Articles | Volume 11, issue 6
https://doi.org/10.5194/amt-11-3339-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-11-3339-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
A full-mission data set of H2O and HDO columns from SCIAMACHY 2.3 µm reflectance measurements
Andreas Schneider
CORRESPONDING AUTHOR
Earth science group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands
Tobias Borsdorff
Earth science group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands
Joost aan de Brugh
Earth science group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands
Haili Hu
Earth science group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands
Jochen Landgraf
Earth science group, SRON Netherlands Institute for Space Research, Utrecht, the Netherlands
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Atmos. Meas. Tech., 15, 297–320, https://doi.org/10.5194/amt-15-297-2022, https://doi.org/10.5194/amt-15-297-2022, 2022
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Atmos. Meas. Tech., 14, 1993–2011, https://doi.org/10.5194/amt-14-1993-2021, https://doi.org/10.5194/amt-14-1993-2021, 2021
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Alba Lorente, Tobias Borsdorff, Andre Butz, Otto Hasekamp, Joost aan de Brugh, Andreas Schneider, Lianghai Wu, Frank Hase, Rigel Kivi, Debra Wunch, David F. Pollard, Kei Shiomi, Nicholas M. Deutscher, Voltaire A. Velazco, Coleen M. Roehl, Paul O. Wennberg, Thorsten Warneke, and Jochen Landgraf
Atmos. Meas. Tech., 14, 665–684, https://doi.org/10.5194/amt-14-665-2021, https://doi.org/10.5194/amt-14-665-2021, 2021
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TROPOMI aboard Sentinel-5P satellite provides methane (CH4) measurements with exceptional temporal and spatial resolution. The study describes a series of improvements developed to retrieve CH4 from TROPOMI. The updated CH4 product features (among others) a more accurate a posteriori correction derived independently of any reference data. The validation of the improved data product shows good agreement with ground-based and satellite measurements, which highlights the quality of the TROPOMI CH4.
Andreas Schneider, Tobias Borsdorff, Joost aan de Brugh, Franziska Aemisegger, Dietrich G. Feist, Rigel Kivi, Frank Hase, Matthias Schneider, and Jochen Landgraf
Atmos. Meas. Tech., 13, 85–100, https://doi.org/10.5194/amt-13-85-2020, https://doi.org/10.5194/amt-13-85-2020, 2020
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This paper presents a new H2O/HDO data set from TROPOMI short-wave infrared measurements. It is validated against recent ground-based FTIR measurements from the TCCON network. A bias in TCCON HDO (which is not verified) is corrected by fitting a correction factor for the HDO column to match MUSICA δD for common observations. The use of the new TROPOMI data set is demonstrated using a case study of a blocking anticyclone over Europe in July 2018.
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Atmos. Meas. Tech., 12, 5443–5455, https://doi.org/10.5194/amt-12-5443-2019, https://doi.org/10.5194/amt-12-5443-2019, 2019
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The study presents possible improvements of the TROPOMI CO dataset, which is a primary product of ESA's Sentinel-5P mission. We discuss the use of different molecular spectroscopic databases in the CO retrieval, the induced biases between TROPOMI CO and TCCON validation measurements, and the latitudinally dependent bias between TROPOMI CO and the CAMS-IFS model. Additionally, two methods for the stripe correction of single TROPOMI CO orbits are presented.
Jens Faber, Michael Gerding, Andreas Schneider, Andreas Dörnbrack, Henrike Wilms, Johannes Wagner, and Franz-Josef Lübken
Atmos. Meas. Tech., 12, 4191–4210, https://doi.org/10.5194/amt-12-4191-2019, https://doi.org/10.5194/amt-12-4191-2019, 2019
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Atmospheric measurements on rising balloons can be compromised by the balloon's wake. The aim of this study is to provide a tool for assessing the likelihood of encountering the balloon's wake at the position of the gondola. This includes an uncertainty analysis of the calculation and a retrieval of vertical winds. We find an average wake encounter probability of 28 % for a standard radiosonde. Additionally, we evaluate the influence of wake from smaller objects on turbulence measurements.
Andreas Schneider, Johannes Wagner, Jens Faber, Michael Gerding, and Franz-Josef Lübken
Atmos. Chem. Phys., 17, 7941–7954, https://doi.org/10.5194/acp-17-7941-2017, https://doi.org/10.5194/acp-17-7941-2017, 2017
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Qiang Li, Markus Rapp, Anne Schrön, Andreas Schneider, and Gunter Stober
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Berend J. Schuit, Joannes D. Maasakkers, Pieter Bijl, Gourav Mahapatra, Anne-Wil van den Berg, Sudhanshu Pandey, Alba Lorente, Tobias Borsdorff, Sander Houweling, Daniel J. Varon, Jason McKeever, Dylan Jervis, Marianne Girard, Itziar Irakulis-Loitxate, Javier Gorroño, Luis Guanter, Daniel H. Cusworth, and Ilse Aben
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Manu Goudar, Juliëtte C. S. Anema, Rajesh Kumar, Tobias Borsdorff, and Jochen Landgraf
Geosci. Model Dev., 16, 4835–4852, https://doi.org/10.5194/gmd-16-4835-2023, https://doi.org/10.5194/gmd-16-4835-2023, 2023
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A framework was developed to automatically detect plumes and compute emission estimates with cross-sectional flux method (CFM) for biomass burning events in TROPOMI CO datasets using Visible Infrared Imaging Radiometer Suite active fire data. The emissions were more reliable when changing plume height in downwind direction was used instead of constant injection height. The CFM had uncertainty even when the meteorological conditions were accurate; thus there is a need for better inversion models.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, and Ilse Aben
Atmos. Chem. Phys., 23, 8899–8919, https://doi.org/10.5194/acp-23-8899-2023, https://doi.org/10.5194/acp-23-8899-2023, 2023
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Daniel J. Varon, Daniel J. Jacob, Benjamin Hmiel, Ritesh Gautam, David R. Lyon, Mark Omara, Melissa Sulprizio, Lu Shen, Drew Pendergrass, Hannah Nesser, Zhen Qu, Zachary R. Barkley, Natasha L. Miles, Scott J. Richardson, Kenneth J. Davis, Sudhanshu Pandey, Xiao Lu, Alba Lorente, Tobias Borsdorff, Joannes D. Maasakkers, and Ilse Aben
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Tobias Borsdorff, Teresa Campos, Natalie Kille, Kyle J. Zarzana, Rainer Volkamer, and Jochen Landgraf
Atmos. Meas. Tech., 16, 3027–3038, https://doi.org/10.5194/amt-16-3027-2023, https://doi.org/10.5194/amt-16-3027-2023, 2023
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ECMWF plans to assimilate TROPOMI CO with their CAMS-IFS model. This will constrain the total column and the vertical CO distribution of the model. To show this, we combine individual TROPOMI CO column retrievals with different vertical sensitivities and obtain a vertical CO concentration profile. We test the approach on three CO pollution events in comparison with CAMS-IFS simulations that do not assimilate TROPOMI CO data and in situ airborne measurements of the BB-FLUX campaign.
Anna Agustí-Panareda, Jérôme Barré, Sébastien Massart, Antje Inness, Ilse Aben, Melanie Ades, Bianca C. Baier, Gianpaolo Balsamo, Tobias Borsdorff, Nicolas Bousserez, Souhail Boussetta, Michael Buchwitz, Luca Cantarello, Cyril Crevoisier, Richard Engelen, Henk Eskes, Johannes Flemming, Sébastien Garrigues, Otto Hasekamp, Vincent Huijnen, Luke Jones, Zak Kipling, Bavo Langerock, Joe McNorton, Nicolas Meilhac, Stefan Noël, Mark Parrington, Vincent-Henri Peuch, Michel Ramonet, Miha Razinger, Maximilian Reuter, Roberto Ribas, Martin Suttie, Colm Sweeney, Jérôme Tarniewicz, and Lianghai Wu
Atmos. Chem. Phys., 23, 3829–3859, https://doi.org/10.5194/acp-23-3829-2023, https://doi.org/10.5194/acp-23-3829-2023, 2023
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Alba Lorente, Tobias Borsdorff, Mari C. Martinez-Velarte, and Jochen Landgraf
Atmos. Meas. Tech., 16, 1597–1608, https://doi.org/10.5194/amt-16-1597-2023, https://doi.org/10.5194/amt-16-1597-2023, 2023
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In the TROPOMI methane data, there are few false methane anomalies that can be misinterpreted as enhancements caused by strong emission sources. These artefacts are caused by features of the underlying surfaces that are not well characterized in the retrieval algorithm. Here we improve the representation of the surface reflectance dependency with wavelength in the forward model, removing the artificial localized CH4 enhancements found in several locations like Siberia, Australia and Algeria.
Adriana Bailey, Franziska Aemisegger, Leonie Villiger, Sebastian A. Los, Gilles Reverdin, Estefanía Quiñones Meléndez, Claudia Acquistapace, Dariusz B. Baranowski, Tobias Böck, Sandrine Bony, Tobias Bordsdorff, Derek Coffman, Simon P. de Szoeke, Christopher J. Diekmann, Marina Dütsch, Benjamin Ertl, Joseph Galewsky, Dean Henze, Przemyslaw Makuch, David Noone, Patricia K. Quinn, Michael Rösch, Andreas Schneider, Matthias Schneider, Sabrina Speich, Bjorn Stevens, and Elizabeth J. Thompson
Earth Syst. Sci. Data, 15, 465–495, https://doi.org/10.5194/essd-15-465-2023, https://doi.org/10.5194/essd-15-465-2023, 2023
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One of the novel ways EUREC4A set out to investigate trade wind clouds and their coupling to the large-scale circulation was through an extensive network of isotopic measurements in water vapor, precipitation, and seawater. Samples were taken from the island of Barbados, from aboard two aircraft, and from aboard four ships. This paper describes the full collection of EUREC4A isotopic in situ data and guides readers to complementary remotely sensed water vapor isotope ratios.
Alba Lorente, Tobias Borsdorff, Mari C. Martinez-Velarte, Andre Butz, Otto P. Hasekamp, Lianghai Wu, and Jochen Landgraf
Atmos. Meas. Tech., 15, 6585–6603, https://doi.org/10.5194/amt-15-6585-2022, https://doi.org/10.5194/amt-15-6585-2022, 2022
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The TROPOspheric Monitoring Instrument (TROPOMI) performs observations over ocean in every orbit, enhancing the monitoring capabilities of methane from space. In the sun glint geometry the mirror-like reflection at the water surface provides a signal that is high enough to retrieve methane with high accuracy and precision. We present 4 years of methane concentrations over the ocean, and we assess its quality. We also show the importance of ocean observations to quantify total CH4 emissions.
Antje Inness, Ilse Aben, Melanie Ades, Tobias Borsdorff, Johannes Flemming, Luke Jones, Jochen Landgraf, Bavo Langerock, Philippe Nedelec, Mark Parrington, and Roberto Ribas
Atmos. Chem. Phys., 22, 14355–14376, https://doi.org/10.5194/acp-22-14355-2022, https://doi.org/10.5194/acp-22-14355-2022, 2022
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The Copernicus Atmosphere Monitoring Service (CAMS) provides daily global air quality forecasts to users worldwide. One of the species of interest is carbon monoxide (CO), an important trace gas in the atmosphere with anthropogenic and natural sources, produced by incomplete combustion, for example, by wildfires. This paper looks at how well CAMS can model CO in the atmosphere and shows that the fields can be improved when blending CO data from the TROPOMI instrument with the CAMS model.
Sara Martínez-Alonso, Merritt N. Deeter, Bianca C. Baier, Kathryn McKain, Helen Worden, Tobias Borsdorff, Colm Sweeney, and Ilse Aben
Atmos. Meas. Tech., 15, 4751–4765, https://doi.org/10.5194/amt-15-4751-2022, https://doi.org/10.5194/amt-15-4751-2022, 2022
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AirCore is a novel balloon sampling system that can measure, among others, vertical profiles of carbon monoxide (CO) from 25–30 km of altitude to near the surface. Our analyses of AirCore and satellite CO data show that AirCore profiles are suited for satellite data validation, the use of shorter aircraft vertical profiles in satellite validation results in small errors (1–3 percent points) mostly at 300 hPa and above, and the error introduced by clouds in TROPOMI land data is small (1–2 %).
Pieternel F. Levelt, Deborah C. Stein Zweers, Ilse Aben, Maite Bauwens, Tobias Borsdorff, Isabelle De Smedt, Henk J. Eskes, Christophe Lerot, Diego G. Loyola, Fabian Romahn, Trissevgeni Stavrakou, Nicolas Theys, Michel Van Roozendael, J. Pepijn Veefkind, and Tijl Verhoelst
Atmos. Chem. Phys., 22, 10319–10351, https://doi.org/10.5194/acp-22-10319-2022, https://doi.org/10.5194/acp-22-10319-2022, 2022
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Using the COVID-19 lockdown periods as an example, we show how Sentinel-5P/TROPOMI trace gas data (NO2, SO2, CO, HCHO and CHOCHO) can be used to understand impacts on air quality for regions and cities around the globe. We also provide information for both experienced and inexperienced users about how we created the data using state-of-the-art algorithms, where to get the data, methods taking meteorological and seasonal variability into consideration, and insights for future studies.
Matthias Schneider, Benjamin Ertl, Qiansi Tu, Christopher J. Diekmann, Farahnaz Khosrawi, Amelie N. Röhling, Frank Hase, Darko Dubravica, Omaira E. García, Eliezer Sepúlveda, Tobias Borsdorff, Jochen Landgraf, Alba Lorente, André Butz, Huilin Chen, Rigel Kivi, Thomas Laemmel, Michel Ramonet, Cyril Crevoisier, Jérome Pernin, Martin Steinbacher, Frank Meinhardt, Kimberly Strong, Debra Wunch, Thorsten Warneke, Coleen Roehl, Paul O. Wennberg, Isamu Morino, Laura T. Iraci, Kei Shiomi, Nicholas M. Deutscher, David W. T. Griffith, Voltaire A. Velazco, and David F. Pollard
Atmos. Meas. Tech., 15, 4339–4371, https://doi.org/10.5194/amt-15-4339-2022, https://doi.org/10.5194/amt-15-4339-2022, 2022
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We present a computationally very efficient method for the synergetic use of level 2 remote-sensing data products. We apply the method to IASI vertical profile and TROPOMI total column space-borne methane observations and thus gain sensitivity for the tropospheric methane partial columns, which is not achievable by the individual use of TROPOMI and IASI. These synergetic effects are evaluated theoretically and empirically by inter-comparisons to independent references of TCCON, AirCore, and GAW.
Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, Alba Lorente, Tobias Borsdorff, John P. Burrows, Justus Notholt, and Matthias Buschmann
Atmos. Meas. Tech., 15, 4063–4074, https://doi.org/10.5194/amt-15-4063-2022, https://doi.org/10.5194/amt-15-4063-2022, 2022
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Sentinel-5P trace gas retrievals rely on elevation data in their calculations. Outdated or inaccurate data can lead to significant errors in e.g. dry-air mole fractions of methane (XCH4). We show that the use of inadequate elevation data leads to strong XCH4 anomalies in Greenland. Similar problems can be expected for other regions with inaccurate elevation data. However, we expect these to be more localized. We show that updating elevation data used in the retrieval solves this issue.
Andreas Schneider, Tobias Borsdorff, Joost aan de Brugh, Alba Lorente, Franziska Aemisegger, David Noone, Dean Henze, Rigel Kivi, and Jochen Landgraf
Atmos. Meas. Tech., 15, 2251–2275, https://doi.org/10.5194/amt-15-2251-2022, https://doi.org/10.5194/amt-15-2251-2022, 2022
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This paper presents an extended H₂O/HDO total column dataset from short-wave infrared measurements by TROPOMI including cloudy and clear-sky scenes. Coverage is tremendously increased compared to previous TROPOMI HDO datasets. The new dataset is validated against recent ground-based FTIR measurements from TCCON and against aircraft measurements over the ocean. The use of the new dataset is demonstrated with a case study of a cold air outbreak in January 2020.
Tobias Küchler, Stefan Noël, Heinrich Bovensmann, John Philip Burrows, Thomas Wagner, Christian Borger, Tobias Borsdorff, and Andreas Schneider
Atmos. Meas. Tech., 15, 297–320, https://doi.org/10.5194/amt-15-297-2022, https://doi.org/10.5194/amt-15-297-2022, 2022
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We applied the air-mass-corrected differential optical absorption spectroscopy (AMC-DOAS) method to derive total column water vapour (TCWV) from Sentinel-5P measurements and compared it to independent data sets. The correlation coefficients of typically more than 0.9 and the small deviations up to 2.5 kg m−2 reveal good agreement between our data product and other TCWV data sets. In particular for the different Sentinel-5P water vapour products, the deviations are around 1 kg m−2.
Qiansi Tu, Frank Hase, Matthias Schneider, Omaira García, Thomas Blumenstock, Tobias Borsdorff, Matthias Frey, Farahnaz Khosrawi, Alba Lorente, Carlos Alberti, Juan J. Bustos, André Butz, Virgilio Carreño, Emilio Cuevas, Roger Curcoll, Christopher J. Diekmann, Darko Dubravica, Benjamin Ertl, Carme Estruch, Sergio Fabián León-Luis, Carlos Marrero, Josep-Anton Morgui, Ramón Ramos, Christian Scharun, Carsten Schneider, Eliezer Sepúlveda, Carlos Toledano, and Carlos Torres
Atmos. Chem. Phys., 22, 295–317, https://doi.org/10.5194/acp-22-295-2022, https://doi.org/10.5194/acp-22-295-2022, 2022
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We use different methane ground- and space-based remote sensing data sets for investigating the emission strength of three waste disposal sites close to Madrid. We present a method that uses wind-assigned anomalies for deriving emission strengths from satellite data and estimate their uncertainty to 9–14 %. The emission strengths estimated from the remote sensing data sets are significantly larger than the values published in the official register.
Tyler Wizenberg, Kimberly Strong, Kaley Walker, Erik Lutsch, Tobias Borsdorff, and Jochen Landgraf
Atmos. Meas. Tech., 14, 7707–7728, https://doi.org/10.5194/amt-14-7707-2021, https://doi.org/10.5194/amt-14-7707-2021, 2021
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CO is an important atmospheric gas that influences both air quality and the climate. Here, we compare CO measurements from TROPOMI with those from ACE-FTS and an Arctic ground-based FTS at Eureka, Nunavut, to further characterize the accuracy of TROPOMI measurements. CO columns from the instruments agree well but show larger differences at high latitudes. Despite this, the results fall within the TROPOMI accuracy target, indicating good data quality at high latitudes.
Luis Guanter, Cédric Bacour, Andreas Schneider, Ilse Aben, Tim A. van Kempen, Fabienne Maignan, Christian Retscher, Philipp Köhler, Christian Frankenberg, Joanna Joiner, and Yongguang Zhang
Earth Syst. Sci. Data, 13, 5423–5440, https://doi.org/10.5194/essd-13-5423-2021, https://doi.org/10.5194/essd-13-5423-2021, 2021
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Sun-induced chlorophyll fluorescence (SIF) is an electromagnetic signal emitted by plants in the red and far-red parts of the spectrum. It has a functional link to photosynthesis and can be measured by satellite instruments, which makes it an important variable for the remote monitoring of the photosynthetic activity of vegetation ecosystems around the world. In this contribution we present a SIF dataset derived from the new Sentinel-5P TROPOMI missions.
Mahesh Kumar Sha, Bavo Langerock, Jean-François L. Blavier, Thomas Blumenstock, Tobias Borsdorff, Matthias Buschmann, Angelika Dehn, Martine De Mazière, Nicholas M. Deutscher, Dietrich G. Feist, Omaira E. García, David W. T. Griffith, Michel Grutter, James W. Hannigan, Frank Hase, Pauli Heikkinen, Christian Hermans, Laura T. Iraci, Pascal Jeseck, Nicholas Jones, Rigel Kivi, Nicolas Kumps, Jochen Landgraf, Alba Lorente, Emmanuel Mahieu, Maria V. Makarova, Johan Mellqvist, Jean-Marc Metzger, Isamu Morino, Tomoo Nagahama, Justus Notholt, Hirofumi Ohyama, Ivan Ortega, Mathias Palm, Christof Petri, David F. Pollard, Markus Rettinger, John Robinson, Sébastien Roche, Coleen M. Roehl, Amelie N. Röhling, Constantina Rousogenous, Matthias Schneider, Kei Shiomi, Dan Smale, Wolfgang Stremme, Kimberly Strong, Ralf Sussmann, Yao Té, Osamu Uchino, Voltaire A. Velazco, Corinne Vigouroux, Mihalis Vrekoussis, Pucai Wang, Thorsten Warneke, Tyler Wizenberg, Debra Wunch, Shoma Yamanouchi, Yang Yang, and Minqiang Zhou
Atmos. Meas. Tech., 14, 6249–6304, https://doi.org/10.5194/amt-14-6249-2021, https://doi.org/10.5194/amt-14-6249-2021, 2021
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This paper presents, for the first time, Sentinel-5 Precursor methane and carbon monoxide validation results covering a period from November 2017 to September 2020. For this study, we used global TCCON and NDACC-IRWG network data covering a wide range of atmospheric and surface conditions across different terrains. We also show the influence of a priori alignment, smoothing uncertainties and the sensitivity of the validation results towards the application of advanced co-location criteria.
Michael Buchwitz, Maximilian Reuter, Stefan Noël, Klaus Bramstedt, Oliver Schneising, Michael Hilker, Blanca Fuentes Andrade, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hartmut Boesch, Lianghai Wu, Jochen Landgraf, Ilse Aben, Christian Retscher, Christopher W. O'Dell, and David Crisp
Atmos. Meas. Tech., 14, 2141–2166, https://doi.org/10.5194/amt-14-2141-2021, https://doi.org/10.5194/amt-14-2141-2021, 2021
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The COVID-19 pandemic resulted in reduced anthropogenic carbon dioxide (CO2) emissions during 2020 in large parts of the world. We have used a small ensemble of satellite retrievals of column-averaged CO2 (XCO2) to find out if a regional-scale reduction of atmospheric CO2 can be detected from space. We focus on East China and show that it is challenging to reliably detect and to accurately quantify the emission reduction, which only results in regional XCO2 reductions of about 0.1–0.2 ppm.
Qiansi Tu, Frank Hase, Thomas Blumenstock, Matthias Schneider, Andreas Schneider, Rigel Kivi, Pauli Heikkinen, Benjamin Ertl, Christopher Diekmann, Farahnaz Khosrawi, Michael Sommer, Tobias Borsdorff, and Uwe Raffalski
Atmos. Meas. Tech., 14, 1993–2011, https://doi.org/10.5194/amt-14-1993-2021, https://doi.org/10.5194/amt-14-1993-2021, 2021
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We compare column-averaged dry-air mole fractions of water vapor (XH2O) retrievals from the COllaborative Carbon Column Observing Network (COCCON) with two co-located ground-based spectrometers as references at two boreal sites. Our study supports the assumption that COCCON also delivers a well-characterized XH2O data product. This is the first published study applying COCCON for MUSICA IASI and TROPOMI validation.
Stephanie P. Rusli, Otto Hasekamp, Joost aan de Brugh, Guangliang Fu, Yasjka Meijer, and Jochen Landgraf
Atmos. Meas. Tech., 14, 1167–1190, https://doi.org/10.5194/amt-14-1167-2021, https://doi.org/10.5194/amt-14-1167-2021, 2021
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This study investigates the added value of multi-angle polarimeter (MAP) measurements for XCO2 retrievals, particularly in the context of the Copernicus Anthropogenic Carbon Dioxide Monitoring (CO2M) mission. In this paper, we derive the required MAP instrument specification, and we demonstrate that MAP observations significantly improve the retrieval performance and are needed to meet the XCO2 precision and accuracy requirements of the CO2M mission.
Marvin Knapp, Ralph Kleinschek, Frank Hase, Anna Agustí-Panareda, Antje Inness, Jérôme Barré, Jochen Landgraf, Tobias Borsdorff, Stefan Kinne, and André Butz
Earth Syst. Sci. Data, 13, 199–211, https://doi.org/10.5194/essd-13-199-2021, https://doi.org/10.5194/essd-13-199-2021, 2021
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We developed a shipborne variant of a remote sensing spectrometer for direct sunlight measurements of column-averaged atmospheric mixing ratios of carbon dioxide, methane, and carbon monoxide. The instrument was deployed on the research vessel Sonne during a longitudinal transect over the Pacific during June 2019. The campaign yielded more than 32 000 observations which compare excellently to atmospheric composition data from a state-of-the-art model (CAMS) and satellite observations (TROPOMI).
Alba Lorente, Tobias Borsdorff, Andre Butz, Otto Hasekamp, Joost aan de Brugh, Andreas Schneider, Lianghai Wu, Frank Hase, Rigel Kivi, Debra Wunch, David F. Pollard, Kei Shiomi, Nicholas M. Deutscher, Voltaire A. Velazco, Coleen M. Roehl, Paul O. Wennberg, Thorsten Warneke, and Jochen Landgraf
Atmos. Meas. Tech., 14, 665–684, https://doi.org/10.5194/amt-14-665-2021, https://doi.org/10.5194/amt-14-665-2021, 2021
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TROPOMI aboard Sentinel-5P satellite provides methane (CH4) measurements with exceptional temporal and spatial resolution. The study describes a series of improvements developed to retrieve CH4 from TROPOMI. The updated CH4 product features (among others) a more accurate a posteriori correction derived independently of any reference data. The validation of the improved data product shows good agreement with ground-based and satellite measurements, which highlights the quality of the TROPOMI CH4.
Sudhanshu Pandey, Sander Houweling, Alba Lorente, Tobias Borsdorff, Maria Tsivlidou, A. Anthony Bloom, Benjamin Poulter, Zhen Zhang, and Ilse Aben
Biogeosciences, 18, 557–572, https://doi.org/10.5194/bg-18-557-2021, https://doi.org/10.5194/bg-18-557-2021, 2021
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We use atmospheric methane observations from the novel TROPOspheric Monitoring Instrument (TROPOMI; Sentinel-5p) to estimate methane emissions from South Sudan's wetlands. Our emission estimates are an order of magnitude larger than the estimate of process-based wetland models. We find that this underestimation by the models is likely due to their misrepresentation of the wetlands' inundation extent and temperature dependences.
Ivar R. van der Velde, Guido R. van der Werf, Sander Houweling, Henk J. Eskes, J. Pepijn Veefkind, Tobias Borsdorff, and Ilse Aben
Atmos. Chem. Phys., 21, 597–616, https://doi.org/10.5194/acp-21-597-2021, https://doi.org/10.5194/acp-21-597-2021, 2021
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This paper compares the relative atmospheric enhancements of CO and NO2 measured by the space-based instrument TROPOMI over different fire-prone ecosystems around the world. We find distinct spatial and temporal patterns in the ΔNO2 / ΔCO ratio that correspond to regional differences in combustion efficiency. This joint analysis provides a better understanding of regional-scale combustion characteristics and can help the fire modeling community to improve existing global emission inventories.
Tobias Borsdorff, Agustín García Reynoso, Gilberto Maldonado, Bertha Mar-Morales, Wolfgang Stremme, Michel Grutter, and Jochen Landgraf
Atmos. Chem. Phys., 20, 15761–15774, https://doi.org/10.5194/acp-20-15761-2020, https://doi.org/10.5194/acp-20-15761-2020, 2020
Sara Martínez-Alonso, Merritt Deeter, Helen Worden, Tobias Borsdorff, Ilse Aben, Róisin Commane, Bruce Daube, Gene Francis, Maya George, Jochen Landgraf, Debbie Mao, Kathryn McKain, and Steven Wofsy
Atmos. Meas. Tech., 13, 4841–4864, https://doi.org/10.5194/amt-13-4841-2020, https://doi.org/10.5194/amt-13-4841-2020, 2020
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CO is of great importance in climate and air quality studies. To understand newly available TROPOMI data in the frame of the global CO record, we compared those to satellite (MOPITT) and airborne (ATom) CO datasets. The MOPITT dataset is the longest to date (2000–present) and is well-characterized. We used ATom to validate cloudy TROPOMI data over oceans and investigate TROPOMI's vertical sensitivity to CO. Our results show that TROPOMI CO data are in excellent agreement with the other datasets.
Qiansi Tu, Frank Hase, Thomas Blumenstock, Rigel Kivi, Pauli Heikkinen, Mahesh Kumar Sha, Uwe Raffalski, Jochen Landgraf, Alba Lorente, Tobias Borsdorff, Huilin Chen, Florian Dietrich, and Jia Chen
Atmos. Meas. Tech., 13, 4751–4771, https://doi.org/10.5194/amt-13-4751-2020, https://doi.org/10.5194/amt-13-4751-2020, 2020
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Two COCCON instruments are used to observe multiyear greenhouse gases in boreal areas and are compared with the CAMS analysis and S5P satellite data. These three datasets predict greenhouse gas gradients with reasonable agreement. The results indicate that the COCCON instrument has the capability of measuring gradients on regional scales, and observations performed with the portable spectrometers can contribute to inferring sources and sinks and to validating spaceborne greenhouse gases.
Srijana Lama, Sander Houweling, K. Folkert Boersma, Henk Eskes, Ilse Aben, Hugo A. C. Denier van der Gon, Maarten C. Krol, Han Dolman, Tobias Borsdorff, and Alba Lorente
Atmos. Chem. Phys., 20, 10295–10310, https://doi.org/10.5194/acp-20-10295-2020, https://doi.org/10.5194/acp-20-10295-2020, 2020
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Rapid urbanization has increased the consumption of fossil fuel, contributing the degradation of urban air quality. Burning efficiency is a major factor determining the impact of fuel burning on the environment. We quantify the burning efficiency of fossil fuel use over six megacities using satellite remote sensing data. City governance can use these results to understand air pollution scenarios and to formulate effective air pollution control strategies.
Jonas Simon Wilzewski, Anke Roiger, Johan Strandgren, Jochen Landgraf, Dietrich G. Feist, Voltaire A. Velazco, Nicholas M. Deutscher, Isamu Morino, Hirofumi Ohyama, Yao Té, Rigel Kivi, Thorsten Warneke, Justus Notholt, Manvendra Dubey, Ralf Sussmann, Markus Rettinger, Frank Hase, Kei Shiomi, and André Butz
Atmos. Meas. Tech., 13, 731–745, https://doi.org/10.5194/amt-13-731-2020, https://doi.org/10.5194/amt-13-731-2020, 2020
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Through spectral degradation of GOSAT measurements in the 1.6 and 2.0 μm spectral bands, we mimic a single-band, passive satellite sensor for monitoring of CO2 emissions at fine spatial scales. We compare retrievals of XCO2 from these bands to TCCON and native GOSAT retrievals. At spectral resolutions near 1.3 nm, XCO2 retrievals from both bands show promising performance, but the 2.0 μm band is favorable due to better noise performance and the potential to retrieve some aerosol information.
Lianghai Wu, Joost aan de Brugh, Yasjka Meijer, Bernd Sierk, Otto Hasekamp, Andre Butz, and Jochen Landgraf
Atmos. Meas. Tech., 13, 713–729, https://doi.org/10.5194/amt-13-713-2020, https://doi.org/10.5194/amt-13-713-2020, 2020
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The future European CO2 monitoring constellation is targeting a moderate spectral resolution of 0.1, 0.3, and 0.3–0.55 nm in the spectral bands of 0.76, 1.61, and 2.06 μm. To assess this choice, we perform XCO2 retrievals using both satellite (OCO-2 and GOSAT) and synthetic observations, which we spectrally degrade to the target spectral resolution. We see that moderate spectral resolution mainly reduces XCO2 precision and has little effect on the the systematic error.
Andreas Schneider, Tobias Borsdorff, Joost aan de Brugh, Franziska Aemisegger, Dietrich G. Feist, Rigel Kivi, Frank Hase, Matthias Schneider, and Jochen Landgraf
Atmos. Meas. Tech., 13, 85–100, https://doi.org/10.5194/amt-13-85-2020, https://doi.org/10.5194/amt-13-85-2020, 2020
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This paper presents a new H2O/HDO data set from TROPOMI short-wave infrared measurements. It is validated against recent ground-based FTIR measurements from the TCCON network. A bias in TCCON HDO (which is not verified) is corrected by fitting a correction factor for the HDO column to match MUSICA δD for common observations. The use of the new TROPOMI data set is demonstrated using a case study of a blocking anticyclone over Europe in July 2018.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, John P. Burrows, Tobias Borsdorff, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Christian Hermans, Laura T. Iraci, Rigel Kivi, Jochen Landgraf, Isamu Morino, Justus Notholt, Christof Petri, David F. Pollard, Sébastien Roche, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Voltaire A. Velazco, Thorsten Warneke, and Debra Wunch
Atmos. Meas. Tech., 12, 6771–6802, https://doi.org/10.5194/amt-12-6771-2019, https://doi.org/10.5194/amt-12-6771-2019, 2019
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We introduce an algorithm that is used to simultaneously derive the abundances of the important atmospheric constituents carbon monoxide and methane from the TROPOMI instrument onboard the Sentinel-5 Precursor satellite, which enables the determination of both gases with an unprecedented level of detail on a global scale. The quality of the resulting data sets is assessed and the first results are presented.
Edward Malina, Haili Hu, Jochen Landgraf, and Ben Veihelmann
Atmos. Meas. Tech., 12, 6273–6301, https://doi.org/10.5194/amt-12-6273-2019, https://doi.org/10.5194/amt-12-6273-2019, 2019
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We present a feasibility study on retrieving 12CH4 and 13CH4 using the recently launched TROPOMI on the Copernicus Sentinel 5P satellite and the future UVNS instrument on Sentinel 5. The ratio of 12CH4 and 13CH4 can be used to calculate the δ13C value, which has been shown to be able to distinguish between biological and non-biological sources of methane. We show that Sentinel 5/UVNS may be used to distinguish between methane source types, while Sentinel 5P/TROPOMI is subject to large biases.
Lianghai Wu, Otto Hasekamp, Haili Hu, Joost aan de Brugh, Jochen Landgraf, Andre Butz, and Ilse Aben
Atmos. Meas. Tech., 12, 6049–6058, https://doi.org/10.5194/amt-12-6049-2019, https://doi.org/10.5194/amt-12-6049-2019, 2019
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We propose a one–band XCO2 retrieval technique which uses only the 2.06 µm band measurements from the Orbiting Carbon Observatory–2 (OCO–2) satellite. Compared to the current state–of–the–art three–band retrievals, XCO2 retrievals using only the 2.06 µm band have similar retrieval accuracy, precision, and data yield. For future missions it may be better to replace the O2 A band with measurements that have larger information content on aerosols, like a multi–angle polarimeter (MAP).
Tobias Borsdorff, Joost aan de Brugh, Andreas Schneider, Alba Lorente, Manfred Birk, Georg Wagner, Rigel Kivi, Frank Hase, Dietrich G. Feist, Ralf Sussmann, Markus Rettinger, Debra Wunch, Thorsten Warneke, and Jochen Landgraf
Atmos. Meas. Tech., 12, 5443–5455, https://doi.org/10.5194/amt-12-5443-2019, https://doi.org/10.5194/amt-12-5443-2019, 2019
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The study presents possible improvements of the TROPOMI CO dataset, which is a primary product of ESA's Sentinel-5P mission. We discuss the use of different molecular spectroscopic databases in the CO retrieval, the induced biases between TROPOMI CO and TCCON validation measurements, and the latitudinally dependent bias between TROPOMI CO and the CAMS-IFS model. Additionally, two methods for the stripe correction of single TROPOMI CO orbits are presented.
Jens Faber, Michael Gerding, Andreas Schneider, Andreas Dörnbrack, Henrike Wilms, Johannes Wagner, and Franz-Josef Lübken
Atmos. Meas. Tech., 12, 4191–4210, https://doi.org/10.5194/amt-12-4191-2019, https://doi.org/10.5194/amt-12-4191-2019, 2019
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Atmospheric measurements on rising balloons can be compromised by the balloon's wake. The aim of this study is to provide a tool for assessing the likelihood of encountering the balloon's wake at the position of the gondola. This includes an uncertainty analysis of the calculation and a retrieval of vertical winds. We find an average wake encounter probability of 28 % for a standard radiosonde. Additionally, we evaluate the influence of wake from smaller objects on turbulence measurements.
Tobias Borsdorff, Joost aan de Brugh, Sudhanshu Pandey, Otto Hasekamp, Ilse Aben, Sander Houweling, and Jochen Landgraf
Atmos. Chem. Phys., 19, 3579–3588, https://doi.org/10.5194/acp-19-3579-2019, https://doi.org/10.5194/acp-19-3579-2019, 2019
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The Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor satellite provides carbon monoxide (CO) total column concentrations based on measurements in the 2.3 μm spectral range with a spatial resolution of 7 km x 7 km and daily global coverage. In this study, we analyzed local CO enhancements in an area around Iran from 1 November to 20 December 2017 using the WRF model and evaluated CO emissions from the cities of Tehran, Yerevan, Urmia, and Tabriz.
Iris N. Dekker, Sander Houweling, Sudhanshu Pandey, Maarten Krol, Thomas Röckmann, Tobias Borsdorff, Jochen Landgraf, and Ilse Aben
Atmos. Chem. Phys., 19, 3433–3445, https://doi.org/10.5194/acp-19-3433-2019, https://doi.org/10.5194/acp-19-3433-2019, 2019
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During November 2017, very high pollution levels were measured in the northern part of India. In this study, satellite (TROPOMI) data and model (WRF) data on carbon monoxide (CO) are studied to investigate the main sources of the CO pollution over the Indo-Gangetic Plain. We found that residential and commercial combustion was a much more important source of CO than the post-monsoon crop burning during this period. Meteorology was found important in the accumulation and ventilation of CO.
Tobias Borsdorff, Joost aan de Brugh, Haili Hu, Otto Hasekamp, Ralf Sussmann, Markus Rettinger, Frank Hase, Jochen Gross, Matthias Schneider, Omaira Garcia, Wolfgang Stremme, Michel Grutter, Dietrich G. Feist, Sabrina G. Arnold, Martine De Mazière, Mahesh Kumar Sha, David F. Pollard, Matthäus Kiel, Coleen Roehl, Paul O. Wennberg, Geoffrey C. Toon, and Jochen Landgraf
Atmos. Meas. Tech., 11, 5507–5518, https://doi.org/10.5194/amt-11-5507-2018, https://doi.org/10.5194/amt-11-5507-2018, 2018
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On 13 October 2017, the S5-P satellite was launched with TROPOMI as its only payload. One of the primary products is atmospheric CO observed with daily global coverage and spatial resolution of 7 × 7 km2. The new dataset allows the sensing of CO enhancements above cities and industrial areas and can track pollution transport from biomass burning regions. Through validation with ground-based TCCON measurements we show that the CO data product is already well within the mission requirement.
Arno de Lange and Jochen Landgraf
Atmos. Meas. Tech., 11, 3815–3828, https://doi.org/10.5194/amt-11-3815-2018, https://doi.org/10.5194/amt-11-3815-2018, 2018
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Atmospheric methane abundances as function of altitude derived from the thermal infrared band of the Japanese GOSAT satellite show a systematic bias. It has been shown that simple correction schemes can lead to undesired consequences. This paper discusses a more elaborate approach, resulting in methane profiles that fall within 2 % of independent reference measurements and models. This is true for different scenes around the globe and over the full altitude range.
Lianghai Wu, Otto Hasekamp, Haili Hu, Jochen Landgraf, Andre Butz, Joost aan de Brugh, Ilse Aben, Dave F. Pollard, David W. T. Griffith, Dietrich G. Feist, Dmitry Koshelev, Frank Hase, Geoffrey C. Toon, Hirofumi Ohyama, Isamu Morino, Justus Notholt, Kei Shiomi, Laura Iraci, Matthias Schneider, Martine de Mazière, Ralf Sussmann, Rigel Kivi, Thorsten Warneke, Tae-Young Goo, and Yao Té
Atmos. Meas. Tech., 11, 3111–3130, https://doi.org/10.5194/amt-11-3111-2018, https://doi.org/10.5194/amt-11-3111-2018, 2018
Tobias Borsdorff, Josip Andrasec, Joost aan de Brugh, Haili Hu, Ilse Aben, and Jochen Landgraf
Atmos. Meas. Tech., 11, 2553–2565, https://doi.org/10.5194/amt-11-2553-2018, https://doi.org/10.5194/amt-11-2553-2018, 2018
Andreas Schneider, Johannes Wagner, Jens Faber, Michael Gerding, and Franz-Josef Lübken
Atmos. Chem. Phys., 17, 7941–7954, https://doi.org/10.5194/acp-17-7941-2017, https://doi.org/10.5194/acp-17-7941-2017, 2017
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Wave breaking is studied with a combination of high-resolution turbulence observations with the balloon-borne instrument LITOS and mesoscale simulations with the WRF model. A relation between observed turbulent energy dissipation rates and the occurrence of wave patterns in modelled vertical winds is found, which is interpreted as the effect of wave saturation. The change of stability plays less of a role for mean dissipation for the flights examined.
Tobias Borsdorff, Joost aan de Brugh, Haili Hu, Philippe Nédélec, Ilse Aben, and Jochen Landgraf
Atmos. Meas. Tech., 10, 1769–1782, https://doi.org/10.5194/amt-10-1769-2017, https://doi.org/10.5194/amt-10-1769-2017, 2017
Qiang Li, Markus Rapp, Anne Schrön, Andreas Schneider, and Gunter Stober
Ann. Geophys., 34, 1209–1229, https://doi.org/10.5194/angeo-34-1209-2016, https://doi.org/10.5194/angeo-34-1209-2016, 2016
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Turbulence is an essential process in the atmosphere and ocean. Clear-air turbulence is a well-known threat for the safety of aviation. Using a powerful MST radar, we detected turbulence and compared it with the results from radiosondes. The correlation between turbulence and background conditions, e.g., Richardson number and wind shears, is determined. There is a nearly negative correlation between turbulence and Richardson number independent of the length scale over which it was calculated.
Haili Hu, Otto Hasekamp, André Butz, André Galli, Jochen Landgraf, Joost Aan de Brugh, Tobias Borsdorff, Remco Scheepmaker, and Ilse Aben
Atmos. Meas. Tech., 9, 5423–5440, https://doi.org/10.5194/amt-9-5423-2016, https://doi.org/10.5194/amt-9-5423-2016, 2016
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In 2017, the TROPOMI spectrometer will be launched on board the Sentinel 5 Precursor satellite. It will deliver, among other things, daily global measurements of methane as part of the Copernicus atmospheric services.
In this paper, we present the algorithm that is used for operational data processing of the methane product from TROPOMI measurements of the shortwave and near-infrared spectral range, and we discuss its performance using realistic simulated measurements.
Jochen Landgraf, Joost aan de Brugh, Remco Scheepmaker, Tobias Borsdorff, Haili Hu, Sander Houweling, Andre Butz, Ilse Aben, and Otto Hasekamp
Atmos. Meas. Tech., 9, 4955–4975, https://doi.org/10.5194/amt-9-4955-2016, https://doi.org/10.5194/amt-9-4955-2016, 2016
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In 2016, the Sentinel 5 Precursor mission will be launched, with the TROPOMI instrument as its single payload. It will deliver daily global measurements of carbon monoxide for air quality monitoring as part of the Copernicus atmospheric services. In this paper, we focus on the operational data processing of the CO product from TROPOMI measurements of the shortwave infrared spectral range, and we discuss the algorithm's maturity.
Remco A. Scheepmaker, Joost aan de Brugh, Haili Hu, Tobias Borsdorff, Christian Frankenberg, Camille Risi, Otto Hasekamp, Ilse Aben, and Jochen Landgraf
Atmos. Meas. Tech., 9, 3921–3937, https://doi.org/10.5194/amt-9-3921-2016, https://doi.org/10.5194/amt-9-3921-2016, 2016
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We have developed an algorithm to measure HDO (heavy water) in the atmosphere using the TROPOMI satellite instrument, scheduled for launch in 2016. Giving an insight in the history of water vapour, these measurements will help to better understand the water cycle and its role in climate change. We use realistic measurement simulations to describe the performance of the algorithm, and show that TROPOMI will greatly improve and extend the HDO datasets from the previous SCIAMACHY and GOSAT missions.
Dejian Fu, Kevin W. Bowman, Helen M. Worden, Vijay Natraj, John R. Worden, Shanshan Yu, Pepijn Veefkind, Ilse Aben, Jochen Landgraf, Larrabee Strow, and Yong Han
Atmos. Meas. Tech., 9, 2567–2579, https://doi.org/10.5194/amt-9-2567-2016, https://doi.org/10.5194/amt-9-2567-2016, 2016
T. Borsdorff, P. Tol, J. E. Williams, J. de Laat, J. aan de Brugh, P. Nédélec, I. Aben, and J. Landgraf
Atmos. Meas. Tech., 9, 227–248, https://doi.org/10.5194/amt-9-227-2016, https://doi.org/10.5194/amt-9-227-2016, 2016
A. Butz, J. Orphal, R. Checa-Garcia, F. Friedl-Vallon, T. von Clarmann, H. Bovensmann, O. Hasekamp, J. Landgraf, T. Knigge, D. Weise, O. Sqalli-Houssini, and D. Kemper
Atmos. Meas. Tech., 8, 4719–4734, https://doi.org/10.5194/amt-8-4719-2015, https://doi.org/10.5194/amt-8-4719-2015, 2015
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The Geostationary Emission Explorer for Europe (G3E) is a mission concept for a greenhouse gas sounder in geostationary orbit. It is designed to provide column-average concentrations of carbon dioxide, methane, and carbon monoxide with high spatial and 2-hour temporal resolution throughout the central European continent. The prospective data density, precision and accuracy suggest G3E as a key component of a future carbon emission monitoring system.
A. Wassmann, T. Borsdorff, J. M. J. aan de Brugh, O. P. Hasekamp, I. Aben, and J. Landgraf
Atmos. Meas. Tech., 8, 4429–4451, https://doi.org/10.5194/amt-8-4429-2015, https://doi.org/10.5194/amt-8-4429-2015, 2015
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We present an extensive sensitivity study of retrieved total ozone columns from clear sky Global Ozone Monitoring Experiment 2 (GOME-2) measurements between 325 and 335nm which are corrected for instrument degradation. We address the choice of the scaling ozone profile, the choice of the radiative transfer solver, and the approximation of Earth's sphericity. Finally, we study the effect of instrument degradation on the retrieved total ozone columns for the first 4 years of the mission.
R. Checa-Garcia, J. Landgraf, A. Galli, F. Hase, V. A. Velazco, H. Tran, V. Boudon, F. Alkemade, and A. Butz
Atmos. Meas. Tech., 8, 3617–3629, https://doi.org/10.5194/amt-8-3617-2015, https://doi.org/10.5194/amt-8-3617-2015, 2015
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The future satellite missions Sentinel-5 and its precursor will monitor methane column average dry air mole fractions. The ambitious accuracy required on regional scales demands a characterization of the systematic error sources in which spectroscopic uncertainties are crucial. This study investigates how methane and water vapour spectroscopic errors propagate into retrieval errors, showing that spectroscopy-induced errors exceed 0.6% in large parts of the
world and are regionally correlated.
R. A. Scheepmaker, C. Frankenberg, N. M. Deutscher, M. Schneider, S. Barthlott, T. Blumenstock, O. E. Garcia, F. Hase, N. Jones, E. Mahieu, J. Notholt, V. Velazco, J. Landgraf, and I. Aben
Atmos. Meas. Tech., 8, 1799–1818, https://doi.org/10.5194/amt-8-1799-2015, https://doi.org/10.5194/amt-8-1799-2015, 2015
L. Guanter, I. Aben, P. Tol, J. M. Krijger, A. Hollstein, P. Köhler, A. Damm, J. Joiner, C. Frankenberg, and J. Landgraf
Atmos. Meas. Tech., 8, 1337–1352, https://doi.org/10.5194/amt-8-1337-2015, https://doi.org/10.5194/amt-8-1337-2015, 2015
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This paper investigates the potential of the upcoming TROPOspheric Monitoring Instrument (TROPOMI) instrument for the retrieval of the chlorophyll fluorescence signal emitted in the 650–850nm spectral range by the photosynthetic machinery of green plants. We find that TROPOMI will allow substantial improvements in the space monitoring of fluorescence with respect to current spaceborne instruments such as GOME-2 and SCIAMACHY.
A. Schneider, M. Gerding, and F.-J. Lübken
Atmos. Chem. Phys., 15, 2159–2166, https://doi.org/10.5194/acp-15-2159-2015, https://doi.org/10.5194/acp-15-2159-2015, 2015
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Stratospheric turbulence is essential for the atmospheric energy budget. We compare in situ observations with our LITOS method based on spectral analysis of mm-scale wind fluctuations with the Thorpe method applied to standard radiosondes. Energy dissipations rates from both methods differ by up to 3 orders of magnitude. Nevertheless, mean values are in good agreement. We present case studies on both methods and examine the applicability of the Thorpe method for calculation of dissipation rates.
R. Sander, P. Jöckel, O. Kirner, A. T. Kunert, J. Landgraf, and A. Pozzer
Geosci. Model Dev., 7, 2653–2662, https://doi.org/10.5194/gmd-7-2653-2014, https://doi.org/10.5194/gmd-7-2653-2014, 2014
A. Galli, S. Guerlet, A. Butz, I. Aben, H. Suto, A. Kuze, N. M. Deutscher, J. Notholt, D. Wunch, P. O. Wennberg, D. W. T. Griffith, O. Hasekamp, and J. Landgraf
Atmos. Meas. Tech., 7, 1105–1119, https://doi.org/10.5194/amt-7-1105-2014, https://doi.org/10.5194/amt-7-1105-2014, 2014
T. Borsdorff, O. P. Hasekamp, A. Wassmann, and J. Landgraf
Atmos. Meas. Tech., 7, 523–535, https://doi.org/10.5194/amt-7-523-2014, https://doi.org/10.5194/amt-7-523-2014, 2014
Related subject area
Subject: Gases | Technique: Remote Sensing | Topic: Data Processing and Information Retrieval
Methane retrievals from airborne HySpex observations in the shortwave infrared
Feasibility analysis of optimal terahertz (THz) bands for passive limb sounding of middle and upper atmospheric wind
Retrieval of temperature and humidity profiles from ground-based high-resolution infrared observations using an adaptive fast iterative algorithm
A retrieval of xCO2 from ground-based mid-infrared NDACC solar absorption spectra and comparison to TCCON
Optimal estimation retrieval of tropospheric ammonia from the Geostationary Interferometric Infrared Sounder on board FengYun-4B
A physically-based correction for stray light in Brewer spectrophotometer data analysis
Stratospheric-trace-gas-profile retrievals from balloon-borne limb imaging of mid-infrared emission spectra
Diurnal carbon monoxide observed from a geostationary infrared hyperspectral sounder: first result from GIIRS on board FengYun-4B
Vertical information of CO from TROPOMI total column measurements in context of the CAMS-IFS data assimilation scheme
Using a deep neural network to detect methane point sources and quantify emissions from PRISMA hyperspectral satellite images
Inferring the vertical distribution of CO and CO2 from TCCON total column values using the TARDISS algorithm
The IASI NH3 version 4 product: averaging kernels and improved consistency
A new accurate retrieval of bromine monoxide inside minor volcanic plumes from Sentinel-5 Precursor/TROPOMI
Estimation of NO2 emission strengths over Riyadh and Madrid from space from a combination of wind-assigned anomalies and a machine learning technique
Michelson Interferometer for Passive Atmospheric Sounding Institute of Meteorology and Climate Research/Instituto de Astrofísica de Andalucía version 8 retrieval of nitric oxide and lower-thermospheric temperature
Near-real-time detection of unexpected atmospheric events using principal component analysis on the Infrared Atmospheric Sounding Interferometer (IASI) radiances
Differences in MOPITT surface level CO retrievals and trends from Level 2 and Level 3 products in coastal grid boxes
Updated merged SAGE-CCI-OMPS+ dataset for the evaluation of ozone trends in the stratosphere
Accounting for meteorological biases in simulated plumes using smarter metrics
Accounting for surface reflectance spectral features in TROPOMI methane retrievals
Investigation of three-dimensional radiative transfer effects for UV–Vis satellite and ground-based observations of volcanic plumes
Retrievals of precipitable water vapor and aerosol optical depth from direct sun measurements with EKO MS711 and MS712 spectroradiometers
Update on the GOSAT TANSO–FTS SWIR Level 2 retrieval algorithm
Correcting 3D cloud effects in XCO2 retrievals from the Orbiting Carbon Observatory-2 (OCO-2)
Version 8 IMK–IAA MIPAS ozone profiles: nominal observation mode
Using portable low-resolution spectrometers to evaluate Total Carbon Column Observing Network (TCCON) biases in North America
A new algorithm to generate a priori trace gas profiles for the GGG2020 retrieval algorithm
POMINO-GEMS: A Research Product for Tropospheric NO2 Columns from Geostationary Environment Monitoring Spectrometer
Highly resolved mapping of NO2 vertical column densities from GeoTASO measurements over a megacity and industrial area during the KORUS-AQ campaign
Advances in retrieving XCH4 and XCO from Sentinel-5 Precursor: improvements in the scientific TROPOMI/WFMD algorithm
Use of machine learning and principal component analysis to retrieve nitrogen dioxide (NO2) with hyperspectral imagers and reduce noise in spectral fitting
Understanding the variations and sources of CO, C2H2, C2H6, H2CO, and HCN columns based on 3 years of new ground-based Fourier transform infrared measurements at Xianghe, China
Detecting and quantifying methane emissions from oil and gas production: algorithm development with ground-truth calibration based on Sentinel-2 satellite imagery
An improved formula for the complete data fusion
TUNER-compliant error estimation for MIPAS: methodology
Synergistic retrieval and complete data fusion methods applied to simulated FORUM and IASI-NG measurements
Retrieval of atmospheric CFC-11 and CFC-12 from high-resolution FTIR observations at Hefei and comparisons with other independent datasets
Evaluation of the methane full-physics retrieval applied to TROPOMI ocean sun glint measurements
Harmonized retrieval of middle atmospheric ozone from two microwave radiometers in Switzerland
Assessment of the error budget for stratospheric ozone profiles retrieved from OMPS limb scatter measurements
Algorithm theoretical basis for ozone and sulfur dioxide retrievals from DSCOVR EPIC
Impact of 3D cloud structures on the atmospheric trace gas products from UV–Vis sounders – Part 2: Impact on NO2 retrieval and mitigation strategies
Tropospheric ozone retrieval by a combination of TROPOMI/S5P measurements with BASCOE assimilated data
A new machine-learning-based analysis for improving satellite-retrieved atmospheric composition data: OMI SO2 as an example
Complementing XCO2 imagery with ground-based CO2 and 14CO2 measurements to monitor CO2 emissions from fossil fuels on a regional to local scale
On the potential of a neural-network-based approach for estimating XCO2 from OCO-2 measurements
The Space Carbon Observatory (SCARBO) concept: assessment of XCO2 and XCH4 retrieval performance
Improved retrieval of SO2 plume height from TROPOMI using an iterative Covariance-Based Retrieval Algorithm
Impact of instrumental line shape characterization on ozone monitoring by FTIR spectrometry
Synergetic use of IASI profile and TROPOMI total-column level 2 methane retrieval products
Philipp Hochstaffl, Franz Schreier, Claas Henning Köhler, Andreas Baumgartner, and Daniele Cerra
Atmos. Meas. Tech., 16, 4195–4214, https://doi.org/10.5194/amt-16-4195-2023, https://doi.org/10.5194/amt-16-4195-2023, 2023
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The study examines methane enhancements inferred from hyperspectral imaging observations using different retrieval schemes. One of the core challenges is the high spatial and moderate spectral resolution as it makes separation of spectral variations caused by molecular absorption and surface reflectivity challenging. It was found that localized methane enhancements can be detected and quantified from HySpex airborne observations using various retrieval schemes.
Wenyu Wang, Jian Xu, and Zhenzhan Wang
Atmos. Meas. Tech., 16, 4137–4153, https://doi.org/10.5194/amt-16-4137-2023, https://doi.org/10.5194/amt-16-4137-2023, 2023
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This article presents a study for feasibility analysis of atmospheric wind measurement using a terahertz (THz) passive limb radiometer with high spectral resolution. The simulations show that line-of-sight wind from 40 to 120 km can be obtained better than 10 m s−1 (at most altitudes it is better than 5 m s−1) using the O3, O2, H2O, and OI bands. This study will provide reference for future payload design.
Wei Huang, Lei Liu, Bin Yang, Shuai Hu, Wanying Yang, Zhenfeng Li, Wantong Li, and Xiaofan Yang
Atmos. Meas. Tech., 16, 4101–4114, https://doi.org/10.5194/amt-16-4101-2023, https://doi.org/10.5194/amt-16-4101-2023, 2023
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To improve the retrieval speed of the AERI optimal estimation (AERIoe) method, a fast-retrieval algorithm named Fast AERIoe is proposed on the basis of the findings that the change in Jacobians during the retrieval process had little effect on the performance of AERIoe. The results of the experiment show that the retrieved profiles from Fast AERIoe are comparable to those of AERIoe and that the retrieval speed is significantly improved, with the average retrieval time reduced by 59 %.
Rafaella Chiarella, Matthias Buschmann, Joshua Laughner, Isamu Morino, Justus Notholt, Christof Petri, Geoffrey Toon, Voltaire A. Velazco, and Thorsten Warneke
Atmos. Meas. Tech., 16, 3987–4007, https://doi.org/10.5194/amt-16-3987-2023, https://doi.org/10.5194/amt-16-3987-2023, 2023
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The goal is to establish a window and strategy for xCO2 retrieval from ground-based Fourier transform spectrometers for NDACC. In the study we describe the spectroscopy of the region, the locations and instruments used, and the methods of calculating the retrieved xCO2. We performed tests to assess the sensitivity to diverse factors and sources of errors while comparing the retrieval to a well-established xCO2 retrieval from TCCON.
Zhao-Cheng Zeng, Lu Lee, Chengli Qi, Lieven Clarisse, and Martin Van Damme
Atmos. Meas. Tech., 16, 3693–3713, https://doi.org/10.5194/amt-16-3693-2023, https://doi.org/10.5194/amt-16-3693-2023, 2023
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This study presents an NH3 retrieval algorithm based on the optimal estimation method for the Geostationary Interferometric Infrared Sounder (GIIRS) on board China’s FengYun-4B satellite (FY-4B/GIIRS). Retrieval results demonstrate the capability of FY-4B/GIIRS in capturing the diurnal NH3 changes in East Asia. This operational geostationary observation by FY-4B/GIIRS represents an important advancement over the twice-per-day observations provided by current low-Earth-orbit (LEO) instruments.
Vladimir Savastiouk, Henri Diémoz, and C. Thomas McElroy
EGUsphere, https://doi.org/10.5194/egusphere-2023-1461, https://doi.org/10.5194/egusphere-2023-1461, 2023
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This paper describes a way to significantly improve ozone measurements at low sun elevations and large ozone amounts when using the Brewer ozone spectrophotometer. The proposed algorithm will allow more uniform ozone measurements across the monitoring network. This will contribute to more reliable trend analysis and support the satellite validation. This research contributes to better understanding of the physics of the instrument and the new algorithm is based on this new knowledge.
Ethan Runge, Jeff Langille, Daniel Zawada, Adam Bourassa, and Doug Degenstein
Atmos. Meas. Tech., 16, 3123–3139, https://doi.org/10.5194/amt-16-3123-2023, https://doi.org/10.5194/amt-16-3123-2023, 2023
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The Limb Imaging Fourier Transform Spectrometer Experiment (LIFE) instrument takes vertical images of limb radiance across a wide mid-infrared spectral band from a stratospheric balloon. Measurements are used to infer vertical-trace-gas-profile retrievals of H2O, O3, HNO3, CH4, and N2O. Nearly time-/space-coincident observations from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) and Microwave Limb Sounder (MLS) instruments are compared to the LIFE results.
Zhao-Cheng Zeng, Lu Lee, and Chengli Qi
Atmos. Meas. Tech., 16, 3059–3083, https://doi.org/10.5194/amt-16-3059-2023, https://doi.org/10.5194/amt-16-3059-2023, 2023
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Observations from geostationary orbit provide contiguous coverage with a high temporal resolution, representing an important advancement over current low-Earth-orbit instruments. Using measurements from GIIRS on board China's FengYun satellite, the world’s first geostationary hyperspectral infrared sounder, we showed the first results of diurnal CO in eastern Asia from a geostationary orbit, which will have great potential in improving local and global air quality and climate research.
Tobias Borsdorff, Teresa Campos, Natalie Kille, Kyle J. Zarzana, Rainer Volkamer, and Jochen Landgraf
Atmos. Meas. Tech., 16, 3027–3038, https://doi.org/10.5194/amt-16-3027-2023, https://doi.org/10.5194/amt-16-3027-2023, 2023
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ECMWF plans to assimilate TROPOMI CO with their CAMS-IFS model. This will constrain the total column and the vertical CO distribution of the model. To show this, we combine individual TROPOMI CO column retrievals with different vertical sensitivities and obtain a vertical CO concentration profile. We test the approach on three CO pollution events in comparison with CAMS-IFS simulations that do not assimilate TROPOMI CO data and in situ airborne measurements of the BB-FLUX campaign.
Peter Joyce, Cristina Ruiz Villena, Yahui Huang, Alex Webb, Manuel Gloor, Fabien H. Wagner, Martyn P. Chipperfield, Rocío Barrio Guilló, Chris Wilson, and Hartmut Boesch
Atmos. Meas. Tech., 16, 2627–2640, https://doi.org/10.5194/amt-16-2627-2023, https://doi.org/10.5194/amt-16-2627-2023, 2023
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Methane emissions are responsible for a lot of the warming caused by the greenhouse effect, much of which comes from a small number of point sources. We can identify methane point sources by analysing satellite data, but it requires a lot of time invested by experts and is prone to very high errors. Here, we produce a neural network that can automatically identify methane point sources and estimate the mass of methane that is being released per hour and are able to do so with far smaller errors.
Harrison A. Parker, Joshua L. Laughner, Geoffrey C. Toon, Debra Wunch, Coleen M. Roehl, Laura T. Iraci, James R. Podolske, Kathryn McKain, Bianca C. Baier, and Paul O. Wennberg
Atmos. Meas. Tech., 16, 2601–2625, https://doi.org/10.5194/amt-16-2601-2023, https://doi.org/10.5194/amt-16-2601-2023, 2023
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We describe a retrieval algorithm for determining limited information about the vertical distribution of carbon monoxide (CO) and carbon dioxide (CO2) from total column observations from ground-based observations. Our retrieved partial column values compare well with integrated in situ data. The average error for our retrieval is 1.51 ppb (~ 2 %) for CO and 5.09 ppm (~ 1.25 %) for CO2. We anticipate that this approach will find broad application for use in carbon cycle science.
Lieven Clarisse, Bruno Franco, Martin Van Damme, Tommaso Di Gioacchino, Juliette Hadji-Lazaro, Simon Whitburn, Lara Noppen, Daniel Hurtmans, Cathy Clerbaux, and Pierre Coheur
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-48, https://doi.org/10.5194/amt-2023-48, 2023
Revised manuscript accepted for AMT
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Ammonia is an important atmospheric pollutant. This article presents version 4 of the algorithm which retrieves abundances from the infrared measurements of the satellite sounder IASI. A measurement operator is introduced that can be used to emulate the measurements (so-called averaging kernels) and measurement uncertainty is better characterized. Several other changes to the product itself are also documented, most of which improve the temporal consistency of the 2007–2022 IASI NH3 dataset.
Simon Warnach, Holger Sihler, Christian Borger, Nicole Bobrowski, Steffen Beirle, Ulrich Platt, and Thomas Wagner
EGUsphere, https://doi.org/10.5194/egusphere-2023-933, https://doi.org/10.5194/egusphere-2023-933, 2023
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The paper discusses how to best detect gases inside volcanic plumes, namely BrO. Volcanic gases correspond to the magmatic signal and can be used to characterize the volcano. Satellite observations of high accuracy can provide a global inventory of this important quantity. The increase in accuracy provided in this paper can pave the way towards a most-complete inventory of volcanic gas composition.
Qiansi Tu, Frank Hase, Zihan Chen, Matthias Schneider, Omaira García, Farahnaz Khosrawi, Shuo Chen, Thomas Blumenstock, Fang Liu, Kai Qin, Jason Cohen, Qin He, Song Lin, Hongyan Jiang, and Dianjun Fang
Atmos. Meas. Tech., 16, 2237–2262, https://doi.org/10.5194/amt-16-2237-2023, https://doi.org/10.5194/amt-16-2237-2023, 2023
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Four-year TROPOMI observations are used to derive tropospheric NO2 emissions in two mega(cities) with high anthropogenic activity. Wind-assigned anomalies are calculated, and the emission rates and spatial patterns are estimated based on a machine learning algorithm. The results are in reasonable agreement with previous studies and the inventory. Our method is quite robust and can be used as a simple method to estimate the emissions of NO2 as well as other gases in other regions.
Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Manuel López-Puertas, Gabriele P. Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 16, 2167–2196, https://doi.org/10.5194/amt-16-2167-2023, https://doi.org/10.5194/amt-16-2167-2023, 2023
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New global nitric oxide (NO) volume-mixing-ratio and lower-thermospheric temperature data products, retrieved from Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) spectra with the IMK-IAA MIPAS data processor, have been released. The dataset covers the entire Envisat mission lifetime and includes retrieval results from all MIPAS observation modes. The data are based on ESA version 8 calibration and were processed using an improved retrieval approach.
Adrien Vu Van, Anne Boynard, Pascal Prunet, Dominique Jolivet, Olivier Lezeaux, Patrice Henry, Claude Camy-Peyret, Lieven Clarisse, Bruno Franco, Pierre-François Coheur, and Cathy Clerbaux
Atmos. Meas. Tech., 16, 2107–2127, https://doi.org/10.5194/amt-16-2107-2023, https://doi.org/10.5194/amt-16-2107-2023, 2023
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With its near-real-time observations and good horizontal coverage, the Infrared Atmospheric Sounding Interferometer (IASI) instrument can contribute to the monitoring systems for a systematic and continuous detection of exceptional atmospheric events such as fires, anthropogenic pollution episodes, volcanic eruptions, or industrial releases. In this paper, a new approach is described for the detection and characterization of unexpected events in terms of trace gases using IASI radiance spectra.
Ian Ashpole and Aldona Wiacek
Atmos. Meas. Tech., 16, 1923–1949, https://doi.org/10.5194/amt-16-1923-2023, https://doi.org/10.5194/amt-16-1923-2023, 2023
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The MOPITT instrument has been measuring atmospheric carbon monoxide (CO) from space since 2000. Its data products are valuable for CO trend analysis. This paper compares products with different spatial resolutions to identify discrepancies in mean CO amounts and detectable trends for coastal grid boxes. It is found that CO amounts and trends differ significantly between data products for a large number of these grid boxes, essentially due to how the coarser-resolution products are created.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Carlo Arosio, Alexei Rozanov, Mark Weber, Doug Degenstein, Adam Bourassa, Daniel Zawada, Michael Kiefer, Alexandra Laeng, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Christian Retscher, Robert Damadeo, and Jerry D. Lumpe
Atmos. Meas. Tech., 16, 1881–1899, https://doi.org/10.5194/amt-16-1881-2023, https://doi.org/10.5194/amt-16-1881-2023, 2023
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The paper presents the updated SAGE-CCI-OMPS+ climate data record of monthly zonal mean ozone profiles. This dataset covers the stratosphere and combines measurements by nine limb and occultation satellite instruments (SAGE II, OSIRIS, MIPAS, SCIAMACHY, GOMOS, ACE-FTS, OMPS-LP, POAM III, and SAGE III/ISS). The update includes new versions of MIPAS, ACE-FTS, and OSIRIS datasets and introduces data from additional sensors (POAM III and SAGE III/ISS) and retrieval processors (OMPS-LP).
Pierre J. Vanderbecken, Joffrey Dumont Le Brazidec, Alban Farchi, Marc Bocquet, Yelva Roustan, Élise Potier, and Grégoire Broquet
Atmos. Meas. Tech., 16, 1745–1766, https://doi.org/10.5194/amt-16-1745-2023, https://doi.org/10.5194/amt-16-1745-2023, 2023
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Instruments dedicated to monitoring atmospheric gaseous compounds from space will provide images of urban-scale plumes. We discuss here the use of new metrics to compare observed plumes with model predictions that will be less sensitive to meteorology uncertainties. We have evaluated our metrics on diverse plumes and shown that by eliminating some aspects of the discrepancies, they are indeed less sensitive to meteorological variations.
Alba Lorente, Tobias Borsdorff, Mari C. Martinez-Velarte, and Jochen Landgraf
Atmos. Meas. Tech., 16, 1597–1608, https://doi.org/10.5194/amt-16-1597-2023, https://doi.org/10.5194/amt-16-1597-2023, 2023
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In the TROPOMI methane data, there are few false methane anomalies that can be misinterpreted as enhancements caused by strong emission sources. These artefacts are caused by features of the underlying surfaces that are not well characterized in the retrieval algorithm. Here we improve the representation of the surface reflectance dependency with wavelength in the forward model, removing the artificial localized CH4 enhancements found in several locations like Siberia, Australia and Algeria.
Thomas Wagner, Simon Warnach, Steffen Beirle, Nicole Bobrowski, Adrian Jost, Janis Puķīte, and Nicolas Theys
Atmos. Meas. Tech., 16, 1609–1662, https://doi.org/10.5194/amt-16-1609-2023, https://doi.org/10.5194/amt-16-1609-2023, 2023
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We investigate 3D effects of volcanic plumes on the retrieval results of satellite and ground-based UV–Vis observations. With its small ground pixels of 3.5 x 5.5 km², the TROPOMI instrument can detect much smaller volcanic plumes than previous instruments. At the same time, 3D effects become important. The effect of horizontal photon paths especially can lead to a strong underestimation of the derived plume contents of up to > 50 %, which can be further increased for strong absorbers like SO2.
Congcong Qiao, Song Liu, Juan Huo, Xihan Mu, Ping Wang, Shengjie Jia, Xuehua Fan, and Minzheng Duan
Atmos. Meas. Tech., 16, 1539–1549, https://doi.org/10.5194/amt-16-1539-2023, https://doi.org/10.5194/amt-16-1539-2023, 2023
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We established a spectral-fitting method to derive precipitable water vapor (PWV) and aerosol optical depth based on a strict radiative transfer theory by the spectral measurements of direct sun from EKO MS711 and MS712 spectroradiometers. The retrievals were compared with that of the colocated CE-318 photometer; the results showed a high degree of consistency. In the PWV inversion, a strong water vapor absorption band around 1370 nm is introduced to retrieve PWV in a relatively dry atmosphere.
Yu Someya, Yukio Yoshida, Hirofumi Ohyama, Shohei Nomura, Akihide Kamei, Isamu Morino, Hitoshi Mukai, Tsuneo Matsunaga, Joshua L. Laughner, Voltaire A. Velazco, Benedikt Herkommer, Yao Té, Mahesh Kumar Sha, Rigel Kivi, Minqiang Zhou, Young Suk Oh, Nicholas M. Deutscher, and David W. T. Griffith
Atmos. Meas. Tech., 16, 1477–1501, https://doi.org/10.5194/amt-16-1477-2023, https://doi.org/10.5194/amt-16-1477-2023, 2023
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The updated retrieval algorithm for the Greenhouse gases Observing SATellite level 2 product is presented. The main changes in the algorithm from the previous one are the treatment of cirrus clouds, the degradation model of the sensor, solar irradiance, and gas absorption coefficient tables. The retrieval results showed improvements in fitting accuracy and an increase in the data amount over land. On the other hand, there are still large biases of XCO2 which should be corrected over the ocean.
Steffen Mauceri, Steven Massie, and Sebastian Schmidt
Atmos. Meas. Tech., 16, 1461–1476, https://doi.org/10.5194/amt-16-1461-2023, https://doi.org/10.5194/amt-16-1461-2023, 2023
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The Orbiting Carbon Observatory-2 makes space-based measurements of reflected sunlight. Using a retrieval algorithm these measurements are converted to CO2 concentrations in the atmosphere. However, the converted CO2 concentrations contain errors for observations close to clouds. Using a simple machine learning approach, we developed a model to correct these remaining errors. The model is able to reduce errors over land and ocean by 20 % and 40 %, respectively.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 1443–1460, https://doi.org/10.5194/amt-16-1443-2023, https://doi.org/10.5194/amt-16-1443-2023, 2023
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A new ozone data set, derived from radiation measurements of the space-borne instrument MIPAS, is presented. It consists of more than 2 million single ozone profiles from 2002–2012, covering virtually all latitudes and altitudes between 5 and 70 km. Progress in data calibration and processing methods allowed for significant improvement of the data quality, compared to previous data versions. Hence, the data set will help to better understand e.g. the time evolution of ozone in the stratosphere.
Nasrin Mostafavi Pak, Jacob K. Hedelius, Sébastien Roche, Liz Cunningham, Bianca Baier, Colm Sweeney, Coleen Roehl, Joshua Laughner, Geoffrey Toon, Paul Wennberg, Harrison Parker, Colin Arrowsmith, Joseph Mendonca, Pierre Fogal, Tyler Wizenberg, Beatriz Herrera, Kimberly Strong, Kaley A. Walker, Felix Vogel, and Debra Wunch
Atmos. Meas. Tech., 16, 1239–1261, https://doi.org/10.5194/amt-16-1239-2023, https://doi.org/10.5194/amt-16-1239-2023, 2023
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Ground-based remote sensing instruments in the Total Carbon Column Observing Network (TCCON) measure greenhouse gases in the atmosphere. Consistency between TCCON measurements is crucial to accurately infer changes in atmospheric composition. We use portable remote sensing instruments (EM27/SUN) to evaluate biases between TCCON stations in North America. We also improve the retrievals of EM27/SUN instruments and evaluate the previous (GGG2014) and newest (GGG2020) retrieval algorithms.
Joshua L. Laughner, Sébastien Roche, Matthäus Kiel, Geoffrey C. Toon, Debra Wunch, Bianca C. Baier, Sébastien Biraud, Huilin Chen, Rigel Kivi, Thomas Laemmel, Kathryn McKain, Pierre-Yves Quéhé, Constantina Rousogenous, Britton B. Stephens, Kaley Walker, and Paul O. Wennberg
Atmos. Meas. Tech., 16, 1121–1146, https://doi.org/10.5194/amt-16-1121-2023, https://doi.org/10.5194/amt-16-1121-2023, 2023
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Observations using sunlight to measure surface-to-space total column of greenhouse gases in the atmosphere need an initial guess of the vertical distribution of those gases to start from. We have developed an approach to provide those initial guess profiles that uses readily available meteorological data as input. This lets us make these guesses without simulating them with a global model. The profiles generated this way match independent observations well.
Yuhang Zhang, Jintai Lin, Jhoon Kim, Hanlim Lee, Junsung Park, Hyunkee Hong, Michel Van Roozendael, Francois Hendrick, Ting Wang, Pucai Wang, Qin He, Kai Qin, Yongjoo Choi, Yugo Kanaya, Jin Xu, Pinhua Xie, Xin Tian, Sanbao Zhang, Shanshan Wang, Robert Spurr, Lulu Chen, Hao Kong, and Mengyao Liu
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-46, https://doi.org/10.5194/amt-2023-46, 2023
Revised manuscript accepted for AMT
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We build a research product of tropospheric NO2 VCDs with high spatiotemporal resolution based on the Geostationary Environment Monitoring Spectrometer (GEMS) named as POMINO-GEMS. Strong hotspot signals and diurnal variation of tropospheric NO2 are clearly presented. Validations with TROPOMI observations and ground-based MAX-DOAS as well as MEE measurements exhibit overall great performance of POMINO-GEMS NO2 VCDs, indicating the capability for application in extensive environmental researches.
Gyo-Hwang Choo, Kyunghwa Lee, Hyunkee Hong, Ukkyo Jeong, Wonei Choi, and Scott J. Janz
Atmos. Meas. Tech., 16, 625–644, https://doi.org/10.5194/amt-16-625-2023, https://doi.org/10.5194/amt-16-625-2023, 2023
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This study discusses the morning and afternoon distribution of NO2 emissions in large cities and industrial areas in South Korea, one of the largest NO2 emitters around the world, using GeoTASO, an airborne remote sensing instrument developed to support geostationary satellite missions. NO2 measurements from GeoTASO were compared with those from ground-based remote sensing instruments including Pandora and in situ sensors.
Oliver Schneising, Michael Buchwitz, Jonas Hachmeister, Steffen Vanselow, Maximilian Reuter, Matthias Buschmann, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 16, 669–694, https://doi.org/10.5194/amt-16-669-2023, https://doi.org/10.5194/amt-16-669-2023, 2023
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Methane and carbon monoxide are important constituents of the atmosphere in the context of climate change and air pollution. We present the latest advances in the TROPOMI/WFMD algorithm to simultaneously retrieve atmospheric methane and carbon monoxide abundances from space. The changes in the latest product version are described in detail, and the resulting improvements are demonstrated. An overview of the products is provided including a discussion of annual increases and validation results.
Joanna Joiner, Sergey Marchenko, Zachary Fasnacht, Lok Lamsal, Can Li, Alexander Vasilkov, and Nickolay Krotkov
Atmos. Meas. Tech., 16, 481–500, https://doi.org/10.5194/amt-16-481-2023, https://doi.org/10.5194/amt-16-481-2023, 2023
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Nitrogen dioxide (NO2) is an important trace gas for both air quality and climate. NO2 affects satellite ocean color products. A new ocean color instrument – OCI (Ocean Color Instrument) – will be launched in 2024 on a NASA satellite. We show that it will be possible to measure NO2 from OCI even though it was not designed for this. The techniques developed here, based on machine learning, can also be applied to instruments already in space to speed up algorithms and reduce the effects of noise.
Minqiang Zhou, Bavo Langerock, Pucai Wang, Corinne Vigouroux, Qichen Ni, Christian Hermans, Bart Dils, Nicolas Kumps, Weidong Nan, and Martine De Mazière
Atmos. Meas. Tech., 16, 273–293, https://doi.org/10.5194/amt-16-273-2023, https://doi.org/10.5194/amt-16-273-2023, 2023
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The ground-based FTIR measurements at Xianghe provide carbon monoxide (CO), acetylene (C2H2), ethane (C2H6), formaldehyde (H2CO), and hydrogen cyanide (HCN) total columns between June 2018 and November 2021. The retrieval strategies, information, and uncertainties of these five important trace gases are presented and discussed. This study provides insight into the time series, variations, and correlations of these five species in northern China.
Zhan Zhang, Evan D. Sherwin, Daniel J. Varon, and Adam R. Brandt
Atmos. Meas. Tech., 15, 7155–7169, https://doi.org/10.5194/amt-15-7155-2022, https://doi.org/10.5194/amt-15-7155-2022, 2022
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This work developed a multi-band–multi-pass–multi-comparison-date Sentinel-2 methane retrieval algorithm, and the method was calibrated by data from a controlled release test. To our knowledge, this is the first study that validates the performance of a Sentinel-2 methane detection algorithm by calibration with a ground-truth testing. It illustrates the potential for additional validation with systematic future experiments wherein algorithms can be tuned to meet different detection expectations.
Simone Ceccherini, Nicola Zoppetti, and Bruno Carli
Atmos. Meas. Tech., 15, 7039–7048, https://doi.org/10.5194/amt-15-7039-2022, https://doi.org/10.5194/amt-15-7039-2022, 2022
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A new formula of the complete data fusion that, differently from the original one, does not contain matrices that can be singular is discussed. We show that the new formula is a generalization of the original one and analytically and numerically, using a real IASI ozone measurement, derive the errors made with the old formula when the generalized inverse of singular matrices is used. An operational version of the new formula that includes interpolation and coincidence errors is also provided.
Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Bernd Funke, Michael Kiefer, Anne Kleinert, Gabriele P. Stiller, Andrea Linden, and Sylvia Kellmann
Atmos. Meas. Tech., 15, 6991–7018, https://doi.org/10.5194/amt-15-6991-2022, https://doi.org/10.5194/amt-15-6991-2022, 2022
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Errors of profiles of temperature and mixing ratios retrieved from spectra recorded with the Michelson Interferometer for Passive Atmospheric Sounding are estimated. All known and quantified sources of uncertainty are considered. Some ongoing uncertaities contribute to both the random and to the systematic errors. In some cases, one source of uncertainty propagates onto the error budget via multiple pathways. Problems arise when the correlations of errors to be propagated are unknown.
Marco Ridolfi, Cecilia Tirelli, Simone Ceccherini, Claudio Belotti, Ugo Cortesi, and Luca Palchetti
Atmos. Meas. Tech., 15, 6723–6737, https://doi.org/10.5194/amt-15-6723-2022, https://doi.org/10.5194/amt-15-6723-2022, 2022
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Synergistic retrieval (SR) and complete data fusion (CDF) methods exploit the complementarity of coinciding remote-sensing measurements. We assess the performance of the SR and CDF methods on the basis of synthetic measurements of the FORUM and IASI-NG missions. In the case of perfectly matching measurements, SR and CDF results differ by less than 1 / 10 of the error due to measurement noise. In the case of a realistic mismatch, the two methods show differences in the order of their error bars.
Xiangyu Zeng, Wei Wang, Cheng Liu, Changgong Shan, Yu Xie, Peng Wu, Qianqian Zhu, Minqiang Zhou, Martine De Mazière, Emmanuel Mahieu, Irene Pardo Cantos, Jamal Makkor, and Alexander Polyakov
Atmos. Meas. Tech., 15, 6739–6754, https://doi.org/10.5194/amt-15-6739-2022, https://doi.org/10.5194/amt-15-6739-2022, 2022
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CFC-11 and CFC-12, which are classified as ozone-depleting substances, also have high global warming potentials. This paper describes obtaining the CFC-11 and CFC-12 total columns from the solar spectra based on ground-based Fourier transform infrared spectroscopy at Hefei, China. The seasonal variation and annual trend of the two gases are analyzed, and then the data are compared with other independent datasets.
Alba Lorente, Tobias Borsdorff, Mari C. Martinez-Velarte, Andre Butz, Otto P. Hasekamp, Lianghai Wu, and Jochen Landgraf
Atmos. Meas. Tech., 15, 6585–6603, https://doi.org/10.5194/amt-15-6585-2022, https://doi.org/10.5194/amt-15-6585-2022, 2022
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The TROPOspheric Monitoring Instrument (TROPOMI) performs observations over ocean in every orbit, enhancing the monitoring capabilities of methane from space. In the sun glint geometry the mirror-like reflection at the water surface provides a signal that is high enough to retrieve methane with high accuracy and precision. We present 4 years of methane concentrations over the ocean, and we assess its quality. We also show the importance of ocean observations to quantify total CH4 emissions.
Eric Sauvageat, Eliane Maillard Barras, Klemens Hocke, Alexander Haefele, and Axel Murk
Atmos. Meas. Tech., 15, 6395–6417, https://doi.org/10.5194/amt-15-6395-2022, https://doi.org/10.5194/amt-15-6395-2022, 2022
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We present new harmonized ozone time series from two ground-based microwave radiometers in Switzerland. The new series consist of hourly ozone profiles in the middle atmosphere (~ 20–70 km) from 2009 until 2021. Cross-validation of the new data series shows the benefit of the harmonization process compared to the previous versions. Comparisons with collocated satellite observations is used to further validate these time series for long-term ozone monitoring over central Europe.
Carlo Arosio, Alexei Rozanov, Victor Gorshelev, Alexandra Laeng, and John P. Burrows
Atmos. Meas. Tech., 15, 5949–5967, https://doi.org/10.5194/amt-15-5949-2022, https://doi.org/10.5194/amt-15-5949-2022, 2022
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This paper characterizes the uncertainties affecting the ozone profiles retrieved at the University of Bremen through OMPS limb satellite observations. An accurate knowledge of the uncertainties is relevant for the validation of the product and to correctly interpret the retrieval results. We investigate several sources of uncertainties, estimate a total random and systematic component, and verify the consistency of the combined OMPS-MLS total uncertainty.
Xinzhou Huang and Kai Yang
Atmos. Meas. Tech., 15, 5877–5915, https://doi.org/10.5194/amt-15-5877-2022, https://doi.org/10.5194/amt-15-5877-2022, 2022
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This paper describes the algorithm for O3 and SO2 retrievals from DSCOVR EPIC. Algorithm advances, including the improved O3 profile representation and the regulated direct fitting inversion technique, improve the accuracy of O3 and SO2 from the multi-channel measurements of DSCOVR EPIC. A thorough error analysis is provided to quantify O3 and SO2 retrieval uncertainties due to various error sources and simplified algorithm physics treatments.
Huan Yu, Claudia Emde, Arve Kylling, Ben Veihelmann, Bernhard Mayer, Kerstin Stebel, and Michel Van Roozendael
Atmos. Meas. Tech., 15, 5743–5768, https://doi.org/10.5194/amt-15-5743-2022, https://doi.org/10.5194/amt-15-5743-2022, 2022
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In this study, we have investigated the impact of 3D clouds on the tropospheric NO2 retrieval from UV–visible sensors. We applied standard NO2 retrieval methods including cloud corrections to synthetic data generated by the 3D radiative transfer model. A sensitivity study was done for synthetic data, and dependencies on various parameters were investigated. Possible mitigation strategies were investigated and compared based on 3D simulations and observed data.
Klaus-Peter Heue, Diego Loyola, Fabian Romahn, Walter Zimmer, Simon Chabrillat, Quentin Errera, Jerry Ziemke, and Natalya Kramarova
Atmos. Meas. Tech., 15, 5563–5579, https://doi.org/10.5194/amt-15-5563-2022, https://doi.org/10.5194/amt-15-5563-2022, 2022
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To retrieve tropospheric ozone column information, we subtract stratospheric column data of BASCOE from TROPOMI/S5P total ozone columns.
The new S5P-BASCOE data agree well with existing tropospheric data like OMPS-MERRA-2. The data are also compared to ozone soundings.
The tropospheric ozone columns show the expected temporal and spatial patterns. We will also apply the algorithm to future UV nadir missions like Sentinel 4 or 5 or to recent and ongoing missions like GOME_2 or OMI.
Can Li, Joanna Joiner, Fei Liu, Nickolay A. Krotkov, Vitali Fioletov, and Chris McLinden
Atmos. Meas. Tech., 15, 5497–5514, https://doi.org/10.5194/amt-15-5497-2022, https://doi.org/10.5194/amt-15-5497-2022, 2022
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Satellite observations provide information on the sources of SO2, an important pollutant that affects both air quality and climate. However, these observations suffer from relatively poor data quality due to weak signals of SO2. Here, we use a machine learning technique to analyze satellite SO2 observations in order to reduce the noise and artifacts over relatively clean areas while keeping the signals near pollution sources. This leads to significant improvement in satellite SO2 data.
Elise Potier, Grégoire Broquet, Yilong Wang, Diego Santaren, Antoine Berchet, Isabelle Pison, Julia Marshall, Philippe Ciais, François-Marie Bréon, and Frédéric Chevallier
Atmos. Meas. Tech., 15, 5261–5288, https://doi.org/10.5194/amt-15-5261-2022, https://doi.org/10.5194/amt-15-5261-2022, 2022
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Atmospheric inversion at local–regional scales over Europe and pseudo-data assimilation are used to evaluate how CO2 and 14CO2 ground-based measurement networks could complement satellite CO2 imagers to monitor fossil fuel (FF) CO2 emissions. This combination significantly improves precision in the FF emission estimates in areas with a dense network but does not strongly support the separation of the FF from the biogenic signals or the spatio-temporal extrapolation of the satellite information.
François-Marie Bréon, Leslie David, Pierre Chatelanaz, and Frédéric Chevallier
Atmos. Meas. Tech., 15, 5219–5234, https://doi.org/10.5194/amt-15-5219-2022, https://doi.org/10.5194/amt-15-5219-2022, 2022
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The estimate of atmospheric CO2 from space measurement is difficult. Current methods are based on a detailed description of the atmospheric radiative transfer. These are affected by significant biases and errors and are very computer intensive. Instead we have proposed using a neural network approach. A first attempt led to confusing results. Here we provide an interpretation for these results and describe a new version that leads to high-quality estimates.
Matthieu Dogniaux, Cyril Crevoisier, Silvère Gousset, Étienne Le Coarer, Yann Ferrec, Laurence Croizé, Lianghai Wu, Otto Hasekamp, Bojan Sic, and Laure Brooker
Atmos. Meas. Tech., 15, 4835–4858, https://doi.org/10.5194/amt-15-4835-2022, https://doi.org/10.5194/amt-15-4835-2022, 2022
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The Space Carbon Observatory (SCARBO) concept proposes a constellation of small satellites that would carry a miniaturized Fabry–Pérot imaging interferometer named NanoCarb and an aerosol instrument named SPEXone. In this work, we assess the performance of this concept for the retrieval of the total weighted columns of CO2 and CH4 and show the interest of adding the SPEXone aerosol instrument to improve the CO2 and CH4 column retrieval.
Nicolas Theys, Christophe Lerot, Hugues Brenot, Jeroen van Gent, Isabelle De Smedt, Lieven Clarisse, Mike Burton, Matthew Varnam, Catherine Hayer, Benjamin Esse, and Michel Van Roozendael
Atmos. Meas. Tech., 15, 4801–4817, https://doi.org/10.5194/amt-15-4801-2022, https://doi.org/10.5194/amt-15-4801-2022, 2022
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Sulfur dioxide plume height after a volcanic eruption is an important piece of information for many different scientific studies and applications. Satellite UV retrievals are useful in this respect, but available algorithms have shown so far limited sensitivity to SO2 height. Here we present a new technique to improve the retrieval of SO2 plume height for SO2 columns as low as 5 DU. We demonstrate the algorithm using TROPOMI measurements and compare with other height estimates.
Omaira E. García, Esther Sanromá, Frank Hase, Matthias Schneider, Sergio Fabián León-Luis, Thomas Blumenstock, Eliezer Sepúlveda, Carlos Torres, Natalia Prats, Alberto Redondas, and Virgilio Carreño
Atmos. Meas. Tech., 15, 4547–4567, https://doi.org/10.5194/amt-15-4547-2022, https://doi.org/10.5194/amt-15-4547-2022, 2022
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Retrieving high-precision concentrations of atmospheric trace gases from FTIR (Fourier transform infrared) spectrometry requires a precise knowledge of the instrumental performance. In this context, this paper examines the impact on the ozone (O3) retrievals of several approaches used to characterise the instrumental line shape (ILS) function of ground-based FTIR spectrometers within NDACC (Network for the Detection of Atmospheric Composition Change).
Matthias Schneider, Benjamin Ertl, Qiansi Tu, Christopher J. Diekmann, Farahnaz Khosrawi, Amelie N. Röhling, Frank Hase, Darko Dubravica, Omaira E. García, Eliezer Sepúlveda, Tobias Borsdorff, Jochen Landgraf, Alba Lorente, André Butz, Huilin Chen, Rigel Kivi, Thomas Laemmel, Michel Ramonet, Cyril Crevoisier, Jérome Pernin, Martin Steinbacher, Frank Meinhardt, Kimberly Strong, Debra Wunch, Thorsten Warneke, Coleen Roehl, Paul O. Wennberg, Isamu Morino, Laura T. Iraci, Kei Shiomi, Nicholas M. Deutscher, David W. T. Griffith, Voltaire A. Velazco, and David F. Pollard
Atmos. Meas. Tech., 15, 4339–4371, https://doi.org/10.5194/amt-15-4339-2022, https://doi.org/10.5194/amt-15-4339-2022, 2022
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We present a computationally very efficient method for the synergetic use of level 2 remote-sensing data products. We apply the method to IASI vertical profile and TROPOMI total column space-borne methane observations and thus gain sensitivity for the tropospheric methane partial columns, which is not achievable by the individual use of TROPOMI and IASI. These synergetic effects are evaluated theoretically and empirically by inter-comparisons to independent references of TCCON, AirCore, and GAW.
Cited articles
Barthlott, S., Schneider, M., Hase, F., Blumenstock, T., Mengistu Tsidu, G., Grutter de la Mora, M., Strong, K., Notholt, J., Mahieu, E., Jones, N., and Smale, D.: The ground-based MUSICA dataset: Tropospheric water vapour isotopologues (H216O, H218O and HD16O) as obtained from NDACC/FTIR solar absorption spectra, https://doi.org/10.5281/zenodo.48902, 2016.
Barthlott, S., Schneider, M., Hase, F., Blumenstock, T., Kiel, M., Dubravica, D., García, O. E., Sepúlveda, E., Mengistu Tsidu, G., Takele Kenea, S., Grutter, M., Plaza-Medina, E. F., Stremme, W., Strong, K., Weaver, D., Palm, M., Warneke, T., Notholt, J., Mahieu, E., Servais, C., Jones, N., Griffith, D. W. T., Smale, D., and Robinson, J.: Tropospheric water vapour isotopologue data (H216O, H218O, and HD16O) as obtained from NDACC/FTIR solar absorption spectra, Earth Syst. Sci. Data, 9, 15–29, https://doi.org/10.5194/essd-9-15-2017, 2017.
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Boesch, H., Deutscher, N. M., Warneke, T., Byckling, K., Cogan, A. J., Griffith, D. W. T., Notholt, J., Parker, R. J., and Wang, Z.: HDO/H2O ratio retrievals from GOSAT, Atmos. Meas. Tech., 6, 599–612, https://doi.org/10.5194/amt-6-599-2013, 2013.
Borsdorff, T., Hasekamp, O. P., Wassmann, A., and Landgraf, J.: Insights into Tikhonov regularization: application to trace gas column retrieval and the efficient calculation of total column averaging kernels, Atmos. Meas. Tech., 7, 523–535, https://doi.org/10.5194/amt-7-523-2014, 2014.
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Scheepmaker, R. A., Frankenberg, C., Galli, A., Butz, A., Schrijver, H., Deutscher, N. M., Wunch, D., Warneke, T., Fally, S., and Aben, I.: Improved water vapour spectroscopy in the 4174–4300 cm−1 region and its impact on SCIAMACHY HDO/H2O measurements, Atmos. Meas. Tech., 6, 879–894, https://doi.org/10.5194/amt-6-879-2013, 2013.
Scheepmaker, R. A., Frankenberg, C., Deutscher, N. M., Schneider, M., Barthlott, S., Blumenstock, T., Garcia, O. E., Hase, F., Jones, N., Mahieu, E., Notholt, J., Velazco, V., Landgraf, J., and Aben, I.: Validation of SCIAMACHY HDO/H2O measurements using the TCCON and NDACC-MUSICA networks, Atmos. Meas. Tech., 8, 1799–1818, https://doi.org/10.5194/amt-8-1799-2015, 2015.
Scheepmaker, R. A., aan de Brugh, J., Hu, H., Borsdorff, T., Frankenberg, C., Risi, C., Hasekamp, O., Aben, I., and Landgraf, J.: HDO and H2O total column retrievals from TROPOMI shortwave infrared measurements, Atmos. Meas. Tech., 9, 3921–3937, https://doi.org/10.5194/amt-9-3921-2016, 2016.
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Short summary
A new data set of vertical column densities of the water vapour isotopologues H2O and HDO retrieved from short-wave infrared measurements (2339 nm to 2383 nm) by the SCIAMACHY satellite instrument for the whole of the mission period from 2003 to 2012 is presented. The data are validated against ground-based Fourier transform infrared measurements. High-altitude stations observe different air columns; thus in this case collocated scenes with clouds around station height are needed for agreement.
A new data set of vertical column densities of the water vapour isotopologues H2O and HDO...