Articles | Volume 13, issue 11
https://doi.org/10.5194/amt-13-5923-2020
https://doi.org/10.5194/amt-13-5923-2020
Research article
 | 
09 Nov 2020
Research article |  | 09 Nov 2020

Optimizing the detection, ablation, and ion extraction efficiency of a single-particle laser ablation mass spectrometer for application in environments with low aerosol particle concentrations

Hans-Christian Clemen, Johannes Schneider, Thomas Klimach, Frank Helleis, Franziska Köllner, Andreas Hünig, Florian Rubach, Stephan Mertes, Heike Wex, Frank Stratmann, André Welti, Rebecca Kohl, Fabian Frank, and Stephan Borrmann

Related authors

Overview: Quasi-Lagrangian observations of Arctic air mass transformations – Introduction and initial results of the HALO–(AC)3 aircraft campaign
Manfred Wendisch, Susanne Crewell, André Ehrlich, Andreas Herber, Benjamin Kirbus, Christof Lüpkes, Mario Mech, Steven J. Abel, Elisa F. Akansu, Felix Ament, Clémantyne Aubry, Sebastian Becker, Stephan Borrmann, Heiko Bozem, Marlen Brückner, Hans-Christian Clemen, Sandro Dahlke, Georgios Dekoutsidis, Julien Delanoë, Elena De La Torre Castro, Henning Dorff, Regis Dupuy, Oliver Eppers, Florian Ewald, Geet George, Irina V. Gorodetskaya, Sarah Grawe, Silke Groß, Jörg Hartmann, Silvia Henning, Lutz Hirsch, Evelyn Jäkel, Philipp Joppe, Olivier Jourdan, Zsofia Jurányi, Michail Karalis, Mona Kellermann, Marcus Klingebiel, Michael Lonardi, Johannes Lucke, Anna Luebke, Maximilian Maahn, Nina Maherndl, Marion Maturilli, Bernhard Mayer, Johanna Mayer, Stephan Mertes, Janosch Michaelis, Michel Michalkov, Guillaume Mioche, Manuel Moser, Hanno Müller, Roel Neggers, Davide Ori, Daria Paul, Fiona Paulus, Christian Pilz, Felix Pithan, Mira Pöhlker, Veronika Pörtge, Maximilian Ringel, Nils Risse, Gregory C. Roberts, Sophie Rosenburg, Johannes Röttenbacher, Janna Rückert, Michael Schäfer, Jonas Schäfer, Vera Schemannn, Imke Schirmacher, Jörg Schmidt, Sebastian Schmidt, Johannes Schneider, Sabrina Schnitt, Anja Schwarz, Holger Siebert, Harald Sodemann, Tim Sperzel, Gunnar Spreen, Bjorn Stevens, Frank Stratmann, Gunilla Svensson, Christian Tatzelt, Thomas Tuch, Timo Vihma, Christiane Voigt, Lea Volkmer, Andreas Walbröl, Anna Weber, Birgit Wehner, Bruno Wetzel, Martin Wirth, and Tobias Zinner
EGUsphere, https://doi.org/10.5194/egusphere-2024-783,https://doi.org/10.5194/egusphere-2024-783, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques
Andreas Hünig, Oliver Appel, Antonis Dragoneas, Sergej Molleker, Hans-Christian Clemen, Frank Helleis, Thomas Klimach, Franziska Köllner, Thomas Böttger, Frank Drewnick, Johannes Schneider, and Stephan Borrmann
Atmos. Meas. Tech., 15, 2889–2921, https://doi.org/10.5194/amt-15-2889-2022,https://doi.org/10.5194/amt-15-2889-2022, 2022
Short summary
Sources and nature of ice-nucleating particles in the free troposphere at Jungfraujoch in winter 2017
Larissa Lacher, Hans-Christian Clemen, Xiaoli Shen, Stephan Mertes, Martin Gysel-Beer, Alireza Moallemi, Martin Steinbacher, Stephan Henne, Harald Saathoff, Ottmar Möhler, Kristina Höhler, Thea Schiebel, Daniel Weber, Jann Schrod, Johannes Schneider, and Zamin A. Kanji
Atmos. Chem. Phys., 21, 16925–16953, https://doi.org/10.5194/acp-21-16925-2021,https://doi.org/10.5194/acp-21-16925-2021, 2021
Short summary
Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N
Johannes Schneider, Ralf Weigel, Thomas Klimach, Antonis Dragoneas, Oliver Appel, Andreas Hünig, Sergej Molleker, Franziska Köllner, Hans-Christian Clemen, Oliver Eppers, Peter Hoppe, Peter Hoor, Christoph Mahnke, Martina Krämer, Christian Rolf, Jens-Uwe Grooß, Andreas Zahn, Florian Obersteiner, Fabrizio Ravegnani, Alexey Ulanovsky, Hans Schlager, Monika Scheibe, Glenn S. Diskin, Joshua P. DiGangi, John B. Nowak, Martin Zöger, and Stephan Borrmann
Atmos. Chem. Phys., 21, 989–1013, https://doi.org/10.5194/acp-21-989-2021,https://doi.org/10.5194/acp-21-989-2021, 2021
Short summary
Application of an O-ring pinch device as a constant-pressure inlet (CPI) for airborne sampling
Sergej Molleker, Frank Helleis, Thomas Klimach, Oliver Appel, Hans-Christian Clemen, Antonis Dragoneas, Christian Gurk, Andreas Hünig, Franziska Köllner, Florian Rubach, Christiane Schulz, Johannes Schneider, and Stephan Borrmann
Atmos. Meas. Tech., 13, 3651–3660, https://doi.org/10.5194/amt-13-3651-2020,https://doi.org/10.5194/amt-13-3651-2020, 2020
Short summary

Related subject area

Subject: Aerosols | Technique: In Situ Measurement | Topic: Instruments and Platforms
Modular Multiplatform Compatible Air Measurement System (MoMuCAMS): a new modular platform for boundary layer aerosol and trace gas vertical measurements in extreme environments
Roman Pohorsky, Andrea Baccarini, Julie Tolu, Lenny H. E. Winkel, and Julia Schmale
Atmos. Meas. Tech., 17, 731–754, https://doi.org/10.5194/amt-17-731-2024,https://doi.org/10.5194/amt-17-731-2024, 2024
Short summary
Two new multirotor uncrewed aerial vehicles (UAVs) for glaciogenic cloud seeding and aerosol measurements within the CLOUDLAB project
Anna J. Miller, Fabiola Ramelli, Christopher Fuchs, Nadja Omanovic, Robert Spirig, Huiying Zhang, Ulrike Lohmann, Zamin A. Kanji, and Jan Henneberger
Atmos. Meas. Tech., 17, 601–625, https://doi.org/10.5194/amt-17-601-2024,https://doi.org/10.5194/amt-17-601-2024, 2024
Short summary
Real-time pollen identification using holographic imaging and fluorescence measurements
Sophie Erb, Elias Graf, Yanick Zeder, Simone Lionetti, Alexis Berne, Bernard Clot, Gian Lieberherr, Fiona Tummon, Pascal Wullschleger, and Benoît Crouzy
Atmos. Meas. Tech., 17, 441–451, https://doi.org/10.5194/amt-17-441-2024,https://doi.org/10.5194/amt-17-441-2024, 2024
Short summary
Assessing potential indicators of aerosol wet scavenging during long-range transport
Miguel Ricardo A. Hilario, Avelino F. Arellano, Ali Behrangi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Michael A. Shook, Luke D. Ziemba, and Armin Sorooshian
Atmos. Meas. Tech., 17, 37–55, https://doi.org/10.5194/amt-17-37-2024,https://doi.org/10.5194/amt-17-37-2024, 2024
Short summary
Next-generation ice-nucleating particle sampling on board aircraft: characterization of the High-volume flow aERosol particle filter sAmpler (HERA)
Sarah Grawe, Conrad Jentzsch, Jonas Schaefer, Heike Wex, Stephan Mertes, and Frank Stratmann
Atmos. Meas. Tech., 16, 4551–4570, https://doi.org/10.5194/amt-16-4551-2023,https://doi.org/10.5194/amt-16-4551-2023, 2023
Short summary

Cited articles

Adler, G., Koop, T., Haspel, C., Taraniuk, I., Moise, T., Koren, I., Heiblum, R. H., and Rudich, Y.: Formation of Highly Porous Aerosol Particles by Atmospheric Freeze-Drying in Ice Clouds, P. Natl. Acad. Sci. USA, 110, 20414–20419, https://doi.org/10.1073/pnas.1317209110, 2013. a
Amoruso, S., Armenante, M., Berardi, V., Bruzzese, R., Velotta, R., and Wang, X.: High Fluence Visible and Ultraviolet Laser Ablation of Metallic Targets, Appl. Surf. Sci., 127–129, 1017–1022, https://doi.org/10.1016/S0169-4332(97)00786-1, 1998. a
Augustin, S., Wex, H., Niedermeier, D., Pummer, B., Grothe, H., Hartmann, S., Tomsche, L., Clauss, T., Voigtländer, J., Ignatius, K., and Stratmann, F.: Immersion freezing of birch pollen washing water, Atmos. Chem. Phys., 13, 10989–11003, https://doi.org/10.5194/acp-13-10989-2013, 2013. a
Augustin-Bauditz, S., Wex, H., Kanter, S., Ebert, M., Niedermeier, D., Stolz, F., Prager, A., and Stratmann, F.: The Immersion Mode Ice Nucleation Behavior of Mineral Dusts: A Comparison of Different Pure and Surface Modified Dusts, Geophys. Res. Lett., 41, 7375–7382, https://doi.org/10.1002/2014GL061317, 2014. a
Baustian, K. J., Cziczo, D. J., Wise, M. E., Pratt, K. A., Kulkarni, G., Hallar, A. G., and Tolbert, M. A.: Importance of Aerosol Composition, Mixing State, and Morphology for Heterogeneous Ice Nucleation: A Combined Field and Laboratory Approach, J. Geophys. Res.-Atmos., 117, D06217, https://doi.org/10.1029/2011JD016784, 2012. a
Download
Short summary
We improved the efficiency of a single-particle mass spectrometer with a newly developed aerodynamic lens system, delayed ion extraction, and better electric shielding. The new components result in significantly improved particle analysis and sample statistics. This is particularly important for measurements of low-number-density particles, such as ice-nucleating particles, and for aircraft-based measurements at high altitudes or where high temporal and spatial resolution is required.