Articles | Volume 17, issue 16
https://doi.org/10.5194/amt-17-4915-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-17-4915-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
27 Aug 2024
Research article |
| 27 Aug 2024
| 27 Aug 2024
A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system
Tianle Pan
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Andrew T. Lambe
Aerodyne Research Inc., Billerica, MA 01821, USA
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Yicong He
Department of Mechanical Engineering, Colorado State University, Fort Collins, CO 80523, USA
now at: State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
Minghao Hu
China–UK Low Carbon College, Shanghai Jiao Tong University, Shanghai 201306, China
Huaishan Zhou
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Xinming Wang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Qingqing Hu
Key Laboratory of Organic Compound Pollution Control Engineering, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China
Hui Chen
Key Laboratory of Organic Compound Pollution Control Engineering, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China
School of Environmental Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China
Yuanlong Huang
Department of Environmental Science and Engineering, California Institute of Technology, Pasadena, CA 91125, USA
Doug R. Worsnop
Aerodyne Research Inc., Billerica, MA 01821, USA
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Cooperative Institute for Research in the Environmental Sciences (CIRES), University of Colorado at Boulder, Boulder, CO 80309, USA
Department of Chemistry, University of Colorado at Boulder, Boulder, CO 80309, USA
Melissa A. Morris
Cooperative Institute for Research in the Environmental Sciences (CIRES), University of Colorado at Boulder, Boulder, CO 80309, USA
Department of Chemistry, University of Colorado at Boulder, Boulder, CO 80309, USA
Douglas A. Day
Cooperative Institute for Research in the Environmental Sciences (CIRES), University of Colorado at Boulder, Boulder, CO 80309, USA
Department of Chemistry, University of Colorado at Boulder, Boulder, CO 80309, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in the Environmental Sciences (CIRES), University of Colorado at Boulder, Boulder, CO 80309, USA
Department of Chemistry, University of Colorado at Boulder, Boulder, CO 80309, USA
Jose-Luis Jimenez
Cooperative Institute for Research in the Environmental Sciences (CIRES), University of Colorado at Boulder, Boulder, CO 80309, USA
Department of Chemistry, University of Colorado at Boulder, Boulder, CO 80309, USA
Shantanu H. Jathar
Department of Mechanical Engineering, Colorado State University, Fort Collins, CO 80523, USA
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Short summary
This study systematically characterizes the temperature enhancement in the lamp-enclosed oxidation flow reactor (OFR). The enhancement varied multiple dimensional factors, emphasizing the complexity of temperature inside of OFR. The effects of temperature on the flow field and gas- or particle-phase reaction inside OFR were also evaluated with experiments and model simulations. Finally, multiple mitigation strategies were demonstrated to minimize this temperature increase.
This study systematically characterizes the temperature enhancement in the lamp-enclosed...
