Articles | Volume 9, issue 10
https://doi.org/10.5194/amt-9-5227-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-9-5227-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
27 Oct 2016
Research article |
| 27 Oct 2016
Quantification of uncertainties in OCO-2 measurements of XCO2: simulations and linear error analysis
Brian Connor
CORRESPONDING AUTHOR
BC Scientific Consulting, Stony Brook, NY, USA
Hartmut Bösch
EOS Group, Department of Physics and Astronomy, University
of Leicester, Leicester, UK
National Centre for Earth Observation NCEO, University of Leicester,
Leicester, UK
James McDuffie
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Tommy Taylor
Cooperative Institute for Research in the Atmosphere, Fort Collins,
CO, USA
Dejian Fu
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Christian Frankenberg
California Institute of Technology, Pasadena, CA, USA
Chris O'Dell
Cooperative Institute for Research in the Atmosphere, Fort Collins,
CO, USA
Vivienne H. Payne
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Michael Gunson
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Randy Pollock
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Jonathan Hobbs
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Fabiano Oyafuso
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Yibo Jiang
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
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A small percentage of data from the Orbiting Carbon Observatory-3 (OCO-3) instrument has been shown to have a geometry-related bias in the earliest public data release. This work shows that the bias is due to a complex interplay of aerosols and viewing geometry and is largely mitigated in the latest data version through improved bias correction and quality filtering.
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Atmos. Meas. Tech., 15, 5383–5398, https://doi.org/10.5194/amt-15-5383-2022, https://doi.org/10.5194/amt-15-5383-2022, 2022
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Revised manuscript not accepted
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We review the capability of satellite observations of atmospheric methane to quantify methane emissions on all scales. We cover retrieval methods, precision requirements, inverse methods for inferring emissions, source detection thresholds, and observations of system completeness. We show that current instruments already enable quantification of regional and national emissions including contributions from large point sources. Coverage and resolution will increase significantly in coming years.
Vivienne H. Payne, Susan S. Kulawik, Emily V. Fischer, Jared F. Brewer, L. Gregory Huey, Kazuyuki Miyazaki, John R. Worden, Kevin W. Bowman, Eric J. Hintsa, Fred Moore, James W. Elkins, and Julieta Juncosa Calahorrano
Atmos. Meas. Tech., 15, 3497–3511, https://doi.org/10.5194/amt-15-3497-2022, https://doi.org/10.5194/amt-15-3497-2022, 2022
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We compare new satellite measurements of peroxyacetyl nitrate (PAN) with reference aircraft measurements from two different instruments flown on the same platform. While there is a systematic difference between the two aircraft datasets, both show the same large-scale distribution of PAN and the discrepancy between aircraft datasets is small compared to the satellite uncertainties. The satellite measurements show skill in capturing large-scale variations in PAN.
Russell Doughty, Thomas P. Kurosu, Nicholas Parazoo, Philipp Köhler, Yujie Wang, Ying Sun, and Christian Frankenberg
Earth Syst. Sci. Data, 14, 1513–1529, https://doi.org/10.5194/essd-14-1513-2022, https://doi.org/10.5194/essd-14-1513-2022, 2022
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We describe and compare solar-induced chlorophyll fluorescence data produced by NASA from the Greenhouse Gases Observing Satellite (GOSAT) and the Orbiting Carbon Observatory-2 (OCO-2) and OCO-3 platforms.
Johannes Gensheimer, Alexander J. Turner, Philipp Köhler, Christian Frankenberg, and Jia Chen
Biogeosciences, 19, 1777–1793, https://doi.org/10.5194/bg-19-1777-2022, https://doi.org/10.5194/bg-19-1777-2022, 2022
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We develop a convolutional neural network, named SIFnet, that increases the spatial resolution of SIF from TROPOMI by a factor of 10 to a spatial resolution of 0.005°. SIFnet utilizes coarse SIF observations, together with a broad range of high-resolution auxiliary data. The insights gained from interpretable machine learning techniques allow us to make quantitative claims about the relationships between SIF and other common parameters related to photosynthesis.
Vijay Natraj, Ming Luo, Jean-Francois Blavier, Vivienne H. Payne, Derek J. Posselt, Stanley P. Sander, Zhao-Cheng Zeng, Jessica L. Neu, Denis Tremblay, Longtao Wu, Jacola A. Roman, Yen-Hung Wu, and Leonard I. Dorsky
Atmos. Meas. Tech., 15, 1251–1267, https://doi.org/10.5194/amt-15-1251-2022, https://doi.org/10.5194/amt-15-1251-2022, 2022
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High-fidelity monitoring and forecast of air quality and the hydrological cycle require understanding the vertical distribution of temperature, humidity, and trace gases at high spatiotemporal resolution. We describe a new instrument concept, called the JPL GEO-IR Sounder, that would provide this information for the first time from a single instrument platform. Simulations demonstrate the benefits of combining measurements from multiple wavelengths for this purpose from geostationary orbit.
Thomas E. Taylor, Christopher W. O'Dell, David Crisp, Akhiko Kuze, Hannakaisa Lindqvist, Paul O. Wennberg, Abhishek Chatterjee, Michael Gunson, Annmarie Eldering, Brendan Fisher, Matthäus Kiel, Robert R. Nelson, Aronne Merrelli, Greg Osterman, Frédéric Chevallier, Paul I. Palmer, Liang Feng, Nicholas M. Deutscher, Manvendra K. Dubey, Dietrich G. Feist, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Cheng Liu, Martine De Mazière, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Matthias Schneider, Coleen M. Roehl, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Mihalis Vrekoussis, Thorsten Warneke, and Debra Wunch
Earth Syst. Sci. Data, 14, 325–360, https://doi.org/10.5194/essd-14-325-2022, https://doi.org/10.5194/essd-14-325-2022, 2022
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We provide an analysis of an 11-year record of atmospheric carbon dioxide (CO2) concentrations derived using an optimal estimation retrieval algorithm on measurements made by the GOSAT satellite. The new product (version 9) shows improvement over the previous version (v7.3) as evaluated against independent estimates of CO2 from ground-based sensors and atmospheric inversion systems. We also compare the new GOSAT CO2 values to collocated estimates from NASA's Orbiting Carbon Observatory-2.
Hélène Peiro, Sean Crowell, Andrew Schuh, David F. Baker, Chris O'Dell, Andrew R. Jacobson, Frédéric Chevallier, Junjie Liu, Annmarie Eldering, David Crisp, Feng Deng, Brad Weir, Sourish Basu, Matthew S. Johnson, Sajeev Philip, and Ian Baker
Atmos. Chem. Phys., 22, 1097–1130, https://doi.org/10.5194/acp-22-1097-2022, https://doi.org/10.5194/acp-22-1097-2022, 2022
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Satellite CO2 observations are constantly improved. We study an ensemble of different atmospheric models (inversions) from 2015 to 2018 using separate ground-based data or two versions of the OCO-2 satellite. Our study aims to determine if different satellite data corrections can yield different estimates of carbon cycle flux. A difference in the carbon budget between the two versions is found over tropical Africa, which seems to show the impact of corrections applied in satellite data.
Jennifer D. Hegarty, Karen E. Cady-Pereira, Vivienne H. Payne, Susan S. Kulawik, John R. Worden, Valentin Kantchev, Helen M. Worden, Kathryn McKain, Jasna V. Pittman, Róisín Commane, Bruce C. Daube Jr., and Eric A. Kort
Atmos. Meas. Tech., 15, 205–223, https://doi.org/10.5194/amt-15-205-2022, https://doi.org/10.5194/amt-15-205-2022, 2022
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Carbon monoxide (CO) is produced by combustion of substances such as fossil fuels and plays an important role in atmospheric pollution and climate. We evaluated estimates of atmospheric CO derived from outgoing radiation measurements of the Atmospheric Infrared Sounder (AIRS) on a satellite orbiting the Earth against CO measurements from aircraft to show that these satellite measurements are reliable for continuous global monitoring of atmospheric CO concentrations.
Yujie Wang and Christian Frankenberg
Biogeosciences, 19, 29–45, https://doi.org/10.5194/bg-19-29-2022, https://doi.org/10.5194/bg-19-29-2022, 2022
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Modeling vegetation canopy is important in predicting whether the land remains a carbon sink to mitigate climate change in the near future. Vegetation canopy model complexity, however, impacts the model-predicted carbon and water fluxes as well as canopy fluorescence, even if the same suite of model inputs is used. Given the biases caused by canopy model complexity, we recommend not misusing parameters inverted using different models or assumptions.
Alexander J. Turner, Philipp Köhler, Troy S. Magney, Christian Frankenberg, Inez Fung, and Ronald C. Cohen
Biogeosciences, 18, 6579–6588, https://doi.org/10.5194/bg-18-6579-2021, https://doi.org/10.5194/bg-18-6579-2021, 2021
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This work builds a high-resolution estimate (500 m) of gross primary productivity (GPP) over the US using satellite measurements of solar-induced chlorophyll fluorescence (SIF) from the TROPOspheric Monitoring Instrument (TROPOMI) between 2018 and 2020. We identify ecosystem-specific scaling factors for estimating gross primary productivity (GPP) from TROPOMI SIF. Extreme precipitation events drive four regional GPP anomalies that account for 28 % of year-to-year GPP differences across the US.
Siraput Jongaramrungruang, Georgios Matheou, Andrew K. Thorpe, Zhao-Cheng Zeng, and Christian Frankenberg
Atmos. Meas. Tech., 14, 7999–8017, https://doi.org/10.5194/amt-14-7999-2021, https://doi.org/10.5194/amt-14-7999-2021, 2021
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This study shows how precision error and bias in column methane retrieval change with different instrument specifications and the impact of spectrally complex surface albedos on retrievals. We show how surface interferences can be mitigated with an optimal spectral resolution and a higher polynomial degree in a retrieval process. The findings can inform future satellite instrument designs to have robust observations capable of separating real CH4 plume enhancements from surface interferences.
Joseph Mendonca, Ray Nassar, Christopher W. O'Dell, Rigel Kivi, Isamu Morino, Justus Notholt, Christof Petri, Kimberly Strong, and Debra Wunch
Atmos. Meas. Tech., 14, 7511–7524, https://doi.org/10.5194/amt-14-7511-2021, https://doi.org/10.5194/amt-14-7511-2021, 2021
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Machine learning has become an important tool for pattern recognition in many applications. In this study, we used a neural network to improve the data quality of OCO-2 measurements made at northern high latitudes. The neural network was trained and used as a binary classifier to filter out bad OCO-2 measurements in order to increase the accuracy and precision of OCO-2 XCO2 measurements in the Boreal and Arctic regions.
Luis Guanter, Cédric Bacour, Andreas Schneider, Ilse Aben, Tim A. van Kempen, Fabienne Maignan, Christian Retscher, Philipp Köhler, Christian Frankenberg, Joanna Joiner, and Yongguang Zhang
Earth Syst. Sci. Data, 13, 5423–5440, https://doi.org/10.5194/essd-13-5423-2021, https://doi.org/10.5194/essd-13-5423-2021, 2021
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Sun-induced chlorophyll fluorescence (SIF) is an electromagnetic signal emitted by plants in the red and far-red parts of the spectrum. It has a functional link to photosynthesis and can be measured by satellite instruments, which makes it an important variable for the remote monitoring of the photosynthetic activity of vegetation ecosystems around the world. In this contribution we present a SIF dataset derived from the new Sentinel-5P TROPOMI missions.
Yujie Wang, Philipp Köhler, Liyin He, Russell Doughty, Renato K. Braghiere, Jeffrey D. Wood, and Christian Frankenberg
Geosci. Model Dev., 14, 6741–6763, https://doi.org/10.5194/gmd-14-6741-2021, https://doi.org/10.5194/gmd-14-6741-2021, 2021
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We present the first step in testing a new land model as part of a new Earth system model. Our model links plant hydraulics, stomatal optimization theory, and a comprehensive canopy radiation scheme. We compared model-predicted carbon and water fluxes to flux tower observations and model-predicted sun-induced chlorophyll fluorescence to satellite retrievals. Our model quantitatively predicted the carbon and water fluxes as well as the canopy fluorescence yield.
Yi Yin, Frederic Chevallier, Philippe Ciais, Philippe Bousquet, Marielle Saunois, Bo Zheng, John Worden, A. Anthony Bloom, Robert J. Parker, Daniel J. Jacob, Edward J. Dlugokencky, and Christian Frankenberg
Atmos. Chem. Phys., 21, 12631–12647, https://doi.org/10.5194/acp-21-12631-2021, https://doi.org/10.5194/acp-21-12631-2021, 2021
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The growth of methane, the second-most important anthropogenic greenhouse gas after carbon dioxide, has been accelerating in recent years. Using an ensemble of multi-tracer atmospheric inversions constrained by surface or satellite observations, we show that global methane emissions increased by nearly 1 % per year from 2010–2017, with leading contributions from the tropics and East Asia.
Michael Buchwitz, Maximilian Reuter, Stefan Noël, Klaus Bramstedt, Oliver Schneising, Michael Hilker, Blanca Fuentes Andrade, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hartmut Boesch, Lianghai Wu, Jochen Landgraf, Ilse Aben, Christian Retscher, Christopher W. O'Dell, and David Crisp
Atmos. Meas. Tech., 14, 2141–2166, https://doi.org/10.5194/amt-14-2141-2021, https://doi.org/10.5194/amt-14-2141-2021, 2021
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The COVID-19 pandemic resulted in reduced anthropogenic carbon dioxide (CO2) emissions during 2020 in large parts of the world. We have used a small ensemble of satellite retrievals of column-averaged CO2 (XCO2) to find out if a regional-scale reduction of atmospheric CO2 can be detected from space. We focus on East China and show that it is challenging to reliably detect and to accurately quantify the emission reduction, which only results in regional XCO2 reductions of about 0.1–0.2 ppm.
Steven T. Massie, Heather Cronk, Aronne Merrelli, Christopher O'Dell, K. Sebastian Schmidt, Hong Chen, and David Baker
Atmos. Meas. Tech., 14, 1475–1499, https://doi.org/10.5194/amt-14-1475-2021, https://doi.org/10.5194/amt-14-1475-2021, 2021
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The OCO-2 science team is working to retrieve CO2 measurements that can be used by the carbon cycle community to calculate regional sources and sinks of CO2. The retrieved data, however, are in need of improvements in accuracy. This paper discusses several ways in which 3D cloud metrics (such as the distance of a measurement to the nearest cloud) can be used to account for cloud effects in the OCO-2 CO2 data files.
Jakob Borchardt, Konstantin Gerilowski, Sven Krautwurst, Heinrich Bovensmann, Andrew K. Thorpe, David R. Thompson, Christian Frankenberg, Charles E. Miller, Riley M. Duren, and John Philip Burrows
Atmos. Meas. Tech., 14, 1267–1291, https://doi.org/10.5194/amt-14-1267-2021, https://doi.org/10.5194/amt-14-1267-2021, 2021
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The AVIRIS-NG hyperspectral imager has been used successfully to identify and quantify anthropogenic methane sources utilizing different retrieval and inversion methods. Here, we examine the adaption and application of the WFM-DOAS algorithm to AVIRIS-NG measurements to retrieve local methane column enhancements, compare the results with other retrievals, and quantify the uncertainties resulting from the retrieval method. Additionally, we estimate emissions from five detected methane plumes.
Susan S. Kulawik, John R. Worden, Vivienne H. Payne, Dejian Fu, Steven C. Wofsy, Kathryn McKain, Colm Sweeney, Bruce C. Daube Jr., Alan Lipton, Igor Polonsky, Yuguang He, Karen E. Cady-Pereira, Edward J. Dlugokencky, Daniel J. Jacob, and Yi Yin
Atmos. Meas. Tech., 14, 335–354, https://doi.org/10.5194/amt-14-335-2021, https://doi.org/10.5194/amt-14-335-2021, 2021
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This paper shows comparisons of a new single-footprint methane product from the AIRS satellite to aircraft-based observations. We show that this AIRS methane product provides useful information to study seasonal and global methane trends of this important greenhouse gas.
Robert R. Nelson, Annmarie Eldering, David Crisp, Aronne J. Merrelli, and Christopher W. O'Dell
Atmos. Meas. Tech., 13, 6889–6899, https://doi.org/10.5194/amt-13-6889-2020, https://doi.org/10.5194/amt-13-6889-2020, 2020
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Measurements of surface wind speed over oceans are scientifically useful. Here we show that the Orbiting Carbon Observatory-2 (OCO-2), originally designed to measure carbon dioxide using reflected sunlight, can also accurately and precisely measure wind speed. OCO-2's high spatial resolution means that it can observe close to coastlines and therefore be used to study coastal wind processes and inform related economic sectors.
Nicole Jacobs, William R. Simpson, Debra Wunch, Christopher W. O'Dell, Gregory B. Osterman, Frank Hase, Thomas Blumenstock, Qiansi Tu, Matthias Frey, Manvendra K. Dubey, Harrison A. Parker, Rigel Kivi, and Pauli Heikkinen
Atmos. Meas. Tech., 13, 5033–5063, https://doi.org/10.5194/amt-13-5033-2020, https://doi.org/10.5194/amt-13-5033-2020, 2020
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The boreal forest is the largest seasonally varying biospheric CO2-exchange region on Earth. This region is also undergoing amplified climate warming, leading to concerns about the potential for altered regional carbon exchange. Satellite missions, such as the Orbiting Carbon Observatory-2 (OCO-2) project, can measure CO2 abundance over the boreal forest but need validation for the assurance of accuracy. Therefore, we carried out a ground-based validation of OCO-2 CO2 data at three locations.
Kazuyuki Miyazaki, Kevin Bowman, Takashi Sekiya, Henk Eskes, Folkert Boersma, Helen Worden, Nathaniel Livesey, Vivienne H. Payne, Kengo Sudo, Yugo Kanaya, Masayuki Takigawa, and Koji Ogochi
Earth Syst. Sci. Data, 12, 2223–2259, https://doi.org/10.5194/essd-12-2223-2020, https://doi.org/10.5194/essd-12-2223-2020, 2020
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This study presents the results from the Tropospheric Chemistry Reanalysis version 2 (TCR-2) for 2005–2018 obtained from the assimilation of multiple satellite measurements of ozone, CO, NO2, HNO3, and SO2 from the OMI, SCIAMACHY, GOME-2, TES, MLS, and MOPITT instruments. The evaluation results demonstrate the capability of the reanalysis products to improve understanding of the processes controlling variations in atmospheric composition, including long-term changes in air quality and emissions.
Mark Richardson, Matthew D. Lebsock, James McDuffie, and Graeme L. Stephens
Atmos. Meas. Tech., 13, 4947–4961, https://doi.org/10.5194/amt-13-4947-2020, https://doi.org/10.5194/amt-13-4947-2020, 2020
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We previously combined CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) lidar data and reflected-sunlight measurements from OCO-2 (Orbiting Carbon Observatory 2) for information about low clouds over oceans. The satellites are no longer formation-flying, so this work is a step towards getting new information about these clouds using only OCO-2. We can rapidly and accurately identify liquid oceanic clouds and obtain their height better than a widely used passive sensor.
Rui Cheng, Troy S. Magney, Debsunder Dutta, David R. Bowling, Barry A. Logan, Sean P. Burns, Peter D. Blanken, Katja Grossmann, Sophia Lopez, Andrew D. Richardson, Jochen Stutz, and Christian Frankenberg
Biogeosciences, 17, 4523–4544, https://doi.org/10.5194/bg-17-4523-2020, https://doi.org/10.5194/bg-17-4523-2020, 2020
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We measured reflected sunlight from an evergreen canopy for a year to detect changes in pigments that play an important role in regulating the seasonality of photosynthesis. Results show a strong mechanistic link between spectral reflectance features and pigment content, which is validated using a biophysical model. Our results show spectrally where, why, and when spectral features change over the course of the season and show promise for estimating photosynthesis remotely.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
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Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Nicholas C. Parazoo, Troy Magney, Alex Norton, Brett Raczka, Cédric Bacour, Fabienne Maignan, Ian Baker, Yongguang Zhang, Bo Qiu, Mingjie Shi, Natasha MacBean, Dave R. Bowling, Sean P. Burns, Peter D. Blanken, Jochen Stutz, Katja Grossmann, and Christian Frankenberg
Biogeosciences, 17, 3733–3755, https://doi.org/10.5194/bg-17-3733-2020, https://doi.org/10.5194/bg-17-3733-2020, 2020
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Satellite measurements of solar-induced chlorophyll fluorescence (SIF) provide a global measure of photosynthetic change. This enables scientists to better track carbon cycle responses to environmental change and tune biochemical processes in vegetation models for an improved simulation of future change. We use tower-instrumented SIF measurements and controlled model experiments to assess the state of the art in terrestrial biosphere SIF modeling and find a wide range of sensitivities to light.
Marielle Saunois, Ann R. Stavert, Ben Poulter, Philippe Bousquet, Josep G. Canadell, Robert B. Jackson, Peter A. Raymond, Edward J. Dlugokencky, Sander Houweling, Prabir K. Patra, Philippe Ciais, Vivek K. Arora, David Bastviken, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Kimberly M. Carlson, Mark Carrol, Simona Castaldi, Naveen Chandra, Cyril Crevoisier, Patrick M. Crill, Kristofer Covey, Charles L. Curry, Giuseppe Etiope, Christian Frankenberg, Nicola Gedney, Michaela I. Hegglin, Lena Höglund-Isaksson, Gustaf Hugelius, Misa Ishizawa, Akihiko Ito, Greet Janssens-Maenhout, Katherine M. Jensen, Fortunat Joos, Thomas Kleinen, Paul B. Krummel, Ray L. Langenfelds, Goulven G. Laruelle, Licheng Liu, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Joe McNorton, Paul A. Miller, Joe R. Melton, Isamu Morino, Jurek Müller, Fabiola Murguia-Flores, Vaishali Naik, Yosuke Niwa, Sergio Noce, Simon O'Doherty, Robert J. Parker, Changhui Peng, Shushi Peng, Glen P. Peters, Catherine Prigent, Ronald Prinn, Michel Ramonet, Pierre Regnier, William J. Riley, Judith A. Rosentreter, Arjo Segers, Isobel J. Simpson, Hao Shi, Steven J. Smith, L. Paul Steele, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Francesco N. Tubiello, Aki Tsuruta, Nicolas Viovy, Apostolos Voulgarakis, Thomas S. Weber, Michiel van Weele, Guido R. van der Werf, Ray F. Weiss, Doug Worthy, Debra Wunch, Yi Yin, Yukio Yoshida, Wenxin Zhang, Zhen Zhang, Yuanhong Zhao, Bo Zheng, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Earth Syst. Sci. Data, 12, 1561–1623, https://doi.org/10.5194/essd-12-1561-2020, https://doi.org/10.5194/essd-12-1561-2020, 2020
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Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. We have established a consortium of multidisciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate new research aimed at improving and regularly updating the global methane budget. This is the second version of the review dedicated to the decadal methane budget, integrating results of top-down and bottom-up estimates.
Gregory Duveiller, Federico Filipponi, Sophia Walther, Philipp Köhler, Christian Frankenberg, Luis Guanter, and Alessandro Cescatti
Earth Syst. Sci. Data, 12, 1101–1116, https://doi.org/10.5194/essd-12-1101-2020, https://doi.org/10.5194/essd-12-1101-2020, 2020
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Sun-induced chlorophyll fluorescence is a valuable indicator of vegetation productivity, but our capacity to measure it from space using satellite remote techniques has been hampered by a lack of spatial detail. Based on prior knowledge of how ecosystems should respond to growing conditions in some modelling along with ancillary satellite observations, we provide here a new enhanced dataset with higher spatial resolution that better represents the spatial patterns of vegetation growth over land.
Robert L. Herman, John Worden, David Noone, Dean Henze, Kevin Bowman, Karen Cady-Pereira, Vivienne H. Payne, Susan S. Kulawik, and Dejian Fu
Atmos. Meas. Tech., 13, 1825–1834, https://doi.org/10.5194/amt-13-1825-2020, https://doi.org/10.5194/amt-13-1825-2020, 2020
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This study is the first assessment and validation of AIRS HDO / H2O retrieved by optimal estimation. Initial comparisons with in situ measurements from NASA ORACLES are promising: the small bias and consistent rms of AIRS suggest that AIRS has well-characterized HDO / H2O. This analysis opens the possibility of a new 17-year long-term data record of global tropospheric HDO / H2O measured from space.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Stefan Noël, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Antonio Di Noia, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Lianghai Wu, Otto P. Hasekamp, Ilse Aben, Akihiko Kuze, Hiroshi Suto, Kei Shiomi, Yukio Yoshida, Isamu Morino, David Crisp, Christopher W. O'Dell, Justus Notholt, Christof Petri, Thorsten Warneke, Voltaire A. Velazco, Nicholas M. Deutscher, David W. T. Griffith, Rigel Kivi, David F. Pollard, Frank Hase, Ralf Sussmann, Yao V. Té, Kimberly Strong, Sébastien Roche, Mahesh K. Sha, Martine De Mazière, Dietrich G. Feist, Laura T. Iraci, Coleen M. Roehl, Christian Retscher, and Dinand Schepers
Atmos. Meas. Tech., 13, 789–819, https://doi.org/10.5194/amt-13-789-2020, https://doi.org/10.5194/amt-13-789-2020, 2020
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We present new satellite-derived data sets of atmospheric carbon dioxide (CO2) and methane (CH4). The data products are column-averaged dry-air mole fractions of CO2 and CH4, denoted XCO2 and XCH4. The products cover the years 2003–2018 and are merged Level 2 (satellite footprints) and merged Level 3 (gridded at monthly time and 5° x 5° spatial resolution) products obtained from combining several individual sensor products. We present the merging algorithms and product validation results.
Alexander J. Turner, Philipp Köhler, Troy S. Magney, Christian Frankenberg, Inez Fung, and Ronald C. Cohen
Biogeosciences, 17, 405–422, https://doi.org/10.5194/bg-17-405-2020, https://doi.org/10.5194/bg-17-405-2020, 2020
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We present the highest resolution solar-induced chlorophyll fluorescence (SIF) dataset from satellite measurements, providing previously unobservable phenomena related to plant photosynthesis. We find a strong correspondence between TROPOMI SIF and AmeriFlux GPP. We then observe a double peak in the seasonality of California's photosynthesis, not seen by traditional vegetation indices (e.g., MODIS). This is further corroborated by EOF/PC analysis.
Siraput Jongaramrungruang, Christian Frankenberg, Georgios Matheou, Andrew K. Thorpe, David R. Thompson, Le Kuai, and Riley M. Duren
Atmos. Meas. Tech., 12, 6667–6681, https://doi.org/10.5194/amt-12-6667-2019, https://doi.org/10.5194/amt-12-6667-2019, 2019
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This paper demonstrates the use of high-resolution 2-D plume imagery from airborne remote sensing retrievals to quantify methane point-source emissions. It shows significant improvements on the flux estimates without the need for direct wind speed measurements. This paves the way for enhanced flux estimates in future field campaign and space-based observations to better understand the magnitude and distribution of various point sources of methane.
Daniel H. Cusworth, Daniel J. Jacob, Daniel J. Varon, Christopher Chan Miller, Xiong Liu, Kelly Chance, Andrew K. Thorpe, Riley M. Duren, Charles E. Miller, David R. Thompson, Christian Frankenberg, Luis Guanter, and Cynthia A. Randles
Atmos. Meas. Tech., 12, 5655–5668, https://doi.org/10.5194/amt-12-5655-2019, https://doi.org/10.5194/amt-12-5655-2019, 2019
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We examine the potential for global detection of methane plumes from individual point sources with the new generation of spaceborne imaging spectrometers scheduled for launch in 2019–2025. We perform methane retrievals on simulated scenes with varying surfaces and atmospheric methane concentrations. Our results suggest that imaging spectrometers in space could play a transformative role in the future for quantifying methane emissions from point sources on a global scale.
Susan S. Kulawik, Chris O'Dell, Robert R. Nelson, and Thomas E. Taylor
Atmos. Meas. Tech., 12, 5317–5334, https://doi.org/10.5194/amt-12-5317-2019, https://doi.org/10.5194/amt-12-5317-2019, 2019
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This work investigates errors in CO2 near-infrared estimates retrieved from simulated radiances. We find that interferent errors are underpredicted and that nonlinearity causes significant errors.
Sean Crowell, David Baker, Andrew Schuh, Sourish Basu, Andrew R. Jacobson, Frederic Chevallier, Junjie Liu, Feng Deng, Liang Feng, Kathryn McKain, Abhishek Chatterjee, John B. Miller, Britton B. Stephens, Annmarie Eldering, David Crisp, David Schimel, Ray Nassar, Christopher W. O'Dell, Tomohiro Oda, Colm Sweeney, Paul I. Palmer, and Dylan B. A. Jones
Atmos. Chem. Phys., 19, 9797–9831, https://doi.org/10.5194/acp-19-9797-2019, https://doi.org/10.5194/acp-19-9797-2019, 2019
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Space-based retrievals of carbon dioxide offer the potential to provide dense data in regions that are sparsely observed by the surface network. We find that flux estimates that are informed by the Orbiting Carbon Observatory-2 (OCO-2) show different character from that inferred using surface measurements in tropical land regions, particularly in Africa, with a much larger total emission and larger amplitude seasonal cycle.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Sven Krautwurst, Christopher W. O'Dell, Andreas Richter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 19, 9371–9383, https://doi.org/10.5194/acp-19-9371-2019, https://doi.org/10.5194/acp-19-9371-2019, 2019
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The quantification of anthropogenic emissions with current CO2 satellite sensors is difficult, but NO2 is co-emitted, making it a suitable tracer of recently emitted CO2. We analyze enhancements of CO2 and NO2 observed by OCO-2 and S5P and estimate the CO2 plume cross-sectional fluxes that we compare with emission databases. Our results demonstrate the usefulness of simultaneous satellite observations of CO2 and NO2 as envisaged for the European Copernicus anthropogenic CO2 monitoring mission
Annmarie Eldering, Thomas E. Taylor, Christopher W. O'Dell, and Ryan Pavlick
Atmos. Meas. Tech., 12, 2341–2370, https://doi.org/10.5194/amt-12-2341-2019, https://doi.org/10.5194/amt-12-2341-2019, 2019
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NASA's Orbiting Carbon Observatory-3 (OCO-3) is scheduled for a 2019 launch to the International Space Station (ISS). It is expected to continue the record of column carbon dioxide (XCO2) and solar-induced chlorophyll fluorescence (SIF) measurements from space used to study and constrain the Earth's carbon cycle. This work highlights the measurement objectives and uses simulated data to show that the expected instrument performance is on par with that of OCO-2.
John R. Worden, Susan S. Kulawik, Dejian Fu, Vivienne H. Payne, Alan E. Lipton, Igor Polonsky, Yuguang He, Karen Cady-Pereira, Jean-Luc Moncet, Robert L. Herman, Fredrick W. Irion, and Kevin W. Bowman
Atmos. Meas. Tech., 12, 2331–2339, https://doi.org/10.5194/amt-12-2331-2019, https://doi.org/10.5194/amt-12-2331-2019, 2019
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In this paper we take the first steps towards generating a multi-decadal record of the deuterium content of water vapor, useful for evaluating the moisture sources and processes affecting water vapor, by estimating the deuterium content from thermal IR radiances from the AIRS instrument. We find the AIRS-based measurements are sensitive to the deuterium content of water vapor in the middle and lower troposphere with a single measurement uncertainty of ~ 3 % and an accuracy of ~ 0.7 %.
Matthäus Kiel, Christopher W. O'Dell, Brendan Fisher, Annmarie Eldering, Ray Nassar, Cameron G. MacDonald, and Paul O. Wennberg
Atmos. Meas. Tech., 12, 2241–2259, https://doi.org/10.5194/amt-12-2241-2019, https://doi.org/10.5194/amt-12-2241-2019, 2019
Robert R. Nelson and Christopher W. O'Dell
Atmos. Meas. Tech., 12, 1495–1512, https://doi.org/10.5194/amt-12-1495-2019, https://doi.org/10.5194/amt-12-1495-2019, 2019
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Accurate measurements of carbon dioxide are essential when studying climate change. In this work, we try to improve measurements of carbon dioxide from the Orbiting Carbon Observatory-2 by using better informed aerosol priors from an atmospheric model. We find that this makes the carbon dioxide measurements slightly more accurate and that certain ways of using modeled aerosol information are more promising than others.
Debsunder Dutta, David S. Schimel, Ying Sun, Christiaan van der Tol, and Christian Frankenberg
Biogeosciences, 16, 77–103, https://doi.org/10.5194/bg-16-77-2019, https://doi.org/10.5194/bg-16-77-2019, 2019
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Canopy structural and leaf photosynthesis parameterizations are often fixed over time in Earth system models and represent large sources of uncertainty in predictions of carbon and water fluxes. We develop a moving window nonlinear optimal parameter inversion framework using constraining flux and satellite reflectance observations. The results demonstrate the applicability of the approach for error reduction and capturing the seasonal variability of key ecosystem parameters.
Christopher W. O'Dell, Annmarie Eldering, Paul O. Wennberg, David Crisp, Michael R. Gunson, Brendan Fisher, Christian Frankenberg, Matthäus Kiel, Hannakaisa Lindqvist, Lukas Mandrake, Aronne Merrelli, Vijay Natraj, Robert R. Nelson, Gregory B. Osterman, Vivienne H. Payne, Thomas E. Taylor, Debra Wunch, Brian J. Drouin, Fabiano Oyafuso, Albert Chang, James McDuffie, Michael Smyth, David F. Baker, Sourish Basu, Frédéric Chevallier, Sean M. R. Crowell, Liang Feng, Paul I. Palmer, Mavendra Dubey, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, Coleen M. Roehl, Mahesh K. Sha, Kimberly Strong, Ralf Sussmann, Yao Te, Osamu Uchino, and Voltaire A. Velazco
Atmos. Meas. Tech., 11, 6539–6576, https://doi.org/10.5194/amt-11-6539-2018, https://doi.org/10.5194/amt-11-6539-2018, 2018
Michael Buchwitz, Maximilian Reuter, Oliver Schneising, Stefan Noël, Bettina Gier, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Akihiko Kuze, Hiroshi Suto, Yukio Yoshida, David Crisp, and Christopher O'Dell
Atmos. Chem. Phys., 18, 17355–17370, https://doi.org/10.5194/acp-18-17355-2018, https://doi.org/10.5194/acp-18-17355-2018, 2018
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We present a new satellite data set of column-averaged mixing ratios of carbon dioxide (CO2), which covers the time period 2003 to 2016. We used this data set to compute annual mean atmospheric CO2 growth rates. We show that the growth rate is highest during 2015 and 2016 despite nearly constant CO2 emissions from fossil fuel burning in recent years. The high growth rates are attributed to year 2015-2016 El Nino episodes. We present correlations with fossil fuel emissions and ENSO indices.
Dejian Fu, Susan S. Kulawik, Kazuyuki Miyazaki, Kevin W. Bowman, John R. Worden, Annmarie Eldering, Nathaniel J. Livesey, Joao Teixeira, Fredrick W. Irion, Robert L. Herman, Gregory B. Osterman, Xiong Liu, Pieternel F. Levelt, Anne M. Thompson, and Ming Luo
Atmos. Meas. Tech., 11, 5587–5605, https://doi.org/10.5194/amt-11-5587-2018, https://doi.org/10.5194/amt-11-5587-2018, 2018
Anand K. Ramanathan, Hai M. Nguyen, Xiaoli Sun, Jianping Mao, James B. Abshire, Jonathan M. Hobbs, and Amy J. Braverman
Atmos. Meas. Tech., 11, 4909–4928, https://doi.org/10.5194/amt-11-4909-2018, https://doi.org/10.5194/amt-11-4909-2018, 2018
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Remote sensing of greenhouse gases (GHG) such as CO2 and CH4 in the atmosphere from space is important for studying emissions and the carbon cycle. Present-day techniques measure the absorption of light passing through the atmosphere and determine the column-averaged gas concentration in the atmosphere. Here, we draw from a well-known singular value decomposition (SVD) framework to develop a technique of extracting information about the GHG concentration profile from the column absorption.
Pieternel F. Levelt, Joanna Joiner, Johanna Tamminen, J. Pepijn Veefkind, Pawan K. Bhartia, Deborah C. Stein Zweers, Bryan N. Duncan, David G. Streets, Henk Eskes, Ronald van der A, Chris McLinden, Vitali Fioletov, Simon Carn, Jos de Laat, Matthew DeLand, Sergey Marchenko, Richard McPeters, Jerald Ziemke, Dejian Fu, Xiong Liu, Kenneth Pickering, Arnoud Apituley, Gonzalo González Abad, Antti Arola, Folkert Boersma, Christopher Chan Miller, Kelly Chance, Martin de Graaf, Janne Hakkarainen, Seppo Hassinen, Iolanda Ialongo, Quintus Kleipool, Nickolay Krotkov, Can Li, Lok Lamsal, Paul Newman, Caroline Nowlan, Raid Suleiman, Lieuwe Gijsbert Tilstra, Omar Torres, Huiqun Wang, and Krzysztof Wargan
Atmos. Chem. Phys., 18, 5699–5745, https://doi.org/10.5194/acp-18-5699-2018, https://doi.org/10.5194/acp-18-5699-2018, 2018
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The aim of this paper is to highlight the many successes of the Ozone Monitoring Instrument (OMI) spanning more than 13 years. Data from OMI have been used in a wide range of applications. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI plays a unique role in measuring trace gases important for the ozone layer, air quality, and climate change. OMI data continue to be used for new research and applications.
Emily V. Fischer, Liye Zhu, Vivienne H. Payne, John R. Worden, Zhe Jiang, Susan S. Kulawik, Steven Brey, Arsineh Hecobian, Daniel Gombos, Karen Cady-Pereira, and Frank Flocke
Atmos. Chem. Phys., 18, 5639–5653, https://doi.org/10.5194/acp-18-5639-2018, https://doi.org/10.5194/acp-18-5639-2018, 2018
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PAN is an atmospheric reservoir for nitrogen oxide radicals, and it plays a lead role in their redistribution in the troposphere. We analyze new Tropospheric Emission Spectrometer (TES) PAN observations over North America during July 2006 to 2009. We identify smoke-impacted TES PAN retrievals by co-location with NOAA Hazard Mapping System (HMS) smoke plumes. Depending on the year, 15–32 % of cases where elevated PAN is identified in TES observations overlap with smoke plumes.
Fredrick W. Irion, Brian H. Kahn, Mathias M. Schreier, Eric J. Fetzer, Evan Fishbein, Dejian Fu, Peter Kalmus, R. Chris Wilson, Sun Wong, and Qing Yue
Atmos. Meas. Tech., 11, 971–995, https://doi.org/10.5194/amt-11-971-2018, https://doi.org/10.5194/amt-11-971-2018, 2018
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We describe a new algorithm for the Atmospheric Infrared Sounder (AIRS) that uses its thermal infrared spectra directly rather than using “cloud-clearing.” By additionally modelling clouds within an AIRS field-of-view, we retrieve temperature and water vapor profiles on the AIRS ~13.5 km horizontal footprint (at nadir) rather than the ~45 km footprint of cloud-cleared spectra. Initial validation is presented, and avenues for future development are discussed.
David F. Pollard, Vanessa Sherlock, John Robinson, Nicholas M. Deutscher, Brian Connor, and Hisako Shiona
Earth Syst. Sci. Data, 9, 977–992, https://doi.org/10.5194/essd-9-977-2017, https://doi.org/10.5194/essd-9-977-2017, 2017
Andrew K. Thorpe, Christian Frankenberg, David R. Thompson, Riley M. Duren, Andrew D. Aubrey, Brian D. Bue, Robert O. Green, Konstantin Gerilowski, Thomas Krings, Jakob Borchardt, Eric A. Kort, Colm Sweeney, Stephen Conley, Dar A. Roberts, and Philip E. Dennison
Atmos. Meas. Tech., 10, 3833–3850, https://doi.org/10.5194/amt-10-3833-2017, https://doi.org/10.5194/amt-10-3833-2017, 2017
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At local scales emissions of methane (CH4) and carbon dioxide (CO2) are highly uncertain. The AVIRIS-NG imaging spectrometer maps large regions and generates high-spatial-resolution CH4 and CO2 concentration maps from anthropogenic and natural sources. Examples include CH4 from a processing plant, tank, pipeline leak, seep, mine vent shafts, and CO2 from power plants. This demonstrates a greenhouse gas monitoring capability that targets the two dominant anthropogenic climate-forcing agents.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Ray Weiss, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Atmos. Chem. Phys., 17, 11135–11161, https://doi.org/10.5194/acp-17-11135-2017, https://doi.org/10.5194/acp-17-11135-2017, 2017
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Following the Global Methane Budget 2000–2012 published in Saunois et al. (2016), we use the same dataset of bottom-up and top-down approaches to discuss the variations in methane emissions over the period 2000–2012. The changes in emissions are discussed both in terms of trends and quasi-decadal changes. The ensemble gathered here allows us to synthesise the robust changes in terms of regional and sectorial contributions to the increasing methane emissions.
Debora Griffin, Kaley A. Walker, Stephanie Conway, Felicia Kolonjari, Kimberly Strong, Rebecca Batchelor, Chris D. Boone, Lin Dan, James R. Drummond, Pierre F. Fogal, Dejian Fu, Rodica Lindenmaier, Gloria L. Manney, and Dan Weaver
Atmos. Meas. Tech., 10, 3273–3294, https://doi.org/10.5194/amt-10-3273-2017, https://doi.org/10.5194/amt-10-3273-2017, 2017
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Measurements in the high Arctic from two ground-based and one space-borne infrared Fourier transform spectrometer agree well over an 8-year time period (2006–2013). These comparisons show no notable degradation, indicating the consistency of these data sets and suggesting that the space-borne measurements have been stable. Increasing ozone, as well as increases of some other atmospheric gases, has been found over this same time period.
Karen E. Cady-Pereira, Vivienne H. Payne, Jessica L. Neu, Kevin W. Bowman, Kazuyuki Miyazaki, Eloise A. Marais, Susan Kulawik, Zitely A. Tzompa-Sosa, and Jennifer D. Hegarty
Atmos. Chem. Phys., 17, 9379–9398, https://doi.org/10.5194/acp-17-9379-2017, https://doi.org/10.5194/acp-17-9379-2017, 2017
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Air quality is a major issue for megacities. Our paper looks at satellite measurements over Mexico City and Lagos of several trace gases gases related to air quality to determine the temporal and spatial variability of these gases, and it relates this variability to local conditions, such as topography, winds and biomass burning events. We find that, while Mexico City is known for severe pollution events, the levels of of pollution in Lagos are much higher and more persistent.
John R. Worden, Gary Doran, Susan Kulawik, Annmarie Eldering, David Crisp, Christian Frankenberg, Chris O'Dell, and Kevin Bowman
Atmos. Meas. Tech., 10, 2759–2771, https://doi.org/10.5194/amt-10-2759-2017, https://doi.org/10.5194/amt-10-2759-2017, 2017
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This paper evaluates the uncertainties of the total column carbon dioxide (XCO2) measurements from the NASA OCO-2 instrument by comparing observed variations in small geographical regions to the calculated uncertainties of the data within this region. In general we find that the reported XCO2 precision is related to that expected from the XCO2 radiance noise. However, the reported accuracy is at least smaller than the actual accuracy by a factor of 2–4.
Zhe Jiang, Helen Worden, John R. Worden, Daven K. Henze, Dylan B. A. Jones, Avelino F. Arellano, Emily V. Fischer, Liye Zhu, Kazuyuki Miyazaki, K. Folkert Boersma, and Vivienne H. Payne
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-382, https://doi.org/10.5194/acp-2017-382, 2017
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We investigated the variation of US tropospheric NO2 in the past decade. We demonstrated significant divergence between the time variation in tropospheric NO2 columns from OMI retrievals and surface measurements. Our analysis suggests limited contributions from local effects such as fossil fuel emissions, lightning, or instrument artifacts, and indicates possible important contributions from long-range transport of Asian emissions that are modulated by ENSO.
Vivienne H. Payne, Emily V. Fischer, John R. Worden, Zhe Jiang, Liye Zhu, Thomas P. Kurosu, and Susan S. Kulawik
Atmos. Chem. Phys., 17, 6341–6351, https://doi.org/10.5194/acp-17-6341-2017, https://doi.org/10.5194/acp-17-6341-2017, 2017
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Peroxyacetyl nitrate (PAN) plays a key role in atmospheric chemistry and long-range transport of pollution. In this paper, we present measurements of PAN from the Tropospheric Emission Spectrometer, an instrument on board the NASA Aura satellite since 2004. We focus on measurements of PAN in tropical regions, where data from ground-based and aircraft campaigns are particularly sparse. We observe temporal changes in PAN associated with changes in fires, convection and emissions.
Robert L. Herman, Eric A. Ray, Karen H. Rosenlof, Kristopher M. Bedka, Michael J. Schwartz, William G. Read, Robert F. Troy, Keith Chin, Lance E. Christensen, Dejian Fu, Robert A. Stachnik, T. Paul Bui, and Jonathan M. Dean-Day
Atmos. Chem. Phys., 17, 6113–6124, https://doi.org/10.5194/acp-17-6113-2017, https://doi.org/10.5194/acp-17-6113-2017, 2017
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This study reports new aircraft field observations of elevated water vapor greater than 10 ppmv in the overworld stratosphere over the summertime continental US. Back trajectories from the flight track intersect overshooting convective tops within the previous 1 to 7 days, suggesting that ice is convectively and irreversibly transported to the stratosphere in the most energetic overshooting convective events. Satellite measurements (Aura MLS) indicate that such events are uncommon (< 1 %).
Michael Buchwitz, Oliver Schneising, Maximilian Reuter, Jens Heymann, Sven Krautwurst, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Christian Frankenberg, and Alexander J. Turner
Atmos. Chem. Phys., 17, 5751–5774, https://doi.org/10.5194/acp-17-5751-2017, https://doi.org/10.5194/acp-17-5751-2017, 2017
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Methane is an important greenhouse gas and increasing atmospheric concentrations result in global warming. We present a simple method to derive annual methane emission estimates of methane hotspot areas from satellite data. We present results for four source areas. We found that our estimates are in good agreement with other studies/data sets for the Four Corners region in the USA and for Azerbaijan but we also found higher emissions for parts of California and Turkmenistan.
Min Huang, Gregory R. Carmichael, R. Bradley Pierce, Duseong S. Jo, Rokjin J. Park, Johannes Flemming, Louisa K. Emmons, Kevin W. Bowman, Daven K. Henze, Yanko Davila, Kengo Sudo, Jan Eiof Jonson, Marianne Tronstad Lund, Greet Janssens-Maenhout, Frank J. Dentener, Terry J. Keating, Hilke Oetjen, and Vivienne H. Payne
Atmos. Chem. Phys., 17, 5721–5750, https://doi.org/10.5194/acp-17-5721-2017, https://doi.org/10.5194/acp-17-5721-2017, 2017
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In support of the HTAP phase 2 experiment, we conducted a number of regional-scale Sulfur Transport and dEposition Model base and sensitivity simulations over North America during May–June 2010. The STEM chemical boundary conditions were downscaled from three (GEOS-Chem, RAQMS, and ECMWF C-IFS) global chemical transport models' simulations. Analyses were performed on large spatial–temporal scales relative to HTAP1 and also on subcontinental and event scales including the use of satellite data.
Susan S. Kulawik, Chris O'Dell, Vivienne H. Payne, Le Kuai, Helen M. Worden, Sebastien C. Biraud, Colm Sweeney, Britton Stephens, Laura T. Iraci, Emma L. Yates, and Tomoaki Tanaka
Atmos. Chem. Phys., 17, 5407–5438, https://doi.org/10.5194/acp-17-5407-2017, https://doi.org/10.5194/acp-17-5407-2017, 2017
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We introduce new vertically resolved GOSAT products that better separate locally and remotely influenced CO2. Current GOSAT column results for CO2 (XCO2) are sensitive to fluxes on continental scales, whereas flux estimates from surface and tower measurements are affected by sampling bias and model transport uncertainty. These new GOSAT measurements of boundary layer CO2 are validated against aircraft and surface observations of CO2 and are compared to vertically resolved MOPITT CO.
Kang Sun, Xiong Liu, Caroline R. Nowlan, Zhaonan Cai, Kelly Chance, Christian Frankenberg, Richard A. M. Lee, Randy Pollock, Robert Rosenberg, and David Crisp
Atmos. Meas. Tech., 10, 939–953, https://doi.org/10.5194/amt-10-939-2017, https://doi.org/10.5194/amt-10-939-2017, 2017
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Accurately characterizing the instrument line shape (ILS) of the Orbiting Carbon Observatory-2 (OCO-2) is challenging and highly important due to its high spectral resolution and requirement for retrieval accuracy. Measured ILS during preflight experiments has been used in the OCO-2 CO2 retrieval. This study derives the on-orbit ILS of OCO-2 using its solar measurements and answers the questions whether on-orbit ILS has changed compared to preflight and whether it varies during the mission.
Zhao-Cheng Zeng, Qiong Zhang, Vijay Natraj, Jack S. Margolis, Run-Lie Shia, Sally Newman, Dejian Fu, Thomas J. Pongetti, Kam W. Wong, Stanley P. Sander, Paul O. Wennberg, and Yuk L. Yung
Atmos. Chem. Phys., 17, 2495–2508, https://doi.org/10.5194/acp-17-2495-2017, https://doi.org/10.5194/acp-17-2495-2017, 2017
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We propose a novel approach to describing the scattering effects of atmospheric aerosols using H2O retrievals in the near infrared. We found that the aerosol scattering effect is the primary contributor to the variations in the wavelength dependence of the H2O SCD retrievals and the scattering effects can be derived using H2O retrievals from multiple bands. This proposed method could potentially contribute towards reducing biases in greenhouse gas retrievals from space.
Annmarie Eldering, Chris W. O'Dell, Paul O. Wennberg, David Crisp, Michael R. Gunson, Camille Viatte, Charles Avis, Amy Braverman, Rebecca Castano, Albert Chang, Lars Chapsky, Cecilia Cheng, Brian Connor, Lan Dang, Gary Doran, Brendan Fisher, Christian Frankenberg, Dejian Fu, Robert Granat, Jonathan Hobbs, Richard A. M. Lee, Lukas Mandrake, James McDuffie, Charles E. Miller, Vicky Myers, Vijay Natraj, Denis O'Brien, Gregory B. Osterman, Fabiano Oyafuso, Vivienne H. Payne, Harold R. Pollock, Igor Polonsky, Coleen M. Roehl, Robert Rosenberg, Florian Schwandner, Mike Smyth, Vivian Tang, Thomas E. Taylor, Cathy To, Debra Wunch, and Jan Yoshimizu
Atmos. Meas. Tech., 10, 549–563, https://doi.org/10.5194/amt-10-549-2017, https://doi.org/10.5194/amt-10-549-2017, 2017
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This paper describes the measurements of atmospheric carbon dioxide collected in the first 18 months of the satellite mission known as the Orbiting Carbon Observatory-2 (OCO-2). The paper shows maps of the carbon dioxide data, data density, and other data fields that illustrate the data quality. This mission has collected a more precise, more dense dataset of carbon dioxide then we have ever had previously.
David Crisp, Harold R. Pollock, Robert Rosenberg, Lars Chapsky, Richard A. M. Lee, Fabiano A. Oyafuso, Christian Frankenberg, Christopher W. O'Dell, Carol J. Bruegge, Gary B. Doran, Annmarie Eldering, Brendan M. Fisher, Dejian Fu, Michael R. Gunson, Lukas Mandrake, Gregory B. Osterman, Florian M. Schwandner, Kang Sun, Tommy E. Taylor, Paul O. Wennberg, and Debra Wunch
Atmos. Meas. Tech., 10, 59–81, https://doi.org/10.5194/amt-10-59-2017, https://doi.org/10.5194/amt-10-59-2017, 2017
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The Orbiting Carbon Observatory-2 carries and points a three-channel imaging grating spectrometer designed to collect high-resolution spectra of reflected sunlight within the molecular oxygen A-band at 0.765 microns and the carbon dioxide bands at 1.61 and 2.06 microns. Here, we describe the OCO-2 instrument, its data products, and its performance during its first 18 months in orbit.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Victor Brovkin, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Charles Curry, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Julia Marshall, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Catherine Prigent, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Paul Steele, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Michiel van Weele, Guido R. van der Werf, Ray Weiss, Christine Wiedinmyer, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Earth Syst. Sci. Data, 8, 697–751, https://doi.org/10.5194/essd-8-697-2016, https://doi.org/10.5194/essd-8-697-2016, 2016
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An accurate assessment of the methane budget is important to understand the atmospheric methane concentrations and trends and to provide realistic pathways for climate change mitigation. The various and diffuse sources of methane as well and its oxidation by a very short lifetime radical challenge this assessment. We quantify the methane sources and sinks as well as their uncertainties based on both bottom-up and top-down approaches provided by a broad international scientific community.
Daniel J. Jacob, Alexander J. Turner, Joannes D. Maasakkers, Jianxiong Sheng, Kang Sun, Xiong Liu, Kelly Chance, Ilse Aben, Jason McKeever, and Christian Frankenberg
Atmos. Chem. Phys., 16, 14371–14396, https://doi.org/10.5194/acp-16-14371-2016, https://doi.org/10.5194/acp-16-14371-2016, 2016
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Methane is a greenhouse gas emitted by a range of natural and anthropogenic sources. Atmospheric methane has been measured continuously from space since 2003, and new instruments are planned to launch in the near future that will greatly expand the capabilities of space-based observations. We review the value of current, future, and proposed satellite observations to better quantify methane emissions from the global scale down to the scale of point sources.
Zeli Tan, Qianlai Zhuang, Daven K. Henze, Christian Frankenberg, Ed Dlugokencky, Colm Sweeney, Alexander J. Turner, Motoki Sasakawa, and Toshinobu Machida
Atmos. Chem. Phys., 16, 12649–12666, https://doi.org/10.5194/acp-16-12649-2016, https://doi.org/10.5194/acp-16-12649-2016, 2016
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Methane emissions from the pan-Arctic could be important in understanding the global carbon cycle but are still poorly constrained to date. This study demonstrated that satellite retrievals can be used to reduce the uncertainty of the estimates of these emissions. We also provided additional evidence for the existence of large methane emissions from pan-Arctic lakes in the Siberian yedoma permafrost region. We found that biogeochemical models should be improved for better estimates.
Gerald E. Nedoluha, Brian J. Connor, Thomas Mooney, James W. Barrett, Alan Parrish, R. Michael Gomez, Ian Boyd, Douglas R. Allen, Michael Kotkamp, Stefanie Kremser, Terry Deshler, Paul Newman, and Michelle L. Santee
Atmos. Chem. Phys., 16, 10725–10734, https://doi.org/10.5194/acp-16-10725-2016, https://doi.org/10.5194/acp-16-10725-2016, 2016
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Chlorine monoxide (ClO) is central to the formation of the springtime Antarctic ozone hole since it is the catalytic agent in the most important ozone-depleting chemical cycle. We present 20 years of measurements of ClO from the Chlorine monOxide Experiment at Scott Base, Antarctica, and 12 years of measurements from the Aura Microwave Limb Sounder to show that the trends in ClO during the ozone hole season are consistent with changes in stratospheric chlorine observed elsewhere.
Remco A. Scheepmaker, Joost aan de Brugh, Haili Hu, Tobias Borsdorff, Christian Frankenberg, Camille Risi, Otto Hasekamp, Ilse Aben, and Jochen Landgraf
Atmos. Meas. Tech., 9, 3921–3937, https://doi.org/10.5194/amt-9-3921-2016, https://doi.org/10.5194/amt-9-3921-2016, 2016
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We have developed an algorithm to measure HDO (heavy water) in the atmosphere using the TROPOMI satellite instrument, scheduled for launch in 2016. Giving an insight in the history of water vapour, these measurements will help to better understand the water cycle and its role in climate change. We use realistic measurement simulations to describe the performance of the algorithm, and show that TROPOMI will greatly improve and extend the HDO datasets from the previous SCIAMACHY and GOSAT missions.
Hilke Oetjen, Vivienne H. Payne, Jessica L. Neu, Susan S. Kulawik, David P. Edwards, Annmarie Eldering, Helen M. Worden, and John R. Worden
Atmos. Chem. Phys., 16, 10229–10239, https://doi.org/10.5194/acp-16-10229-2016, https://doi.org/10.5194/acp-16-10229-2016, 2016
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We developed and tested a strategy for combining TES and IASI free-tropospheric ozone data. A time series of the merged ozone data is presented for regional monthly means over the western US, Europe, and eastern Asia. We show that free-tropospheric ozone over Europe and the western US has remained relatively constant over the past decade but that, contrary to expectations, ozone over Asia in recent years does not continue the rapid rate of increase observed from 2004–2010.
Brian J. Connor, Vanessa Sherlock, Geoff Toon, Debra Wunch, and Paul O. Wennberg
Atmos. Meas. Tech., 9, 3513–3525, https://doi.org/10.5194/amt-9-3513-2016, https://doi.org/10.5194/amt-9-3513-2016, 2016
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An algorithm for retrieval of vertical profiles of CO2 from ground-based spectra is described. Retrieval of CO2 vertical profiles from would be very beneficial for carbon cycle studies and the validation of satellite measurements. There are approximately 3 degrees of freedom for the CO2 profile. The accuracy of retrievals of CO2 from the spectral band used is limited by small errors in the calculated spectrum. Ongoing research is needed and described.
Christian Frankenberg, Susan S. Kulawik, Steven C. Wofsy, Frédéric Chevallier, Bruce Daube, Eric A. Kort, Christopher O'Dell, Edward T. Olsen, and Gregory Osterman
Atmos. Chem. Phys., 16, 7867–7878, https://doi.org/10.5194/acp-16-7867-2016, https://doi.org/10.5194/acp-16-7867-2016, 2016
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We use observations from the HIAPER Pole-to-Pole Observations (HIPPO) flights from January 2009 through September 2011 to validate CO2 measurements from satellites (GOSAT, TES, AIRS) and atmospheric inversion models (CarbonTracker CT2013B, MACC v13r1).
Dejian Fu, Kevin W. Bowman, Helen M. Worden, Vijay Natraj, John R. Worden, Shanshan Yu, Pepijn Veefkind, Ilse Aben, Jochen Landgraf, Larrabee Strow, and Yong Han
Atmos. Meas. Tech., 9, 2567–2579, https://doi.org/10.5194/amt-9-2567-2016, https://doi.org/10.5194/amt-9-2567-2016, 2016
Akihiko Kuze, Hiroshi Suto, Kei Shiomi, Shuji Kawakami, Makoto Tanaka, Yoko Ueda, Akira Deguchi, Jun Yoshida, Yoshifumi Yamamoto, Fumie Kataoka, Thomas E. Taylor, and Henry L. Buijs
Atmos. Meas. Tech., 9, 2445–2461, https://doi.org/10.5194/amt-9-2445-2016, https://doi.org/10.5194/amt-9-2445-2016, 2016
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A more than 6-year data set has been acquired by TANSO-FTS onboard GOSAT. This paper provides updates on the performance and describes important changes to the data product for the typical accuracy of retrieved CO2 and CH4 of 2 ppm and 13 ppb, respectively. The V201 Level 1B have long-term uniform quality and provide consistent retrieval accuracy even after the three anomalies of the satellite system. In addition, we discuss the unique observation abilities by an agile pointing mechanism.
Glynn C. Hulley, Riley M. Duren, Francesca M. Hopkins, Simon J. Hook, Nick Vance, Pierre Guillevic, William R. Johnson, Bjorn T. Eng, Jonathan M. Mihaly, Veljko M. Jovanovic, Seth L. Chazanoff, Zak K. Staniszewski, Le Kuai, John Worden, Christian Frankenberg, Gerardo Rivera, Andrew D. Aubrey, Charles E. Miller, Nabin K. Malakar, Juan M. Sánchez Tomás, and Kendall T. Holmes
Atmos. Meas. Tech., 9, 2393–2408, https://doi.org/10.5194/amt-9-2393-2016, https://doi.org/10.5194/amt-9-2393-2016, 2016
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Using data from a new airborne Hyperspectral Thermal Emission Spectrometer (HyTES) instrument, we present a technique for the detection and wide-area mapping of emission plumes of methane and other atmospheric trace gas species over challenging and diverse environmental conditions with high spatial resolution, that permits direct attribution to sources in complex environments.
Hélène Brogniez, Stephen English, Jean-François Mahfouf, Andreas Behrendt, Wesley Berg, Sid Boukabara, Stefan Alexander Buehler, Philippe Chambon, Antonia Gambacorta, Alan Geer, William Ingram, E. Robert Kursinski, Marco Matricardi, Tatyana A. Odintsova, Vivienne H. Payne, Peter W. Thorne, Mikhail Yu. Tretyakov, and Junhong Wang
Atmos. Meas. Tech., 9, 2207–2221, https://doi.org/10.5194/amt-9-2207-2016, https://doi.org/10.5194/amt-9-2207-2016, 2016
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Because a systematic difference between measurements of water vapor performed by space-borne observing instruments in the microwave spectral domain and their numerical modeling was recently highlighted, this work discusses and gives an overview of the various errors and uncertainties associated with each element in the comparison process. Indeed, the knowledge of absolute errors in any observation of the climate system is key, more specifically because we need to detect small changes.
Robert R. Nelson, Christopher W. O'Dell, Thomas E. Taylor, Lukas Mandrake, and Mike Smyth
Atmos. Meas. Tech., 9, 1671–1684, https://doi.org/10.5194/amt-9-1671-2016, https://doi.org/10.5194/amt-9-1671-2016, 2016
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In this work, we test the hypothesis that clear-sky retrievals may perform as well as full-physics retrievals for very clear scenes. It was found that for simulated OCO-2 measurements, the clear-sky retrieval had errors comparable to those of the full-physics retrieval. For real GOSAT data, the clear-sky retrieval had errors 0–20 % larger than the full-physics retrieval over land and 20–35 % larger over ocean. This work implies that clear-sky retrievals may be more useful than previously assumed.
Thomas E. Taylor, Christopher W. O'Dell, Christian Frankenberg, Philip T. Partain, Heather Q. Cronk, Andrey Savtchenko, Robert R. Nelson, Emily J. Rosenthal, Albert Y. Chang, Brenden Fisher, Gregory B. Osterman, Randy H. Pollock, David Crisp, Annmarie Eldering, and Michael R. Gunson
Atmos. Meas. Tech., 9, 973–989, https://doi.org/10.5194/amt-9-973-2016, https://doi.org/10.5194/amt-9-973-2016, 2016
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NASA's Orbiting Carbon Observatory-2 (OCO-2) is providing approximately 1 million soundings per day of the total column of carbon dioxide (XCO2). The retrieval of XCO2 can only be performed for soundings sufficiently free of cloud and aerosol. This work highlights comparisons of OCO-2 cloud screening algorithms to the MODIS cloud mask product. We find agreement approximately 85 % of the time with some significant spatial and small seasonal dependencies.
Susan Kulawik, Debra Wunch, Christopher O'Dell, Christian Frankenberg, Maximilian Reuter, Tomohiro Oda, Frederic Chevallier, Vanessa Sherlock, Michael Buchwitz, Greg Osterman, Charles E. Miller, Paul O. Wennberg, David Griffith, Isamu Morino, Manvendra K. Dubey, Nicholas M. Deutscher, Justus Notholt, Frank Hase, Thorsten Warneke, Ralf Sussmann, John Robinson, Kimberly Strong, Matthias Schneider, Martine De Mazière, Kei Shiomi, Dietrich G. Feist, Laura T. Iraci, and Joyce Wolf
Atmos. Meas. Tech., 9, 683–709, https://doi.org/10.5194/amt-9-683-2016, https://doi.org/10.5194/amt-9-683-2016, 2016
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To accurately estimate source and sink locations of carbon dioxide, systematic errors in satellite measurements and models must be characterized. This paper examines two satellite data sets (GOSAT, launched 2009, and SCIAMACHY, launched 2002), and two models (CarbonTracker and MACC) vs. the TCCON CO2 validation data set. We assess biases and errors by season and latitude, satellite performance under averaging, and diurnal variability. Our findings are useful for assimilation of satellite data.
D. R. Thompson, I. Leifer, H. Bovensmann, M. Eastwood, M. Fladeland, C. Frankenberg, K. Gerilowski, R. O. Green, S. Kratwurst, T. Krings, B. Luna, and A. K. Thorpe
Atmos. Meas. Tech., 8, 4383–4397, https://doi.org/10.5194/amt-8-4383-2015, https://doi.org/10.5194/amt-8-4383-2015, 2015
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We discuss principles for real-time infrared spectral signature detection and measurement, and report performance onboard the NASA Airborne Visible Infrared Spectrometer - Next Generation (AVIRIS-NG). We describe a case study of the NASA/ESA CO2 and MEthane eXperiment (COMEX), a multi-platform campaign to measure CH4 plumes released from anthropogenic sources including oil and gas infrastructure. AVIRIS-NG successfully detected CH4 plumes in concert with other in situ and remote instruments.
J. R. Worden, A. J. Turner, A. Bloom, S. S. Kulawik, J. Liu, M. Lee, R. Weidner, K. Bowman, C. Frankenberg, R. Parker, and V. H. Payne
Atmos. Meas. Tech., 8, 3433–3445, https://doi.org/10.5194/amt-8-3433-2015, https://doi.org/10.5194/amt-8-3433-2015, 2015
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Here we demonstrate the potential for estimating lower tropospheric CH4 concentrations through the combination of free-tropospheric methane measurements from the Aura Tropospheric Emission Spectrometer (TES) and XCH4 (dry-mole air fraction of methane) from the Greenhouse Gases Observing Satellite - Thermal And Near-infrared for carbon Observation (GOSAT TANSO).
E. N. Koffi, P. J. Rayner, A. J. Norton, C. Frankenberg, and M. Scholze
Biogeosciences, 12, 4067–4084, https://doi.org/10.5194/bg-12-4067-2015, https://doi.org/10.5194/bg-12-4067-2015, 2015
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We investigate the utility of satellite measurements of solar-induced chlorophyll fluorescence (SIF) in constraining gross primary productivity (GPP). We simulate SIF with the biosphere model BETHY coupled with the fluorescence model SCOPE. The model simulates well the patterns of SIF. SIF is sensitive to leaf chlorophyll and incoming radiation but not to the key physiological parameter Vcmax controlling GPP. Thus, further model development is necessary before SIF can be used to constrain GPP.
A. J. Turner, D. J. Jacob, K. J. Wecht, J. D. Maasakkers, E. Lundgren, A. E. Andrews, S. C. Biraud, H. Boesch, K. W. Bowman, N. M. Deutscher, M. K. Dubey, D. W. T. Griffith, F. Hase, A. Kuze, J. Notholt, H. Ohyama, R. Parker, V. H. Payne, R. Sussmann, C. Sweeney, V. A. Velazco, T. Warneke, P. O. Wennberg, and D. Wunch
Atmos. Chem. Phys., 15, 7049–7069, https://doi.org/10.5194/acp-15-7049-2015, https://doi.org/10.5194/acp-15-7049-2015, 2015
G. E. Nedoluha, I. S. Boyd, A. Parrish, R. M. Gomez, D. R. Allen, L. Froidevaux, B. J. Connor, and R. R. Querel
Atmos. Chem. Phys., 15, 6817–6826, https://doi.org/10.5194/acp-15-6817-2015, https://doi.org/10.5194/acp-15-6817-2015, 2015
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This paper highlights 2 unusual mid-stratospheric O3 anomalies in our 22-year ground-based data set. One of these is a large month long increase in June 2001 which we are able to associate with very unusually low equatorial air which persists over Lauder for much of June. The other O3 anomaly persists for ~4 years; using MLS data, we show that this is associated with unusually high N2O during this period. During this period there is also a low O3 and N2O anomaly in the tropics.
R. A. Scheepmaker, C. Frankenberg, N. M. Deutscher, M. Schneider, S. Barthlott, T. Blumenstock, O. E. Garcia, F. Hase, N. Jones, E. Mahieu, J. Notholt, V. Velazco, J. Landgraf, and I. Aben
Atmos. Meas. Tech., 8, 1799–1818, https://doi.org/10.5194/amt-8-1799-2015, https://doi.org/10.5194/amt-8-1799-2015, 2015
A. Merrelli, R. Bennartz, C. W. O'Dell, and T. E. Taylor
Atmos. Meas. Tech., 8, 1641–1656, https://doi.org/10.5194/amt-8-1641-2015, https://doi.org/10.5194/amt-8-1641-2015, 2015
L. Guanter, I. Aben, P. Tol, J. M. Krijger, A. Hollstein, P. Köhler, A. Damm, J. Joiner, C. Frankenberg, and J. Landgraf
Atmos. Meas. Tech., 8, 1337–1352, https://doi.org/10.5194/amt-8-1337-2015, https://doi.org/10.5194/amt-8-1337-2015, 2015
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This paper investigates the potential of the upcoming TROPOspheric Monitoring Instrument (TROPOMI) instrument for the retrieval of the chlorophyll fluorescence signal emitted in the 650–850nm spectral range by the photosynthetic machinery of green plants. We find that TROPOMI will allow substantial improvements in the space monitoring of fluorescence with respect to current spaceborne instruments such as GOME-2 and SCIAMACHY.
M. J. Alvarado, V. H. Payne, K. E. Cady-Pereira, J. D. Hegarty, S. S. Kulawik, K. J. Wecht, J. R. Worden, J. V. Pittman, and S. C. Wofsy
Atmos. Meas. Tech., 8, 965–985, https://doi.org/10.5194/amt-8-965-2015, https://doi.org/10.5194/amt-8-965-2015, 2015
C. Frankenberg, R. Pollock, R. A. M. Lee, R. Rosenberg, J.-F. Blavier, D. Crisp, C. W. O'Dell, G. B. Osterman, C. Roehl, P. O. Wennberg, and D. Wunch
Atmos. Meas. Tech., 8, 301–313, https://doi.org/10.5194/amt-8-301-2015, https://doi.org/10.5194/amt-8-301-2015, 2015
K. W. Wong, D. Fu, T. J. Pongetti, S. Newman, E. A. Kort, R. Duren, Y.-K. Hsu, C. E. Miller, Y. L. Yung, and S. P. Sander
Atmos. Chem. Phys., 15, 241–252, https://doi.org/10.5194/acp-15-241-2015, https://doi.org/10.5194/acp-15-241-2015, 2015
M. Alexe, P. Bergamaschi, A. Segers, R. Detmers, A. Butz, O. Hasekamp, S. Guerlet, R. Parker, H. Boesch, C. Frankenberg, R. A. Scheepmaker, E. Dlugokencky, C. Sweeney, S. C. Wofsy, and E. A. Kort
Atmos. Chem. Phys., 15, 113–133, https://doi.org/10.5194/acp-15-113-2015, https://doi.org/10.5194/acp-15-113-2015, 2015
H. Oetjen, V. H. Payne, S. S. Kulawik, A. Eldering, J. Worden, D. P. Edwards, G. L. Francis, H. M. Worden, C. Clerbaux, J. Hadji-Lazaro, and D. Hurtmans
Atmos. Meas. Tech., 7, 4223–4236, https://doi.org/10.5194/amt-7-4223-2014, https://doi.org/10.5194/amt-7-4223-2014, 2014
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We apply the TES ozone retrieval algorithm to IASI radiances and characterise the uncertainties and information content of the retrieved ozone profiles. We find that our biases with respect to sondes and our degrees of freedom for signal for ozone are comparable to previously published results from other IASI ozone algorithms. We find that predicted and empirical errors are consistent. In general, the precision of the IASI ozone profiles is better than 20%.
V. H. Payne, M. J. Alvarado, K. E. Cady-Pereira, J. R. Worden, S. S. Kulawik, and E. V. Fischer
Atmos. Meas. Tech., 7, 3737–3749, https://doi.org/10.5194/amt-7-3737-2014, https://doi.org/10.5194/amt-7-3737-2014, 2014
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Peroxyacetyl nitrate (PAN) plays an important role in the distribution of lower-atmospheric ozone. PAN can be transported far from the original pollution source, leading to ozone formation and degraded air quality in remote areas. Satellite observations from the Tropospheric Emission Spectrometer (TES) are sensitive to PAN at lower altitude than previous global data sets. We describe characteristics of the data and show elevated PAN associated with boreal fires and outflow of Asian pollution.
N. M. Deutscher, V. Sherlock, S. E. Mikaloff Fletcher, D. W. T. Griffith, J. Notholt, R. Macatangay, B. J. Connor, J. Robinson, H. Shiona, V. A. Velazco, Y. Wang, P. O. Wennberg, and D. Wunch
Atmos. Chem. Phys., 14, 9883–9901, https://doi.org/10.5194/acp-14-9883-2014, https://doi.org/10.5194/acp-14-9883-2014, 2014
V. Gryazin, C. Risi, J. Jouzel, N. Kurita, J. Worden, C. Frankenberg, V. Bastrikov, K. Gribanov, and O. Stukova
Atmos. Chem. Phys., 14, 9807–9830, https://doi.org/10.5194/acp-14-9807-2014, https://doi.org/10.5194/acp-14-9807-2014, 2014
K. M. Saad, D. Wunch, G. C. Toon, P. Bernath, C. Boone, B. Connor, N. M. Deutscher, D. W. T. Griffith, R. Kivi, J. Notholt, C. Roehl, M. Schneider, V. Sherlock, and P. O. Wennberg
Atmos. Meas. Tech., 7, 2907–2918, https://doi.org/10.5194/amt-7-2907-2014, https://doi.org/10.5194/amt-7-2907-2014, 2014
A. Parrish, I. S. Boyd, G. E. Nedoluha, P. K. Bhartia, S. M. Frith, N. A. Kramarova, B. J. Connor, G. E. Bodeker, L. Froidevaux, M. Shiotani, and T. Sakazaki
Atmos. Chem. Phys., 14, 7255–7272, https://doi.org/10.5194/acp-14-7255-2014, https://doi.org/10.5194/acp-14-7255-2014, 2014
S. Massart, A. Agusti-Panareda, I. Aben, A. Butz, F. Chevallier, C. Crevoisier, R. Engelen, C. Frankenberg, and O. Hasekamp
Atmos. Chem. Phys., 14, 6139–6158, https://doi.org/10.5194/acp-14-6139-2014, https://doi.org/10.5194/acp-14-6139-2014, 2014
B. Dils, M. Buchwitz, M. Reuter, O. Schneising, H. Boesch, R. Parker, S. Guerlet, I. Aben, T. Blumenstock, J. P. Burrows, A. Butz, N. M. Deutscher, C. Frankenberg, F. Hase, O. P. Hasekamp, J. Heymann, M. De Mazière, J. Notholt, R. Sussmann, T. Warneke, D. Griffith, V. Sherlock, and D. Wunch
Atmos. Meas. Tech., 7, 1723–1744, https://doi.org/10.5194/amt-7-1723-2014, https://doi.org/10.5194/amt-7-1723-2014, 2014
S. Houweling, M. Krol, P. Bergamaschi, C. Frankenberg, E. J. Dlugokencky, I. Morino, J. Notholt, V. Sherlock, D. Wunch, V. Beck, C. Gerbig, H. Chen, E. A. Kort, T. Röckmann, and I. Aben
Atmos. Chem. Phys., 14, 3991–4012, https://doi.org/10.5194/acp-14-3991-2014, https://doi.org/10.5194/acp-14-3991-2014, 2014
D. Fu, T. J. Pongetti, J.-F. L. Blavier, T. J. Crawford, K. S. Manatt, G. C. Toon, K. W. Wong, and S. P. Sander
Atmos. Meas. Tech., 7, 713–729, https://doi.org/10.5194/amt-7-713-2014, https://doi.org/10.5194/amt-7-713-2014, 2014
C. Liu, S. Beirle, T. Butler, P. Hoor, C. Frankenberg, P. Jöckel, M. Penning de Vries, U. Platt, A. Pozzer, M. G. Lawrence, J. Lelieveld, H. Tost, and T. Wagner
Atmos. Chem. Phys., 14, 1717–1732, https://doi.org/10.5194/acp-14-1717-2014, https://doi.org/10.5194/acp-14-1717-2014, 2014
A. K. Thorpe, C. Frankenberg, and D. A. Roberts
Atmos. Meas. Tech., 7, 491–506, https://doi.org/10.5194/amt-7-491-2014, https://doi.org/10.5194/amt-7-491-2014, 2014
J. Joiner, L. Guanter, R. Lindstrot, M. Voigt, A. P. Vasilkov, E. M. Middleton, K. F. Huemmrich, Y. Yoshida, and C. Frankenberg
Atmos. Meas. Tech., 6, 2803–2823, https://doi.org/10.5194/amt-6-2803-2013, https://doi.org/10.5194/amt-6-2803-2013, 2013
L. Mandrake, C. Frankenberg, C. W. O'Dell, G. Osterman, P. Wennberg, and D. Wunch
Atmos. Meas. Tech., 6, 2851–2864, https://doi.org/10.5194/amt-6-2851-2013, https://doi.org/10.5194/amt-6-2851-2013, 2013
B. J. Connor, T. Mooney, G. E. Nedoluha, J. W. Barrett, A. Parrish, J. Koda, M. L. Santee, and R. M. Gomez
Atmos. Chem. Phys., 13, 8643–8650, https://doi.org/10.5194/acp-13-8643-2013, https://doi.org/10.5194/acp-13-8643-2013, 2013
M. J. Alvarado, V. H. Payne, E. J. Mlawer, G. Uymin, M. W. Shephard, K. E. Cady-Pereira, J. S. Delamere, and J.-L. Moncet
Atmos. Chem. Phys., 13, 6687–6711, https://doi.org/10.5194/acp-13-6687-2013, https://doi.org/10.5194/acp-13-6687-2013, 2013
H. M. Worden, D. P. Edwards, M. N. Deeter, D. Fu, S. S. Kulawik, J. R. Worden, and A. Arellano
Atmos. Meas. Tech., 6, 1633–1646, https://doi.org/10.5194/amt-6-1633-2013, https://doi.org/10.5194/amt-6-1633-2013, 2013
Y. Yoshida, N. Kikuchi, I. Morino, O. Uchino, S. Oshchepkov, A. Bril, T. Saeki, N. Schutgens, G. C. Toon, D. Wunch, C. M. Roehl, P. O. Wennberg, D. W. T. Griffith, N. M. Deutscher, T. Warneke, J. Notholt, J. Robinson, V. Sherlock, B. Connor, M. Rettinger, R. Sussmann, P. Ahonen, P. Heikkinen, E. Kyrö, J. Mendonca, K. Strong, F. Hase, S. Dohe, and T. Yokota
Atmos. Meas. Tech., 6, 1533–1547, https://doi.org/10.5194/amt-6-1533-2013, https://doi.org/10.5194/amt-6-1533-2013, 2013
R. A. Scheepmaker, C. Frankenberg, A. Galli, A. Butz, H. Schrijver, N. M. Deutscher, D. Wunch, T. Warneke, S. Fally, and I. Aben
Atmos. Meas. Tech., 6, 879–894, https://doi.org/10.5194/amt-6-879-2013, https://doi.org/10.5194/amt-6-879-2013, 2013
J. Worden, K. Wecht, C. Frankenberg, M. Alvarado, K. Bowman, E. Kort, S. Kulawik, M. Lee, V. Payne, and H. Worden
Atmos. Chem. Phys., 13, 3679–3692, https://doi.org/10.5194/acp-13-3679-2013, https://doi.org/10.5194/acp-13-3679-2013, 2013
D. Fu, J. R. Worden, X. Liu, S. S. Kulawik, K. W. Bowman, and V. Natraj
Atmos. Chem. Phys., 13, 3445–3462, https://doi.org/10.5194/acp-13-3445-2013, https://doi.org/10.5194/acp-13-3445-2013, 2013
C. Frankenberg, D. Wunch, G. Toon, C. Risi, R. Scheepmaker, J.-E. Lee, P. Wennberg, and J. Worden
Atmos. Meas. Tech., 6, 263–274, https://doi.org/10.5194/amt-6-263-2013, https://doi.org/10.5194/amt-6-263-2013, 2013
H. M. Worden, M. N. Deeter, C. Frankenberg, M. George, F. Nichitiu, J. Worden, I. Aben, K. W. Bowman, C. Clerbaux, P. F. Coheur, A. T. J. de Laat, R. Detweiler, J. R. Drummond, D. P. Edwards, J. C. Gille, D. Hurtmans, M. Luo, S. Martínez-Alonso, S. Massie, G. Pfister, and J. X. Warner
Atmos. Chem. Phys., 13, 837–850, https://doi.org/10.5194/acp-13-837-2013, https://doi.org/10.5194/acp-13-837-2013, 2013
Related subject area
Subject: Gases | Technique: Remote Sensing | Topic: Data Processing and Information Retrieval
Hourly surface nitrogen dioxide retrieval from GEMS tropospheric vertical column densities: benefit of using time-contiguous input features for machine learning models
Remote sensing estimates of time-resolved HONO and NO2 emission rates and lifetimes in wildfires
A study of measurement scenarios for the future CO2M mission: avoidance of detector saturation and the impact on XCO2 retrievals
Assimilation of volcanic sulfur dioxide products from IASI and TROPOMI into the chemical transport model MOCAGE: case study of the 2021 La Soufrière Saint Vincent eruption with the March 2022 version of MOCAGE
In-flight estimation of instrument spectral response functions using sparse representations
Robustness of atmospheric trace gas retrievals obtained from low-spectral-resolution Fourier transform infrared absorption spectra under variations of interferogram length
Retrieval of NO2 profiles from 3 years of Pandora MAX-DOAS measurements in Toronto, Canada
A channel selection methodology for enhancing volcanic SO2 monitoring using FY-3E/HIRAS-II hyperspectral data
Predictions of failed satellite retrieval of air quality using machine learning
Deep transfer learning method for seasonal TROPOMI XCH4 albedo correction
Global retrieval of TROPOMI tropospheric HCHO and NO2 columns with improved consistency based on the updated Peking University OMI NO2 algorithm
Tightening-up methane plume source rate estimation in EnMAP and PRISMA images
Potential CO2 measurement capabilities of a transportable Near Infrared Laser Heterodyne Radiometer (LHR)
Quantitative estimate of several sources of uncertainty in drone-based methane emission measurements
Implementation and application of an improved phase spectrum determination scheme for Fourier transform spectrometry
Improved detection of global NOx emissions from shipping in Sentinel-5P TROPOMI data
Remote sensing of lower-middle-thermosphere temperatures using the N2 Lyman–Birge–Hopfield (LBH) bands
Retrievals of water vapour and temperature exploiting the far-infrared: application to aircraft observations in preparation for the FORUM mission
Global decadal measurements of methanol, ethene, ethyne, and HCN from the Cross-track Infrared Sounder
Forward model emulator for atmospheric radiative transfer using Gaussian processes and cross validation
The novel GOME-type Ozone Profile Essential Climate Variable (GOP-ECV) data record covering the past 26 years
Developments on a 22 GHz microwave radiometer and reprocessing of 13-year time series for water vapour studies
Optimal selection of satellite XCO2 images for urban CO2 emission monitoring
Separating and quantifying facility-level methane emissions with overlapping plumes for spaceborne methane monitoring
Retrieving the atmospheric concentrations of carbon dioxide and methane from the European Copernicus CO2M satellite mission using artificial neural networks
Surface reflectance biases in XCH4 retrievals from the 2.3 μm band are enhanced in the presence of aerosols
Remote sensing of methane point sources with the MethaneAIR airborne spectrometer
Optimal Estimation Retrieval Framework for Daytime Clear-Sky Total Column Water Vapour from MTG-FCI Near-Infrared Measurements
The differences between remote sensing and in situ air pollutant measurements over the Canadian oil sands
NitroNet – a machine learning model for the prediction of tropospheric NO2 profiles from TROPOMI observations
Improved convective cloud differential (CCD) tropospheric ozone from S5P-TROPOMI satellite data using local cloud fields
Atmospheric propane (C3H8) column retrievals from ground-based FTIR observations in Xianghe, China
Can the remote sensing of combustion phase improve estimates of landscape fire smoke emission rate and composition?
Tropospheric NO2 retrieval algorithm for geostationary satellite instruments: applications to GEMS
Troposphere–stratosphere-integrated bromine monoxide (BrO) profile retrieval over the central Pacific Ocean
Local and regional enhancements of CH4, CO, and CO2 inferred from TCCON column measurements
Merging TEMPEST microwave and GOES-16 geostationary IR soundings for improved water vapor profiles
Methane retrieval from MethaneAIR using the CO2 proxy approach: a demonstration for the upcoming MethaneSAT mission
Mapping the CO2 total column retrieval performance from shortwave infrared measurements: synthetic impacts of the spectral resolution, signal-to-noise ratio, and spectral band selection
Assessment of the contribution of the Meteosat Third Generation Infrared Sounder (MTG-IRS) for the characterisation of ozone over Europe
Assessing the potential of free-tropospheric water vapour isotopologue satellite observations for improving the analyses of convective events
Current potential of CH4 emission estimates using TROPOMI in the Middle East
A bias-corrected GEMS geostationary satellite product for nitrogen dioxide using machine learning to enforce consistency with the TROPOMI satellite instrument
Estimation of biogenic volatile organic compound (BVOC) emissions in forest ecosystems using drone-based lidar, photogrammetry, and image recognition technologies
Fast retrieval of XCO2 over east Asia based on Orbiting Carbon Observatory-2 (OCO-2) spectral measurements
A new method for estimating megacity NOx emissions and lifetimes from satellite observations
Accounting for the effect of aerosols in GHGSat methane retrieval
A survey of methane point source emissions from coal mines in Shanxi province of China using AHSI on board Gaofen-5B
Global retrieval of stratospheric and tropospheric BrO columns from the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) on board the Suomi-NPP satellite
IMK–IAA MIPAS retrieval version 8: CH4 and N2O
Janek Gödeke, Andreas Richter, Kezia Lange, Peter Maaß, Hyunkee Hong, Hanlim Lee, and Junsung Park
Atmos. Meas. Tech., 18, 3747–3779, https://doi.org/10.5194/amt-18-3747-2025, https://doi.org/10.5194/amt-18-3747-2025, 2025
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The Korean Geostationary Environmental Monitoring Spectrometer (GEMS) monitors trace gases over Asia, e.g., NO2. GEMS provides hourly data, improving the time resolution compared to the daily overpasses by other satellites. For the prediction of hourly surface NO2 over South Korea from GEMS observations and meteorological data, this study shows that machine learning models benefit from this higher time resolution. This is achieved by using observations from previous hours as additional inputs.
Carley D. Fredrickson, Scott J. Janz, Lok N. Lamsal, Ursula A. Jongebloed, Joshua L. Laughner, and Joel A. Thornton
Atmos. Meas. Tech., 18, 3669–3689, https://doi.org/10.5194/amt-18-3669-2025, https://doi.org/10.5194/amt-18-3669-2025, 2025
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We present an analysis of high-resolution remote sensing measurements of nitrogen-containing trace gases emitted by wildfires. The measurements were made using an instrument on the NASA ER-2 aircraft in the summer of 2019. We find that time-resolved fire intensity is critical to quantify trace gas emissions over a fire's entire lifespan. These findings have implications for improving air pollution forecasts downwind of wildfires using computer models of atmospheric chemistry and meteorology.
Michael Weimer, Michael Hilker, Stefan Noël, Max Reuter, Michael Buchwitz, Blanca Fuentes Andrade, Rüdiger Lang, Bernd Sierk, Yasjka Meijer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Meas. Tech., 18, 3321–3340, https://doi.org/10.5194/amt-18-3321-2025, https://doi.org/10.5194/amt-18-3321-2025, 2025
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Optical detectors have a maximum signal (saturation). Exceedance means that the measurement has to be discarded. We investigate where saturation will occur for the future European satellite mission dedicated to CO2 monitoring (CO2M) and strategies to avoid saturation. Saturation impacts coverage and precision, both of which are important for estimation of local CO2 emissions. We find that taking two pictures per sampling should be sufficient to avoid saturation for CO2M, with some impact on CO2 precision.
Mickaël Bacles, Jonathan Améric, and Vincent Guidard
Atmos. Meas. Tech., 18, 2659–2680, https://doi.org/10.5194/amt-18-2659-2025, https://doi.org/10.5194/amt-18-2659-2025, 2025
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Sulfur dioxide emitted during volcanic eruptions can be hazardous for aviation safety. A recent development aims at improving the forecasts of volcanic sulfur dioxide quantities made by the chemistry transport model developed at Météo-France by assimilated infrared and ultraviolet satellite instruments. We focus on the eruption event of the La Soufrière Saint Vincent volcano in April 2021. The combined assimilation of these observations always leads to better analyses and forecasts.
Jihanne El Haouari, Jean-Michel Gaucel, Christelle Pittet, Jean-Yves Tourneret, and Herwig Wendt
Atmos. Meas. Tech., 18, 2573–2590, https://doi.org/10.5194/amt-18-2573-2025, https://doi.org/10.5194/amt-18-2573-2025, 2025
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This paper explores new techniques based on sparse representations for estimating the spectral response functions of high-resolution spectrometers. The method is highly competitive, with commonly used parametric models yielding more accurate estimates while accounting for wavelength dependence. The resulting normalized estimation errors of the spectrometer spectral responses are less than 1 %, which will allow for better quantification of trace gas concentrations at the Earth surface.
Bavo Langerock, Martine De Mazière, Filip Desmet, Pauli Heikkinen, Rigel Kivi, Mahesh Kumar Sha, Corinne Vigouroux, Minqiang Zhou, Gopala Krishna Darbha, and Mohmmed Talib
Atmos. Meas. Tech., 18, 2439–2446, https://doi.org/10.5194/amt-18-2439-2025, https://doi.org/10.5194/amt-18-2439-2025, 2025
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Ground-based Fourier transform interferometer instruments have been used for many decades to measure direct solar light in the infrared to obtain high-resolution spectra from which atmospheric gas profile concentrations can be derived. It is shown that the typical processing chain used to derive atmospheric gas columns can be sensitive to relatively small shortenings of the recorded interferograms. Low-resolution recordings, used in more recent years, are more sensitive to such adaptations.
Ramina Alwarda, Kristof Bognar, Xiaoyi Zhao, Vitali Fioletov, Jonathan Davies, Sum Chi Lee, Debora Griffin, Alexandru Lupu, Udo Frieß, Alexander Cede, Yushan Su, and Kimberly Strong
Atmos. Meas. Tech., 18, 2397–2423, https://doi.org/10.5194/amt-18-2397-2025, https://doi.org/10.5194/amt-18-2397-2025, 2025
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Nitrogen dioxide (NO2) is a pollutant with a short lifetime and large variability, but there are limited measurements of its distribution in the lower atmosphere. We present a new 3-year dataset of NO2 vertical profiles in Toronto, Canada, and evaluate it using NO2 from satellite and surface monitoring networks and simulations by an air quality forecast model. We quantify and explain the differences among the datasets to provide information that can be used to understand NO2 variability.
Xinyu Li, Lin Zhu, Hongfu Sun, Jun Li, Ximing Lv, Chengli Qi, and Huanhuan Yan
Atmos. Meas. Tech., 18, 2333–2352, https://doi.org/10.5194/amt-18-2333-2025, https://doi.org/10.5194/amt-18-2333-2025, 2025
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This paper proposes a novel methodology for selecting sulfur-dioxide-sensitive channels from FY-3E/HIRAS-II hyperspectral IR atmospheric sensors to quantitatively monitor volcanic sulfur dioxide. This methodology considers the interference of atmospheric temperature, humidity, and surface temperature with sulfur dioxide detection and retrieval, laying the groundwork for developing a more accurate and flexible volcanic sulfur dioxide retrieval algorithm under different atmospheric conditions.
Edward Malina, Jure Brence, Jennifer Adams, Jovan Tanevski, Sašo Džeroski, Valentin Kantchev, and Kevin W. Bowman
Atmos. Meas. Tech., 18, 1689–1715, https://doi.org/10.5194/amt-18-1689-2025, https://doi.org/10.5194/amt-18-1689-2025, 2025
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The large fleet of Earth observation satellites in orbit currently generate huge volumes of data, requiring significant computational resources to process these data in a timely manner. We present a method for predicting poor-quality measurements using machine learning. We find that machine learning methods can accurately predict poor-quality measurements and remove them from the processing chain, saving time and computational resources.
Alexander C. Bradley, Barbara Dix, Fergus Mackenzie, J. Pepijn Veefkind, and Joost A. de Gouw
Atmos. Meas. Tech., 18, 1675–1687, https://doi.org/10.5194/amt-18-1675-2025, https://doi.org/10.5194/amt-18-1675-2025, 2025
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Currently, measurement of methane from the TROPOMI satellite is biased with respect to surface reflectance. This study demonstrates a new method of correcting for this bias on a seasonal timescale to allow for differences in surface reflectance in areas of intense agriculture where growing seasons may introduce a reflectance bias. We have successfully implemented this technique in the Denver–Julesburg basin, where agriculture and methane extraction infrastructure is often co-located.
Yuhang Zhang, Huan Yu, Isabelle De Smedt, Jintai Lin, Nicolas Theys, Michel Van Roozendael, Gaia Pinardi, Steven Compernolle, Ruijing Ni, Fangxuan Ren, Sijie Wang, Lulu Chen, Jos Van Geffen, Mengyao Liu, Alexander M. Cede, Martin Tiefengraber, Alexis Merlaud, Martina M. Friedrich, Andreas Richter, Ankie Piters, Vinod Kumar, Vinayak Sinha, Thomas Wagner, Yongjoo Choi, Hisahiro Takashima, Yugo Kanaya, Hitoshi Irie, Robert Spurr, Wenfu Sun, and Lorenzo Fabris
Atmos. Meas. Tech., 18, 1561–1589, https://doi.org/10.5194/amt-18-1561-2025, https://doi.org/10.5194/amt-18-1561-2025, 2025
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We developed an advanced algorithm for global retrieval of TROPOspheric Monitoring Instrument (TROPOMI) HCHO and NO2 vertical column densities with much improved consistency. Sensitivity tests demonstrate the complexity and nonlinear interactions of auxiliary parameters in the air mass factor calculation. An improved agreement is found with measurements from a global ground-based instrument network. The scientific retrieval provides a useful source of information for studies combining HCHO and NO2.
Elyes Ouerghi, Thibaud Ehret, Gabriele Facciolo, Enric Meinhardt, Rodolphe Marion, and Jean-Michel Morel
EGUsphere, https://doi.org/10.5194/egusphere-2025-1075, https://doi.org/10.5194/egusphere-2025-1075, 2025
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Reducing methane emissions is essential to tackle climate change. In this paper, we introduce MetFluxNet, a deep learning model for methane plume source rate estimation. This model is trained on a new synthetic dataset designed to avoid network overfit. MetFluxNet can accurately estimate low source rates even in the case of heterogeneous backgrounds. To demonstrate its reliability for real-world plume estimation, we validated its predictions on real plumes with known source rates.
Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, Hervé Herbin, and Weidong Chen
EGUsphere, https://doi.org/10.5194/egusphere-2025-250, https://doi.org/10.5194/egusphere-2025-250, 2025
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This study, part of my 2024 postdoctoral research at ULCO, explores an all-fiber coupled laser heterodyne radiometer (LHR) for CO2 measurements using a tunable diode laser. The LHR employs balanced detection to measure tropospheric CO2 column concentrations. Simulations with the ARAHMIS model are validated against instruments like EM27/SUN and IFS125HR. This work enhances greenhouse gas monitoring and supports campaigns like MAGIC for emissions studies and satellite validation.
Tannaz H. Mohammadloo, Matthew Jones, Bas van de Kerkhof, Kyle Dawson, Brendan J. Smith, Stephen Conley, Abigail Corbett, and Rutger IJzermans
Atmos. Meas. Tech., 18, 1301–1324, https://doi.org/10.5194/amt-18-1301-2025, https://doi.org/10.5194/amt-18-1301-2025, 2025
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Methane is a potent greenhouse gas. Trustable detection and quantification of methane emissions at facility level are critical for identifying the largest sources and prioritizing them for repair. We provide a systematic analysis of several sources of uncertainty in drone-based methane emission surveys based on theoretical considerations and historical data sets. We provide guidelines for industry on how to avoid or minimize errors in drone-based methane emission quantification surveys.
Frank Hase, Paolo Castracane, Angelika Dehn, Omaira Elena García, David W. T. Griffith, Lukas Heizmann, Nicholas B. Jones, Tomi Karppinen, Rigel Kivi, Martine de Mazière, Justus Notholt, and Mahesh Kumar Sha
Atmos. Meas. Tech., 18, 1257–1267, https://doi.org/10.5194/amt-18-1257-2025, https://doi.org/10.5194/amt-18-1257-2025, 2025
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The primary measurement result delivered by a Fourier transform spectrometer is an interferogram, and the spectrum required for further analysis needs to be calculated from the interferogram by Fourier analysis. The paper deals with technical aspects of this process and shows how the reconstruction of the spectrum can be optimized.
Miriam Latsch, Andreas Richter, John P. Burrows, and Hartmut Bösch
EGUsphere, https://doi.org/10.5194/egusphere-2025-107, https://doi.org/10.5194/egusphere-2025-107, 2025
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This study presents our advanced methods to better detect ship-related nitrogen dioxide (NO2) emissions in TROPOMI satellite data. By applying filtering techniques, we identify numerous global shipping routes, including previously undetectable ones, and emissions from offshore platforms. Additionally, we compare the filtered satellite data with CAMS global model data to estimate the differences between observed and modelled NO2 emissions.
Richard Eastes, J. Scott Evans, Quan Gan, William McClintock, and Jerry Lumpe
Atmos. Meas. Tech., 18, 921–928, https://doi.org/10.5194/amt-18-921-2025, https://doi.org/10.5194/amt-18-921-2025, 2025
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Temperature is essential to understanding the thermosphere. Most temperature measurements have been indirect or had large uncertainties, especially in the lower-middle thermosphere, where data are rarely available. Since October 2018, NASA’s GOLD mission has produced disk images of neutral temperatures near 160 km at locations over the Americas and Atlantic Ocean. This paper discusses both temperature retrieval techniques and issues in interpreting GOLD’s images of thermospheric temperatures.
Sanjeevani Panditharatne, Helen Brindley, Caroline Cox, Richard Siddans, Jonathan Murray, Laura Warwick, and Stuart Fox
Atmos. Meas. Tech., 18, 717–735, https://doi.org/10.5194/amt-18-717-2025, https://doi.org/10.5194/amt-18-717-2025, 2025
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Observations from the upcoming European Space Agency’s Far-Infrared Outgoing Radiation Understanding and Monitoring (FORUM) satellite are theorised to be highly sensitive to distributions of water vapour within Earth’s atmosphere. We exploit this sensitivity and extend the Infrared Microwave Sounding retrieval scheme for use on observations from FORUM. This scheme is evaluated on both simulated and observed measurements and shows good agreement with references of the atmospheric state.
Kelley C. Wells, Dylan B. Millet, Jared F. Brewer, Vivienne H. Payne, Karen E. Cady-Pereira, Rick Pernak, Susan Kulawik, Corinne Vigouroux, Nicholas Jones, Emmanuel Mahieu, Maria Makarova, Tomoo Nagahama, Ivan Ortega, Mathias Palm, Kimberly Strong, Matthias Schneider, Dan Smale, Ralf Sussmann, and Minqiang Zhou
Atmos. Meas. Tech., 18, 695–716, https://doi.org/10.5194/amt-18-695-2025, https://doi.org/10.5194/amt-18-695-2025, 2025
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Atmospheric volatile organic compounds (VOCs) affect both air quality and climate. Satellite measurements can help us to assess and predict their global impacts. We present new decadal (2012–2023) measurements of four key VOCs – methanol, ethene, ethyne, and hydrogen cyanide (HCN) – from the Cross-track Infrared Sounder. The measurements reflect emissions from major forests, wildfires, and industry and provide new information to advance understanding of these sources and their changes over time.
Otto Lamminpää, Jouni Susiluoto, Jonathan Hobbs, James McDuffie, Amy Braverman, and Houman Owhadi
Atmos. Meas. Tech., 18, 673–694, https://doi.org/10.5194/amt-18-673-2025, https://doi.org/10.5194/amt-18-673-2025, 2025
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We develop and demonstrate a fast forward function emulator for remote sensing of greenhouse gases. These forward functions are computationally expensive to evaluate, and as such the key challenge for many satellite missions in their data processing is the time used in these evaluations. Our method is fast and accurate enough, less than 1 % relative error, so that it could be safely used in operational processing.
Melanie Coldewey-Egbers, Diego G. Loyola, Barry Latter, Richard Siddans, Brian Kerridge, Daan Hubert, Michel van Roozendael, and Michael Eisinger
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-196, https://doi.org/10.5194/amt-2024-196, 2025
Revised manuscript accepted for AMT
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The GOME-type Ozone Profile Essential Climate Variable (GOP-ECV) data record provides monthly mean ozone profiles with global coverage from 1995 to 2021 at a spatial resolution of 5°x5°. Measurements from five nadir-viewing satellite sensors are first harmonized and then merged into a coherent record. The long-term stability of the data record is further improved through scaling of the profiles using as a reference the GOME-type Total Ozone Essential Climate Variable (GTO-ECV) data record.
Alistair Bell, Eric Sauvageat, Gunter Stober, Klemens Hocke, and Axel Murk
Atmos. Meas. Tech., 18, 555–567, https://doi.org/10.5194/amt-18-555-2025, https://doi.org/10.5194/amt-18-555-2025, 2025
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Hardware and software developments have been made on a 22 GHz microwave radiometer for the measurement of middle-atmospheric water vapour near Bern, Switzerland. Previous measurements dating back to 2010 have been re-calibrated and an improved optimal estimation retrieval performed on these measurements, giving a 13-year dataset. Measurements made with new and improved instrumental hardware are used to correct previous measurements, which show better agreement than the non-corrected dataset.
Alexandre Danjou, Grégoire Broquet, Andrew Schuh, François-Marie Bréon, and Thomas Lauvaux
Atmos. Meas. Tech., 18, 533–554, https://doi.org/10.5194/amt-18-533-2025, https://doi.org/10.5194/amt-18-533-2025, 2025
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We study the capacity of XCO2 spaceborne imagery to estimate urban CO2 emissions with synthetic data. We define automatic and standard methods and objective criteria for image selection. The wind variability and urban emission budget guide the emission estimation error. Images with low wind variability and high urban emissions account for 47 % of images and give a bias in the emission estimation of −7 % and a spread of 56 %. Other images give a bias of −31 % and a spread of 99 %.
Yiguo Pang, Longfei Tian, Denghui Hu, Shuang Gao, and Guohua Liu
Atmos. Meas. Tech., 18, 455–470, https://doi.org/10.5194/amt-18-455-2025, https://doi.org/10.5194/amt-18-455-2025, 2025
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The spatial adjacency of methane point sources can result in plume overlapping, presenting challenges for quantification from space. A separation and quantification method combining the Gaussian plume model and the integrated mass enhancement method is proposed. A modern parameter estimation technique is introduced to separate the overlapping plumes from satellite observations. The proposed method is evaluated with synthesized observations and real satellite observations.
Maximilian Reuter, Michael Hilker, Stefan Noël, Antonio Di Noia, Michael Weimer, Oliver Schneising, Michael Buchwitz, Heinrich Bovensmann, John P. Burrows, Hartmut Bösch, and Ruediger Lang
Atmos. Meas. Tech., 18, 241–264, https://doi.org/10.5194/amt-18-241-2025, https://doi.org/10.5194/amt-18-241-2025, 2025
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Carbon dioxide (CO2) and methane (CH4) are the main anthropogenic greenhouse gases. The European Copernicus CO2 monitoring satellite mission CO2M will provide measurements of their atmospheric concentrations, but the accuracy requirements are demanding and conventional retrieval methods computationally expensive. We present a new retrieval algorithm based on artificial neural networks that has the potential to meet the stringent requirements of the CO2M mission with minimal computational effort.
Peter Somkuti, Greg M. McGarragh, Christopher O'Dell, Antonio Di Noia, Leif Vogel, Sean Crowell, Lesley E. Ott, and Hartmut Bösch
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-145, https://doi.org/10.5194/amt-2024-145, 2025
Revised manuscript accepted for AMT
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In space-based estimates of atmospheric methane concentrations, one can often observe biases that look like imprints of surface features. We performed realistic simulation experiments and find the root cause to be unaccounted aerosols. Since good knowledge of aerosols is difficult to achieve for operational science data processing, we conclude that a comprehensive surface bias correction scheme is highly important for missions utilizing the 2.3 µm spectral band for methane retrievals.
Luis Guanter, Jack Warren, Mark Omara, Apisada Chulakadabba, Javier Roger, Maryann Sargent, Jonathan E. Franklin, Steven C. Wofsy, and Ritesh Gautam
EGUsphere, https://doi.org/10.5194/egusphere-2024-3577, https://doi.org/10.5194/egusphere-2024-3577, 2025
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This study presents a data processing scheme for the detection and quantification of methane emissions using the MethaneAIR airborne spectrometer. We show that the proposed methods enable the detection of smaller plumes than other existing methods, and that improves the potential of MethaneAIR to survey methane point sources across large regions
Jan El Kassar, Cintia Carbajal Henken, Xavier Calbet, Pilar Rípodas, Rene Preusker, and Jürgen Fischer
EGUsphere, https://doi.org/10.5194/egusphere-2024-3605, https://doi.org/10.5194/egusphere-2024-3605, 2024
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Water vapour is a key ingredient in virtually all meteorological processes. We present an algorithm which uses observations of the Flexible Combined Imager (FCI) to estimate the total column of water vapour over sun-lit, clear-sky pixels. FCI is a satellite instrument and every 10 minutes it takes an image which covers Europe, Africa and the Atlantic with a resolution of 1 km. Such high resolution water vapour fields will provide valuable information for weather forecasters and researchers.
Xiaoyi Zhao, Vitali Fioletov, Debora Griffin, Chris McLinden, Ralf Staebler, Cristian Mihele, Kevin Strawbridge, Jonathan Davies, Ihab Abboud, Sum Chi Lee, Alexander Cede, Martin Tiefengraber, and Robert Swap
Atmos. Meas. Tech., 17, 6889–6912, https://doi.org/10.5194/amt-17-6889-2024, https://doi.org/10.5194/amt-17-6889-2024, 2024
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This study explores differences between remote sensing and in situ instruments in terms of their vertical, horizontal, and temporal sampling differences. Understanding and resolving these differences are critical for future analyses linking satellite, ground-based remote sensing, and in situ observations in air quality monitoring. It shows that the meteorological conditions (wind directions, speed, and boundary layer conditions) will strongly affect the agreement between the two measurements.
Leon Kuhn, Steffen Beirle, Sergey Osipov, Andrea Pozzer, and Thomas Wagner
Atmos. Meas. Tech., 17, 6485–6516, https://doi.org/10.5194/amt-17-6485-2024, https://doi.org/10.5194/amt-17-6485-2024, 2024
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This paper presents a new machine learning model that allows us to compute NO2 concentration profiles from satellite observations. A neural network was trained on synthetic data from the regional chemistry and transport model WRF-Chem. This is the first model of its kind. We present a thorough model validation study, covering various seasons and regions of the world.
Swathi Maratt Satheesan, Kai-Uwe Eichmann, John P. Burrows, Mark Weber, Ryan Stauffer, Anne M. Thompson, and Debra Kollonige
Atmos. Meas. Tech., 17, 6459–6484, https://doi.org/10.5194/amt-17-6459-2024, https://doi.org/10.5194/amt-17-6459-2024, 2024
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CHORA, an advanced cloud convective differential technique, enhances the accuracy of tropospheric-ozone retrievals. Unlike the traditional Pacific cloud reference sector scheme, CHORA introduces a local-cloud reference sector and an alternative approach (CLCT) for precision. Analysing monthly averaged TROPOMI data from 2018 to 2022 and validating with SHADOZ ozonesonde data, CLCT outperforms other methods and so is the preferred choice, especially in future geostationary satellite missions.
Minqiang Zhou, Pucai Wang, Bart Dils, Bavo Langerock, Geoff Toon, Christian Hermans, Weidong Nan, Qun Cheng, and Martine De Mazière
Atmos. Meas. Tech., 17, 6385–6396, https://doi.org/10.5194/amt-17-6385-2024, https://doi.org/10.5194/amt-17-6385-2024, 2024
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Solar absorption spectra near 2967 cm−1 recorded by a ground-based FTIR with a high spectral resolution of 0.0035 cm-1 are applied to retrieve C3H8 columns for the first time in Xianghe, China, within the NDACC-IRWG. The mean and standard deviation of the C3H8 columns are 1.80 ± 0.81 (1σ) × 1015 molec. cm-2. Good correlations are found between C3H8 and other non-methane hydrocarbons, such as C2H6 (R = 0.84) and C2H2 (R = 0.79), as well as between C3H8 and CO (R = 0.72).
Farrer Owsley-Brown, Martin J. Wooster, Mark J. Grosvenor, and Yanan Liu
Atmos. Meas. Tech., 17, 6247–6264, https://doi.org/10.5194/amt-17-6247-2024, https://doi.org/10.5194/amt-17-6247-2024, 2024
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Landscape fires produce vast amounts of smoke, affecting the atmosphere locally and globally. Whether a fire is flaming or smouldering strongly impacts the rate at which smoke is produced as well as its composition. This study tested two methods to determine these combustion phases in laboratory fires and compared them to the smoke emitted. One of these methods improved estimates of smoke emission significantly. This suggests potential for improvement in global emission estimates.
Sora Seo, Pieter Valks, Ronny Lutz, Klaus-Peter Heue, Pascal Hedelt, Víctor Molina García, Diego Loyola, Hanlim Lee, and Jhoon Kim
Atmos. Meas. Tech., 17, 6163–6191, https://doi.org/10.5194/amt-17-6163-2024, https://doi.org/10.5194/amt-17-6163-2024, 2024
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In this study, we developed an advanced retrieval algorithm for tropospheric NO2 columns from geostationary satellite spectrometers and applied it to GEMS measurements. The DLR GEMS NO2 retrieval algorithm follows the heritage from previous and existing algorithms, but improved approaches are applied to reflect the specific features of geostationary satellites. The DLR GEMS NO2 retrievals demonstrate a good capability for monitoring diurnal variability with a high spatial resolution.
Theodore K. Koenig, François Hendrick, Douglas Kinnison, Christopher F. Lee, Michel Van Roozendael, and Rainer Volkamer
Atmos. Meas. Tech., 17, 5911–5934, https://doi.org/10.5194/amt-17-5911-2024, https://doi.org/10.5194/amt-17-5911-2024, 2024
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Atmospheric bromine destroys ozone, impacts oxidation capacity, and oxidizes mercury into its toxic form. We constrain bromine by remote sensing of BrO from a mountaintop. Previous measurements retrieved two to three pieces of information vertically; we apply new methods to get five and a half vertically and two more in time. We compare with aircraft measurements to validate the methods and look at variations in BrO over the Pacific.
Kavitha Mottungan, Chayan Roychoudhury, Vanessa Brocchi, Benjamin Gaubert, Wenfu Tang, Mohammad Amin Mirrezaei, John McKinnon, Yafang Guo, David W. T. Griffith, Dietrich G. Feist, Isamu Morino, Mahesh K. Sha, Manvendra K. Dubey, Martine De Mazière, Nicholas M. Deutscher, Paul O. Wennberg, Ralf Sussmann, Rigel Kivi, Tae-Young Goo, Voltaire A. Velazco, Wei Wang, and Avelino F. Arellano Jr.
Atmos. Meas. Tech., 17, 5861–5885, https://doi.org/10.5194/amt-17-5861-2024, https://doi.org/10.5194/amt-17-5861-2024, 2024
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A combination of data analysis techniques is introduced to separate local and regional influences on observed levels of carbon dioxide, carbon monoxide, and methane from an established ground-based remote sensing network. We take advantage of the covariations in these trace gases to identify the dominant type of sources driving these levels. Applying these methods in conjunction with existing approaches to other datasets can better address uncertainties in identifying sources and sinks.
Chia-Pang Kuo and Christian Kummerow
Atmos. Meas. Tech., 17, 5637–5653, https://doi.org/10.5194/amt-17-5637-2024, https://doi.org/10.5194/amt-17-5637-2024, 2024
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A small satellite about the size of a shoe box, named TEMPEST, carries only a microwave sensor and is designed to measure the water cycle of the Earth from space in an economical way compared with traditional satellites, which have additional infrared sensors. To overcome the limitation, extra infrared signals from GOES-R ABI are combined with TEMPEST microwave measurements. Compared with ground observations, improved humidity information is extracted from the merged TEMPEST and ABI signals.
Christopher Chan Miller, Sébastien Roche, Jonas S. Wilzewski, Xiong Liu, Kelly Chance, Amir H. Souri, Eamon Conway, Bingkun Luo, Jenna Samra, Jacob Hawthorne, Kang Sun, Carly Staebell, Apisada Chulakadabba, Maryann Sargent, Joshua S. Benmergui, Jonathan E. Franklin, Bruce C. Daube, Yang Li, Joshua L. Laughner, Bianca C. Baier, Ritesh Gautam, Mark Omara, and Steven C. Wofsy
Atmos. Meas. Tech., 17, 5429–5454, https://doi.org/10.5194/amt-17-5429-2024, https://doi.org/10.5194/amt-17-5429-2024, 2024
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MethaneSAT is an upcoming satellite mission designed to monitor methane emissions from the oil and gas (O&G) industry globally. Here, we present observations from the first flight campaign of MethaneAIR, a MethaneSAT-like instrument mounted on an aircraft. MethaneAIR can map methane with high precision and accuracy over a typically sized oil and gas basin (~200 km2) in a single flight. This paper demonstrates the capability of the upcoming satellite to routinely track global O&G emissions.
Matthieu Dogniaux and Cyril Crevoisier
Atmos. Meas. Tech., 17, 5373–5396, https://doi.org/10.5194/amt-17-5373-2024, https://doi.org/10.5194/amt-17-5373-2024, 2024
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Many CO2-observing satellite concepts, with very different design choices and trade-offs, are expected to be put into orbit during the upcoming decade. This work uses numerical simulations to explore the impact of critical design parameters on the performance of upcoming CO2-observing satellite concepts.
Francesca Vittorioso, Vincent Guidard, and Nadia Fourrié
Atmos. Meas. Tech., 17, 5279–5299, https://doi.org/10.5194/amt-17-5279-2024, https://doi.org/10.5194/amt-17-5279-2024, 2024
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The future Meteosat Third Generation Infrared Sounder (MTG-IRS) will represent a major innovation for the monitoring of the chemical state of the atmosphere. MTG-IRS will have the advantage of being based on a geostationary platform and acquiring data with a high temporal frequency. This work aims to evaluate its potential impact over Europe within a chemical transport model (MOCAGE). The results indicate that the assimilation of these data always has a positive impact on ozone analysis.
Matthias Schneider, Kinya Toride, Farahnaz Khosrawi, Frank Hase, Benjamin Ertl, Christopher J. Diekmann, and Kei Yoshimura
Atmos. Meas. Tech., 17, 5243–5259, https://doi.org/10.5194/amt-17-5243-2024, https://doi.org/10.5194/amt-17-5243-2024, 2024
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Despite its importance for extreme weather and climate feedbacks, atmospheric convection is not well constrained. This study assesses the potential of novel tropospheric water vapour isotopologue satellite observations for improving the analyses of convective events. We find that the impact of the isotopologues is small for stable atmospheric conditions but significant for unstable conditions, which have the strongest societal impacts (e.g. storms and flooding).
Mengyao Liu, Ronald van der A, Michiel van Weele, Lotte Bryan, Henk Eskes, Pepijn Veefkind, Yongxue Liu, Xiaojuan Lin, Jos de Laat, and Jieying Ding
Atmos. Meas. Tech., 17, 5261–5277, https://doi.org/10.5194/amt-17-5261-2024, https://doi.org/10.5194/amt-17-5261-2024, 2024
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A new divergence method was developed and applied to estimate methane emissions from TROPOMI observations over the Middle East, where it is typically challenging for a satellite to measure methane due to its complicated orography and surface albedo. Our results show the potential of TROPOMI to quantify methane emissions from various sources rather than big emitters from space after objectively excluding the artifacts in the retrieval.
Yujin J. Oak, Daniel J. Jacob, Nicholas Balasus, Laura H. Yang, Heesung Chong, Junsung Park, Hanlim Lee, Gitaek T. Lee, Eunjo S. Ha, Rokjin J. Park, Hyeong-Ahn Kwon, and Jhoon Kim
Atmos. Meas. Tech., 17, 5147–5159, https://doi.org/10.5194/amt-17-5147-2024, https://doi.org/10.5194/amt-17-5147-2024, 2024
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We present an improved NO2 product from GEMS by calibrating it to TROPOMI using machine learning and by reprocessing both satellite products to adopt common NO2 profiles. Our corrected GEMS product combines the high data density of GEMS with the accuracy of TROPOMI, supporting the combined use for analyses of East Asia air quality including emissions and chemistry. This method can be extended to other species and geostationary satellites including TEMPO and Sentinel-4.
Xianzhong Duan, Ming Chang, Guotong Wu, Suping Situ, Shengjie Zhu, Qi Zhang, Yibo Huangfu, Weiwen Wang, Weihua Chen, Bin Yuan, and Xuemei Wang
Atmos. Meas. Tech., 17, 4065–4079, https://doi.org/10.5194/amt-17-4065-2024, https://doi.org/10.5194/amt-17-4065-2024, 2024
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Accurately estimating biogenic volatile organic compound (BVOC) emissions in forest ecosystems has been challenging. This research presents a framework that utilizes drone-based lidar, photogrammetry, and image recognition technologies to identify plant species and estimate BVOC emissions. The largest cumulative isoprene emissions were found in the Myrtaceae family, while those of monoterpenes were from the Rubiaceae family.
Fengxin Xie, Tao Ren, Changying Zhao, Yuan Wen, Yilei Gu, Minqiang Zhou, Pucai Wang, Kei Shiomi, and Isamu Morino
Atmos. Meas. Tech., 17, 3949–3967, https://doi.org/10.5194/amt-17-3949-2024, https://doi.org/10.5194/amt-17-3949-2024, 2024
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This study demonstrates a new machine learning approach to efficiently and accurately estimate atmospheric carbon dioxide levels from satellite data. Rather than using traditional complex physics-based retrieval methods, neural network models are trained on simulated data to rapidly predict CO2 concentrations directly from satellite spectral measurements.
Steffen Beirle and Thomas Wagner
Atmos. Meas. Tech., 17, 3439–3453, https://doi.org/10.5194/amt-17-3439-2024, https://doi.org/10.5194/amt-17-3439-2024, 2024
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We present a new method for estimating emissions and lifetimes for nitrogen oxides emitted from large cities by using satellite NO2 observations combined with wind fields. The estimate is based on the simultaneous evaluation of the downwind plumes for opposing wind directions. This allows us to derive seasonal mean emissions and lifetimes for 100 cities around the globe.
Qiurun Yu, Dylan Jervis, and Yi Huang
Atmos. Meas. Tech., 17, 3347–3366, https://doi.org/10.5194/amt-17-3347-2024, https://doi.org/10.5194/amt-17-3347-2024, 2024
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This study estimated the effects of aerosols on GHGSat satellite methane retrieval and investigated the performance of simultaneously retrieving aerosol and methane information using a multi-angle viewing method. Results suggested that the performance of GHGSat methane retrieval improved when aerosols were considered, and the multi-angle viewing method is insensitive to the satellite angle setting. This performance assessment is useful for improving future GHGSat-like instruments.
Zhonghua He, Ling Gao, Miao Liang, and Zhao-Cheng Zeng
Atmos. Meas. Tech., 17, 2937–2956, https://doi.org/10.5194/amt-17-2937-2024, https://doi.org/10.5194/amt-17-2937-2024, 2024
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Using Gaofen-5B satellite data, this study detected 93 methane plume events from 32 coal mines in Shanxi, China, with emission rates spanning from 761.78 ± 185.00 to 12729.12 ± 4658.13 kg h-1, showing significant variability among sources. This study highlights Gaofen-5B’s capacity for monitoring large methane point sources, offering valuable support in reducing greenhouse gas emissions.
Heesung Chong, Gonzalo González Abad, Caroline R. Nowlan, Christopher Chan Miller, Alfonso Saiz-Lopez, Rafael P. Fernandez, Hyeong-Ahn Kwon, Zolal Ayazpour, Huiqun Wang, Amir H. Souri, Xiong Liu, Kelly Chance, Ewan O'Sullivan, Jhoon Kim, Ja-Ho Koo, William R. Simpson, François Hendrick, Richard Querel, Glen Jaross, Colin Seftor, and Raid M. Suleiman
Atmos. Meas. Tech., 17, 2873–2916, https://doi.org/10.5194/amt-17-2873-2024, https://doi.org/10.5194/amt-17-2873-2024, 2024
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We present a new bromine monoxide (BrO) product derived using radiances measured from OMPS-NM on board the Suomi-NPP satellite. This product provides nearly a decade of global stratospheric and tropospheric column retrievals, a feature that is currently rare in publicly accessible datasets. Both stratospheric and tropospheric columns from OMPS-NM demonstrate robust performance, exhibiting good agreement with ground-based observations collected at three stations (Lauder, Utqiagvik, and Harestua).
Norbert Glatthor, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 17, 2849–2871, https://doi.org/10.5194/amt-17-2849-2024, https://doi.org/10.5194/amt-17-2849-2024, 2024
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We present global atmospheric methane (CH4) and nitrous oxide (N2O) distributions retrieved from measurements of the MIPAS instrument on board the Environmental Satellite (Envisat) during 2002 to 2012. Monitoring of these gases is of scientific interest because both of them are strong greenhouse gases. We analyze the latest, improved version of calibrated MIPAS measurements. Further, we apply a new retrieval scheme leading to an improved CH4 and N2O data product .
Cited articles
Benner, D. C., Devi, V. M., Nugent, E., Sung, K., Brown, L. R., Miller C. E., and Toth, R. A.: Line parameters of carbon dioxide in the 4850 cm−1 region, Twenty-second Coll. on High Res. Mol. Spectrosc., Dijon, France, poster N19, 2011.
Bösch, H., Baker, D., Connor, B., Crisp, D., and Miller, C.: Global Characterization of CO2 Column Retrievals from Shortwave-Infrared Satellite Observations of the Orbiting Carbon Observatory-2 Mission, Remote Sens., 3, 270–304, 2011.
Brown, L. R. and Plymate, C.: Experimental Line Parameters of the Oxygen A Band at 760 nm, J. Mol. Spectrosc. 199, 166–179, 2000.
Buchard, V., da Silva, A. M., Colarco, P. R., Darmenov, A., Randles, C. A., Govindaraju, R., Torres, O., Campbell, J., and Spurr, R.: Using the OMI aerosol index and absorption aerosol optical depth to evaluate the NASA MERRA Aerosol Reanalysis, Atmos. Chem. Phys., 15, 5743–5760, https://doi.org/10.5194/acp-15-5743-2015, 2015.
Butz, A., Hasekamp, O. P., Frankenberg, C., and Aben, I.: Retrievals of atmospheric CO2 from simulated space-borne measurements of backscattered near-infrared sunlight: accounting for aerosol effects, Appl. Optics, 48, 3322–3336, 2009.
Connor, B. J., Bösch, H., Toon, G., Sen, B., Miller, C., and Crisp, D.: Orbiting Carbon Observatory: Inverse method and prospective error analysis, J. Geophys. Res., 113, D05305, https://doi.org/10.1029/2006JD008336, 2008.
Crisp, D., Miller, C., and DeCola, P.: NASA Orbiting Carbon Observatory; measuring the column averaged carbon dioxide mole fraction from space, J. Appl. Remote Sens., 2, 023508, https://doi.org/10.1117/1.2898457, 2008.
Devi, V. M., Benner, D. C., Brown, L. R., Miller, C. E., and Toth, R. A.: Line mixing and speed dependence in CO2 at 6227.9 cm−1: Constrained multispectrum analysis of intensities and line shapes in the 30013 ← 00001 band, J. Mol. Spectrosc. 245, 52–80, 2007.
Devi, V. M., Benner, D. C., Sung, K., Brown, L. R., Crawford, T. J., Miller, C. E., Drouin, B. J., Payne, V. H., Yu, S., Smith, M. A. H., Mantz, A. M., and Gamache, R. R.: Line parameters including temperature dependences of self- and air-broadened line shapes of 12C16O2: 1.6-μm region, J. Quant. Spectrosc. and Ra., 177, 117–144, 2016.
Drouin, B. J., Benner, D. C., Brown, L. R., Cich, M. J., Crawford, T. J., Devi, V. M., Guillaume, A., Hodges, J. T., Mlawer, E. J., Robichaud, D. J., Oyafuso, F., Payne, V. H., Sung, K., Wishnow, E. H., and Yu, S.: Multispectrum analysis of the oxygen A-band, J. Quant. Spectrosc. Ra., in press, 2016.
Joly, L., Marnas, F., Gibert, F., Bruneau, D., Grouiz, B., Flamant, P. H., Durry, G., Dumelie, N., Parvitte, B., and Zeninari, V.: Laser diode absorption spectroscopy for accurate CO2 line parameters at 2 microns: consequences for space-based DIAL measurements and potential biases, Appl. Optics, 48, 5475–5483, 2009.
JPL: OCO-2 Level 2 Full Physics Retrieval Algorithm Theoretical Basis, Version 2.0 Rev 2, available at: http://disc.sci.gsfc.nasa.gov/OCO-2/documentation/oco-2-v6/OCO2_L2_ATBD.V6.pdf, 2015.
Jung, Y., Kim, J., Kim, W. Boesch, H., Lee, H., Cho, C., and Tae-Young, G.: Impact of Aerosol Property on the Accuracy of a CO2 Retrieval Algorithm from Satellite Remote Sensing, Remote Sens., 8, 322, https://doi.org/10.3390/rs8040322, 2016.
Lee, R. A. M., O'Dell, C. W., Wunch, D., Roehl, C. M., Osterman, G. B., Blavier, J.-F., Rosenberg, R., Chapsky, L., Frankenberg, C., Hunyadi-Lay, S. L., Fisher, B. M., Rider, D. M., Crisp, D., and Pollock, R.: Preflight Spectral Calibration of the Orbiting Carbon Observatory, IEEE T. Geosci. Remote, submitted, 2016.
Long, D. A., Havey, D. K., Okumura, M., Miller, C. E., and Hodges, J. T.: O2 A-band line parameters to support atmospheric remote sensing, J. Quant. Spectrosc. Ra., 111, 2021–2036, https://doi.org/10.1016/j.jqsrt.2010.05.011, 2010.
Long, D. A., Robichaud, D. J., and Hodges, J. T.: Frequency-stabilized cavity ring-down spectroscopy measurements of line mixing and collision-induced absorption in the O2 A-band, J. Chem. Phys. 137, 014307; https://doi.org/10.1063/1.4731290, 2012.
O'Brien, D. M., Polonsky, I., O'Dell, C., and Carheden, A.: Orbiting Carbon Observatory (OCO), Algorithm Theoretical Basis Document, the OCO simulator, Technical Report ISSN 0737-5352-85, Cooperative Institute for Research in the Atmosphere, Colorado State University, Fort Collins, CO, USA, 2009.
O'Dell, C. W., Connor, B., Bösch, H., O'Brien, D., Frankenberg, C., Castano, R., Christi, M., Eldering, D., Fisher, B., Gunson, M., McDuffie, J., Miller, C. E., Natraj, V., Oyafuso, F., Polonsky, I., Smyth, M., Taylor, T., Toon, G. C., Wennberg, P. O., and Wunch, D.: The ACOS CO2 retrieval algorithm – Part 1: Description and validation against synthetic observations, Atmos. Meas. Tech., 5, 99–121, https://doi.org/10.5194/amt-5-99-2012, 2012.
Polyansky, O. L., Bielska, K., Ghysels, M., Lodi, L., Zobov, N. F., Hodges, J. T., and Tennyson, J.: High-accuracy CO2 line intensities determined from theory and experiment, Phys. Rev. Lett., 114, 243001, https://doi.org/10.1103/PhysRevLett.114.243001, 2015.
Rienecker, M. M., Suarez, M. J., Gelaro, R., Todling, R., Bacmeister, J., Liu, E., Bosilovich, M. G., Schubert, S. D., Takacs, L., Kim, G.-K., Bloom, S., Chen, J., Collins, D., Conaty, A., da Silva, A., Gu, W., Joiner, J., Koster, R. D., Lucchesi, R., Molod, A., Owens, T., Pawson, S., Pegion, P., Redder, C. R., Reichle, R., Robertson, F. R., Ruddick, A. G., Sienkiewicz, M., and Woollen, J., MERRA: NASA's Modern-Era Retrospective Analysis for Research and Applications, J. Climate, 24, 3624–3648, 2011.
Robichaud, D. J., Hodges, J. T., Brown, L. R., Lisak, D., Maslowski, P., Yeung, L. Y., Okumura, M., and Miller, C. E.: Experimental intensity and line shape parameters of the oxygen A-band using frequency-stabilized cavity ring-down spectroscopy, J. Mol. Spectrosc., 248, 1–13, 2008.
Rodgers C. D.: Inverse Methods for Atmospheric Sounding, World Scientific, Singapore, 2000.
Rodgers, C. D. and Connor, B. J.: Intercomparison of remote sounding instruments, J. Geophys. Res. 108, 4116, https://doi.org/10.1029/2002JD002299, 2003.
Rosenberg, R., Maxwell, S., Johnson B. C., Chapsky, L., Lee, R. A. M., and Pollock, R.: Preflight Radiometric Calibration of Orbiting Carbon Observatory, IEEE T. Geosci. Remote, 2, in press, 2016.
Sung, K., Brown, L. R., Toth, R. A., and Crawford, T. J.: Fourier transform infrared spectroscopy measurements of H20-broadened half-widths of CO2 at 4.3 um, Can. J. Phys., 87, 469–484, 2009.
Taylor, T. E., O'Dell, C. W., Frankenberg, C., Partain, P. T., Cronk, H. Q., Savtchenko, A., Nelson, R. R., Rosenthal, E. J., Chang, A. Y., Fisher, B., Osterman, G. B., Pollock, R. H., Crisp, D., Eldering, A., and Gunson, M. R.: Orbiting Carbon Observatory-2 (OCO-2) cloud screening algorithms: validation against collocated MODIS and CALIOP data, Atmos. Meas. Tech., 9, 973–989, https://doi.org/10.5194/amt-9-973-2016, 2016.
Wunch, D., Wennberg, P. O., Toon, G. C., Connor, B. J., Fisher, B., Osterman, G. B., Frankenberg, C., Mandrake, L., O'Dell, C., Ahonen, P., Biraud, S. C., Castano, R., Cressie, N., Crisp, D., Deutscher, N. M., Eldering, A., Fisher, M. L., Griffith, D. W. T., Gunson, M., Heikkinen, P., Keppel-Aleks, G., Kyrö, E., Lindenmaier, R., Macatangay, R., Mendonca, J., Messerschmidt, J., Miller, C. E., Morino, I., Notholt, J., Oyafuso, F. A., Rettinger, M., Robinson, J., Roehl, C. M., Salawitch, R. J., Sherlock, V., Strong, K., Sussmann, R., Tanaka, T., Thompson, D. R., Uchino, O., Warneke, T., and Wofsy, S. C.: A method for evaluating bias in global measurements of CO2 total columns from space, Atmos. Chem. Phys., 11, 12317–12337, https://doi.org/10.5194/acp-11-12317-2011, 2011.
Yoshida, Y., Ota, Y., Eguchi, N., Kikuchi, N., Nobuta, K., Tran, H., Morino, I., and Yokota, T.: Retrieval algorithm for CO2 and CH4 column abundances from short-wavelength infrared spectral observations by the Greenhouse gases observing satellite, Atmos. Meas. Tech., 4, 717–734, https://doi.org/10.5194/amt-4-717-2011, 2011.
Short summary
We present an analysis of uncertainties in global measurements of the column-averaged dry-air mole fraction of CO2 (XCO2) by the satellite OCO-2. The analysis is based on our best estimates for uncertainties in the OCO-2 operational algorithm and its inputs. From these results we estimate the "variable error", which differs between soundings, to infer the error in the difference of XCO2 between any two soundings. Variable errors are usually < 1 ppm over ocean and ~ 0.5–2 ppm over land.
We present an analysis of uncertainties in global measurements of the column-averaged dry-air...
