guangzhou, 510530, China
Xue Li
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Zhen Zhou
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Zhengxu Huang
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Wei Gao
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou, 510632, China
Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollution, Guangzhou, 510632, China
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Cited
13 citations as recorded by crossref.
- Algorithm for improving the sizing accuracy in real-time bioaerosol single particle mass spectrometer S. Li et al. https://doi.org/10.1016/j.jaerosci.2024.106501
- Real-Time Detection of Urban Atmospheric Micro–Nanoplastics and Their Chemical Mixing State Using Bioaerosol Single-Particle Mass Spectrometry C. Zhang et al. https://doi.org/10.1021/acs.est.5c06513
- Investigation of brake wear particle emissions via single particle mass spectral signatures: Comparison of laboratory and ambient measurements S. Jeong et al. https://doi.org/10.1016/j.scitotenv.2025.181277
- Basic Principles, Approaches, and Instruments for Studying, Characterizing, and Applying Natural and Artificial Fogs P. Todorov et al. https://doi.org/10.3390/w18010029
- A Semi‐Continuous Versatile Aerosol Concentration Enrichment System Coupled to Online Extraction and Lc–Ms for Molecular‐Level Analysis of Atmospheric Aerosol Organic Matter H. Xiong et al. https://doi.org/10.1002/smtd.202501649
- Preliminary characterization of a single-particle aerosol mass spectrometer with fluorescence pre-selection capability R. Lu et al. https://doi.org/10.1016/j.microc.2026.117981
- Technical note: Determining chemical composition of atmospheric single particles by a standard-free mass calibration algorithm S. Shi et al. https://doi.org/10.5194/acp-24-7001-2024
- Size-dependent airborne metal solubility and associated analytical techniques at bulk and single particle levels: A review Y. Zhao et al. https://doi.org/10.1016/j.atmosenv.2025.121343
- Single-particle decoding of aerosol pollutants size-composition relationships: An interpretable XGBoost-SHAP framework with DTEWD-enhanced SPAMS analysis Y. Ye et al. https://doi.org/10.1016/j.jhazmat.2025.140397
- Design of a wide-particle-size-range aerodynamic injection system with a new pre-focus structure J. Huang et al. https://doi.org/10.5194/amt-18-2739-2025
- Measurement report: The Fifth International Workshop on Ice Nucleation phase 1 (FIN-01): intercomparison of single-particle mass spectrometers X. Shen et al. https://doi.org/10.5194/acp-24-10869-2024
- Chemically Resolved Respiratory Deposition of Ultrafine Particles Characterized by Number Concentration in the Urban Atmosphere J. Zhai et al. https://doi.org/10.1021/acs.est.4c03279
- Integrated Aerosol Collection and Thermal-Desorption Chemical Ionization TOFMS for Rapid Particulate-Composition Analysis Z. Wang et al. https://doi.org/10.1021/acs.analchem.6c00711
13 citations as recorded by crossref.
- Algorithm for improving the sizing accuracy in real-time bioaerosol single particle mass spectrometer S. Li et al. https://doi.org/10.1016/j.jaerosci.2024.106501
- Real-Time Detection of Urban Atmospheric Micro–Nanoplastics and Their Chemical Mixing State Using Bioaerosol Single-Particle Mass Spectrometry C. Zhang et al. https://doi.org/10.1021/acs.est.5c06513
- Investigation of brake wear particle emissions via single particle mass spectral signatures: Comparison of laboratory and ambient measurements S. Jeong et al. https://doi.org/10.1016/j.scitotenv.2025.181277
- Basic Principles, Approaches, and Instruments for Studying, Characterizing, and Applying Natural and Artificial Fogs P. Todorov et al. https://doi.org/10.3390/w18010029
- A Semi‐Continuous Versatile Aerosol Concentration Enrichment System Coupled to Online Extraction and Lc–Ms for Molecular‐Level Analysis of Atmospheric Aerosol Organic Matter H. Xiong et al. https://doi.org/10.1002/smtd.202501649
- Preliminary characterization of a single-particle aerosol mass spectrometer with fluorescence pre-selection capability R. Lu et al. https://doi.org/10.1016/j.microc.2026.117981
- Technical note: Determining chemical composition of atmospheric single particles by a standard-free mass calibration algorithm S. Shi et al. https://doi.org/10.5194/acp-24-7001-2024
- Size-dependent airborne metal solubility and associated analytical techniques at bulk and single particle levels: A review Y. Zhao et al. https://doi.org/10.1016/j.atmosenv.2025.121343
- Single-particle decoding of aerosol pollutants size-composition relationships: An interpretable XGBoost-SHAP framework with DTEWD-enhanced SPAMS analysis Y. Ye et al. https://doi.org/10.1016/j.jhazmat.2025.140397
- Design of a wide-particle-size-range aerodynamic injection system with a new pre-focus structure J. Huang et al. https://doi.org/10.5194/amt-18-2739-2025
- Measurement report: The Fifth International Workshop on Ice Nucleation phase 1 (FIN-01): intercomparison of single-particle mass spectrometers X. Shen et al. https://doi.org/10.5194/acp-24-10869-2024
- Chemically Resolved Respiratory Deposition of Ultrafine Particles Characterized by Number Concentration in the Urban Atmosphere J. Zhai et al. https://doi.org/10.1021/acs.est.4c03279
- Integrated Aerosol Collection and Thermal-Desorption Chemical Ionization TOFMS for Rapid Particulate-Composition Analysis Z. Wang et al. https://doi.org/10.1021/acs.analchem.6c00711
Saved (final revised paper)
Latest update: 29 Sep 2026
Short summary
Currently, the limitations of single-particle mass spectrometry detection capabilities render it not yet well suited for analyzing complex aerosol components in low-concentration environments. In this study, a new high-performance single-particle aerosol mass spectrometer (HP-SPAMS) is developed to enhance instrument performance regarding the number of detected particles, transmission efficiency, resolution, and sensitivity, which will help in aerosol science.
Currently, the limitations of single-particle mass spectrometry detection capabilities render it...
