Articles | Volume 15, issue 9
https://doi.org/10.5194/amt-15-2889-2022
https://doi.org/10.5194/amt-15-2889-2022
Research article
 | 
11 May 2022
Research article |  | 11 May 2022

Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques

Andreas Hünig, Oliver Appel, Antonis Dragoneas, Sergej Molleker, Hans-Christian Clemen, Frank Helleis, Thomas Klimach, Franziska Köllner, Thomas Böttger, Frank Drewnick, Johannes Schneider, and Stephan Borrmann

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Revised manuscript accepted for AMT
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Cited articles

Allan, J. D., Delia, A. E., Coe, H., Bower, K. N., Alfarra, M. R., Jimenez, J. L., Middlebrook, A. M., Drewnick, F., Onasch, T. B., Canagaratna, M. R., Jayne, J. T., and Worsnop, D. R.: A generalised method for the extraction of chemically resolved mass spectra from Aerodyne aerosol mass spectrometer data, J. Aerosol Sci., 35, 909–922, https://doi.org/10.1016/j.jaerosci.2004.02.007, 2004. 
Appel, O., Köllner, F., Dragoneas, A., Hünig, A., Molleker, S., Schlager, H., Mahnke, C., Weigel, R., Port, M., Schulz, C., Drewnick, F., Vogel, B., Stroh, F., and Borrmann, S.: Chemical analysis of the Asian Tropopause Aerosol Layer (ATAL) with emphasis on secondary aerosol particles using aircraft based in situ aerosol mass spectrometry, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2022-92, in review, 2022. 
Araújo, M., Silva, R., Lima, E., Pereira, D., and De Oliveira, P.: Measurement of Gaussian laser beam radius using the knife-edge technique: Improvement on data analysis, Appl. Opt., 48, 393–396, https://doi.org/10.1364/AO.48.000393, 2009. 
Ault, A. P., Moore, M. J., Furutani, H., and Prather, K. A.: Impact of Emissions from the Los Angeles Port Region on San Diego Air Quality during Regional Transport Events, Environ. Sci. Technol., 43, 3500–3506, https://doi.org/10.1021/es8018918, 2009. 
Short summary
We have serially combined the two well-established methods for in situ real-time measurement of fine particle chemical composition, the single-particle laser ablation method and the flash evaporation with electron impact ionization method, into a novel instrument. Here we present the design; instrument characteristics, as derived from laboratory and field measurements; and results from the first field deployment during the 2017 StratoClim aircraft campaign.