Articles | Volume 13, issue 11
https://doi.org/10.5194/amt-13-5923-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-13-5923-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
09 Nov 2020
Research article |
| 09 Nov 2020
| 09 Nov 2020
Optimizing the detection, ablation, and ion extraction efficiency of a single-particle laser ablation mass spectrometer for application in environments with low aerosol particle concentrations
Hans-Christian Clemen
Max Planck Institute for Chemistry, Mainz, Germany
Johannes Schneider
CORRESPONDING AUTHOR
Max Planck Institute for Chemistry, Mainz, Germany
Thomas Klimach
Max Planck Institute for Chemistry, Mainz, Germany
Frank Helleis
Max Planck Institute for Chemistry, Mainz, Germany
Franziska Köllner
Max Planck Institute for Chemistry, Mainz, Germany
Andreas Hünig
Max Planck Institute for Chemistry, Mainz, Germany
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
Florian Rubach
Max Planck Institute for Chemistry, Mainz, Germany
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Stephan Mertes
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Heike Wex
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Frank Stratmann
Leibniz Institute for Tropospheric Research, Leipzig, Germany
André Welti
Leibniz Institute for Tropospheric Research, Leipzig, Germany
now at: Finnish Meteorological Institute, Helsinki, Finland
Rebecca Kohl
Institute for Atmospheric and Environmental Sciences, Goethe University, Frankfurt am Main, Germany
Fabian Frank
Institute for Atmospheric and Environmental Sciences, Goethe University, Frankfurt am Main, Germany
Stephan Borrmann
Max Planck Institute for Chemistry, Mainz, Germany
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
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Cited
12 citations as recorded by crossref.
- Atomic spectrometry update – a review of advances in environmental analysis J. Bacon et al. 10.1039/D1JA90054D
- Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques A. Hünig et al. 10.5194/amt-15-2889-2022
- Sources and nature of ice-nucleating particles in the free troposphere at Jungfraujoch in winter 2017 L. Lacher et al. 10.5194/acp-21-16925-2021
- Chemically Resolved Respiratory Deposition of Ultrafine Particles Characterized by Number Concentration in the Urban Atmosphere J. Zhai et al. 10.1021/acs.est.4c03279
- Development of Heterogeneous Ice Nucleation Rate Coefficient Parameterizations From Ambient Measurements G. Cornwell et al. 10.1029/2021GL095359
- Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N J. Schneider et al. 10.5194/acp-21-989-2021
- Technical note: Sea salt interference with black carbon quantification in snow samples using the single particle soot photometer M. Zanatta et al. 10.5194/acp-21-9329-2021
- Design and Simulation of Aerosol Inlet System for Particulate Matter with a Wide Size Range X. Du et al. 10.3390/atmos14040664
- Development and characterization of a high-performance single-particle aerosol mass spectrometer (HP-SPAMS) X. Du et al. 10.5194/amt-17-1037-2024
- Overview: quasi-Lagrangian observations of Arctic air mass transformations – introduction and initial results of the HALO–(𝒜 𝒞)3 aircraft campaign M. Wendisch et al. 10.5194/acp-24-8865-2024
- Measurement report: The Fifth International Workshop on Ice Nucleation phase 1 (FIN-01): intercomparison of single-particle mass spectrometers X. Shen et al. 10.5194/acp-24-10869-2024
- Technical note: Determining chemical composition of atmospheric single particles by a standard-free mass calibration algorithm S. Shi et al. 10.5194/acp-24-7001-2024
12 citations as recorded by crossref.
- Atomic spectrometry update – a review of advances in environmental analysis J. Bacon et al. 10.1039/D1JA90054D
- Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques A. Hünig et al. 10.5194/amt-15-2889-2022
- Sources and nature of ice-nucleating particles in the free troposphere at Jungfraujoch in winter 2017 L. Lacher et al. 10.5194/acp-21-16925-2021
- Chemically Resolved Respiratory Deposition of Ultrafine Particles Characterized by Number Concentration in the Urban Atmosphere J. Zhai et al. 10.1021/acs.est.4c03279
- Development of Heterogeneous Ice Nucleation Rate Coefficient Parameterizations From Ambient Measurements G. Cornwell et al. 10.1029/2021GL095359
- Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N J. Schneider et al. 10.5194/acp-21-989-2021
- Technical note: Sea salt interference with black carbon quantification in snow samples using the single particle soot photometer M. Zanatta et al. 10.5194/acp-21-9329-2021
- Design and Simulation of Aerosol Inlet System for Particulate Matter with a Wide Size Range X. Du et al. 10.3390/atmos14040664
- Development and characterization of a high-performance single-particle aerosol mass spectrometer (HP-SPAMS) X. Du et al. 10.5194/amt-17-1037-2024
- Overview: quasi-Lagrangian observations of Arctic air mass transformations – introduction and initial results of the HALO–(𝒜 𝒞)3 aircraft campaign M. Wendisch et al. 10.5194/acp-24-8865-2024
- Measurement report: The Fifth International Workshop on Ice Nucleation phase 1 (FIN-01): intercomparison of single-particle mass spectrometers X. Shen et al. 10.5194/acp-24-10869-2024
- Technical note: Determining chemical composition of atmospheric single particles by a standard-free mass calibration algorithm S. Shi et al. 10.5194/acp-24-7001-2024
Latest update: 20 Nov 2024
Short summary
We improved the efficiency of a single-particle mass spectrometer with a newly developed aerodynamic lens system, delayed ion extraction, and better electric shielding. The new components result in significantly improved particle analysis and sample statistics. This is particularly important for measurements of low-number-density particles, such as ice-nucleating particles, and for aircraft-based measurements at high altitudes or where high temporal and spatial resolution is required.
We improved the efficiency of a single-particle mass spectrometer with a newly developed...
