Articles | Volume 13, issue 12
https://doi.org/10.5194/amt-13-6755-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-13-6755-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Quantifying the impact of aerosol scattering on the retrieval of methane from airborne remote sensing measurements
Yunxia Huang
School of Science, Nantong University, Nantong, 226007, China
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA 91125, USA
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA 91109, USA
Zhao-Cheng Zeng
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA 91125, USA
Joint Institute for Regional Earth System Science and Engineering,
University of California, Los Angeles, CA 90095, USA
Pushkar Kopparla
Graduate School of Frontier Sciences, The University of Tokyo,
Kashiwa, Chiba 277-0882, Japan
Yuk L. Yung
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA 91125, USA
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA 91109, USA
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Edward Malina, Kevin W. Bowman, Valentin Kantchev, Le Kuai, Thomas P. Kurosu, Kazuyuki Miyazaki, Vijay Natraj, Gregory B. Osterman, Fabiano Oyafuso, and Matthew D. Thill
Atmos. Meas. Tech., 17, 5341–5371, https://doi.org/10.5194/amt-17-5341-2024, https://doi.org/10.5194/amt-17-5341-2024, 2024
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Characterizing the distribution of ozone in the atmosphere is a challenging problem, with current Earth observation satellites using either thermal infrared (TIR) or ultraviolet (UV) instruments, sensitive to different portions of the atmosphere, making it difficult to gain a full picture. In this work, we combine measurements from the TIR and UV instruments Suomi NPP CrIS and Sentinel-5P/TROPOMI to improve sensitivity through the whole atmosphere and improve knowledge of ozone distribution.
Jan-Lukas Tirpitz, Santo Fedele Colosimo, Nathaniel Brockway, Robert Spurr, Matt Christi, Samuel Hall, Kirk Ullmann, Johnathan Hair, Taylor Shingler, Rodney Weber, Jack Dibb, Richard Moore, Elizabeth Wiggins, Vijay Natraj, Nicolas Theys, and Jochen Stutz
EGUsphere, https://doi.org/10.5194/egusphere-2024-2353, https://doi.org/10.5194/egusphere-2024-2353, 2024
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To calculate distributions of actinic flux and photolysis frequencies in a wildfire plume, we combine plume composition data from the 2019 NASA FIREX-AQ campaign with state-of-the-art radiative transfer modeling techniques. Excellent agreement of model and observations demonstrates the applicability of this approach to constrain photochemistry in such plumes. We identify limiting factors for the modeling accuracy and discuss spatial and spectral features of the distributions.
Zhonghua He, Ling Gao, Miao Liang, and Zhao-Cheng Zeng
Atmos. Meas. Tech., 17, 2937–2956, https://doi.org/10.5194/amt-17-2937-2024, https://doi.org/10.5194/amt-17-2937-2024, 2024
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Using Gaofen-5B satellite data, this study detected 93 methane plume events from 32 coal mines in Shanxi, China, with emission rates spanning from 761.78 ± 185.00 to 12729.12 ± 4658.13 kg h-1, showing significant variability among sources. This study highlights Gaofen-5B’s capacity for monitoring large methane point sources, offering valuable support in reducing greenhouse gas emissions.
Santo Fedele Colosimo, Nathaniel Brockway, Vijay Natraj, Robert Spurr, Klaus Pfeilsticker, Lisa Scalone, Max Spolaor, Sarah Woods, and Jochen Stutz
Atmos. Meas. Tech., 17, 2367–2385, https://doi.org/10.5194/amt-17-2367-2024, https://doi.org/10.5194/amt-17-2367-2024, 2024
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Cirrus clouds are poorly understood components of the climate system, in part due to the challenge of observing thin, sub-visible ice clouds. We address this issue with a new observational approach that uses the remote sensing of near-infrared ice water absorption features from a high-altitude aircraft. We describe the underlying principle of this approach and present a new procedure to retrieve ice concentration in cirrus clouds. Our retrievals compare well with in situ observations.
Zhao-Cheng Zeng, Lu Lee, Chengli Qi, Lieven Clarisse, and Martin Van Damme
Atmos. Meas. Tech., 16, 3693–3713, https://doi.org/10.5194/amt-16-3693-2023, https://doi.org/10.5194/amt-16-3693-2023, 2023
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This study presents an NH3 retrieval algorithm based on the optimal estimation method for the Geostationary Interferometric Infrared Sounder (GIIRS) on board China’s FengYun-4B satellite (FY-4B/GIIRS). Retrieval results demonstrate the capability of FY-4B/GIIRS in capturing the diurnal NH3 changes in East Asia. This operational geostationary observation by FY-4B/GIIRS represents an important advancement over the twice-per-day observations provided by current low-Earth-orbit (LEO) instruments.
Yuan Wang, Xiaojian Zheng, Xiquan Dong, Baike Xi, and Yuk L. Yung
Atmos. Chem. Phys., 23, 8591–8605, https://doi.org/10.5194/acp-23-8591-2023, https://doi.org/10.5194/acp-23-8591-2023, 2023
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Marine boundary layer clouds remain poorly predicted in global climate models due to multiple entangled uncertainty sources. This study uses the in situ observations from a recent field campaign to constrain and evaluate cloud physics in a simplified version of a climate model. Progress and remaining issues in the cloud physics parameterizations are identified. We systematically evaluate the impacts of large-scale forcing, microphysical scheme, and aerosol concentrations on the cloud property.
Zhao-Cheng Zeng, Lu Lee, and Chengli Qi
Atmos. Meas. Tech., 16, 3059–3083, https://doi.org/10.5194/amt-16-3059-2023, https://doi.org/10.5194/amt-16-3059-2023, 2023
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Observations from geostationary orbit provide contiguous coverage with a high temporal resolution, representing an important advancement over current low-Earth-orbit instruments. Using measurements from GIIRS on board China's FengYun satellite, the world’s first geostationary hyperspectral infrared sounder, we showed the first results of diurnal CO in eastern Asia from a geostationary orbit, which will have great potential in improving local and global air quality and climate research.
Vijay Natraj, Ming Luo, Jean-Francois Blavier, Vivienne H. Payne, Derek J. Posselt, Stanley P. Sander, Zhao-Cheng Zeng, Jessica L. Neu, Denis Tremblay, Longtao Wu, Jacola A. Roman, Yen-Hung Wu, and Leonard I. Dorsky
Atmos. Meas. Tech., 15, 1251–1267, https://doi.org/10.5194/amt-15-1251-2022, https://doi.org/10.5194/amt-15-1251-2022, 2022
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High-fidelity monitoring and forecast of air quality and the hydrological cycle require understanding the vertical distribution of temperature, humidity, and trace gases at high spatiotemporal resolution. We describe a new instrument concept, called the JPL GEO-IR Sounder, that would provide this information for the first time from a single instrument platform. Simulations demonstrate the benefits of combining measurements from multiple wavelengths for this purpose from geostationary orbit.
Siraput Jongaramrungruang, Georgios Matheou, Andrew K. Thorpe, Zhao-Cheng Zeng, and Christian Frankenberg
Atmos. Meas. Tech., 14, 7999–8017, https://doi.org/10.5194/amt-14-7999-2021, https://doi.org/10.5194/amt-14-7999-2021, 2021
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This study shows how precision error and bias in column methane retrieval change with different instrument specifications and the impact of spectrally complex surface albedos on retrievals. We show how surface interferences can be mitigated with an optimal spectral resolution and a higher polynomial degree in a retrieval process. The findings can inform future satellite instrument designs to have robust observations capable of separating real CH4 plume enhancements from surface interferences.
King-Fai Li, Ryan Khoury, Thomas J. Pongetti, Stanley P. Sander, Franklin P. Mills, and Yuk L. Yung
Atmos. Meas. Tech., 14, 7495–7510, https://doi.org/10.5194/amt-14-7495-2021, https://doi.org/10.5194/amt-14-7495-2021, 2021
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Nitrogen dioxide (NO2) plays a dominant role in the stratospheric ozone-destroying catalytic cycle. We have retrieved the diurnal cycle of NO2 over Table Mountain in Southern California, USA, during a week in October 2018. Under clean conditions, we are able to predict the diurnal cycle using standard photochemistry. On a day with significant pollution, we see the effect of NO2 sources in the nearby Los Angeles Basin.
Zhao-Cheng Zeng, Vijay Natraj, Feng Xu, Sihe Chen, Fang-Ying Gong, Thomas J. Pongetti, Keeyoon Sung, Geoffrey Toon, Stanley P. Sander, and Yuk L. Yung
Atmos. Meas. Tech., 14, 6483–6507, https://doi.org/10.5194/amt-14-6483-2021, https://doi.org/10.5194/amt-14-6483-2021, 2021
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Large carbon source regions such as megacities are also typically associated with heavy aerosol loading, which introduces uncertainties in the retrieval of greenhouse gases from reflected and scattered sunlight measurements. In this study, we developed a full physics algorithm to retrieve greenhouse gases in the presence of aerosols and demonstrated its performance by retrieving CO2 and CH4 columns from remote sensing measurements in the Los Angeles megacity.
Yuan Wang, Xiaojian Zheng, Xiquan Dong, Baike Xi, Peng Wu, Timothy Logan, and Yuk L. Yung
Atmos. Chem. Phys., 20, 14741–14755, https://doi.org/10.5194/acp-20-14741-2020, https://doi.org/10.5194/acp-20-14741-2020, 2020
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A recent aircraft field campaign near the Azores in the summer of 2017 provides ample observations of aerosols and clouds with detailed vertical information. This study utilizes those observational data in combination with the aerosol-aware large-eddy simulations and aerosol reanalysis data to examine the significance of the long-range-transported aerosol effect on marine-boundary-layer clouds. It is the first time that the ACE-ENA aircraft campaign data are used for this topic.
Brigitte Rooney, Yuan Wang, Jonathan H. Jiang, Bin Zhao, Zhao-Cheng Zeng, and John H. Seinfeld
Atmos. Chem. Phys., 20, 14597–14616, https://doi.org/10.5194/acp-20-14597-2020, https://doi.org/10.5194/acp-20-14597-2020, 2020
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Wildfires have become increasingly prevalent. Intense smoke consisting of particulate matter (PM) leads to an increased risk of morbidity and mortality. The record-breaking Camp Fire ravaged Northern California for two weeks in 2018. Here, we employ a comprehensive chemical transport model along with ground-based and satellite observations to characterize the PM concentrations across Northern California and to investigate the pollution sensitivity predictions to key parameters of the model.
Brian D. Bue, David R. Thompson, Shubhankar Deshpande, Michael Eastwood, Robert O. Green, Vijay Natraj, Terry Mullen, and Mario Parente
Atmos. Meas. Tech., 12, 2567–2578, https://doi.org/10.5194/amt-12-2567-2019, https://doi.org/10.5194/amt-12-2567-2019, 2019
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Imaging spectrometers provide valuable remote measurements of Earth's surface and atmosphere. These measurements rely on computationally expensive radiative transfer models (RTMs). Spectrometers produce too much data to process with RTMs directly, requiring approximations that trade accuracy for speed. We demonstrate that neural networks can quickly emulate RTM calculations more accurately than current approaches, enabling the application of more sophisticated RTMs than current methods permit.
Christopher W. O'Dell, Annmarie Eldering, Paul O. Wennberg, David Crisp, Michael R. Gunson, Brendan Fisher, Christian Frankenberg, Matthäus Kiel, Hannakaisa Lindqvist, Lukas Mandrake, Aronne Merrelli, Vijay Natraj, Robert R. Nelson, Gregory B. Osterman, Vivienne H. Payne, Thomas E. Taylor, Debra Wunch, Brian J. Drouin, Fabiano Oyafuso, Albert Chang, James McDuffie, Michael Smyth, David F. Baker, Sourish Basu, Frédéric Chevallier, Sean M. R. Crowell, Liang Feng, Paul I. Palmer, Mavendra Dubey, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, Coleen M. Roehl, Mahesh K. Sha, Kimberly Strong, Ralf Sussmann, Yao Te, Osamu Uchino, and Voltaire A. Velazco
Atmos. Meas. Tech., 11, 6539–6576, https://doi.org/10.5194/amt-11-6539-2018, https://doi.org/10.5194/amt-11-6539-2018, 2018
Si-Wan Kim, Vijay Natraj, Seoyoung Lee, Hyeong-Ahn Kwon, Rokjin Park, Joost de Gouw, Gregory Frost, Jhoon Kim, Jochen Stutz, Michael Trainer, Catalina Tsai, and Carsten Warneke
Atmos. Chem. Phys., 18, 7639–7655, https://doi.org/10.5194/acp-18-7639-2018, https://doi.org/10.5194/acp-18-7639-2018, 2018
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Formaldehyde (HCHO) is a hazardous air pollutant and is associated with tropospheric ozone production. HCHO has been monitored from space. In this study, to acquire high-quality satellite-based HCHO observations, we utilize fine-resolution atmospheric chemistry model results as an input to the computer code for satellite retrievals over the Los Angeles Basin. Our study indicates that the use of fine-resolution profile shapes helps to identify HCHO plumes from space.
Zhao-Cheng Zeng, Qiong Zhang, Vijay Natraj, Jack S. Margolis, Run-Lie Shia, Sally Newman, Dejian Fu, Thomas J. Pongetti, Kam W. Wong, Stanley P. Sander, Paul O. Wennberg, and Yuk L. Yung
Atmos. Chem. Phys., 17, 2495–2508, https://doi.org/10.5194/acp-17-2495-2017, https://doi.org/10.5194/acp-17-2495-2017, 2017
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We propose a novel approach to describing the scattering effects of atmospheric aerosols using H2O retrievals in the near infrared. We found that the aerosol scattering effect is the primary contributor to the variations in the wavelength dependence of the H2O SCD retrievals and the scattering effects can be derived using H2O retrievals from multiple bands. This proposed method could potentially contribute towards reducing biases in greenhouse gas retrievals from space.
Clare K. Wong, Thomas J. Pongetti, Tom Oda, Preeti Rao, Kevin R. Gurney, Sally Newman, Riley M. Duren, Charles E. Miller, Yuk L. Yung, and Stanley P. Sander
Atmos. Chem. Phys., 16, 13121–13130, https://doi.org/10.5194/acp-16-13121-2016, https://doi.org/10.5194/acp-16-13121-2016, 2016
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Methane is the second most important greenhouse gas and a target of new emissions regulations in the United States. Despite its importance, its emissions are poorly understood. In this study, we used a remote sensing instrument located on Mount Wilson to estimate the monthly and annual methane emissions from Los Angeles. Derived methane emissions from Los Angeles showed consistent peaks in late summer/early fall and winter during the study period from 2011 to 2015.
Sha Feng, Thomas Lauvaux, Sally Newman, Preeti Rao, Ravan Ahmadov, Aijun Deng, Liza I. Díaz-Isaac, Riley M. Duren, Marc L. Fischer, Christoph Gerbig, Kevin R. Gurney, Jianhua Huang, Seongeun Jeong, Zhijin Li, Charles E. Miller, Darragh O'Keeffe, Risa Patarasuk, Stanley P. Sander, Yang Song, Kam W. Wong, and Yuk L. Yung
Atmos. Chem. Phys., 16, 9019–9045, https://doi.org/10.5194/acp-16-9019-2016, https://doi.org/10.5194/acp-16-9019-2016, 2016
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We developed a high-resolution land–atmosphere modelling system for urban CO2 emissions over the LA Basin. We evaluated various model configurations, FFCO2 products, and the impact of the model resolution. FFCO2 emissions outpace the atmospheric model resolution to represent the CO2 concentration variability across the basin. A novel forward model approach is presented to evaluate the surface measurement network, reinforcing the importance of using high-resolution emission products.
Sally Newman, Xiaomei Xu, Kevin R. Gurney, Ying Kuang Hsu, King Fai Li, Xun Jiang, Ralph Keeling, Sha Feng, Darragh O'Keefe, Risa Patarasuk, Kam Weng Wong, Preeti Rao, Marc L. Fischer, and Yuk L. Yung
Atmos. Chem. Phys., 16, 3843–3863, https://doi.org/10.5194/acp-16-3843-2016, https://doi.org/10.5194/acp-16-3843-2016, 2016
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Combining 14C and 13C data from the Los Angeles, CA megacity with background data allows source attribution of CO2 emissions among biosphere, natural gas, and gasoline. The 8-year record of CO2 emissions from fossil fuel burning is consistent with "The Great Recession" of 2008–2010. The long-term trend and source attribution are consistent with government inventories. Seasonal patterns agree with the high-resolution Hestia-LA emission data product, when seasonal wind directions are considered.
X. Xi, V. Natraj, R. L. Shia, M. Luo, Q. Zhang, S. Newman, S. P. Sander, and Y. L. Yung
Atmos. Meas. Tech., 8, 4817–4830, https://doi.org/10.5194/amt-8-4817-2015, https://doi.org/10.5194/amt-8-4817-2015, 2015
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The Geostationary Fourier Transform Spectrometer (GeoFTS) is designed to measure high-resolution spectra of reflected sunlight in near-infrared bands and to deliver simultaneous retrievals of column-averaged dry air mole fractions of CO2, CH4, CO, and H2O at different times of day. We perform radiative transfer simulations over both clear-sky and all-sky scenes and estimate the prospective performance of retrievals based on results from Bayesian error analysis and characterization.
K. W. Wong, D. Fu, T. J. Pongetti, S. Newman, E. A. Kort, R. Duren, Y.-K. Hsu, C. E. Miller, Y. L. Yung, and S. P. Sander
Atmos. Chem. Phys., 15, 241–252, https://doi.org/10.5194/acp-15-241-2015, https://doi.org/10.5194/acp-15-241-2015, 2015
E. Hache, J.-L. Attié, C. Tourneur, P. Ricaud, L. Coret, W. A. Lahoz, L. El Amraoui, B. Josse, P. Hamer, J. Warner, X. Liu, K. Chance, M. Höpfner, R. Spurr, V. Natraj, S. Kulawik, A. Eldering, and J. Orphal
Atmos. Meas. Tech., 7, 2185–2201, https://doi.org/10.5194/amt-7-2185-2014, https://doi.org/10.5194/amt-7-2185-2014, 2014
D. Fu, J. R. Worden, X. Liu, S. S. Kulawik, K. W. Bowman, and V. Natraj
Atmos. Chem. Phys., 13, 3445–3462, https://doi.org/10.5194/acp-13-3445-2013, https://doi.org/10.5194/acp-13-3445-2013, 2013
Related subject area
Subject: Gases | Technique: Remote Sensing | Topic: Data Processing and Information Retrieval
The differences between remote sensing and in situ air pollutant measurements over the Canadian oil sands
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Improved convective cloud differential (CCD) tropospheric ozone from S5P-TROPOMI satellite data using local cloud fields
Atmospheric propane (C3H8) column retrievals from ground-based FTIR observations in Xianghe, China
Can the remote sensing of combustion phase improve estimates of landscape fire smoke emission rate and composition?
Tropospheric NO2 retrieval algorithm for geostationary satellite instruments: applications to GEMS
Troposphere–stratosphere-integrated bromine monoxide (BrO) profile retrieval over the central Pacific Ocean
Local and regional enhancements of CH4, CO, and CO2 inferred from TCCON column measurements
Merging TEMPEST microwave and GOES-16 geostationary IR soundings for improved water vapor profiles
Methane retrieval from MethaneAIR using the CO2 proxy approach: a demonstration for the upcoming MethaneSAT mission
Mapping the CO2 total column retrieval performance from shortwave infrared measurements: synthetic impacts of the spectral resolution, signal-to-noise ratio, and spectral band selection
Assessment of the contribution of the Meteosat Third Generation Infrared Sounder (MTG-IRS) for the characterisation of ozone over Europe
Assessing the potential of free-tropospheric water vapour isotopologue satellite observations for improving the analyses of convective events
Current potential of CH4 emission estimates using TROPOMI in the Middle East
A bias-corrected GEMS geostationary satellite product for nitrogen dioxide using machine learning to enforce consistency with the TROPOMI satellite instrument
Developments on a 22GHz Microwave Radiometer and Reprocessing of 13-Year Time Series for Water Vapour Studies
Retrievals of water vapour and temperature exploiting the far-infrared: application to aircraft observations in preparation for the FORUM mission
Retrieving the atmospheric concentrations of carbon dioxide and methane from the European Copernicus CO2M satellite mission using artificial neural networks
Quantitative estimate of sources of uncertainty in drone-based methane emission measurements
Estimation of biogenic volatile organic compound (BVOC) emissions in forest ecosystems using drone-based lidar, photogrammetry, and image recognition technologies
Fast retrieval of XCO2 over east Asia based on Orbiting Carbon Observatory-2 (OCO-2) spectral measurements
Long-term global measurements of methanol, ethene, ethyne, and HCN from the Cross-track Infrared Sounder
A new method for estimating megacity NOx emissions and lifetimes from satellite observations
Accounting for the effect of aerosols in GHGSat methane retrieval
A survey of methane point source emissions from coal mines in Shanxi province of China using AHSI on board Gaofen-5B
Global retrieval of stratospheric and tropospheric BrO columns from the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) on board the Suomi-NPP satellite
IMK–IAA MIPAS retrieval version 8: CH4 and N2O
Report on Landsat 8 and Sentinel-2B observations of the Nord Stream 2 pipeline methane leak
U-Plume: automated algorithm for plume detection and source quantification by satellite point-source imagers
CH4Net: a deep learning model for monitoring methane super-emitters with Sentinel-2 imagery
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Quantitative imaging of carbon dioxide plumes using a ground-based shortwave infrared spectral camera
The transition to new ozone absorption cross sections for Dobson and Brewer total ozone measurements
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Version 8 IMK/IAA MIPAS measurements of CFC-11, CFC-12, and HCFC-22
The importance of digital elevation model accuracy in XCO2 retrievals: improving the Orbiting Carbon Observatory 2 Atmospheric Carbon Observations from Space version 11 retrieval product
Level0 to Level1B processor for MethaneAIR
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Xiaoyi Zhao, Vitali Fioletov, Debora Griffin, Chris McLinden, Ralf Staebler, Cristian Mihele, Kevin Strawbridge, Jonathan Davies, Ihab Abboud, Sum Chi Lee, Alexander Cede, Martin Tiefengraber, and Robert Swap
Atmos. Meas. Tech., 17, 6889–6912, https://doi.org/10.5194/amt-17-6889-2024, https://doi.org/10.5194/amt-17-6889-2024, 2024
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This study explores differences between remote sensing and in situ instruments in terms of their vertical, horizontal, and temporal sampling differences. Understanding and resolving these differences are critical for future analyses linking satellite, ground-based remote sensing, and in situ observations in air quality monitoring. It shows that the meteorological conditions (wind directions, speed, and boundary layer conditions) will strongly affect the agreement between the two measurements.
Leon Kuhn, Steffen Beirle, Sergey Osipov, Andrea Pozzer, and Thomas Wagner
Atmos. Meas. Tech., 17, 6485–6516, https://doi.org/10.5194/amt-17-6485-2024, https://doi.org/10.5194/amt-17-6485-2024, 2024
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This paper presents a new machine learning model that allows us to compute NO2 concentration profiles from satellite observations. A neural network was trained on synthetic data from the regional chemistry and transport model WRF-Chem. This is the first model of its kind. We present a thorough model validation study, covering various seasons and regions of the world.
Swathi Maratt Satheesan, Kai-Uwe Eichmann, John P. Burrows, Mark Weber, Ryan Stauffer, Anne M. Thompson, and Debra Kollonige
Atmos. Meas. Tech., 17, 6459–6484, https://doi.org/10.5194/amt-17-6459-2024, https://doi.org/10.5194/amt-17-6459-2024, 2024
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CHORA, an advanced cloud convective differential technique, enhances the accuracy of tropospheric-ozone retrievals. Unlike the traditional Pacific cloud reference sector scheme, CHORA introduces a local-cloud reference sector and an alternative approach (CLCT) for precision. Analysing monthly averaged TROPOMI data from 2018 to 2022 and validating with SHADOZ ozonesonde data, CLCT outperforms other methods and so is the preferred choice, especially in future geostationary satellite missions.
Minqiang Zhou, Pucai Wang, Bart Dils, Bavo Langerock, Geoff Toon, Christian Hermans, Weidong Nan, Qun Cheng, and Martine De Mazière
Atmos. Meas. Tech., 17, 6385–6396, https://doi.org/10.5194/amt-17-6385-2024, https://doi.org/10.5194/amt-17-6385-2024, 2024
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Solar absorption spectra near 2967 cm−1 recorded by a ground-based FTIR with a high spectral resolution of 0.0035 cm-1 are applied to retrieve C3H8 columns for the first time in Xianghe, China, within the NDACC-IRWG. The mean and standard deviation of the C3H8 columns are 1.80 ± 0.81 (1σ) × 1015 molec. cm-2. Good correlations are found between C3H8 and other non-methane hydrocarbons, such as C2H6 (R = 0.84) and C2H2 (R = 0.79), as well as between C3H8 and CO (R = 0.72).
Farrer Owsley-Brown, Martin J. Wooster, Mark J. Grosvenor, and Yanan Liu
Atmos. Meas. Tech., 17, 6247–6264, https://doi.org/10.5194/amt-17-6247-2024, https://doi.org/10.5194/amt-17-6247-2024, 2024
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Landscape fires produce vast amounts of smoke, affecting the atmosphere locally and globally. Whether a fire is flaming or smouldering strongly impacts the rate at which smoke is produced as well as its composition. This study tested two methods to determine these combustion phases in laboratory fires and compared them to the smoke emitted. One of these methods improved estimates of smoke emission significantly. This suggests potential for improvement in global emission estimates.
Sora Seo, Pieter Valks, Ronny Lutz, Klaus-Peter Heue, Pascal Hedelt, Víctor Molina García, Diego Loyola, Hanlim Lee, and Jhoon Kim
Atmos. Meas. Tech., 17, 6163–6191, https://doi.org/10.5194/amt-17-6163-2024, https://doi.org/10.5194/amt-17-6163-2024, 2024
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In this study, we developed an advanced retrieval algorithm for tropospheric NO2 columns from geostationary satellite spectrometers and applied it to GEMS measurements. The DLR GEMS NO2 retrieval algorithm follows the heritage from previous and existing algorithms, but improved approaches are applied to reflect the specific features of geostationary satellites. The DLR GEMS NO2 retrievals demonstrate a good capability for monitoring diurnal variability with a high spatial resolution.
Theodore K. Koenig, François Hendrick, Douglas Kinnison, Christopher F. Lee, Michel Van Roozendael, and Rainer Volkamer
Atmos. Meas. Tech., 17, 5911–5934, https://doi.org/10.5194/amt-17-5911-2024, https://doi.org/10.5194/amt-17-5911-2024, 2024
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Atmospheric bromine destroys ozone, impacts oxidation capacity, and oxidizes mercury into its toxic form. We constrain bromine by remote sensing of BrO from a mountaintop. Previous measurements retrieved two to three pieces of information vertically; we apply new methods to get five and a half vertically and two more in time. We compare with aircraft measurements to validate the methods and look at variations in BrO over the Pacific.
Kavitha Mottungan, Chayan Roychoudhury, Vanessa Brocchi, Benjamin Gaubert, Wenfu Tang, Mohammad Amin Mirrezaei, John McKinnon, Yafang Guo, David W. T. Griffith, Dietrich G. Feist, Isamu Morino, Mahesh K. Sha, Manvendra K. Dubey, Martine De Mazière, Nicholas M. Deutscher, Paul O. Wennberg, Ralf Sussmann, Rigel Kivi, Tae-Young Goo, Voltaire A. Velazco, Wei Wang, and Avelino F. Arellano Jr.
Atmos. Meas. Tech., 17, 5861–5885, https://doi.org/10.5194/amt-17-5861-2024, https://doi.org/10.5194/amt-17-5861-2024, 2024
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A combination of data analysis techniques is introduced to separate local and regional influences on observed levels of carbon dioxide, carbon monoxide, and methane from an established ground-based remote sensing network. We take advantage of the covariations in these trace gases to identify the dominant type of sources driving these levels. Applying these methods in conjunction with existing approaches to other datasets can better address uncertainties in identifying sources and sinks.
Chia-Pang Kuo and Christian Kummerow
Atmos. Meas. Tech., 17, 5637–5653, https://doi.org/10.5194/amt-17-5637-2024, https://doi.org/10.5194/amt-17-5637-2024, 2024
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A small satellite about the size of a shoe box, named TEMPEST, carries only a microwave sensor and is designed to measure the water cycle of the Earth from space in an economical way compared with traditional satellites, which have additional infrared sensors. To overcome the limitation, extra infrared signals from GOES-R ABI are combined with TEMPEST microwave measurements. Compared with ground observations, improved humidity information is extracted from the merged TEMPEST and ABI signals.
Christopher Chan Miller, Sébastien Roche, Jonas S. Wilzewski, Xiong Liu, Kelly Chance, Amir H. Souri, Eamon Conway, Bingkun Luo, Jenna Samra, Jacob Hawthorne, Kang Sun, Carly Staebell, Apisada Chulakadabba, Maryann Sargent, Joshua S. Benmergui, Jonathan E. Franklin, Bruce C. Daube, Yang Li, Joshua L. Laughner, Bianca C. Baier, Ritesh Gautam, Mark Omara, and Steven C. Wofsy
Atmos. Meas. Tech., 17, 5429–5454, https://doi.org/10.5194/amt-17-5429-2024, https://doi.org/10.5194/amt-17-5429-2024, 2024
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MethaneSAT is an upcoming satellite mission designed to monitor methane emissions from the oil and gas (O&G) industry globally. Here, we present observations from the first flight campaign of MethaneAIR, a MethaneSAT-like instrument mounted on an aircraft. MethaneAIR can map methane with high precision and accuracy over a typically sized oil and gas basin (~200 km2) in a single flight. This paper demonstrates the capability of the upcoming satellite to routinely track global O&G emissions.
Matthieu Dogniaux and Cyril Crevoisier
Atmos. Meas. Tech., 17, 5373–5396, https://doi.org/10.5194/amt-17-5373-2024, https://doi.org/10.5194/amt-17-5373-2024, 2024
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Many CO2-observing satellite concepts, with very different design choices and trade-offs, are expected to be put into orbit during the upcoming decade. This work uses numerical simulations to explore the impact of critical design parameters on the performance of upcoming CO2-observing satellite concepts.
Francesca Vittorioso, Vincent Guidard, and Nadia Fourrié
Atmos. Meas. Tech., 17, 5279–5299, https://doi.org/10.5194/amt-17-5279-2024, https://doi.org/10.5194/amt-17-5279-2024, 2024
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The future Meteosat Third Generation Infrared Sounder (MTG-IRS) will represent a major innovation for the monitoring of the chemical state of the atmosphere. MTG-IRS will have the advantage of being based on a geostationary platform and acquiring data with a high temporal frequency. This work aims to evaluate its potential impact over Europe within a chemical transport model (MOCAGE). The results indicate that the assimilation of these data always has a positive impact on ozone analysis.
Matthias Schneider, Kinya Toride, Farahnaz Khosrawi, Frank Hase, Benjamin Ertl, Christopher J. Diekmann, and Kei Yoshimura
Atmos. Meas. Tech., 17, 5243–5259, https://doi.org/10.5194/amt-17-5243-2024, https://doi.org/10.5194/amt-17-5243-2024, 2024
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Despite its importance for extreme weather and climate feedbacks, atmospheric convection is not well constrained. This study assesses the potential of novel tropospheric water vapour isotopologue satellite observations for improving the analyses of convective events. We find that the impact of the isotopologues is small for stable atmospheric conditions but significant for unstable conditions, which have the strongest societal impacts (e.g. storms and flooding).
Mengyao Liu, Ronald van der A, Michiel van Weele, Lotte Bryan, Henk Eskes, Pepijn Veefkind, Yongxue Liu, Xiaojuan Lin, Jos de Laat, and Jieying Ding
Atmos. Meas. Tech., 17, 5261–5277, https://doi.org/10.5194/amt-17-5261-2024, https://doi.org/10.5194/amt-17-5261-2024, 2024
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A new divergence method was developed and applied to estimate methane emissions from TROPOMI observations over the Middle East, where it is typically challenging for a satellite to measure methane due to its complicated orography and surface albedo. Our results show the potential of TROPOMI to quantify methane emissions from various sources rather than big emitters from space after objectively excluding the artifacts in the retrieval.
Yujin J. Oak, Daniel J. Jacob, Nicholas Balasus, Laura H. Yang, Heesung Chong, Junsung Park, Hanlim Lee, Gitaek T. Lee, Eunjo S. Ha, Rokjin J. Park, Hyeong-Ahn Kwon, and Jhoon Kim
Atmos. Meas. Tech., 17, 5147–5159, https://doi.org/10.5194/amt-17-5147-2024, https://doi.org/10.5194/amt-17-5147-2024, 2024
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We present an improved NO2 product from GEMS by calibrating it to TROPOMI using machine learning and by reprocessing both satellite products to adopt common NO2 profiles. Our corrected GEMS product combines the high data density of GEMS with the accuracy of TROPOMI, supporting the combined use for analyses of East Asia air quality including emissions and chemistry. This method can be extended to other species and geostationary satellites including TEMPO and Sentinel-4.
Alistair Bell, Eric Sauvageat, Gunter Stober, Klemens Hocke, and Axel Murk
EGUsphere, https://doi.org/10.5194/egusphere-2024-2474, https://doi.org/10.5194/egusphere-2024-2474, 2024
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Hardware and software developments have been made on a 22 GHz microwave radiometer for the measurement of middle atmosphere water vapour near Bern, Switzerland. Previous measurements dating back to 2010 have been re-calibrated and an improved optimal estimation retrieval performed on these measurements, giving a 13 year long dataset. Measurements made with new and improved instrumental hardware are used to correct previous measurements, which show better agreement than the non-corrected dataset.
Sanjeevani Panditharatne, Helen Brindley, Caroline Cox, Richard Siddans, Jonathan Murray, Laura Warwick, and Stuart Fox
EGUsphere, https://doi.org/10.5194/egusphere-2024-2419, https://doi.org/10.5194/egusphere-2024-2419, 2024
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Understanding the distribution of water vapour within our atmosphere is vital for understanding the Earth’s energy balance. Observations from the upcoming FORUM satellite are theorised to be particularly sensitive to this distribution. We exploit this sensitivity to extend the RAL Infrared Microwave Sounding retrieval scheme for the FORUM satellite. This scheme is evaluated on both simulated and observed measurements and shows a good agreement to references of the atmospheric state.
Maximilian Reuter, Michael Hilker, Stefan Noël, Antonio Di Noia, Michael Weimer, Oliver Schneising, Michael Buchwitz, Heinrich Bovensmann, John P. Burrows, Hartmut Bösch, and Ruediger Lang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2365, https://doi.org/10.5194/egusphere-2024-2365, 2024
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Carbon dioxide (CO2) and methane (CH4) are the main anthropogenic greenhouse gases. The European Copernicus CO2 monitoring satellite mission CO2M will provide measurements of their atmospheric concentrations, but the accuracy requirements are demanding and conventional retrieval methods computationally expensive. We present a new retrieval algorithm based on artificial neural networks that has the potential to meet the stringent requirements of the CO2M mission with minimal computational effort.
Tannaz H. Mohammadloo, Matthew Jones, Bas van de Kerkhof, Kyle Dawson, Brendan James Smith, Stephen Conley, Abigail Corbett, and Rutger IJzermans
EGUsphere, https://doi.org/10.5194/egusphere-2024-1175, https://doi.org/10.5194/egusphere-2024-1175, 2024
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Methane is a potent greenhouse gas. Trustable detection and quantification of methane emissions at facility level is critical to identify the largest sources, and to prioritize them for repair. We provide a systematic analysis of the uncertainty in drone-based methane emission surveys, based on theoretical considerations and historical data sets. We provide guidelines to industry on how to avoid or minimize potential errors in drone-based measurements for methane emission quantification.
Xianzhong Duan, Ming Chang, Guotong Wu, Suping Situ, Shengjie Zhu, Qi Zhang, Yibo Huangfu, Weiwen Wang, Weihua Chen, Bin Yuan, and Xuemei Wang
Atmos. Meas. Tech., 17, 4065–4079, https://doi.org/10.5194/amt-17-4065-2024, https://doi.org/10.5194/amt-17-4065-2024, 2024
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Accurately estimating biogenic volatile organic compound (BVOC) emissions in forest ecosystems has been challenging. This research presents a framework that utilizes drone-based lidar, photogrammetry, and image recognition technologies to identify plant species and estimate BVOC emissions. The largest cumulative isoprene emissions were found in the Myrtaceae family, while those of monoterpenes were from the Rubiaceae family.
Fengxin Xie, Tao Ren, Changying Zhao, Yuan Wen, Yilei Gu, Minqiang Zhou, Pucai Wang, Kei Shiomi, and Isamu Morino
Atmos. Meas. Tech., 17, 3949–3967, https://doi.org/10.5194/amt-17-3949-2024, https://doi.org/10.5194/amt-17-3949-2024, 2024
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This study demonstrates a new machine learning approach to efficiently and accurately estimate atmospheric carbon dioxide levels from satellite data. Rather than using traditional complex physics-based retrieval methods, neural network models are trained on simulated data to rapidly predict CO2 concentrations directly from satellite spectral measurements.
Kelley Wells, Dylan Millet, Jared Brewer, Vivienne Payne, Karen Cady-Pereira, Rick Pernak, Susan Kulawik, Corinne Vigouroux, Nicholas Jones, Emmanuel Mahieu, Maria Makarova, Tomoo Nagahama, Ivan Ortega, Mathias Palm, Kimberly Strong, Matthias Schneider, Dan Smale, Ralf Sussmann, and Minqiang Zhou
EGUsphere, https://doi.org/10.5194/egusphere-2024-1551, https://doi.org/10.5194/egusphere-2024-1551, 2024
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Atmospheric volatile organic compounds affect both air quality and climate. Satellite measurements can help us to assess and predict their global impacts. We present new long-term (2012–2023) measurements of four key VOCs: methanol, ethene, ethyne, and hydrogen cyanide (HCN) from the Cross-track Infrared Sounder. The measurements reflect emissions from major forests, wildfires, and industry, and provide new information to advance understanding of these sources and their changes over time.
Steffen Beirle and Thomas Wagner
Atmos. Meas. Tech., 17, 3439–3453, https://doi.org/10.5194/amt-17-3439-2024, https://doi.org/10.5194/amt-17-3439-2024, 2024
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We present a new method for estimating emissions and lifetimes for nitrogen oxides emitted from large cities by using satellite NO2 observations combined with wind fields. The estimate is based on the simultaneous evaluation of the downwind plumes for opposing wind directions. This allows us to derive seasonal mean emissions and lifetimes for 100 cities around the globe.
Qiurun Yu, Dylan Jervis, and Yi Huang
Atmos. Meas. Tech., 17, 3347–3366, https://doi.org/10.5194/amt-17-3347-2024, https://doi.org/10.5194/amt-17-3347-2024, 2024
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This study estimated the effects of aerosols on GHGSat satellite methane retrieval and investigated the performance of simultaneously retrieving aerosol and methane information using a multi-angle viewing method. Results suggested that the performance of GHGSat methane retrieval improved when aerosols were considered, and the multi-angle viewing method is insensitive to the satellite angle setting. This performance assessment is useful for improving future GHGSat-like instruments.
Zhonghua He, Ling Gao, Miao Liang, and Zhao-Cheng Zeng
Atmos. Meas. Tech., 17, 2937–2956, https://doi.org/10.5194/amt-17-2937-2024, https://doi.org/10.5194/amt-17-2937-2024, 2024
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Using Gaofen-5B satellite data, this study detected 93 methane plume events from 32 coal mines in Shanxi, China, with emission rates spanning from 761.78 ± 185.00 to 12729.12 ± 4658.13 kg h-1, showing significant variability among sources. This study highlights Gaofen-5B’s capacity for monitoring large methane point sources, offering valuable support in reducing greenhouse gas emissions.
Heesung Chong, Gonzalo González Abad, Caroline R. Nowlan, Christopher Chan Miller, Alfonso Saiz-Lopez, Rafael P. Fernandez, Hyeong-Ahn Kwon, Zolal Ayazpour, Huiqun Wang, Amir H. Souri, Xiong Liu, Kelly Chance, Ewan O'Sullivan, Jhoon Kim, Ja-Ho Koo, William R. Simpson, François Hendrick, Richard Querel, Glen Jaross, Colin Seftor, and Raid M. Suleiman
Atmos. Meas. Tech., 17, 2873–2916, https://doi.org/10.5194/amt-17-2873-2024, https://doi.org/10.5194/amt-17-2873-2024, 2024
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We present a new bromine monoxide (BrO) product derived using radiances measured from OMPS-NM on board the Suomi-NPP satellite. This product provides nearly a decade of global stratospheric and tropospheric column retrievals, a feature that is currently rare in publicly accessible datasets. Both stratospheric and tropospheric columns from OMPS-NM demonstrate robust performance, exhibiting good agreement with ground-based observations collected at three stations (Lauder, Utqiagvik, and Harestua).
Norbert Glatthor, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 17, 2849–2871, https://doi.org/10.5194/amt-17-2849-2024, https://doi.org/10.5194/amt-17-2849-2024, 2024
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We present global atmospheric methane (CH4) and nitrous oxide (N2O) distributions retrieved from measurements of the MIPAS instrument on board the Environmental Satellite (Envisat) during 2002 to 2012. Monitoring of these gases is of scientific interest because both of them are strong greenhouse gases. We analyze the latest, improved version of calibrated MIPAS measurements. Further, we apply a new retrieval scheme leading to an improved CH4 and N2O data product .
Matthieu Dogniaux, Joannes D. Maasakkers, Daniel J. Varon, and Ilse Aben
Atmos. Meas. Tech., 17, 2777–2787, https://doi.org/10.5194/amt-17-2777-2024, https://doi.org/10.5194/amt-17-2777-2024, 2024
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We analyze Landsat 8 (L8) and Sentinel-2B (S-2B) observations of the 2022 Nord Stream 2 methane leak and show how challenging this case is for usual data analysis methods. We provide customized calibrations for this Nord Stream 2 case and assess that no firm conclusion can be drawn from L8 or S-2B single overpasses. However, if we opportunistically assume that L8 and S-2B results are independent, we find an averaged L8 and S-2B combined methane leak rate of 502 ± 464 t h−1.
Jack H. Bruno, Dylan Jervis, Daniel J. Varon, and Daniel J. Jacob
Atmos. Meas. Tech., 17, 2625–2636, https://doi.org/10.5194/amt-17-2625-2024, https://doi.org/10.5194/amt-17-2625-2024, 2024
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Methane is a potent greenhouse gas and a current high-priority target for short- to mid-term climate change mitigation. Detection of individual methane emitters from space has become possible in recent years, and the volume of data for this task has been rapidly growing, outpacing processing capabilities. We introduce an automated approach, U-Plume, which can detect and quantify emissions from individual methane sources in high-spatial-resolution satellite data.
Anna Vaughan, Gonzalo Mateo-García, Luis Gómez-Chova, Vít Růžička, Luis Guanter, and Itziar Irakulis-Loitxate
Atmos. Meas. Tech., 17, 2583–2593, https://doi.org/10.5194/amt-17-2583-2024, https://doi.org/10.5194/amt-17-2583-2024, 2024
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Methane is a potent greenhouse gas that has been responsible for around 25 % of global warming since the industrial revolution. Consequently identifying and mitigating methane emissions comprise an important step in combating the climate crisis. We develop a new deep learning model to automatically detect methane plumes from satellite images and demonstrate that this can be applied to monitor large methane emissions resulting from the oil and gas industry.
Otto M. Lamminpää, Jouni I. Susiluoto, Jonathan M. Hobbs, James L. McDuffie, Amy J. Braverman, and Houman Owhadi
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-63, https://doi.org/10.5194/amt-2024-63, 2024
Revised manuscript accepted for AMT
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We develop and demonstrate a fast forward function emulator for remote sensing of greenhouse gases. These forward functions are computationally expensive to evaluate, and as such the key challenge for many satellite missions in their data processing is the time used in these evaluations. Our method is fast and accurate enough, less than 1 % relative error, so that it could be safely used in operational processing.
Stefan Noël, Michael Buchwitz, Michael Hilker, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, Hartmut Bösch, and Ruediger Lang
Atmos. Meas. Tech., 17, 2317–2334, https://doi.org/10.5194/amt-17-2317-2024, https://doi.org/10.5194/amt-17-2317-2024, 2024
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FOCAL-CO2M is one of the three operational retrieval algorithms which will be used to derive XCO2 and XCH4 from measurements of the forthcoming European CO2M mission. We present results of applications of FOCAL-CO2M to simulated spectra, from which confidence is gained that the algorithm is able to fulfil the challenging requirements on systematic errors for the CO2M mission (spatio-temporal bias ≤ 0.5 ppm for XCO2 and ≤ 5 ppb for XCH4).
Marvin Knapp, Ralph Kleinschek, Sanam N. Vardag, Felix Külheim, Helge Haveresch, Moritz Sindram, Tim Siegel, Bruno Burger, and André Butz
Atmos. Meas. Tech., 17, 2257–2275, https://doi.org/10.5194/amt-17-2257-2024, https://doi.org/10.5194/amt-17-2257-2024, 2024
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Imaging carbon dioxide (CO2) plumes of anthropogenic sources from planes and satellites has proven valuable for detecting emitters and monitoring climate mitigation efforts. We present the first images of CO2 plumes taken with a ground-based spectral camera, observing a coal-fired power plant as a validation target. We develop a technique to find the source emission strength with an hourly resolution, which reasonably agrees with the expected emissions under favorable conditions.
Karl Voglmeier, Voltaire A. Velazco, Luca Egli, Julian Gröbner, Alberto Redondas, and Wolfgang Steinbrecht
Atmos. Meas. Tech., 17, 2277–2294, https://doi.org/10.5194/amt-17-2277-2024, https://doi.org/10.5194/amt-17-2277-2024, 2024
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Comparison between total ozone column (TOC) measurements from ground-based Dobson and Brewer spectrophotometers generally reveals seasonally varying differences of a few percent. This study recommends a new TOC retrieval approach, which effectively eliminates these seasonally varying differences by applying new ozone absorption cross sections, appropriate slit functions for the Dobson instrument, and climatological values for the effective ozone temperature.
Wenfu Tang, Benjamin Gaubert, Louisa Emmons, Daniel Ziskin, Debbie Mao, David Edwards, Avelino Arellano, Kevin Raeder, Jeffrey Anderson, and Helen Worden
Atmos. Meas. Tech., 17, 1941–1963, https://doi.org/10.5194/amt-17-1941-2024, https://doi.org/10.5194/amt-17-1941-2024, 2024
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We assimilate different MOPITT CO products to understand the impact of (1) assimilating multispectral and joint retrievals versus single spectral products, (2) assimilating satellite profile products versus column products, and (3) assimilating multispectral and joint retrievals versus assimilating individual products separately.
Juseon Bak, Xiong Liu, Kai Yang, Gonzalo Gonzalez Abad, Ewan O'Sullivan, Kelly Chance, and Cheol-Hee Kim
Atmos. Meas. Tech., 17, 1891–1911, https://doi.org/10.5194/amt-17-1891-2024, https://doi.org/10.5194/amt-17-1891-2024, 2024
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The new version (V2) of the OMI ozone profile product is introduced to improve retrieval quality and long-term consistency of tropospheric ozone by incorporating the recent collection 4 OMI L1b spectral products and refining radiometric correction, forward model calculation, and a priori ozone data.
Andrea Orfanoz-Cheuquelaf, Carlo Arosio, Alexei Rozanov, Mark Weber, Annette Ladstätter-Weißenmayer, John P. Burrows, Anne M. Thompson, Ryan M. Stauffer, and Debra E. Kollonige
Atmos. Meas. Tech., 17, 1791–1809, https://doi.org/10.5194/amt-17-1791-2024, https://doi.org/10.5194/amt-17-1791-2024, 2024
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Valuable information on the tropospheric ozone column (TrOC) can be obtained globally by combining space-borne limb and nadir measurements (limb–nadir matching, LNM). This study describes the retrieval of TrOC from the OMPS instrument (since 2012) using the LNM technique. The OMPS-LNM TrOC was compared with ozonesondes and other satellite measurements, showing a good agreement with a negative bias within 1 to 4 DU. This new dataset is suitable for pollution studies.
Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Bernd Funke, Maya García-Comas, and Manuel López-Puertas
Atmos. Meas. Tech., 17, 1759–1789, https://doi.org/10.5194/amt-17-1759-2024, https://doi.org/10.5194/amt-17-1759-2024, 2024
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CFC-11, CFC-12, and HCFC-22 contribute to the depletion of ozone and are potent greenhouse gases. They have been banned by the Montreal protocol. With MIPAS on Envisat the atmospheric composition could be observed between 2002 and 2012. We present here the retrieval of their atmospheric distributions for the final data version 8. We characterise the derived data by their error budget and their spatial resolution. An additional representation for direct comparison to models is also provided.
Nicole Jacobs, Christopher W. O'Dell, Thomas E. Taylor, Thomas L. Logan, Brendan Byrne, Matthäus Kiel, Rigel Kivi, Pauli Heikkinen, Aronne Merrelli, Vivienne H. Payne, and Abhishek Chatterjee
Atmos. Meas. Tech., 17, 1375–1401, https://doi.org/10.5194/amt-17-1375-2024, https://doi.org/10.5194/amt-17-1375-2024, 2024
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The accuracy of trace gas retrievals from spaceborne observations, like those from the Orbiting Carbon Observatory 2 (OCO-2), are sensitive to the referenced digital elevation model (DEM). Therefore, we evaluate several global DEMs, used in versions 10 and 11 of the OCO-2 retrieval along with the Copernicus DEM. We explore the impacts of changing the DEM on biases in OCO-2-retrieved XCO2 and inferred CO2 fluxes. Our findings led to an update to OCO-2 v11.1 using the Copernicus DEM globally.
Eamon K. Conway, Amir H. Souri, Joshua Benmergui, Kang Sun, Xiong Liu, Carly Staebell, Christopher Chan Miller, Jonathan Franklin, Jenna Samra, Jonas Wilzewski, Sebastien Roche, Bingkun Luo, Apisada Chulakadabba, Maryann Sargent, Jacob Hohl, Bruce Daube, Iouli Gordon, Kelly Chance, and Steven Wofsy
Atmos. Meas. Tech., 17, 1347–1362, https://doi.org/10.5194/amt-17-1347-2024, https://doi.org/10.5194/amt-17-1347-2024, 2024
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The work presented here describes the processes required to convert raw sensor data for the MethaneAIR instrument to geometrically calibrated data. Each algorithm is described in detail. MethaneAIR is the airborne simulator for MethaneSAT, a new satellite under development by MethaneSAT LLC, a subsidiary of the EDF. MethaneSAT's goals are to precisely map over 80 % of the production sources of methane emissions from oil and gas fields across the globe to a high degree of accuracy.
Javier Roger, Luis Guanter, Javier Gorroño, and Itziar Irakulis-Loitxate
Atmos. Meas. Tech., 17, 1333–1346, https://doi.org/10.5194/amt-17-1333-2024, https://doi.org/10.5194/amt-17-1333-2024, 2024
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Methane emissions can be identified using remote sensing, but surface-related structures disturb detection. In this work, a variation of the matched filter method that exploits a large fraction of the near-infrared range (1000–2500 nm) is applied. In comparison to the raw matched filter, it reduces background noise and strongly attenuates the surface-related artifacts, which leads to a greater detection capability. We propose this variation as a standard methodology for methane detection.
Blanca Fuentes Andrade, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Andreas Richter, Hartmut Boesch, and John P. Burrows
Atmos. Meas. Tech., 17, 1145–1173, https://doi.org/10.5194/amt-17-1145-2024, https://doi.org/10.5194/amt-17-1145-2024, 2024
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We developed a method to estimate CO2 emissions from localized sources, such as power plants, using satellite data and applied it to estimate CO2 emissions from the Bełchatów Power Station (Poland). As the detection of CO2 emission plumes from satellite data is difficult, we used observations of co-emitted NO2 to constrain the emission plume region. Our results agree with CO2 emission estimations based on the power-plant-generated power and emission factors.
Gregory R. McGarragh, Christopher W. O'Dell, Sean M. R. Crowell, Peter Somkuti, Eric B. Burgh, and Berrien Moore III
Atmos. Meas. Tech., 17, 1091–1121, https://doi.org/10.5194/amt-17-1091-2024, https://doi.org/10.5194/amt-17-1091-2024, 2024
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Carbon dioxide and methane are greenhouse gases that have been rapidly increasing due to human activity since the industrial revolution, leading to global warming and subsequently negative affects on the climate. It is important to measure the concentrations of these gases in order to make climate predictions that drive policy changes to mitigate climate change. GeoCarb aims to measure the concentrations of these gases from space over the Americas at unprecedented spatial and temporal scales.
Jianping Mao, James B. Abshire, S. Randy Kawa, Xiaoli Sun, and Haris Riris
Atmos. Meas. Tech., 17, 1061–1074, https://doi.org/10.5194/amt-17-1061-2024, https://doi.org/10.5194/amt-17-1061-2024, 2024
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NASA Goddard Space Flight Center has developed an integrated-path, differential absorption lidar approach to measure column-averaged atmospheric CO2 (XCO2). We demonstrated the lidar’s capability to measure XCO2 to cloud tops ,as well as to the ground, with the data from the summer 2017 airborne campaign in the US and Canada. This active remote sensing technique can provide all-sky data coverage and high-quality XCO2 measurements for future airborne science campaigns and space missions.
Jong-Uk Park, Hyun-Jae Kim, Jin-Soo Park, Jinsoo Choi, Sang Seo Park, Kangho Bae, Jong-Jae Lee, Chang-Keun Song, Soojin Park, Kyuseok Shim, Yeonsoo Cho, and Sang-Woo Kim
Atmos. Meas. Tech., 17, 197–217, https://doi.org/10.5194/amt-17-197-2024, https://doi.org/10.5194/amt-17-197-2024, 2024
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The high-spatial-resolution NO2 vertical column densities (VCDs) were measured from airborne observations using the low-cost hyperspectral imaging sensor (HIS) at three industrial areas in South Korea with the newly developed versatile NO2 VCD retrieval algorithm apt to be applied to the instruments with volatile optical and radiometric properties. The airborne HIS observations emphasized the intensifying satellite sub-grid variability in NO2 VCDs near the emission sources.
Yiguo Pang, Longfei Tian, Denghui Hu, Shuang Gao, and Guohua Liu
EGUsphere, https://doi.org/10.5194/egusphere-2023-1693, https://doi.org/10.5194/egusphere-2023-1693, 2023
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The spatial adjacency of methane point sources can result in plume overlapping, presenting challenges for the quantification from space. A modern parameter estimation technique is introduced to separate the overlapping plumes from satellite observations. This separation method allows traditional quantification methods to be applied beyond scenarios with a single source. A new optimization metric is also proposed for better separation of relatively weaker sources.
William R. Keely, Steffen Mauceri, Sean Crowell, and Christopher W. O'Dell
Atmos. Meas. Tech., 16, 5725–5748, https://doi.org/10.5194/amt-16-5725-2023, https://doi.org/10.5194/amt-16-5725-2023, 2023
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Measurement errors in satellite observations of CO2 attributed to co-estimated atmospheric variables are corrected using a linear regression on quality-filtered data. We propose a nonlinear method that improves correction against a set of ground truth proxies and allows for high throughput of well-corrected data.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 5609–5645, https://doi.org/10.5194/amt-16-5609-2023, https://doi.org/10.5194/amt-16-5609-2023, 2023
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This paper describes a new version (V8) of ozone data from MIPAS middle-atmosphere spectra. The dataset comprises high-quality ozone profiles from 20 to 100 km, with pole-to-pole latitude coverage for the day- and nighttime, spanning 2005 until 2012. An exhaustive treatment of errors has been performed. Compared to other satellite instruments, MIPAS ozone shows a positive bias of 5 %–8 % below 70 km. In the upper mesosphere, this new version agrees much better than previous ones (within 10 %).
Minqiang Zhou, Bavo Langerock, Mahesh Kumar Sha, Christian Hermans, Nicolas Kumps, Rigel Kivi, Pauli Heikkinen, Christof Petri, Justus Notholt, Huilin Chen, and Martine De Mazière
Atmos. Meas. Tech., 16, 5593–5608, https://doi.org/10.5194/amt-16-5593-2023, https://doi.org/10.5194/amt-16-5593-2023, 2023
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Atmospheric N2O and CH4 columns are successfully retrieved from low-resolution FTIR spectra recorded by a Bruker VERTEX 70. The 1-year measurements at Sodankylä show that the N2O total columns retrieved from 125HR and VERTEX 70 spectra are −0.3 ± 0.7 % with an R value of 0.93. The relative differences between the CH4 total columns retrieved from the 125HR and VERTEX spectra are 0.0 ± 0.8 % with an R value of 0.87. Such a technique can help to fill the gap in NDACC N2O and CH4 measurements.
Simon Warnach, Holger Sihler, Christian Borger, Nicole Bobrowski, Steffen Beirle, Ulrich Platt, and Thomas Wagner
Atmos. Meas. Tech., 16, 5537–5573, https://doi.org/10.5194/amt-16-5537-2023, https://doi.org/10.5194/amt-16-5537-2023, 2023
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BrO inside volcanic gas plumes but can be used in combination with SO2 to characterize the volcanic property and its activity state. High-quality satellite observations can provide a global inventory of this important quantity. This paper investigates how to accurately detect BrO inside volcanic plumes from the satellite UV spectrum. A sophisticated novel non-volcanic background correction scheme is presented, and systematic errors including cross-interference with formaldehyde are minimized.
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Short summary
As a greenhouse gas with strong global warming potential, atmospheric methane emissions have attracted a great deal of attention. However, accurate assessment of these emissions is challenging in the presence of atmospheric particulates called aerosols. We quantify the aerosol impact on methane quantification from airborne measurements using two techniques, one that has traditionally been used by the imaging spectroscopy community and the other commonly employed in trace gas remote sensing.
As a greenhouse gas with strong global warming potential, atmospheric methane emissions have...