Articles | Volume 16, issue 20
https://doi.org/10.5194/amt-16-4961-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-16-4961-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Numerical investigation on retrieval errors of mixing states of fractal black carbon aerosols using single-particle soot photometer based on Mie scattering and the effects on radiative forcing estimation
Non-destructive Testing Laboratory, School of Quality and Technical Supervision, Hebei University, Baoding, 071002, China
National & Local Joint Engineering Research Center of Metrology Instrument and System, Baoding, 071002, China
Hebei Key Laboratory of Energy Metering and Safety Testing Technology, Baoding, 071002, China
Guangya Wang
Non-destructive Testing Laboratory, School of Quality and Technical Supervision, Hebei University, Baoding, 071002, China
National & Local Joint Engineering Research Center of Metrology Instrument and System, Baoding, 071002, China
Hebei Key Laboratory of Energy Metering and Safety Testing Technology, Baoding, 071002, China
Cancan Zhu
Non-destructive Testing Laboratory, School of Quality and Technical Supervision, Hebei University, Baoding, 071002, China
National & Local Joint Engineering Research Center of Metrology Instrument and System, Baoding, 071002, China
Hebei Key Laboratory of Energy Metering and Safety Testing Technology, Baoding, 071002, China
Donghui Zhou
Non-destructive Testing Laboratory, School of Quality and Technical Supervision, Hebei University, Baoding, 071002, China
National & Local Joint Engineering Research Center of Metrology Instrument and System, Baoding, 071002, China
Hebei Key Laboratory of Energy Metering and Safety Testing Technology, Baoding, 071002, China
Lin Wang
Non-destructive Testing Laboratory, School of Quality and Technical Supervision, Hebei University, Baoding, 071002, China
National & Local Joint Engineering Research Center of Metrology Instrument and System, Baoding, 071002, China
Hebei Key Laboratory of Energy Metering and Safety Testing Technology, Baoding, 071002, China
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Single-particle soot photometer (SP2) measures the mixing state (Dp/Dc) of coated black carbon (BC) using core-shell Mie theory and coating refractive index is set to 1.50+0i. The retrieved Dp/Dc contains error due to the non-sphericity of BC and coatings with various refractive indices. We reveal the remarkable effects of coatings on the Dp/Dc retrieval accuracy of SP2 based on optical simulation of fractal BC aerosols, and further evaluate the simple radiative forcing efficiency of coated BC.
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
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Single-particle soot photometer (SP2) measures the mixing state (Dp/Dc) of coated black carbon (BC) using core-shell Mie theory and coating refractive index is set to 1.50+0i. The retrieved Dp/Dc contains error due to the non-sphericity of BC and coatings with various refractive indices. We reveal the remarkable effects of coatings on the Dp/Dc retrieval accuracy of SP2 based on optical simulation of fractal BC aerosols, and further evaluate the simple radiative forcing efficiency of coated BC.
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
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Short summary
Single-particle soot photometer (SP2) employs the core-shell model to represent coated BC particles, which introduces retrieval errors in the mixing state (Dp/Dc) of BC. We construct fractal models to represent thinly and thickly coated BC particles, and the retrieval errors of the mixing state are investigated from the numerical aspect. We find that errors in Dp/Dc are noteworthy, and the errors in Dp/Dc can further affect the evaluation accuracy of the radiative forcing of BC.
Single-particle soot photometer (SP2) employs the core-shell model to represent coated BC...