Optimizing the detection, ablation, and ion extraction efficiency of a single-particle laser ablation mass spectrometer for application in environments with low aerosol particle concentrations

Clemen, Hans-Christian; Schneider, Johannes; Klimach, Thomas; Helleis, Frank; Köllner, Franziska; Hünig, Andreas; Rubach, Florian; Mertes, Stephan; Wex, Heike; Stratmann, Frank; Welti, André; Kohl, Rebecca; Frank, Fabian; Borrmann, Stephan

doi:https://doi.org/10.5194/amt-13-5923-2020

Articles | Volume 13, issue 11

https://doi.org/10.5194/amt-13-5923-2020

© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

https://doi.org/10.5194/amt-13-5923-2020

© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Articles | Volume 13, issue 11

Research article

|

09 Nov 2020

Research article |

| 09 Nov 2020

Optimizing the detection, ablation, and ion extraction efficiency of a single-particle laser ablation mass spectrometer for application in environments with low aerosol particle concentrations

Hans-Christian Clemen, Johannes Schneider, Thomas Klimach, Frank Helleis, Franziska Köllner, Andreas Hünig, Florian Rubach, Stephan Mertes, Heike Wex, Frank Stratmann, André Welti, Rebecca Kohl, Fabian Frank, and Stephan Borrmann

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Final revised paper (published on 09 Nov 2020)
Supplement to the final revised paper
Preprint (discussion started on 23 Jun 2020)
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Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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RC1: 'Referee comments', Giuseppe Petrucci, 09 Jul 2020
- AC1: 'Replies to the Referee Professor Giuseppe Petrucci', Hans-Christian Clemen, 15 Sep 2020
RC2: 'Referee Comment', Anonymous Referee #2, 25 Jul 2020
- AC2: 'Replies to Referee 2', Hans-Christian Clemen, 15 Sep 2020

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Hans-Christian Clemen on behalf of the Authors (15 Sep 2020) Author's response Manuscript

ED: Publish as is (23 Sep 2020) by Pierre Herckes

Short summary

We improved the efficiency of a single-particle mass spectrometer with a newly developed aerodynamic lens system, delayed ion extraction, and better electric shielding. The new components result in significantly improved particle analysis and sample statistics. This is particularly important for measurements of low-number-density particles, such as ice-nucleating particles, and for aircraft-based measurements at high altitudes or where high temporal and spatial resolution is required.