Articles | Volume 19, issue 15
https://doi.org/10.5194/amt-19-5243-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-19-5243-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Evaluation of DMSO as working fluid in condensation particle counters
Sarah Kirchhoff
CORRESPONDING AUTHOR
Institute of Climate and Energy Systems – Troposphere (ICE-3), Forschungszentrum Jülich GmbH, Jülich, Germany
Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany
Institute of Climate and Energy Systems – Troposphere (ICE-3), Forschungszentrum Jülich GmbH, Jülich, Germany
Oliver F. Bischof
Institute of Climate and Energy Systems – Troposphere (ICE-3), Forschungszentrum Jülich GmbH, Jülich, Germany
TSI GmbH, Particle Instruments, Aachen, Germany
Gerhard Steiner
GRIMM Aerosol Technik Ainring GmbH, Ainring, Germany
Christian Kunath
GRIMM Aerosol Technik Ainring GmbH, Ainring, Germany
Lothar Keck
GRIMM Aerosol Technik Ainring GmbH, Ainring, Germany
Victoria M. Fruhmann
Institute of Electrical Measurement and Sensor Systems, Graz University of Technology, Graz, Austria
Helmut Krasa
Institute of Electrical Measurement and Sensor Systems, Graz University of Technology, Graz, Austria
now at: AVL DiTEST GmbH, Graz, Austria
Alexander Bergmann
Institute of Electrical Measurement and Sensor Systems, Graz University of Technology, Graz, Austria
Andreas Petzold
Institute of Climate and Energy Systems – Troposphere (ICE-3), Forschungszentrum Jülich GmbH, Jülich, Germany
Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany
Ulrich Bundke
Institute of Climate and Energy Systems – Troposphere (ICE-3), Forschungszentrum Jülich GmbH, Jülich, Germany
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J. Sens. Sens. Syst., 15, 1–8, https://doi.org/10.5194/jsss-15-1-2026, https://doi.org/10.5194/jsss-15-1-2026, 2026
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Sara Arriolabengoa, Pierre Crispel, Olivier Jaron, Yves Bouteloup, Benoît Vié, Yun Li, Andreas Petzold, and Matthieu Plu
Atmos. Chem. Phys., 25, 18051–18076, https://doi.org/10.5194/acp-25-18051-2025, https://doi.org/10.5194/acp-25-18051-2025, 2025
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Patrick Konjari, Christian Rolf, Martina Krämer, Armin Afchine, Nicole Spelten, Irene Bartolome Garcia, Annette Miltenberger, Nicolas Emig, Philipp Joppe, Johannes Schneider, Yun Li, Andreas Petzold, Heiko Bozem, and Peter Hoor
Atmos. Chem. Phys., 25, 18031–18050, https://doi.org/10.5194/acp-25-18031-2025, https://doi.org/10.5194/acp-25-18031-2025, 2025
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Heiko Bozem, Philipp Joppe, Yun Li, Nicolas Emig, Armin Afchine, Anna Breuninger, Joachim Curtius, Stefan Hofmann, Sadath Ismayil, Konrad Kandler, Daniel Kunkel, Arthur Kutschka, Hans-Christoph Lachnitt, Andreas Petzold, Sarah Richter, Timo Röschenthaler, Christian Rolf, Lisa Schneider, Johannes Schneider, Alexander Vogel, and Peter Hoor
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Nicolas Emig, Annette K. Miltenberger, Peter M. Hoor, and Andreas Petzold
Atmos. Chem. Phys., 25, 13077–13101, https://doi.org/10.5194/acp-25-13077-2025, https://doi.org/10.5194/acp-25-13077-2025, 2025
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Herman G. J. Smit, Torben Galle, Romain Blot, Florian Obersteiner, Philippe Nédélec, Andreas Zahn, Jean-Marc Cousin, Ulrich Bundke, Andreas Petzold, Valerie Thouret, and Hannah Clark
Atmos. Meas. Tech., 18, 4985–5001, https://doi.org/10.5194/amt-18-4985-2025, https://doi.org/10.5194/amt-18-4985-2025, 2025
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Preprint archived
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Andreas Petzold, Ulrich Bundke, Anca Hienola, Paolo Laj, Cathrine Lund Myhre, Alex Vermeulen, Angeliki Adamaki, Werner Kutsch, Valerie Thouret, Damien Boulanger, Markus Fiebig, Markus Stocker, Zhiming Zhao, and Ari Asmi
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Atmos. Meas. Tech., 17, 2481–2505, https://doi.org/10.5194/amt-17-2481-2024, https://doi.org/10.5194/amt-17-2481-2024, 2024
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Alexander Schossmann, Michael Töfferl, Christoph Schmidt, and Alexander Bergmann
J. Sens. Sens. Syst., 13, 31–39, https://doi.org/10.5194/jsss-13-31-2024, https://doi.org/10.5194/jsss-13-31-2024, 2024
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Yann Cohen, Didier Hauglustaine, Bastien Sauvage, Susanne Rohs, Patrick Konjari, Ulrich Bundke, Andreas Petzold, Valérie Thouret, Andreas Zahn, and Helmut Ziereis
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The upper troposphere–lower stratosphere (UTLS) is a key region regarding the lower atmospheric composition. This study consists of a comprehensive evaluation of an up-to-date chemistry–climate model in this layer, using regular in situ measurements based on passenger aircraft. For this purpose, a specific software (Interpol-IAGOS) has been updated and made publicly available. The model reproduces the carbon monoxide peaks due to biomass burning over the continental tropics particularly well.
Patrick Weber, Oliver F. Bischof, Benedikt Fischer, Marcel Berg, Susanne Hering, Steven Spielman, Gregory Lewis, Andreas Petzold, and Ulrich Bundke
Atmos. Meas. Tech., 16, 3505–3514, https://doi.org/10.5194/amt-16-3505-2023, https://doi.org/10.5194/amt-16-3505-2023, 2023
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This study tests the new water condensation particle counter (MAGIC 210-LP) for deployment on passenger aircraft coordinated by the European research infrastructure IAGOS. We conducted a series of laboratory experiments for flight altitude conditions. We demonstrate that this water condensation particle counter model shows excellent agreement with a butanol-based instrument used in parallel and a Faraday cup electrometer as reference instrument at all tested pressure conditions.
Patrick Weber, Oliver F. Bischof, Benedikt Fischer, Marcel Berg, Jannik Schmitt, Gerhard Steiner, Lothar Keck, Andreas Petzold, and Ulrich Bundke
Aerosol Research, 1, 1–12, https://doi.org/10.5194/ar-1-1-2023, https://doi.org/10.5194/ar-1-1-2023, 2023
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The aerosol number concentration is essential information for aerosol science. A condensation particle counter (CPC) can robustly provide this information. Butanol is often used as a working fluid in a CPC. We could show that dimethyl sulfoxide (DMSO) behaves equivalently to butanol in terms of the instrument`s counting efficiency, cut-off diameter and concentration linearity. We tested this on different aerosols, including sodium chloride, ammonium sulfate and fresh combustion soot.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
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The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Markus Leiminger, Lukas Fischer, Sophia Brilke, Julian Resch, Paul Martin Winkler, Armin Hansel, and Gerhard Steiner
Atmos. Meas. Tech., 15, 3705–3720, https://doi.org/10.5194/amt-15-3705-2022, https://doi.org/10.5194/amt-15-3705-2022, 2022
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We developed an axial ion mobility classifier coupled to an atmospheric-pressure interface time-of-flight (APi-TOF) mass spectrometer to measure size-segregated atmospheric ions. We characterize the performance of the novel instrument with bipolar-electrospray-generated ion mobility standards and compare the results with CFD simulations and a simplified numerical particle-tracking model. Ultimately, we report first mass–mobility measurements of atmospheric ions in Innsbruck, Austria.
Patrick Weber, Andreas Petzold, Oliver F. Bischof, Benedikt Fischer, Marcel Berg, Andrew Freedman, Timothy B. Onasch, and Ulrich Bundke
Atmos. Meas. Tech., 15, 3279–3296, https://doi.org/10.5194/amt-15-3279-2022, https://doi.org/10.5194/amt-15-3279-2022, 2022
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In our laboratory closure study, we measured the full set of aerosol optical properties for different light-absorbing aerosols using a set of instruments.
Our key finding is that the extensive and intensive aerosol optical properties obtained agree with data from reference instruments, except the absorption Ångström exponent of externally mixed aerosols. The reported uncertainty in the single-scattering albedo fulfils the defined goals for Global Climate Observing System applications of 10 %.
Ajit Ahlawat, Kay Weinhold, Jesus Marval, Paolo Tronville, Ari Leskinen, Mika Komppula, Holger Gerwig, Lars Gerling, Stephan Weber, Rikke Bramming Jørgensen, Thomas Nørregaard Jensen, Marouane Merizak, Ulrich Vogt, Carla Ribalta, Mar Viana, Andre Schmitz, Maria Chiesa, Giacomo Gerosa, Lothar Keck, Markus Pesch, Gerhard Steiner, Thomas Krinke, Torsten Tritscher, Wolfram Birmili, and Alfred Wiedensohler
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-155, https://doi.org/10.5194/amt-2022-155, 2022
Revised manuscript not accepted
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Measurements of ultrafine particles must be done with quality-assured instruments. The performance of portable instruments such as NanoScan SMPS, and GRIMM Mini WRAS spectrometer measuring the particle number size distribution in the range from 10 to 200 nm were investigated. The influence of different aerosol types and maintenance activities on these instruments were explored. The results show that these portable instruments are suitable for mobile UFP measurements for source identification.
Martin J. Osborne, Johannes de Leeuw, Claire Witham, Anja Schmidt, Frances Beckett, Nina Kristiansen, Joelle Buxmann, Cameron Saint, Ellsworth J. Welton, Javier Fochesatto, Ana R. Gomes, Ulrich Bundke, Andreas Petzold, Franco Marenco, and Jim Haywood
Atmos. Chem. Phys., 22, 2975–2997, https://doi.org/10.5194/acp-22-2975-2022, https://doi.org/10.5194/acp-22-2975-2022, 2022
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Using the Met Office NAME dispersion model, supported by satellite- and ground-based remote-sensing observations, we describe the dispersion of aerosols from the 2019 Raikoke eruption and the concurrent wildfires in Alberta Canada. We show how the synergy of dispersion modelling and multiple observation sources allowed observers in the London VAAC to arrive at a more complete picture of the aerosol loading at altitudes commonly used by aviation.
Hannah Clark, Yasmine Bennouna, Maria Tsivlidou, Pawel Wolff, Bastien Sauvage, Brice Barret, Eric Le Flochmoën, Romain Blot, Damien Boulanger, Jean-Marc Cousin, Philippe Nédélec, Andreas Petzold, and Valérie Thouret
Atmos. Chem. Phys., 21, 16237–16256, https://doi.org/10.5194/acp-21-16237-2021, https://doi.org/10.5194/acp-21-16237-2021, 2021
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We examined 27 years of IAGOS (In-service Aircraft for a Global Observing System) profiles at Frankfurt to see if there were unusual features during the spring of 2020 related to COVID-19 lockdowns in Europe. Increased ozone near the surface was partly linked to the reduction in emissions. Carbon monoxide decreased near the surface, but the impact of the lockdowns was offset by polluted air masses from elsewhere. There were small reductions in ozone and carbon monoxide in the free troposphere.
Cited articles
Aalto, P., Hämeri, K., Paatero, P., Kulmala, M., Bellander, T., Berglind, N., Bouso, L., Castaño-Vinyals, G., Sunyer, J., Cattani, G., Marconi, A., Cyrys, J., von Klot, S., Peters, A., Zetzsche, K., Lanki, T., Pekkanen, J., Nyberg, F., Sjövall, B., and Forastiere, F.: Aerosol Particle Number Concentration Measurements in Five European Cities Using TSI-3022 Condensation Particle Counter over a Three-Year Period during Health Effects of Air Pollution on Susceptible Subpopulations, J. Air Waste Manage., 55, 1064–1076, https://doi.org/10.1080/10473289.2005.10464702, 2005. a
Alam, A., Shi, J. P., and Harrison, R. M.: Observations of new particle formation in urban air, J. Geophys. Res.-Atmos., 108, https://doi.org/10.1029/2001JD001417, 2003. a
Astbury, G. R., Bugand-Bugandet, J., Grollet, E., and Stell, K. M.: Flash points of aqueous solutions of flammable solvents, Institution of Chemical Engineers, Symposium Series, 150, https://api.semanticscholar.org/ (last access: 4 June 2026), 2004. a
Balendra, S., Kale, A., Pongetti, J., Kazemimanesh, M., Haugen, M., Weller, L., and Boies, A.: Condensation particle counters: Exploring the limits of miniaturisation, J. Aerosol Sci., 175, 106266, https://doi.org/10.1016/j.jaerosci.2023.106266, 2024. a
Bauer, P. S., Spät, D., Eisenhut, M., Gattringer, A., and Weinzierl, B.: Pressure-dependent performance of two CEN-specified condensation particle counters, Atmos. Meas. Tech., 16, 4445–4460, https://doi.org/10.5194/amt-16-4445-2023, 2023. a, b, c, d
Bezantakos, S. and Biskos, G.: Temperature and pressure effects on the performance of the portable TSI 3007 condensation particle counter: Implications on ground and aerial observations, J. Aerosol Sci., 159, 105877, https://doi.org/10.1016/j.jaerosci.2021.105877, 2022. a, b, c
Bischof, O. F.: Application-specific calibration of condensation particle counters under low pressure conditions: = Anwendungsspezifische Kalibrierung von Kondensationspartikelzählern unter Niederdruckbedingungen, in: Schriften des Forschungszentrums Jülich Reihe Energie und Umwelt, Bd./vol. 579, energy and environment, Forschungszentrum Jülich GmbH, Zentralbibliothek, Verlag, Aachen, ISBN 978-3-95806-629-8, 2022. a, b, c, d, e, f
Brock, C. A., Schröder, F., Kärcher, B., Petzold, A., Busen, R., and Fiebig, M.: Ultrafine particle size distributions measured in aircraft exhaust plumes, J. Geophys. Res., 105, 26555–26568, https://doi.org/10.1029/2000JD900360, 2000. a
Bundke, U., Berg, M., Houben, N., Ibrahim, A., Fiebig, M., Tettich, F., Klaus, C., Franke, H., and Petzold, A.: The IAGOS-CORE aerosol package: instrument design, operation and performance for continuous measurement aboard in-service aircraft, Tellus B, 67, 28339, https://doi.org/10.3402/tellusb.v67.28339, 2015. a, b, c, d, e, f, g, h, i, j
Cozic, J., Verheggen, B., Mertes, S., Connolly, P., Bower, K., Petzold, A., Baltensperger, U., and Weingartner, E.: Scavenging of black carbon in mixed phase clouds at the high alpine site Jungfraujoch, Atmos. Chem. Phys., 7, 1797–1807, https://doi.org/10.5194/acp-7-1797-2007, 2007 a
Gao, R. S., Telg, H., McLaughlin, R. J., Ciciora, S. J., Watts, L. A., Richardson, M. S., Schwarz, J. P., Perring, A. E., Thornberry, T. D., Rollins, A. W., Markovic, M. Z., Bates, T. S., Johnson, J. E., and Fahey, D. W.: A light-weight, high-sensitivity particle spectrometer for PM2.5 aerosol measurements, Aerosol Sci. Tech., 50, 88–99, 2016. a
Hao, W., Stolzenburg, M., Attoui, M., Zhang, J., and Wang, Y.: Optimizing the activation efficiency of sub-3 nm particles in a laminar flow condensation particle counter: Model simulation, J. Aerosol Sci., 158, 105841, https://doi.org/10.1016/j.jaerosci.2021.105841, 2021. a
Havemeyer, R. N.: Freezing Point Curve of Dimethyl Sulfoxide–Water Solutions, J. Pharm. Sci., 55, 851–853, https://doi.org/10.1002/jps.2600550822, 1966. a
Hering, S. V., Spielman, S. R., and Lewis, G. S.: Moderated, Water-Based, Condensational Particle Growth in a Laminar Flow, Aerosol Sci. Tech., 48, 401–408, https://doi.org/10.1080/02786826.2014.881460, 2014. a
Hong, A. C., Young, C. J., Hurley, M. D., Wallington, T. J., and Mabury, S. A.: Perfluorotributylamine: A novel long-lived greenhouse gas, Geophys. Res. Lett., 40, 6010–6015, https://doi.org/10.1002/2013GL058010, 2013. a
IPCC: Climate Change 2021: The Physical Science Basis, Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, United Kingdom, and New York, NY, USA, https://doi.org/10.1017/9781009157896, 2021. a, b
Jarrett, D. G. and Owen, M. C.: Traceability for Aerosol Electrometer in the fA Range, Instrumentation Viewpoint, 14, 17, https://doi.org/10.5821/iwp.2013.14.15417, 2013. a
Jurányi, Z., Gysel, M., Weingartner, E., DeCarlo, P. F., Kammermann, L., and Baltensperger, U.: Measured and modelled cloud condensation nuclei number concentration at the high alpine site Jungfraujoch, Atmos. Chem. Phys., 10, 7891–7906, https://doi.org/10.5194/acp-10-7891-2010, 2010. a
Kahn, R. A., Andrews, E., Brock, C. A., Chin, M., Feingold, G., Gettelman, A., Levy, R. C., Murphy, D. M., Nenes, A., Pierce, J. R., Popp, T., Redemann, J., Sayer, A. M., Da Silva, A. M., Sogacheva, L., and Stier, P.: Reducing Aerosol Forcing Uncertainty by Combining Models With Satellite and Within-The-Atmosphere Observations: A Three-Way Street, Rev. Geophys., 61, e2022RG000796, https://doi.org/10.1029/2022RG000796, 2023. a
Kim, W. Y., Lee, S. G., Lee, H., and Ahn, K.-H.: Investigation of Vertical Profiles of Particulate Matter and Meteorological Variables up to 2.5 km in Altitude Using a Drone-Based Monitoring System, Atmosphere, 16, 93, https://doi.org/10.3390/atmos16010093, 2025. a
Krasa, H., Fruhmann, V. M., Schurl, S., Kupper, M., and Bergmann, A.: Condensation diffusion charging – particle number measurement of high concentrations down to 3 nm, Aerosol Research, 3, 521–534, https://doi.org/10.5194/ar-3-521-2025, 2025. a, b
Kulkarni, P., Baron, P. A., and Willeke, K.: Aerosol Measurement: Principles, Techniques, and Applications, 3rd edn., John Wiley & Sons Ltd., ISBN 978-0-470-38741-2, 2011. a
Laj, P., Lund Myhre, C., Riffault, V., Amiridis, V., Fuchs, H., Eleftheriadis, K., Petäjä, T., Salameh, T., Kivekäs, N., Juurola, E., Saponaro, G., Philippin, S., Cornacchia, C., Alados Arboledas, L., Baars, H., Claude, A., De Mazière, M., Dils, B., Dufresne, M., Evangeliou, N., Favez, O., Fiebig, M., Haeffelin, M., Herrmann, H., Höhler, K., Illmann, N., Kreuter, A., Ludewig, E., Marinou, E., Möhler, O., Mona, L., Eder Murberg, L., Nicolae, D., Novelli, A., O’Connor, E., Ohneiser, K., Petracca Altieri, R. M., Picquet-Varrault, B., Van Pinxteren, D., Pospichal, B., Putaud, J.-P., Reimann, S., Siomos, N., Stachlewska, I., Tillmann, R., Voudouri, K. A., Wandinger, U., Wiedensohler, A., Apituley, A., Comerón, A., Gysel-Beer, M., Mihalopoulos, N., Nikolova, N., Pietruczuk, A., Sauvage, S., Sciare, J., Skov, H., Svendby, T., Swietlicki, E., Tonev, D., Vaughan, G., Zdimal, V., Baltensperger, U., Doussin, J.-F., Kulmala, M., Pappalardo, G., Sorvari Sundet, S., and Vana, M.: Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS): The European Research Infrastructure Supporting Atmospheric Science, B. Am. Meteorol. Soc., 105, E1098–E1136, https://doi.org/10.1175/BAMS-D-23-0064.1, 2024. a
Lee, L. A., Reddington, C. L., and Carslaw, K. S.: On the relationship between aerosol model uncertainty and radiative forcing uncertainty, P. Natl. Acad. Sci. USA, 113, 5820–5827, https://doi.org/10.1073/pnas.1507050113, 2016. a
Lewis, G. S. and Hering, S. V.: Minimizing Concentration Effects in Water-Based, Laminar-Flow Condensation Particle Counters, Aerosol Sci. Tech., 47, 645–654, https://doi.org/10.1080/02786826.2013.779629, 2013. a, b, c
Mamakos, A., Giechaskiel, B., and Drossinos, Y.: Experimental and Theoretical Investigations of the Effect of the Calibration Aerosol Material on the Counting Efficiencies of TSI 3790 Condensation Particle Counters, Aerosol Sci. Tech., 47, 11–21, https://doi.org/10.1080/02786826.2012.716174, 2013. a
Maring, H. and Schwartze, G.: A condensation particle counter for long-term continuous use in the remote marine environment, Atmos. Environ., 28, 3293–3298, 1994. a
McNeill, V. F.: Atmospheric Aerosols: Clouds, Chemistry, and Climate, Annu. Rev. Chem. Biomol., 8, 427–444, https://doi.org/10.1146/annurev-chembioeng-060816-101538, 2017. a
Mei, F., Spielman, S., Hering, S., Wang, J., Pekour, M. S., Lewis, G., Schmid, B., Tomlinson, J., and Havlicek, M.: Simulation-aided characterization of a versatile water-based condensation particle counter for atmospheric airborne research, Atmos. Meas. Tech., 14, 7329–7340, https://doi.org/10.5194/amt-14-7329-2021, 2021. a, b, c, d, e
Mordas, G., Sipilä, M., and Kulmala, M.: Nanoparticle Detection Using Nucleation Regime of the CPC, in: Nucleation and Atmospheric Aerosols, edited by: O'Dowd, C. D. and Wagner, P. E., Springer Netherlands, Dordrecht, 209–213, https://doi.org/10.1007/978-1-4020-6475-3_43, 2007. a
Nishimura, M., Nakayama, M., and Yano, T.: Vapor pressure of pure DMSO and vapor-liquid equilibria in DMSO−H2O system under isobaric conditions, J. Chem. Eng. Jpn., 5, 223–226, https://doi.org/10.1252/jcej.5.223, 1972. a
OJ EU, 2024/2881: ELI: http://data.europa.eu/eli/dir/2024/2881/oj (last access: 3 July 2026), 2024. a
Pandis, J. H. and Pandis, S. N.: Atmospheric Chemistry and Physics: From Air Pollution to Climate Change, 3rd edn., Wiley-VCH, New York, ISBN 978-1-118-94740-1, 2016. a
Petzold, A., Thouret, V., Gerbig, C., Zahn, A., Brenninkmeijer, C. A. M., Gallagher, M., Hermann, M., Pontaud, M., Ziereis, H., Boulanger, D., Marshall, J., Nédélec, P., Smit, H. G. J., Friess, U., Flaud, J.-M., Wahner, A., Cammas, J.-P., Volz-Thomas, A., and Team, I.: Global-scale atmosphere monitoring by in-service aircraft – current achievements and future prospects of the European Research Infrastructure IAGOS, Tellus B, 67, 28452, https://doi.org/10.3402/tellusb.v67.28452, 2015. a
Polyanskiy, M. N.: Refractiveindex.info database of optical constants, Scientific Data, 11, https://doi.org/10.1038/s41597-023-02898-2, 2024. a
Pöschl, U.: Atmospheric Aerosols: Composition, Transformation, Climate and Health Effects, Angew. Chem. Int. Edit., 44, 7520–7540, https://doi.org/10.1002/anie.200501122, 2005. a
Richter, S., Keber, T., Heinritzi, M., Beck, L., Merkel, L., Kirchhoff, S., Schrod, J., Weber, P., and Curtius, J.: Characterization and operation of a multi-channel Condensation Particle Counter (mc-CPC) for aircraft-based measurements, Atmos. Meas. Tech., 19, 1093–1116, https://doi.org/10.5194/amt-19-1093-2026, 2026. a
Thouret, V., Clark, H., Petzold, A., Nédélec, P., and Zahn, A.: IAGOS: Monitoring Atmospheric Composition for Air Quality and Climate by Passenger Aircraft, in: Handbook of Air Quality and Climate Change, edited by: Akimoto, H. and Tanimoto, H., Springer Nature Singapore, Singapore, 1–14, https://doi.org/10.1007/978-981-15-2527-8_57-1, 2022. a
Watson-Parris, D. and Smith, C. J.: Large uncertainty in future warming due to aerosol forcing, Nature Clim. Change, 12, 1111–1113, https://doi.org/10.1038/s41558-022-01516-0, 2022. a
Weber, P., Petzold, A., Bischof, O. F., Fischer, B., Berg, M., Freedman, A., Onasch, T. B., and Bundke, U.: Relative errors in derived multi-wavelength intensive aerosol optical properties using cavity attenuated phase shift single-scattering albedo monitors, a nephelometer, and tricolour absorption photometer measurements, Atmos. Meas. Tech., 15, 3279–3296, https://doi.org/10.5194/amt-15-3279-2022, 2022. a
Weber, P., Bischof, O. F., Fischer, B., Berg, M., Hering, S., Spielman, S., Lewis, G., Petzold, A., and Bundke, U.: Characterisation of a self-sustained, water-based condensation particle counter for aircraft cruising pressure level operation, Atmos. Meas. Tech., 16, 3505–3514, https://doi.org/10.5194/amt-16-3505-2023, 2023a. a, b
Weber, P., Bischof, O. F., Fischer, B., Berg, M., Schmitt, J., Steiner, G., Keck, L., Petzold, A., and Bundke, U.: A new working fluid for condensation particle counters for use in sensitive working environments, Aerosol Research, 1, 1–12, https://doi.org/10.5194/ar-1-1-2023, 2023b. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o, p, q, r, s, t
Wendisch, M. and Brenguier, J.-L.: Airborne Measurements for Environmental Research, John Wiley & Sons Ltd., ISBN 978-3-527-40996-9, 2013. a
Wiedensohler, A., Wiesner, A., Weinhold, K., Birmili, W., Hermann, M., Merkel, M., Müller, T., Pfeifer, S., Schmidt, A., Tuch, T., Velarde, F., Quincey, P., Seeger, S., and Nowak, A.: Mobility particle size spectrometers: Calibration procedures and measurement uncertainties, Aerosol Sci. Tech., 52, 146–164, https://doi.org/10.1080/02786826.2017.1387229, 2018. a
Yaws, C. L.: Yaws’ handbook of thermodynamic and physical properties of chemical compounds: physical, thermodynamic and transport properties for 5000 organic chemical compounds, 1st edn., Knovel, ISBN 1591244447, 2003. a
Zhang, Z. and Liu, B. Y. H.: Performance of TSI 3760 Condensation Nuclei Counter at Reduced Pressures and Flow Rates, Aerosol Sci. Tech., 15, 228–238, https://doi.org/10.1080/02786829108959530, 1991. a, b
Zhang, Z. Q. and Liu, B. Y. H.: Dependence of the Performance of TSI 3020 Condensation Nucleus Counter on Pressure, Flow Rate, and Temperature, Aerosol Sci. Tech., 13, 493–504, https://doi.org/10.1080/02786829008959464, 1990. a
Short summary
We evaluated dimethyl sulfoxide (DMSO) as a safe, non-flammable working fluid for condensation particle counters, comparing it with butanol under varied pressures, temperatures, and aerosols. Laboratory, field, and simulation results show reliable particle activation, comparable counting efficiency, reduced fluid use, and stable long-term operation. Mixtures with water extend usability, supporting safe monitoring in remote or harsh environments.
We evaluated dimethyl sulfoxide (DMSO) as a safe, non-flammable working fluid for condensation...