Articles | Volume 15, issue 14 
            
                
                    
            
            
            https://doi.org/10.5194/amt-15-4195-2022
                    © Author(s) 2022. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-15-4195-2022
                    © Author(s) 2022. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
Automated identification of local contamination in remote atmospheric composition time series
Ivo Beck
CORRESPONDING AUTHOR
                                            
                                    
                                            Extreme Environments Research Laboratory, École Polytechnique Fédérale de Lausanne, Sion, Switzerland
                                        
                                    Hélène Angot
                                            Extreme Environments Research Laboratory, École Polytechnique Fédérale de Lausanne, Sion, Switzerland
                                        
                                    Andrea Baccarini
                                            Extreme Environments Research Laboratory, École Polytechnique Fédérale de Lausanne, Sion, Switzerland
                                        
                                    Lubna Dada
                                            Extreme Environments Research Laboratory, École Polytechnique Fédérale de Lausanne, Sion, Switzerland
                                        
                                    Lauriane Quéléver
                                            Institute for Atmospheric and Earth System Research, INAR/Physics, 00014 University of Helsinki, Helsinki, Finland
                                        
                                    Tuija Jokinen
                                            Institute for Atmospheric and Earth System Research, INAR/Physics, 00014 University of Helsinki, Helsinki, Finland
                                        
                                    
                                            Climate & Atmosphere Research Centre (CARE-C), The Cyprus Institute, P.O. Box 27456, Nicosia, 1645, Cyprus
                                        
                                    Tiia Laurila
                                            Institute for Atmospheric and Earth System Research, INAR/Physics, 00014 University of Helsinki, Helsinki, Finland
                                        
                                    Markus Lampimäki
                                            Institute for Atmospheric and Earth System Research, INAR/Physics, 00014 University of Helsinki, Helsinki, Finland
                                        
                                    Nicolas Bukowiecki
                                            Atmospheric Sciences, Department of Environmental Sciences, University of Basel, Basel, Switzerland
                                        
                                    Matthew Boyer
                                            Institute for Atmospheric and Earth System Research, INAR/Physics, 00014 University of Helsinki, Helsinki, Finland
                                        
                                    Xianda Gong
                                            Center for Aerosol Science and Engineering, Department of Energy, Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis, MO, USA
                                        
                                    Martin Gysel-Beer
                                            Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland
                                        
                                    Tuukka Petäjä
                                            Institute for Atmospheric and Earth System Research, INAR/Physics, 00014 University of Helsinki, Helsinki, Finland
                                        
                                    Jian Wang
                                            Center for Aerosol Science and Engineering, Department of Energy, Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis, MO, USA
                                        
                                    
                                            Extreme Environments Research Laboratory, École Polytechnique Fédérale de Lausanne, Sion, Switzerland
                                        
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                            Cited
22 citations as recorded by crossref.
- Year-round trace gas measurements in the central Arctic during the MOSAiC expedition H. Angot et al. 10.1038/s41597-022-01769-6
 - Arctic warming by abundant fine sea salt aerosols from blowing snow X. Gong et al. 10.1038/s41561-023-01254-8
 - Ice nucleating particle sources and transports between the Central and Southern Arctic regions during winter cold air outbreaks P. DeMott et al. 10.1525/elementa.2024.00063
 - Observations of high-time-resolution and size-resolved aerosol chemical composition and microphysics in the central Arctic: implications for climate-relevant particle properties B. Heutte et al. 10.5194/acp-25-2207-2025
 - Widespread detection of chlorine oxyacids in the Arctic atmosphere Y. Tham et al. 10.1038/s41467-023-37387-y
 - A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition M. Boyer et al. 10.5194/acp-23-389-2023
 - A central arctic extreme aerosol event triggered by a warm air-mass intrusion L. Dada et al. 10.1038/s41467-022-32872-2
 - An Arctic Marine Source of Fluorescent Primary Biological Aerosol Particles During the Transition from Summer to Autumn at the North Pole J. Kojoj et al. 10.16993/tellusb.1880
 - Characteristics and effects of aerosols during blowing snow events in the central Arctic N. Bergner et al. 10.1525/elementa.2024.00047
 - Measurement report: Wintertime aerosol characterization at an urban traffic site in Helsinki, Finland K. Teinilä et al. 10.5194/acp-25-4907-2025
 - Links between atmospheric aerosols and sea state in the Arctic Ocean A. Moallemi et al. 10.1016/j.atmosenv.2024.120844
 - Organic aerosols in the inland Tibetan Plateau: New insights from molecular tracers X. Wan et al. 10.1016/j.scitotenv.2023.163797
 - Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget J. Barten et al. 10.1525/elementa.2022.00086
 - Measurements of aerosol microphysical and chemical properties in the central Arctic atmosphere during MOSAiC B. Heutte et al. 10.1038/s41597-023-02586-1
 - Particle flux–gradient relationships in the high Arctic: emission and deposition patterns across three surface types T. Mathes et al. 10.5194/acp-25-8455-2025
 - The annual cycle and sources of relevant aerosol precursor vapors in the central Arctic during the MOSAiC expedition M. Boyer et al. 10.5194/acp-24-12595-2024
 - Characteristics and sources of fluorescent aerosols in the central Arctic Ocean I. Beck et al. 10.1525/elementa.2023.00125
 - Direct observation of Arctic Sea salt aerosol production from blowing snow and modeling over a changing sea ice environment A. Ranjithkumar et al. 10.1525/elementa.2024.00006
 - Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause A. Ansmann et al. 10.5194/acp-23-12821-2023
 - Highly Hygroscopic Aerosols Facilitate Summer and Early‐Autumn Cloud Formation at Extremely Low Concentrations Over the Central Arctic Ocean P. Duplessis et al. 10.1029/2023JD039159
 - The Marginal Ice Zone as a dominant source region of atmospheric mercury during central Arctic summertime F. Yue et al. 10.1038/s41467-023-40660-9
 - Sources and Composition of Organic Aerosols in the Central Arctic during Spring and Summer B. Heutte et al. 10.1021/acs.est.5c09788
 
22 citations as recorded by crossref.
- Year-round trace gas measurements in the central Arctic during the MOSAiC expedition H. Angot et al. 10.1038/s41597-022-01769-6
 - Arctic warming by abundant fine sea salt aerosols from blowing snow X. Gong et al. 10.1038/s41561-023-01254-8
 - Ice nucleating particle sources and transports between the Central and Southern Arctic regions during winter cold air outbreaks P. DeMott et al. 10.1525/elementa.2024.00063
 - Observations of high-time-resolution and size-resolved aerosol chemical composition and microphysics in the central Arctic: implications for climate-relevant particle properties B. Heutte et al. 10.5194/acp-25-2207-2025
 - Widespread detection of chlorine oxyacids in the Arctic atmosphere Y. Tham et al. 10.1038/s41467-023-37387-y
 - A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition M. Boyer et al. 10.5194/acp-23-389-2023
 - A central arctic extreme aerosol event triggered by a warm air-mass intrusion L. Dada et al. 10.1038/s41467-022-32872-2
 - An Arctic Marine Source of Fluorescent Primary Biological Aerosol Particles During the Transition from Summer to Autumn at the North Pole J. Kojoj et al. 10.16993/tellusb.1880
 - Characteristics and effects of aerosols during blowing snow events in the central Arctic N. Bergner et al. 10.1525/elementa.2024.00047
 - Measurement report: Wintertime aerosol characterization at an urban traffic site in Helsinki, Finland K. Teinilä et al. 10.5194/acp-25-4907-2025
 - Links between atmospheric aerosols and sea state in the Arctic Ocean A. Moallemi et al. 10.1016/j.atmosenv.2024.120844
 - Organic aerosols in the inland Tibetan Plateau: New insights from molecular tracers X. Wan et al. 10.1016/j.scitotenv.2023.163797
 - Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget J. Barten et al. 10.1525/elementa.2022.00086
 - Measurements of aerosol microphysical and chemical properties in the central Arctic atmosphere during MOSAiC B. Heutte et al. 10.1038/s41597-023-02586-1
 - Particle flux–gradient relationships in the high Arctic: emission and deposition patterns across three surface types T. Mathes et al. 10.5194/acp-25-8455-2025
 - The annual cycle and sources of relevant aerosol precursor vapors in the central Arctic during the MOSAiC expedition M. Boyer et al. 10.5194/acp-24-12595-2024
 - Characteristics and sources of fluorescent aerosols in the central Arctic Ocean I. Beck et al. 10.1525/elementa.2023.00125
 - Direct observation of Arctic Sea salt aerosol production from blowing snow and modeling over a changing sea ice environment A. Ranjithkumar et al. 10.1525/elementa.2024.00006
 - Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause A. Ansmann et al. 10.5194/acp-23-12821-2023
 - Highly Hygroscopic Aerosols Facilitate Summer and Early‐Autumn Cloud Formation at Extremely Low Concentrations Over the Central Arctic Ocean P. Duplessis et al. 10.1029/2023JD039159
 - The Marginal Ice Zone as a dominant source region of atmospheric mercury during central Arctic summertime F. Yue et al. 10.1038/s41467-023-40660-9
 - Sources and Composition of Organic Aerosols in the Central Arctic during Spring and Summer B. Heutte et al. 10.1021/acs.est.5c09788
 
Latest update: 03 Nov 2025
Short summary
            We present the pollution detection algorithm (PDA), a new method to identify local primary pollution in remote atmospheric aerosol and trace gas time series. The PDA identifies periods of contaminated data and relies only on the target dataset itself; i.e., it is independent of ancillary data such as meteorological variables. The parameters of all pollution identification steps are adjustable so that the PDA can be tuned to different locations and situations. It is available as open-access code.
            We present the pollution detection algorithm (PDA), a new method to identify local primary...