Articles | Volume 13, issue 8
https://doi.org/10.5194/amt-13-4461-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-13-4461-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Aerosol optical properties as observed from an ultralight aircraft over the Strait of Gibraltar
Patrick Chazette
CORRESPONDING AUTHOR
Laboratoire des Sciences du Climat et de l'Environnement (LSCE),
Laboratoire mixte CEA-CNRS-UVSQ, UMR 1572, CEA Saclay, 91191 Gif-sur-Yvette, France
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Between October 2022 and January 2023, the Water Vapour Lidar Network Assimilation (WaLiNeAs) campaign was conducted on the western Mediterranean by four European countries. To improve the forecasting of heavy precipitation events, eight ground-based stations equipped with water vapour Raman lidars were strategically deployed. They offered a valuable chance to verify the consistency of the water vapour products of both the Infrared Atmospheric Sounding Interferometer (IASI) and ERA5 reanalysis.
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Smoke from Southern African and South American wildfires can travel for thousands of kilometers before reaching the Indian Ocean and Reunion Island. In this study, we use instruments measuring from the ground, from satellites, as well as atmospheric models, to track these smoke plumes and identify their origins and properties. Our findings should help future research focusing on the impact of these plumes on the atmospheric temperature.
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This article presents the evolution of aerosol optical properties as derived from a Raman lidar in relation to relative humidity over the Paris area. It examines the influence of aerosol chemical compounds linked to air mass origins, as well as their relationship with the efficiency of aerosol growth. Such a study provides a better understanding of the interactions between aerosols and water vapour, which is important for reducing the uncertainties surrounding the Earth's radiative balance.
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Space photographs of the Earth show that clouds form diverse, common but poorly understood cloud patterns. The analysis of observations gathered from research aircraft over the tropical ocean shows that the merging of thermals and clouds in the first kilometer of the atmosphere plays a key role in controlling the size, depth and spacing of clouds. This reveals a fundamental process through which clouds interact with each other and with their environment.
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High-resolution airborne observations reveal that mixing between the free troposphere and surface evapotranspiration flux primarily modulates the water vapor isotopic composition in the lower troposphere. Water vapor isotope structure variations occur on the scale of hundreds of meters, underlining the utility of stable isotopes for studying microscale atmospheric dynamics. This study also provides the basis for better validation of water vapor isotope remote sensing retrievals with surface observations.
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The use of active remote sensing instruments to sample the atmospheric environment requires accurate calibration that is stable over time so that measurements are reproducible. This is the case for measurements of atmospheric water vapour using Raman lidar, which are of growing interest in the context of climate risks such as extreme precipitation. This study addresses this issue. It is based on six campaigns spread over a period of 7 years between 2016 and 2022.
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Earth Syst. Sci. Data, 16, 5579–5602, https://doi.org/10.5194/essd-16-5579-2024, https://doi.org/10.5194/essd-16-5579-2024, 2024
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We present a dataset of water vapor mixing ratio profiles acquired during the Water Vapor Lidar Network Assimilation campaign in fall and winter 2022 and summer 2023, using three lidar systems deployed on the western Mediterranean coastline. This innovative campaign provides access to lower-tropospheric water vapor variability to constrain meteorological forecasting models. The scientific objective is to improve forecasting of heavy-precipation events that lead to flash floods and landslides.
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The French ATR42 research aircraft participated in the EUREC4A international field campaign that took place in 2020 over the tropical Atlantic, east of Barbados. We present the extensive instrumentation of the aircraft, the research flights and the different measurements. We show that the ATR measurements of humidity, wind, aerosols and cloudiness in the lower atmosphere are robust and consistent with each other. They will make it possible to advance understanding of cloud–climate interactions.
Karine Desboeufs, Franck Fu, Matthieu Bressac, Antonio Tovar-Sánchez, Sylvain Triquet, Jean-François Doussin, Chiara Giorio, Patrick Chazette, Julie Disnaquet, Anaïs Feron, Paola Formenti, Franck Maisonneuve, Araceli Rodríguez-Romero, Pascal Zapf, François Dulac, and Cécile Guieu
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Short summary
Short summary
This article reports the first concurrent sampling of wet deposition samples and surface seawater and was performed during the PEACETIME cruise in the remote Mediterranean (May–June 2017). Through the chemical composition of trace metals (TMs) in these samples, it emphasizes the decrease of atmospheric metal pollution in this area during the last few decades and the critical role of wet deposition as source of TMs for Mediterranean surface seawater, especially for intense dust deposition events.
Patrick Chazette, Alexandre Baron, and Cyrille Flamant
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Short summary
Short summary
Within the framework of the international EUREC4A project, horizontal lidar measurements were carried out over Barbados from the French research aircraft ATR-42. These measurements highlighted the strong heterogeneity of the aerosol field (mainly dust and biomass burning aerosols) and therefore of the associated optical properties. This heterogeneity varies according to meteorological conditions and could significantly modulate the climatic impact of aerosols trapped over the tropical Atlantic.
Julien Totems, Patrick Chazette, and Alexandre Baron
Atmos. Meas. Tech., 14, 7525–7544, https://doi.org/10.5194/amt-14-7525-2021, https://doi.org/10.5194/amt-14-7525-2021, 2021
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We describe in detail the design and calibration of the new Raman channels for the WALI system, going over the important sources of bias and uncertainty on retrieved temperature profiles. For the first time, their impact is investigated using horizontal shots in a homogenous atmosphere: the magnitude of the highlighted biases can be much larger than the targeted absolute accuracy of 1° C. Actual measurement errors are quantified using radiosoundings launched close to the lidar site.
Jonas Hamperl, Clément Capitaine, Jean-Baptiste Dherbecourt, Myriam Raybaut, Patrick Chazette, Julien Totems, Bruno Grouiez, Laurence Régalia, Rosa Santagata, Corinne Evesque, Jean-Michel Melkonian, Antoine Godard, Andrew Seidl, Harald Sodemann, and Cyrille Flamant
Atmos. Meas. Tech., 14, 6675–6693, https://doi.org/10.5194/amt-14-6675-2021, https://doi.org/10.5194/amt-14-6675-2021, 2021
Short summary
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Laser active remote sensing of tropospheric water vapor is a promising technology for enhancing our understanding of processes governing the global hydrological cycle. We investigate the potential of a ground-based lidar to monitor the main water vapor isotopes at high spatio-temporal resolutions in the lower troposphere. Using a realistic end-to-end simulator, we show that high-precision measurements can be achieved within a range of 1.5 km, in mid-latitude or tropical environments.
Patrick Chazette, Andreas Behrendt, Adolfo Comerón, Paolo Di Girolamo, Marco Di Paolantonio, Davide Dionisi, Cyrille Flamant, José Luis Gómez-Amo, Jérémy Lagarrigue, Frédéric Laly, Diego Lange, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Michaël Sicard, Donato Summa, Julien Totems, María Pilar Utrillas, Pedro C. Valdelomar, and Volker Wulfmeyer
Atmos. Meas. Tech., 19, 5223–5242, https://doi.org/10.5194/amt-19-5223-2026, https://doi.org/10.5194/amt-19-5223-2026, 2026
Short summary
Short summary
Between October 2022 and January 2023, the Water Vapour Lidar Network Assimilation (WaLiNeAs) campaign was conducted on the western Mediterranean by four European countries. To improve the forecasting of heavy precipitation events, eight ground-based stations equipped with water vapour Raman lidars were strategically deployed. They offered a valuable chance to verify the consistency of the water vapour products of both the Infrared Atmospheric Sounding Interferometer (IASI) and ERA5 reanalysis.
Dominique Gantois, Alexandre Baron, Michaël Sicard, Valentin Duflot, Niels Groenen, Nelson Bègue, Sabine Eckhardt, Nikolaos Evangeliou, Martine De Mazière, Corinne Vigouroux, Guillaume Payen, Nicolas Marquestaut, Jean-Marc Metzger, Patrick Chazette, and Cyrille Flamant
EGUsphere, https://doi.org/10.5194/egusphere-2026-3070, https://doi.org/10.5194/egusphere-2026-3070, 2026
Short summary
Short summary
Smoke from Southern African and South American wildfires can travel for thousands of kilometers before reaching the Indian Ocean and Reunion Island. In this study, we use instruments measuring from the ground, from satellites, as well as atmospheric models, to track these smoke plumes and identify their origins and properties. Our findings should help future research focusing on the impact of these plumes on the atmospheric temperature.
Patrick Chazette
Atmos. Meas. Tech., 19, 4293–4311, https://doi.org/10.5194/amt-19-4293-2026, https://doi.org/10.5194/amt-19-4293-2026, 2026
Short summary
Short summary
A novel aerosol classification methodology based on Raman lidar observations is presented and applied to measurements acquired during the FENNEC field campaign. The temporal evolution of aerosol classes and optical properties is then used to perform a quantitative evaluation of numerical simulations from the Copernicus Atmosphere Monitoring Service (CAMS) global reanalysis (EAC4).
Frédéric Laly, Patrick Chazette, Julien Totems, Vincent Crenn, David Ledur, and Alexandre Marpillat
Atmos. Meas. Tech., 18, 7629–7649, https://doi.org/10.5194/amt-18-7629-2025, https://doi.org/10.5194/amt-18-7629-2025, 2025
Short summary
Short summary
This article presents the evolution of aerosol optical properties as derived from a Raman lidar in relation to relative humidity over the Paris area. It examines the influence of aerosol chemical compounds linked to air mass origins, as well as their relationship with the efficiency of aerosol growth. Such a study provides a better understanding of the interactions between aerosols and water vapour, which is important for reducing the uncertainties surrounding the Earth's radiative balance.
Sandrine Bony, Basile Poujol, Brett McKim, Nicolas Rochetin, Marie Lothon, Julia Windmiller, Nicolas Maury, Clarisse Dufaux, Louis Jaffeux, Patrick Chazette, and Julien Delanoë
Atmos. Chem. Phys., 25, 17331–17362, https://doi.org/10.5194/acp-25-17331-2025, https://doi.org/10.5194/acp-25-17331-2025, 2025
Short summary
Short summary
Space photographs of the Earth show that clouds form diverse, common but poorly understood cloud patterns. The analysis of observations gathered from research aircraft over the tropical ocean shows that the merging of thermals and clouds in the first kilometer of the atmosphere plays a key role in controlling the size, depth and spacing of clouds. This reveals a fundamental process through which clouds interact with each other and with their environment.
Daniele Zannoni, Hans Christian Steen-Larsen, Harald Sodemann, Iris Thurnherr, Cyrille Flamant, Patrick Chazette, Julien Totems, Martin Werner, and Myriam Raybaut
Atmos. Chem. Phys., 25, 9471–9495, https://doi.org/10.5194/acp-25-9471-2025, https://doi.org/10.5194/acp-25-9471-2025, 2025
Short summary
Short summary
High-resolution airborne observations reveal that mixing between the free troposphere and surface evapotranspiration flux primarily modulates the water vapor isotopic composition in the lower troposphere. Water vapor isotope structure variations occur on the scale of hundreds of meters, underlining the utility of stable isotopes for studying microscale atmospheric dynamics. This study also provides the basis for better validation of water vapor isotope remote sensing retrievals with surface observations.
Patrick Chazette, Julien Totems, and Frédéric Laly
Atmos. Meas. Tech., 18, 2681–2699, https://doi.org/10.5194/amt-18-2681-2025, https://doi.org/10.5194/amt-18-2681-2025, 2025
Short summary
Short summary
The use of active remote sensing instruments to sample the atmospheric environment requires accurate calibration that is stable over time so that measurements are reproducible. This is the case for measurements of atmospheric water vapour using Raman lidar, which are of growing interest in the context of climate risks such as extreme precipitation. This study addresses this issue. It is based on six campaigns spread over a period of 7 years between 2016 and 2022.
Frédéric Laly, Patrick Chazette, Julien Totems, Jérémy Lagarrigue, Laurent Forges, and Cyrille Flamant
Earth Syst. Sci. Data, 16, 5579–5602, https://doi.org/10.5194/essd-16-5579-2024, https://doi.org/10.5194/essd-16-5579-2024, 2024
Short summary
Short summary
We present a dataset of water vapor mixing ratio profiles acquired during the Water Vapor Lidar Network Assimilation campaign in fall and winter 2022 and summer 2023, using three lidar systems deployed on the western Mediterranean coastline. This innovative campaign provides access to lower-tropospheric water vapor variability to constrain meteorological forecasting models. The scientific objective is to improve forecasting of heavy-precipation events that lead to flash floods and landslides.
Maëlie Chazette, Patrick Chazette, Ilja M. Reiter, Xiaoxia Shang, Julien Totems, Jean-Philippe Orts, Irène Xueref-Remy, and Nicolas Montes
Biogeosciences, 21, 3289–3303, https://doi.org/10.5194/bg-21-3289-2024, https://doi.org/10.5194/bg-21-3289-2024, 2024
Short summary
Short summary
The approach presented is original in its coupling between field observations and airborne lidar observations. It has been applied to an instrumented reference forest site in the south of France, which is heavily impacted by climate change. It leads to the evaluation of tree heights and ends with assessments of aerial and root carbon stocks. A detailed assessment of uncertainties is presented to add a level of reliability to the scientific products delivered.
Patrick Chazette and Jean-Christophe Raut
Atmos. Meas. Tech., 16, 5847–5861, https://doi.org/10.5194/amt-16-5847-2023, https://doi.org/10.5194/amt-16-5847-2023, 2023
Short summary
Short summary
The vertical profiles of the effective radii of ice crystals and ice water content in Arctic semi-transparent stratiform clouds were assessed using quantitative ground-based lidar measurements. The field campaign was part of the Pollution in the ARCtic System (PARCS) project which took place from 13 to 26 May 2016 in Hammerfest (70° 39′ 48″ N, 23° 41′ 00″ E). We show that under certain cloud conditions, lidar measurement combined with a dedicated algorithmic approach is an efficient tool.
Leonie Villiger, Marina Dütsch, Sandrine Bony, Marie Lothon, Stephan Pfahl, Heini Wernli, Pierre-Etienne Brilouet, Patrick Chazette, Pierre Coutris, Julien Delanoë, Cyrille Flamant, Alfons Schwarzenboeck, Martin Werner, and Franziska Aemisegger
Atmos. Chem. Phys., 23, 14643–14672, https://doi.org/10.5194/acp-23-14643-2023, https://doi.org/10.5194/acp-23-14643-2023, 2023
Short summary
Short summary
This study evaluates three numerical simulations performed with an isotope-enabled weather forecast model and investigates the coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. We show that the simulations reproduce key characteristics of shallow trade-wind clouds as observed during the field experiment EUREC4A and that the spatial distribution of stable-water-vapour isotopes is shaped by the overturning circulation associated with these clouds.
Cyrille Flamant, Marco Gaetani, Jean-Pierre Chaboureau, Patrick Chazette, Juan Cuesta, Stuart John Piketh, and Paola Formenti
Atmos. Chem. Phys., 22, 5701–5724, https://doi.org/10.5194/acp-22-5701-2022, https://doi.org/10.5194/acp-22-5701-2022, 2022
Short summary
Short summary
Rivers of smoke extend from tropical southern Africa towards the Indian Ocean during the winter fire season, controlled by the interaction of tropical easterly waves, and westerly waves at mid latitudes. During the AEROCLO-sA field campaign in 2017, a river of smoke was directly observed over Namibia. In this paper, the evolution and atmospheric drivers of the river of smoke are described, and the role of a mid-latitude cut-off low in lifting the smoke to the upper troposphere is highlighted.
Sandrine Bony, Marie Lothon, Julien Delanoë, Pierre Coutris, Jean-Claude Etienne, Franziska Aemisegger, Anna Lea Albright, Thierry André, Hubert Bellec, Alexandre Baron, Jean-François Bourdinot, Pierre-Etienne Brilouet, Aurélien Bourdon, Jean-Christophe Canonici, Christophe Caudoux, Patrick Chazette, Michel Cluzeau, Céline Cornet, Jean-Philippe Desbios, Dominique Duchanoy, Cyrille Flamant, Benjamin Fildier, Christophe Gourbeyre, Laurent Guiraud, Tetyana Jiang, Claude Lainard, Christophe Le Gac, Christian Lendroit, Julien Lernould, Thierry Perrin, Frédéric Pouvesle, Pascal Richard, Nicolas Rochetin, Kevin Salaün, Alfons Schwarzenboeck, Guillaume Seurat, Bjorn Stevens, Julien Totems, Ludovic Touzé-Peiffer, Gilles Vergez, Jessica Vial, Leonie Villiger, and Raphaela Vogel
Earth Syst. Sci. Data, 14, 2021–2064, https://doi.org/10.5194/essd-14-2021-2022, https://doi.org/10.5194/essd-14-2021-2022, 2022
Short summary
Short summary
The French ATR42 research aircraft participated in the EUREC4A international field campaign that took place in 2020 over the tropical Atlantic, east of Barbados. We present the extensive instrumentation of the aircraft, the research flights and the different measurements. We show that the ATR measurements of humidity, wind, aerosols and cloudiness in the lower atmosphere are robust and consistent with each other. They will make it possible to advance understanding of cloud–climate interactions.
Karine Desboeufs, Franck Fu, Matthieu Bressac, Antonio Tovar-Sánchez, Sylvain Triquet, Jean-François Doussin, Chiara Giorio, Patrick Chazette, Julie Disnaquet, Anaïs Feron, Paola Formenti, Franck Maisonneuve, Araceli Rodríguez-Romero, Pascal Zapf, François Dulac, and Cécile Guieu
Atmos. Chem. Phys., 22, 2309–2332, https://doi.org/10.5194/acp-22-2309-2022, https://doi.org/10.5194/acp-22-2309-2022, 2022
Short summary
Short summary
This article reports the first concurrent sampling of wet deposition samples and surface seawater and was performed during the PEACETIME cruise in the remote Mediterranean (May–June 2017). Through the chemical composition of trace metals (TMs) in these samples, it emphasizes the decrease of atmospheric metal pollution in this area during the last few decades and the critical role of wet deposition as source of TMs for Mediterranean surface seawater, especially for intense dust deposition events.
Patrick Chazette, Alexandre Baron, and Cyrille Flamant
Atmos. Chem. Phys., 22, 1271–1292, https://doi.org/10.5194/acp-22-1271-2022, https://doi.org/10.5194/acp-22-1271-2022, 2022
Short summary
Short summary
Within the framework of the international EUREC4A project, horizontal lidar measurements were carried out over Barbados from the French research aircraft ATR-42. These measurements highlighted the strong heterogeneity of the aerosol field (mainly dust and biomass burning aerosols) and therefore of the associated optical properties. This heterogeneity varies according to meteorological conditions and could significantly modulate the climatic impact of aerosols trapped over the tropical Atlantic.
Julien Totems, Patrick Chazette, and Alexandre Baron
Atmos. Meas. Tech., 14, 7525–7544, https://doi.org/10.5194/amt-14-7525-2021, https://doi.org/10.5194/amt-14-7525-2021, 2021
Short summary
Short summary
We describe in detail the design and calibration of the new Raman channels for the WALI system, going over the important sources of bias and uncertainty on retrieved temperature profiles. For the first time, their impact is investigated using horizontal shots in a homogenous atmosphere: the magnitude of the highlighted biases can be much larger than the targeted absolute accuracy of 1° C. Actual measurement errors are quantified using radiosoundings launched close to the lidar site.
Jonas Hamperl, Clément Capitaine, Jean-Baptiste Dherbecourt, Myriam Raybaut, Patrick Chazette, Julien Totems, Bruno Grouiez, Laurence Régalia, Rosa Santagata, Corinne Evesque, Jean-Michel Melkonian, Antoine Godard, Andrew Seidl, Harald Sodemann, and Cyrille Flamant
Atmos. Meas. Tech., 14, 6675–6693, https://doi.org/10.5194/amt-14-6675-2021, https://doi.org/10.5194/amt-14-6675-2021, 2021
Short summary
Short summary
Laser active remote sensing of tropospheric water vapor is a promising technology for enhancing our understanding of processes governing the global hydrological cycle. We investigate the potential of a ground-based lidar to monitor the main water vapor isotopes at high spatio-temporal resolutions in the lower troposphere. Using a realistic end-to-end simulator, we show that high-precision measurements can be achieved within a range of 1.5 km, in mid-latitude or tropical environments.
Cited articles
Ancellet, G., Pelon, J., Totems, J., Chazette, P., Bazureau, A., Sicard, M., Di Iorio, T., Dulac, F., and Mallet, M.: Long-range transport and mixing of aerosol sources during the 2013 North American biomass burning episode: analysis of multiple lidar observations in the western Mediterranean basin, Atmos. Chem. Phys., 16, 4725–4742, https://doi.org/10.5194/acp-16-4725-2016, 2016.
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Short summary
By coupling lidar on board a ULA and ground-based lidar measurements, this paper highlights aerosol transport over the Strait of Gibraltar. It shows that the lidar-derived aerosol optical properties can be different from what is commonly accepted. It presents unprecedented vertical profiles over this region and relates them to the origin of air masses. The results are based on ground, airborne, and spaceborne observations, as well as multiple retro-trajectory analyses.
By coupling lidar on board a ULA and ground-based lidar measurements, this paper highlights...