Articles | Volume 14, issue 4
https://doi.org/10.5194/amt-14-2993-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/amt-14-2993-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
22 Apr 2021
Research article |
| 22 Apr 2021
| 22 Apr 2021
A method for random uncertainties validation and probing the natural variability with application to TROPOMI on board Sentinel-5P total ozone measurements
Viktoria F. Sofieva
CORRESPONDING AUTHOR
Space and Earth Observation Centre, Finnish Meteorological Institute, Helsinki, Finland
Hei Shing Lee
Space and Earth Observation Centre, Finnish Meteorological Institute, Helsinki, Finland
Atmospheric Sciences Department, University of Helsinki, Helsinki, Finland
Johanna Tamminen
Space and Earth Observation Centre, Finnish Meteorological Institute, Helsinki, Finland
Christophe Lerot
Belgian Institute for Space Aeronomy (BIRA-IASB), Brussels, Belgium
Fabian Romahn
German Aerospace Centre (DLR), Remote Sensing Technology Institute,
Oberpfaffenhofen, Germany
Diego G. Loyola
German Aerospace Centre (DLR), Remote Sensing Technology Institute,
Oberpfaffenhofen, Germany
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Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data of six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 to December 2023. It can be used in various climate-related studies.
Robert P. Damadeo, Viktoria F. Sofieva, Alexei Rozanov, and Larry W. Thomason
Atmos. Meas. Tech., 17, 3669–3678, https://doi.org/10.5194/amt-17-3669-2024, https://doi.org/10.5194/amt-17-3669-2024, 2024
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Comparing different aerosol data sets for scientific studies often requires converting aerosol extinction data between different wavelengths. A common approximation for the spectral behavior of aerosol is the Ångström formula; however, this introduces biases. Using measurements across many different wavelengths from a single instrument, we derive an empirical relationship to both characterize this bias and offer a correction for other studies that may employ this analysis approach.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Didier Fussen, Christine Bingen, Filip Vanhellemont, Nina Mateshvili, Alexei Rozanov, and Christine Pohl
Atmos. Meas. Tech., 17, 3085–3101, https://doi.org/10.5194/amt-17-3085-2024, https://doi.org/10.5194/amt-17-3085-2024, 2024
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We have developed the new multi-wavelength dataset of aerosol extinction profiles, which are retrieved from the averaged transmittance spectra by the Global Ozone Monitoring by Occultation of Stars instrument aboard Envisat. The retrieved aerosol extinction profiles are provided in the altitude range 10–40 km at 400, 440, 452, 470, 500, 525, 550, 672 and 750 nm for the period 2002–2012. FMI-GOMOSaero aerosol profiles have improved quality; they are in good agreement with other datasets.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Carlo Arosio, Alexei Rozanov, Mark Weber, Doug Degenstein, Adam Bourassa, Daniel Zawada, Michael Kiefer, Alexandra Laeng, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Christian Retscher, Robert Damadeo, and Jerry D. Lumpe
Atmos. Meas. Tech., 16, 1881–1899, https://doi.org/10.5194/amt-16-1881-2023, https://doi.org/10.5194/amt-16-1881-2023, 2023
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The paper presents the updated SAGE-CCI-OMPS+ climate data record of monthly zonal mean ozone profiles. This dataset covers the stratosphere and combines measurements by nine limb and occultation satellite instruments (SAGE II, OSIRIS, MIPAS, SCIAMACHY, GOMOS, ACE-FTS, OMPS-LP, POAM III, and SAGE III/ISS). The update includes new versions of MIPAS, ACE-FTS, and OSIRIS datasets and introduces data from additional sensors (POAM III and SAGE III/ISS) and retrieval processors (OMPS-LP).
Sophie Godin-Beekmann, Niramson Azouz, Viktoria F. Sofieva, Daan Hubert, Irina Petropavlovskikh, Peter Effertz, Gérard Ancellet, Doug A. Degenstein, Daniel Zawada, Lucien Froidevaux, Stacey Frith, Jeannette Wild, Sean Davis, Wolfgang Steinbrecht, Thierry Leblanc, Richard Querel, Kleareti Tourpali, Robert Damadeo, Eliane Maillard Barras, René Stübi, Corinne Vigouroux, Carlo Arosio, Gerald Nedoluha, Ian Boyd, Roeland Van Malderen, Emmanuel Mahieu, Dan Smale, and Ralf Sussmann
Atmos. Chem. Phys., 22, 11657–11673, https://doi.org/10.5194/acp-22-11657-2022, https://doi.org/10.5194/acp-22-11657-2022, 2022
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An updated evaluation up to 2020 of stratospheric ozone profile long-term trends at extrapolar latitudes based on satellite and ground-based records is presented. Ozone increase in the upper stratosphere is confirmed, with significant trends at most latitudes. In this altitude region, a very good agreement is found with trends derived from chemistry–climate model simulations. Observed and modelled trends diverge in the lower stratosphere, but the differences are non-significant.
Niilo Kalakoski, Viktoria F. Sofieva, René Preusker, Claire Henocq, Matthieu Denisselle, Steffen Dransfeld, and Silvia Scifoni
Atmos. Meas. Tech., 15, 5129–5140, https://doi.org/10.5194/amt-15-5129-2022, https://doi.org/10.5194/amt-15-5129-2022, 2022
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Geophysical validation of the Integrated Water Vapour (IWV) product from the Sentinel-3 Ocean and Land Colour Instrument (OLCI) was performed against reference observations from SUOMINET and IGRA databases. Results for cloud-free matchups over land show a wet bias of 7 %–10 % for OLCI, with a high correlation against the reference observations (0.98 against SUOMINET and 0.90 against IGRA). Special attention is given to validation of uncertainty estimates and cloud flagging.
Viktoria F. Sofieva, Risto Hänninen, Mikhail Sofiev, Monika Szeląg, Hei Shing Lee, Johanna Tamminen, and Christian Retscher
Atmos. Meas. Tech., 15, 3193–3212, https://doi.org/10.5194/amt-15-3193-2022, https://doi.org/10.5194/amt-15-3193-2022, 2022
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We present tropospheric ozone column datasets that have been created using combinations of total ozone column from OMI and TROPOMI with stratospheric ozone column datasets from several available limb-viewing instruments (MLS, OSIRIS, MIPAS, SCIAMACHY, OMPS-LP, GOMOS). The main results are (i) several methodological developments, (ii) new tropospheric ozone column datasets from OMI and TROPOMI, and (iii) a new high-resolution dataset of ozone profiles from limb satellite instruments.
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
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The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
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Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Monika E. Szeląg, Viktoria F. Sofieva, Doug Degenstein, Chris Roth, Sean Davis, and Lucien Froidevaux
Atmos. Chem. Phys., 20, 7035–7047, https://doi.org/10.5194/acp-20-7035-2020, https://doi.org/10.5194/acp-20-7035-2020, 2020
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We analyze seasonal dependence of stratospheric ozone trends over 2000–2018. We demonstrate that the mid-latitude upper stratospheric ozone recovery maximizes during local winters and equinoxes. In the tropics, a very strong seasonal dependence of ozone trends is observed at all altitudes. We found hemispheric asymmetry of summertime ozone trend patterns below 35 km. The seasonal dependence of ozone trends and stratospheric temperature trends shows a clear inter-relation of the trend patterns.
Mikhail Sofiev, Rostislav Kouznetsov, Risto Hänninen, and Viktoria F. Sofieva
Atmos. Chem. Phys., 20, 1839–1847, https://doi.org/10.5194/acp-20-1839-2020, https://doi.org/10.5194/acp-20-1839-2020, 2020
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An episode of anomalously low ozone concentrations in the stratosphere over northern Europe occurred on 3–5 November 2018. The 30 % reduction of the ozone layer was predicted by the global chemistry-transport model of the Finnish Meteorological Institute driven by weather forecasts of ECMWF. The reduction was subsequently observed by ozone monitoring satellites. The episode was caused by a storm in the northern Atlantic, which uplifted air from the troposphere to stratosphere.
Alain Hauchecorne, Laurent Blanot, Robin Wing, Philippe Keckhut, Sergey Khaykin, Jean-Loup Bertaux, Mustapha Meftah, Chantal Claud, and Viktoria Sofieva
Atmos. Meas. Tech., 12, 749–761, https://doi.org/10.5194/amt-12-749-2019, https://doi.org/10.5194/amt-12-749-2019, 2019
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This paper presents a new dataset of temperature profiles in the upper stratosphere and mesosphere acquired with the GOMOS spectrometer on board the European satellite ENVISAT. The principle is to observe the scattering of sunlight by air molecules at the Earth limb. The observed signal is proportional to the atmospheric density from which the temperature is derived. This technique provides a new source of information on temperature where satellite observations are sparse.
Viktoria F. Sofieva, Francis Dalaudier, Alain Hauchecorne, and Valery Kan
Atmos. Meas. Tech., 12, 585–598, https://doi.org/10.5194/amt-12-585-2019, https://doi.org/10.5194/amt-12-585-2019, 2019
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This paper describes the temperature profiles in the stratosphere obtained from unique stellar scintillation measurements by the GOMOS instrument operated on board Envisat in 2002–2012. The high-resolution temperature profiles (HRTPs) are retrieved with a very good vertical resolution of ~ 200 m and a high accuracy of ~ 1–3 K for altitudes 15–32 km as well as a global coverage. HRTPs can be assimilated into atmospheric models and used in analyses of internal gravity wave activity.
Christos Zerefos, John Kapsomenakis, Kostas Eleftheratos, Kleareti Tourpali, Irina Petropavlovskikh, Daan Hubert, Sophie Godin-Beekmann, Wolfgang Steinbrecht, Stacey Frith, Viktoria Sofieva, and Birgit Hassler
Atmos. Chem. Phys., 18, 6427–6440, https://doi.org/10.5194/acp-18-6427-2018, https://doi.org/10.5194/acp-18-6427-2018, 2018
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We point out the representativeness of single lidar stations for zonally averaged ozone profile variations in the middle/upper stratosphere. We examine the contribution of chemistry and natural proxies to ozone profile trends. Above 10 hPa an “inflection point” between 1997–99 marks the end of significant negative ozone trends, followed by a recent period of positive ozone change in 1998–2015. Below 15 hPa the pre-1998 negative ozone trends tend to become insignificant as we move to 2015.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Alexandra Laeng, Martin Kaufmann, Viktoria F. Sofieva, Lucien Froidevaux, Kaley A. Walker, and Masato Shiotani
Atmos. Meas. Tech., 11, 2187–2212, https://doi.org/10.5194/amt-11-2187-2018, https://doi.org/10.5194/amt-11-2187-2018, 2018
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This paper describes the inversion of O3 data from MIPAS middle atmosphere spectra which requires non-LTE. The O3 dataset comprises from 20 to 100 km, has a pole-to-pole latitude coverage, day and nighttime, and span from 2005 until 2012. A validation of the data against other satellite measurements and an overall description of O3 is also presented. This is an important dataset for the community and describes the major characteristics of stratospheric and mesospheric O3.
Valery Kan, Michael E. Gorbunov, and Viktoria F. Sofieva
Atmos. Meas. Tech., 11, 663–680, https://doi.org/10.5194/amt-11-663-2018, https://doi.org/10.5194/amt-11-663-2018, 2018
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We discuss the relationships that link the observed fluctuation spectra of the amplitude and phase of signals used for the radio occultation sounding of the Earth's atmosphere with the spectra of atmospheric inhomogeneities. We demonstrate that the main contribution into the radio signal fluctuations comes from the internal gravity waves. These results may serve as the basis for the global monitoring of the wave activity in the stratosphere and upper troposphere.
William T. Ball, Justin Alsing, Daniel J. Mortlock, Johannes Staehelin, Joanna D. Haigh, Thomas Peter, Fiona Tummon, Rene Stübi, Andrea Stenke, John Anderson, Adam Bourassa, Sean M. Davis, Doug Degenstein, Stacey Frith, Lucien Froidevaux, Chris Roth, Viktoria Sofieva, Ray Wang, Jeannette Wild, Pengfei Yu, Jerald R. Ziemke, and Eugene V. Rozanov
Atmos. Chem. Phys., 18, 1379–1394, https://doi.org/10.5194/acp-18-1379-2018, https://doi.org/10.5194/acp-18-1379-2018, 2018
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Using a robust analysis, with artefact-corrected ozone data, we confirm upper stratospheric ozone is recovering following the Montreal Protocol, but that lower stratospheric ozone (50° S–50° N) has continued to decrease since 1998, and the ozone layer as a whole (60° S–60° N) may be lower today than in 1998. No change in total column ozone may be due to increasing tropospheric ozone. State-of-the-art models do not reproduce lower stratospheric ozone decreases.
Viktoria F. Sofieva, Erkki Kyrölä, Marko Laine, Johanna Tamminen, Doug Degenstein, Adam Bourassa, Chris Roth, Daniel Zawada, Mark Weber, Alexei Rozanov, Nabiz Rahpoe, Gabriele Stiller, Alexandra Laeng, Thomas von Clarmann, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Claus Zehner, Robert Damadeo, Joseph Zawodny, Natalya Kramarova, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 12533–12552, https://doi.org/10.5194/acp-17-12533-2017, https://doi.org/10.5194/acp-17-12533-2017, 2017
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We present a merged dataset of ozone profiles from several satellite instruments: SAGE II, GOMOS, SCIAMACHY, MIPAS, OSIRIS, ACE-FTS and OMPS. For merging, we used the latest versions of the original ozone datasets.
The merged SAGE–CCI–OMPS dataset is used for evaluating ozone trends in the stratosphere through multiple linear regression. Negative ozone trends in the upper stratosphere are observed before 1997 and positive trends are found after 1997.
Wolfgang Steinbrecht, Lucien Froidevaux, Ryan Fuller, Ray Wang, John Anderson, Chris Roth, Adam Bourassa, Doug Degenstein, Robert Damadeo, Joe Zawodny, Stacey Frith, Richard McPeters, Pawan Bhartia, Jeannette Wild, Craig Long, Sean Davis, Karen Rosenlof, Viktoria Sofieva, Kaley Walker, Nabiz Rahpoe, Alexei Rozanov, Mark Weber, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Natalya Kramarova, Sophie Godin-Beekmann, Thierry Leblanc, Richard Querel, Daan Swart, Ian Boyd, Klemens Hocke, Niklaus Kämpfer, Eliane Maillard Barras, Lorena Moreira, Gerald Nedoluha, Corinne Vigouroux, Thomas Blumenstock, Matthias Schneider, Omaira García, Nicholas Jones, Emmanuel Mahieu, Dan Smale, Michael Kotkamp, John Robinson, Irina Petropavlovskikh, Neil Harris, Birgit Hassler, Daan Hubert, and Fiona Tummon
Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, https://doi.org/10.5194/acp-17-10675-2017, 2017
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Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000.
Christopher J. Merchant, Frank Paul, Thomas Popp, Michael Ablain, Sophie Bontemps, Pierre Defourny, Rainer Hollmann, Thomas Lavergne, Alexandra Laeng, Gerrit de Leeuw, Jonathan Mittaz, Caroline Poulsen, Adam C. Povey, Max Reuter, Shubha Sathyendranath, Stein Sandven, Viktoria F. Sofieva, and Wolfgang Wagner
Earth Syst. Sci. Data, 9, 511–527, https://doi.org/10.5194/essd-9-511-2017, https://doi.org/10.5194/essd-9-511-2017, 2017
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Climate data records (CDRs) contain data describing Earth's climate and should address uncertainty in the data to communicate what is known about climate variability or change and what range of doubt exists. This paper discusses good practice for including uncertainty information in CDRs for the essential climate variables (ECVs) derived from satellite data. Recommendations emerge from the shared experience of diverse ECV projects within the European Space Agency Climate Change Initiative.
Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Bianca Maria Dinelli, Anu Dudhia, Piera Raspollini, Norbert Glatthor, Udo Grabowski, Viktoria Sofieva, Lucien Froidevaux, Kaley A. Walker, and Claus Zehner
Atmos. Meas. Tech., 10, 1511–1518, https://doi.org/10.5194/amt-10-1511-2017, https://doi.org/10.5194/amt-10-1511-2017, 2017
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A MIPAS instrument was flown in 2002–2012 on the Envisat satellite and measured atmospheric composition. There exist four processors retrieving atmospheric profiles from MIPAS spectra. We performed a mathematically clean merging of 2007–2008 datasets of ozone from these four processors. The merged product was compared with ozone datasets from ACE-FTS and MLS instruments. The advantages and the shortcomings of this merged product are discussed.
Viktoria F. Sofieva, Iolanda Ialongo, Janne Hakkarainen, Erkki Kyrölä, Johanna Tamminen, Marko Laine, Daan Hubert, Alain Hauchecorne, Francis Dalaudier, Jean-Loup Bertaux, Didier Fussen, Laurent Blanot, Gilbert Barrot, and Angelika Dehn
Atmos. Meas. Tech., 10, 231–246, https://doi.org/10.5194/amt-10-231-2017, https://doi.org/10.5194/amt-10-231-2017, 2017
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This paper presents a new ozone profile inversion algorithm for GOMOS/Envisat satellite data. This algorithm is enhanced with a DOAS-type method at visible wavelengths in the upper troposphere and the lower stratosphere. The new GOMOS ozone profiles have a significantly improved data quality in the UTLS compared to the official IPF V6 ozone profiles. The paper describes the inversion algorithm and present inter-comparisons with ozonesonde and satellite measurements.
Filip Vanhellemont, Nina Mateshvili, Laurent Blanot, Charles Étienne Robert, Christine Bingen, Viktoria Sofieva, Francis Dalaudier, Cédric Tétard, Didier Fussen, Emmanuel Dekemper, Erkki Kyrölä, Marko Laine, Johanna Tamminen, and Claus Zehner
Atmos. Meas. Tech., 9, 4687–4700, https://doi.org/10.5194/amt-9-4687-2016, https://doi.org/10.5194/amt-9-4687-2016, 2016
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The GOMOS instrument on Envisat has delivered a valuable aerosol extinction data set for the Earth's upper troposphere and stratosphere, from 2002 to 2012. However, at many optical wavelengths, data quality was not optimal. This article describes the AerGOM retrieval algorithm that was built to solve the problem and presents a first look at the reprocessed GOMOS data, clearly demonstrating the improvement. Multi-wavelength studies of atmospheric aerosol–cloud properties will now be possible.
Niilo Kalakoski, Jukka Kujanpää, Viktoria Sofieva, Johanna Tamminen, Margherita Grossi, and Pieter Valks
Atmos. Meas. Tech., 9, 1533–1544, https://doi.org/10.5194/amt-9-1533-2016, https://doi.org/10.5194/amt-9-1533-2016, 2016
A. Kauppi, O. N. E. Tuinder, S. Tukiainen, V. Sofieva, and J. Tamminen
Atmos. Meas. Tech., 9, 249–261, https://doi.org/10.5194/amt-9-249-2016, https://doi.org/10.5194/amt-9-249-2016, 2016
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This paper presents a comparison of operational vertical ozone profiles retrieved by OPERA algorithm from the GOME-2 measurements on board Metop-A with space borne high-vertical-resolution ozone profiles by GOMOS, OSIRIS and MLS. The overall agreement of ozone profiles from GOME-2 and reference instruments is within 15 % below 35–40 km depending on latitude. The GOME-2 ozone profiles from non-degradation corrected radiances have a tendency to underestimate the ozone concentration above 30 km.
N. Rahpoe, M. Weber, A. V. Rozanov, K. Weigel, H. Bovensmann, J. P. Burrows, A. Laeng, G. Stiller, T. von Clarmann, E. Kyrölä, V. F. Sofieva, J. Tamminen, K. Walker, D. Degenstein, A. E. Bourassa, R. Hargreaves, P. Bernath, J. Urban, and D. P. Murtagh
Atmos. Meas. Tech., 8, 4369–4381, https://doi.org/10.5194/amt-8-4369-2015, https://doi.org/10.5194/amt-8-4369-2015, 2015
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The analyses among six satellite instruments measuring ozone reveals that the relative drift between the sensors is not significant in the stratosphere and we conclude that merging of data from these instruments is possible. The merged ozone profiles can then be ingested in global climate models for long-term forecasts of ozone and climate change in the atmosphere. The added drift uncertainty is estimated at about 3% per decade (1 sigma) and should be applied in the calculation of ozone trends.
A. Laeng, U. Grabowski, T. von Clarmann, G. Stiller, N. Glatthor, M. Höpfner, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, V. Sofieva, I. Petropavlovskikh, D. Hubert, T. Bathgate, P. Bernath, C. D. Boone, C. Clerbaux, P. Coheur, R. Damadeo, D. Degenstein, S. Frith, L. Froidevaux, J. Gille, K. Hoppel, M. McHugh, Y. Kasai, J. Lumpe, N. Rahpoe, G. Toon, T. Sano, M. Suzuki, J. Tamminen, J. Urban, K. Walker, M. Weber, and J. Zawodny
Atmos. Meas. Tech., 7, 3971–3987, https://doi.org/10.5194/amt-7-3971-2014, https://doi.org/10.5194/amt-7-3971-2014, 2014
V. F. Sofieva, J. Tamminen, E. Kyrölä, A. Laeng, T. von Clarmann, F. Dalaudier, A. Hauchecorne, J.-L. Bertaux, G. Barrot, L. Blanot, D. Fussen, and F. Vanhellemont
Atmos. Meas. Tech., 7, 2147–2158, https://doi.org/10.5194/amt-7-2147-2014, https://doi.org/10.5194/amt-7-2147-2014, 2014
V. F. Sofieva, N. Kalakoski, S.-M. Päivärinta, J. Tamminen, M. Laine, and L. Froidevaux
Atmos. Meas. Tech., 7, 1891–1900, https://doi.org/10.5194/amt-7-1891-2014, https://doi.org/10.5194/amt-7-1891-2014, 2014
V. Kan, V. F. Sofieva, and F. Dalaudier
Atmos. Meas. Tech., 7, 1861–1872, https://doi.org/10.5194/amt-7-1861-2014, https://doi.org/10.5194/amt-7-1861-2014, 2014
V. F. Sofieva, J. Tamminen, E. Kyrölä, T. Mielonen, P. Veefkind, B. Hassler, and G.E. Bodeker
Atmos. Chem. Phys., 14, 283–299, https://doi.org/10.5194/acp-14-283-2014, https://doi.org/10.5194/acp-14-283-2014, 2014
C. Adams, A. E. Bourassa, V. Sofieva, L. Froidevaux, C. A. McLinden, D. Hubert, J.-C. Lambert, C. E. Sioris, and D. A. Degenstein
Atmos. Meas. Tech., 7, 49–64, https://doi.org/10.5194/amt-7-49-2014, https://doi.org/10.5194/amt-7-49-2014, 2014
V. F. Sofieva, N. Rahpoe, J. Tamminen, E. Kyrölä, N. Kalakoski, M. Weber, A. Rozanov, C. von Savigny, A. Laeng, T. von Clarmann, G. Stiller, S. Lossow, D. Degenstein, A. Bourassa, C. Adams, C. Roth, N. Lloyd, P. Bernath, R. J. Hargreaves, J. Urban, D. Murtagh, A. Hauchecorne, F. Dalaudier, M. van Roozendael, N. Kalb, and C. Zehner
Earth Syst. Sci. Data, 5, 349–363, https://doi.org/10.5194/essd-5-349-2013, https://doi.org/10.5194/essd-5-349-2013, 2013
E. Kyrölä, M. Laine, V. Sofieva, J. Tamminen, S.-M. Päivärinta, S. Tukiainen, J. Zawodny, and L. Thomason
Atmos. Chem. Phys., 13, 10645–10658, https://doi.org/10.5194/acp-13-10645-2013, https://doi.org/10.5194/acp-13-10645-2013, 2013
C. Tétard, D. Fussen, F. Vanhellemont, C. Bingen, E. Dekemper, N. Mateshvili, D. Pieroux, C. Robert, E. Kyrölä, J. Tamminen, V. Sofieva, A. Hauchecorne, F. Dalaudier, J.-L. Bertaux, O. Fanton d'Andon, G. Barrot, L. Blanot, A. Dehn, and L. Saavedra de Miguel
Atmos. Meas. Tech., 6, 2953–2964, https://doi.org/10.5194/amt-6-2953-2013, https://doi.org/10.5194/amt-6-2953-2013, 2013
Diego Santaren, Janne Hakkarainen, Gerrit Kuhlmann, Erik Koene, Frédéric Chevallier, Iolanda Ialongo, Hannakaisa Lindqvist, Janne Nurmela, Johanna Tamminen, Laia Amorós, Dominik Brunner, and Grégoire Broquet
Atmos. Meas. Tech., 18, 211–239, https://doi.org/10.5194/amt-18-211-2025, https://doi.org/10.5194/amt-18-211-2025, 2025
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This study evaluates data-driven inversion methods for estimating CO2 emissions from local sources, such as power plants and cities, using meteorological data and XCO2 and NO2 satellite images rather than atmospheric transport modeling. We assess and compare the performance of five different methods using simulations of 1 year of satellite images, taken from the upcoming Copernicus CO2 Monitoring Mission, covering 15 power plants and the city of Berlin, Germany.
Carlo Arosio, Viktoria Sofieva, Andrea Orfanoz-Cheuquelaf, Alexei Rozanov, Klaus-Peter Heue, Edward Malina, Ryan M. Stauffer, David Tarasick, Roeland Van Malderen, Jerry R. Ziemke, and Mark Weber
EGUsphere, https://doi.org/10.5194/egusphere-2024-3737, https://doi.org/10.5194/egusphere-2024-3737, 2024
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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Tropospheric ozone affects air quality and climate, being a pollutant and a greenhouse gas. We analysed satellite data of tropospheric ozone that combine two types of observations: one providing stratospheric ozone and another measuring total ozone. We compare common climatological features and study the influence of the tropopause (troposphere to stratosphere boundary) on the results. We also examine trends over the last 20 years and compare satellite data with ozonesondes to identify drifts.
Viktoria F. Sofieva, Alexei Rozanov, Monika Szelag, John P. Burrows, Christian Retscher, Robert Damadeo, Doug Degenstein, Landon A. Rieger, and Adam Bourassa
Earth Syst. Sci. Data, 16, 5227–5241, https://doi.org/10.5194/essd-16-5227-2024, https://doi.org/10.5194/essd-16-5227-2024, 2024
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Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data of six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 to December 2023. It can be used in various climate-related studies.
Athina Argyrouli, Diego Loyola, Fabian Romahn, Ronny Lutz, Víctor Molina García, Pascal Hedelt, Klaus-Peter Heue, and Richard Siddans
Atmos. Meas. Tech., 17, 6345–6367, https://doi.org/10.5194/amt-17-6345-2024, https://doi.org/10.5194/amt-17-6345-2024, 2024
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This paper describes a new treatment of the spatial misregistration of cloud properties for Sentinel-5 Precursor, when the footprints of different spectral bands are not perfectly aligned. The methodology exploits synergies between spectrometers and imagers, like TROPOMI and VIIRS. The largest improvements have been identified for heterogeneous scenes at cloud edges. This approach is generic and can also be applied to future Sentinel-4 and Sentinel-5 instruments.
Sora Seo, Pieter Valks, Ronny Lutz, Klaus-Peter Heue, Pascal Hedelt, Víctor Molina García, Diego Loyola, Hanlim Lee, and Jhoon Kim
Atmos. Meas. Tech., 17, 6163–6191, https://doi.org/10.5194/amt-17-6163-2024, https://doi.org/10.5194/amt-17-6163-2024, 2024
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In this study, we developed an advanced retrieval algorithm for tropospheric NO2 columns from geostationary satellite spectrometers and applied it to GEMS measurements. The DLR GEMS NO2 retrieval algorithm follows the heritage from previous and existing algorithms, but improved approaches are applied to reflect the specific features of geostationary satellites. The DLR GEMS NO2 retrievals demonstrate a good capability for monitoring diurnal variability with a high spatial resolution.
Tim Trent, Marc Schröder, Shu-Peng Ho, Steffen Beirle, Ralf Bennartz, Eva Borbas, Christian Borger, Helene Brogniez, Xavier Calbet, Elisa Castelli, Gilbert P. Compo, Wesley Ebisuzaki, Ulrike Falk, Frank Fell, John Forsythe, Hans Hersbach, Misako Kachi, Shinya Kobayashi, Robert E. Kursinski, Diego Loyola, Zhengzao Luo, Johannes K. Nielsen, Enzo Papandrea, Laurence Picon, Rene Preusker, Anthony Reale, Lei Shi, Laura Slivinski, Joao Teixeira, Tom Vonder Haar, and Thomas Wagner
Atmos. Chem. Phys., 24, 9667–9695, https://doi.org/10.5194/acp-24-9667-2024, https://doi.org/10.5194/acp-24-9667-2024, 2024
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In a warmer future, water vapour will spend more time in the atmosphere, changing global rainfall patterns. In this study, we analysed the performance of 28 water vapour records between 1988 and 2014. We find sensitivity to surface warming generally outside expected ranges, attributed to breakpoints in individual record trends and differing representations of climate variability. The implication is that longer records are required for high confidence in assessing climate trends.
Gerrit Kuhlmann, Erik Koene, Sandro Meier, Diego Santaren, Grégoire Broquet, Frédéric Chevallier, Janne Hakkarainen, Janne Nurmela, Laia Amorós, Johanna Tamminen, and Dominik Brunner
Geosci. Model Dev., 17, 4773–4789, https://doi.org/10.5194/gmd-17-4773-2024, https://doi.org/10.5194/gmd-17-4773-2024, 2024
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We present a Python software library for data-driven emission quantification (ddeq). It can be used to determine the emissions of hot spots (cities, power plants and industry) from remote sensing images using different methods. ddeq can be extended for new datasets and methods, providing a powerful community tool for users and developers. The application of the methods is shown using Jupyter notebooks included in the library.
Robert P. Damadeo, Viktoria F. Sofieva, Alexei Rozanov, and Larry W. Thomason
Atmos. Meas. Tech., 17, 3669–3678, https://doi.org/10.5194/amt-17-3669-2024, https://doi.org/10.5194/amt-17-3669-2024, 2024
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Comparing different aerosol data sets for scientific studies often requires converting aerosol extinction data between different wavelengths. A common approximation for the spectral behavior of aerosol is the Ångström formula; however, this introduces biases. Using measurements across many different wavelengths from a single instrument, we derive an empirical relationship to both characterize this bias and offer a correction for other studies that may employ this analysis approach.
Pascal Hedelt, Jens Reichardt, Felix Lauermann, Benjamin Weiß, Nicolas Theys, Alberto Redondas, Africa Barreto, Omaira Garcia, and Diego Loyola
EGUsphere, https://doi.org/10.5194/egusphere-2024-1710, https://doi.org/10.5194/egusphere-2024-1710, 2024
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The 2021 volcanic eruption of Tajogaite on La Palma is investigated using ground-based and satellite measurements. In addition, the atmospheric transport of the volcanic cloud towards Europe isstudied in detail. The amount of SO2 released during the eruption as well as the height of the volcanic plume is in excellent agreement between the different measurements. Furthermore, volcanic aerosol microphysical properties could be retrieved using a new retrieval approach based on Lidar measurements.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Didier Fussen, Christine Bingen, Filip Vanhellemont, Nina Mateshvili, Alexei Rozanov, and Christine Pohl
Atmos. Meas. Tech., 17, 3085–3101, https://doi.org/10.5194/amt-17-3085-2024, https://doi.org/10.5194/amt-17-3085-2024, 2024
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We have developed the new multi-wavelength dataset of aerosol extinction profiles, which are retrieved from the averaged transmittance spectra by the Global Ozone Monitoring by Occultation of Stars instrument aboard Envisat. The retrieved aerosol extinction profiles are provided in the altitude range 10–40 km at 400, 440, 452, 470, 500, 525, 550, 672 and 750 nm for the period 2002–2012. FMI-GOMOSaero aerosol profiles have improved quality; they are in good agreement with other datasets.
Markku Kulmala, Anna Lintunen, Hanna Lappalainen, Annele Virtanen, Chao Yan, Ekaterina Ezhova, Tuomo Nieminen, Ilona Riipinen, Risto Makkonen, Johanna Tamminen, Anu-Maija Sundström, Antti Arola, Armin Hansel, Kari Lehtinen, Timo Vesala, Tuukka Petäjä, Jaana Bäck, Tom Kokkonen, and Veli-Matti Kerminen
Atmos. Chem. Phys., 23, 14949–14971, https://doi.org/10.5194/acp-23-14949-2023, https://doi.org/10.5194/acp-23-14949-2023, 2023
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To be able to meet global grand challenges, we need comprehensive open data with proper metadata. In this opinion paper, we describe the SMEAR (Station for Measuring Earth surface – Atmosphere Relations) concept and include several examples (cases), such as new particle formation and growth, feedback loops and the effect of COVID-19, and what has been learned from these investigations. The future needs and the potential of comprehensive observations of the environment are summarized.
Yingqi Zheng, Minttu Havu, Huizhi Liu, Xueling Cheng, Yifan Wen, Hei Shing Lee, Joyson Ahongshangbam, and Leena Järvi
Geosci. Model Dev., 16, 4551–4579, https://doi.org/10.5194/gmd-16-4551-2023, https://doi.org/10.5194/gmd-16-4551-2023, 2023
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The performance of the Surface Urban Energy and Water Balance Scheme (SUEWS) is evaluated against the observed surface exchanges (fluxes) of heat and carbon dioxide in a densely built neighborhood in Beijing. The heat flux modeling is noticeably improved by using the observed maximum conductance and by optimizing the vegetation phenology modeling. SUEWS also performs well in simulating carbon dioxide flux.
Ka Lok Chan, Pieter Valks, Klaus-Peter Heue, Ronny Lutz, Pascal Hedelt, Diego Loyola, Gaia Pinardi, Michel Van Roozendael, François Hendrick, Thomas Wagner, Vinod Kumar, Alkis Bais, Ankie Piters, Hitoshi Irie, Hisahiro Takashima, Yugo Kanaya, Yongjoo Choi, Kihong Park, Jihyo Chong, Alexander Cede, Udo Frieß, Andreas Richter, Jianzhong Ma, Nuria Benavent, Robert Holla, Oleg Postylyakov, Claudia Rivera Cárdenas, and Mark Wenig
Earth Syst. Sci. Data, 15, 1831–1870, https://doi.org/10.5194/essd-15-1831-2023, https://doi.org/10.5194/essd-15-1831-2023, 2023
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This paper presents the theoretical basis as well as verification and validation of the Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Carlo Arosio, Alexei Rozanov, Mark Weber, Doug Degenstein, Adam Bourassa, Daniel Zawada, Michael Kiefer, Alexandra Laeng, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Christian Retscher, Robert Damadeo, and Jerry D. Lumpe
Atmos. Meas. Tech., 16, 1881–1899, https://doi.org/10.5194/amt-16-1881-2023, https://doi.org/10.5194/amt-16-1881-2023, 2023
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The paper presents the updated SAGE-CCI-OMPS+ climate data record of monthly zonal mean ozone profiles. This dataset covers the stratosphere and combines measurements by nine limb and occultation satellite instruments (SAGE II, OSIRIS, MIPAS, SCIAMACHY, GOMOS, ACE-FTS, OMPS-LP, POAM III, and SAGE III/ISS). The update includes new versions of MIPAS, ACE-FTS, and OSIRIS datasets and introduces data from additional sensors (POAM III and SAGE III/ISS) and retrieval processors (OMPS-LP).
Flora Kluge, Tilman Hüneke, Christophe Lerot, Simon Rosanka, Meike K. Rotermund, Domenico Taraborrelli, Benjamin Weyland, and Klaus Pfeilsticker
Atmos. Chem. Phys., 23, 1369–1401, https://doi.org/10.5194/acp-23-1369-2023, https://doi.org/10.5194/acp-23-1369-2023, 2023
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Using airborne glyoxal concentration and vertical column density measurements, vertical profiles are inferred for eight global regions in aged biomass burning plumes and the tropical marine boundary layer. Using TROPOMI observations, an analysis of space- and airborne measurements is performed. A comparison to EMAC simulations shows a general glyoxal underprediction, which points to various missing sources and precursors from anthropogenic activities, biomass burning, and the sea surface.
Katerina Garane, Ka Lok Chan, Maria-Elissavet Koukouli, Diego Loyola, and Dimitris Balis
Atmos. Meas. Tech., 16, 57–74, https://doi.org/10.5194/amt-16-57-2023, https://doi.org/10.5194/amt-16-57-2023, 2023
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In this work, 2.5 years of TROPOMI/S5P Total Column Water Vapor (TCWV) observations retrieved from the blue wavelength band are validated against co-located precipitable water measurements from NASA AERONET, which uses Cimel Sun photometers globally. Overall, the TCWV product agrees well on a global scale with the ground-based dataset (Pearson correl. coefficient 0.909) and has a mean relative bias of −2.7 ± 4.9 % with respect to the AERONET observations for moderate albedo and cloudiness.
Miriam Latsch, Andreas Richter, Henk Eskes, Maarten Sneep, Ping Wang, Pepijn Veefkind, Ronny Lutz, Diego Loyola, Athina Argyrouli, Pieter Valks, Thomas Wagner, Holger Sihler, Michel van Roozendael, Nicolas Theys, Huan Yu, Richard Siddans, and John P. Burrows
Atmos. Meas. Tech., 15, 6257–6283, https://doi.org/10.5194/amt-15-6257-2022, https://doi.org/10.5194/amt-15-6257-2022, 2022
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The article investigates different S5P TROPOMI cloud retrieval algorithms for tropospheric trace gas retrievals. The cloud products show differences primarily over snow and ice and for scenes under sun glint. Some issues regarding across-track dependence are found for the cloud fractions as well as for the cloud heights.
Klaus-Peter Heue, Diego Loyola, Fabian Romahn, Walter Zimmer, Simon Chabrillat, Quentin Errera, Jerry Ziemke, and Natalya Kramarova
Atmos. Meas. Tech., 15, 5563–5579, https://doi.org/10.5194/amt-15-5563-2022, https://doi.org/10.5194/amt-15-5563-2022, 2022
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To retrieve tropospheric ozone column information, we subtract stratospheric column data of BASCOE from TROPOMI/S5P total ozone columns.
The new S5P-BASCOE data agree well with existing tropospheric data like OMPS-MERRA-2. The data are also compared to ozone soundings.
The tropospheric ozone columns show the expected temporal and spatial patterns. We will also apply the algorithm to future UV nadir missions like Sentinel 4 or 5 or to recent and ongoing missions like GOME_2 or OMI.
Chao Yan, Yicheng Shen, Dominik Stolzenburg, Lubna Dada, Ximeng Qi, Simo Hakala, Anu-Maija Sundström, Yishuo Guo, Antti Lipponen, Tom V. Kokkonen, Jenni Kontkanen, Runlong Cai, Jing Cai, Tommy Chan, Liangduo Chen, Biwu Chu, Chenjuan Deng, Wei Du, Xiaolong Fan, Xu-Cheng He, Juha Kangasluoma, Joni Kujansuu, Mona Kurppa, Chang Li, Yiran Li, Zhuohui Lin, Yiliang Liu, Yuliang Liu, Yiqun Lu, Wei Nie, Jouni Pulliainen, Xiaohui Qiao, Yonghong Wang, Yifan Wen, Ye Wu, Gan Yang, Lei Yao, Rujing Yin, Gen Zhang, Shaojun Zhang, Feixue Zheng, Ying Zhou, Antti Arola, Johanna Tamminen, Pauli Paasonen, Yele Sun, Lin Wang, Neil M. Donahue, Yongchun Liu, Federico Bianchi, Kaspar R. Daellenbach, Douglas R. Worsnop, Veli-Matti Kerminen, Tuukka Petäjä, Aijun Ding, Jingkun Jiang, and Markku Kulmala
Atmos. Chem. Phys., 22, 12207–12220, https://doi.org/10.5194/acp-22-12207-2022, https://doi.org/10.5194/acp-22-12207-2022, 2022
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Atmospheric new particle formation (NPF) is a dominant source of atmospheric ultrafine particles. In urban environments, traffic emissions are a major source of primary pollutants, but their contribution to NPF remains under debate. During the COVID-19 lockdown, traffic emissions were significantly reduced, providing a unique chance to examine their relevance to NPF. Based on our comprehensive measurements, we demonstrate that traffic emissions alone are not able to explain the NPF in Beijing.
Sophie Godin-Beekmann, Niramson Azouz, Viktoria F. Sofieva, Daan Hubert, Irina Petropavlovskikh, Peter Effertz, Gérard Ancellet, Doug A. Degenstein, Daniel Zawada, Lucien Froidevaux, Stacey Frith, Jeannette Wild, Sean Davis, Wolfgang Steinbrecht, Thierry Leblanc, Richard Querel, Kleareti Tourpali, Robert Damadeo, Eliane Maillard Barras, René Stübi, Corinne Vigouroux, Carlo Arosio, Gerald Nedoluha, Ian Boyd, Roeland Van Malderen, Emmanuel Mahieu, Dan Smale, and Ralf Sussmann
Atmos. Chem. Phys., 22, 11657–11673, https://doi.org/10.5194/acp-22-11657-2022, https://doi.org/10.5194/acp-22-11657-2022, 2022
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An updated evaluation up to 2020 of stratospheric ozone profile long-term trends at extrapolar latitudes based on satellite and ground-based records is presented. Ozone increase in the upper stratosphere is confirmed, with significant trends at most latitudes. In this altitude region, a very good agreement is found with trends derived from chemistry–climate model simulations. Observed and modelled trends diverge in the lower stratosphere, but the differences are non-significant.
Niilo Kalakoski, Viktoria F. Sofieva, René Preusker, Claire Henocq, Matthieu Denisselle, Steffen Dransfeld, and Silvia Scifoni
Atmos. Meas. Tech., 15, 5129–5140, https://doi.org/10.5194/amt-15-5129-2022, https://doi.org/10.5194/amt-15-5129-2022, 2022
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Geophysical validation of the Integrated Water Vapour (IWV) product from the Sentinel-3 Ocean and Land Colour Instrument (OLCI) was performed against reference observations from SUOMINET and IGRA databases. Results for cloud-free matchups over land show a wet bias of 7 %–10 % for OLCI, with a high correlation against the reference observations (0.98 against SUOMINET and 0.90 against IGRA). Special attention is given to validation of uncertainty estimates and cloud flagging.
Nicolas Theys, Christophe Lerot, Hugues Brenot, Jeroen van Gent, Isabelle De Smedt, Lieven Clarisse, Mike Burton, Matthew Varnam, Catherine Hayer, Benjamin Esse, and Michel Van Roozendael
Atmos. Meas. Tech., 15, 4801–4817, https://doi.org/10.5194/amt-15-4801-2022, https://doi.org/10.5194/amt-15-4801-2022, 2022
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Sulfur dioxide plume height after a volcanic eruption is an important piece of information for many different scientific studies and applications. Satellite UV retrievals are useful in this respect, but available algorithms have shown so far limited sensitivity to SO2 height. Here we present a new technique to improve the retrieval of SO2 plume height for SO2 columns as low as 5 DU. We demonstrate the algorithm using TROPOMI measurements and compare with other height estimates.
Pieternel F. Levelt, Deborah C. Stein Zweers, Ilse Aben, Maite Bauwens, Tobias Borsdorff, Isabelle De Smedt, Henk J. Eskes, Christophe Lerot, Diego G. Loyola, Fabian Romahn, Trissevgeni Stavrakou, Nicolas Theys, Michel Van Roozendael, J. Pepijn Veefkind, and Tijl Verhoelst
Atmos. Chem. Phys., 22, 10319–10351, https://doi.org/10.5194/acp-22-10319-2022, https://doi.org/10.5194/acp-22-10319-2022, 2022
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Using the COVID-19 lockdown periods as an example, we show how Sentinel-5P/TROPOMI trace gas data (NO2, SO2, CO, HCHO and CHOCHO) can be used to understand impacts on air quality for regions and cities around the globe. We also provide information for both experienced and inexperienced users about how we created the data using state-of-the-art algorithms, where to get the data, methods taking meteorological and seasonal variability into consideration, and insights for future studies.
Francisco J. Pérez-Invernón, Heidi Huntrieser, Thilo Erbertseder, Diego Loyola, Pieter Valks, Song Liu, Dale J. Allen, Kenneth E. Pickering, Eric J. Bucsela, Patrick Jöckel, Jos van Geffen, Henk Eskes, Sergio Soler, Francisco J. Gordillo-Vázquez, and Jeff Lapierre
Atmos. Meas. Tech., 15, 3329–3351, https://doi.org/10.5194/amt-15-3329-2022, https://doi.org/10.5194/amt-15-3329-2022, 2022
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Lightning, one of the major sources of nitrogen oxides in the atmosphere, contributes to the tropospheric concentration of ozone and to the oxidizing capacity of the atmosphere. In this work, we contribute to improving the estimation of lightning-produced nitrogen oxides in the Ebro Valley and the Pyrenees by using two different TROPOMI products and comparing the results.
Viktoria F. Sofieva, Risto Hänninen, Mikhail Sofiev, Monika Szeląg, Hei Shing Lee, Johanna Tamminen, and Christian Retscher
Atmos. Meas. Tech., 15, 3193–3212, https://doi.org/10.5194/amt-15-3193-2022, https://doi.org/10.5194/amt-15-3193-2022, 2022
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We present tropospheric ozone column datasets that have been created using combinations of total ozone column from OMI and TROPOMI with stratospheric ozone column datasets from several available limb-viewing instruments (MLS, OSIRIS, MIPAS, SCIAMACHY, OMPS-LP, GOMOS). The main results are (i) several methodological developments, (ii) new tropospheric ozone column datasets from OMI and TROPOMI, and (iii) a new high-resolution dataset of ozone profiles from limb satellite instruments.
Melanie Coldewey-Egbers, Diego G. Loyola, Christophe Lerot, and Michel Van Roozendael
Atmos. Chem. Phys., 22, 6861–6878, https://doi.org/10.5194/acp-22-6861-2022, https://doi.org/10.5194/acp-22-6861-2022, 2022
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Monitoring the long-term evolution of ozone and the evaluation of trends is essential to assess the efficacy of the Montreal Protocol and its amendments. The first signs of recovery as a consequence of decreasing amounts of ozone-depleting substances have been reported, but the impact needs to be investigated in more detail. In the Southern Hemisphere significant positive trends were found, but in the Northern Hemisphere the expected increase is still not yet visible.
Mark Weber, Carlo Arosio, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, Kleareti Tourpali, John P. Burrows, and Diego Loyola
Atmos. Chem. Phys., 22, 6843–6859, https://doi.org/10.5194/acp-22-6843-2022, https://doi.org/10.5194/acp-22-6843-2022, 2022
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Long-term trends in column ozone have been determined from five merged total ozone datasets spanning the period 1978–2020. We show that ozone recovery due to the decline in stratospheric halogens after the 1990s (as regulated by the Montreal Protocol) is evident outside the tropical region and amounts to half a percent per decade. The ozone recovery in the Northern Hemisphere is however compensated for by the negative long-term trend contribution from atmospheric dynamics since the year 2000.
Maria-Elissavet Koukouli, Konstantinos Michailidis, Pascal Hedelt, Isabelle A. Taylor, Antje Inness, Lieven Clarisse, Dimitris Balis, Dmitry Efremenko, Diego Loyola, Roy G. Grainger, and Christian Retscher
Atmos. Chem. Phys., 22, 5665–5683, https://doi.org/10.5194/acp-22-5665-2022, https://doi.org/10.5194/acp-22-5665-2022, 2022
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Volcanic eruptions eject large amounts of ash and trace gases into the atmosphere. The use of space-borne instruments enables the global monitoring of volcanic SO2 emissions in an economical and risk-free manner. The main aim of this paper is to present its extensive verification, accomplished within the ESA S5P+I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements, as well as assess its impact on the forecasts provided by CAMS.
Antje Inness, Melanie Ades, Dimitris Balis, Dmitry Efremenko, Johannes Flemming, Pascal Hedelt, Maria-Elissavet Koukouli, Diego Loyola, and Roberto Ribas
Geosci. Model Dev., 15, 971–994, https://doi.org/10.5194/gmd-15-971-2022, https://doi.org/10.5194/gmd-15-971-2022, 2022
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This paper describes the way that the Copernicus Atmosphere Monitoring Service (CAMS) produces forecasts of volcanic SO2. These forecasts are provided routinely every day. They are created by blending SO2 data from satellite instruments (TROPOMI and GOME-2) with the CAMS model. We show that the quality of the CAMS SO2 forecasts can be improved if additional information about the height of volcanic plumes is provided in the satellite data.
Christophe Lerot, François Hendrick, Michel Van Roozendael, Leonardo M. A. Alvarado, Andreas Richter, Isabelle De Smedt, Nicolas Theys, Jonas Vlietinck, Huan Yu, Jeroen Van Gent, Trissevgeni Stavrakou, Jean-François Müller, Pieter Valks, Diego Loyola, Hitoshi Irie, Vinod Kumar, Thomas Wagner, Stefan F. Schreier, Vinayak Sinha, Ting Wang, Pucai Wang, and Christian Retscher
Atmos. Meas. Tech., 14, 7775–7807, https://doi.org/10.5194/amt-14-7775-2021, https://doi.org/10.5194/amt-14-7775-2021, 2021
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Global measurements of glyoxal tropospheric columns from the satellite instrument TROPOMI are presented. Such measurements can contribute to the estimation of atmospheric emissions of volatile organic compounds. This new glyoxal product has been fully characterized with a comprehensive error budget, with comparison with other satellite data sets as well as with validation based on independent ground-based remote sensing glyoxal observations.
Daan Hubert, Klaus-Peter Heue, Jean-Christopher Lambert, Tijl Verhoelst, Marc Allaart, Steven Compernolle, Patrick D. Cullis, Angelika Dehn, Christian Félix, Bryan J. Johnson, Arno Keppens, Debra E. Kollonige, Christophe Lerot, Diego Loyola, Matakite Maata, Sukarni Mitro, Maznorizan Mohamad, Ankie Piters, Fabian Romahn, Henry B. Selkirk, Francisco R. da Silva, Ryan M. Stauffer, Anne M. Thompson, J. Pepijn Veefkind, Holger Vömel, Jacquelyn C. Witte, and Claus Zehner
Atmos. Meas. Tech., 14, 7405–7433, https://doi.org/10.5194/amt-14-7405-2021, https://doi.org/10.5194/amt-14-7405-2021, 2021
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We assess the first 2 years of TROPOMI tropical tropospheric ozone column data. Comparisons to reference measurements by ozonesonde and satellite sensors show that TROPOMI bias (−0.1 to +2.3 DU) and precision (1.5 to 2.5 DU) meet mission requirements. Potential causes of bias and its spatio-temporal structure are discussed, as well as ways to identify sampling errors. Our analysis of known geophysical patterns demonstrates the improved performance of TROPOMI with respect to its predecessors.
Song Liu, Pieter Valks, Gaia Pinardi, Jian Xu, Ka Lok Chan, Athina Argyrouli, Ronny Lutz, Steffen Beirle, Ehsan Khorsandi, Frank Baier, Vincent Huijnen, Alkiviadis Bais, Sebastian Donner, Steffen Dörner, Myrto Gratsea, François Hendrick, Dimitris Karagkiozidis, Kezia Lange, Ankie J. M. Piters, Julia Remmers, Andreas Richter, Michel Van Roozendael, Thomas Wagner, Mark Wenig, and Diego G. Loyola
Atmos. Meas. Tech., 14, 7297–7327, https://doi.org/10.5194/amt-14-7297-2021, https://doi.org/10.5194/amt-14-7297-2021, 2021
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In this work, an improved tropospheric NO2 retrieval algorithm from TROPOMI measurements over Europe is presented. The stratospheric estimation is implemented with correction for the dependency of the stratospheric NO2 on the viewing geometry. The AMF calculation is implemented using improved surface albedo, a priori NO2 profiles, and cloud correction. The improved tropospheric NO2 data show good correlations with ground-based MAX-DOAS measurements.
Nicolas Theys, Vitali Fioletov, Can Li, Isabelle De Smedt, Christophe Lerot, Chris McLinden, Nickolay Krotkov, Debora Griffin, Lieven Clarisse, Pascal Hedelt, Diego Loyola, Thomas Wagner, Vinod Kumar, Antje Innes, Roberto Ribas, François Hendrick, Jonas Vlietinck, Hugues Brenot, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 16727–16744, https://doi.org/10.5194/acp-21-16727-2021, https://doi.org/10.5194/acp-21-16727-2021, 2021
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We present a new algorithm to retrieve sulfur dioxide from space UV measurements. We apply the technique to high-resolution TROPOMI measurements and demonstrate the high sensitivity of the approach to weak SO2 emissions worldwide with an unprecedented limit of detection of 8 kt yr−1. This result has broad implications for atmospheric science studies dealing with improving emission inventories and identifying and quantifying missing sources, in the context of air quality and climate.
Anu Kauppi, Antti Kukkurainen, Antti Lipponen, Marko Laine, Antti Arola, Hannakaisa Lindqvist, and Johanna Tamminen
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-328, https://doi.org/10.5194/amt-2021-328, 2021
Revised manuscript not accepted
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We present a methodology in Bayesian framework for retrieving atmospheric aerosol optical depth and aerosol type from the pre-computed look-up tables (LUTs). Especially, we consider Bayesian model averaging and uncertainty originating from aerosol model selection and imperfect forward modelling. Our aim is to get more realistic uncertainty estimates. We have applied the methodology to TROPOMI/S5P satellite observations and evaluated the results against ground-based data from the AERONET.
Isabelle De Smedt, Gaia Pinardi, Corinne Vigouroux, Steven Compernolle, Alkis Bais, Nuria Benavent, Folkert Boersma, Ka-Lok Chan, Sebastian Donner, Kai-Uwe Eichmann, Pascal Hedelt, François Hendrick, Hitoshi Irie, Vinod Kumar, Jean-Christopher Lambert, Bavo Langerock, Christophe Lerot, Cheng Liu, Diego Loyola, Ankie Piters, Andreas Richter, Claudia Rivera Cárdenas, Fabian Romahn, Robert George Ryan, Vinayak Sinha, Nicolas Theys, Jonas Vlietinck, Thomas Wagner, Ting Wang, Huan Yu, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 12561–12593, https://doi.org/10.5194/acp-21-12561-2021, https://doi.org/10.5194/acp-21-12561-2021, 2021
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This paper assess the performances of the TROPOMI formaldehyde observations compared to its predecessor OMI at different spatial and temporal scales. We also use a global network of MAX-DOAS instruments to validate both satellite datasets for a large range of HCHO columns. The precision obtained with daily TROPOMI observations is comparable to monthly OMI observations. We present clear detection of weak HCHO column enhancements related to shipping emissions in the Indian Ocean.
Antti Arola, William Wandji Nyamsi, Antti Lipponen, Stelios Kazadzis, Nickolay A. Krotkov, and Johanna Tamminen
Atmos. Meas. Tech., 14, 4947–4957, https://doi.org/10.5194/amt-14-4947-2021, https://doi.org/10.5194/amt-14-4947-2021, 2021
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Methods to estimate surface UV radiation from satellite measurements offer the only means to obtain global coverage, and the development of satellite-based UV algorithms has been ongoing since the early 1990s. One of the main challenges in this development has been how to account for the overall effect of absorption by atmospheric aerosols. One such method was suggested roughly a decade ago, and in this study we propose further improvements for this kind of approach.
Nikita M. Fedkin, Can Li, Nickolay A. Krotkov, Pascal Hedelt, Diego G. Loyola, Russell R. Dickerson, and Robert Spurr
Atmos. Meas. Tech., 14, 3673–3691, https://doi.org/10.5194/amt-14-3673-2021, https://doi.org/10.5194/amt-14-3673-2021, 2021
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This study presents a new volcanic sulfur dioxide (SO2) layer height retrieval algorithm for the Ozone Monitoring Instrument (OMI). We generated a large spectral dataset with a radiative transfer model and used it to train neural networks to predict SO2 height from OMI radiance data. The algorithm is fast and takes less than 10 min for a single orbit. Retrievals were tested on four eruption cases, and results had reasonable agreement (within 2 km) with other retrievals and previous studies.
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
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The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Steven Compernolle, Athina Argyrouli, Ronny Lutz, Maarten Sneep, Jean-Christopher Lambert, Ann Mari Fjæraa, Daan Hubert, Arno Keppens, Diego Loyola, Ewan O'Connor, Fabian Romahn, Piet Stammes, Tijl Verhoelst, and Ping Wang
Atmos. Meas. Tech., 14, 2451–2476, https://doi.org/10.5194/amt-14-2451-2021, https://doi.org/10.5194/amt-14-2451-2021, 2021
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The high-resolution satellite Sentinel-5p TROPOMI observes several atmospheric gases. To account for cloud interference with the observations, S5P cloud data products (CLOUD OCRA/ROCINN_CAL, OCRA/ROCINN_CRB, and FRESCO) provide vital input: cloud fraction, cloud height, and cloud optical thickness. Here, S5P cloud parameters are validated by comparing with other satellite sensors (VIIRS, MODIS, and OMI) and with ground-based CloudNet data. The agreement depends on product type and cloud height.
Emily M. Gordon, Annika Seppälä, Bernd Funke, Johanna Tamminen, and Kaley A. Walker
Atmos. Chem. Phys., 21, 2819–2836, https://doi.org/10.5194/acp-21-2819-2021, https://doi.org/10.5194/acp-21-2819-2021, 2021
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Energetic particle precipitation (EPP) is the rain of solar energetic particles into the Earth's atmosphere. EPP is known to deplete O3 in the polar mesosphere–upper stratosphere via the formation of NOx. NOx also causes chlorine deactivation in the lower stratosphere and has, thus, been proposed to potentially result in reduced ozone depletion in the spring. We provide the first evidence to show that NOx formed by EPP is able to remove active chlorine, resulting in enhanced total ozone column.
Martin Dameris, Diego G. Loyola, Matthias Nützel, Melanie Coldewey-Egbers, Christophe Lerot, Fabian Romahn, and Michel van Roozendael
Atmos. Chem. Phys., 21, 617–633, https://doi.org/10.5194/acp-21-617-2021, https://doi.org/10.5194/acp-21-617-2021, 2021
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Record low ozone values were observed in March 2020. Dynamical and chemical circumstances leading to low ozone values in spring 2020 are discussed and are compared to similar dynamical conditions in the Northern Hemisphere in 1996/1997 and 2010/2011. 2019/2020 showed an unusual persistent polar vortex with low stratospheric temperatures, which were permanently below 195 K at 50 hPa. This enabled enhanced formation of polar stratospheric clouds and a subsequent clear reduction of total ozone.
Kaisa Lakkala, Jukka Kujanpää, Colette Brogniez, Nicolas Henriot, Antti Arola, Margit Aun, Frédérique Auriol, Alkiviadis F. Bais, Germar Bernhard, Veerle De Bock, Maxime Catalfamo, Christine Deroo, Henri Diémoz, Luca Egli, Jean-Baptiste Forestier, Ilias Fountoulakis, Katerina Garane, Rosa Delia Garcia, Julian Gröbner, Seppo Hassinen, Anu Heikkilä, Stuart Henderson, Gregor Hülsen, Bjørn Johnsen, Niilo Kalakoski, Angelos Karanikolas, Tomi Karppinen, Kevin Lamy, Sergio F. León-Luis, Anders V. Lindfors, Jean-Marc Metzger, Fanny Minvielle, Harel B. Muskatel, Thierry Portafaix, Alberto Redondas, Ricardo Sanchez, Anna Maria Siani, Tove Svendby, and Johanna Tamminen
Atmos. Meas. Tech., 13, 6999–7024, https://doi.org/10.5194/amt-13-6999-2020, https://doi.org/10.5194/amt-13-6999-2020, 2020
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The TROPOspheric Monitoring Instrument (TROPOMI) onboard the Sentinel-5 Precursor (S5P) satellite was launched on 13 October 2017 to provide the atmospheric composition for atmosphere and climate research. Ground-based data from 25 sites located in Arctic, subarctic, temperate, equatorial and Antarctic
areas were used for the validation of the TROPOMI surface ultraviolet (UV) radiation product. For most sites 60 %–80 % of TROPOMI data was within ± 20 % of ground-based data.
Omar Torres, Hiren Jethva, Changwoo Ahn, Glen Jaross, and Diego G. Loyola
Atmos. Meas. Tech., 13, 6789–6806, https://doi.org/10.5194/amt-13-6789-2020, https://doi.org/10.5194/amt-13-6789-2020, 2020
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TROPOMI measures the quantity of small suspended particles (aerosols). We describe initial results of aerosol measurements using a NASA algorithm that retrieves the UV aerosol index, aerosol optical depth, and single-scattering albedo. An evaluation of derived products using sun-photometer observations shows close agreement. We also use these results to discuss important biomass burning and wildfire events around the world that got the attention of scientists and news media alike.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
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Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Ka Lok Chan, Pieter Valks, Sander Slijkhuis, Claas Köhler, and Diego Loyola
Atmos. Meas. Tech., 13, 4169–4193, https://doi.org/10.5194/amt-13-4169-2020, https://doi.org/10.5194/amt-13-4169-2020, 2020
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The paper presents a new water vapor retrieval algorithm in the blue spectral band for the Global Ozone Monitoring Experience-2 (GOME-2) satellite instruments. The new retrieval features a dynamic a priori optimization module, which makes it less dependent on input from chemistry transport models and better suited for climate studies. As the blue band wavelength is available to various satellites, retrieving water vapor in the blue band potentially extends the water vapor climate record.
Corinne Vigouroux, Bavo Langerock, Carlos Augusto Bauer Aquino, Thomas Blumenstock, Zhibin Cheng, Martine De Mazière, Isabelle De Smedt, Michel Grutter, James W. Hannigan, Nicholas Jones, Rigel Kivi, Diego Loyola, Erik Lutsch, Emmanuel Mahieu, Maria Makarova, Jean-Marc Metzger, Isamu Morino, Isao Murata, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Gaia Pinardi, Amelie Röhling, Dan Smale, Wolfgang Stremme, Kim Strong, Ralf Sussmann, Yao Té, Michel van Roozendael, Pucai Wang, and Holger Winkler
Atmos. Meas. Tech., 13, 3751–3767, https://doi.org/10.5194/amt-13-3751-2020, https://doi.org/10.5194/amt-13-3751-2020, 2020
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We validate the TROPOMI HCHO product with ground-based FTIR (Fourier-transform infrared) measurements from 25 stations. We find that TROPOMI overestimates HCHO under clean conditions, while it underestimates it at high HCHO levels. Both TROPOMI precision and accuracy reach the pre-launch requirements, and its precision can even be 2 times better. The observed TROPOMI seasonal variability is in agreement with the FTIR data. The TROPOMI random uncertainty and data filtering should be refined.
Monika E. Szeląg, Viktoria F. Sofieva, Doug Degenstein, Chris Roth, Sean Davis, and Lucien Froidevaux
Atmos. Chem. Phys., 20, 7035–7047, https://doi.org/10.5194/acp-20-7035-2020, https://doi.org/10.5194/acp-20-7035-2020, 2020
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We analyze seasonal dependence of stratospheric ozone trends over 2000–2018. We demonstrate that the mid-latitude upper stratospheric ozone recovery maximizes during local winters and equinoxes. In the tropics, a very strong seasonal dependence of ozone trends is observed at all altitudes. We found hemispheric asymmetry of summertime ozone trend patterns below 35 km. The seasonal dependence of ozone trends and stratospheric temperature trends shows a clear inter-relation of the trend patterns.
Emily M. Gordon, Annika Seppälä, and Johanna Tamminen
Atmos. Chem. Phys., 20, 6259–6271, https://doi.org/10.5194/acp-20-6259-2020, https://doi.org/10.5194/acp-20-6259-2020, 2020
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The Sun constantly emits high-energy charged particles that produce the ozone destroying chemical NOx in the polar atmosphere. NOx is transported to the stratosphere, where the ozone layer is. Satellite observations show that the NOx gases remain in the atmosphere longer than previously reported. This is influenced by the strength of atmospheric large-scale dynamics, suggesting that there are specific times when this type of solar influence on the Antarctic atmosphere becomes more pronounced.
Vitali Fioletov, Chris A. McLinden, Debora Griffin, Nicolas Theys, Diego G. Loyola, Pascal Hedelt, Nickolay A. Krotkov, and Can Li
Atmos. Chem. Phys., 20, 5591–5607, https://doi.org/10.5194/acp-20-5591-2020, https://doi.org/10.5194/acp-20-5591-2020, 2020
Melanie Coldewey-Egbers, Diego G. Loyola, Gordon Labow, and Stacey M. Frith
Atmos. Meas. Tech., 13, 1633–1654, https://doi.org/10.5194/amt-13-1633-2020, https://doi.org/10.5194/amt-13-1633-2020, 2020
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We compare total ozone columns from the satellite-based GOME-type Total Ozone Essential Climate Variable record and the adjusted Modern Era Retrospective Analysis for Research and Applications version 2 reanalysis during their overlap period from 1995 to 2018. Ozone columns and anomalies show a very good agreement in terms of spatial and temporal patterns. In the tropics the interannual variability is assessed by means of an EOF analysis and both data records show a remarkable consistency.
Diego G. Loyola, Jian Xu, Klaus-Peter Heue, and Walter Zimmer
Atmos. Meas. Tech., 13, 985–999, https://doi.org/10.5194/amt-13-985-2020, https://doi.org/10.5194/amt-13-985-2020, 2020
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In this paper we present a novel algorithm for the retrieval of geometry-dependent effective Lambertian equivalent reflectivity (GE_LER) from UVN sensors based on the full-physics inverse learning machine (FP_ILM) retrieval.
The GE_LER retrieval is optimized for the trace gas retrievals using the DOAS technique and the large amount of data of TROPOMI on board the EU/ESA Sentinel-5 Precursor mission.
Mikhail Sofiev, Rostislav Kouznetsov, Risto Hänninen, and Viktoria F. Sofieva
Atmos. Chem. Phys., 20, 1839–1847, https://doi.org/10.5194/acp-20-1839-2020, https://doi.org/10.5194/acp-20-1839-2020, 2020
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An episode of anomalously low ozone concentrations in the stratosphere over northern Europe occurred on 3–5 November 2018. The 30 % reduction of the ozone layer was predicted by the global chemistry-transport model of the Finnish Meteorological Institute driven by weather forecasts of ECMWF. The reduction was subsequently observed by ozone monitoring satellites. The episode was caused by a storm in the northern Atlantic, which uplifted air from the troposphere to stratosphere.
Samuel Quesada-Ruiz, Jean-Luc Attié, William A. Lahoz, Rachid Abida, Philippe Ricaud, Laaziz El Amraoui, Régina Zbinden, Andrea Piacentini, Mathieu Joly, Henk Eskes, Arjo Segers, Lyana Curier, Johan de Haan, Jukka Kujanpää, Albert Christiaan Plechelmus Oude Nijhuis, Johanna Tamminen, Renske Timmermans, and Pepijn Veefkind
Atmos. Meas. Tech., 13, 131–152, https://doi.org/10.5194/amt-13-131-2020, https://doi.org/10.5194/amt-13-131-2020, 2020
Pascal Hedelt, Dmitry S. Efremenko, Diego G. Loyola, Robert Spurr, and Lieven Clarisse
Atmos. Meas. Tech., 12, 5503–5517, https://doi.org/10.5194/amt-12-5503-2019, https://doi.org/10.5194/amt-12-5503-2019, 2019
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Sulfur dioxide (SO2) emitted during volcanic eruptions poses not only a major threat to local populations, air quality, and aviation but also has an impact on the climate. The satellite-based detection of the SO2 plume is easy; however, it requires exact knowledge of the SO2 layer height. This paper presents a new method for the extremely fast and accurate determination of the layer height, which is essential in volcanic plume forecasts and the exact determination of the SO2 density.
Katerina Garane, Maria-Elissavet Koukouli, Tijl Verhoelst, Christophe Lerot, Klaus-Peter Heue, Vitali Fioletov, Dimitrios Balis, Alkiviadis Bais, Ariane Bazureau, Angelika Dehn, Florence Goutail, Jose Granville, Debora Griffin, Daan Hubert, Arno Keppens, Jean-Christopher Lambert, Diego Loyola, Chris McLinden, Andrea Pazmino, Jean-Pierre Pommereau, Alberto Redondas, Fabian Romahn, Pieter Valks, Michel Van Roozendael, Jian Xu, Claus Zehner, Christos Zerefos, and Walter Zimmer
Atmos. Meas. Tech., 12, 5263–5287, https://doi.org/10.5194/amt-12-5263-2019, https://doi.org/10.5194/amt-12-5263-2019, 2019
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The Sentinel-5 Precursor TROPOMI near real time (NRTI) and offline (OFFL) total ozone column (TOC) products are validated against direct-sun and twilight zenith-sky ground-based TOC measurements and other already known spaceborne sensors. The results show that the TROPOMI TOC measurements are in very good agreement with the ground-based measurements and satellite sensor measurements and that they are well within the product requirements.
Antje Inness, Johannes Flemming, Klaus-Peter Heue, Christophe Lerot, Diego Loyola, Roberto Ribas, Pieter Valks, Michel van Roozendael, Jian Xu, and Walter Zimmer
Atmos. Chem. Phys., 19, 3939–3962, https://doi.org/10.5194/acp-19-3939-2019, https://doi.org/10.5194/acp-19-3939-2019, 2019
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This paper documents the use of total column ozone data from the TROPOMI satellite in the global forecasting system of the Copernicus Atmosphere Monitoring Service (CAMS). The data are of good quality over large parts of the globe but have some issues at high latitudes, at low solar elevations and over snow/ice. Assimilating the data in the CAMS system has a small positive impact, especially in the tropical troposphere.
Kostas Eleftheratos, Christos S. Zerefos, Dimitris S. Balis, Maria-Elissavet Koukouli, John Kapsomenakis, Diego G. Loyola, Pieter Valks, Melanie Coldewey-Egbers, Christophe Lerot, Stacey M. Frith, Amund S. Haslerud, Ivar S. A. Isaksen, and Seppo Hassinen
Atmos. Meas. Tech., 12, 987–1011, https://doi.org/10.5194/amt-12-987-2019, https://doi.org/10.5194/amt-12-987-2019, 2019
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We examine the ability of GOME-2A total ozone data to capture variability related to known natural oscillations, such as the QBO, ENSO and NAO, with respect to other satellite datasets, ground-based data, and chemical transport model simulations. The analysis is based on the GOME-2 satellite total ozone columns for the period 2007–2016 which form part of the operational EUMETSAT AC SAF GOME-2 MetOp A GDP4.8 latest data product.
Alain Hauchecorne, Laurent Blanot, Robin Wing, Philippe Keckhut, Sergey Khaykin, Jean-Loup Bertaux, Mustapha Meftah, Chantal Claud, and Viktoria Sofieva
Atmos. Meas. Tech., 12, 749–761, https://doi.org/10.5194/amt-12-749-2019, https://doi.org/10.5194/amt-12-749-2019, 2019
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This paper presents a new dataset of temperature profiles in the upper stratosphere and mesosphere acquired with the GOMOS spectrometer on board the European satellite ENVISAT. The principle is to observe the scattering of sunlight by air molecules at the Earth limb. The observed signal is proportional to the atmospheric density from which the temperature is derived. This technique provides a new source of information on temperature where satellite observations are sparse.
Viktoria F. Sofieva, Francis Dalaudier, Alain Hauchecorne, and Valery Kan
Atmos. Meas. Tech., 12, 585–598, https://doi.org/10.5194/amt-12-585-2019, https://doi.org/10.5194/amt-12-585-2019, 2019
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This paper describes the temperature profiles in the stratosphere obtained from unique stellar scintillation measurements by the GOMOS instrument operated on board Envisat in 2002–2012. The high-resolution temperature profiles (HRTPs) are retrieved with a very good vertical resolution of ~ 200 m and a high accuracy of ~ 1–3 K for altitudes 15–32 km as well as a global coverage. HRTPs can be assimilated into atmospheric models and used in analyses of internal gravity wave activity.
Hansen Cao, Tzung-May Fu, Lin Zhang, Daven K. Henze, Christopher Chan Miller, Christophe Lerot, Gonzalo González Abad, Isabelle De Smedt, Qiang Zhang, Michel van Roozendael, François Hendrick, Kelly Chance, Jie Li, Junyu Zheng, and Yuanhong Zhao
Atmos. Chem. Phys., 18, 15017–15046, https://doi.org/10.5194/acp-18-15017-2018, https://doi.org/10.5194/acp-18-15017-2018, 2018
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Our top-down estimates for annual total Chinese NMVOC emissions was 30.7 to 49.5 Tg y−1, including 16.4 to 23.6 Tg y−1 from anthropogenic sources, 12.2 to 22.8 Tg y−1 from biogenic sources, and 2.08 to 3.13 Tg y−1 from biomass burning. Our four inversions consistently showed that the emissions of Chinese anthropogenic NMVOC precursors of glyoxal were larger than the a priori estimates. The glyoxal and formaldehyde constraints helped distinguish the NMVOC species from different sources.
Melanie Coldewey-Egbers, Sander Slijkhuis, Bernd Aberle, Diego Loyola, and Angelika Dehn
Atmos. Meas. Tech., 11, 5237–5259, https://doi.org/10.5194/amt-11-5237-2018, https://doi.org/10.5194/amt-11-5237-2018, 2018
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We present a detailed analysis of the long-term performance of the Global Ozone Monitoring Experiment (GOME) on-board ERS-2, which provided measurements of atmospheric constituents for the 16-year period from 1995 to 2011. By means of various in-flight calibration parameters, we monitor the behavior and stability during the entire mission. Furthermore, we introduce the new homogenized level 1 product generated using the recently developed GOME Data Processor Version 5.1.
Anne Boynard, Daniel Hurtmans, Katerina Garane, Florence Goutail, Juliette Hadji-Lazaro, Maria Elissavet Koukouli, Catherine Wespes, Corinne Vigouroux, Arno Keppens, Jean-Pierre Pommereau, Andrea Pazmino, Dimitris Balis, Diego Loyola, Pieter Valks, Ralf Sussmann, Dan Smale, Pierre-François Coheur, and Cathy Clerbaux
Atmos. Meas. Tech., 11, 5125–5152, https://doi.org/10.5194/amt-11-5125-2018, https://doi.org/10.5194/amt-11-5125-2018, 2018
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In this paper, we perform a comprehensive validation of the IASI/Metop ozone data using independent observations (satellite, ground-based and ozonesonde). The quality of the IASI total and tropospheric ozone columns in terms of bias and long-term stability is generally good. Compared with ozonesonde data, IASI overestimates (underestimates) the ozone abundance in the stratosphere (troposphere). A negative drift in tropospheric ozone is observed, which is not well understood at this point.
Marc Schröder, Maarit Lockhoff, Frank Fell, John Forsythe, Tim Trent, Ralf Bennartz, Eva Borbas, Michael G. Bosilovich, Elisa Castelli, Hans Hersbach, Misako Kachi, Shinya Kobayashi, E. Robert Kursinski, Diego Loyola, Carl Mears, Rene Preusker, William B. Rossow, and Suranjana Saha
Earth Syst. Sci. Data, 10, 1093–1117, https://doi.org/10.5194/essd-10-1093-2018, https://doi.org/10.5194/essd-10-1093-2018, 2018
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This publication presents results achieved within the GEWEX Water Vapor Assessment (G-VAP). An overview of available water vapour data records based on satellite observations and reanalysis is given. If a minimum temporal coverage of 10 years is applied, 22 data records remain. These form the G-VAP data archive, which contains total column water vapour, specific humidity profiles and temperature profiles. The G-VAP data archive is designed to ease intercomparison and climate model evaluation.
Christos Zerefos, John Kapsomenakis, Kostas Eleftheratos, Kleareti Tourpali, Irina Petropavlovskikh, Daan Hubert, Sophie Godin-Beekmann, Wolfgang Steinbrecht, Stacey Frith, Viktoria Sofieva, and Birgit Hassler
Atmos. Chem. Phys., 18, 6427–6440, https://doi.org/10.5194/acp-18-6427-2018, https://doi.org/10.5194/acp-18-6427-2018, 2018
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We point out the representativeness of single lidar stations for zonally averaged ozone profile variations in the middle/upper stratosphere. We examine the contribution of chemistry and natural proxies to ozone profile trends. Above 10 hPa an “inflection point” between 1997–99 marks the end of significant negative ozone trends, followed by a recent period of positive ozone change in 1998–2015. Below 15 hPa the pre-1998 negative ozone trends tend to become insignificant as we move to 2015.
J. Xu, K.-P. Heue, M. Coldewey-Egbers, F. Romahn, A. Doicu, and D. Loyola
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 1995–1998, https://doi.org/10.5194/isprs-archives-XLII-3-1995-2018, https://doi.org/10.5194/isprs-archives-XLII-3-1995-2018, 2018
Isabelle De Smedt, Nicolas Theys, Huan Yu, Thomas Danckaert, Christophe Lerot, Steven Compernolle, Michel Van Roozendael, Andreas Richter, Andreas Hilboll, Enno Peters, Mattia Pedergnana, Diego Loyola, Steffen Beirle, Thomas Wagner, Henk Eskes, Jos van Geffen, Klaas Folkert Boersma, and Pepijn Veefkind
Atmos. Meas. Tech., 11, 2395–2426, https://doi.org/10.5194/amt-11-2395-2018, https://doi.org/10.5194/amt-11-2395-2018, 2018
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This paper introduces the formaldehyde (HCHO) tropospheric vertical column retrieval algorithm implemented in the TROPOMI/Sentinel-5 Precursor operational processor, and comprehensively describes its various retrieval steps. Furthermore, algorithmic improvements developed in the framework of the EU FP7-project QA4ECV are described for future updates of the processor. Detailed error estimates are discussed in the light of Copernicus user requirements and needs for validation are highlighted.
Pieternel F. Levelt, Joanna Joiner, Johanna Tamminen, J. Pepijn Veefkind, Pawan K. Bhartia, Deborah C. Stein Zweers, Bryan N. Duncan, David G. Streets, Henk Eskes, Ronald van der A, Chris McLinden, Vitali Fioletov, Simon Carn, Jos de Laat, Matthew DeLand, Sergey Marchenko, Richard McPeters, Jerald Ziemke, Dejian Fu, Xiong Liu, Kenneth Pickering, Arnoud Apituley, Gonzalo González Abad, Antti Arola, Folkert Boersma, Christopher Chan Miller, Kelly Chance, Martin de Graaf, Janne Hakkarainen, Seppo Hassinen, Iolanda Ialongo, Quintus Kleipool, Nickolay Krotkov, Can Li, Lok Lamsal, Paul Newman, Caroline Nowlan, Raid Suleiman, Lieuwe Gijsbert Tilstra, Omar Torres, Huiqun Wang, and Krzysztof Wargan
Atmos. Chem. Phys., 18, 5699–5745, https://doi.org/10.5194/acp-18-5699-2018, https://doi.org/10.5194/acp-18-5699-2018, 2018
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The aim of this paper is to highlight the many successes of the Ozone Monitoring Instrument (OMI) spanning more than 13 years. Data from OMI have been used in a wide range of applications. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI plays a unique role in measuring trace gases important for the ozone layer, air quality, and climate change. OMI data continue to be used for new research and applications.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Alexandra Laeng, Martin Kaufmann, Viktoria F. Sofieva, Lucien Froidevaux, Kaley A. Walker, and Masato Shiotani
Atmos. Meas. Tech., 11, 2187–2212, https://doi.org/10.5194/amt-11-2187-2018, https://doi.org/10.5194/amt-11-2187-2018, 2018
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This paper describes the inversion of O3 data from MIPAS middle atmosphere spectra which requires non-LTE. The O3 dataset comprises from 20 to 100 km, has a pole-to-pole latitude coverage, day and nighttime, and span from 2005 until 2012. A validation of the data against other satellite measurements and an overall description of O3 is also presented. This is an important dataset for the community and describes the major characteristics of stratospheric and mesospheric O3.
Steffen Beirle, Johannes Lampel, Yang Wang, Kornelia Mies, Steffen Dörner, Margherita Grossi, Diego Loyola, Angelika Dehn, Anja Danielczok, Marc Schröder, and Thomas Wagner
Earth Syst. Sci. Data, 10, 449–468, https://doi.org/10.5194/essd-10-449-2018, https://doi.org/10.5194/essd-10-449-2018, 2018
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We present time series of the global distribution of water vapor over more than 2 decades based on satellite measurements from different sensors. A particular focus is the consistency amongst the different sensors to avoid jumps from one instrument to another. This is reached by applying robust and simple retrieval settings consistently. The resulting
Climateproduct allows the study of the temporal evolution of water vapor over the last 20 years on a global scale.
Katerina Garane, Christophe Lerot, Melanie Coldewey-Egbers, Tijl Verhoelst, Maria Elissavet Koukouli, Irene Zyrichidou, Dimitris S. Balis, Thomas Danckaert, Florence Goutail, Jose Granville, Daan Hubert, Arno Keppens, Jean-Christopher Lambert, Diego Loyola, Jean-Pierre Pommereau, Michel Van Roozendael, and Claus Zehner
Atmos. Meas. Tech., 11, 1385–1402, https://doi.org/10.5194/amt-11-1385-2018, https://doi.org/10.5194/amt-11-1385-2018, 2018
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The GOME-type Total Ozone Essential Climate Variable (GTO-ECV) is a level-3 data record, which combines individual sensor products into one single cohesive record covering the 22-year period from 1995 to 2017, generated in the frame of the European Space Agency's Climate Change Initiative Phase II. The exceptional quality of the level-3 GTO-ECV v3 TOC record temporal stability satisfies well the requirements for the total ozone measurement decadal stability of between 1 and 3 %.
Anders V. Lindfors, Jukka Kujanpää, Niilo Kalakoski, Anu Heikkilä, Kaisa Lakkala, Tero Mielonen, Maarten Sneep, Nickolay A. Krotkov, Antti Arola, and Johanna Tamminen
Atmos. Meas. Tech., 11, 997–1008, https://doi.org/10.5194/amt-11-997-2018, https://doi.org/10.5194/amt-11-997-2018, 2018
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This paper describes the algorithm that will be used for estimating surface UV radiation from TROPOMI (TROPOspheric Monitoring Instrument) measurements. TROPOMI is the only payload of the Sentinel-5 Precursor (S5P), which is a polar-orbiting satellite mission of the European Space Agency (ESA). The presented algorithm has been tested using input based on previous satellite measurements. These preliminary results indicate that the algorithm is functioning according to expectations.
Mark Weber, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, John P. Burrows, Craig S. Long, and Diego Loyola
Atmos. Chem. Phys., 18, 2097–2117, https://doi.org/10.5194/acp-18-2097-2018, https://doi.org/10.5194/acp-18-2097-2018, 2018
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This paper commemorates the 30-year anniversary of the initial signing of the Montreal Protocol (MP) on substances that deplete the ozone layer. The MP is so far successful in reducing ozone-depleting substances, and total ozone decline was successfully stopped by the late 1990s. Total ozone levels have been mostly stable since then. In some regions, barely significant upward trends are observed that suggest an emergence into the expected ozone recovery phase.
Valery Kan, Michael E. Gorbunov, and Viktoria F. Sofieva
Atmos. Meas. Tech., 11, 663–680, https://doi.org/10.5194/amt-11-663-2018, https://doi.org/10.5194/amt-11-663-2018, 2018
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We discuss the relationships that link the observed fluctuation spectra of the amplitude and phase of signals used for the radio occultation sounding of the Earth's atmosphere with the spectra of atmospheric inhomogeneities. We demonstrate that the main contribution into the radio signal fluctuations comes from the internal gravity waves. These results may serve as the basis for the global monitoring of the wave activity in the stratosphere and upper troposphere.
William T. Ball, Justin Alsing, Daniel J. Mortlock, Johannes Staehelin, Joanna D. Haigh, Thomas Peter, Fiona Tummon, Rene Stübi, Andrea Stenke, John Anderson, Adam Bourassa, Sean M. Davis, Doug Degenstein, Stacey Frith, Lucien Froidevaux, Chris Roth, Viktoria Sofieva, Ray Wang, Jeannette Wild, Pengfei Yu, Jerald R. Ziemke, and Eugene V. Rozanov
Atmos. Chem. Phys., 18, 1379–1394, https://doi.org/10.5194/acp-18-1379-2018, https://doi.org/10.5194/acp-18-1379-2018, 2018
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Using a robust analysis, with artefact-corrected ozone data, we confirm upper stratospheric ozone is recovering following the Montreal Protocol, but that lower stratospheric ozone (50° S–50° N) has continued to decrease since 1998, and the ozone layer as a whole (60° S–60° N) may be lower today than in 1998. No change in total column ozone may be due to increasing tropospheric ozone. State-of-the-art models do not reproduce lower stratospheric ozone decreases.
Diego G. Loyola, Sebastián Gimeno García, Ronny Lutz, Athina Argyrouli, Fabian Romahn, Robert J. D. Spurr, Mattia Pedergnana, Adrian Doicu, Víctor Molina García, and Olena Schüssler
Atmos. Meas. Tech., 11, 409–427, https://doi.org/10.5194/amt-11-409-2018, https://doi.org/10.5194/amt-11-409-2018, 2018
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In this paper we present the operational cloud retrieval algorithms for the TROPOspheric Monitoring Instrument (TROPOMI) on board the Sentinel-5 Precursor (S5P) mission: OCRA (Optical Cloud Recognition Algorithm) retrieves the cloud fraction using measurements in the UV–VIS spectral regions, and ROCINN (Retrieval of Cloud Information using Neural Networks) retrieves the cloud top height and optical thickness using measurements in and around the oxygen A-band in the NIR.
Anu Kauppi, Pekka Kolmonen, Marko Laine, and Johanna Tamminen
Atmos. Meas. Tech., 10, 4079–4098, https://doi.org/10.5194/amt-10-4079-2017, https://doi.org/10.5194/amt-10-4079-2017, 2017
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The paper focuses on the aerosol microphysical model selection and characterisation of uncertainty in the retrieved aerosol type and aerosol optical depth (AOD). The proposed method is based on Bayesian inference approach and can account for the model error and also include the model selection uncertainty in the total uncertainty budget. The method is applied to OMI measurements but is also applicable to other instruments. The retrieval was evaluated by comparison with ground-based measurements.
Viktoria F. Sofieva, Erkki Kyrölä, Marko Laine, Johanna Tamminen, Doug Degenstein, Adam Bourassa, Chris Roth, Daniel Zawada, Mark Weber, Alexei Rozanov, Nabiz Rahpoe, Gabriele Stiller, Alexandra Laeng, Thomas von Clarmann, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Claus Zehner, Robert Damadeo, Joseph Zawodny, Natalya Kramarova, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 12533–12552, https://doi.org/10.5194/acp-17-12533-2017, https://doi.org/10.5194/acp-17-12533-2017, 2017
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We present a merged dataset of ozone profiles from several satellite instruments: SAGE II, GOMOS, SCIAMACHY, MIPAS, OSIRIS, ACE-FTS and OMPS. For merging, we used the latest versions of the original ozone datasets.
The merged SAGE–CCI–OMPS dataset is used for evaluating ozone trends in the stratosphere through multiple linear regression. Negative ozone trends in the upper stratosphere are observed before 1997 and positive trends are found after 1997.
Wolfgang Steinbrecht, Lucien Froidevaux, Ryan Fuller, Ray Wang, John Anderson, Chris Roth, Adam Bourassa, Doug Degenstein, Robert Damadeo, Joe Zawodny, Stacey Frith, Richard McPeters, Pawan Bhartia, Jeannette Wild, Craig Long, Sean Davis, Karen Rosenlof, Viktoria Sofieva, Kaley Walker, Nabiz Rahpoe, Alexei Rozanov, Mark Weber, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Natalya Kramarova, Sophie Godin-Beekmann, Thierry Leblanc, Richard Querel, Daan Swart, Ian Boyd, Klemens Hocke, Niklaus Kämpfer, Eliane Maillard Barras, Lorena Moreira, Gerald Nedoluha, Corinne Vigouroux, Thomas Blumenstock, Matthias Schneider, Omaira García, Nicholas Jones, Emmanuel Mahieu, Dan Smale, Michael Kotkamp, John Robinson, Irina Petropavlovskikh, Neil Harris, Birgit Hassler, Daan Hubert, and Fiona Tummon
Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, https://doi.org/10.5194/acp-17-10675-2017, 2017
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Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000.
Christopher J. Merchant, Frank Paul, Thomas Popp, Michael Ablain, Sophie Bontemps, Pierre Defourny, Rainer Hollmann, Thomas Lavergne, Alexandra Laeng, Gerrit de Leeuw, Jonathan Mittaz, Caroline Poulsen, Adam C. Povey, Max Reuter, Shubha Sathyendranath, Stein Sandven, Viktoria F. Sofieva, and Wolfgang Wagner
Earth Syst. Sci. Data, 9, 511–527, https://doi.org/10.5194/essd-9-511-2017, https://doi.org/10.5194/essd-9-511-2017, 2017
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Climate data records (CDRs) contain data describing Earth's climate and should address uncertainty in the data to communicate what is known about climate variability or change and what range of doubt exists. This paper discusses good practice for including uncertainty information in CDRs for the essential climate variables (ECVs) derived from satellite data. Recommendations emerge from the shared experience of diverse ECV projects within the European Space Agency Climate Change Initiative.
Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Bianca Maria Dinelli, Anu Dudhia, Piera Raspollini, Norbert Glatthor, Udo Grabowski, Viktoria Sofieva, Lucien Froidevaux, Kaley A. Walker, and Claus Zehner
Atmos. Meas. Tech., 10, 1511–1518, https://doi.org/10.5194/amt-10-1511-2017, https://doi.org/10.5194/amt-10-1511-2017, 2017
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A MIPAS instrument was flown in 2002–2012 on the Envisat satellite and measured atmospheric composition. There exist four processors retrieving atmospheric profiles from MIPAS spectra. We performed a mathematically clean merging of 2007–2008 datasets of ozone from these four processors. The merged product was compared with ozone datasets from ACE-FTS and MLS instruments. The advantages and the shortcomings of this merged product are discussed.
Michael P. Barkley, Gonzalo González Abad, Thomas P. Kurosu, Robert Spurr, Sara Torbatian, and Christophe Lerot
Atmos. Chem. Phys., 17, 4687–4709, https://doi.org/10.5194/acp-17-4687-2017, https://doi.org/10.5194/acp-17-4687-2017, 2017
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Using Ozone Monitoring Instrument (OMI) trace gas vertical column observations of NO2, HCHO, SO2, and CHOCHO, we have conducted a robust and detailed time series analysis to assess changes in local air quality for over 1000 locations (focussing on urban, oil refinery, oil port, and power plant targets) over the Middle East for 2005–2014. We find that for many locations in the Middle East, OMI observes a degradation in air quality during this time period.
Steffen Beirle, Johannes Lampel, Christophe Lerot, Holger Sihler, and Thomas Wagner
Atmos. Meas. Tech., 10, 581–598, https://doi.org/10.5194/amt-10-581-2017, https://doi.org/10.5194/amt-10-581-2017, 2017
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We propose to parameterize the instrumental spectral response function (ISRF) as a "super-Gaussian", which can reproduce a variety of shapes, from point-hat to boxcar shape, by just adding one parameter to the "classical" Gaussian.
In addition, the super-Gaussian allows for a straightforward parametrization of the effect of ISRF changes.
Rachid Abida, Jean-Luc Attié, Laaziz El Amraoui, Philippe Ricaud, William Lahoz, Henk Eskes, Arjo Segers, Lyana Curier, Johan de Haan, Jukka Kujanpää, Albert Oude Nijhuis, Johanna Tamminen, Renske Timmermans, and Pepijn Veefkind
Atmos. Chem. Phys., 17, 1081–1103, https://doi.org/10.5194/acp-17-1081-2017, https://doi.org/10.5194/acp-17-1081-2017, 2017
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A detailed Observing System Simulation Experiment is performed to quantify the impact of future satellite instrument S-5P carbon monoxide (CO) on tropospheric analyses and forecasts. We focus on Europe for the period of northern summer 2003, when there was a severe heat wave episode. S-5P is able to capture the CO from forest fires that occurred in Portugal. Furthermore, our results provide evidence of S-5P CO benefits for monitoring processes contributing to atmospheric pollution.
Viktoria F. Sofieva, Iolanda Ialongo, Janne Hakkarainen, Erkki Kyrölä, Johanna Tamminen, Marko Laine, Daan Hubert, Alain Hauchecorne, Francis Dalaudier, Jean-Loup Bertaux, Didier Fussen, Laurent Blanot, Gilbert Barrot, and Angelika Dehn
Atmos. Meas. Tech., 10, 231–246, https://doi.org/10.5194/amt-10-231-2017, https://doi.org/10.5194/amt-10-231-2017, 2017
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This paper presents a new ozone profile inversion algorithm for GOMOS/Envisat satellite data. This algorithm is enhanced with a DOAS-type method at visible wavelengths in the upper troposphere and the lower stratosphere. The new GOMOS ozone profiles have a significantly improved data quality in the UTLS compared to the official IPF V6 ozone profiles. The paper describes the inversion algorithm and present inter-comparisons with ozonesonde and satellite measurements.
Nicolas Theys, Isabelle De Smedt, Huan Yu, Thomas Danckaert, Jeroen van Gent, Christoph Hörmann, Thomas Wagner, Pascal Hedelt, Heiko Bauer, Fabian Romahn, Mattia Pedergnana, Diego Loyola, and Michel Van Roozendael
Atmos. Meas. Tech., 10, 119–153, https://doi.org/10.5194/amt-10-119-2017, https://doi.org/10.5194/amt-10-119-2017, 2017
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This paper provides a thorough description of the algorithm to retrieve SO2 columns from TROPOMI/Sentinel-5 Precursor measurements. The different algorithmic steps including error analysis are detailed. Scientific verification of the algorithm and validation needs are also discussed.
Iolanda Ialongo, Jay Herman, Nick Krotkov, Lok Lamsal, K. Folkert Boersma, Jari Hovila, and Johanna Tamminen
Atmos. Meas. Tech., 9, 5203–5212, https://doi.org/10.5194/amt-9-5203-2016, https://doi.org/10.5194/amt-9-5203-2016, 2016
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We present the comparison between satellite- and ground-based atmospheric NO2 observations in Helsinki (Finland). The results show that, despite some limitations due to cloud contamination and low solar angles, satellite data are able to describe urban air quality features such as the weekly and seasonal cycles. The results support air quality satellite data exploitation at high latitudes and prepare for similar applications for future missions.
Klaus-Peter Heue, Melanie Coldewey-Egbers, Andy Delcloo, Christophe Lerot, Diego Loyola, Pieter Valks, and Michel van Roozendael
Atmos. Meas. Tech., 9, 5037–5051, https://doi.org/10.5194/amt-9-5037-2016, https://doi.org/10.5194/amt-9-5037-2016, 2016
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The tropical tropospheric column ozone (TCO) from 5 GOME-type satellite instruments were harmonised to get a consistent time series of tropospheric ozone for 20 years. The time series showed a global ozone trend below 10 km of 0.7 DU per decade. Also the regional trends were analysed and trends up to 1.8 DU per decade or decreases as low as 0.8 DU per decade were observed. The TCO will be part of the operation product for Tropomi/S5P and thereby extended for at least 7 years.
Filip Vanhellemont, Nina Mateshvili, Laurent Blanot, Charles Étienne Robert, Christine Bingen, Viktoria Sofieva, Francis Dalaudier, Cédric Tétard, Didier Fussen, Emmanuel Dekemper, Erkki Kyrölä, Marko Laine, Johanna Tamminen, and Claus Zehner
Atmos. Meas. Tech., 9, 4687–4700, https://doi.org/10.5194/amt-9-4687-2016, https://doi.org/10.5194/amt-9-4687-2016, 2016
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The GOMOS instrument on Envisat has delivered a valuable aerosol extinction data set for the Earth's upper troposphere and stratosphere, from 2002 to 2012. However, at many optical wavelengths, data quality was not optimal. This article describes the AerGOM retrieval algorithm that was built to solve the problem and presents a first look at the reprocessed GOMOS data, clearly demonstrating the improvement. Multi-wavelength studies of atmospheric aerosol–cloud properties will now be possible.
Anne Boynard, Daniel Hurtmans, Mariliza E. Koukouli, Florence Goutail, Jérôme Bureau, Sarah Safieddine, Christophe Lerot, Juliette Hadji-Lazaro, Catherine Wespes, Jean-Pierre Pommereau, Andrea Pazmino, Irene Zyrichidou, Dimitris Balis, Alain Barbe, Semen N. Mikhailenko, Diego Loyola, Pieter Valks, Michel Van Roozendael, Pierre-François Coheur, and Cathy Clerbaux
Atmos. Meas. Tech., 9, 4327–4353, https://doi.org/10.5194/amt-9-4327-2016, https://doi.org/10.5194/amt-9-4327-2016, 2016
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Seven years of O3 observations retrieved from IASI/MetOp satellite instruments are validated with independent data (UV satellite and ground-based data along with ozonesonde profiles). Overall IASI overestimates the total ozone columns (TOC) by 2–7 % depending on the latitude. The assessment of an updated version of the IASI O3 retrieval sofware shows a correction of ~ 4 % in the IASI TOC product, bringing the overall global bias with UV ground-based and satellite data to ~ 1–2 % on average.
Ronny Lutz, Diego Loyola, Sebastián Gimeno García, and Fabian Romahn
Atmos. Meas. Tech., 9, 2357–2379, https://doi.org/10.5194/amt-9-2357-2016, https://doi.org/10.5194/amt-9-2357-2016, 2016
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This paper presents a method for determining global cloud cover by analyzing satellite data. Knowledge of cloud coverage is not only important for climate studies but also provides valuable information in the monitoring of atmospheric trace gases. The research presented here is embedded in an operational chain, which allows us to derive the cloud-cover information in near real time, i.e., only hours after sensing by the satellite.
Emmihenna Jääskeläinen, Terhikki Manninen, Johanna Tamminen, and Marko Laine
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-180, https://doi.org/10.5194/amt-2016-180, 2016
Revised manuscript not accepted
Maria Elissavet Koukouli, Marina Zara, Christophe Lerot, Konstantinos Fragkos, Dimitris Balis, Michel van Roozendael, Marcus Antonius Franciscus Allart, and Ronald Johannes van der A
Atmos. Meas. Tech., 9, 2055–2065, https://doi.org/10.5194/amt-9-2055-2016, https://doi.org/10.5194/amt-9-2055-2016, 2016
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The main aim of the paper is to demonstrate an approach for the post-processing of the Dobson spectrophotometers' total ozone columns (TOCs) in order to compensate for their known stratospheric effective temperature dependency
and its resulting effect on the usage of the Dobson TOCs for satellite TOCs' validation.
Niilo Kalakoski, Jukka Kujanpää, Viktoria Sofieva, Johanna Tamminen, Margherita Grossi, and Pieter Valks
Atmos. Meas. Tech., 9, 1533–1544, https://doi.org/10.5194/amt-9-1533-2016, https://doi.org/10.5194/amt-9-1533-2016, 2016
S. Hassinen, D. Balis, H. Bauer, M. Begoin, A. Delcloo, K. Eleftheratos, S. Gimeno Garcia, J. Granville, M. Grossi, N. Hao, P. Hedelt, F. Hendrick, M. Hess, K.-P. Heue, J. Hovila, H. Jønch-Sørensen, N. Kalakoski, A. Kauppi, S. Kiemle, L. Kins, M. E. Koukouli, J. Kujanpää, J.-C. Lambert, R. Lang, C. Lerot, D. Loyola, M. Pedergnana, G. Pinardi, F. Romahn, M. van Roozendael, R. Lutz, I. De Smedt, P. Stammes, W. Steinbrecht, J. Tamminen, N. Theys, L. G. Tilstra, O. N. E. Tuinder, P. Valks, C. Zerefos, W. Zimmer, and I. Zyrichidou
Atmos. Meas. Tech., 9, 383–407, https://doi.org/10.5194/amt-9-383-2016, https://doi.org/10.5194/amt-9-383-2016, 2016
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The three GOME-2 instruments will provide unique and long data sets for atmospheric research and applications. The complete time period will be 2007–2022, including the period of ozone depletion as well as the beginning of ozone layer recovery. The GOME-2 products (ozone, trace gases, aerosols and UV radiation) are important for ozone chemistry, air quality studies, climate modeling, policy monitoring and hazard warnings. The processing and dissemination is done by EUMETSAT O3M SAF project.
A. Kauppi, O. N. E. Tuinder, S. Tukiainen, V. Sofieva, and J. Tamminen
Atmos. Meas. Tech., 9, 249–261, https://doi.org/10.5194/amt-9-249-2016, https://doi.org/10.5194/amt-9-249-2016, 2016
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This paper presents a comparison of operational vertical ozone profiles retrieved by OPERA algorithm from the GOME-2 measurements on board Metop-A with space borne high-vertical-resolution ozone profiles by GOMOS, OSIRIS and MLS. The overall agreement of ozone profiles from GOME-2 and reference instruments is within 15 % below 35–40 km depending on latitude. The GOME-2 ozone profiles from non-degradation corrected radiances have a tendency to underestimate the ozone concentration above 30 km.
T. Verhoelst, J. Granville, F. Hendrick, U. Köhler, C. Lerot, J.-P. Pommereau, A. Redondas, M. Van Roozendael, and J.-C. Lambert
Atmos. Meas. Tech., 8, 5039–5062, https://doi.org/10.5194/amt-8-5039-2015, https://doi.org/10.5194/amt-8-5039-2015, 2015
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Comparisons between satellite and ground-based measurements of the
atmosphere are inevitably affected by natural variability due to
mismatches in spatial and temporal co-location. These
additional terms in the comparison error budget are quantified here
for total ozone column comparisons using an Observing System Simulation
Experiment. Even when using tight co-location criteria, atmospheric
variability is found to impact the comparisons significantly.
I. De Smedt, T. Stavrakou, F. Hendrick, T. Danckaert, T. Vlemmix, G. Pinardi, N. Theys, C. Lerot, C. Gielen, C. Vigouroux, C. Hermans, C. Fayt, P. Veefkind, J.-F. Müller, and M. Van Roozendael
Atmos. Chem. Phys., 15, 12519–12545, https://doi.org/10.5194/acp-15-12519-2015, https://doi.org/10.5194/acp-15-12519-2015, 2015
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We present the new version of the BIRA-IASB algorithm for the retrieval of H2CO columns from OMI and GOME-2A and B measurements. Validation results at seven stations in Europe, China and Africa confirm the capacity of the satellite measurements to resolve diurnal variations in H2CO columns. Furthermore, vertical profiles derived from MAX-DOAS measurements in Beijing and in Bujumbura are used for a more detailed validation exercise. Finally trends are estimated using 10 years of OMI observations.
N. Rahpoe, M. Weber, A. V. Rozanov, K. Weigel, H. Bovensmann, J. P. Burrows, A. Laeng, G. Stiller, T. von Clarmann, E. Kyrölä, V. F. Sofieva, J. Tamminen, K. Walker, D. Degenstein, A. E. Bourassa, R. Hargreaves, P. Bernath, J. Urban, and D. P. Murtagh
Atmos. Meas. Tech., 8, 4369–4381, https://doi.org/10.5194/amt-8-4369-2015, https://doi.org/10.5194/amt-8-4369-2015, 2015
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The analyses among six satellite instruments measuring ozone reveals that the relative drift between the sensors is not significant in the stratosphere and we conclude that merging of data from these instruments is possible. The merged ozone profiles can then be ingested in global climate models for long-term forecasts of ozone and climate change in the atmosphere. The added drift uncertainty is estimated at about 3% per decade (1 sigma) and should be applied in the calculation of ozone trends.
M. Coldewey-Egbers, D. G. Loyola, M. Koukouli, D. Balis, J.-C. Lambert, T. Verhoelst, J. Granville, M. van Roozendael, C. Lerot, R. Spurr, S. M. Frith, and C. Zehner
Atmos. Meas. Tech., 8, 3923–3940, https://doi.org/10.5194/amt-8-3923-2015, https://doi.org/10.5194/amt-8-3923-2015, 2015
N. R. P. Harris, B. Hassler, F. Tummon, G. E. Bodeker, D. Hubert, I. Petropavlovskikh, W. Steinbrecht, J. Anderson, P. K. Bhartia, C. D. Boone, A. Bourassa, S. M. Davis, D. Degenstein, A. Delcloo, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, N. Jones, M. J. Kurylo, E. Kyrölä, M. Laine, S. T. Leblanc, J.-C. Lambert, B. Liley, E. Mahieu, A. Maycock, M. de Mazière, A. Parrish, R. Querel, K. H. Rosenlof, C. Roth, C. Sioris, J. Staehelin, R. S. Stolarski, R. Stübi, J. Tamminen, C. Vigouroux, K. A. Walker, H. J. Wang, J. Wild, and J. M. Zawodny
Atmos. Chem. Phys., 15, 9965–9982, https://doi.org/10.5194/acp-15-9965-2015, https://doi.org/10.5194/acp-15-9965-2015, 2015
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Trends in the vertical distribution of ozone are reported for new and recently revised data sets. The amount of ozone-depleting compounds in the stratosphere peaked in the second half of the 1990s. We examine the trends before and after that peak to see if any change in trend is discernible. The previously reported decreases are confirmed. Furthermore, the downward trend in upper stratospheric ozone has not continued. The possible significance of any increase is discussed in detail.
S. Tukiainen, E. Kyrölä, J. Tamminen, J. Kujanpää, and L. Blanot
Atmos. Meas. Tech., 8, 3107–3115, https://doi.org/10.5194/amt-8-3107-2015, https://doi.org/10.5194/amt-8-3107-2015, 2015
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A novel daytime ozone profile data set was created from the measurements of the Global Ozone Monitoring by Occultation of Stars (GOMOS) instrument on board the Envisat satellite. These stratospheric ozone profiles cover the years 2002-2012 with good accuracy, vertical resolution, and global coverage.
G. Bernhard, A. Arola, A. Dahlback, V. Fioletov, A. Heikkilä, B. Johnsen, T. Koskela, K. Lakkala, T. Svendby, and J. Tamminen
Atmos. Chem. Phys., 15, 7391–7412, https://doi.org/10.5194/acp-15-7391-2015, https://doi.org/10.5194/acp-15-7391-2015, 2015
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Surface erythemal UV data from the Ozone Monitoring Instrument (OMI) are validated for high northern latitudes (Arctic and Scandinavia) using ground-based measurements. The bias in OMI data caused by incorrect assumptions of the surface albedo are quantified and the mechanism that causes this bias is discussed. Methods to improve the accuracy of OMI data products are presented.
I. Ialongo, J. Hakkarainen, R. Kivi, P. Anttila, N. A. Krotkov, K. Yang, C. Li, S. Tukiainen, S. Hassinen, and J. Tamminen
Atmos. Meas. Tech., 8, 2279–2289, https://doi.org/10.5194/amt-8-2279-2015, https://doi.org/10.5194/amt-8-2279-2015, 2015
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The SO2 observations from OMI and OMPS satellite instruments are compared to ground-based measurements during the Icelandic Holuhraun fissure eruption in September 2014. The best agreement with the Brewer observations in Sodankylä, Finland can be found, assuming the SO2 predominantly located in the lowest levels of the atmosphere. The analysis of the SO2 surface concentrations in northern Finland supports the hypothesis that the volcanic plume was located very close to the surface.
M. Antón, D. Loyola, R. Román, and H. Vömel
Atmos. Meas. Tech., 8, 1135–1145, https://doi.org/10.5194/amt-8-1135-2015, https://doi.org/10.5194/amt-8-1135-2015, 2015
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The main goal of this article was to validate the total water vapour column (TWVC) measured by the Global Ozone Monitoring Experiment-2 (GOME-2) satellite sensor highly accurate sounding measurements. The smallest relative differences found in this satellite-sounding comparison (below 10%) were achieved for those cloud-free cases with satellite SZA below 50º which can be considered as a good result for satellite retrievals.
M. Grossi, P. Valks, D. Loyola, B. Aberle, S. Slijkhuis, T. Wagner, S. Beirle, and R. Lang
Atmos. Meas. Tech., 8, 1111–1133, https://doi.org/10.5194/amt-8-1111-2015, https://doi.org/10.5194/amt-8-1111-2015, 2015
S. J. Lawson, P. W. Selleck, I. E. Galbally, M. D. Keywood, M. J. Harvey, C. Lerot, D. Helmig, and Z. Ristovski
Atmos. Chem. Phys., 15, 223–240, https://doi.org/10.5194/acp-15-223-2015, https://doi.org/10.5194/acp-15-223-2015, 2015
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Glyoxal and methylglyoxal are short-lived organic trace gases and important precursors of secondary organic aerosol. Measurements over oceans are sparse. We present the first in situ glyoxal and methylglyoxal observations over remote temperate oceans, alongside observations of precursor gases. Precursor gases cannot explain observed mixing ratios, highlighting an unknown source. We show a large discrepancy between calculated vertical column densities of glyoxal and those retrieved by satellite.
A. Laeng, U. Grabowski, T. von Clarmann, G. Stiller, N. Glatthor, M. Höpfner, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, V. Sofieva, I. Petropavlovskikh, D. Hubert, T. Bathgate, P. Bernath, C. D. Boone, C. Clerbaux, P. Coheur, R. Damadeo, D. Degenstein, S. Frith, L. Froidevaux, J. Gille, K. Hoppel, M. McHugh, Y. Kasai, J. Lumpe, N. Rahpoe, G. Toon, T. Sano, M. Suzuki, J. Tamminen, J. Urban, K. Walker, M. Weber, and J. Zawodny
Atmos. Meas. Tech., 7, 3971–3987, https://doi.org/10.5194/amt-7-3971-2014, https://doi.org/10.5194/amt-7-3971-2014, 2014
N. Hao, M. E. Koukouli, A. Inness, P. Valks, D. G. Loyola, W. Zimmer, D. S. Balis, I. Zyrichidou, M. Van Roozendael, C. Lerot, and R. J. D. Spurr
Atmos. Meas. Tech., 7, 2937–2951, https://doi.org/10.5194/amt-7-2937-2014, https://doi.org/10.5194/amt-7-2937-2014, 2014
P. Valks, N. Hao, S. Gimeno Garcia, D. Loyola, M. Dameris, P. Jöckel, and A. Delcloo
Atmos. Meas. Tech., 7, 2513–2530, https://doi.org/10.5194/amt-7-2513-2014, https://doi.org/10.5194/amt-7-2513-2014, 2014
I. Ialongo, J. Hakkarainen, N. Hyttinen, J.-P. Jalkanen, L. Johansson, K. F. Boersma, N. Krotkov, and J. Tamminen
Atmos. Chem. Phys., 14, 7795–7805, https://doi.org/10.5194/acp-14-7795-2014, https://doi.org/10.5194/acp-14-7795-2014, 2014
V. F. Sofieva, J. Tamminen, E. Kyrölä, A. Laeng, T. von Clarmann, F. Dalaudier, A. Hauchecorne, J.-L. Bertaux, G. Barrot, L. Blanot, D. Fussen, and F. Vanhellemont
Atmos. Meas. Tech., 7, 2147–2158, https://doi.org/10.5194/amt-7-2147-2014, https://doi.org/10.5194/amt-7-2147-2014, 2014
V. F. Sofieva, N. Kalakoski, S.-M. Päivärinta, J. Tamminen, M. Laine, and L. Froidevaux
Atmos. Meas. Tech., 7, 1891–1900, https://doi.org/10.5194/amt-7-1891-2014, https://doi.org/10.5194/amt-7-1891-2014, 2014
V. Kan, V. F. Sofieva, and F. Dalaudier
Atmos. Meas. Tech., 7, 1861–1872, https://doi.org/10.5194/amt-7-1861-2014, https://doi.org/10.5194/amt-7-1861-2014, 2014
E. W. Chiou, P. K. Bhartia, R. D. McPeters, D. G. Loyola, M. Coldewey-Egbers, V. E. Fioletov, M. Van Roozendael, R. Spurr, C. Lerot, and S. M. Frith
Atmos. Meas. Tech., 7, 1681–1692, https://doi.org/10.5194/amt-7-1681-2014, https://doi.org/10.5194/amt-7-1681-2014, 2014
B. Hassler, I. Petropavlovskikh, J. Staehelin, T. August, P. K. Bhartia, C. Clerbaux, D. Degenstein, M. De Mazière, B. M. Dinelli, A. Dudhia, G. Dufour, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, J. Granville, N. R. P. Harris, K. Hoppel, D. Hubert, Y. Kasai, M. J. Kurylo, E. Kyrölä, J.-C. Lambert, P. F. Levelt, C. T. McElroy, R. D. McPeters, R. Munro, H. Nakajima, A. Parrish, P. Raspollini, E. E. Remsberg, K. H. Rosenlof, A. Rozanov, T. Sano, Y. Sasano, M. Shiotani, H. G. J. Smit, G. Stiller, J. Tamminen, D. W. Tarasick, J. Urban, R. J. van der A, J. P. Veefkind, C. Vigouroux, T. von Clarmann, C. von Savigny, K. A. Walker, M. Weber, J. Wild, and J. M. Zawodny
Atmos. Meas. Tech., 7, 1395–1427, https://doi.org/10.5194/amt-7-1395-2014, https://doi.org/10.5194/amt-7-1395-2014, 2014
A. Määttä, M. Laine, J. Tamminen, and J. P. Veefkind
Atmos. Meas. Tech., 7, 1185–1199, https://doi.org/10.5194/amt-7-1185-2014, https://doi.org/10.5194/amt-7-1185-2014, 2014
V. F. Sofieva, J. Tamminen, E. Kyrölä, T. Mielonen, P. Veefkind, B. Hassler, and G.E. Bodeker
Atmos. Chem. Phys., 14, 283–299, https://doi.org/10.5194/acp-14-283-2014, https://doi.org/10.5194/acp-14-283-2014, 2014
C. Adams, A. E. Bourassa, V. Sofieva, L. Froidevaux, C. A. McLinden, D. Hubert, J.-C. Lambert, C. E. Sioris, and D. A. Degenstein
Atmos. Meas. Tech., 7, 49–64, https://doi.org/10.5194/amt-7-49-2014, https://doi.org/10.5194/amt-7-49-2014, 2014
V. F. Sofieva, N. Rahpoe, J. Tamminen, E. Kyrölä, N. Kalakoski, M. Weber, A. Rozanov, C. von Savigny, A. Laeng, T. von Clarmann, G. Stiller, S. Lossow, D. Degenstein, A. Bourassa, C. Adams, C. Roth, N. Lloyd, P. Bernath, R. J. Hargreaves, J. Urban, D. Murtagh, A. Hauchecorne, F. Dalaudier, M. van Roozendael, N. Kalb, and C. Zehner
Earth Syst. Sci. Data, 5, 349–363, https://doi.org/10.5194/essd-5-349-2013, https://doi.org/10.5194/essd-5-349-2013, 2013
E. Kyrölä, M. Laine, V. Sofieva, J. Tamminen, S.-M. Päivärinta, S. Tukiainen, J. Zawodny, and L. Thomason
Atmos. Chem. Phys., 13, 10645–10658, https://doi.org/10.5194/acp-13-10645-2013, https://doi.org/10.5194/acp-13-10645-2013, 2013
C. Tétard, D. Fussen, F. Vanhellemont, C. Bingen, E. Dekemper, N. Mateshvili, D. Pieroux, C. Robert, E. Kyrölä, J. Tamminen, V. Sofieva, A. Hauchecorne, F. Dalaudier, J.-L. Bertaux, O. Fanton d'Andon, G. Barrot, L. Blanot, A. Dehn, and L. Saavedra de Miguel
Atmos. Meas. Tech., 6, 2953–2964, https://doi.org/10.5194/amt-6-2953-2013, https://doi.org/10.5194/amt-6-2953-2013, 2013
G. Saponaro, P. Kolmonen, J. Karhunen, J. Tamminen, and G. de Leeuw
Atmos. Meas. Tech., 6, 2301–2309, https://doi.org/10.5194/amt-6-2301-2013, https://doi.org/10.5194/amt-6-2301-2013, 2013
Related subject area
Subject: Gases | Technique: Remote Sensing | Topic: Validation and Intercomparisons
Benchmarking data-driven inversion methods for the estimation of local CO2 emissions from synthetic satellite images of XCO2 and NO2
Validation of 12 years (2008–2019) of IASI-A CO with IAGOS aircraft observations
Diurnal variations of NO2 tropospheric vertical column density over the Seoul metropolitan area from the Geostationary Environment Monitoring Spectrometer (GEMS): seasonal differences and the influence of the a priori NO2 profile
Validation of ACE-FTS version 5.2 ozone data with ozonesonde measurements
Intercomparison of long-term ground-based measurements of total, tropospheric, and stratospheric ozone at Lauder, New Zealand
First evaluation of the GEMS glyoxal products against TROPOMI and ground-based measurements
Validation of GEMS tropospheric NO2 columns and their diurnal variation with ground-based DOAS measurements
Using open-path dual-comb spectroscopy to monitor methane emissions from simulated grazing cattle
Greenhouse gas column observations from a portable spectrometer in Uganda
Independent validation of IASI/MetOp-A LMD and RAL CH4 products using CAMS model, in situ profiles, and ground-based FTIR measurements
Joint spectral retrievals of ozone with Suomi NPP CrIS augmented by S5P/TROPOMI
An evaluation of atmospheric absorption models at millimetre and sub-millimetre wavelengths using airborne observations
Validation of the version 4.5 MAESTRO ozone and NO2 measurements
Applicability of the inverse dispersion method to measure emissions from animal housings
5 years of Sentinel-5P TROPOMI operational ozone profiling and geophysical validation using ozonesonde and lidar ground-based networks
Using a portable FTIR spectrometer to evaluate the consistency of Total Carbon Column Observing Network (TCCON) measurements on a global scale: the Collaborative Carbon Column Observing Network (COCCON) travel standard
Comparison of the H2O, HDO and δD stratospheric climatologies between the MIPAS-ESA V8, MIPAS-IMK V5 and ACE-FTS V4.1/4.2 satellite datasets
TROPESS-CrIS CO single-pixel vertical profiles: intercomparisons with MOPITT and model simulations for 2020 western US wildfires
TOLNet validation of satellite ozone profiles in the troposphere: impact of retrieval wavelengths
An uncertainty methodology for solar occultation flux measurements: ammonia emissions from livestock production
Validation of Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) chlorodifluoromethane (HCFC-22) in the upper troposphere and lower stratosphere
First validation of high-resolution satellite-derived methane emissions from an active gas leak in the UK
Ship- and aircraft-based XCH4 over oceans as a new tool for satellite validation
Single-blind test of nine methane-sensing satellite systems from three continents
Water vapor measurements inside clouds and storms using a differential absorption radar
Evaluation of the first year of Pandora NO2 measurements over Beijing and application to satellite validation
Validation of MUSES NH3 observations from AIRS and CrIS against aircraft measurements from DISCOVER-AQ and a surface network in the Magic Valley
Performance and sensitivity of column-wise and pixel-wise methane retrievals for imaging spectrometers
Methane point source quantification using MethaneAIR: a new airborne imaging spectrometer
Evaluation of total ozone measurements from Geostationary Environmental Monitoring Spectrometer (GEMS)
To new heights by flying low: comparison of aircraft vertical NO2 profiles to model simulations and implications for TROPOMI NO2 retrievals
Local comparisons of tropospheric ozone: vertical soundings at two neighbouring stations in southern Bavaria
Ground-based Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations of NO2 and H2CO at Kinshasa and comparisons with TROPOMI observations
Total column ozone trends from the NASA Merged Ozone time series 1979 to 2021 showing latitude-dependent ozone recovery dates (1994 to 1998)
The SPARC water vapour assessment II: biases and drifts of water vapour satellite data records with respect to frost point hygrometer records
Vicarious calibration of the Tropospheric Monitoring Instrument (TROPOMI) short-wave infrared (SWIR) module over the Railroad Valley Playa
First-time comparison between NO2 vertical columns from Geostationary Environmental Monitoring Spectrometer (GEMS) and Pandora measurements
A blended TROPOMI+GOSAT satellite data product for atmospheric methane using machine learning to correct retrieval biases
Evaluating the consistency between OCO-2 and OCO-3 XCO2 estimates derived from the NASA ACOS version 10 retrieval algorithm
OLCI-A/B tandem phase: evaluation of FLuorescence EXplorer (FLEX)-like radiances and estimation of systematic differences between OLCI-A and OLCI-FLEX
Multi-parameter dynamical diagnostics for upper tropospheric and lower stratospheric studies
An approach to track instrument calibration and produce consistent products with the version-8 total column ozone algorithm (V8TOZ)
Satellite remote-sensing capability to assess tropospheric-column ratios of formaldehyde and nitrogen dioxide: case study during the Long Island Sound Tropospheric Ozone Study 2018 (LISTOS 2018) field campaign
Validation of Sentinel-5P TROPOMI tropospheric NO2 products by comparison with NO2 measurements from airborne imaging DOAS, ground-based stationary DOAS, and mobile car DOAS measurements during the S5P-VAL-DE-Ruhr campaign
Evaluation of open- and closed-path sampling systems for the determination of emission rates of NH3 and CH4 with inverse dispersion modeling
Performance of AIRS ozone retrieval over the central Himalayas: use of ozonesonde and other satellite datasets
Solar occultation measurement of mesospheric ozone by SAGE III/ISS: impact of variations along the line of sight caused by photochemistry
Understanding the potential of Sentinel-2 for monitoring methane point emissions
TROPOMI/S5P Total Column Water Vapor validation against AERONET ground-based measurements
Assessing the consistency of satellite-derived upper tropospheric humidity measurements
Diego Santaren, Janne Hakkarainen, Gerrit Kuhlmann, Erik Koene, Frédéric Chevallier, Iolanda Ialongo, Hannakaisa Lindqvist, Janne Nurmela, Johanna Tamminen, Laia Amorós, Dominik Brunner, and Grégoire Broquet
Atmos. Meas. Tech., 18, 211–239, https://doi.org/10.5194/amt-18-211-2025, https://doi.org/10.5194/amt-18-211-2025, 2025
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This study evaluates data-driven inversion methods for estimating CO2 emissions from local sources, such as power plants and cities, using meteorological data and XCO2 and NO2 satellite images rather than atmospheric transport modeling. We assess and compare the performance of five different methods using simulations of 1 year of satellite images, taken from the upcoming Copernicus CO2 Monitoring Mission, covering 15 power plants and the city of Berlin, Germany.
Brice Barret, Pierre Loicq, Eric Le Flochmoën, Yasmine Bennouna, Juliette Hadji-Lazaro, Daniel Hurtmans, and Bastien Sauvage
Atmos. Meas. Tech., 18, 129–149, https://doi.org/10.5194/amt-18-129-2025, https://doi.org/10.5194/amt-18-129-2025, 2025
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Profiles of carbon monoxide (CO) retrieved from the Infrared Atmospheric Sounding Interferometer (IASI) with the SOftware for a Fast Retrieval of IASI Data (SOFRID) and Fast Optimal Retrievals on Layers for IASI (FORLI) are validated with 8500 observations at 33 airports from the In-service Aircraft for a Global Observing System (IAGOS) for 2008–2019. IASI retrievals underestimate CO, with stronger bias in the middle to upper troposphere for SOFRID and in the lower troposphere for FORLI.
Seunghwan Seo, Si-Wan Kim, Kyoung-Min Kim, Andreas Richter, Kezia Lange, John P. Burrows, Junsung Park, Hyunkee Hong, Hanlim Lee, Ukkyo Jeong, Jung-Hun Woo, and Jhoon Kim
Atmos. Meas. Tech., 18, 115–128, https://doi.org/10.5194/amt-18-115-2025, https://doi.org/10.5194/amt-18-115-2025, 2025
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Over the Seoul metropolitan area, tropospheric NO2 vertical column densities from the Geostationary Environment Monitoring Spectrometer show distinct seasonal features. Also, varying a priori data have substantial impacts on the observed NO2 columns. The a priori data from different chemical transport models resulted in differences of up to −18.3 %. Notably, diurnal patterns of observed NO2 columns are similar for all datasets, although their a priori data exhibit contrasting diurnal patterns.
Jiansheng Zou, Kaley A. Walker, Patrick E. Sheese, Chris D. Boone, Ryan M. Stauffer, Anne M. Thompson, and David W. Tarasick
Atmos. Meas. Tech., 17, 6983–7005, https://doi.org/10.5194/amt-17-6983-2024, https://doi.org/10.5194/amt-17-6983-2024, 2024
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Ozone measurements from the ACE-FTS satellite instrument have been compared to worldwide balloon-borne ozonesonde profiles using pairs of closely spaced profiles and monthly averaged profiles. ACE-FTS typically measures more ozone in the stratosphere by up to 10 %. The long-term stability of the ACE-FTS ozone data is good, exhibiting small (but non-significant) drifts of less than 3 % per decade in the stratosphere. Lower in the profiles, the calculated drifts are larger (up to 10 % per decade).
Robin Björklund, Corinne Vigouroux, Peter Effertz, Omaira E. García, Alex Geddes, James Hannigan, Koji Miyagawa, Michael Kotkamp, Bavo Langerock, Gerald Nedoluha, Ivan Ortega, Irina Petropavlovskikh, Deniz Poyraz, Richard Querel, John Robinson, Hisako Shiona, Dan Smale, Penny Smale, Roeland Van Malderen, and Martine De Mazière
Atmos. Meas. Tech., 17, 6819–6849, https://doi.org/10.5194/amt-17-6819-2024, https://doi.org/10.5194/amt-17-6819-2024, 2024
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Different ground-based ozone measurements from the last 2 decades at Lauder are compared to each other. We want to know why different trends have been observed in the stratosphere. Also, the quality and relevance of tropospheric datasets need to be evaluated. While remaining drifts are still present, our study explains roughly half of the differences in observed trends in previous studies and shows the necessity for continuous review and improvement of the measurements.
Eunjo S. Ha, Rokjin J. Park, Hyeong-Ahn Kwon, Gitaek T. Lee, Sieun D. Lee, Seunga Shin, Dong-Won Lee, Hyunkee Hong, Christophe Lerot, Isabelle De Smedt, Thomas Danckaert, Francois Hendrick, and Hitoshi Irie
Atmos. Meas. Tech., 17, 6369–6384, https://doi.org/10.5194/amt-17-6369-2024, https://doi.org/10.5194/amt-17-6369-2024, 2024
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In this study, we evaluated the GEMS glyoxal products by comparing them with TROPOMI and MAX-DOAS measurements. GEMS and TROPOMI VCDs present similar spatial distributions. Monthly variations in GEMS VCDs and TROPOMI and MAX-DOAS VCDs differ in northeastern Asia, which we attributed to a polluted reference spectrum and high NO2 concentrations. GEMS glyoxal products with unparalleled temporal resolution would enrich our understanding of VOC emissions and diurnal variation.
Kezia Lange, Andreas Richter, Tim Bösch, Bianca Zilker, Miriam Latsch, Lisa K. Behrens, Chisom M. Okafor, Hartmut Bösch, John P. Burrows, Alexis Merlaud, Gaia Pinardi, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Steffen Ziegler, Simona Ripperger-Lukosiunaite, Leon Kuhn, Bianca Lauster, Thomas Wagner, Hyunkee Hong, Donghee Kim, Lim-Seok Chang, Kangho Bae, Chang-Keun Song, Jong-Uk Park, and Hanlim Lee
Atmos. Meas. Tech., 17, 6315–6344, https://doi.org/10.5194/amt-17-6315-2024, https://doi.org/10.5194/amt-17-6315-2024, 2024
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Instruments for air quality observations on geostationary satellites provide multiple observations per day and allow for the analysis of the diurnal variation of important air pollutants such as nitrogen dioxide (NO2) over large areas. The South Korean instrument GEMS, launched in February 2020, is the first instrument in geostationary orbit and covers a large part of Asia. Our investigations show the observed diurnal evolution of NO2 at different measurement sites.
Chinthaka Weerasekara, Lindsay C. Morris, Nathan A. Malarich, Fabrizio R. Giorgetta, Daniel I. Herman, Kevin C. Cossel, Nathan R. Newbury, Clenton E. Owensby, Stephen M. Welch, Cosmin Blaga, Brett D. DePaola, Ian Coddington, Brian R. Washburn, and Eduardo A. Santos
Atmos. Meas. Tech., 17, 6107–6117, https://doi.org/10.5194/amt-17-6107-2024, https://doi.org/10.5194/amt-17-6107-2024, 2024
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Most methane emissions during the life cycle of beef cattle occur during the grazing phase. Measuring methane in grazing systems is difficult due to the high mobility and low density of animals. This work investigates if dual-comb spectroscopy can measure methane emissions from small cattle herds. An enhancement of 10 nmol mol-1 methane above the atmospheric background was measured, equivalent to 20 head located 60 m away. The calculated methane flux was within 5 % of the actual release rate.
Neil Humpage, Hartmut Boesch, William Okello, Jia Chen, Florian Dietrich, Mark F. Lunt, Liang Feng, Paul I. Palmer, and Frank Hase
Atmos. Meas. Tech., 17, 5679–5707, https://doi.org/10.5194/amt-17-5679-2024, https://doi.org/10.5194/amt-17-5679-2024, 2024
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We used a Bruker EM27/SUN spectrometer within an automated weatherproof enclosure to measure greenhouse gas column concentrations over a 3-month period in Jinja, Uganda. The portability of the EM27/SUN allows us to evaluate satellite and model data in locations not covered by traditional validation networks. This is of particular value in tropical Africa, where extensive terrestrial ecosystems are a significant store of carbon and play a key role in the atmospheric budgets of CO2 and CH4.
Bart Dils, Minqiang Zhou, Claude Camy-Peyret, Martine De Mazière, Yannick Kangah, Bavo Langerock, Pascal Prunet, Carmine Serio, Richard Siddans, and Brian Kerridge
Atmos. Meas. Tech., 17, 5491–5524, https://doi.org/10.5194/amt-17-5491-2024, https://doi.org/10.5194/amt-17-5491-2024, 2024
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The paper discusses two very distinct methane products from the IASI instrument aboard the MetOp-A satellite. One (referred to as LMD NLISv8.3) uses a machine-learning approach, while the other (RALv2.0) uses a more conventional optimal estimation approach. We used a variety of model and independent reference measurement data to assess both products' overall quality, their differences, and specific aspects of each product that would benefit from further analysis by the product development teams.
Edward Malina, Kevin W. Bowman, Valentin Kantchev, Le Kuai, Thomas P. Kurosu, Kazuyuki Miyazaki, Vijay Natraj, Gregory B. Osterman, Fabiano Oyafuso, and Matthew D. Thill
Atmos. Meas. Tech., 17, 5341–5371, https://doi.org/10.5194/amt-17-5341-2024, https://doi.org/10.5194/amt-17-5341-2024, 2024
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Characterizing the distribution of ozone in the atmosphere is a challenging problem, with current Earth observation satellites using either thermal infrared (TIR) or ultraviolet (UV) instruments, sensitive to different portions of the atmosphere, making it difficult to gain a full picture. In this work, we combine measurements from the TIR and UV instruments Suomi NPP CrIS and Sentinel-5P/TROPOMI to improve sensitivity through the whole atmosphere and improve knowledge of ozone distribution.
Stuart Fox, Vinia Mattioli, Emma Turner, Alan Vance, Domenico Cimini, and Donatello Gallucci
Atmos. Meas. Tech., 17, 4957–4978, https://doi.org/10.5194/amt-17-4957-2024, https://doi.org/10.5194/amt-17-4957-2024, 2024
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Airborne observations are used to evaluate two models for absorption and emission by atmospheric gases, including water vapour and oxygen, at microwave and sub-millimetre wavelengths. These models are needed for the Ice Cloud Imager (ICI) on the next generation of European polar-orbiting weather satellites, which measures at frequencies up to 664 GHz. Both models can provide a good match to measurements from airborne radiometers and are sufficiently accurate for use with ICI.
Paul S. Jeffery, James R. Drummond, C. Thomas McElroy, Kaley A. Walker, and Jiansheng Zou
EGUsphere, https://doi.org/10.5194/egusphere-2024-2115, https://doi.org/10.5194/egusphere-2024-2115, 2024
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The MAESTRO instrument has been monitoring ozone and NO2 since February 2004. A new version of these data products has recently been released; however, these new products must be validated against other datasets to ensure their validity. This study presents such an assessment, using measurements from eleven satellite instruments to characterize the new MAESTRO products. In the stratosphere, good agreement is found for ozone and acceptable agreement is found for NO2 with these other datasets.
Marcel Bühler, Christoph Häni, Albrecht Neftel, Patrice Bühler, Christof Ammann, and Thomas Kupper
Atmos. Meas. Tech., 17, 4649–4658, https://doi.org/10.5194/amt-17-4649-2024, https://doi.org/10.5194/amt-17-4649-2024, 2024
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Methane was released from an artificial source inside a barn to test the applicability of the inverse dispersion method (IDM). Multiple open-path concentration devices and ultrasonic anemometers were used at the site. It is concluded that, for the present study case, the effect of a building and a tree in the main wind axis led to a systematic underestimation of the IDM-derived emission rate probably due to deviations in the wind field and turbulent dispersion from the ideal assumptions.
Arno Keppens, Serena Di Pede, Daan Hubert, Jean-Christopher Lambert, Pepijn Veefkind, Maarten Sneep, Johan De Haan, Mark ter Linden, Thierry Leblanc, Steven Compernolle, Tijl Verhoelst, José Granville, Oindrila Nath, Ann Mari Fjæraa, Ian Boyd, Sander Niemeijer, Roeland Van Malderen, Herman G. J. Smit, Valentin Duflot, Sophie Godin-Beekmann, Bryan J. Johnson, Wolfgang Steinbrecht, David W. Tarasick, Debra E. Kollonige, Ryan M. Stauffer, Anne M. Thompson, Angelika Dehn, and Claus Zehner
Atmos. Meas. Tech., 17, 3969–3993, https://doi.org/10.5194/amt-17-3969-2024, https://doi.org/10.5194/amt-17-3969-2024, 2024
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The Sentinel-5P satellite operated by the European Space Agency has carried the TROPOspheric Monitoring Instrument (TROPOMI) around the Earth since October 2017. This mission also produces atmospheric ozone profile data which are described in detail for May 2018 to April 2023. Independent validation using ground-based reference measurements demonstrates that the operational ozone profile product mostly fully and at least partially complies with all mission requirements.
Benedikt Herkommer, Carlos Alberti, Paolo Castracane, Jia Chen, Angelika Dehn, Florian Dietrich, Nicholas M. Deutscher, Matthias Max Frey, Jochen Groß, Lawson Gillespie, Frank Hase, Isamu Morino, Nasrin Mostafavi Pak, Brittany Walker, and Debra Wunch
Atmos. Meas. Tech., 17, 3467–3494, https://doi.org/10.5194/amt-17-3467-2024, https://doi.org/10.5194/amt-17-3467-2024, 2024
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The Total Carbon Column Observing Network is a network of ground-based Fourier transform infrared (FTIR) spectrometers used mainly for satellite validation. To ensure the highest-quality validation data, the network needs to be highly consistent. This is a major challenge, which so far is solved by site comparisons with airborne in situ measurements. In this work, we describe the use of a portable FTIR spectrometer as a travel standard for evaluating the consistency of TCCON sites.
Karen De Los Ríos, Paulina Ordoñez, Gabriele P. Stiller, Piera Raspollini, Marco Gai, Kaley A. Walker, Cristina Peña-Ortiz, and Luis Acosta
Atmos. Meas. Tech., 17, 3401–3418, https://doi.org/10.5194/amt-17-3401-2024, https://doi.org/10.5194/amt-17-3401-2024, 2024
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This study examines newer versions of H2O and HDO retrievals from Envisat/MIPAS and SCISAT/ACE-FTS. Results reveal a better agreement in stratospheric H2O profiles than in HDO profiles. The H2O tape recorder signal is consistent across databases, but δD tape recorder composites show differences that impact the interpretation of water vapour transport. These findings enhance the need for intercomparisons to refine our insights.
Ming Luo, Helen M. Worden, Robert D. Field, Kostas Tsigaridis, and Gregory S. Elsaesser
Atmos. Meas. Tech., 17, 2611–2624, https://doi.org/10.5194/amt-17-2611-2024, https://doi.org/10.5194/amt-17-2611-2024, 2024
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The TROPESS CrIS single-pixel CO profile retrievals are compared to the MOPITT CO products in steps of adjusting them to the common a priori assumptions. The two data sets are found to agree within 5 %. We also demonstrated and analyzed the proper steps in evaluating GISS ModelE CO simulations using satellite CO retrieval products for the western US wildfire events in September 2020.
Matthew S. Johnson, Alexei Rozanov, Mark Weber, Nora Mettig, John Sullivan, Michael J. Newchurch, Shi Kuang, Thierry Leblanc, Fernando Chouza, Timothy A. Berkoff, Guillaume Gronoff, Kevin B. Strawbridge, Raul J. Alvarez, Andrew O. Langford, Christoph J. Senff, Guillaume Kirgis, Brandi McCarty, and Larry Twigg
Atmos. Meas. Tech., 17, 2559–2582, https://doi.org/10.5194/amt-17-2559-2024, https://doi.org/10.5194/amt-17-2559-2024, 2024
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Monitoring tropospheric ozone (O3), a harmful pollutant negatively impacting human health, is primarily done using ground-based measurements and ozonesondes. However, these observation types lack the coverage to fully understand tropospheric O3. Satellites can retrieve tropospheric ozone with near-daily global coverage; however, they are known to have biases and errors. This study uses ground-based lidars to validate multiple satellites' ability to observe tropospheric O3.
Johan Mellqvist, Nathalia T. Vechi, Charlotte Scheutz, Marc Durif, Francois Gautier, John Johansson, Jerker Samuelsson, Brian Offerle, and Samuel Brohede
Atmos. Meas. Tech., 17, 2465–2479, https://doi.org/10.5194/amt-17-2465-2024, https://doi.org/10.5194/amt-17-2465-2024, 2024
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The solar occultation flux method retrieves ammonia gas columns from the solar spectrum. Emissions are obtained by multiplying the integrated plume concentration by the wind speed profile. The methodology for uncertainty estimation was established considering an error budget with systematic and random components, resulting in an expanded uncertainty in the range of 20 % to 30 %. The method was validated in a controlled release, and its application was demonstrated in different farms.
Felicia Kolonjari, Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, David A. Plummer, Andreas Engel, Stephen A. Montzka, David E. Oram, Tanja Schuck, Gabriele P. Stiller, and Geoffrey C. Toon
Atmos. Meas. Tech., 17, 2429–2449, https://doi.org/10.5194/amt-17-2429-2024, https://doi.org/10.5194/amt-17-2429-2024, 2024
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The Canadian Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) satellite instrument is currently providing the only vertically resolved chlorodifluoromethane (HCFC-22) measurements from space. This study assesses the most current ACE-FTS HCFC-22 data product in the upper troposphere and lower stratosphere, as well as modelled HCFC-22 from a 39-year run of the Canadian Middle Atmosphere Model (CMAM39) in the same region.
Emily Dowd, Alistair J. Manning, Bryn Orth-Lashley, Marianne Girard, James France, Rebecca E. Fisher, Dave Lowry, Mathias Lanoisellé, Joseph R. Pitt, Kieran M. Stanley, Simon O'Doherty, Dickon Young, Glen Thistlethwaite, Martyn P. Chipperfield, Emanuel Gloor, and Chris Wilson
Atmos. Meas. Tech., 17, 1599–1615, https://doi.org/10.5194/amt-17-1599-2024, https://doi.org/10.5194/amt-17-1599-2024, 2024
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We provide the first validation of the satellite-derived emission estimates using surface-based mobile greenhouse gas surveys of an active gas leak detected near Cheltenham, UK. GHGSat’s emission estimates broadly agree with the surface-based mobile survey and steps were taken to fix the leak, highlighting the importance of satellite data in identifying emissions and helping to reduce our human impact on climate change.
Astrid Müller, Hiroshi Tanimoto, Takafumi Sugita, Prabir K. Patra, Shin-ichiro Nakaoka, Toshinobu Machida, Isamu Morino, André Butz, and Kei Shiomi
Atmos. Meas. Tech., 17, 1297–1316, https://doi.org/10.5194/amt-17-1297-2024, https://doi.org/10.5194/amt-17-1297-2024, 2024
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Satellite CH4 observations with high accuracy are needed to understand changes in atmospheric CH4 concentrations. But over oceans, reference data are limited. We combine various ship and aircraft observations with the help of atmospheric chemistry models to derive observation-based column-averaged mixing ratios of CH4 (obs. XCH4). We discuss three different approaches and demonstrate the applicability of the new reference dataset for carbon cycle studies and satellite evaluation.
Evan D. Sherwin, Sahar H. El Abbadi, Philippine M. Burdeau, Zhan Zhang, Zhenlin Chen, Jeffrey S. Rutherford, Yuanlei Chen, and Adam R. Brandt
Atmos. Meas. Tech., 17, 765–782, https://doi.org/10.5194/amt-17-765-2024, https://doi.org/10.5194/amt-17-765-2024, 2024
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Countries and companies increasingly rely on a growing fleet of satellites to find large emissions of climate-warming methane, particularly from oil and natural gas systems across the globe. We independently assessed the performance of nine such systems by releasing controlled, undisclosed amounts of methane as satellites passed overhead. The tested systems produced reliable detection and quantification results, including the smallest-ever emission detected from space in such a test.
Luis F. Millán, Matthew D. Lebsock, Ken B. Cooper, Jose V. Siles, Robert Dengler, Raquel Rodriguez Monje, Amin Nehrir, Rory A. Barton-Grimley, James E. Collins, Claire E. Robinson, Kenneth L. Thornhill, and Holger Vömel
Atmos. Meas. Tech., 17, 539–559, https://doi.org/10.5194/amt-17-539-2024, https://doi.org/10.5194/amt-17-539-2024, 2024
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In this study, we describe and validate a new technique in which three radar tones are used to estimate the water vapor inside clouds and precipitation. This instrument flew on board NASA's P-3 aircraft during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) campaign and the Synergies Of Active optical and Active microwave Remote Sensing Experiment (SOA2RSE) campaign.
Ouyang Liu, Zhengqiang Li, Yangyan Lin, Cheng Fan, Ying Zhang, Kaitao Li, Peng Zhang, Yuanyuan Wei, Tianzeng Chen, Jiantao Dong, and Gerrit de Leeuw
Atmos. Meas. Tech., 17, 377–395, https://doi.org/10.5194/amt-17-377-2024, https://doi.org/10.5194/amt-17-377-2024, 2024
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Nitrogen dioxide (NO2) is a trace gas which is important for atmospheric chemistry and may affect human health. To understand processes leading to harmful concentrations, it is important to monitor NO2 concentrations near the surface and higher up. To this end, a Pandora instrument has been installed in Beijing. An overview of the first year of data shows the large variability on diurnal to seasonal timescales and how this is affected by wind speed and direction and chemistry.
Karen E. Cady-Pereira, Xuehui Guo, Rui Wang, April B. Leytem, Chase Calkins, Elizabeth Berry, Kang Sun, Markus Müller, Armin Wisthaler, Vivienne H. Payne, Mark W. Shephard, Mark A. Zondlo, and Valentin Kantchev
Atmos. Meas. Tech., 17, 15–36, https://doi.org/10.5194/amt-17-15-2024, https://doi.org/10.5194/amt-17-15-2024, 2024
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Ammonia is a significant precursor of PM2.5 particles and thus contributes to poor air quality in many regions. Furthermore, ammonia concentrations are rising due to the increase of large-scale, intensive agricultural activities. Here we evaluate satellite measurements of ammonia against aircraft and surface network data, and show that there are differences in magnitude, but the satellite data are spatially and temporally well correlated with the in situ data.
Alana K. Ayasse, Daniel Cusworth, Kelly O'Neill, Justin Fisk, Andrew K. Thorpe, and Riley Duren
Atmos. Meas. Tech., 16, 6065–6074, https://doi.org/10.5194/amt-16-6065-2023, https://doi.org/10.5194/amt-16-6065-2023, 2023
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Methane is a powerful greenhouse gas, and a significant portion of methane comes from large individual plumes. Recently, airplane-mounted infrared technologies have proven very good at detecting and quantifying these plumes. In order to extract the methane signal from the infrared image, there are two widely used approaches. In this study, we assess the performance of both approaches using controlled-release experiments. We also examine the minimum detection limit of the infrared technology.
Apisada Chulakadabba, Maryann Sargent, Thomas Lauvaux, Joshua S. Benmergui, Jonathan E. Franklin, Christopher Chan Miller, Jonas S. Wilzewski, Sébastien Roche, Eamon Conway, Amir H. Souri, Kang Sun, Bingkun Luo, Jacob Hawthrone, Jenna Samra, Bruce C. Daube, Xiong Liu, Kelly Chance, Yang Li, Ritesh Gautam, Mark Omara, Jeff S. Rutherford, Evan D. Sherwin, Adam Brandt, and Steven C. Wofsy
Atmos. Meas. Tech., 16, 5771–5785, https://doi.org/10.5194/amt-16-5771-2023, https://doi.org/10.5194/amt-16-5771-2023, 2023
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We show that MethaneAIR, a precursor to the MethaneSAT satellite, demonstrates accurate point source quantification during controlled release experiments and regional observations in 2021 and 2022. Results from our two independent quantification methods suggest the accuracy of our sensor and algorithms is better than 25 % for sources emitting 200 kg h−1 or more. Insights from these measurements help establish the capabilities of MethaneSAT and MethaneAIR.
Kanghyun Baek, Jae Hwan Kim, Juseon Bak, David P. Haffner, Mina Kang, and Hyunkee Hong
Atmos. Meas. Tech., 16, 5461–5478, https://doi.org/10.5194/amt-16-5461-2023, https://doi.org/10.5194/amt-16-5461-2023, 2023
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The GEMS mission was the first mission of the geostationary satellite constellation for hourly atmospheric composition monitoring. The GEMS ozone measurements were cross-compared to those of Pandora, OMPS, and TROPOMI satellite sensors and excellent agreement was found. GEMS has proven to be a powerful new instrument for monitoring and assessing the diurnal variation in atmospheric ozone. This experience can be used to advance research with future geostationary environmental satellite missions.
Tobias Christoph Valentin Werner Riess, Klaas Folkert Boersma, Ward Van Roy, Jos de Laat, Enrico Dammers, and Jasper van Vliet
Atmos. Meas. Tech., 16, 5287–5304, https://doi.org/10.5194/amt-16-5287-2023, https://doi.org/10.5194/amt-16-5287-2023, 2023
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Satellite retrievals of trace gases require prior knowledge of the vertical distribution of the pollutant, which is usually obtained from models. Using aircraft-measured vertical NO2 profiles over the North Sea in summer 2021, we evaluate the Transport Model 5 profiles used in the TROPOMI NO2 retrieval. We conclude that driven by the low horizontal resolution and the overestimated vertical mixing, resulting NO2 columns are 20 % too low. This has important implications for emission estimates.
Thomas Trickl, Martin Adelwart, Dina Khordakova, Ludwig Ries, Christian Rolf, Michael Sprenger, Wolfgang Steinbrecht, and Hannes Vogelmann
Atmos. Meas. Tech., 16, 5145–5165, https://doi.org/10.5194/amt-16-5145-2023, https://doi.org/10.5194/amt-16-5145-2023, 2023
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Tropospheric ozone have been measured for more than a century. Highly quantitative ozone measurements have been made at monitoring stations. However, deficits have been reported for vertical sounding systems. Here, we report a thorough intercomparison effort between a differential-absorption lidar system and two types of balloon-borne ozone sondes, also using ozone sensors at nearby mountain sites as references. The sondes agree very well with the lidar after offset corrections.
Rodriguez Yombo Phaka, Alexis Merlaud, Gaia Pinardi, Martina M. Friedrich, Michel Van Roozendael, Jean-François Müller, Trissevgeni Stavrakou, Isabelle De Smedt, François Hendrick, Ermioni Dimitropoulou, Richard Bopili Mbotia Lepiba, Edmond Phuku Phuati, Buenimio Lomami Djibi, Lars Jacobs, Caroline Fayt, Jean-Pierre Mbungu Tsumbu, and Emmanuel Mahieu
Atmos. Meas. Tech., 16, 5029–5050, https://doi.org/10.5194/amt-16-5029-2023, https://doi.org/10.5194/amt-16-5029-2023, 2023
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We present air quality measurements in Kinshasa, Democratic Republic of the Congo, performed with a newly developed instrument which was installed on a roof of the University of Kinshasa in November 2019. The instrument records spectra of the scattered sunlight, from which we derive the abundances of nitrogen dioxide and formaldehyde, two important pollutants. We compare our ground-based measurements with those of the TROPOspheric Monitoring Instrument (TROPOMI).
Jay Herman, Jerald Ziemke, and Richard McPeters
Atmos. Meas. Tech., 16, 4693–4707, https://doi.org/10.5194/amt-16-4693-2023, https://doi.org/10.5194/amt-16-4693-2023, 2023
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Fourier series multivariate linear regression trends (% per decade) in ozone were estimated from the Merged Ozone Data Set (MOD) from 1979 to 2021 in two different regimes, from 1979 to TA (the date when ozone stopped decreasing) and TA to 2021. The derived TA is a latitude-dependent date, ranging from 1994 to 1998. TA(θ) is a marker for photochemistry dynamics models attempting to represent ozone change over the past 42 years.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
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We quantify biases and drifts (and their uncertainties) between the stratospheric water vapor measurement records of 15 satellite-based instruments (SATs, with 31 different retrievals) and balloon-borne frost point hygrometers (FPs) launched at 27 globally distributed stations. These comparisons of measurements during the period 2000–2016 are made using robust, consistent statistical methods. With some exceptions, the biases and drifts determined for most SAT–FP pairs are < 10 % and < 1 % yr−1.
Tim A. van Kempen, Tim J. Rotmans, Richard M. van Hees, Carol Bruegge, Dejian Fu, Ruud Hoogeveen, Thomas J. Pongetti, Robert Rosenberg, and Ilse Aben
Atmos. Meas. Tech., 16, 4507–4527, https://doi.org/10.5194/amt-16-4507-2023, https://doi.org/10.5194/amt-16-4507-2023, 2023
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Validation of satellite measurements is essential for providing reliable and consistent products. In this paper, a validation method for TROPOMI-SWIR (Tropospheric Measurement Instrument in the short-wavelength infrared) is explored. TROPOMI-SWIR has been shown to be exceptionally stable, a necessity to explore the methodology. Railroad Valley, Nevada, is a prime location to perform the necessary measurements to validate the satellite measurements of TROPOMI-SWIR.
Serin Kim, Daewon Kim, Hyunkee Hong, Lim-Seok Chang, Hanlim Lee, Deok-Rae Kim, Donghee Kim, Jeong-Ah Yu, Dongwon Lee, Ukkyo Jeong, Chang-Kuen Song, Sang-Woo Kim, Sang Seo Park, Jhoon Kim, Thomas F. Hanisco, Junsung Park, Wonei Choi, and Kwangyul Lee
Atmos. Meas. Tech., 16, 3959–3972, https://doi.org/10.5194/amt-16-3959-2023, https://doi.org/10.5194/amt-16-3959-2023, 2023
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A first evaluation of the Geostationary Environmental Monitoring Spectrometer (GEMS) NO2 was carried out via comparison with the NO2 data obtained from the ground-based Pandora direct-sun measurements at four sites in Seosan, Republic of Korea. Comparisons between GEMS NO2 and Pandora NO2 were performed according to GEMS cloud fraction. GEMS NO2 showed good agreement with that of Pandora NO2 under less cloudy conditions.
Nicholas Balasus, Daniel J. Jacob, Alba Lorente, Joannes D. Maasakkers, Robert J. Parker, Hartmut Boesch, Zichong Chen, Makoto M. Kelp, Hannah Nesser, and Daniel J. Varon
Atmos. Meas. Tech., 16, 3787–3807, https://doi.org/10.5194/amt-16-3787-2023, https://doi.org/10.5194/amt-16-3787-2023, 2023
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We use machine learning to remove biases in TROPOMI satellite observations of atmospheric methane, with GOSAT observations serving as a reference. We find that the TROPOMI biases relative to GOSAT are related to the presence of aerosols and clouds, the surface brightness, and the specific detector that makes the observation aboard TROPOMI. The resulting blended TROPOMI+GOSAT product is more reliable for quantifying methane emissions.
Thomas E. Taylor, Christopher W. O'Dell, David Baker, Carol Bruegge, Albert Chang, Lars Chapsky, Abhishek Chatterjee, Cecilia Cheng, Frédéric Chevallier, David Crisp, Lan Dang, Brian Drouin, Annmarie Eldering, Liang Feng, Brendan Fisher, Dejian Fu, Michael Gunson, Vance Haemmerle, Graziela R. Keller, Matthäus Kiel, Le Kuai, Thomas Kurosu, Alyn Lambert, Joshua Laughner, Richard Lee, Junjie Liu, Lucas Mandrake, Yuliya Marchetti, Gregory McGarragh, Aronne Merrelli, Robert R. Nelson, Greg Osterman, Fabiano Oyafuso, Paul I. Palmer, Vivienne H. Payne, Robert Rosenberg, Peter Somkuti, Gary Spiers, Cathy To, Brad Weir, Paul O. Wennberg, Shanshan Yu, and Jia Zong
Atmos. Meas. Tech., 16, 3173–3209, https://doi.org/10.5194/amt-16-3173-2023, https://doi.org/10.5194/amt-16-3173-2023, 2023
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NASA's Orbiting Carbon Observatory 2 and 3 (OCO-2 and OCO-3, respectively) provide complementary spatiotemporal coverage from a sun-synchronous and precession orbit, respectively. Estimates of total column carbon dioxide (XCO2) derived from the two sensors using the same retrieval algorithm show broad consistency over a 2.5-year overlapping time record. This suggests that data from the two satellites may be used together for scientific analysis.
Lena Katharina Jänicke, Rene Preusker, Marco Celesti, Marin Tudoroiu, Jürgen Fischer, Dirk Schüttemeyer, and Matthias Drusch
Atmos. Meas. Tech., 16, 3101–3121, https://doi.org/10.5194/amt-16-3101-2023, https://doi.org/10.5194/amt-16-3101-2023, 2023
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To compare two top-of-atmosphere radiances measured by instruments with different spectral characteristics, a transfer function has been developed. It is applied to a tandem data set of Sentinel-3A and B, for which OLCI-B mimicked the ESA’s eighth Earth Explorer FLEX. We found that OLCI-A measured radiances about 2 % brighter than OLCI-FLEX. Only at larger wavelengths were OLCI-A measurements about 5 % darker. The method is thus successful, being sensitive to calibration and processing issues.
Luis F. Millán, Gloria L. Manney, Harald Boenisch, Michaela I. Hegglin, Peter Hoor, Daniel Kunkel, Thierry Leblanc, Irina Petropavlovskikh, Kaley Walker, Krzysztof Wargan, and Andreas Zahn
Atmos. Meas. Tech., 16, 2957–2988, https://doi.org/10.5194/amt-16-2957-2023, https://doi.org/10.5194/amt-16-2957-2023, 2023
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The determination of atmospheric composition trends in the upper troposphere and lower stratosphere (UTLS) is still highly uncertain. We present the creation of dynamical diagnostics to map several ozone datasets (ozonesondes, lidars, aircraft, and satellite measurements) in geophysically based coordinate systems. The diagnostics can also be used to analyze other greenhouse gases relevant to surface climate and UTLS chemistry.
Zhihua Zhang, Jianguo Niu, Lawrence E. Flynn, Eric Beach, and Trevor Beck
Atmos. Meas. Tech., 16, 2919–2941, https://doi.org/10.5194/amt-16-2919-2023, https://doi.org/10.5194/amt-16-2919-2023, 2023
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This study mainly focused on addressing stability and improvement when using a broadband approach, establishing soft-calibration adjustments for both OMPS S-NPP and N20, analyzing error biases based on multi-sensor bias correction, and comparing total column ozone and aerosol index retrievals from NOAA OMPS with those from other products.
Matthew S. Johnson, Amir H. Souri, Sajeev Philip, Rajesh Kumar, Aaron Naeger, Jeffrey Geddes, Laura Judd, Scott Janz, Heesung Chong, and John Sullivan
Atmos. Meas. Tech., 16, 2431–2454, https://doi.org/10.5194/amt-16-2431-2023, https://doi.org/10.5194/amt-16-2431-2023, 2023
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Satellites provide vital information for studying the processes controlling ozone formation. Based on the abundance of particular gases in the atmosphere, ozone formation is sensitive to specific human-induced and natural emission sources. However, errors and biases in satellite retrievals hinder this data source’s application for studying ozone formation sensitivity. We conducted a thorough statistical evaluation of two commonly applied satellites for investigating ozone formation sensitivity.
Kezia Lange, Andreas Richter, Anja Schönhardt, Andreas C. Meier, Tim Bösch, André Seyler, Kai Krause, Lisa K. Behrens, Folkard Wittrock, Alexis Merlaud, Frederik Tack, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Vinod Kumar, Sebastian Donner, Steffen Dörner, Bianca Lauster, Maria Razi, Christian Borger, Katharina Uhlmannsiek, Thomas Wagner, Thomas Ruhtz, Henk Eskes, Birger Bohn, Daniel Santana Diaz, Nader Abuhassan, Dirk Schüttemeyer, and John P. Burrows
Atmos. Meas. Tech., 16, 1357–1389, https://doi.org/10.5194/amt-16-1357-2023, https://doi.org/10.5194/amt-16-1357-2023, 2023
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We present airborne imaging DOAS and ground-based stationary and car DOAS measurements conducted during the S5P-VAL-DE-Ruhr campaign in the Rhine-Ruhr region. The measurements are used to validate spaceborne NO2 data products from the Sentinel-5 Precursor TROPOspheric Monitoring Instrument (TROPOMI). Auxiliary data of the TROPOMI NO2 retrieval, such as spatially higher resolved a priori NO2 vertical profiles, surface reflectivity, and cloud treatment are investigated to evaluate their impact.
Yolanda Maria Lemes, Christoph Häni, Jesper Nørlem Kamp, and Anders Feilberg
Atmos. Meas. Tech., 16, 1295–1309, https://doi.org/10.5194/amt-16-1295-2023, https://doi.org/10.5194/amt-16-1295-2023, 2023
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The implementation of a new method, line-averaged concentration measurement with a closed-path analyzer, will enable the measurement of fluxes of multiple gases from different types of sources and will evaluate the effects of mitigation strategies on emissions. In addition, this method allows for continuous online measurements that resolve temporal variation in ammonia emissions and the peak emissions of methane.
Prajjwal Rawat, Manish Naja, Evan Fishbein, Pradeep K. Thapliyal, Rajesh Kumar, Piyush Bhardwaj, Aditya Jaiswal, Sugriva N. Tiwari, Sethuraman Venkataramani, and Shyam Lal
Atmos. Meas. Tech., 16, 889–909, https://doi.org/10.5194/amt-16-889-2023, https://doi.org/10.5194/amt-16-889-2023, 2023
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Satellite-based ozone observations have gained importance due to their global coverage. However, satellite-retrieved products are indirect and need to be validated, particularly over mountains. Ozonesondes launched from a Himalayan site are used to assess the Atmospheric Infrared Sounder (AIRS) ozone retrieval. AIRS is shown to overestimate ozone in the upper troposphere and lower stratosphere, while the differences from ozonesondes are more minor in the middle troposphere and stratosphere.
Murali Natarajan, Robert Damadeo, and David Flittner
Atmos. Meas. Tech., 16, 75–87, https://doi.org/10.5194/amt-16-75-2023, https://doi.org/10.5194/amt-16-75-2023, 2023
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Photochemically induced changes in mesospheric O3 concentration at twilight can cause asymmetry in the distribution along the line of sight of solar occultation observations that must be considered in the retrieval algorithm. Correction factors developed from diurnal photochemical model simulations were used to modify the archived SAGE III/ISS mesospheric O3 concentrations. For June 2021 the bias caused by the neglect of diurnal variations is over 30% at 64 km altitude and low latitudes.
Javier Gorroño, Daniel J. Varon, Itziar Irakulis-Loitxate, and Luis Guanter
Atmos. Meas. Tech., 16, 89–107, https://doi.org/10.5194/amt-16-89-2023, https://doi.org/10.5194/amt-16-89-2023, 2023
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We present a methane flux rate retrieval methodology using the Sentinel-2 mission, validating the algorithm for different scenes and plumes. The detection limit is 1000–2000 kg h−1 for homogeneous scenes and temporally invariant surfaces and above 5000 kg h−1 for heterogeneous ones. Dominant quantification errors are wind-related or plume mask-related. For heterogeneous scenes, the surface structure underlying the methane plume can become a dominant source of uncertainty.
Katerina Garane, Ka Lok Chan, Maria-Elissavet Koukouli, Diego Loyola, and Dimitris Balis
Atmos. Meas. Tech., 16, 57–74, https://doi.org/10.5194/amt-16-57-2023, https://doi.org/10.5194/amt-16-57-2023, 2023
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In this work, 2.5 years of TROPOMI/S5P Total Column Water Vapor (TCWV) observations retrieved from the blue wavelength band are validated against co-located precipitable water measurements from NASA AERONET, which uses Cimel Sun photometers globally. Overall, the TCWV product agrees well on a global scale with the ground-based dataset (Pearson correl. coefficient 0.909) and has a mean relative bias of −2.7 ± 4.9 % with respect to the AERONET observations for moderate albedo and cloudiness.
Lei Shi, Carl J. Schreck III, Viju O. John, Eui-Seok Chung, Theresa Lang, Stefan A. Buehler, and Brian J. Soden
Atmos. Meas. Tech., 15, 6949–6963, https://doi.org/10.5194/amt-15-6949-2022, https://doi.org/10.5194/amt-15-6949-2022, 2022
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Four upper tropospheric humidity (UTH) datasets derived from satellite microwave and infrared sounders are evaluated to assess their consistency as part of the activities for the Global Energy and Water Exchanges (GEWEX) water vapor assessment project. The study shows that the four datasets are consistent in the interannual temporal and spatial variability of the tropics. However, differences are found in the magnitudes of the anomalies and in the changing rates during the common period.
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Short summary
Our paper discusses the structure function method, which allows validation of random uncertainties in the data and, at the same time, probing of the small-scale natural variability. We applied this method to the clear-sky total ozone measurements by TROPOMI Sentinel-5P satellite instrument and found that the TROPOMI random error estimation is adequate. The discussed method is a powerful tool, which can be used in various applications.
Our paper discusses the structure function method, which allows validation of random...
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