Articles | Volume 9, issue 7
https://doi.org/10.5194/amt-9-3131-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-9-3131-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
20 Jul 2016
Research article |
| 20 Jul 2016
PHIPS–HALO: the airborne Particle Habit Imaging and Polar Scattering probe – Part 1: Design and operation
Ahmed Abdelmonem
CORRESPONDING AUTHOR
Institute for Meteorology and Climate Research, Karlsruhe Institute of
Technology, Karlsruhe, Germany
Emma Järvinen
Institute for Meteorology and Climate Research, Karlsruhe Institute of
Technology, Karlsruhe, Germany
Denis Duft
Institute for Meteorology and Climate Research, Karlsruhe Institute of
Technology, Karlsruhe, Germany
Edwin Hirst
Centre for Atmospheric and Instrumentation Research, University of
Hertfordshire, Hatfield, AL10 9AB, UK
Steffen Vogt
Institute for Meteorology and Climate Research, Karlsruhe Institute of
Technology, Karlsruhe, Germany
Thomas Leisner
Institute for Meteorology and Climate Research, Karlsruhe Institute of
Technology, Karlsruhe, Germany
Martin Schnaiter
CORRESPONDING AUTHOR
Institute for Meteorology and Climate Research, Karlsruhe Institute of
Technology, Karlsruhe, Germany
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Magdalena Vallon, Linyu Gao, Feng Jiang, Bianca Krumm, Jens Nadolny, Junwei Song, Thomas Leisner, and Harald Saathoff
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Lucía Caudillo, Birte Rörup, Martin Heinritzi, Guillaume Marie, Mario Simon, Andrea C. Wagner, Tatjana Müller, Manuel Granzin, Antonio Amorim, Farnoush Ataei, Rima Baalbaki, Barbara Bertozzi, Zoé Brasseur, Randall Chiu, Biwu Chu, Lubna Dada, Jonathan Duplissy, Henning Finkenzeller, Loïc Gonzalez Carracedo, Xu-Cheng He, Victoria Hofbauer, Weimeng Kong, Houssni Lamkaddam, Chuan P. Lee, Brandon Lopez, Naser G. A. Mahfouz, Vladimir Makhmutov, Hanna E. Manninen, Ruby Marten, Dario Massabò, Roy L. Mauldin, Bernhard Mentler, Ugo Molteni, Antti Onnela, Joschka Pfeifer, Maxim Philippov, Ana A. Piedehierro, Meredith Schervish, Wiebke Scholz, Benjamin Schulze, Jiali Shen, Dominik Stolzenburg, Yuri Stozhkov, Mihnea Surdu, Christian Tauber, Yee Jun Tham, Ping Tian, António Tomé, Steffen Vogt, Mingyi Wang, Dongyu S. Wang, Stefan K. Weber, André Welti, Wang Yonghong, Wu Yusheng, Marcel Zauner-Wieczorek, Urs Baltensperger, Imad El Haddad, Richard C. Flagan, Armin Hansel, Kristina Höhler, Jasper Kirkby, Markku Kulmala, Katrianne Lehtipalo, Ottmar Möhler, Harald Saathoff, Rainer Volkamer, Paul M. Winkler, Neil M. Donahue, Andreas Kürten, and Joachim Curtius
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Ulrich Platt, Thomas Wagner, Jonas Kuhn, and Thomas Leisner
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Janne Lampilahti, Hanna E. Manninen, Tuomo Nieminen, Sander Mirme, Mikael Ehn, Iida Pullinen, Katri Leino, Siegfried Schobesberger, Juha Kangasluoma, Jenni Kontkanen, Emma Järvinen, Riikka Väänänen, Taina Yli-Juuti, Radovan Krejci, Katrianne Lehtipalo, Janne Levula, Aadu Mirme, Stefano Decesari, Ralf Tillmann, Douglas R. Worsnop, Franz Rohrer, Astrid Kiendler-Scharr, Tuukka Petäjä, Veli-Matti Kerminen, Thomas F. Mentel, and Markku Kulmala
Atmos. Chem. Phys., 21, 12649–12663, https://doi.org/10.5194/acp-21-12649-2021, https://doi.org/10.5194/acp-21-12649-2021, 2021
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Alexei A. Kiselev, Alice Keinert, Tilia Gaedeke, Thomas Leisner, Christoph Sutter, Elena Petrishcheva, and Rainer Abart
Atmos. Chem. Phys., 21, 11801–11814, https://doi.org/10.5194/acp-21-11801-2021, https://doi.org/10.5194/acp-21-11801-2021, 2021
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Hengheng Zhang, Frank Wagner, Harald Saathoff, Heike Vogel, Gholam Ali Hoshyaripour, Vanessa Bachmann, Jochen Förstner, and Thomas Leisner
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-193, https://doi.org/10.5194/amt-2021-193, 2021
Revised manuscript not accepted
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Barbara Bertozzi, Robert Wagner, Junwei Song, Kristina Höhler, Joschka Pfeifer, Harald Saathoff, Thomas Leisner, and Ottmar Möhler
Atmos. Chem. Phys., 21, 10779–10798, https://doi.org/10.5194/acp-21-10779-2021, https://doi.org/10.5194/acp-21-10779-2021, 2021
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Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Meas. Tech., 14, 3049–3070, https://doi.org/10.5194/amt-14-3049-2021, https://doi.org/10.5194/amt-14-3049-2021, 2021
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A major challenge in the observations of mixed-phase clouds remains the phase discrimination and sizing of cloud droplets and ice crystals, especially for particles with diameters smaller than 0.1 mm. Here, we present a new method to derive the phase and size of single cloud particles using their angular-light-scattering information. Comparisons with other in situ instruments in three case studies show good agreement.
Julia Schneider, Kristina Höhler, Paavo Heikkilä, Jorma Keskinen, Barbara Bertozzi, Pia Bogert, Tobias Schorr, Nsikanabasi Silas Umo, Franziska Vogel, Zoé Brasseur, Yusheng Wu, Simo Hakala, Jonathan Duplissy, Dmitri Moisseev, Markku Kulmala, Michael P. Adams, Benjamin J. Murray, Kimmo Korhonen, Liqing Hao, Erik S. Thomson, Dimitri Castarède, Thomas Leisner, Tuukka Petäjä, and Ottmar Möhler
Atmos. Chem. Phys., 21, 3899–3918, https://doi.org/10.5194/acp-21-3899-2021, https://doi.org/10.5194/acp-21-3899-2021, 2021
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By triggering the formation of ice crystals, ice-nucleating particles (INP) strongly influence cloud formation. Continuous, long-term measurements are needed to characterize the atmospheric INP variability. Here, a first long-term time series of INP spectra measured in the boreal forest for more than 1 year is presented, showing a clear seasonal cycle. It is shown that the seasonal dependency of INP concentrations and prevalent INP types is driven by the abundance of biogenic aerosol.
Robert Wagner, Baptiste Testa, Michael Höpfner, Alexei Kiselev, Ottmar Möhler, Harald Saathoff, Jörn Ungermann, and Thomas Leisner
Atmos. Meas. Tech., 14, 1977–1991, https://doi.org/10.5194/amt-14-1977-2021, https://doi.org/10.5194/amt-14-1977-2021, 2021
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Michael Krayer, Agathe Chouippe, Markus Uhlmann, Jan Dušek, and Thomas Leisner
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Alexei Korolev and Thomas Leisner
Atmos. Chem. Phys., 20, 11767–11797, https://doi.org/10.5194/acp-20-11767-2020, https://doi.org/10.5194/acp-20-11767-2020, 2020
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Secondary ice production (SIP) plays a key role in the formation of ice particles in tropospheric clouds. This work presents a critical review of the laboratory studies related to secondary ice production. It aims to identify gaps in our knowledge of SIP as well as to stimulate further laboratory studies focused on obtaining a quantitative description of efficiencies for each SIP mechanism.
Isabelle Steinke, Naruki Hiranuma, Roger Funk, Kristina Höhler, Nadine Tüllmann, Nsikanabasi Silas Umo, Peter G. Weidler, Ottmar Möhler, and Thomas Leisner
Atmos. Chem. Phys., 20, 11387–11397, https://doi.org/10.5194/acp-20-11387-2020, https://doi.org/10.5194/acp-20-11387-2020, 2020
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In this study, we highlight the potential impact of particles from certain terrestrial sources on the formation of ice crystals in clouds. In particular, we focus on biogenic particles consisting of various organic compounds, which makes it very difficult to predict the ice nucleation properties of complex ambient particles. We find that these ambient particles are often more ice active than individual components.
Ahmed Abdelmonem, Sanduni Ratnayake, Jonathan D. Toner, and Johannes Lützenkirchen
Atmos. Chem. Phys., 20, 1075–1087, https://doi.org/10.5194/acp-20-1075-2020, https://doi.org/10.5194/acp-20-1075-2020, 2020
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We address, on the molecular level, the potential for, and consequences of, surface property variations in aerosol particles in the atmosphere. Aerosol surface aging changes the interfacial chemistry, giving rise to marked variations in the ice nucleation ability of the surface. This study provides new insights into atmospheric processes, particularly cloud formation and aerosol aging in the atmosphere, with potential implications for the pharmaceutical and food industries.
Helen R. Smith, Zbigniew Ulanowski, Paul H. Kaye, Edwin Hirst, Warren Stanley, Richard Kaye, Andreas Wieser, Chris Stopford, Maria Kezoudi, Joseph Girdwood, Richard Greenaway, and Robert Mackenzie
Atmos. Meas. Tech., 12, 6579–6599, https://doi.org/10.5194/amt-12-6579-2019, https://doi.org/10.5194/amt-12-6579-2019, 2019
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The Universal Cloud and Aerosol Sounding System (UCASS) is a low-cost miniature optical particle counter (OPC) capable of sizing particles in the size range 0.4–40 μm. The open-geometry design makes the instrument suitable for deployment on balloon-borne sounding systems, dropsonde systems or as part of an unmanned aerial vehicle (UAV). Laboratory and field experiments show good agreement with reference instruments in a range of cloudy and dusty environments.
André Ehrlich, Manfred Wendisch, Christof Lüpkes, Matthias Buschmann, Heiko Bozem, Dmitri Chechin, Hans-Christian Clemen, Régis Dupuy, Olliver Eppers, Jörg Hartmann, Andreas Herber, Evelyn Jäkel, Emma Järvinen, Olivier Jourdan, Udo Kästner, Leif-Leonard Kliesch, Franziska Köllner, Mario Mech, Stephan Mertes, Roland Neuber, Elena Ruiz-Donoso, Martin Schnaiter, Johannes Schneider, Johannes Stapf, and Marco Zanatta
Earth Syst. Sci. Data, 11, 1853–1881, https://doi.org/10.5194/essd-11-1853-2019, https://doi.org/10.5194/essd-11-1853-2019, 2019
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During the Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) campaign, two research aircraft (Polar 5 and 6) jointly performed 22 research flights over the transition zone between open ocean and closed sea ice. The data set combines remote sensing and in situ measurement of cloud, aerosol, and trace gas properties, as well as turbulent and radiative fluxes, which will be used to study Arctic boundary layer and mid-level clouds and their role in Arctic amplification.
Xiaoli Shen, Heike Vogel, Bernhard Vogel, Wei Huang, Claudia Mohr, Ramakrishna Ramisetty, Thomas Leisner, André S. H. Prévôt, and Harald Saathoff
Atmos. Chem. Phys., 19, 13189–13208, https://doi.org/10.5194/acp-19-13189-2019, https://doi.org/10.5194/acp-19-13189-2019, 2019
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This study provides good insight into the chemical nature and complex origin of aerosols by combining comprehensive field observations and transport modelling. We suggest that factors related to topography, metrological conditions, local emissions, in situ formation and growth, regional transport, and the interaction of biogenic and anthropogenic compounds need to be considered for a comprehensive understanding of aerosol processes.
Tasha Aylett, James S. A. Brooke, Alexander D. James, Mario Nachbar, Denis Duft, Thomas Leisner, and John M. C. Plane
Atmos. Chem. Phys., 19, 12767–12777, https://doi.org/10.5194/acp-19-12767-2019, https://doi.org/10.5194/acp-19-12767-2019, 2019
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Interplanetary dust particles entering the Earth's atmosphere often melt and evaporate, injecting metals such as iron and magnesium into the atmosphere between 80 and 105 km. These metals become oxidized and then coagulate into small particles a few nanometres is size, known as meteoric smoke. In this study, iron oxide smoke particles were created in the laboratory, and their composition and optical properties were determined in order to understand satellite measurements.
Wei Huang, Harald Saathoff, Xiaoli Shen, Ramakrishna Ramisetty, Thomas Leisner, and Claudia Mohr
Atmos. Chem. Phys., 19, 11687–11700, https://doi.org/10.5194/acp-19-11687-2019, https://doi.org/10.5194/acp-19-11687-2019, 2019
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We investigate the molecular composition and volatility of oxygenated organic aerosol (OOA) particles in summer and winter in Stuttgart, Germany. OOA in summer is more influenced by biogenic emissions, while in winter biomass burning emissions are an important source. OOA in winter is also less volatile. Potential reasons are discussed in our paper. Our study shows the important contributions of nonfossil OA from biogenic and biomass burning even in an urban area with high traffic emissions.
Martin Schnaiter, Claudia Linke, Inas Ibrahim, Alexei Kiselev, Fritz Waitz, Thomas Leisner, Stefan Norra, and Till Rehm
Atmos. Chem. Phys., 19, 10829–10844, https://doi.org/10.5194/acp-19-10829-2019, https://doi.org/10.5194/acp-19-10829-2019, 2019
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When combustion particles are deposited to the ground, they darken Earth's snow and ice surfaces by even tiny quantities. This darkening reduces the back reflection of sunlight and induces an additional climate warming. Particles from fresh snow samples were investigated according to their light absorption strength. Enhanced absorption was found in the snow that cannot fully be attributed to combustion particles. Dust and biogenic matter are likely the cause of this additional snow darkening.
Nsikanabasi Silas Umo, Robert Wagner, Romy Ullrich, Alexei Kiselev, Harald Saathoff, Peter G. Weidler, Daniel J. Cziczo, Thomas Leisner, and Ottmar Möhler
Atmos. Chem. Phys., 19, 8783–8800, https://doi.org/10.5194/acp-19-8783-2019, https://doi.org/10.5194/acp-19-8783-2019, 2019
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Annually, over 600 Tg of coal fly ash (CFA) is produced; a significant proportion of this amount is injected into the atmosphere, which could significantly contribute to heterogeneous ice formation in clouds. This study presents an improved understanding of CFA particles' behaviour in forming ice in clouds, especially when exposed to lower temperatures before being re-circulated in the upper troposphere or entrained into the lower troposphere.
Xiaoli Shen, Harald Saathoff, Wei Huang, Claudia Mohr, Ramakrishna Ramisetty, and Thomas Leisner
Atmos. Meas. Tech., 12, 2219–2240, https://doi.org/10.5194/amt-12-2219-2019, https://doi.org/10.5194/amt-12-2219-2019, 2019
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Based on single-particle mass spectra from field measurements in the upper Rhine valley, we identified characteristic particle classes and estimated their mass contributions without the need of a reference instrument in the field. Our study provides a good example for quantitative interpretation of single-particle data. Together with the complimentary results from bulk measurements, we have shown how a better understanding of the mixing state of ambient aerosol particles can be achieved.
Mario Nachbar, Henrike Wilms, Denis Duft, Tasha Aylett, Kensei Kitajima, Takuya Majima, John M. C. Plane, Markus Rapp, and Thomas Leisner
Atmos. Chem. Phys., 19, 4311–4322, https://doi.org/10.5194/acp-19-4311-2019, https://doi.org/10.5194/acp-19-4311-2019, 2019
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Polar mesospheric clouds (PMC) are water ice clouds forming on nanoparticles in the polar summer mesopause. We investigate the impact of solar radiation on PMC formation in the laboratory. We show that Mie theory calculations combined with an equilibrium temperature model presented in this work predict the warming of the particles very well. Using this model we demonstrate that the impact of solar radiation on ice particle formation is significantly lower than previously assumed.
Shiwen Teng, Chao Liu, Martin Schnaiter, Rajan K. Chakrabarty, and Fengshan Liu
Atmos. Chem. Phys., 19, 2917–2931, https://doi.org/10.5194/acp-19-2917-2019, https://doi.org/10.5194/acp-19-2917-2019, 2019
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Black carbon (BC) possesses complex minor structures besides the overall aggregate geometry, thus altering their optical properties. This study introduces volume variation to quantify and unify different minor structures and develops an empirical relation to account for their effects on BC optical properties. We find the effects of minor structures are mainly contributed by their influence on particle volume/mass, and a relative difference of 5 % is noticed after removing volume differences.
Denis Duft, Mario Nachbar, and Thomas Leisner
Atmos. Chem. Phys., 19, 2871–2879, https://doi.org/10.5194/acp-19-2871-2019, https://doi.org/10.5194/acp-19-2871-2019, 2019
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How ice particles form in polar mesospheric clouds is still a challenging question. We measured the water adsorption and onset conditions for ice growth on meteoric smoke analogue particles in the laboratory. We find that the particles activate by growth of amorphous ice and at much warmer conditions than previously assumed, affirming meteoric smoke as likely seeds in mesospheric ice clouds. We propose an ice-activation model and show that the particle charge does not play a significant role.
Emma Järvinen, Olivier Jourdan, David Neubauer, Bin Yao, Chao Liu, Meinrat O. Andreae, Ulrike Lohmann, Manfred Wendisch, Greg M. McFarquhar, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 18, 15767–15781, https://doi.org/10.5194/acp-18-15767-2018, https://doi.org/10.5194/acp-18-15767-2018, 2018
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Using light diffraction it is possible to detect microscopic features within ice particles that have not yet been fully characterized. Here, this technique was applied in airborne measurements, where it was found that majority of atmospheric ice particles have features that significantly change the way ice particles interact with solar light. The microscopic features make ice-containing clouds more reflective than previously thought, which could have consequences for predicting our climate.
Ramakrishna Ramisetty, Ahmed Abdelmonem, Xiaoli Shen, Harald Saathoff, Thomas Leisner, and Claudia Mohr
Atmos. Meas. Tech., 11, 4345–4360, https://doi.org/10.5194/amt-11-4345-2018, https://doi.org/10.5194/amt-11-4345-2018, 2018
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In this study we coupled a laser ablation aerosol time-of-flight (LAAPTOF) single-particle mass spectrometer, originally equipped with an excimer laser, to a femtosecond laser. The objective was to assess the influence of the higher laser power density of the femtosecond laser on ablation–ionization of atmospheric particles, ion signal, and ultimately quantitative abilities of the single-particle mass spectrometer.
Chao Liu, Chul Eddy Chung, Yan Yin, and Martin Schnaiter
Atmos. Chem. Phys., 18, 6259–6273, https://doi.org/10.5194/acp-18-6259-2018, https://doi.org/10.5194/acp-18-6259-2018, 2018
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The absorption Ångström exponent (AAE) of black carbon (BC) is widely accepted to be 1.0, although observational estimates give a quite wide range of 0.6–1.1. This study investigates BC AAE numerically using realistic particle properties and accurate numerical models. The significantly influence of BC microphysical properties on BC AAE is revealed by simple linear formulas, and the widely accepted BC AAE value of 1.0 is not correct for even small BC with wavelength-independent refractive index.
Xiaoli Shen, Ramakrishna Ramisetty, Claudia Mohr, Wei Huang, Thomas Leisner, and Harald Saathoff
Atmos. Meas. Tech., 11, 2325–2343, https://doi.org/10.5194/amt-11-2325-2018, https://doi.org/10.5194/amt-11-2325-2018, 2018
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This paper presents performance data and reference spectra from the commercially available single-particle mass spectrometer LAAPTOF. The main characteristics of the instrument, like its detection efficiency, are given for a wide particle size range. Furthermore, reference mass spectra for 32 well-defined different particle types relevant for atmospheric aerosol compounds are presented. It is shown that these reference mass spectra are very useful in analysis of atmospheric aerosol particles.
Mario Nachbar, Denis Duft, and Thomas Leisner
Atmos. Chem. Phys., 18, 3419–3431, https://doi.org/10.5194/acp-18-3419-2018, https://doi.org/10.5194/acp-18-3419-2018, 2018
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The crystallization process of amorphous ice below 160 K forms nano-crystalline ice. We report high-quality vapor pressure measurements over ice crystallized from amorphous ice below 160 K. We show that the vapor pressure is increased by more than 100 % compared to bulk crystalline ice and that amorphous ice always forms first, followed by the crystallization of nano-crystalline ice. Our findings are relevant for cold ice clouds in the atmospheres of planets, e.g., Earth and Mars.
Wei Huang, Harald Saathoff, Aki Pajunoja, Xiaoli Shen, Karl-Heinz Naumann, Robert Wagner, Annele Virtanen, Thomas Leisner, and Claudia Mohr
Atmos. Chem. Phys., 18, 2883–2898, https://doi.org/10.5194/acp-18-2883-2018, https://doi.org/10.5194/acp-18-2883-2018, 2018
Sylvia C. Sullivan, Corinna Hoose, Alexei Kiselev, Thomas Leisner, and Athanasios Nenes
Atmos. Chem. Phys., 18, 1593–1610, https://doi.org/10.5194/acp-18-1593-2018, https://doi.org/10.5194/acp-18-1593-2018, 2018
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Ice multiplication (IM) processes can have a profound impact on cloud and precipitation development but are poorly understood. Here we study whether a lower limit of ice nuclei exists to initiate IM. The lower limit is found to be extremely low (0.01 per liter or less). A counterintuitive but profound conclusion thus emerges: IM requires cloud formation around a thermodynamic
sweet spotand is sensitive to fluctuations in cloud condensation nuclei concentration alone.
Meinrat O. Andreae, Armin Afchine, Rachel Albrecht, Bruna Amorim Holanda, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Micael A. Cecchini, Anja Costa, Maximilian Dollner, Daniel Fütterer, Emma Järvinen, Tina Jurkat, Thomas Klimach, Tobias Konemann, Christoph Knote, Martina Krämer, Trismono Krisna, Luiz A. T. Machado, Stephan Mertes, Andreas Minikin, Christopher Pöhlker, Mira L. Pöhlker, Ulrich Pöschl, Daniel Rosenfeld, Daniel Sauer, Hans Schlager, Martin Schnaiter, Johannes Schneider, Christiane Schulz, Antonio Spanu, Vinicius B. Sperling, Christiane Voigt, Adrian Walser, Jian Wang, Bernadett Weinzierl, Manfred Wendisch, and Helmut Ziereis
Atmos. Chem. Phys., 18, 921–961, https://doi.org/10.5194/acp-18-921-2018, https://doi.org/10.5194/acp-18-921-2018, 2018
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We made airborne measurements of aerosol particle concentrations and properties over the Amazon Basin. We found extremely high concentrations of very small particles in the region between 8 and 14 km altitude all across the basin, which had been recently formed by gas-to-particle conversion at these altitudes. This makes the upper troposphere a very important source region of atmospheric particles with significant implications for the Earth's climate system.
Martin Schnaiter, Emma Järvinen, Ahmed Abdelmonem, and Thomas Leisner
Atmos. Meas. Tech., 11, 341–357, https://doi.org/10.5194/amt-11-341-2018, https://doi.org/10.5194/amt-11-341-2018, 2018
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PHIPS-HALO is a novel aircraft instrument for cloud research. It combines microscopic imaging of single cloud particles with the measurement of their spacial light scattering properties. The knowledge of how atmospheric ice particles in clouds scatter visible light is important for improving future climate models.
Ahmed Abdelmonem
Atmos. Chem. Phys., 17, 10733–10741, https://doi.org/10.5194/acp-17-10733-2017, https://doi.org/10.5194/acp-17-10733-2017, 2017
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On the basis of supercooled SHG spectroscopy, I report molecular-level evidence for the existence of one- and two-step deposition freezing depending on the surface type and the supersaturation conditions. In addition, immersion freezing shows a transient ice phase with a lifetime of c. 1 min. This study provides new insights into atmospheric processes and can impact various industrial and research branches, particularly climate change, weather modification, and tracing water in the hydrosphere.
Leonid Nichman, Emma Järvinen, James Dorsey, Paul Connolly, Jonathan Duplissy, Claudia Fuchs, Karoliina Ignatius, Kamalika Sengupta, Frank Stratmann, Ottmar Möhler, Martin Schnaiter, and Martin Gallagher
Atmos. Meas. Tech., 10, 3231–3248, https://doi.org/10.5194/amt-10-3231-2017, https://doi.org/10.5194/amt-10-3231-2017, 2017
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Optical probes are frequently used for the detection of cloud particles. The detected microphysical properties may affect particle growth and accretion mechanisms and the light scattering properties of cirrus clouds. In the CLOUD chamber study at CERN, we compared four optical measurement techniques. We show that shape derivation alone is not sufficient to determine the phase of the small cloud particles. None of the instruments were able to unambiguously determine the phase of small particles.
Ahmed Abdelmonem, Ellen H. G. Backus, Nadine Hoffmann, M. Alejandra Sánchez, Jenée D. Cyran, Alexei Kiselev, and Mischa Bonn
Atmos. Chem. Phys., 17, 7827–7837, https://doi.org/10.5194/acp-17-7827-2017, https://doi.org/10.5194/acp-17-7827-2017, 2017
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We report the effect of surface charge on heterogeneous immersion freezing for the atmospherically relevant sapphire surface. Combining linear and nonlinear optical techniques and investigating isolated drops, we find that charge-induced surface templating is detrimental for ice nucleation on α-alumina surface. This study provides new insights into atmospheric processes and can impact various industrial and research branches, particularly climate change and tracing of water in the hydrosphere.
Claudia Linke, Inas Ibrahim, Nina Schleicher, Regina Hitzenberger, Meinrat O. Andreae, Thomas Leisner, and Martin Schnaiter
Atmos. Meas. Tech., 9, 5331–5346, https://doi.org/10.5194/amt-9-5331-2016, https://doi.org/10.5194/amt-9-5331-2016, 2016
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Various carbonaceous materials are present in the atmosphere. Besides gaseous organic compounds, carbonaceous particles like soot are emitted into the air from traffic sources, residential wood combustion, or wildfires. Variable chemical compositions of such materials, which often result from incomplete combustion processes, show differences in the absorption behavior at visible wavelengths. Our instrument is able to measure the absorption at three visible wavelengths.
Andreas Peckhaus, Alexei Kiselev, Thibault Hiron, Martin Ebert, and Thomas Leisner
Atmos. Chem. Phys., 16, 11477–11496, https://doi.org/10.5194/acp-16-11477-2016, https://doi.org/10.5194/acp-16-11477-2016, 2016
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The precipitation in midlatitude clouds proceeds predominantly via nucleation of ice in the supercooled droplets containing foreign inclusions, like feldspar mineral dust, that have been recently identified as one of the most active ice nucleating agents in the atmosphere. We have built an apparatus to observe the freezing of feldspar immersed in up to 1500 identical droplets simultaneously. With this setup we investigated four feldspar samples and show that it can induce freezing at −5 °C.
Naruki Hiranuma, Ottmar Möhler, Gourihar Kulkarni, Martin Schnaiter, Steffen Vogt, Paul Vochezer, Emma Järvinen, Robert Wagner, David M. Bell, Jacqueline Wilson, Alla Zelenyuk, and Daniel J. Cziczo
Atmos. Meas. Tech., 9, 3817–3836, https://doi.org/10.5194/amt-9-3817-2016, https://doi.org/10.5194/amt-9-3817-2016, 2016
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A new pumped counterflow virtual impactor (PCVI) called the ice-selecting PCVI (IS-PCVI) has been developed to collect ice crystal residuals for investigating physico-chemical properties of ice-nucleating particles. The results show that the ice crystals of volume-equivalent diameter ~ 10 to 30 µm can be efficiently separated from the supercooled droplets and interstitial particles. The IS-PCVI is efficient when the counterflow-to-input flow ratio is within 0.09 to 0.18.
Yvonne Boose, Berko Sierau, M. Isabel García, Sergio Rodríguez, Andrés Alastuey, Claudia Linke, Martin Schnaiter, Piotr Kupiszewski, Zamin A. Kanji, and Ulrike Lohmann
Atmos. Chem. Phys., 16, 9067–9087, https://doi.org/10.5194/acp-16-9067-2016, https://doi.org/10.5194/acp-16-9067-2016, 2016
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Mineral dust is known to be among the most prevalent ice-nucleating particles (INPs) in the atmosphere, playing a crucial role for ice cloud formation. We present 2 months of ground-based in situ measurements of INP concentrations in the free troposphere close to the largest global dust source, the Sahara. We find that some atmospheric processes such as mixing with biological particles and ammonium increase the dust INP ability. This is important when predicting INPs based on emissions.
Karoliina Ignatius, Thomas B. Kristensen, Emma Järvinen, Leonid Nichman, Claudia Fuchs, Hamish Gordon, Paul Herenz, Christopher R. Hoyle, Jonathan Duplissy, Sarvesh Garimella, Antonio Dias, Carla Frege, Niko Höppel, Jasmin Tröstl, Robert Wagner, Chao Yan, Antonio Amorim, Urs Baltensperger, Joachim Curtius, Neil M. Donahue, Martin W. Gallagher, Jasper Kirkby, Markku Kulmala, Ottmar Möhler, Harald Saathoff, Martin Schnaiter, Antonio Tomé, Annele Virtanen, Douglas Worsnop, and Frank Stratmann
Atmos. Chem. Phys., 16, 6495–6509, https://doi.org/10.5194/acp-16-6495-2016, https://doi.org/10.5194/acp-16-6495-2016, 2016
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Viscous solid or semi-solid secondary organic aerosol (SOA) may influence cloud properties through ice nucleation in the atmosphere. Here, we observed heterogeneous ice nucleation of viscous α-pinene SOA at temperatures between −39 °C and −37.2 °C with ice saturation ratios significantly below the homogeneous freezing limit. Global modelling suggests that viscous biogenic SOA are present in regions where cirrus formation takes place and could contribute to the global ice nuclei budget.
Martin Schnaiter, Emma Järvinen, Paul Vochezer, Ahmed Abdelmonem, Robert Wagner, Olivier Jourdan, Guillaume Mioche, Valery N. Shcherbakov, Carl G. Schmitt, Ugo Tricoli, Zbigniew Ulanowski, and Andrew J. Heymsfield
Atmos. Chem. Phys., 16, 5091–5110, https://doi.org/10.5194/acp-16-5091-2016, https://doi.org/10.5194/acp-16-5091-2016, 2016
Emma Järvinen, Karoliina Ignatius, Leonid Nichman, Thomas B. Kristensen, Claudia Fuchs, Christopher R. Hoyle, Niko Höppel, Joel C. Corbin, Jill Craven, Jonathan Duplissy, Sebastian Ehrhart, Imad El Haddad, Carla Frege, Hamish Gordon, Tuija Jokinen, Peter Kallinger, Jasper Kirkby, Alexei Kiselev, Karl-Heinz Naumann, Tuukka Petäjä, Tamara Pinterich, Andre S. H. Prevot, Harald Saathoff, Thea Schiebel, Kamalika Sengupta, Mario Simon, Jay G. Slowik, Jasmin Tröstl, Annele Virtanen, Paul Vochezer, Steffen Vogt, Andrea C. Wagner, Robert Wagner, Christina Williamson, Paul M. Winkler, Chao Yan, Urs Baltensperger, Neil M. Donahue, Rick C. Flagan, Martin Gallagher, Armin Hansel, Markku Kulmala, Frank Stratmann, Douglas R. Worsnop, Ottmar Möhler, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 16, 4423–4438, https://doi.org/10.5194/acp-16-4423-2016, https://doi.org/10.5194/acp-16-4423-2016, 2016
Leonid Nichman, Claudia Fuchs, Emma Järvinen, Karoliina Ignatius, Niko Florian Höppel, Antonio Dias, Martin Heinritzi, Mario Simon, Jasmin Tröstl, Andrea Christine Wagner, Robert Wagner, Christina Williamson, Chao Yan, Paul James Connolly, James Robert Dorsey, Jonathan Duplissy, Sebastian Ehrhart, Carla Frege, Hamish Gordon, Christopher Robert Hoyle, Thomas Bjerring Kristensen, Gerhard Steiner, Neil McPherson Donahue, Richard Flagan, Martin William Gallagher, Jasper Kirkby, Ottmar Möhler, Harald Saathoff, Martin Schnaiter, Frank Stratmann, and António Tomé
Atmos. Chem. Phys., 16, 3651–3664, https://doi.org/10.5194/acp-16-3651-2016, https://doi.org/10.5194/acp-16-3651-2016, 2016
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Processes in the atmosphere are often governed by the physical and chemical properties of small cloud particles. Ice, water, and mixed clouds, as well as viscous aerosols, were formed under controlled conditions at the CLOUD-CERN facility. The experimental results show a link between cloud particle properties and their unique optical fingerprints. The classification map presented here allows easier discrimination between various particles such as viscous organic aerosol, salt, ice, and liquid.
Jenni Kontkanen, Emma Järvinen, Hanna E. Manninen, Katrianne Lehtipalo, Juha Kangasluoma, Stefano Decesari, Gian Paolo Gobbi, Ari Laaksonen, Tuukka Petäjä, and Markku Kulmala
Atmos. Chem. Phys., 16, 1919–1935, https://doi.org/10.5194/acp-16-1919-2016, https://doi.org/10.5194/acp-16-1919-2016, 2016
C. R. Hoyle, C. Fuchs, E. Järvinen, H. Saathoff, A. Dias, I. El Haddad, M. Gysel, S. C. Coburn, J. Tröstl, A.-K. Bernhammer, F. Bianchi, M. Breitenlechner, J. C. Corbin, J. Craven, N. M. Donahue, J. Duplissy, S. Ehrhart, C. Frege, H. Gordon, N. Höppel, M. Heinritzi, T. B. Kristensen, U. Molteni, L. Nichman, T. Pinterich, A. S. H. Prévôt, M. Simon, J. G. Slowik, G. Steiner, A. Tomé, A. L. Vogel, R. Volkamer, A. C. Wagner, R. Wagner, A. S. Wexler, C. Williamson, P. M. Winkler, C. Yan, A. Amorim, J. Dommen, J. Curtius, M. W. Gallagher, R. C. Flagan, A. Hansel, J. Kirkby, M. Kulmala, O. Möhler, F. Stratmann, D. R. Worsnop, and U. Baltensperger
Atmos. Chem. Phys., 16, 1693–1712, https://doi.org/10.5194/acp-16-1693-2016, https://doi.org/10.5194/acp-16-1693-2016, 2016
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A significant portion of sulphate, an important constituent of atmospheric aerosols, is formed via the aqueous phase oxidation of sulphur dioxide by ozone. The rate of this reaction has previously only been measured over a relatively small temperature range. Here, we use the state of the art CLOUD chamber at CERN to perform the first measurements of this reaction rate in super-cooled droplets, confirming that the existing extrapolation of the reaction rate to sub-zero temperatures is accurate.
P. Vochezer, E. Järvinen, R. Wagner, P. Kupiszewski, T. Leisner, and M. Schnaiter
Atmos. Meas. Tech., 9, 159–177, https://doi.org/10.5194/amt-9-159-2016, https://doi.org/10.5194/amt-9-159-2016, 2016
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To study clouds constituting of liquid droplets as well as ice particles we used the latest versions of the Small Ice Detector which record high resolution scattering patterns of individual small cloud particles. In the case of a droplet its precise size is obtained and for ice particles its shape is deduced from the scattering pattern.We present results from artificial clouds at the AIDA cloud chamber and natural clouds probed at a mountain top station as well as from an aircraft in the arctic.
A. Abdelmonem, J. Lützenkirchen, and T. Leisner
Atmos. Meas. Tech., 8, 3519–3526, https://doi.org/10.5194/amt-8-3519-2015, https://doi.org/10.5194/amt-8-3519-2015, 2015
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This manuscript belongs and is important to the environmental and atmospheric science, particularly cloud formation and cloud seeding, and presents a setup to apply Second Harmonic Generation spectroscopy to heterogeneous freezing research. We describe the setup and provide first results on temperature-dependent structural changes of water on the surfaces of two relevant atmospheric aerosol substances (sapphire and mica as poor and good ice nucleators, respectively).
P. Kupiszewski, E. Weingartner, P. Vochezer, M. Schnaiter, A. Bigi, M. Gysel, B. Rosati, E. Toprak, S. Mertes, and U. Baltensperger
Atmos. Meas. Tech., 8, 3087–3106, https://doi.org/10.5194/amt-8-3087-2015, https://doi.org/10.5194/amt-8-3087-2015, 2015
M. Hummel, C. Hoose, M. Gallagher, D. A. Healy, J. A. Huffman, D. O'Connor, U. Pöschl, C. Pöhlker, N. H. Robinson, M. Schnaiter, J. R. Sodeau, M. Stengel, E. Toprak, and H. Vogel
Atmos. Chem. Phys., 15, 6127–6146, https://doi.org/10.5194/acp-15-6127-2015, https://doi.org/10.5194/acp-15-6127-2015, 2015
I. Steinke, C. Hoose, O. Möhler, P. Connolly, and T. Leisner
Atmos. Chem. Phys., 15, 3703–3717, https://doi.org/10.5194/acp-15-3703-2015, https://doi.org/10.5194/acp-15-3703-2015, 2015
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Ice nucleation in clouds has a significant influence on the global radiative budget and the hydrological cycle. Several studies have investigated the ice formation in droplets and parameterizations have been developed in order to include immersion freezing in climate models. In contrast, there are fewer studies regarding the conversion of water vapor into ice (so-called deposition nucleation) which is the topic of this paper which investigates deposition nucleation by Arizona Test dust in detail
N. Hiranuma, S. Augustin-Bauditz, H. Bingemer, C. Budke, J. Curtius, A. Danielczok, K. Diehl, K. Dreischmeier, M. Ebert, F. Frank, N. Hoffmann, K. Kandler, A. Kiselev, T. Koop, T. Leisner, O. Möhler, B. Nillius, A. Peckhaus, D. Rose, S. Weinbruch, H. Wex, Y. Boose, P. J. DeMott, J. D. Hader, T. C. J. Hill, Z. A. Kanji, G. Kulkarni, E. J. T. Levin, C. S. McCluskey, M. Murakami, B. J. Murray, D. Niedermeier, M. D. Petters, D. O'Sullivan, A. Saito, G. P. Schill, T. Tajiri, M. A. Tolbert, A. Welti, T. F. Whale, T. P. Wright, and K. Yamashita
Atmos. Chem. Phys., 15, 2489–2518, https://doi.org/10.5194/acp-15-2489-2015, https://doi.org/10.5194/acp-15-2489-2015, 2015
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Seventeen ice nucleation measurement techniques contributed to investigate the immersion freezing behavior of illite NX. All data showed a similar temperature trend, but the measured ice nucleation activity was on average smaller for the wet suspended samples and higher for the dry-dispersed aerosol samples at high temperatures. A continued investigation and collaboration is necessary to obtain further insights into consistency or diversity of ice nucleation measurements.
N. Hiranuma, M. Paukert, I. Steinke, K. Zhang, G. Kulkarni, C. Hoose, M. Schnaiter, H. Saathoff, and O. Möhler
Atmos. Chem. Phys., 14, 13145–13158, https://doi.org/10.5194/acp-14-13145-2014, https://doi.org/10.5194/acp-14-13145-2014, 2014
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A new heterogeneous ice nucleation parameterization is developed and implemented in cloud models. The results of our simulations suggest stronger influence of dust particles lifted to the upper troposphere on heterogeneous nucleation and more ice nucleation at temperature and humidity conditions relevant to both mixed-phase and cirrus clouds when compared to the existing parametrical frameworks.
Z. Ulanowski, P. H. Kaye, E. Hirst, R. S. Greenaway, R. J. Cotton, E. Hesse, and C. T. Collier
Atmos. Chem. Phys., 14, 1649–1662, https://doi.org/10.5194/acp-14-1649-2014, https://doi.org/10.5194/acp-14-1649-2014, 2014
N. Hoffmann, A. Kiselev, D. Rzesanke, D. Duft, and T. Leisner
Atmos. Meas. Tech., 6, 2373–2382, https://doi.org/10.5194/amt-6-2373-2013, https://doi.org/10.5194/amt-6-2373-2013, 2013
H. Saathoff, S. Henin, K. Stelmaszczyk, M. Petrarca, R. Delagrange, Z. Hao, J. Lüder, O. Möhler, Y. Petit, P. Rohwetter, M. Schnaiter, J. Kasparian, T. Leisner, J.-P. Wolf, and L. Wöste
Atmos. Chem. Phys., 13, 4593–4604, https://doi.org/10.5194/acp-13-4593-2013, https://doi.org/10.5194/acp-13-4593-2013, 2013
J. Skrotzki, P. Connolly, M. Schnaiter, H. Saathoff, O. Möhler, R. Wagner, M. Niemand, V. Ebert, and T. Leisner
Atmos. Chem. Phys., 13, 4451–4466, https://doi.org/10.5194/acp-13-4451-2013, https://doi.org/10.5194/acp-13-4451-2013, 2013
E. Toprak and M. Schnaiter
Atmos. Chem. Phys., 13, 225–243, https://doi.org/10.5194/acp-13-225-2013, https://doi.org/10.5194/acp-13-225-2013, 2013
M. Laborde, M. Schnaiter, C. Linke, H. Saathoff, K.-H. Naumann, O. Möhler, S. Berlenz, U. Wagner, J. W. Taylor, D. Liu, M. Flynn, J. D. Allan, H. Coe, K. Heimerl, F. Dahlkötter, B. Weinzierl, A. G. Wollny, M. Zanatta, J. Cozic, P. Laj, R. Hitzenberger, J. P. Schwarz, and M. Gysel
Atmos. Meas. Tech., 5, 3077–3097, https://doi.org/10.5194/amt-5-3077-2012, https://doi.org/10.5194/amt-5-3077-2012, 2012
Related subject area
Subject: Clouds | Technique: In Situ Measurement | Topic: Instruments and Platforms
Development and preliminary testing of a temporally controllable weather modification rocket with spatial seeding capacity
Design and evaluation of BOOGIE: a collector for the analysis of cloud composition and processes: Biological, Organics, Oxidants, soluble Gases, inorganic Ions and metal Elements
A lightweight holographic imager for cloud microphysical studies from an untethered balloon
Identifying the seeding signature in cloud particles from hydrometeor residuals
Design and rocket deployment of a trackable pseudo-Lagrangian drifter-based meteorological probe into the Lawrence/Linwood EF4 tornado and mesocyclone on 28 May 2019
A comparative analysis of in situ measurements of high-altitude cirrus in the tropics
In situ ground-based mobile measurement of lightning events above central Europe
A phase separation inlet for droplets, ice residuals, and interstitial aerosol particles
Simulation and field campaign evaluation of an optical particle counter on a fixed-wing UAV
Cloud microphysical measurements at a mountain observatory: comparison between shadowgraph imaging and phase Doppler interferometry
Use of large-eddy simulations to design an adaptive sampling strategy to assess cumulus cloud heterogeneities by remotely piloted aircraft
Post-flight analysis of detailed size distributions of warm cloud droplets, as determined in situ by cloud and aerosol spectrometers
PHIPS-HALO: the airborne Particle Habit Imaging and Polar Scattering probe – Part 3: Single-particle phase discrimination and particle size distribution based on the angular-scattering function
Applicability of the VisiSize D30 shadowgraph system for cloud microphysical measurements
Characterising optical array particle imaging probes: implications for small-ice-crystal observations
The De-Icing Comparison Experiment (D-ICE): a study of broadband radiometric measurements under icing conditions in the Arctic
The Portable Ice Nucleation Experiment (PINE): a new online instrument for laboratory studies and automated long-term field observations of ice-nucleating particles
Cézeaux-Aulnat-Opme-Puy De Dôme: a multi-site for the long-term survey of the tropospheric composition and climate change
Using a holographic imager on a tethered balloon system for microphysical observations of boundary layer clouds
Evaluation of ARM tethered-balloon system instrumentation for supercooled liquid water and distributed temperature sensing in mixed-phase Arctic clouds
Revisiting particle sizing using greyscale optical array probes: evaluation using laboratory experiments and synthetic data
Cloud fraction determined by thermal infrared and visible all-sky cameras
Development and characterization of a high-efficiency, aircraft-based axial cyclone cloud water collector
Ice particle sampling from aircraft – influence of the probing position on the ice water content
PHIPS-HALO: the airborne particle habit imaging and polar scattering probe – Part 2: Characterization and first results
A tandem approach for collocated measurements of microphysical and radiative cirrus properties
HoloGondel: in situ cloud observations on a cable car in the Swiss Alps using a holographic imager
Development of a cloud particle sensor for radiosonde sounding
Thermodynamic correction of particle concentrations measured by underwing probes on fast-flying aircraft
Quantitative evaluation of seven optical sensors for cloud microphysical measurements at the Puy-de-Dôme Observatory, France
Schneefernerhaus as a mountain research station for clouds and turbulence
High-resolution measurement of cloud microphysics and turbulence at a mountaintop station
Dual-channel photoacoustic hygrometer for airborne measurements: background, calibration, laboratory and in-flight intercomparison tests
A comparison of ice water content measurement techniques on the FAAM BAe-146 aircraft
Cloud shadow speed sensor
The backscatter cloud probe – a compact low-profile autonomous optical spectrometer
A fiber-coupled laser hygrometer for airborne total water measurement
HOLIMO II: a digital holographic instrument for ground-based in situ observations of microphysical properties of mixed-phase clouds
Evaluating the capabilities and uncertainties of droplet measurements for the fog droplet spectrometer (FM-100)
PHOCUS radiometer
First correlated measurements of the shape and light scattering properties of cloud particles using the new Particle Habit Imaging and Polar Scattering (PHIPS) probe
Effects of ice particles shattering on the 2D-S probe
Water droplet calibration of the Cloud Droplet Probe (CDP) and in-flight performance in liquid, ice and mixed-phase clouds during ARCPAC
Development of a Bioaerosol single particle detector (BIO IN) for the Fast Ice Nucleus CHamber FINCH
Xiaobo Dong, Xiaoqing Wang, Yongde Liu, and Xiaorong Wang
Atmos. Meas. Tech., 17, 5551–5559, https://doi.org/10.5194/amt-17-5551-2024, https://doi.org/10.5194/amt-17-5551-2024, 2024
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This study develops a time-controllable weather modification rocket with space seeding capabilities. Therefore, in artificial weather modification operations, parameters such as the height, thickness, and operating temperature of the target cloud can be obtained through detection. These parameters can be used to automatically calculate the appropriate sowing time, sowing height, and sowing dosage to improve the accuracy of artificial catalytic cloud operations.
Mickael Vaitilingom, Christophe Bernard, Mickael Ribeiro, Christophe Berthod, Angelica Bianco, and Laurent Deguillaume
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-95, https://doi.org/10.5194/amt-2024-95, 2024
Revised manuscript accepted for AMT
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The new collector BOOGIE has been designed and evaluated to sample cloud droplets. Computational fluid dynamic simulations are performed to evaluate the sampling efficiency for different droplets size. In situ measurements show very good water collection rates and sampling efficiency. BOOGIE is compared to other cloud collectors and the efficiency is comparable, as well as the chemical and biological compositions.
Thomas Edward Chambers, Iain Murray Reid, and Murray Hamilton
Atmos. Meas. Tech., 17, 3237–3253, https://doi.org/10.5194/amt-17-3237-2024, https://doi.org/10.5194/amt-17-3237-2024, 2024
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Clouds have been identified as the largest source of uncertainty in climate modelling. We report an untethered balloon launch of a holographic imager through clouds. This is the first time a holographic imager has been deployed in this way, enabled by the light weight and low cost of the imager. This work creates the potential to significantly increase the availability of cloud microphysical measurements required for the calibration and validation of climate models and remote sensing methods.
Mahen Konwar, Benjamin Werden, Edward C. Fortner, Sudarsan Bera, Mercy Varghese, Subharthi Chowdhuri, Kurt Hibert, Philip Croteau, John Jayne, Manjula Canagaratna, Neelam Malap, Sandeep Jayakumar, Shivsai A. Dixit, Palani Murugavel, Duncan Axisa, Darrel Baumgardner, Peter F. DeCarlo, Doug R. Worsnop, and Thara Prabhakaran
Atmos. Meas. Tech., 17, 2387–2400, https://doi.org/10.5194/amt-17-2387-2024, https://doi.org/10.5194/amt-17-2387-2024, 2024
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In a warm cloud seeding experiment hygroscopic particles are released to alter cloud processes to induce early raindrops. During the Cloud–Aerosol Interaction and Precipitation Enhancement Experiment, airborne mini aerosol mass spectrometers analyse the particles on which clouds form. The seeded clouds showed higher concentrations of chlorine and potassium, the oxidizing agents of flares. Small cloud droplet concentrations increased, and seeding particles were detected in deep cloud depths.
Reed Timmer, Mark Simpson, Sean Schofer, and Curtis Brooks
Atmos. Meas. Tech., 17, 943–960, https://doi.org/10.5194/amt-17-943-2024, https://doi.org/10.5194/amt-17-943-2024, 2024
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This work discusses a probe launched by a model rocket into an EF4 tornado and is the first time an airborne probe has directly sampled a tornado. The rocket deployed a parachuted probe recording wind speeds of 306 km h-1 in addition to temperature, humidity, and pressure deficit. Data from the probe were sent in real time to a receiver in an armored vehicle. Taking measurements directly from inside tornadoes provides new data about this violent phenomenon.
Francesco Cairo, Martina Krämer, Armin Afchine, Guido Di Donfrancesco, Luca Di Liberto, Sergey Khaykin, Lorenza Lucaferri, Valentin Mitev, Max Port, Christian Rolf, Marcel Snels, Nicole Spelten, Ralf Weigel, and Stephan Borrmann
Atmos. Meas. Tech., 16, 4899–4925, https://doi.org/10.5194/amt-16-4899-2023, https://doi.org/10.5194/amt-16-4899-2023, 2023
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Cirrus clouds have been observed over the Himalayan region between 10 km and the tropopause at 17–18 km. Data from backscattersonde, hygrometers, and particle cloud spectrometers have been compared to assess their consistency. Empirical relationships between optical parameters accessible with remote sensing lidars and cloud microphysical parameters (such as ice water content, particle number and surface area density, and particle aspherical fraction) have been established.
Jakub Kákona, Jan Mikeš, Iva Ambrožová, Ondřej Ploc, Olena Velychko, Lembit Sihver, and Martin Kákona
Atmos. Meas. Tech., 16, 547–561, https://doi.org/10.5194/amt-16-547-2023, https://doi.org/10.5194/amt-16-547-2023, 2023
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Storm activity is sometimes associated with the generation of ionizing radiation. Our motivation for performing this research was to understand its origin. Using measuring cars fitted with new instruments, it was found that the duration of lightning is longer than generally thought. In most cases, lightning occurs only inside the cloud; however, rarely, it is also visible outside the cloud. In such cases, the course of emission over time can be used to assume what it looks like inside the cloud.
Libby Koolik, Michael Roesch, Carmen Dameto de Espana, Christopher Nathan Rapp, Lesly J. Franco Deloya, Chuanyang Shen, A. Gannet Hallar, Ian B. McCubbin, and Daniel J. Cziczo
Atmos. Meas. Tech., 15, 3213–3222, https://doi.org/10.5194/amt-15-3213-2022, https://doi.org/10.5194/amt-15-3213-2022, 2022
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A new inlet for studying the small particles, droplets, and ice crystals that constitute mixed-phase clouds has been constructed and is described here. This new inlet was tested in the laboratory. We present the performance of the new inlet to demonstrate its capability of separating ice, droplets, and small particles.
Joseph Girdwood, Warren Stanley, Chris Stopford, and David Brus
Atmos. Meas. Tech., 15, 2061–2076, https://doi.org/10.5194/amt-15-2061-2022, https://doi.org/10.5194/amt-15-2061-2022, 2022
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UAVs have great potential to be used for airborne measurements of cloud and aerosol properties, which are of particular importance due to the largely uncharacterised nature of such phenomena. However, since UAVs are a new tool in atmospheric physics expensive platform validation and characterisation of UAV-instrument combinations needs to be performed. This paper presents an evaluation of a fixed-wing UAV in combination with an instrument that measures cloud droplet diameter.
Moein Mohammadi, Jakub L. Nowak, Guus Bertens, Jan Moláček, Wojciech Kumala, and Szymon P. Malinowski
Atmos. Meas. Tech., 15, 965–985, https://doi.org/10.5194/amt-15-965-2022, https://doi.org/10.5194/amt-15-965-2022, 2022
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To compare two instruments, a VisiSize D30 shadowgraph system and a phase Doppler interferometer (PDI-FPDR), we performed a series of measurements of cloud droplet size and number concentration in orographic clouds. After applying essential modifications and filters to the data, the results from the two instruments showed better agreement in droplet sizing and velocimetry than droplet number concentration or liquid water content. Discrepancies were observed for droplets smaller than 13 µm.
Nicolas Maury, Gregory C. Roberts, Fleur Couvreux, Titouan Verdu, Pierre Narvor, Najda Villefranque, Simon Lacroix, and Gautier Hattenberger
Atmos. Meas. Tech., 15, 335–352, https://doi.org/10.5194/amt-15-335-2022, https://doi.org/10.5194/amt-15-335-2022, 2022
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The paper aims to use large-eddy simulations of cumulus clouds to design a sampling strategy that allows following cumulus clouds with remotely piloted aircraft (RPA) and documenting the cloud spatial heterogeneities. Different possible explorations by RPA are investigated, and the use of Gaussian process regression permits the reconstruction of liquid water content (LWC) distribution with only one RPA.
Sorin Nicolae Vâjâiac, Andreea Calcan, Robert Oscar David, Denisa-Elena Moacă, Gabriela Iorga, Trude Storelvmo, Viorel Vulturescu, and Valeriu Filip
Atmos. Meas. Tech., 14, 6777–6794, https://doi.org/10.5194/amt-14-6777-2021, https://doi.org/10.5194/amt-14-6777-2021, 2021
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Warm clouds (with liquid droplets) play an important role in modulating the amount of incoming solar radiation to Earth’s surface and thus the climate. The most efficient way to study them is by in situ optical measurements. This paper proposes a new methodology for providing more detailed and reliable structural analyses of warm clouds through post-flight processing of collected data. The impact fine aerosol incorporation in water droplets might have on such measurements is also discussed.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Meas. Tech., 14, 3049–3070, https://doi.org/10.5194/amt-14-3049-2021, https://doi.org/10.5194/amt-14-3049-2021, 2021
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A major challenge in the observations of mixed-phase clouds remains the phase discrimination and sizing of cloud droplets and ice crystals, especially for particles with diameters smaller than 0.1 mm. Here, we present a new method to derive the phase and size of single cloud particles using their angular-light-scattering information. Comparisons with other in situ instruments in three case studies show good agreement.
Jakub L. Nowak, Moein Mohammadi, and Szymon P. Malinowski
Atmos. Meas. Tech., 14, 2615–2633, https://doi.org/10.5194/amt-14-2615-2021, https://doi.org/10.5194/amt-14-2615-2021, 2021
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A commercial instrument that characterizes sprays via shadowgraphy imaging was applied to measure the number concentration and size distribution of cloud droplets. Laboratory and field tests were performed to verify the resolution, detection reliability and sizing accuracy. We developed a correction to the data processing method which improves the estimation of cloud microphysical properties. The paper concludes with recommendations concerning the use of the instrument in cloud physics studies.
Sebastian O'Shea, Jonathan Crosier, James Dorsey, Louis Gallagher, Waldemar Schledewitz, Keith Bower, Oliver Schlenczek, Stephan Borrmann, Richard Cotton, Christopher Westbrook, and Zbigniew Ulanowski
Atmos. Meas. Tech., 14, 1917–1939, https://doi.org/10.5194/amt-14-1917-2021, https://doi.org/10.5194/amt-14-1917-2021, 2021
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The number, shape, and size of ice crystals in clouds are important properties that influence the Earth's radiation budget, cloud evolution, and precipitation formation. This work suggests that one of the most widely used methods for in situ measurements of these properties has significant uncertainties and biases. We suggest methods that dramatically improve these measurements, which can be applied to past and future datasets from these instruments.
Christopher J. Cox, Sara M. Morris, Taneil Uttal, Ross Burgener, Emiel Hall, Mark Kutchenreiter, Allison McComiskey, Charles N. Long, Bryan D. Thomas, and James Wendell
Atmos. Meas. Tech., 14, 1205–1224, https://doi.org/10.5194/amt-14-1205-2021, https://doi.org/10.5194/amt-14-1205-2021, 2021
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Solar and infrared radiation are measured regularly for research, industry, and climate monitoring. In cold climates, icing of sensors is a poorly constrained source of uncertainty. D-ICE was carried out in Alaska to document the effectiveness of ice-mitigation technology and quantify errors associated with ice. Technology was more effective than anticipated, and while instantaneous errors were large, mean biases were small. Attributes of effective ice mitigation design were identified.
Ottmar Möhler, Michael Adams, Larissa Lacher, Franziska Vogel, Jens Nadolny, Romy Ullrich, Cristian Boffo, Tatjana Pfeuffer, Achim Hobl, Maximilian Weiß, Hemanth S. K. Vepuri, Naruki Hiranuma, and Benjamin J. Murray
Atmos. Meas. Tech., 14, 1143–1166, https://doi.org/10.5194/amt-14-1143-2021, https://doi.org/10.5194/amt-14-1143-2021, 2021
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The Earth's climate is influenced by clouds, which are impacted by ice-nucleating particles (INPs), a minor fraction of atmospheric aerosols. INPs induce ice formation in clouds and thus often initiate precipitation formation. The Portable Ice Nucleation Experiment (PINE) is the first fully automated instrument to study cloud ice formation and to obtain long-term records of INPs. This is a timely development, and the capabilities it offers for research and atmospheric monitoring are significant.
Jean-Luc Baray, Laurent Deguillaume, Aurélie Colomb, Karine Sellegri, Evelyn Freney, Clémence Rose, Joël Van Baelen, Jean-Marc Pichon, David Picard, Patrick Fréville, Laëtitia Bouvier, Mickaël Ribeiro, Pierre Amato, Sandra Banson, Angelica Bianco, Agnès Borbon, Lauréline Bourcier, Yannick Bras, Marcello Brigante, Philippe Cacault, Aurélien Chauvigné, Tiffany Charbouillot, Nadine Chaumerliac, Anne-Marie Delort, Marc Delmotte, Régis Dupuy, Antoine Farah, Guy Febvre, Andrea Flossmann, Christophe Gourbeyre, Claude Hervier, Maxime Hervo, Nathalie Huret, Muriel Joly, Victor Kazan, Morgan Lopez, Gilles Mailhot, Angela Marinoni, Olivier Masson, Nadège Montoux, Marius Parazols, Frédéric Peyrin, Yves Pointin, Michel Ramonet, Manon Rocco, Martine Sancelme, Stéphane Sauvage, Martina Schmidt, Emmanuel Tison, Mickaël Vaïtilingom, Paolo Villani, Miao Wang, Camille Yver-Kwok, and Paolo Laj
Atmos. Meas. Tech., 13, 3413–3445, https://doi.org/10.5194/amt-13-3413-2020, https://doi.org/10.5194/amt-13-3413-2020, 2020
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CO-PDD (Cézeaux-Aulnat-Opme-puy de Dôme) is a fully instrumented platform for atmospheric research. The four sites located at different altitudes from 330 to 1465 m around Clermont-Ferrand (France) host in situ and remote sensing instruments to measure atmospheric composition, including long-term trends and variability, to study interconnected processes (microphysical, chemical, biological, chemical, and dynamical) and to provide a reference point for climate models.
Fabiola Ramelli, Alexander Beck, Jan Henneberger, and Ulrike Lohmann
Atmos. Meas. Tech., 13, 925–939, https://doi.org/10.5194/amt-13-925-2020, https://doi.org/10.5194/amt-13-925-2020, 2020
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Boundary layer clouds are influenced by many physical and dynamical processes, making accurate forecasting difficult. Here we present a new measurement platform on a tethered balloon to measure cloud microphysical and meteorological profiles. The unique combination of holography and balloon-borne observations allows high-resolution measurements in a well-defined volume. Field measurements in stratus clouds over the Swiss Plateau revealed unique microphysical signatures in the cloud structure.
Darielle Dexheimer, Martin Airey, Erika Roesler, Casey Longbottom, Keri Nicoll, Stefan Kneifel, Fan Mei, R. Giles Harrison, Graeme Marlton, and Paul D. Williams
Atmos. Meas. Tech., 12, 6845–6864, https://doi.org/10.5194/amt-12-6845-2019, https://doi.org/10.5194/amt-12-6845-2019, 2019
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A tethered-balloon system deployed supercooled liquid water content sondes and fiber optic distributed temperature sensing to collect in situ atmospheric measurements within mixed-phase Arctic clouds. These data were validated against collocated surface-based and remote sensing datasets. From these measurements and sensor evaluations, tethered-balloon flights are shown to offer an effective method of collecting data to inform numerical models and calibrate remote sensing instrumentation.
Sebastian J. O'Shea, Jonathan Crosier, James Dorsey, Waldemar Schledewitz, Ian Crawford, Stephan Borrmann, Richard Cotton, and Aaron Bansemer
Atmos. Meas. Tech., 12, 3067–3079, https://doi.org/10.5194/amt-12-3067-2019, https://doi.org/10.5194/amt-12-3067-2019, 2019
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Optical array probe measurements of clouds are widely used to inform and validate numerical weather and climate models. In this paper, we discuss artefacts which may bias data from these instruments. Using laboratory and synthetic datasets, we demonstrate how greyscale analysis can be used to filter data, constraining the sample volume and improving data quality particularly at small sizes where their measurements are considered unreliable.
Christine Aebi, Julian Gröbner, and Niklaus Kämpfer
Atmos. Meas. Tech., 11, 5549–5563, https://doi.org/10.5194/amt-11-5549-2018, https://doi.org/10.5194/amt-11-5549-2018, 2018
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A newly developed hemispherical thermal infrared cloud camera (IRCCAM) is presented. The IRCCAM allows automatic cloud detection during the day and at night-time. The cloud fraction determined from the IRCCAM is compared with the cloud fraction determined from other instruments over a time period of 2 years. The IRCCAM has an agreement of +/- 2 oktas cloud fraction in 90 % of the data compared to other instruments. There are no significant differences between seasons or different times of day.
Ewan Crosbie, Matthew D. Brown, Michael Shook, Luke Ziemba, Richard H. Moore, Taylor Shingler, Edward Winstead, K. Lee Thornhill, Claire Robinson, Alexander B. MacDonald, Hossein Dadashazar, Armin Sorooshian, Andreas Beyersdorf, Alexis Eugene, Jeffrey Collett Jr., Derek Straub, and Bruce Anderson
Atmos. Meas. Tech., 11, 5025–5048, https://doi.org/10.5194/amt-11-5025-2018, https://doi.org/10.5194/amt-11-5025-2018, 2018
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A new aircraft-mounted probe for collecting samples of cloud water has been designed, fabricated, and extensively tested. Cloud drop composition provides valuable insight into atmospheric processes, but separating liquid samples from the airstream in a controlled way at flight speeds has proven difficult. The features of the design have been analysed with detailed numerical flow simulations and the new probe has demonstrated improved efficiency and performance through extensive flight testing.
Armin Afchine, Christian Rolf, Anja Costa, Nicole Spelten, Martin Riese, Bernhard Buchholz, Volker Ebert, Romy Heller, Stefan Kaufmann, Andreas Minikin, Christiane Voigt, Martin Zöger, Jessica Smith, Paul Lawson, Alexey Lykov, Sergey Khaykin, and Martina Krämer
Atmos. Meas. Tech., 11, 4015–4031, https://doi.org/10.5194/amt-11-4015-2018, https://doi.org/10.5194/amt-11-4015-2018, 2018
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The ice water content (IWC) of cirrus clouds is an essential parameter that determines their radiative properties and is thus important for climate simulations. Experimental investigations of IWCs measured on board research aircraft reveal that their accuracy is influenced by the sampling position. IWCs detected at the aircraft roof deviate significantly from wing, side or bottom IWCs. The reasons are deflections of the gas streamlines and ice particle trajectories behind the aircraft cockpit.
Martin Schnaiter, Emma Järvinen, Ahmed Abdelmonem, and Thomas Leisner
Atmos. Meas. Tech., 11, 341–357, https://doi.org/10.5194/amt-11-341-2018, https://doi.org/10.5194/amt-11-341-2018, 2018
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PHIPS-HALO is a novel aircraft instrument for cloud research. It combines microscopic imaging of single cloud particles with the measurement of their spacial light scattering properties. The knowledge of how atmospheric ice particles in clouds scatter visible light is important for improving future climate models.
Marcus Klingebiel, André Ehrlich, Fanny Finger, Timo Röschenthaler, Suad Jakirlić, Matthias Voigt, Stefan Müller, Rolf Maser, Manfred Wendisch, Peter Hoor, Peter Spichtinger, and Stephan Borrmann
Atmos. Meas. Tech., 10, 3485–3498, https://doi.org/10.5194/amt-10-3485-2017, https://doi.org/10.5194/amt-10-3485-2017, 2017
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Microphysical and radiation measurements were collected with the unique AIRcraft TOwed Sensor Shuttle (AIRTOSS) – Learjet tandem platform. It is a combination of a Learjet 35A research aircraft and an instrumented aerodynamic bird, which can be detached from and retracted back to the aircraft during flight.
AIRTOSS and Learjet are equipped with radiative, cloud microphysical, trace gas,
and meteorological instruments to study cirrus clouds.
Alexander Beck, Jan Henneberger, Sarah Schöpfer, Jacob Fugal, and Ulrike Lohmann
Atmos. Meas. Tech., 10, 459–476, https://doi.org/10.5194/amt-10-459-2017, https://doi.org/10.5194/amt-10-459-2017, 2017
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In situ observations of cloud properties in complex alpine terrain are commonly conducted at mountain-top research stations and limited to single-point measurements. The HoloGondel platform overcomes this limitation by using a cable car to obtain vertical profiles of the microphysical and meteorological cloud parameters. In this work example measurements of the vertical profiles observed in a liquid cloud and a mixed-phase cloud at the Eggishorn in the Swiss Alps are presented.
Masatomo Fujiwara, Takuji Sugidachi, Toru Arai, Kensaku Shimizu, Mayumi Hayashi, Yasuhisa Noma, Hideaki Kawagita, Kazuo Sagara, Taro Nakagawa, Satoshi Okumura, Yoichi Inai, Takashi Shibata, Suginori Iwasaki, and Atsushi Shimizu
Atmos. Meas. Tech., 9, 5911–5931, https://doi.org/10.5194/amt-9-5911-2016, https://doi.org/10.5194/amt-9-5911-2016, 2016
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A meteorological balloon-borne cloud sensor called the cloud particle sensor (CPS) has been developed. The CPS can count the number of particles per second and can obtain the cloud phase information (i.e. liquid, ice, or mixed). Twenty-five test flights have been made between 2012 and 2015 at midlatitude and tropical sites. The results from the four flights are discussed.
Ralf Weigel, Peter Spichtinger, Christoph Mahnke, Marcus Klingebiel, Armin Afchine, Andreas Petzold, Martina Krämer, Anja Costa, Sergej Molleker, Philipp Reutter, Miklós Szakáll, Max Port, Lucas Grulich, Tina Jurkat, Andreas Minikin, and Stephan Borrmann
Atmos. Meas. Tech., 9, 5135–5162, https://doi.org/10.5194/amt-9-5135-2016, https://doi.org/10.5194/amt-9-5135-2016, 2016
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The subject of our study concerns measurements with optical array probes (OAPs) on fast-flying aircraft such as the G550 (HALO or HIAPER). At up to Mach 0.7 the effect of air compression upstream of underwing-mounted instruments and particles' inertia need consideration for determining ambient particle concentrations. Compared to conventional practices the introduced correction procedure eliminates ambiguities and exhibits consistency over flight speeds between 50 and 250 m s−.
G. Guyot, C. Gourbeyre, G. Febvre, V. Shcherbakov, F. Burnet, J.-C. Dupont, K. Sellegri, and O. Jourdan
Atmos. Meas. Tech., 8, 4347–4367, https://doi.org/10.5194/amt-8-4347-2015, https://doi.org/10.5194/amt-8-4347-2015, 2015
S. Risius, H. Xu, F. Di Lorenzo, H. Xi, H. Siebert, R. A. Shaw, and E. Bodenschatz
Atmos. Meas. Tech., 8, 3209–3218, https://doi.org/10.5194/amt-8-3209-2015, https://doi.org/10.5194/amt-8-3209-2015, 2015
H. Siebert, R. A. Shaw, J. Ditas, T. Schmeissner, S. P. Malinowski, E. Bodenschatz, and H. Xu
Atmos. Meas. Tech., 8, 3219–3228, https://doi.org/10.5194/amt-8-3219-2015, https://doi.org/10.5194/amt-8-3219-2015, 2015
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We report results from simultaneous, high-resolution and collocated measurements of cloud microphysical and turbulence properties during several warm cloud events at the Umweltforschungsstation Schneefernerhaus (UFS) on Zugspitze in the German Alps. The data gathered were found to be representative of observations made with similar instrumentation in free clouds.
D. Tátrai, Z. Bozóki, H. Smit, C. Rolf, N. Spelten, M. Krämer, A. Filges, C. Gerbig, G. Gulyás, and G. Szabó
Atmos. Meas. Tech., 8, 33–42, https://doi.org/10.5194/amt-8-33-2015, https://doi.org/10.5194/amt-8-33-2015, 2015
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Airborne hygrometry is very important in climate research, and the interest in knowing not only water vapor concentration but (cirrus) cloud content as well is increasing. The authors provide a photoacoustic spectroscopy-based dual-channel hygrometer system that can be a good solution for such measurements. The instrument was proven to operate properly from ground level up to the lower stratosphere, giving the possibility even for cirrus cloud studies.
S. J. Abel, R. J. Cotton, P. A. Barrett, and A. K. Vance
Atmos. Meas. Tech., 7, 3007–3022, https://doi.org/10.5194/amt-7-3007-2014, https://doi.org/10.5194/amt-7-3007-2014, 2014
V. Fung, J. L. Bosch, S. W. Roberts, and J. Kleissl
Atmos. Meas. Tech., 7, 1693–1700, https://doi.org/10.5194/amt-7-1693-2014, https://doi.org/10.5194/amt-7-1693-2014, 2014
K. Beswick, D. Baumgardner, M. Gallagher, A. Volz-Thomas, P. Nedelec, K.-Y. Wang, and S. Lance
Atmos. Meas. Tech., 7, 1443–1457, https://doi.org/10.5194/amt-7-1443-2014, https://doi.org/10.5194/amt-7-1443-2014, 2014
S. W. Dorsi, L. E. Kalnajs, D. W. Toohey, and L. M. Avallone
Atmos. Meas. Tech., 7, 215–223, https://doi.org/10.5194/amt-7-215-2014, https://doi.org/10.5194/amt-7-215-2014, 2014
J. Henneberger, J. P. Fugal, O. Stetzer, and U. Lohmann
Atmos. Meas. Tech., 6, 2975–2987, https://doi.org/10.5194/amt-6-2975-2013, https://doi.org/10.5194/amt-6-2975-2013, 2013
J. K. Spiegel, P. Zieger, N. Bukowiecki, E. Hammer, E. Weingartner, and W. Eugster
Atmos. Meas. Tech., 5, 2237–2260, https://doi.org/10.5194/amt-5-2237-2012, https://doi.org/10.5194/amt-5-2237-2012, 2012
O. Nyström, D. Murtagh, and V. Belitsky
Atmos. Meas. Tech., 5, 1359–1373, https://doi.org/10.5194/amt-5-1359-2012, https://doi.org/10.5194/amt-5-1359-2012, 2012
A. Abdelmonem, M. Schnaiter, P. Amsler, E. Hesse, J. Meyer, and T. Leisner
Atmos. Meas. Tech., 4, 2125–2142, https://doi.org/10.5194/amt-4-2125-2011, https://doi.org/10.5194/amt-4-2125-2011, 2011
R. P. Lawson
Atmos. Meas. Tech., 4, 1361–1381, https://doi.org/10.5194/amt-4-1361-2011, https://doi.org/10.5194/amt-4-1361-2011, 2011
S. Lance, C. A. Brock, D. Rogers, and J. A. Gordon
Atmos. Meas. Tech., 3, 1683–1706, https://doi.org/10.5194/amt-3-1683-2010, https://doi.org/10.5194/amt-3-1683-2010, 2010
U. Bundke, B. Reimann, B. Nillius, R. Jaenicke, and H. Bingemer
Atmos. Meas. Tech., 3, 263–271, https://doi.org/10.5194/amt-3-263-2010, https://doi.org/10.5194/amt-3-263-2010, 2010
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Short summary
The properties of ice crystals present in mixed-phase and ice clouds influence the radiation properties, precipitation occurrence and lifetime of these clouds. It is necessary to investigate the optical and microphysical properties of cloud particles particularly in situ, and to get correlation between these properties. To this end we have developed PHIPS-HALO to measure the optical properties and the corresponding microphysical parameters of individual cloud particles simultaneously.
The properties of ice crystals present in mixed-phase and ice clouds influence the radiation...
