Articles | Volume 11, issue 3
https://doi.org/10.5194/amt-11-1833-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-11-1833-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
29 Mar 2018
Research article |
| 29 Mar 2018
| 29 Mar 2018
COCAP: a carbon dioxide analyser for small unmanned aircraft systems
Max Planck Institute for Biogeochemistry, Jena, Germany
Jost V. Lavric
Max Planck Institute for Biogeochemistry, Jena, Germany
Christoph Gerbig
Max Planck Institute for Biogeochemistry, Jena, Germany
Pieter Tans
NOAA Earth System Research Laboratory, Global Monitoring Division,
Boulder, Colorado, USA
Don Neff
NOAA Earth System Research Laboratory, Global Monitoring Division,
Boulder, Colorado, USA
Christine Hummelgård
SenseAir AB, Delsbo, Sweden
Hans Martin
SenseAir AB, Delsbo, Sweden
Henrik Rödjegård
SenseAir AB, Delsbo, Sweden
Burkhard Wrenger
Ostwestfalen-Lippe University of Applied Sciences, Höxter, Germany
Martin Heimann
Max Planck Institute for Biogeochemistry, Jena, Germany
Division of Atmospheric Sciences, Department of Physics, University
of Helsinki, Helsinki, Finland
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Earth Syst. Sci. Data, 15, 4295–4370, https://doi.org/10.5194/essd-15-4295-2023, https://doi.org/10.5194/essd-15-4295-2023, 2023
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Accurate estimation of fluxes of carbon dioxide from the land surface is essential for understanding future impacts of greenhouse gas emissions on the climate system. A wide variety of methods currently exist to estimate these sources and sinks. We are continuing work to develop annual comparisons of these diverse methods in order to clarify what they all actually calculate and to resolve apparent disagreement, in addition to highlighting opportunities for increased understanding.
Theertha Kariyathan, Ana Bastos, Julia Marshall, Wouter Peters, Pieter Tans, and Markus Reichstein
Atmos. Meas. Tech., 16, 3299–3312, https://doi.org/10.5194/amt-16-3299-2023, https://doi.org/10.5194/amt-16-3299-2023, 2023
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Saqr Munassar, Guillaume Monteil, Marko Scholze, Ute Karstens, Christian Rödenbeck, Frank-Thomas Koch, Kai U. Totsche, and Christoph Gerbig
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Dominik Brunner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys., 23, 2699–2728, https://doi.org/10.5194/acp-23-2699-2023, https://doi.org/10.5194/acp-23-2699-2023, 2023
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We evaluated six atmospheric transport models for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet (Carbon Dioxide and Methane Mission) campaign in 2018. The study analyzed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Sourish Basu, Xin Lan, Edward Dlugokencky, Sylvia Michel, Stefan Schwietzke, John B. Miller, Lori Bruhwiler, Youmi Oh, Pieter P. Tans, Francesco Apadula, Luciana V. Gatti, Armin Jordan, Jaroslaw Necki, Motoki Sasakawa, Shinji Morimoto, Tatiana Di Iorio, Haeyoung Lee, Jgor Arduini, and Giovanni Manca
Atmos. Chem. Phys., 22, 15351–15377, https://doi.org/10.5194/acp-22-15351-2022, https://doi.org/10.5194/acp-22-15351-2022, 2022
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Vishnu Thilakan, Dhanyalekshmi Pillai, Christoph Gerbig, Michal Galkowski, Aparnna Ravi, and Thara Anna Mathew
Atmos. Chem. Phys., 22, 15287–15312, https://doi.org/10.5194/acp-22-15287-2022, https://doi.org/10.5194/acp-22-15287-2022, 2022
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This paper demonstrates how we can use atmospheric observations to improve the CO2 flux estimates in India. This is achieved by improving the representation of terrain, mesoscale transport, and flux variations. We quantify the impact of the unresolved variations in the current models on optimally estimated fluxes via inverse modelling and quantify the associated flux uncertainty. We illustrate how a parameterization scheme captures this variability in the coarse models.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Luke Gregor, Judith Hauck, Corinne Le Quéré, Ingrid T. Luijkx, Are Olsen, Glen P. Peters, Wouter Peters, Julia Pongratz, Clemens Schwingshackl, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone R. Alin, Ramdane Alkama, Almut Arneth, Vivek K. Arora, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Henry C. Bittig, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Margot Cronin, Wiley Evans, Stefanie Falk, Richard A. Feely, Thomas Gasser, Marion Gehlen, Thanos Gkritzalis, Lucas Gloege, Giacomo Grassi, Nicolas Gruber, Özgür Gürses, Ian Harris, Matthew Hefner, Richard A. Houghton, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Atul K. Jain, Annika Jersild, Koji Kadono, Etsushi Kato, Daniel Kennedy, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Peter Landschützer, Nathalie Lefèvre, Keith Lindsay, Junjie Liu, Zhu Liu, Gregg Marland, Nicolas Mayot, Matthew J. McGrath, Nicolas Metzl, Natalie M. Monacci, David R. Munro, Shin-Ichiro Nakaoka, Yosuke Niwa, Kevin O'Brien, Tsuneo Ono, Paul I. Palmer, Naiqing Pan, Denis Pierrot, Katie Pocock, Benjamin Poulter, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Carmen Rodriguez, Thais M. Rosan, Jörg Schwinger, Roland Séférian, Jamie D. Shutler, Ingunn Skjelvan, Tobias Steinhoff, Qing Sun, Adrienne J. Sutton, Colm Sweeney, Shintaro Takao, Toste Tanhua, Pieter P. Tans, Xiangjun Tian, Hanqin Tian, Bronte Tilbrook, Hiroyuki Tsujino, Francesco Tubiello, Guido R. van der Werf, Anthony P. Walker, Rik Wanninkhof, Chris Whitehead, Anna Willstrand Wranne, Rebecca Wright, Wenping Yuan, Chao Yue, Xu Yue, Sönke Zaehle, Jiye Zeng, and Bo Zheng
Earth Syst. Sci. Data, 14, 4811–4900, https://doi.org/10.5194/essd-14-4811-2022, https://doi.org/10.5194/essd-14-4811-2022, 2022
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The Global Carbon Budget 2022 describes the datasets and methodology used to quantify the anthropogenic emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, the land ecosystems, and the ocean. These living datasets are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Simone M. Pieber, Béla Tuzson, Stephan Henne, Ute Karstens, Christoph Gerbig, Frank-Thomas Koch, Dominik Brunner, Martin Steinbacher, and Lukas Emmenegger
Atmos. Chem. Phys., 22, 10721–10749, https://doi.org/10.5194/acp-22-10721-2022, https://doi.org/10.5194/acp-22-10721-2022, 2022
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Understanding regional greenhouse gas emissions into the atmosphere is a prerequisite to mitigate climate change. In this study, we investigated the regional contributions of carbon dioxide (CO2) at the location of the high Alpine observatory Jungfraujoch (JFJ, Switzerland, 3580 m a.s.l.). To this purpose, we combined receptor-oriented atmospheric transport simulations for CO2 concentration in the period 2009–2017 with stable carbon isotope (δ13C–CO2) information.
Fabian Maier, Christoph Gerbig, Ingeborg Levin, Ingrid Super, Julia Marshall, and Samuel Hammer
Geosci. Model Dev., 15, 5391–5406, https://doi.org/10.5194/gmd-15-5391-2022, https://doi.org/10.5194/gmd-15-5391-2022, 2022
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We show that the default representation of point source emissions in WRF–STILT leads to large overestimations when modelling fossil fuel CO2 concentrations for a 30 m high observation site during stable atmospheric conditions. We therefore introduce a novel point source modelling approach in WRF-STILT that takes into account their effective emission heights and results in a much better agreement with observations.
Saqr Munassar, Christian Rödenbeck, Frank-Thomas Koch, Kai U. Totsche, Michał Gałkowski, Sophia Walther, and Christoph Gerbig
Atmos. Chem. Phys., 22, 7875–7892, https://doi.org/10.5194/acp-22-7875-2022, https://doi.org/10.5194/acp-22-7875-2022, 2022
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The results obtained from ensembles of inversions over 13 years show the largest spread in the a posteriori fluxes over the station set ensemble. Using different prior fluxes in the inversions led to a smaller impact. Drought occurrences in 2018 and 2019 affected CO2 fluxes as seen in net ecosystem exchange estimates. Our study highlights the importance of expanding the atmospheric site network across Europe to better constrain CO2 fluxes in inverse modelling.
Pierre Friedlingstein, Matthew W. Jones, Michael O'Sullivan, Robbie M. Andrew, Dorothee C. E. Bakker, Judith Hauck, Corinne Le Quéré, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Rob B. Jackson, Simone R. Alin, Peter Anthoni, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Laurent Bopp, Thi Tuyet Trang Chau, Frédéric Chevallier, Louise P. Chini, Margot Cronin, Kim I. Currie, Bertrand Decharme, Laique M. Djeutchouang, Xinyu Dou, Wiley Evans, Richard A. Feely, Liang Feng, Thomas Gasser, Dennis Gilfillan, Thanos Gkritzalis, Giacomo Grassi, Luke Gregor, Nicolas Gruber, Özgür Gürses, Ian Harris, Richard A. Houghton, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Ingrid T. Luijkx, Atul Jain, Steve D. Jones, Etsushi Kato, Daniel Kennedy, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Arne Körtzinger, Peter Landschützer, Siv K. Lauvset, Nathalie Lefèvre, Sebastian Lienert, Junjie Liu, Gregg Marland, Patrick C. McGuire, Joe R. Melton, David R. Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Yosuke Niwa, Tsuneo Ono, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Thais M. Rosan, Jörg Schwinger, Clemens Schwingshackl, Roland Séférian, Adrienne J. Sutton, Colm Sweeney, Toste Tanhua, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco Tubiello, Guido R. van der Werf, Nicolas Vuichard, Chisato Wada, Rik Wanninkhof, Andrew J. Watson, David Willis, Andrew J. Wiltshire, Wenping Yuan, Chao Yue, Xu Yue, Sönke Zaehle, and Jiye Zeng
Earth Syst. Sci. Data, 14, 1917–2005, https://doi.org/10.5194/essd-14-1917-2022, https://doi.org/10.5194/essd-14-1917-2022, 2022
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The Global Carbon Budget 2021 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Hanna K. Lappalainen, Tuukka Petäjä, Timo Vihma, Jouni Räisänen, Alexander Baklanov, Sergey Chalov, Igor Esau, Ekaterina Ezhova, Matti Leppäranta, Dmitry Pozdnyakov, Jukka Pumpanen, Meinrat O. Andreae, Mikhail Arshinov, Eija Asmi, Jianhui Bai, Igor Bashmachnikov, Boris Belan, Federico Bianchi, Boris Biskaborn, Michael Boy, Jaana Bäck, Bin Cheng, Natalia Chubarova, Jonathan Duplissy, Egor Dyukarev, Konstantinos Eleftheriadis, Martin Forsius, Martin Heimann, Sirkku Juhola, Vladimir Konovalov, Igor Konovalov, Pavel Konstantinov, Kajar Köster, Elena Lapshina, Anna Lintunen, Alexander Mahura, Risto Makkonen, Svetlana Malkhazova, Ivan Mammarella, Stefano Mammola, Stephany Buenrostro Mazon, Outi Meinander, Eugene Mikhailov, Victoria Miles, Stanislav Myslenkov, Dmitry Orlov, Jean-Daniel Paris, Roberta Pirazzini, Olga Popovicheva, Jouni Pulliainen, Kimmo Rautiainen, Torsten Sachs, Vladimir Shevchenko, Andrey Skorokhod, Andreas Stohl, Elli Suhonen, Erik S. Thomson, Marina Tsidilina, Veli-Pekka Tynkkynen, Petteri Uotila, Aki Virkkula, Nadezhda Voropay, Tobias Wolf, Sayaka Yasunaka, Jiahua Zhang, Yubao Qiu, Aijun Ding, Huadong Guo, Valery Bondur, Nikolay Kasimov, Sergej Zilitinkevich, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 22, 4413–4469, https://doi.org/10.5194/acp-22-4413-2022, https://doi.org/10.5194/acp-22-4413-2022, 2022
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We summarize results during the last 5 years in the northern Eurasian region, especially from Russia, and introduce recent observations of the air quality in the urban environments in China. Although the scientific knowledge in these regions has increased, there are still gaps in our understanding of large-scale climate–Earth surface interactions and feedbacks. This arises from limitations in research infrastructures and integrative data analyses, hindering a comprehensive system analysis.
Pieter Tans
Atmos. Meas. Tech., 15, 1903–1916, https://doi.org/10.5194/amt-15-1903-2022, https://doi.org/10.5194/amt-15-1903-2022, 2022
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The AirCore collects a continuous air sample in a long tube that can be read later when the captured air is slowly pushed through an analyzer. Much of the variation of gas composition encountered during collection is preserved, like having up to ~ 100 separate air samples. This is illustrated through examples of actual flights, and the analysis algorithm is described. The AirCore provides access to air as high as the mid stratosphere, enabling validation for satellite air composition soundings.
Sven Krautwurst, Konstantin Gerilowski, Jakob Borchardt, Norman Wildmann, Michał Gałkowski, Justyna Swolkień, Julia Marshall, Alina Fiehn, Anke Roiger, Thomas Ruhtz, Christoph Gerbig, Jaroslaw Necki, John P. Burrows, Andreas Fix, and Heinrich Bovensmann
Atmos. Chem. Phys., 21, 17345–17371, https://doi.org/10.5194/acp-21-17345-2021, https://doi.org/10.5194/acp-21-17345-2021, 2021
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Quantification of anthropogenic CH4 emissions remains challenging, but it is essential for near-term climate mitigation strategies. We use airborne remote sensing observations to assess bottom-up estimates of coal mining emissions from one of Europe's largest CH4 emission hot spots located in Poland. The analysis reveals that emissions from small groups of shafts can be disentangled, but caution is advised when comparing observations to commonly reported annual emissions.
Antoine Berchet, Espen Sollum, Rona L. Thompson, Isabelle Pison, Joël Thanwerdas, Grégoire Broquet, Frédéric Chevallier, Tuula Aalto, Adrien Berchet, Peter Bergamaschi, Dominik Brunner, Richard Engelen, Audrey Fortems-Cheiney, Christoph Gerbig, Christine D. Groot Zwaaftink, Jean-Matthieu Haussaire, Stephan Henne, Sander Houweling, Ute Karstens, Werner L. Kutsch, Ingrid T. Luijkx, Guillaume Monteil, Paul I. Palmer, Jacob C. A. van Peet, Wouter Peters, Philippe Peylin, Elise Potier, Christian Rödenbeck, Marielle Saunois, Marko Scholze, Aki Tsuruta, and Yuanhong Zhao
Geosci. Model Dev., 14, 5331–5354, https://doi.org/10.5194/gmd-14-5331-2021, https://doi.org/10.5194/gmd-14-5331-2021, 2021
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We present here the Community Inversion Framework (CIF) to help rationalize development efforts and leverage the strengths of individual inversion systems into a comprehensive framework. The CIF is a programming protocol to allow various inversion bricks to be exchanged among researchers.
The ensemble of bricks makes a flexible, transparent and open-source Python-based tool. We describe the main structure and functionalities and demonstrate it in a simple academic case.
Kyle B. Delwiche, Sara Helen Knox, Avni Malhotra, Etienne Fluet-Chouinard, Gavin McNicol, Sarah Feron, Zutao Ouyang, Dario Papale, Carlo Trotta, Eleonora Canfora, You-Wei Cheah, Danielle Christianson, Ma. Carmelita R. Alberto, Pavel Alekseychik, Mika Aurela, Dennis Baldocchi, Sheel Bansal, David P. Billesbach, Gil Bohrer, Rosvel Bracho, Nina Buchmann, David I. Campbell, Gerardo Celis, Jiquan Chen, Weinan Chen, Housen Chu, Higo J. Dalmagro, Sigrid Dengel, Ankur R. Desai, Matteo Detto, Han Dolman, Elke Eichelmann, Eugenie Euskirchen, Daniela Famulari, Kathrin Fuchs, Mathias Goeckede, Sébastien Gogo, Mangaliso J. Gondwe, Jordan P. Goodrich, Pia Gottschalk, Scott L. Graham, Martin Heimann, Manuel Helbig, Carole Helfter, Kyle S. Hemes, Takashi Hirano, David Hollinger, Lukas Hörtnagl, Hiroki Iwata, Adrien Jacotot, Gerald Jurasinski, Minseok Kang, Kuno Kasak, John King, Janina Klatt, Franziska Koebsch, Ken W. Krauss, Derrick Y. F. Lai, Annalea Lohila, Ivan Mammarella, Luca Belelli Marchesini, Giovanni Manca, Jaclyn Hatala Matthes, Trofim Maximov, Lutz Merbold, Bhaskar Mitra, Timothy H. Morin, Eiko Nemitz, Mats B. Nilsson, Shuli Niu, Walter C. Oechel, Patricia Y. Oikawa, Keisuke Ono, Matthias Peichl, Olli Peltola, Michele L. Reba, Andrew D. Richardson, William Riley, Benjamin R. K. Runkle, Youngryel Ryu, Torsten Sachs, Ayaka Sakabe, Camilo Rey Sanchez, Edward A. Schuur, Karina V. R. Schäfer, Oliver Sonnentag, Jed P. Sparks, Ellen Stuart-Haëntjens, Cove Sturtevant, Ryan C. Sullivan, Daphne J. Szutu, Jonathan E. Thom, Margaret S. Torn, Eeva-Stiina Tuittila, Jessica Turner, Masahito Ueyama, Alex C. Valach, Rodrigo Vargas, Andrej Varlagin, Alma Vazquez-Lule, Joseph G. Verfaillie, Timo Vesala, George L. Vourlitis, Eric J. Ward, Christian Wille, Georg Wohlfahrt, Guan Xhuan Wong, Zhen Zhang, Donatella Zona, Lisamarie Windham-Myers, Benjamin Poulter, and Robert B. Jackson
Earth Syst. Sci. Data, 13, 3607–3689, https://doi.org/10.5194/essd-13-3607-2021, https://doi.org/10.5194/essd-13-3607-2021, 2021
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Methane is an important greenhouse gas, yet we lack knowledge about its global emissions and drivers. We present FLUXNET-CH4, a new global collection of methane measurements and a critical resource for the research community. We use FLUXNET-CH4 data to quantify the seasonality of methane emissions from freshwater wetlands, finding that methane seasonality varies strongly with latitude. Our new database and analysis will improve wetland model accuracy and inform greenhouse gas budgets.
Ana Maria Roxana Petrescu, Matthew J. McGrath, Robbie M. Andrew, Philippe Peylin, Glen P. Peters, Philippe Ciais, Gregoire Broquet, Francesco N. Tubiello, Christoph Gerbig, Julia Pongratz, Greet Janssens-Maenhout, Giacomo Grassi, Gert-Jan Nabuurs, Pierre Regnier, Ronny Lauerwald, Matthias Kuhnert, Juraj Balkovič, Mart-Jan Schelhaas, Hugo A. C. Denier van der
Gon, Efisio Solazzo, Chunjing Qiu, Roberto Pilli, Igor B. Konovalov, Richard A. Houghton, Dirk Günther, Lucia Perugini, Monica Crippa, Raphael Ganzenmüller, Ingrid T. Luijkx, Pete Smith, Saqr Munassar, Rona L. Thompson, Giulia Conchedda, Guillaume Monteil, Marko Scholze, Ute Karstens, Patrick Brockmann, and Albertus Johannes Dolman
Earth Syst. Sci. Data, 13, 2363–2406, https://doi.org/10.5194/essd-13-2363-2021, https://doi.org/10.5194/essd-13-2363-2021, 2021
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This study is topical and provides a state-of-the-art scientific overview of data availability from bottom-up and top-down CO2 fossil emissions and CO2 land fluxes in the EU27+UK. The data integrate recent emission inventories with ecosystem data, land carbon models and regional/global inversions for the European domain, aiming at reconciling CO2 estimates with official country-level UNFCCC national GHG inventories in support to policy and facilitating real-time verification procedures.
Vishnu Thilakan, Dhanyalekshmi Pillai, Christoph Gerbig, Michal Galkowski, Aparnna Ravi, and Thara Anna Mathew
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-392, https://doi.org/10.5194/acp-2021-392, 2021
Revised manuscript not accepted
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This paper demonstrates how we can make use of atmospheric observations to improve the CO2 flux estimates of India. This is achieved by improving the representation of terrain, mesoscale transport and flux variations. We quantify the impact of unresolved variations in the current models on optimally estimated fluxes via inverse modelling and quantify the associated flux uncertainty. We illustrate how a parameterization scheme captures this variability in the coarse models.
Eva Y. Pfannerstill, Nina G. Reijrink, Achim Edtbauer, Akima Ringsdorf, Nora Zannoni, Alessandro Araújo, Florian Ditas, Bruna A. Holanda, Marta O. Sá, Anywhere Tsokankunku, David Walter, Stefan Wolff, Jošt V. Lavrič, Christopher Pöhlker, Matthias Sörgel, and Jonathan Williams
Atmos. Chem. Phys., 21, 6231–6256, https://doi.org/10.5194/acp-21-6231-2021, https://doi.org/10.5194/acp-21-6231-2021, 2021
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Tropical forests are globally significant for atmospheric chemistry. However, the mixture of reactive organic gases emitted by these ecosystems is poorly understood. By comprehensive observations at an Amazon forest site, we show that oxygenated species were previously underestimated in their contribution to the tropical-forest reactant mix. Our results show rain and temperature effects and have implications for models and the understanding of ozone and particle formation above tropical forests.
Bradley D. Hall, Andrew M. Crotwell, Duane R. Kitzis, Thomas Mefford, Benjamin R. Miller, Michael F. Schibig, and Pieter P. Tans
Atmos. Meas. Tech., 14, 3015–3032, https://doi.org/10.5194/amt-14-3015-2021, https://doi.org/10.5194/amt-14-3015-2021, 2021
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We have recently revised the carbon dioxide calibration scale used by numerous laboratories that measure atmospheric CO2. The revision follows from an improved understanding of the manometric method used to determine the absolute amount of CO2 in an atmospheric air sample. The new scale is 0.18 μmol mol−1 (ppm) greater than the previous scale at 400 ppm CO2. While this difference is small in relative terms (0.045 %), it is significant in terms of atmospheric monitoring.
Ashique Vellalassery, Dhanyalekshmi Pillai, Julia Marshall, Christoph Gerbig, Michael Buchwitz, Oliver Schneising, and Aparnna Ravi
Atmos. Chem. Phys., 21, 5393–5414, https://doi.org/10.5194/acp-21-5393-2021, https://doi.org/10.5194/acp-21-5393-2021, 2021
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We investigate factors contributing to the severe and persistent air quality degradation in northern India that has worsened during every winter over the last decade. This is achieved by implementing atmospheric modelling and using recently available Sentinel-5 P satellite data for carbon monoxide. We see a minimal role of biomass burning, except for the state of Punjab. The aim is to focus on residential and industrial emission reduction strategies to tackle air pollution over northern India.
Michał Gałkowski, Armin Jordan, Michael Rothe, Julia Marshall, Frank-Thomas Koch, Jinxuan Chen, Anna Agusti-Panareda, Andreas Fix, and Christoph Gerbig
Atmos. Meas. Tech., 14, 1525–1544, https://doi.org/10.5194/amt-14-1525-2021, https://doi.org/10.5194/amt-14-1525-2021, 2021
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We present results of atmospheric measurements of greenhouse gases, performed over Europe in 2018 aboard German research aircraft HALO as part of the CoMet 1.0 (Carbon Dioxide and Methane Mission). In our analysis, we describe data quality, discuss observed mixing ratios and show an example of describing a regional methane source using stable isotopic composition based on the collected air samples. We also quantitatively compare our results to selected global atmospheric modelling systems.
Shujiro Komiya, Fumiyoshi Kondo, Heiko Moossen, Thomas Seifert, Uwe Schultz, Heike Geilmann, David Walter, and Jost V. Lavric
Atmos. Meas. Tech., 14, 1439–1455, https://doi.org/10.5194/amt-14-1439-2021, https://doi.org/10.5194/amt-14-1439-2021, 2021
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The Amazon basin influences the atmospheric and hydrological cycles on local to global scales. To better understand how, we plan to perform continuous on-site measurements of the stable isotope composition of atmospheric water vapour. For making accurate on-site observations possible, we have investigated the performance of two commercial analysers and determined the best calibration strategy. Well calibrated, both analysers will allow us to record natural signals in the Amazon rainforest.
Carlos A. Sierra, Susan E. Crow, Martin Heimann, Holger Metzler, and Ernst-Detlef Schulze
Biogeosciences, 18, 1029–1048, https://doi.org/10.5194/bg-18-1029-2021, https://doi.org/10.5194/bg-18-1029-2021, 2021
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The climate benefit of carbon sequestration (CBS) is a metric developed to quantify avoided warming by two separate processes: the amount of carbon drawdown from the atmosphere and the time this carbon is stored in a reservoir. This metric can be useful for quantifying the role of forests and soils for climate change mitigation and to better quantify the benefits of carbon removals by sinks.
Robbie Ramsay, Chiara F. Di Marco, Matthias Sörgel, Mathew R. Heal, Samara Carbone, Paulo Artaxo, Alessandro C. de Araùjo, Marta Sá, Christopher Pöhlker, Jost Lavric, Meinrat O. Andreae, and Eiko Nemitz
Atmos. Chem. Phys., 20, 15551–15584, https://doi.org/10.5194/acp-20-15551-2020, https://doi.org/10.5194/acp-20-15551-2020, 2020
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The Amazon rainforest is a unique
laboratoryto study the processes which govern the exchange of gases and aerosols to and from the atmosphere. This study investigated these processes by measuring the atmospheric concentrations of trace gases and particles at the Amazon Tall Tower Observatory. We found that the long-range transport of pollutants can affect the atmospheric composition above the Amazon rainforest and that the gases ammonia and nitrous acid can be emitted from the rainforest.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Judith Hauck, Are Olsen, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Corinne Le Quéré, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone Alin, Luiz E. O. C. Aragão, Almut Arneth, Vivek Arora, Nicholas R. Bates, Meike Becker, Alice Benoit-Cattin, Henry C. Bittig, Laurent Bopp, Selma Bultan, Naveen Chandra, Frédéric Chevallier, Louise P. Chini, Wiley Evans, Liesbeth Florentie, Piers M. Forster, Thomas Gasser, Marion Gehlen, Dennis Gilfillan, Thanos Gkritzalis, Luke Gregor, Nicolas Gruber, Ian Harris, Kerstin Hartung, Vanessa Haverd, Richard A. Houghton, Tatiana Ilyina, Atul K. Jain, Emilie Joetzjer, Koji Kadono, Etsushi Kato, Vassilis Kitidis, Jan Ivar Korsbakken, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Zhu Liu, Danica Lombardozzi, Gregg Marland, Nicolas Metzl, David R. Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Yosuke Niwa, Kevin O'Brien, Tsuneo Ono, Paul I. Palmer, Denis Pierrot, Benjamin Poulter, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Adam J. P. Smith, Adrienne J. Sutton, Toste Tanhua, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Guido van der Werf, Nicolas Vuichard, Anthony P. Walker, Rik Wanninkhof, Andrew J. Watson, David Willis, Andrew J. Wiltshire, Wenping Yuan, Xu Yue, and Sönke Zaehle
Earth Syst. Sci. Data, 12, 3269–3340, https://doi.org/10.5194/essd-12-3269-2020, https://doi.org/10.5194/essd-12-3269-2020, 2020
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The Global Carbon Budget 2020 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Rachel L. Tunnicliffe, Anita L. Ganesan, Robert J. Parker, Hartmut Boesch, Nicola Gedney, Benjamin Poulter, Zhen Zhang, Jošt V. Lavrič, David Walter, Matthew Rigby, Stephan Henne, Dickon Young, and Simon O'Doherty
Atmos. Chem. Phys., 20, 13041–13067, https://doi.org/10.5194/acp-20-13041-2020, https://doi.org/10.5194/acp-20-13041-2020, 2020
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This study quantifies Brazil’s emissions of a potent atmospheric greenhouse gas, methane. This is in the field of atmospheric modelling and uses remotely sensed data and surface measurements of methane concentrations as well as an atmospheric transport model to interpret the data. Because of Brazil’s large emissions from wetlands, agriculture and biomass burning, these emissions affect global methane concentrations and thus are of global significance.
Alina Fiehn, Julian Kostinek, Maximilian Eckl, Theresa Klausner, Michał Gałkowski, Jinxuan Chen, Christoph Gerbig, Thomas Röckmann, Hossein Maazallahi, Martina Schmidt, Piotr Korbeń, Jarosław Neçki, Pawel Jagoda, Norman Wildmann, Christian Mallaun, Rostyslav Bun, Anna-Leah Nickl, Patrick Jöckel, Andreas Fix, and Anke Roiger
Atmos. Chem. Phys., 20, 12675–12695, https://doi.org/10.5194/acp-20-12675-2020, https://doi.org/10.5194/acp-20-12675-2020, 2020
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A severe reduction of greenhouse gas emissions is necessary to fulfill the Paris Agreement. We use aircraft- and ground-based in situ observations of trace gases and wind speed from two flights over the Upper Silesian Coal Basin, Poland, for independent emission estimation. The derived methane emission estimates are within the range of emission inventories, carbon dioxide estimates are in the lower range and carbon monoxide emission estimates are slightly higher than emission inventory values.
Guillaume Monteil, Grégoire Broquet, Marko Scholze, Matthew Lang, Ute Karstens, Christoph Gerbig, Frank-Thomas Koch, Naomi E. Smith, Rona L. Thompson, Ingrid T. Luijkx, Emily White, Antoon Meesters, Philippe Ciais, Anita L. Ganesan, Alistair Manning, Michael Mischurow, Wouter Peters, Philippe Peylin, Jerôme Tarniewicz, Matt Rigby, Christian Rödenbeck, Alex Vermeulen, and Evie M. Walton
Atmos. Chem. Phys., 20, 12063–12091, https://doi.org/10.5194/acp-20-12063-2020, https://doi.org/10.5194/acp-20-12063-2020, 2020
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The paper presents the first results from the EUROCOM project, a regional atmospheric inversion intercomparison exercise involving six European research groups. It aims to produce an estimate of the net carbon flux between the European terrestrial ecosystems and the atmosphere for the period 2006–2015, based on constraints provided by observed CO2 concentrations and using inverse modelling techniques. The use of six different models enables us to investigate the robustness of the results.
Jinxuan Chen, Christoph Gerbig, Julia Marshall, and Kai Uwe Totsche
Geosci. Model Dev., 13, 4091–4106, https://doi.org/10.5194/gmd-13-4091-2020, https://doi.org/10.5194/gmd-13-4091-2020, 2020
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One of the essential challenge for atmospheric CO2 forecasting is predicting CO2 flux variation on synoptic timescale. For CAMS CO2 forecast, a process-based vegetation model is used.
In this research we evaluate another type of model (i.e., the light-use-efficiency model VPRM), which is a data-driven approach and thus ideal for realistic estimation, on its ability of flux prediction. Errors from different sources are assessed, and overall the model is capable of CO2 flux prediction.
Santiago Botía, Christoph Gerbig, Julia Marshall, Jost V. Lavric, David Walter, Christopher Pöhlker, Bruna Holanda, Gilberto Fisch, Alessandro Carioca de Araújo, Marta O. Sá, Paulo R. Teixeira, Angélica F. Resende, Cleo Q. Dias-Junior, Hella van Asperen, Pablo S. Oliveira, Michel Stefanello, and Otávio C. Acevedo
Atmos. Chem. Phys., 20, 6583–6606, https://doi.org/10.5194/acp-20-6583-2020, https://doi.org/10.5194/acp-20-6583-2020, 2020
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A long record of atmospheric methane concentrations in central Amazonia was analyzed. We describe events in which concentrations at 79 m are higher than at 4 m. These events are more frequent during the nighttime of dry season, but we found no association with fire signals. Instead, we suggest that a combination of nighttime transport and a nearby source could explain such events. Our research gives insights into how methane is transported in the complex nocturnal atmosphere in Amazonia.
Bruna A. Holanda, Mira L. Pöhlker, David Walter, Jorge Saturno, Matthias Sörgel, Jeannine Ditas, Florian Ditas, Christiane Schulz, Marco Aurélio Franco, Qiaoqiao Wang, Tobias Donth, Paulo Artaxo, Henrique M. J. Barbosa, Stephan Borrmann, Ramon Braga, Joel Brito, Yafang Cheng, Maximilian Dollner, Johannes W. Kaiser, Thomas Klimach, Christoph Knote, Ovid O. Krüger, Daniel Fütterer, Jošt V. Lavrič, Nan Ma, Luiz A. T. Machado, Jing Ming, Fernando G. Morais, Hauke Paulsen, Daniel Sauer, Hans Schlager, Johannes Schneider, Hang Su, Bernadett Weinzierl, Adrian Walser, Manfred Wendisch, Helmut Ziereis, Martin Zöger, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 20, 4757–4785, https://doi.org/10.5194/acp-20-4757-2020, https://doi.org/10.5194/acp-20-4757-2020, 2020
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Biomass burning smoke from African savanna and grassland is transported across the South Atlantic Ocean in defined layers within the free troposphere. The combination of in situ aircraft and ground-based measurements aided by satellite observations showed that these layers are transported into the Amazon Basin during the early dry season. The influx of aged smoke, enriched in black carbon and cloud condensation nuclei, has important implications for the Amazonian aerosol and cloud cycling.
Anna-Leah Nickl, Mariano Mertens, Anke Roiger, Andreas Fix, Axel Amediek, Alina Fiehn, Christoph Gerbig, Michal Galkowski, Astrid Kerkweg, Theresa Klausner, Maximilian Eckl, and Patrick Jöckel
Geosci. Model Dev., 13, 1925–1943, https://doi.org/10.5194/gmd-13-1925-2020, https://doi.org/10.5194/gmd-13-1925-2020, 2020
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Based on the global and regional chemistry–climate model system MECO(n), we implemented a forecast system to support the planning of measurement campaign research flights with chemical weather forecasts. We applied this system for the first time to provide 6 d forecasts in support of the CoMet 1.0
campaign targeting methane emitted from coal mining ventilation shafts in the Upper Silesian Coal Basin in Poland. We describe the new forecast system and evaluate its forecast skill.
Martin Kunz, Jost V. Lavric, Rainer Gasche, Christoph Gerbig, Richard H. Grant, Frank-Thomas Koch, Marcus Schumacher, Benjamin Wolf, and Matthias Zeeman
Atmos. Meas. Tech., 13, 1671–1692, https://doi.org/10.5194/amt-13-1671-2020, https://doi.org/10.5194/amt-13-1671-2020, 2020
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The nocturnal boundary layer (NBL) budget method enables the quantification of gas fluxes between ecosystems and the atmosphere under nocturnal stable stratification, a condition under which standard approaches struggle. However, up to now the application of the NBL method has been limited by difficulties in obtaining the required measurements. We show how an unmanned aircraft system (UAS) equipped with a carbon dioxide analyser can make this method more accessible.
Pierre Friedlingstein, Matthew W. Jones, Michael O'Sullivan, Robbie M. Andrew, Judith Hauck, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Corinne Le Quéré, Dorothee C. E. Bakker, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Peter Anthoni, Leticia Barbero, Ana Bastos, Vladislav Bastrikov, Meike Becker, Laurent Bopp, Erik Buitenhuis, Naveen Chandra, Frédéric Chevallier, Louise P. Chini, Kim I. Currie, Richard A. Feely, Marion Gehlen, Dennis Gilfillan, Thanos Gkritzalis, Daniel S. Goll, Nicolas Gruber, Sören Gutekunst, Ian Harris, Vanessa Haverd, Richard A. Houghton, George Hurtt, Tatiana Ilyina, Atul K. Jain, Emilie Joetzjer, Jed O. Kaplan, Etsushi Kato, Kees Klein Goldewijk, Jan Ivar Korsbakken, Peter Landschützer, Siv K. Lauvset, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Danica Lombardozzi, Gregg Marland, Patrick C. McGuire, Joe R. Melton, Nicolas Metzl, David R. Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Craig Neill, Abdirahman M. Omar, Tsuneo Ono, Anna Peregon, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Roland Séférian, Jörg Schwinger, Naomi Smith, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Guido R. van der Werf, Andrew J. Wiltshire, and Sönke Zaehle
Earth Syst. Sci. Data, 11, 1783–1838, https://doi.org/10.5194/essd-11-1783-2019, https://doi.org/10.5194/essd-11-1783-2019, 2019
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The Global Carbon Budget 2019 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Friedemann Reum, Mathias Göckede, Jost V. Lavric, Olaf Kolle, Sergey Zimov, Nikita Zimov, Martijn Pallandt, and Martin Heimann
Atmos. Meas. Tech., 12, 5717–5740, https://doi.org/10.5194/amt-12-5717-2019, https://doi.org/10.5194/amt-12-5717-2019, 2019
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We present continuous in situ measurements of atmospheric CO2 and CH4 mole fractions at the new station Ambarchik, located in northeastern Siberia. We describe the site, measurements and quality control, characterize the signals in comparison with data from Barrow, Alaska, and show which regions the measurements are sensitive to. Ambarchik data are available upon request.
Eric J. Morgan, Jost V. Lavric, Damian L. Arévalo-Martínez, Hermann W. Bange, Tobias Steinhoff, Thomas Seifert, and Martin Heimann
Biogeosciences, 16, 4065–4084, https://doi.org/10.5194/bg-16-4065-2019, https://doi.org/10.5194/bg-16-4065-2019, 2019
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Taking a 2-year atmospheric record of atmospheric oxygen and the greenhouse gases N2O, CO2, and CH4, made at a coastal site in the Namib Desert, we estimated the fluxes of these gases from upwelling events in the northern Benguela Current region. We compared these results with flux measurements made on a research vessel in the study area at the same time and found that the two approaches agreed well. The study region was a source of N2O, CO2, and CH4 to the atmosphere during upwelling events.
Jarmo Mäkelä, Jürgen Knauer, Mika Aurela, Andrew Black, Martin Heimann, Hideki Kobayashi, Annalea Lohila, Ivan Mammarella, Hank Margolis, Tiina Markkanen, Jouni Susiluoto, Tea Thum, Toni Viskari, Sönke Zaehle, and Tuula Aalto
Geosci. Model Dev., 12, 4075–4098, https://doi.org/10.5194/gmd-12-4075-2019, https://doi.org/10.5194/gmd-12-4075-2019, 2019
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We assess the differences of six stomatal conductance formulations, embedded into a land–vegetation model JSBACH, on 10 boreal coniferous evergreen forest sites. We calibrate the model parameters using all six functions in a multi-year experiment, as well as for a separate drought event at one of the sites, using the adaptive population importance sampler. The analysis reveals weaknesses in the stomatal conductance formulation-dependent model behaviour that we are able to partially amend.
Youngjoon Jang, Sang Bum Hong, Christo Buizert, Hun-Gyu Lee, Sang-Young Han, Ji-Woong Yang, Yoshinori Iizuka, Akira Hori, Yeongcheol Han, Seong Joon Jun, Pieter Tans, Taejin Choi, Seong-Joong Kim, Soon Do Hur, and Jinho Ahn
The Cryosphere, 13, 2407–2419, https://doi.org/10.5194/tc-13-2407-2019, https://doi.org/10.5194/tc-13-2407-2019, 2019
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We can learn how human activity altered atmospheric air from the interstitial air in the porous snow layer (firn) on top of glaciers. However, old firn air (> 55 years) was observed only at sites where surface temperatures and snow accumulation rates are very low, such as the South Pole. In this study, we report an unusually old firn air with CO2 age of 93 years from Styx Glacier, near the Ross Sea coast in Antarctica. We hypothesize that the large snow density variations increase firn air ages.
Xinxu Zhao, Julia Marshall, Stephan Hachinger, Christoph Gerbig, Matthias Frey, Frank Hase, and Jia Chen
Atmos. Chem. Phys., 19, 11279–11302, https://doi.org/10.5194/acp-19-11279-2019, https://doi.org/10.5194/acp-19-11279-2019, 2019
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The Weather Research and Forecasting model (WRF), coupled with greenhouse gas (GHG) modules (WRF-GHG), is considered to be a suitable basis for precise GHG transport analysis in urban areas, especially when combined with differential column methodology (DCM). DCM is an effective method not only for comparing models to observations independently of biases caused, for example, by initial conditions, but also for detecting and understanding sources of GHG emissions quantitatively in urban areas.
Karel Castro-Morales, Gregor Schürmann, Christoph Köstler, Christian Rödenbeck, Martin Heimann, and Sönke Zaehle
Biogeosciences, 16, 3009–3032, https://doi.org/10.5194/bg-16-3009-2019, https://doi.org/10.5194/bg-16-3009-2019, 2019
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To obtain nearly 30 years of global terrestrial carbon fluxes, we simultaneously incorporated in a land surface model three different time periods of two observational data sets: absorbed photosynthetic active radiation and atmospheric CO2 concentrations. One decade of data is enough to improve the modeled long-term trends and seasonal amplitudes of the assimilated variables, particularly in boreal regions. This model has the potential to provide short-term predictions of land carbon fluxes.
Christopher Pöhlker, David Walter, Hauke Paulsen, Tobias Könemann, Emilio Rodríguez-Caballero, Daniel Moran-Zuloaga, Joel Brito, Samara Carbone, Céline Degrendele, Viviane R. Després, Florian Ditas, Bruna A. Holanda, Johannes W. Kaiser, Gerhard Lammel, Jošt V. Lavrič, Jing Ming, Daniel Pickersgill, Mira L. Pöhlker, Maria Praß, Nina Löbs, Jorge Saturno, Matthias Sörgel, Qiaoqiao Wang, Bettina Weber, Stefan Wolff, Paulo Artaxo, Ulrich Pöschl, and Meinrat O. Andreae
Atmos. Chem. Phys., 19, 8425–8470, https://doi.org/10.5194/acp-19-8425-2019, https://doi.org/10.5194/acp-19-8425-2019, 2019
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The Amazon Tall Tower Observatory (ATTO) has been established to monitor the rain forest's biosphere–atmosphere exchange, which experiences the combined pressures from human-made deforestation and progressing climate change. This work is meant to be a reference study, which characterizes various geospatial properties of the ATTO footprint region and shows how the human-made transformation of Amazonia may impact future atmospheric observations at ATTO.
Friedemann Reum, Christoph Gerbig, Jost V. Lavric, Chris W. Rella, and Mathias Göckede
Atmos. Meas. Tech., 12, 1013–1027, https://doi.org/10.5194/amt-12-1013-2019, https://doi.org/10.5194/amt-12-1013-2019, 2019
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Atmospheric CO2 and CH4 mole fractions are often measured using greenhouse gas analyzers manufactured by Picarro, Inc. We report biases in these measurements that are related to pressure changes in the optical cavity of the analyzers and occur mainly at low water vapor mole fractions. We provide a method to correct the biases, which contributes to keeping the overall accuracy of CO2 and CH4 measurements with Picarro analyzers within the WMO interlaboratory compatibility goals.
Ekaterina Ezhova, Ilona Ylivinkka, Joel Kuusk, Kaupo Komsaare, Marko Vana, Alisa Krasnova, Steffen Noe, Mikhail Arshinov, Boris Belan, Sung-Bin Park, Jošt Valentin Lavrič, Martin Heimann, Tuukka Petäjä, Timo Vesala, Ivan Mammarella, Pasi Kolari, Jaana Bäck, Üllar Rannik, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 18, 17863–17881, https://doi.org/10.5194/acp-18-17863-2018, https://doi.org/10.5194/acp-18-17863-2018, 2018
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Understanding the connections between aerosols, solar radiation and photosynthesis in terrestrial ecosystems is important for estimates of the CO2 balance in the atmosphere. Atmospheric aerosols and clouds influence solar radiation. In this study, we quantify the aerosol effect on solar radiation in boreal forests and study forest ecosystems response to this change in the radiation conditions. The analysis is based on atmospheric observations from several remote stations in Eurasian forests.
Corinne Le Quéré, Robbie M. Andrew, Pierre Friedlingstein, Stephen Sitch, Judith Hauck, Julia Pongratz, Penelope A. Pickers, Jan Ivar Korsbakken, Glen P. Peters, Josep G. Canadell, Almut Arneth, Vivek K. Arora, Leticia Barbero, Ana Bastos, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Scott C. Doney, Thanos Gkritzalis, Daniel S. Goll, Ian Harris, Vanessa Haverd, Forrest M. Hoffman, Mario Hoppema, Richard A. Houghton, George Hurtt, Tatiana Ilyina, Atul K. Jain, Truls Johannessen, Chris D. Jones, Etsushi Kato, Ralph F. Keeling, Kees Klein Goldewijk, Peter Landschützer, Nathalie Lefèvre, Sebastian Lienert, Zhu Liu, Danica Lombardozzi, Nicolas Metzl, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Craig Neill, Are Olsen, Tsueno Ono, Prabir Patra, Anna Peregon, Wouter Peters, Philippe Peylin, Benjamin Pfeil, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Matthias Rocher, Christian Rödenbeck, Ute Schuster, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Tobias Steinhoff, Adrienne Sutton, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Nicolas Viovy, Anthony P. Walker, Andrew J. Wiltshire, Rebecca Wright, Sönke Zaehle, and Bo Zheng
Earth Syst. Sci. Data, 10, 2141–2194, https://doi.org/10.5194/essd-10-2141-2018, https://doi.org/10.5194/essd-10-2141-2018, 2018
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The Global Carbon Budget 2018 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Michael F. Schibig, Duane Kitzis, and Pieter P. Tans
Atmos. Meas. Tech., 11, 5565–5586, https://doi.org/10.5194/amt-11-5565-2018, https://doi.org/10.5194/amt-11-5565-2018, 2018
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For long-term monitoring of CO2 in the atmosphere it is crucial that standard reference gas mixtures stored in high-pressure aluminum cylinders, used to calibrate global measurements, remain stable over their whole time of use. This study finds a reproducible small enrichment as a cylinder is emptied at a low-flow rate, as well as somewhat larger and variable effects when a cylinder is emptied using a high-flow rate.
Annette Filges, Christoph Gerbig, Chris W. Rella, John Hoffnagle, Herman Smit, Martina Krämer, Nicole Spelten, Christian Rolf, Zoltán Bozóki, Bernhard Buchholz, and Volker Ebert
Atmos. Meas. Tech., 11, 5279–5297, https://doi.org/10.5194/amt-11-5279-2018, https://doi.org/10.5194/amt-11-5279-2018, 2018
Jorge Saturno, Bruna A. Holanda, Christopher Pöhlker, Florian Ditas, Qiaoqiao Wang, Daniel Moran-Zuloaga, Joel Brito, Samara Carbone, Yafang Cheng, Xuguang Chi, Jeannine Ditas, Thorsten Hoffmann, Isabella Hrabe de Angelis, Tobias Könemann, Jošt V. Lavrič, Nan Ma, Jing Ming, Hauke Paulsen, Mira L. Pöhlker, Luciana V. Rizzo, Patrick Schlag, Hang Su, David Walter, Stefan Wolff, Yuxuan Zhang, Paulo Artaxo, Ulrich Pöschl, and Meinrat O. Andreae
Atmos. Chem. Phys., 18, 12817–12843, https://doi.org/10.5194/acp-18-12817-2018, https://doi.org/10.5194/acp-18-12817-2018, 2018
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Biomass burning emits light-absorbing aerosol particles that warm the atmosphere. One of them is the primarily emitted black carbon, which strongly absorbs radiation in the visible and UV spectral regions. Another one is the so-called brown carbon, a fraction of organic aerosol particles that are able to absorb radiation, especially in the UV spectral region. The contribution of both kinds of aerosol particles to light absorption over the Amazon rainforest is studied in this paper.
Wei He, Ivar R. van der Velde, Arlyn E. Andrews, Colm Sweeney, John Miller, Pieter Tans, Ingrid T. van der Laan-Luijkx, Thomas Nehrkorn, Marikate Mountain, Weimin Ju, Wouter Peters, and Huilin Chen
Geosci. Model Dev., 11, 3515–3536, https://doi.org/10.5194/gmd-11-3515-2018, https://doi.org/10.5194/gmd-11-3515-2018, 2018
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We have implemented a regional, high-resolution, and computationally attractive carbon dioxide data assimilation system. This system, named CTDAS-Lagrange, is capable of simultaneously optimizing terrestrial biosphere fluxes and the lateral boundary conditions. The CTDAS-Lagrange system can be easily extended to assimilate an additional tracer, e.g., carbonyl sulfide (COS or OCS), for regional estimates of both net and gross carbon fluxes.
Mira L. Pöhlker, Florian Ditas, Jorge Saturno, Thomas Klimach, Isabella Hrabě de Angelis, Alessandro C. Araùjo, Joel Brito, Samara Carbone, Yafang Cheng, Xuguang Chi, Reiner Ditz, Sachin S. Gunthe, Bruna A. Holanda, Konrad Kandler, Jürgen Kesselmeier, Tobias Könemann, Ovid O. Krüger, Jošt V. Lavrič, Scot T. Martin, Eugene Mikhailov, Daniel Moran-Zuloaga, Luciana V. Rizzo, Diana Rose, Hang Su, Ryan Thalman, David Walter, Jian Wang, Stefan Wolff, Henrique M. J. Barbosa, Paulo Artaxo, Meinrat O. Andreae, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10289–10331, https://doi.org/10.5194/acp-18-10289-2018, https://doi.org/10.5194/acp-18-10289-2018, 2018
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This paper presents the aerosol and cloud condensation nuclei (CCN) variability for characteristic atmospheric states – such as biomass burning, long-range transport, and pristine rain forest conditions – in the vulnerable and climate-relevant Amazon Basin. It summarizes the key properties of aerosol and CCN and, thus, provides a basis for an in-depth analysis of aerosol–cloud interactions in the Amazon region.
Daniel Moran-Zuloaga, Florian Ditas, David Walter, Jorge Saturno, Joel Brito, Samara Carbone, Xuguang Chi, Isabella Hrabě de Angelis, Holger Baars, Ricardo H. M. Godoi, Birgit Heese, Bruna A. Holanda, Jošt V. Lavrič, Scot T. Martin, Jing Ming, Mira L. Pöhlker, Nina Ruckteschler, Hang Su, Yaqiang Wang, Qiaoqiao Wang, Zhibin Wang, Bettina Weber, Stefan Wolff, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10055–10088, https://doi.org/10.5194/acp-18-10055-2018, https://doi.org/10.5194/acp-18-10055-2018, 2018
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This study presents multiple years of aerosol coarse mode observations at the remote ATTO site in the Amazon Basin. The results are discussed in light of the frequent and episodic long-range transport of Saharan dust plumes in the early wet season as well as the persistent background bioaerosol cycling in the rain forest ecosystem. This work provides a solid basis for future studies on the dynamic coarse mode aerosol cycling and its biogeochemical relevance in the Amazon.
Fabio Boschetti, Valerie Thouret, Greet Janssens Maenhout, Kai Uwe Totsche, Julia Marshall, and Christoph Gerbig
Atmos. Chem. Phys., 18, 9225–9241, https://doi.org/10.5194/acp-18-9225-2018, https://doi.org/10.5194/acp-18-9225-2018, 2018
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Retrieving surface–atmosphere fluxes from the combination of atmospheric observations with atmospheric transport models can benefit from combining multiple species in a single inversion. The underlying effect is that species such as CO2 and CO have partially overlapping emission patterns for given sectors and fuel types and so share part of the uncertainties, both related to the a priori knowledge of emissions, and to model–data mismatch error. We show this for airborne profile data from IAGOS.
Christian Rödenbeck, Sönke Zaehle, Ralph Keeling, and Martin Heimann
Biogeosciences, 15, 2481–2498, https://doi.org/10.5194/bg-15-2481-2018, https://doi.org/10.5194/bg-15-2481-2018, 2018
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In this paper we investigate how the CO2 exchange between the land vegetation and the atmosphere varies from year to year. We quantify the relation between variations in the CO2 exchange and variations in air temperature. For this quantification, we use long-term measurements of CO2 in the air at many locations, a simulation code for the transport of carbon dioxide through the atmosphere, and a data set of air temperature. The results help us to understand the mechanisms of CO2 exchange.
Corinne Le Quéré, Robbie M. Andrew, Pierre Friedlingstein, Stephen Sitch, Julia Pongratz, Andrew C. Manning, Jan Ivar Korsbakken, Glen P. Peters, Josep G. Canadell, Robert B. Jackson, Thomas A. Boden, Pieter P. Tans, Oliver D. Andrews, Vivek K. Arora, Dorothee C. E. Bakker, Leticia Barbero, Meike Becker, Richard A. Betts, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Catherine E. Cosca, Jessica Cross, Kim Currie, Thomas Gasser, Ian Harris, Judith Hauck, Vanessa Haverd, Richard A. Houghton, Christopher W. Hunt, George Hurtt, Tatiana Ilyina, Atul K. Jain, Etsushi Kato, Markus Kautz, Ralph F. Keeling, Kees Klein Goldewijk, Arne Körtzinger, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Ivan Lima, Danica Lombardozzi, Nicolas Metzl, Frank Millero, Pedro M. S. Monteiro, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Yukihiro Nojiri, X. Antonio Padin, Anna Peregon, Benjamin Pfeil, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Janet Reimer, Christian Rödenbeck, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Benjamin D. Stocker, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Steven van Heuven, Nicolas Viovy, Nicolas Vuichard, Anthony P. Walker, Andrew J. Watson, Andrew J. Wiltshire, Sönke Zaehle, and Dan Zhu
Earth Syst. Sci. Data, 10, 405–448, https://doi.org/10.5194/essd-10-405-2018, https://doi.org/10.5194/essd-10-405-2018, 2018
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The Global Carbon Budget 2017 describes data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. It is the 12th annual update and the 6th published in this journal.
Panagiotis Kountouris, Christoph Gerbig, Christian Rödenbeck, Ute Karstens, Thomas Frank Koch, and Martin Heimann
Atmos. Chem. Phys., 18, 3027–3045, https://doi.org/10.5194/acp-18-3027-2018, https://doi.org/10.5194/acp-18-3027-2018, 2018
Panagiotis Kountouris, Christoph Gerbig, Christian Rödenbeck, Ute Karstens, Thomas F. Koch, and Martin Heimann
Atmos. Chem. Phys., 18, 3047–3064, https://doi.org/10.5194/acp-18-3047-2018, https://doi.org/10.5194/acp-18-3047-2018, 2018
Peter Bergamaschi, Ute Karstens, Alistair J. Manning, Marielle Saunois, Aki Tsuruta, Antoine Berchet, Alexander T. Vermeulen, Tim Arnold, Greet Janssens-Maenhout, Samuel Hammer, Ingeborg Levin, Martina Schmidt, Michel Ramonet, Morgan Lopez, Jost Lavric, Tuula Aalto, Huilin Chen, Dietrich G. Feist, Christoph Gerbig, László Haszpra, Ove Hermansen, Giovanni Manca, John Moncrieff, Frank Meinhardt, Jaroslaw Necki, Michal Galkowski, Simon O'Doherty, Nina Paramonova, Hubertus A. Scheeren, Martin Steinbacher, and Ed Dlugokencky
Atmos. Chem. Phys., 18, 901–920, https://doi.org/10.5194/acp-18-901-2018, https://doi.org/10.5194/acp-18-901-2018, 2018
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European methane (CH4) emissions are estimated for 2006–2012 using atmospheric in situ measurements from 18 European monitoring stations and 7 different inverse models. Our analysis highlights the potential significant contribution of natural emissions from wetlands (including peatlands and wet soils) to the total European emissions. The top-down estimates of total EU-28 CH4 emissions are broadly consistent with the sum of reported anthropogenic CH4 emissions and the estimated natural emissions.
Ivar R. van der Velde, John B. Miller, Michiel K. van der Molen, Pieter P. Tans, Bruce H. Vaughn, James W. C. White, Kevin Schaefer, and Wouter Peters
Geosci. Model Dev., 11, 283–304, https://doi.org/10.5194/gmd-11-283-2018, https://doi.org/10.5194/gmd-11-283-2018, 2018
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We explored an inverse modeling technique to interpret global atmospheric measurements of CO2 and the ratio of its stable carbon isotopes (δ13C). We detected the possible underestimation of drought stress in biosphere models after applying combined atmospheric CO2 and δ13C constraints. This study highlights the importance of improving the representation of the biosphere in carbon–climate models, in particular in a world where droughts become more extreme and more frequent.
Xin Lan, Pieter Tans, Colm Sweeney, Arlyn Andrews, Andrew Jacobson, Molly Crotwell, Edward Dlugokencky, Jonathan Kofler, Patricia Lang, Kirk Thoning, and Sonja Wolter
Atmos. Chem. Phys., 17, 15151–15165, https://doi.org/10.5194/acp-17-15151-2017, https://doi.org/10.5194/acp-17-15151-2017, 2017
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We analyze spatial patterns of column CO2 over North America using well-calibrated aircraft and tall tower measurements. We find that the long-term averaged spatial gradients of column CO2 across North America show a smooth pattern that mainly reflects the large-scale circulation. Our results can serve as a good reference for evaluating current and future column CO2 retrievals from both ground and satellite platforms.
Mathias Göckede, Fanny Kittler, Min Jung Kwon, Ina Burjack, Martin Heimann, Olaf Kolle, Nikita Zimov, and Sergey Zimov
The Cryosphere, 11, 2975–2996, https://doi.org/10.5194/tc-11-2975-2017, https://doi.org/10.5194/tc-11-2975-2017, 2017
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Shifts in hydrologic conditions will be a key factor for the sustainability of Arctic ecosystems under future climate change. Using a long-term manipulation experiment, we analyzed how energy exchange processes within a permafrost ecosystem react to sustained dry conditions. Changes in several important ecosystem characteristics lead to reduced evapotranspiration and increased sensible heat fluxes. Heat transfer into the soil was strongly reduced, keeping the permafrost colder.
Heather Graven, Colin E. Allison, David M. Etheridge, Samuel Hammer, Ralph F. Keeling, Ingeborg Levin, Harro A. J. Meijer, Mauro Rubino, Pieter P. Tans, Cathy M. Trudinger, Bruce H. Vaughn, and James W. C. White
Geosci. Model Dev., 10, 4405–4417, https://doi.org/10.5194/gmd-10-4405-2017, https://doi.org/10.5194/gmd-10-4405-2017, 2017
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Modelling of carbon isotopes 13C and 14C in land and ocean components of Earth system models provides opportunities for new insights and improved understanding of global carbon cycling, and for model evaluation. We compiled existing historical datasets to define the annual mean carbon isotopic composition of atmospheric CO2 for 1850–2015 that can be used in CMIP6 and other modelling activities.
Eugene F. Mikhailov, Svetlana Mironova, Gregory Mironov, Sergey Vlasenko, Alexey Panov, Xuguang Chi, David Walter, Samara Carbone, Paulo Artaxo, Martin Heimann, Jost Lavric, Ulrich Pöschl, and Meinrat O. Andreae
Atmos. Chem. Phys., 17, 14365–14392, https://doi.org/10.5194/acp-17-14365-2017, https://doi.org/10.5194/acp-17-14365-2017, 2017
Pieter P. Tans, Andrew M. Crotwell, and Kirk W. Thoning
Atmos. Meas. Tech., 10, 2669–2685, https://doi.org/10.5194/amt-10-2669-2017, https://doi.org/10.5194/amt-10-2669-2017, 2017
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We describe a new CO2 calibration system for the Central Calibration Laboratory of the World Meteorological Organization Global Atmosphere Watch program. The system uses two laser spectroscopic instruments to measure the three major CO2 isotopologues individually. We account for isotopic differences between standards in the calibration hierarchy when assigning CO2 mole fraction, eliminating bias due to variations in the isotopic composition.
Shreeya Verma, Julia Marshall, Mark Parrington, Anna Agustí-Panareda, Sebastien Massart, Martyn P. Chipperfield, Christopher Wilson, and Christoph Gerbig
Atmos. Chem. Phys., 17, 6663–6678, https://doi.org/10.5194/acp-17-6663-2017, https://doi.org/10.5194/acp-17-6663-2017, 2017
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Aircraft profiles are a useful reference for validation of satellite-based column-averaged dry air mole fraction data. However, these are available only up to about 9–13 km altitude and therefore need to be extended synthetically into the stratosphere using other sources. In this study, we analyse three different data sources that are available for extension of CH4 profiles by comparing the error introduced by each into the total column and provide recommendations regarding the best approach.
Friedemann Reum, Christoph Gerbig, Jost V. Lavric, Chris W. Rella, and Mathias Göckede
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-174, https://doi.org/10.5194/amt-2017-174, 2017
Revised manuscript not accepted
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High-accuracy observations of atmospheric CO2 and CH4 levels, which are vital for quantifying sources and sinks of these gases, are often obtained using Picarro greenhouse gas analyzers. These require a correction for the effects of water vapor. We report biases in CO2 and CH4 levels obtained using the traditional water correction for Picarro analyzers related to pressure changes in the optical cavity and mainly affecting measurements at low water vapor mole fractions, and how to correct them.
Shreeya Verma, Julia Marshall, Christoph Gerbig, Christian Rödenbeck, and Kai Uwe Totsche
Atmos. Chem. Phys., 17, 5665–5675, https://doi.org/10.5194/acp-17-5665-2017, https://doi.org/10.5194/acp-17-5665-2017, 2017
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The inverse modelling approach for estimating surface fluxes is based on transport models that have an imperfect representation of atmospheric processes like vertical mixing. In this paper, we show how assimilating commercial aircraft-based vertical profiles of CO2 into inverse models can help reduce error due to the transport model, thus providing more accurate estimates of surface fluxes. Further, the reduction in flux uncertainty due to aircraft profiles from the IAGOS project is quantified.
Aki Tsuruta, Tuula Aalto, Leif Backman, Janne Hakkarainen, Ingrid T. van der Laan-Luijkx, Maarten C. Krol, Renato Spahni, Sander Houweling, Marko Laine, Ed Dlugokencky, Angel J. Gomez-Pelaez, Marcel van der Schoot, Ray Langenfelds, Raymond Ellul, Jgor Arduini, Francesco Apadula, Christoph Gerbig, Dietrich G. Feist, Rigel Kivi, Yukio Yoshida, and Wouter Peters
Geosci. Model Dev., 10, 1261–1289, https://doi.org/10.5194/gmd-10-1261-2017, https://doi.org/10.5194/gmd-10-1261-2017, 2017
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In this study, we found that the average global methane emission for 2000–2012, estimated by the CTE-CH4 model, was 516±51 Tg CH4 yr-1, and the estimates for 2007–2012 were 4 % larger than for 2000–2006. The model estimates are sensitive to inputs and setups, but according to sensitivity tests the study suggests that the increase in atmospheric methane concentrations during 21st century was due to an increase in emissions from the 35S-EQ latitudinal bands.
Rona L. Thompson, Motoki Sasakawa, Toshinobu Machida, Tuula Aalto, Doug Worthy, Jost V. Lavric, Cathrine Lund Myhre, and Andreas Stohl
Atmos. Chem. Phys., 17, 3553–3572, https://doi.org/10.5194/acp-17-3553-2017, https://doi.org/10.5194/acp-17-3553-2017, 2017
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Methane (CH4) fluxes were estimated for the high northern latitudes for 2005–2013 based on observations of atmospheric CH4 mixing ratios. Methane fluxes were found to be higher than prior estimates in northern Eurasia and Canada, especially in the Western Siberian Lowlands and the Canadian province Alberta. Significant inter-annual variations in the fluxes were found as well as a small positive trend. In Canada, the trend may be related to an increase in soil temperature over the study period.
Sander Houweling, Peter Bergamaschi, Frederic Chevallier, Martin Heimann, Thomas Kaminski, Maarten Krol, Anna M. Michalak, and Prabir Patra
Atmos. Chem. Phys., 17, 235–256, https://doi.org/10.5194/acp-17-235-2017, https://doi.org/10.5194/acp-17-235-2017, 2017
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The aim of this paper is to present an overview of inverse modeling methods, developed over the years, for estimating the global sources and sinks of the greenhouse gas methane from atmospheric measurements. It provides insight into how techniques and estimates have evolved over time, what the remaining shortcomings are, new developments, and promising future directions.
Mira L. Pöhlker, Christopher Pöhlker, Florian Ditas, Thomas Klimach, Isabella Hrabe de Angelis, Alessandro Araújo, Joel Brito, Samara Carbone, Yafang Cheng, Xuguang Chi, Reiner Ditz, Sachin S. Gunthe, Jürgen Kesselmeier, Tobias Könemann, Jošt V. Lavrič, Scot T. Martin, Eugene Mikhailov, Daniel Moran-Zuloaga, Diana Rose, Jorge Saturno, Hang Su, Ryan Thalman, David Walter, Jian Wang, Stefan Wolff, Henrique M. J. Barbosa, Paulo Artaxo, Meinrat O. Andreae, and Ulrich Pöschl
Atmos. Chem. Phys., 16, 15709–15740, https://doi.org/10.5194/acp-16-15709-2016, https://doi.org/10.5194/acp-16-15709-2016, 2016
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The paper presents a systematic characterization of cloud condensation nuclei (CCN) concentration in the central Amazonian atmosphere. Our results show that the CCN population in this globally important ecosystem follows a pollution-related seasonal cycle, in which it mainly depends on changes in total aerosol size distribution and to a minor extent in the aerosol chemical composition. Our results allow an efficient modeling and prediction of the CCN population based on a novel approach.
Qiaoqiao Wang, Jorge Saturno, Xuguang Chi, David Walter, Jost V. Lavric, Daniel Moran-Zuloaga, Florian Ditas, Christopher Pöhlker, Joel Brito, Samara Carbone, Paulo Artaxo, and Meinrat O. Andreae
Atmos. Chem. Phys., 16, 14775–14794, https://doi.org/10.5194/acp-16-14775-2016, https://doi.org/10.5194/acp-16-14775-2016, 2016
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We use a chemical transport model to interpret observed aerosol concentrations and absorption over the Amazon Basin during the wet season. With daily temporal resolution for open fire emissions and modified aerosol optical properties, our model successfully captures the observed variation in aerosol concentrations and absorption over the Amazon Basin. The simulation indicates the important influence of open fire mainly from northern South America and from northern Africa in the wet season.
Hanna K. Lappalainen, Veli-Matti Kerminen, Tuukka Petäjä, Theo Kurten, Aleksander Baklanov, Anatoly Shvidenko, Jaana Bäck, Timo Vihma, Pavel Alekseychik, Meinrat O. Andreae, Stephen R. Arnold, Mikhail Arshinov, Eija Asmi, Boris Belan, Leonid Bobylev, Sergey Chalov, Yafang Cheng, Natalia Chubarova, Gerrit de Leeuw, Aijun Ding, Sergey Dobrolyubov, Sergei Dubtsov, Egor Dyukarev, Nikolai Elansky, Kostas Eleftheriadis, Igor Esau, Nikolay Filatov, Mikhail Flint, Congbin Fu, Olga Glezer, Aleksander Gliko, Martin Heimann, Albert A. M. Holtslag, Urmas Hõrrak, Juha Janhunen, Sirkku Juhola, Leena Järvi, Heikki Järvinen, Anna Kanukhina, Pavel Konstantinov, Vladimir Kotlyakov, Antti-Jussi Kieloaho, Alexander S. Komarov, Joni Kujansuu, Ilmo Kukkonen, Ella-Maria Duplissy, Ari Laaksonen, Tuomas Laurila, Heikki Lihavainen, Alexander Lisitzin, Alexsander Mahura, Alexander Makshtas, Evgeny Mareev, Stephany Mazon, Dmitry Matishov, Vladimir Melnikov, Eugene Mikhailov, Dmitri Moisseev, Robert Nigmatulin, Steffen M. Noe, Anne Ojala, Mari Pihlatie, Olga Popovicheva, Jukka Pumpanen, Tatjana Regerand, Irina Repina, Aleksei Shcherbinin, Vladimir Shevchenko, Mikko Sipilä, Andrey Skorokhod, Dominick V. Spracklen, Hang Su, Dmitry A. Subetto, Junying Sun, Arkady Y. Terzhevik, Yuri Timofeyev, Yuliya Troitskaya, Veli-Pekka Tynkkynen, Viacheslav I. Kharuk, Nina Zaytseva, Jiahua Zhang, Yrjö Viisanen, Timo Vesala, Pertti Hari, Hans Christen Hansson, Gennady G. Matvienko, Nikolai S. Kasimov, Huadong Guo, Valery Bondur, Sergej Zilitinkevich, and Markku Kulmala
Atmos. Chem. Phys., 16, 14421–14461, https://doi.org/10.5194/acp-16-14421-2016, https://doi.org/10.5194/acp-16-14421-2016, 2016
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After kick off in 2012, the Pan-Eurasian Experiment (PEEX) program has expanded fast and today the multi-disciplinary research community covers ca. 80 institutes and a network of ca. 500 scientists from Europe, Russia, and China. Here we introduce scientific topics relevant in this context. This is one of the first multi-disciplinary overviews crossing scientific boundaries, from atmospheric sciences to socio-economics and social sciences.
Corinne Le Quéré, Robbie M. Andrew, Josep G. Canadell, Stephen Sitch, Jan Ivar Korsbakken, Glen P. Peters, Andrew C. Manning, Thomas A. Boden, Pieter P. Tans, Richard A. Houghton, Ralph F. Keeling, Simone Alin, Oliver D. Andrews, Peter Anthoni, Leticia Barbero, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Kim Currie, Christine Delire, Scott C. Doney, Pierre Friedlingstein, Thanos Gkritzalis, Ian Harris, Judith Hauck, Vanessa Haverd, Mario Hoppema, Kees Klein Goldewijk, Atul K. Jain, Etsushi Kato, Arne Körtzinger, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Danica Lombardozzi, Joe R. Melton, Nicolas Metzl, Frank Millero, Pedro M. S. Monteiro, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Kevin O'Brien, Are Olsen, Abdirahman M. Omar, Tsuneo Ono, Denis Pierrot, Benjamin Poulter, Christian Rödenbeck, Joe Salisbury, Ute Schuster, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Benjamin D. Stocker, Adrienne J. Sutton, Taro Takahashi, Hanqin Tian, Bronte Tilbrook, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Nicolas Viovy, Anthony P. Walker, Andrew J. Wiltshire, and Sönke Zaehle
Earth Syst. Sci. Data, 8, 605–649, https://doi.org/10.5194/essd-8-605-2016, https://doi.org/10.5194/essd-8-605-2016, 2016
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The Global Carbon Budget 2016 is the 11th annual update of emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, land, and ocean. This data synthesis brings together measurements, statistical information, and analyses of model results in order to provide an assessment of the global carbon budget and their uncertainties for years 1959 to 2015, with a projection for year 2016.
Christoph Zellweger, Lukas Emmenegger, Mohd Firdaus, Juha Hatakka, Martin Heimann, Elena Kozlova, T. Gerard Spain, Martin Steinbacher, Marcel V. van der Schoot, and Brigitte Buchmann
Atmos. Meas. Tech., 9, 4737–4757, https://doi.org/10.5194/amt-9-4737-2016, https://doi.org/10.5194/amt-9-4737-2016, 2016
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We compared instruments using more traditional techniques for measuring CO2 and CH4 at different stations of the Global Atmosphere Watch (GAW) programme with a travelling instrument using a spectroscopic technique. Our results show that the newer analytical techniques have clear advantages over the traditional methods which will lead to the improved accuracy of atmospheric CO2 and CH4 measurement. The work was carried out in the framework of the GAW quality assurance/quality control system.
Fanny Kittler, Ina Burjack, Chiara A. R. Corradi, Martin Heimann, Olaf Kolle, Lutz Merbold, Nikita Zimov, Sergey Zimov, and Mathias Göckede
Biogeosciences, 13, 5315–5332, https://doi.org/10.5194/bg-13-5315-2016, https://doi.org/10.5194/bg-13-5315-2016, 2016
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We compared growing season CO2 fluxes of a wet tussock tundra ecosystem from an area affected by decadal drainage and an undisturbed area on the Kolyma floodplain in northeastern Siberia. The results show systematically reduced CO2 uptake within the drained area, caused by increased respiration, and that the local permafrost ecosystem is capable of adapting to significantly different hydrologic conditions without losing its capacity to act as a net sink for CO2.
Gregor J. Schürmann, Thomas Kaminski, Christoph Köstler, Nuno Carvalhais, Michael Voßbeck, Jens Kattge, Ralf Giering, Christian Rödenbeck, Martin Heimann, and Sönke Zaehle
Geosci. Model Dev., 9, 2999–3026, https://doi.org/10.5194/gmd-9-2999-2016, https://doi.org/10.5194/gmd-9-2999-2016, 2016
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We describe the Max Planck Institute Carbon Cycle Data Assimilation System (MPI-CCDAS). The system improves the modelled carbon cycle of the terrestrial biosphere by systematically confronting (or assimilating) the model with observations of atmospheric CO2 and fractions of absorbed photosynthetically active radiation. Jointly assimilating both data streams outperforms the single-data stream experiments, thus showing the value of a multi-data stream assimilation.
Dhanyalekshmi Pillai, Michael Buchwitz, Christoph Gerbig, Thomas Koch, Maximilian Reuter, Heinrich Bovensmann, Julia Marshall, and John P. Burrows
Atmos. Chem. Phys., 16, 9591–9610, https://doi.org/10.5194/acp-16-9591-2016, https://doi.org/10.5194/acp-16-9591-2016, 2016
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Approximately 70 % of total CO2 emissions arise from cities; however, there exist large uncertainties in quantifying urban emissions. The present study investigates the potential of a satellite mission like CarbonSat to retrieve the city emissions via inverse modelling techniques. The study makes a valid conclusion that an instrument like CarbonSat has high potential to provide important information on city emissions when exploiting the observations using a high-resolution modelling system.
Makoto Inoue, Isamu Morino, Osamu Uchino, Takahiro Nakatsuru, Yukio Yoshida, Tatsuya Yokota, Debra Wunch, Paul O. Wennberg, Coleen M. Roehl, David W. T. Griffith, Voltaire A. Velazco, Nicholas M. Deutscher, Thorsten Warneke, Justus Notholt, John Robinson, Vanessa Sherlock, Frank Hase, Thomas Blumenstock, Markus Rettinger, Ralf Sussmann, Esko Kyrö, Rigel Kivi, Kei Shiomi, Shuji Kawakami, Martine De Mazière, Sabrina G. Arnold, Dietrich G. Feist, Erica A. Barrow, James Barney, Manvendra Dubey, Matthias Schneider, Laura T. Iraci, James R. Podolske, Patrick W. Hillyard, Toshinobu Machida, Yousuke Sawa, Kazuhiro Tsuboi, Hidekazu Matsueda, Colm Sweeney, Pieter P. Tans, Arlyn E. Andrews, Sebastien C. Biraud, Yukio Fukuyama, Jasna V. Pittman, Eric A. Kort, and Tomoaki Tanaka
Atmos. Meas. Tech., 9, 3491–3512, https://doi.org/10.5194/amt-9-3491-2016, https://doi.org/10.5194/amt-9-3491-2016, 2016
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In this study, we correct the biases of GOSAT XCO2 and XCH4 using TCCON data. To evaluate the effectiveness of our correction method, uncorrected/corrected GOSAT data are compared to independent XCO2 and XCH4 data derived from aircraft measurements. Consequently, we suggest that this method is effective for reducing the biases of the GOSAT data. We consider that our work provides GOSAT data users with valuable information and contributes to the further development of studies on greenhouse gases.
Joan Cuxart, Burkhard Wrenger, Daniel Martínez-Villagrasa, Joachim Reuder, Marius O. Jonassen, Maria A. Jiménez, Marie Lothon, Fabienne Lohou, Oscar Hartogensis, Jens Dünnermann, Laura Conangla, and Anirban Garai
Atmos. Chem. Phys., 16, 9489–9504, https://doi.org/10.5194/acp-16-9489-2016, https://doi.org/10.5194/acp-16-9489-2016, 2016
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Estimations of the effect of thermal advection in the surface energy budget are provided. Data from the experimental campaign BLLAST, held in Southern France in summer 2011, are used, including airborne data by drones and surface-based instrumentation. Model data outputs and satellite information are also inspected. Surface heterogeneities of the order of the kilometer or larger seem to have little effect on the budget, whereas hectometer-scale structures may contribute significantly to it.
Min Jung Kwon, Martin Heimann, Olaf Kolle, Kristina A. Luus, Edward A. G. Schuur, Nikita Zimov, Sergey A. Zimov, and Mathias Göckede
Biogeosciences, 13, 4219–4235, https://doi.org/10.5194/bg-13-4219-2016, https://doi.org/10.5194/bg-13-4219-2016, 2016
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A decade-long drainage on an Arctic floodplain has altered dominant plant species and soil temperature regimes. Consequently, CO2 exchange rates between the atmosphere and the terrestrial ecosystem were modified: CO2 uptake rates by the terrestrial ecosystem decreased and CO2 emission rates to the atmosphere increased. Ongoing global warming may thaw ice-rich permafrost and make some regions drier in the Arctic, and this will reduce carbon accumulation in the terrestrial ecosystem.
Sha Feng, Thomas Lauvaux, Sally Newman, Preeti Rao, Ravan Ahmadov, Aijun Deng, Liza I. Díaz-Isaac, Riley M. Duren, Marc L. Fischer, Christoph Gerbig, Kevin R. Gurney, Jianhua Huang, Seongeun Jeong, Zhijin Li, Charles E. Miller, Darragh O'Keeffe, Risa Patarasuk, Stanley P. Sander, Yang Song, Kam W. Wong, and Yuk L. Yung
Atmos. Chem. Phys., 16, 9019–9045, https://doi.org/10.5194/acp-16-9019-2016, https://doi.org/10.5194/acp-16-9019-2016, 2016
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We developed a high-resolution land–atmosphere modelling system for urban CO2 emissions over the LA Basin. We evaluated various model configurations, FFCO2 products, and the impact of the model resolution. FFCO2 emissions outpace the atmospheric model resolution to represent the CO2 concentration variability across the basin. A novel forward model approach is presented to evaluate the surface measurement network, reinforcing the importance of using high-resolution emission products.
S. Sippel, F. E. L. Otto, M. Forkel, M. R. Allen, B. P. Guillod, M. Heimann, M. Reichstein, S. I. Seneviratne, K. Thonicke, and M. D. Mahecha
Earth Syst. Dynam., 7, 71–88, https://doi.org/10.5194/esd-7-71-2016, https://doi.org/10.5194/esd-7-71-2016, 2016
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We introduce a novel technique to bias correct climate model output for impact simulations that preserves its physical consistency and multivariate structure. The methodology considerably improves the representation of extremes in climatic variables relative to conventional bias correction strategies. Illustrative simulations of biosphere–atmosphere carbon and water fluxes with a biosphere model (LPJmL) show that the novel technique can be usefully applied to drive climate impact models.
P. Kountouris, C. Gerbig, K.-U. Totsche, A. J. Dolman, A. G. C. A. Meesters, G. Broquet, F. Maignan, B. Gioli, L. Montagnani, and C. Helfter
Biogeosciences, 12, 7403–7421, https://doi.org/10.5194/bg-12-7403-2015, https://doi.org/10.5194/bg-12-7403-2015, 2015
N. Kadygrov, G. Broquet, F. Chevallier, L. Rivier, C. Gerbig, and P. Ciais
Atmos. Chem. Phys., 15, 12765–12787, https://doi.org/10.5194/acp-15-12765-2015, https://doi.org/10.5194/acp-15-12765-2015, 2015
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We study the potential of the European Integrated Carbon Observing System (ICOS) atmospheric network for estimating European CO2 ecosystem fluxes. Regional atmospheric inversions with synthetic data are used to derive it in terms of statistical uncertainty. This potential is high in western Europe and future extensions of the network will increase it in eastern Europe. Future improvements of the models underlying the inversion should also significantly decrease uncertainties at high resolution.
S. N. Vardag, C. Gerbig, G. Janssens-Maenhout, and I. Levin
Atmos. Chem. Phys., 15, 12705–12729, https://doi.org/10.5194/acp-15-12705-2015, https://doi.org/10.5194/acp-15-12705-2015, 2015
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In this model sensitivity study we compare and evaluate the surrogate tracers CO2, CO, δ13C-CO2 and Δ14C-CO2 for estimating continuous anthropogenic CO2. The results can be used to optimize the measurement network design with respect to the partitioning of total CO2 into biospheric and anthropogenic CO2 contributions. This enables improvement and validation of highly resolved emission inventories using atmospheric observation and regional modeling.
G. Biavati, D. G. Feist, C. Gerbig, and R. Kretschmer
Atmos. Meas. Tech., 8, 4215–4230, https://doi.org/10.5194/amt-8-4215-2015, https://doi.org/10.5194/amt-8-4215-2015, 2015
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The goal of this work is to present a method that can be used to estimate the uncertainty for a singular estimate for the mixing height. It is defined here as the localization error. The method is based on the actual signal (radiosonde) and its measurement errors, ant it does not consider the physics causing the signal.
It can be applied to all kind of signals and algorithm when standard error propagation cannot be used to asses the uncertainty of a location of a localized property.
M. O. Andreae, O. C. Acevedo, A. Araùjo, P. Artaxo, C. G. G. Barbosa, H. M. J. Barbosa, J. Brito, S. Carbone, X. Chi, B. B. L. Cintra, N. F. da Silva, N. L. Dias, C. Q. Dias-Júnior, F. Ditas, R. Ditz, A. F. L. Godoi, R. H. M. Godoi, M. Heimann, T. Hoffmann, J. Kesselmeier, T. Könemann, M. L. Krüger, J. V. Lavric, A. O. Manzi, A. P. Lopes, D. L. Martins, E. F. Mikhailov, D. Moran-Zuloaga, B. W. Nelson, A. C. Nölscher, D. Santos Nogueira, M. T. F. Piedade, C. Pöhlker, U. Pöschl, C. A. Quesada, L. V. Rizzo, C.-U. Ro, N. Ruckteschler, L. D. A. Sá, M. de Oliveira Sá, C. B. Sales, R. M. N. dos Santos, J. Saturno, J. Schöngart, M. Sörgel, C. M. de Souza, R. A. F. de Souza, H. Su, N. Targhetta, J. Tóta, I. Trebs, S. Trumbore, A. van Eijck, D. Walter, Z. Wang, B. Weber, J. Williams, J. Winderlich, F. Wittmann, S. Wolff, and A. M. Yáñez-Serrano
Atmos. Chem. Phys., 15, 10723–10776, https://doi.org/10.5194/acp-15-10723-2015, https://doi.org/10.5194/acp-15-10723-2015, 2015
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This paper describes the Amazon Tall Tower Observatory (ATTO), a new atmosphere-biosphere observatory located in the remote Amazon Basin. It presents results from ecosystem ecology, meteorology, trace gas, and aerosol measurements collected at the ATTO site during the first 3 years of operation.
A. Berchet, I. Pison, F. Chevallier, J.-D. Paris, P. Bousquet, J.-L. Bonne, M. Y. Arshinov, B. D. Belan, C. Cressot, D. K. Davydov, E. J. Dlugokencky, A. V. Fofonov, A. Galanin, J. Lavrič, T. Machida, R. Parker, M. Sasakawa, R. Spahni, B. D. Stocker, and J. Winderlich
Biogeosciences, 12, 5393–5414, https://doi.org/10.5194/bg-12-5393-2015, https://doi.org/10.5194/bg-12-5393-2015, 2015
V. Proschek, G. Kirchengast, S. Schweitzer, J. S. A. Brooke, P. F. Bernath, C. B. Thomas, J.-G. Wang, K. A. Tereszchuk, G. González Abad, R. J. Hargreaves, C. A. Beale, J. J. Harrison, P. A. Martin, V. L. Kasyutich, C. Gerbig, O. Kolle, and A. Loescher
Atmos. Meas. Tech., 8, 3315–3336, https://doi.org/10.5194/amt-8-3315-2015, https://doi.org/10.5194/amt-8-3315-2015, 2015
E. J. Morgan, J. V. Lavrič, T. Seifert, T. Chicoine, A. Day, J. Gomez, R. Logan, J. Sack, T. Shuuya, E. G. Uushona, K. Vincent, U. Schultz, E.-G. Brunke, C. Labuschagne, R. L. Thompson, S. Schmidt, A. C. Manning, and M. Heimann
Atmos. Meas. Tech., 8, 2233–2250, https://doi.org/10.5194/amt-8-2233-2015, https://doi.org/10.5194/amt-8-2233-2015, 2015
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We describe the analytical techniques used in the creation of a new background site for continuous measurements of greenhouse gases, carbon monoxide, and atmospheric oxygen in the Namib Desert. The measurement system is semi-automated and optimized for operation in a remote locale. Measurement uncertainties, gas handling, calibration schemes, drift corrections, and instrument performance are discussed.
E. Bahlmann, I. Weinberg, J. V. Lavrič, T. Eckhardt, W. Michaelis, R. Santos, and R. Seifert
Biogeosciences, 12, 1683–1696, https://doi.org/10.5194/bg-12-1683-2015, https://doi.org/10.5194/bg-12-1683-2015, 2015
M. M. Bela, K. M. Longo, S. R. Freitas, D. S. Moreira, V. Beck, S. C. Wofsy, C. Gerbig, K. Wiedemann, M. O. Andreae, and P. Artaxo
Atmos. Chem. Phys., 15, 757–782, https://doi.org/10.5194/acp-15-757-2015, https://doi.org/10.5194/acp-15-757-2015, 2015
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In the Amazon Basin, gases that lead to the formation of ozone (O3), an air pollutant and greenhouse gas, are emitted from fire, urban and biogenic sources. This study presents the first basin wide aircraft measurements of O3 during the dry-to-wet and wet-to-dry transition seasons, which show extremely low values above undisturbed forest and increases from fires. This work also demonstrates the capabilities and limitations of regional atmospheric chemistry models in representing O3 in Amazonia.
D. Tátrai, Z. Bozóki, H. Smit, C. Rolf, N. Spelten, M. Krämer, A. Filges, C. Gerbig, G. Gulyás, and G. Szabó
Atmos. Meas. Tech., 8, 33–42, https://doi.org/10.5194/amt-8-33-2015, https://doi.org/10.5194/amt-8-33-2015, 2015
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Airborne hygrometry is very important in climate research, and the interest in knowing not only water vapor concentration but (cirrus) cloud content as well is increasing. The authors provide a photoacoustic spectroscopy-based dual-channel hygrometer system that can be a good solution for such measurements. The instrument was proven to operate properly from ground level up to the lower stratosphere, giving the possibility even for cirrus cloud studies.
M. Reuter, M. Buchwitz, M. Hilker, J. Heymann, O. Schneising, D. Pillai, H. Bovensmann, J. P. Burrows, H. Bösch, R. Parker, A. Butz, O. Hasekamp, C. W. O'Dell, Y. Yoshida, C. Gerbig, T. Nehrkorn, N. M. Deutscher, T. Warneke, J. Notholt, F. Hase, R. Kivi, R. Sussmann, T. Machida, H. Matsueda, and Y. Sawa
Atmos. Chem. Phys., 14, 13739–13753, https://doi.org/10.5194/acp-14-13739-2014, https://doi.org/10.5194/acp-14-13739-2014, 2014
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Current knowledge about the European terrestrial biospheric carbon sink relies upon bottom-up and global surface flux inverse model estimates using in situ measurements. Our analysis of five satellite data sets comprises a regional inversion designed to be insensitive to potential retrieval biases and transport errors. We show that the satellite-derived sink is larger (1.0±0.3GtC/a) than previous estimates (0.4±0.4GtC/a).
Z. Wang, N. M. Deutscher, T. Warneke, J. Notholt, B. Dils, D. W. T. Griffith, M. Schmidt, M. Ramonet, and C. Gerbig
Atmos. Meas. Tech., 7, 3295–3305, https://doi.org/10.5194/amt-7-3295-2014, https://doi.org/10.5194/amt-7-3295-2014, 2014
C. Rödenbeck, D. C. E. Bakker, N. Metzl, A. Olsen, C. Sabine, N. Cassar, F. Reum, R. F. Keeling, and M. Heimann
Biogeosciences, 11, 4599–4613, https://doi.org/10.5194/bg-11-4599-2014, https://doi.org/10.5194/bg-11-4599-2014, 2014
R. Kretschmer, C. Gerbig, U. Karstens, G. Biavati, A. Vermeulen, F. Vogel, S. Hammer, and K. U. Totsche
Atmos. Chem. Phys., 14, 7149–7172, https://doi.org/10.5194/acp-14-7149-2014, https://doi.org/10.5194/acp-14-7149-2014, 2014
P. Ciais, A. J. Dolman, A. Bombelli, R. Duren, A. Peregon, P. J. Rayner, C. Miller, N. Gobron, G. Kinderman, G. Marland, N. Gruber, F. Chevallier, R. J. Andres, G. Balsamo, L. Bopp, F.-M. Bréon, G. Broquet, R. Dargaville, T. J. Battin, A. Borges, H. Bovensmann, M. Buchwitz, J. Butler, J. G. Canadell, R. B. Cook, R. DeFries, R. Engelen, K. R. Gurney, C. Heinze, M. Heimann, A. Held, M. Henry, B. Law, S. Luyssaert, J. Miller, T. Moriyama, C. Moulin, R. B. Myneni, C. Nussli, M. Obersteiner, D. Ojima, Y. Pan, J.-D. Paris, S. L. Piao, B. Poulter, S. Plummer, S. Quegan, P. Raymond, M. Reichstein, L. Rivier, C. Sabine, D. Schimel, O. Tarasova, R. Valentini, R. Wang, G. van der Werf, D. Wickland, M. Williams, and C. Zehner
Biogeosciences, 11, 3547–3602, https://doi.org/10.5194/bg-11-3547-2014, https://doi.org/10.5194/bg-11-3547-2014, 2014
S. Houweling, M. Krol, P. Bergamaschi, C. Frankenberg, E. J. Dlugokencky, I. Morino, J. Notholt, V. Sherlock, D. Wunch, V. Beck, C. Gerbig, H. Chen, E. A. Kort, T. Röckmann, and I. Aben
Atmos. Chem. Phys., 14, 3991–4012, https://doi.org/10.5194/acp-14-3991-2014, https://doi.org/10.5194/acp-14-3991-2014, 2014
J. Winderlich, C. Gerbig, O. Kolle, and M. Heimann
Biogeosciences, 11, 2055–2068, https://doi.org/10.5194/bg-11-2055-2014, https://doi.org/10.5194/bg-11-2055-2014, 2014
M. Heimann
Earth Syst. Dynam., 5, 41–42, https://doi.org/10.5194/esd-5-41-2014, https://doi.org/10.5194/esd-5-41-2014, 2014
X. Chi, J. Winderlich, J.-C. Mayer, A. V. Panov, M. Heimann, W. Birmili, J. Heintzenberg, Y. Cheng, and M. O. Andreae
Atmos. Chem. Phys., 13, 12271–12298, https://doi.org/10.5194/acp-13-12271-2013, https://doi.org/10.5194/acp-13-12271-2013, 2013
M. Buchwitz, M. Reuter, H. Bovensmann, D. Pillai, J. Heymann, O. Schneising, V. Rozanov, T. Krings, J. P. Burrows, H. Boesch, C. Gerbig, Y. Meijer, and A. Löscher
Atmos. Meas. Tech., 6, 3477–3500, https://doi.org/10.5194/amt-6-3477-2013, https://doi.org/10.5194/amt-6-3477-2013, 2013
T. J. Bohn, E. Podest, R. Schroeder, N. Pinto, K. C. McDonald, M. Glagolev, I. Filippov, S. Maksyutov, M. Heimann, X. Chen, and D. P. Lettenmaier
Biogeosciences, 10, 6559–6576, https://doi.org/10.5194/bg-10-6559-2013, https://doi.org/10.5194/bg-10-6559-2013, 2013
B. Badawy, C. Rödenbeck, M. Reichstein, N. Carvalhais, and M. Heimann
Biogeosciences, 10, 6485–6508, https://doi.org/10.5194/bg-10-6485-2013, https://doi.org/10.5194/bg-10-6485-2013, 2013
F. A. Haumann, A. M. Batenburg, G. Pieterse, C. Gerbig, M. C. Krol, and T. Röckmann
Atmos. Chem. Phys., 13, 9401–9413, https://doi.org/10.5194/acp-13-9401-2013, https://doi.org/10.5194/acp-13-9401-2013, 2013
V. Beck, C. Gerbig, T. Koch, M. M. Bela, K. M. Longo, S. R. Freitas, J. O. Kaplan, C. Prigent, P. Bergamaschi, and M. Heimann
Atmos. Chem. Phys., 13, 7961–7982, https://doi.org/10.5194/acp-13-7961-2013, https://doi.org/10.5194/acp-13-7961-2013, 2013
A. Berchet, I. Pison, F. Chevallier, P. Bousquet, S. Conil, M. Geever, T. Laurila, J. Lavrič, M. Lopez, J. Moncrieff, J. Necki, M. Ramonet, M. Schmidt, M. Steinbacher, and J. Tarniewicz
Atmos. Chem. Phys., 13, 7115–7132, https://doi.org/10.5194/acp-13-7115-2013, https://doi.org/10.5194/acp-13-7115-2013, 2013
H. Chen, A. Karion, C. W. Rella, J. Winderlich, C. Gerbig, A. Filges, T. Newberger, C. Sweeney, and P. P. Tans
Atmos. Meas. Tech., 6, 1031–1040, https://doi.org/10.5194/amt-6-1031-2013, https://doi.org/10.5194/amt-6-1031-2013, 2013
C. Rödenbeck, R. F. Keeling, D. C. E. Bakker, N. Metzl, A. Olsen, C. Sabine, and M. Heimann
Ocean Sci., 9, 193–216, https://doi.org/10.5194/os-9-193-2013, https://doi.org/10.5194/os-9-193-2013, 2013
Related subject area
Subject: Gases | Technique: In Situ Measurement | Topic: Instruments and Platforms
Using metal oxide gas sensors to estimate the emission rates and locations of methane leaks in an industrial site: assessment with controlled methane releases
Toward on-demand measurements of greenhouse gas emissions using an uncrewed aircraft AirCore system
Long-term evaluation of commercial air quality sensors: an overview from the QUANT (Quantification of Utility of Atmospheric Network Technologies) study
In-flight characterization of a compact airborne quantum cascade laser absorption spectrometer
Full characterization and calibration of a transfer standard monitor for atmospheric radon measurements
Observing low-altitude features in ozone concentrations in a shoreline environment via uncrewed aerial systems
An integrated uncrewed aerial vehicle platform with sensing and sampling systems for the measurement of air pollutant concentrations
Design and evaluation of a low-cost sensor node for near-background methane measurement
Development of a Multichannel Organics In situ enviRonmental Analyzer (MOIRA) for mobile measurements of volatile organic compounds
Evaluation of Aeris mid-infrared absorption (MIRA), Picarro CRDS (cavity ring-down spectroscopy) G2307, and dinitrophenylhydrazine (DNPH)-based sampling for long-term formaldehyde monitoring efforts
Multi-decadal atmospheric carbon dioxide measurements in Central Europe, Hungary
A New Technique for Airborne Measurements to Quantify Methane Emissions Over a Wide Range: Implementation and Validation
Performance characterization of a laminar gas inlet
Validation and field application of a low-cost device to measure CO2 and evapotranspiration (ET) fluxes
Identifying and correcting interferences to PTR-ToF-MS measurements of isoprene and other urban volatile organic compounds
Development of a continuous UAV-mounted air sampler and application to the quantification of CO2 and CH4 emissions from a major coking plant
Uptake behavior of polycyclic aromatic compounds during field calibrations of the XAD-based passive air sampler across seasons and locations
Drone CO2 Measurements During the Tajogaite Volcanic Eruption
New infrared spectroscopy instrument for reliable low humidity water vapour isotopic composition measurements
Effect of land–sea air mass transport on spatiotemporal distributions of atmospheric CO2 and CH4 mixing ratios over the southern Yellow Sea
HYPHOP: a tool for high-altitude, long-range monitoring of hydrogen peroxide and higher organic peroxides in the atmosphere
Portable, low-cost samplers for distributed sampling of atmospheric gases
SI-traceable validation of a laser spectrometer for balloon-borne measurements of water vapor in the upper atmosphere
Field evaluation of low-cost electrochemical air quality gas sensors under extreme temperature and relative humidity conditions
A novel, cost-effective analytical method for measuring high-resolution vertical profiles of stratospheric trace gases using a gas chromatograph coupled with an electron capture detector
Ethylene oxide monitor with part-per-trillion precision for in situ measurements
Development of an automated pump-efficiency measuring system for ozonesondes utilizing an airbag-type flowmeter
Short-term variability of atmospheric helium revealed through a cryo-enrichment method
Using tunable infrared laser direct absorption spectroscopy for ambient hydrogen chloride detection: HCl-TILDAS
New methods for the calibration of optical resonators: integrated calibration by means of optical modulation (ICOM) and narrow-band cavity ring-down (NB-CRD)
A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
Field comparison of two novel open-path instruments that measure dry deposition and emission of ammonia using flux-gradient and eddy covariance methods
Development of multi-channel whole-air sampling equipment onboard an unmanned aerial vehicle for investigating volatile organic compounds' vertical distribution in the planetary boundary layer
Electrochemical sensors on board a Zeppelin NT: in-flight evaluation of low-cost trace gas measurements
Evaluating the performance of a Picarro G2207-i analyser for high-precision atmospheric O2 measurements
Airborne flux measurements of ammonia over the southern Great Plains using chemical ionization mass spectrometry
Optical receiver characterizations and corrections for ground-based and airborne measurements of spectral actinic flux densities
Development and validation of a new in situ technique to measure total gaseous chlorine in air
True eddy accumulation – Part 1: Solutions to the problem of non-vanishing mean vertical wind velocity
True eddy accumulation – Part 2: Theory and experiment of the short-time eddy accumulation method
A simultaneous CH4 and CO2 flux quantification method for industrial site emissions from in-situ concentration measurements on-board an Unmanned Aircraft Vehicle
Chemical ionization mass spectrometry utilizing ammonium ions (NH4+ CIMS) for measurements of organic compounds in the atmosphere
Direct measurement of N2O5 heterogeneous uptake coefficients on ambient aerosols via an aerosol flow tube system: design, characterization and performance
Online measurements of cycloalkanes based on NO+ chemical ionization in proton transfer reaction time-of-flight mass spectrometry (PTR-ToF-MS)
Intercomparison of in situ measurements of ambient NH3: instrument performance and application under field conditions
A lightweight broadband cavity-enhanced spectrometer for NO2 measurement on uncrewed aerial vehicles
On the development of a new prototype PTR-ToF-MS instrument and its application to the detection of atmospheric amines
Low-complexity methods to mitigate the impact of environmental variables on low-cost UAS-based atmospheric carbon dioxide measurements
Comparison of airborne measurements of NO, NO2, HONO, NOy, and CO during FIREX-AQ
Development of a broadband cavity-enhanced absorption spectrometer for simultaneous measurements of ambient NO3, NO2, and H2O
Rodrigo Rivera-Martinez, Pramod Kumar, Olivier Laurent, Gregoire Broquet, Christopher Caldow, Ford Cropley, Diego Santaren, Adil Shah, Cécile Mallet, Michel Ramonet, Leonard Rivier, Catherine Juery, Olivier Duclaux, Caroline Bouchet, Elisa Allegrini, Hervé Utard, and Philippe Ciais
Atmos. Meas. Tech., 17, 4257–4290, https://doi.org/10.5194/amt-17-4257-2024, https://doi.org/10.5194/amt-17-4257-2024, 2024
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We explore the use of metal oxide semiconductors (MOSs) as a low-cost alternative for detecting and measuring CH4 emissions from industrial facilities. MOSs were exposed to several controlled releases to test their accuracy in detecting and quantifying emissions. Two reconstruction models were compared, and emission estimates were computed using a Gaussian dispersion model. Findings show that MOSs can provide accurate emission estimates with a 25 % emission rate error and a 9.5 m location error.
Zihan Zhu, Javier González-Rocha, Yifan Ding, Isis Frausto-Vicencio, Sajjan Heerah, Akula Venkatram, Manvendra Dubey, Don Collins, and Francesca M. Hopkins
Atmos. Meas. Tech., 17, 3883–3895, https://doi.org/10.5194/amt-17-3883-2024, https://doi.org/10.5194/amt-17-3883-2024, 2024
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Increases in agriculture, oil and gas, and waste management activities have contributed to the increase in atmospheric methane levels and resultant climate warming. In this paper, we explore the use of small uncrewed aircraft systems (sUASs) and AirCore technology to detect and quantify methane emissions. Results from field experiments demonstrate that sUASs and AirCore technology can be effective for detecting and quantifying methane emissions in near real time.
Sebastian Diez, Stuart Lacy, Hugh Coe, Josefina Urquiza, Max Priestman, Michael Flynn, Nicholas Marsden, Nicholas A. Martin, Stefan Gillott, Thomas Bannan, and Pete M. Edwards
Atmos. Meas. Tech., 17, 3809–3827, https://doi.org/10.5194/amt-17-3809-2024, https://doi.org/10.5194/amt-17-3809-2024, 2024
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In this paper we present an overview of the QUANT project, which to our knowledge is one of the largest evaluations of commercial sensors to date. The objective was to evaluate the performance of a range of commercial products and also to nourish the different applications in which these technologies can offer relevant information.
Linda Ort, Lenard Lukas Röder, Uwe Parchatka, Rainer Königstedt, Daniel Crowley, Frank Kunz, Ralf Wittkowski, Jos Lelieveld, and Horst Fischer
Atmos. Meas. Tech., 17, 3553–3565, https://doi.org/10.5194/amt-17-3553-2024, https://doi.org/10.5194/amt-17-3553-2024, 2024
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Airborne in situ measurements are of great importance to collect valuable data to improve our knowledge of the atmosphere but also present challenges which demand specific designs. This study presents an IR spectrometer for airborne trace-gas measurements with high data efficiency and a simple, compact design. Its in-flight performance is characterized with the help of a test flight and a comparison with another spectrometer. Moreover, results from its first campaign highlight its benefits.
Roger Curcoll, Claudia Grossi, Stefan Röttger, and Arturo Vargas
Atmos. Meas. Tech., 17, 3047–3065, https://doi.org/10.5194/amt-17-3047-2024, https://doi.org/10.5194/amt-17-3047-2024, 2024
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This paper presents a new user-friendly version of the Atmospheric Radon MONitor (ARMON). The efficiency of the instrument is of 0.0057 s-1, obtained using different techniques at Spanish and German chambers. The total calculated uncertainty of the ARMON for hourly radon concentrations above 5 Bq m-3 is lower than 10 % (k = 1). Results confirm that the ARMON is suitable to measure low-level radon activity concentrations and to be used as a transfer standard to calibrate in situ radon monitors.
Josie K. Radtke, Benjamin N. Kies, Whitney A. Mottishaw, Sydney M. Zeuli, Aidan T. H. Voon, Kelly L. Koerber, Grant W. Petty, Michael P. Vermeuel, Timothy H. Bertram, Ankur R. Desai, Joseph P. Hupy, R. Bradley Pierce, Timothy J. Wagner, and Patricia A. Cleary
Atmos. Meas. Tech., 17, 2833–2847, https://doi.org/10.5194/amt-17-2833-2024, https://doi.org/10.5194/amt-17-2833-2024, 2024
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The use of uncrewed aircraft systems (UASs) to conduct a vertical profiling of ozone and meteorological variables was evaluated using comparisons between tower or ground observations and UAS-based measurements. Changes to the UAS profiler showed an improvement in performance. The profiler was used to see the impact of Chicago pollution plumes on a shoreline area near Lake Michigan.
Chen-Wei Liang and Chang-Hung Shen
Atmos. Meas. Tech., 17, 2671–2686, https://doi.org/10.5194/amt-17-2671-2024, https://doi.org/10.5194/amt-17-2671-2024, 2024
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In the present study, a UAV platform with sensing and sampling systems was developed for 3D air pollutant concentration measurements. The sensing system of this platform contains multiple microsensors and IoT technologies for obtaining the real-time 3D distributions of critical air pollutants. The sampling system contains gas sampling sets and a 1 L Tedlar bag instead of a canister for the 3D measurement of VOC concentrations in accordance with the TO-15 method of the US EPA.
Daniel Furuta, Bruce Wilson, Albert A. Presto, and Jiayu Li
Atmos. Meas. Tech., 17, 2103–2121, https://doi.org/10.5194/amt-17-2103-2024, https://doi.org/10.5194/amt-17-2103-2024, 2024
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Methane is an important driver of climate change and is challenging to inexpensively sense in low atmospheric concentrations. We developed a low-cost sensor to monitor methane and tested it in indoor and outdoor settings. Our device shows promise for monitoring low levels of methane. We characterize its limitations and suggest future research directions for further development.
Audrey J. Dang, Nathan M. Kreisberg, Tyler L. Cargill, Jhao-Hong Chen, Sydney Hornitschek, Remy Hutheesing, Jay R. Turner, and Brent J. Williams
Atmos. Meas. Tech., 17, 2067–2087, https://doi.org/10.5194/amt-17-2067-2024, https://doi.org/10.5194/amt-17-2067-2024, 2024
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The Multichannel Organics In situ enviRonmental Analyzer (MOIRA) is a new instrument for measuring speciated volatile organic compounds (VOCs) in the air and has been developed for mapping concentrations from a hybrid car. MOIRA is characterized in the lab and pilot field studies of indoor air in a single-family residence and outdoor air during a mobile deployment. Future applications include indoor, outdoor, and lab measurements to grasp the impact of VOCs on air quality, health, and climate.
Asher P. Mouat, Zelda A. Siegel, and Jennifer Kaiser
Atmos. Meas. Tech., 17, 1979–1994, https://doi.org/10.5194/amt-17-1979-2024, https://doi.org/10.5194/amt-17-1979-2024, 2024
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Three fast-measurement formaldehyde monitors were deployed at two field sites in Atlanta, GA, over 1 year. Four different zeroing methods were tested to develop an optimal field setup as well as procedures for instrument calibration. Observations agreed well after calibration but were much higher compared to the TO-11A monitoring method, which is the golden standard. Historical HCHO concentrations were compared with measurements in this work, showing a 22 % reduction in midday HCHO since 1999.
László Haszpra
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-29, https://doi.org/10.5194/amt-2024-29, 2024
Revised manuscript accepted for AMT
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The paper evaluates a 30-year-long atmospheric CO2 data series from a mid-continental Central European site, Hegyhátsál (HUN). It presents the site-specific features observed in the long-term evolution of the atmospheric CO2 concentration. Since the measurement data are widely used in atmospheric inverse models and budget calculations all around the world, the paper provides potentially valuable information for model tuning and interpretation of the model results.
Jonathan F. Dooley, Kenneth Minschwaner, Manvendra K. Dubey, Sahar H. El Abbadi, Evan D. Sherwin, Aaron G. Meyer, Emily Follansbee, and James E. Lee
EGUsphere, https://doi.org/10.5194/egusphere-2024-760, https://doi.org/10.5194/egusphere-2024-760, 2024
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Methane is a powerful greenhouse gas originating from both natural and human activities. We describe a new Unmanned Aerial System (UAS) designed to measure methane emission rates from over a wide range of scales. This system has been used for direct quantification of point sources and distributed emitters over scales of up to 1 km. The system uses simultaneous measurements of methane and ethane to distinguish between different kinds of natural and human-related emission sources.
Da Yang, Margarita Reza, Roy Mauldin, Rainer Volkamer, and Suresh Dhaniyala
Atmos. Meas. Tech., 17, 1463–1474, https://doi.org/10.5194/amt-17-1463-2024, https://doi.org/10.5194/amt-17-1463-2024, 2024
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This paper evaluates the performance of an aircraft gas inlet. Here, we use computational fluid dynamics (CFD) and experiments to demonstrate the role of turbulence in determining sampling performance of a gas inlet and identify ideal conditions for inlet operation to minimize gas loss. Experiments conducted in a high-speed wind tunnel under near-aircraft speeds validated numerical results. We believe that the results obtained from this work will greatly inform future gas inlet studies.
Reena Macagga, Michael Asante, Geoffroy Sossa, Danica Antonijević, Maren Dubbert, and Mathias Hoffmann
Atmos. Meas. Tech., 17, 1317–1332, https://doi.org/10.5194/amt-17-1317-2024, https://doi.org/10.5194/amt-17-1317-2024, 2024
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Using only low-cost microcontrollers and sensors, we constructed a measurement device to accurately and precisely obtain atmospheric carbon dioxide and water fluxes. The device was tested against known concentration increases and high-cost, commercial sensors during a laboratory and field experiment. We additionally tested the device over a longer period in a field study in Ghana during which the net ecosystem carbon balance and water use efficiency of maize cultivation were studied.
Matthew M. Coggon, Chelsea E. Stockwell, Megan S. Claflin, Eva Y. Pfannerstill, Lu Xu, Jessica B. Gilman, Julia Marcantonio, Cong Cao, Kelvin Bates, Georgios I. Gkatzelis, Aaron Lamplugh, Erin F. Katz, Caleb Arata, Eric C. Apel, Rebecca S. Hornbrook, Felix Piel, Francesca Majluf, Donald R. Blake, Armin Wisthaler, Manjula Canagaratna, Brian M. Lerner, Allen H. Goldstein, John E. Mak, and Carsten Warneke
Atmos. Meas. Tech., 17, 801–825, https://doi.org/10.5194/amt-17-801-2024, https://doi.org/10.5194/amt-17-801-2024, 2024
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Mass spectrometry is a tool commonly used to measure air pollutants. This study evaluates measurement artifacts produced in the proton-transfer-reaction mass spectrometer. We provide methods to correct these biases and better measure compounds that degrade air quality.
Tianran Han, Conghui Xie, Yayong Liu, Yanrong Yang, Yuheng Zhang, Yufei Huang, Xiangyu Gao, Xiaohua Zhang, Fangmin Bao, and Shao-Meng Li
Atmos. Meas. Tech., 17, 677–691, https://doi.org/10.5194/amt-17-677-2024, https://doi.org/10.5194/amt-17-677-2024, 2024
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This study reported an integrated UAV measurement platform for GHG monitoring and its application for emission quantification from a coking plant. The key element of this system is a newly designed air sampler, consisting of a 150 m long tube with remote-controlled time stamping. When comparing the top-down results to those derived from the bottom-up inventory method, the present findings indicate that the use of IPCC emission factors for emission calculations can lead to overestimation.
Yuening Li, Faqiang Zhan, Yushan Su, Ying Duan Lei, Chubashini Shunthirasingham, Zilin Zhou, Jonathan P. D. Abbatt, Hayley Hung, and Frank Wania
Atmos. Meas. Tech., 17, 715–729, https://doi.org/10.5194/amt-17-715-2024, https://doi.org/10.5194/amt-17-715-2024, 2024
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A simple device for sampling gases from the atmosphere without the help of pumps was calibrated for an important group of hazardous air pollutants called polycyclic aromatic compounds (PACs). While the sampler appeared to perform well when used for relatively short periods of up to several months, some PACs were lost from the sampler during longer deployments. Sampling rates that can be used to quantitatively interpret the quantities of PACs taken up in the device have been derived.
John Ericksen, Tobias Fischer, G. Matthew Fricke, Scott Nowicki, Nemesio Pérez, Pedro Hernández Pérez, Eleazar Padrón González, and Melanie Moses
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-229, https://doi.org/10.5194/amt-2023-229, 2024
Revised manuscript accepted for AMT
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Volcanic eruptions emit significant quantities of carbon dioxide (CO2) to the atmosphere. We present a new method for directly determining the CO2 emission from a volcanic eruption using om La Palma Island, Spain using an unpiloted areal vehicle (UAV). We also collected samples of the emitted CO2 and analyzed their isotopic composition. Together with the emission rate the isotopic data provide valuable information on the state of volcanic activity and the potential evolution the eruption.
Mathieu Casado, Amaelle Landais, Tim Stoltmann, Justin Chaillot, Mathieu Daëron, Frédéric Prié, Baptiste Bordet, and Samir Kassi
EGUsphere, https://doi.org/10.5194/egusphere-2023-2457, https://doi.org/10.5194/egusphere-2023-2457, 2023
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Measuring water isotopic composition in Antarctica is difficult because of the extremely cold temperature in winter. Here, we designed a new infrared spectrometer able to measure the vapour isotopic composition more than 95 % of the year in the coldest locations of Antarctica, while current commercial instruments are only able to measure during the warm summer months in the interior.
Jiaxin Li, Kunpeng Zang, Yi Lin, Yuanyuan Chen, Shuo Liu, Shanshan Qiu, Kai Jiang, Xuemei Qing, Haoyu Xiong, Haixiang Hong, Shuangxi Fang, Honghui Xu, and Yujun Jiang
Atmos. Meas. Tech., 16, 4757–4768, https://doi.org/10.5194/amt-16-4757-2023, https://doi.org/10.5194/amt-16-4757-2023, 2023
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Based on observed data of CO2 and CH4 and meteorological parameters over the Yellow Sea in November 2012 and June 2013, a data process and quality control method was optimized and established to filter the data influenced by multiple factors. Spatial and seasonal variations in CO2 and CH4 mixing ratios were mainly controlled by the East Asian Monsoon, while the influence of air–sea exchange was slight.
Zaneta Hamryszczak, Antonia Hartmann, Dirk Dienhart, Sascha Hafermann, Bettina Brendel, Rainer Königstedt, Uwe Parchatka, Jos Lelieveld, and Horst Fischer
Atmos. Meas. Tech., 16, 4741–4756, https://doi.org/10.5194/amt-16-4741-2023, https://doi.org/10.5194/amt-16-4741-2023, 2023
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Hydroperoxide measurements improve the understanding of atmospheric oxidation processes. We introduce an instrumental setup for airborne measurements. The aim of the work is the characterization of the measurement method with emphasis on interferences impacting instrumental uncertainty. Technical and physical challenges do not critically impact the instrumental performance. The instrument resolves dynamic processes, such as convective transport, as shown based on the CAFE-Brazil campaign.
James F. Hurley, Alejandra Caceres, Deborah F. McGlynn, Mary E. Tovillo, Suzanne Pinar, Roger Schürch, Ksenia Onufrieva, and Gabriel Isaacman-VanWertz
Atmos. Meas. Tech., 16, 4681–4692, https://doi.org/10.5194/amt-16-4681-2023, https://doi.org/10.5194/amt-16-4681-2023, 2023
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Volatile organic compounds (VOCs) have a wide range of sources and impacts on environments and human health that make them spatially, temporally, and chemically varied. Current methods lack the ability to collect samples in ways that provide spatial and chemical resolution without complex, costly instrumentation. We describe and validate a low-cost, portable VOC sampler and demonstrate its utility in collecting distributed coordinated samples.
Simone Brunamonti, Manuel Graf, Tobias Bühlmann, Céline Pascale, Ivan Ilak, Lukas Emmenegger, and Béla Tuzson
Atmos. Meas. Tech., 16, 4391–4407, https://doi.org/10.5194/amt-16-4391-2023, https://doi.org/10.5194/amt-16-4391-2023, 2023
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The abundance of water vapor (H2O) in the upper atmosphere has a significant impact on the rate of global warming. We developed a new lightweight spectrometer (ALBATROSS) for H2O measurements aboard meteorological balloons. Here, we assess the accuracy and precision of ALBATROSS using metrology-grade reference gases. The results demonstrate the exceptional potential of mid-infrared laser absorption spectroscopy as a new reference method for in situ measurements of H2O in the upper atmosphere.
Roubina Papaconstantinou, Marios Demosthenous, Spyros Bezantakos, Neoclis Hadjigeorgiou, Marinos Costi, Melina Stylianou, Elli Symeou, Chrysanthos Savvides, and George Biskos
Atmos. Meas. Tech., 16, 3313–3329, https://doi.org/10.5194/amt-16-3313-2023, https://doi.org/10.5194/amt-16-3313-2023, 2023
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In this paper, we investigate the performance of low-cost electrochemical gas sensors. We carried out yearlong measurements at a traffic air quality monitoring station, where the low-cost sensors were collocated with reference instruments and exposed to highly variable environmental conditions with extremely high temperatures and low relative humidity (RH). Sensors provide measurements that exhibit increasing errors and decreasing correlations as temperature increases and RH decreases.
Jianghanyang Li, Bianca C. Baier, Fred Moore, Tim Newberger, Sonja Wolter, Jack Higgs, Geoff Dutton, Eric Hintsa, Bradley Hall, and Colm Sweeney
Atmos. Meas. Tech., 16, 2851–2863, https://doi.org/10.5194/amt-16-2851-2023, https://doi.org/10.5194/amt-16-2851-2023, 2023
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Monitoring a suite of trace gases in the stratosphere will help us better understand the stratospheric circulation and its impact on the earth's radiation balance. However, such measurements are rare and usually expensive. We developed an instrument that can measure stratospheric trace gases using a low-cost sampling platform (AirCore). The results showed expected agreement with aircraft measurements, demonstrating this technique provides a low-cost and robust way to observe the stratosphere.
Tara I. Yacovitch, Christoph Dyroff, Joseph R. Roscioli, Conner Daube, J. Barry McManus, and Scott C. Herndon
Atmos. Meas. Tech., 16, 1915–1921, https://doi.org/10.5194/amt-16-1915-2023, https://doi.org/10.5194/amt-16-1915-2023, 2023
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Ethylene oxide is a toxic, carcinogenic compound used in the medical and bulk sterilization industry. Here we describe a precise and fast laser-based ethylene oxide monitor. We report months-long concentrations at a Massachusetts site, and we show how they suggest a potential emission source 35 km away. This source, and another, is confirmed by driving the instrument downwind of the sites, where concentrations were tens to tens of thousands of times greater than background levels.
Tatsumi Nakano and Takashi Morofuji
Atmos. Meas. Tech., 16, 1583–1595, https://doi.org/10.5194/amt-16-1583-2023, https://doi.org/10.5194/amt-16-1583-2023, 2023
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We have developed a system that can automatically measure the pump efficiency of the ECC-type ozonesonde. Operational measurement for 13 years by this system revealed that the efficiency fluctuates in each and slightly increases over time. Those can affect the estimation of total ozone amount by up to 4 %. This result indicates that it is necessary to understand the tendency of the pump correction factor of each ozonesonde in order to detect the actual atmospheric change with high accuracy.
Benjamin Birner, Eric Morgan, and Ralph F. Keeling
Atmos. Meas. Tech., 16, 1551–1561, https://doi.org/10.5194/amt-16-1551-2023, https://doi.org/10.5194/amt-16-1551-2023, 2023
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Atmospheric variations of helium (He) and CO2 are strongly linked due to the co-release of both gases from natural-gas burning. This implies that atmospheric He measurements may be a potentially powerful tool for verifying reported anthropogenic natural-gas usage. Here, we present the development and initial results of a novel measurement system of atmospheric He that paves the way for establishing a global monitoring network in the future.
John W. Halfacre, Jordan Stewart, Scott C. Herndon, Joseph R. Roscioli, Christoph Dyroff, Tara I. Yacovitch, Michael Flynn, Stephen J. Andrews, Steven S. Brown, Patrick R. Veres, and Pete M. Edwards
Atmos. Meas. Tech., 16, 1407–1429, https://doi.org/10.5194/amt-16-1407-2023, https://doi.org/10.5194/amt-16-1407-2023, 2023
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This study details a new sampling method for the optical detection of hydrogen chloride (HCl). HCl is an important atmospheric reservoir for chlorine atoms, which can affect nitrogen oxide cycling and the lifetimes of volatile organic compounds and ozone. However, HCl has a high affinity for interacting with surfaces, thereby preventing fast, quantitative measurements. The sampling technique in this study minimizes these surface interactions and provides a high-quality measurement of HCl.
Henning Finkenzeller, Denis Pöhler, Martin Horbanski, Johannes Lampel, and Ulrich Platt
Atmos. Meas. Tech., 16, 1343–1356, https://doi.org/10.5194/amt-16-1343-2023, https://doi.org/10.5194/amt-16-1343-2023, 2023
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Optical resonators enhance the light path in compact instruments, thereby improving their sensitivity. Determining the established path length in the instrument is a prerequisite for the accurate determination of trace gas concentrations but can be a significant complication in the use of such resonators. Here we show two calibration techniques which are relatively simple and free of consumables but still provide accurate calibrations. This facilitates the use of optical resonators.
Andrew W. Seidl, Harald Sodemann, and Hans Christian Steen-Larsen
Atmos. Meas. Tech., 16, 769–790, https://doi.org/10.5194/amt-16-769-2023, https://doi.org/10.5194/amt-16-769-2023, 2023
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It is challenging to make field measurements of stable water isotopes in the Arctic. To this end, we present a modular stable-water-isotope analyzer profiling system. The system operated for a 2-week field campaign on Svalbard during the Arctic winter. We evaluate the system’s performance and analyze any potential impact that the field conditions might have had on the isotopic measurements and the system's ability to resolve isotope gradients in the lowermost layer of the atmosphere.
Daan Swart, Jun Zhang, Shelley van der Graaf, Susanna Rutledge-Jonker, Arjan Hensen, Stijn Berkhout, Pascal Wintjen, René van der Hoff, Marty Haaima, Arnoud Frumau, Pim van den Bulk, Ruben Schulte, Margreet van Zanten, and Thomas van Goethem
Atmos. Meas. Tech., 16, 529–546, https://doi.org/10.5194/amt-16-529-2023, https://doi.org/10.5194/amt-16-529-2023, 2023
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During a 5-week comparison campaign, we tested two set-ups to measure half hourly ammonia fluxes. The eddy covariance and flux gradient systems showed very similar results when the upwind terrain was both homogeneous and free of obstacles. We discuss the technical performance and practical limitations of both systems. Measurements from these instruments can facilitate the study of processes behind ammonia deposition, an important contributor to eutrophication and acidificationin natural areas.
Suding Yang, Xin Li, Limin Zeng, Xuena Yu, Ying Liu, Sihua Lu, Xiaofeng Huang, Dongmei Zhang, Haibin Xu, Shuchen Lin, Hefan Liu, Miao Feng, Danlin Song, Qinwen Tan, Jinhui Cui, Lifan Wang, Ying Chen, Wenjie Wang, Haijiong Sun, Mengdi Song, Liuwei Kong, Yi Liu, Linhui Wei, Xianwu Zhu, and Yuanhang Zhang
Atmos. Meas. Tech., 16, 501–512, https://doi.org/10.5194/amt-16-501-2023, https://doi.org/10.5194/amt-16-501-2023, 2023
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Vertical observation of volatile organic compounds (VOCs) is essential to study the spatial distribution and evolution patterns of VOCs in the planetary boundary layer (PBL). This paper describes multi-channel whole-air sampling equipment onboard an unmanned aerial vehicle (UAV) for near-continuous VOC vertical observation. Vertical profiles of VOCs and trace gases during the evolution of the PBL in south-western China have been successfully obtained by deploying the newly developed UAV system.
Tobias Schuldt, Georgios I. Gkatzelis, Christian Wesolek, Franz Rohrer, Benjamin Winter, Thomas A. J. Kuhlbusch, Astrid Kiendler-Scharr, and Ralf Tillmann
Atmos. Meas. Tech., 16, 373–386, https://doi.org/10.5194/amt-16-373-2023, https://doi.org/10.5194/amt-16-373-2023, 2023
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We report in situ measurements of air pollutant concentrations within the planetary boundary layer on board a Zeppelin NT in Germany. We highlight the in-flight evaluation of electrochemical sensors that were installed inside a hatch box located on the bottom of the Zeppelin. Results from this work emphasize the potential of these sensors for other in situ airborne applications, e.g., on board unmanned aerial vehicles (UAVs).
Leigh S. Fleming, Andrew C. Manning, Penelope A. Pickers, Grant L. Forster, and Alex J. Etchells
Atmos. Meas. Tech., 16, 387–401, https://doi.org/10.5194/amt-16-387-2023, https://doi.org/10.5194/amt-16-387-2023, 2023
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Measurements of atmospheric O2 can help constrain the carbon cycle processes and quantify fossil fuel CO2 emissions; however, measurement of atmospheric O2 is very challenging, and existing analysers are complex systems to build and maintain. We have tested a new O2 analyser (Picarro Inc. G2207-i) in the laboratory and at Weybourne Atmospheric Observatory. We have found that the G2207-i does not perform as well as an existing O2 analyser from Sable Systems Inc.
Siegfried Schobesberger, Emma L. D'Ambro, Lejish Vettikkat, Ben H. Lee, Qiaoyun Peng, David M. Bell, John E. Shilling, Manish Shrivastava, Mikhail Pekour, Jerome Fast, and Joel A. Thornton
Atmos. Meas. Tech., 16, 247–271, https://doi.org/10.5194/amt-16-247-2023, https://doi.org/10.5194/amt-16-247-2023, 2023
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We present a new, highly sensitive technique for measuring atmospheric ammonia, an important trace gas that is emitted mainly by agriculture. We deployed the instrument on an aircraft during research flights over rural Oklahoma. Due to its fast response, we could analyze correlations with turbulent winds and calculate ammonia emissions from nearby areas at 1 to 2 km resolution. We observed high spatial variability and point sources that are not resolved in the US National Emissions Inventory.
Birger Bohn and Insa Lohse
Atmos. Meas. Tech., 16, 209–233, https://doi.org/10.5194/amt-16-209-2023, https://doi.org/10.5194/amt-16-209-2023, 2023
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Optical receivers for solar spectral actinic radiation are designed for angle-independent sensitivities within a hemisphere. Remaining imperfections can be compensated for by receiver-specific corrections based on laboratory characterizations and radiative transfer calculations of spectral radiance distributions. The corrections cover a wide range of realistic atmospheric conditions and were applied to ground-based and airborne measurements in a wavelength range 280–660 nm.
Teles C. Furlani, RenXi Ye, Jordan Stewart, Leigh R. Crilley, Peter M. Edwards, Tara F. Kahan, and Cora J. Young
Atmos. Meas. Tech., 16, 181–193, https://doi.org/10.5194/amt-16-181-2023, https://doi.org/10.5194/amt-16-181-2023, 2023
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This study describes a new technique to measure total gaseous chlorine, which is the sum of gas-phase chlorine-containing chemicals. The method converts any chlorine-containing molecule to hydrogen chloride that can be detected in real time using a cavity ring-down spectrometer. The new method was validated through laboratory experiments, as well as by making measurements of ambient outdoor air and indoor air during cleaning with a chlorine-based cleaner.
Anas Emad and Lukas Siebicke
Atmos. Meas. Tech., 16, 29–40, https://doi.org/10.5194/amt-16-29-2023, https://doi.org/10.5194/amt-16-29-2023, 2023
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The true eddy accumulation (TEA) method enables measuring atmospheric exchange with slow-response gas analyzers. TEA is formulated assuming ideal conditions with a zero mean vertical wind velocity during the averaging interval. This core assumption is rarely valid under field conditions. Here, we extend the TEA equation to accommodate nonideal conditions. The new equation allows constraining the systematic error term in the measured fluxes and the possibility to minimize or remove it.
Anas Emad and Lukas Siebicke
Atmos. Meas. Tech., 16, 41–55, https://doi.org/10.5194/amt-16-41-2023, https://doi.org/10.5194/amt-16-41-2023, 2023
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A new micrometeorological method to measure atmospheric exchange is proposed, and a prototype sampler is evaluated. The new method, called short-time eddy accumulation, is a variant of the eddy accumulation method, which is suited for use with slow gas analyzers. The new method enables adaptive time-varying accumulation intervals, which brings many advantages to flux measurements such as an improved dynamic range and the ability to run eddy accumulation in a continuous flow-through mode.
Jean-Louis Bonne, Ludovic Donnat, Grégory Albora, Jérémie Burgalat, Nicolas Chauvin, Delphine Combaz, Julien Cousin, Thomas Decarpenterie, Olivier Duclaux, Nicolas Dumelié, Nicolas Galas, Catherine Juery, Florian Parent, Florent Pineau, Abel Maunoury, Olivier Ventre, Marie-France Bénassy, and Lilian Joly
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-334, https://doi.org/10.5194/amt-2022-334, 2023
Revised manuscript accepted for AMT
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We present a top-down approach to quantify CO2 and CH4 emissions at the scale of an industrial site, based on a mass balance model relying on atmospheric concentrations measurements from a new sensor embarked on-board Unmanned Aircraft Vehicles (UAVs). We present a laboratory characterization of our sensor and a field validation of our quantification method, together with field application to the monitoring of two real-world offshore oil and gas platforms.
Lu Xu, Matthew M. Coggon, Chelsea E. Stockwell, Jessica B. Gilman, Michael A. Robinson, Martin Breitenlechner, Aaron Lamplugh, John D. Crounse, Paul O. Wennberg, J. Andrew Neuman, Gordon A. Novak, Patrick R. Veres, Steven S. Brown, and Carsten Warneke
Atmos. Meas. Tech., 15, 7353–7373, https://doi.org/10.5194/amt-15-7353-2022, https://doi.org/10.5194/amt-15-7353-2022, 2022
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We describe the development and operation of a chemical ionization mass spectrometer using an ammonium–water cluster (NH4+·H2O) as a reagent ion. NH4+·H2O is a highly versatile reagent ion for measurements of a wide range of oxygenated organic compounds. The major product ion is the cluster with NH4+ produced via ligand-switching reactions. The instrumental sensitivities of analytes depend on the binding energy of the analyte–NH4+ cluster; sensitivities can be estimated using voltage scanning.
Xiaorui Chen, Haichao Wang, Tianyu Zhai, Chunmeng Li, and Keding Lu
Atmos. Meas. Tech., 15, 7019–7037, https://doi.org/10.5194/amt-15-7019-2022, https://doi.org/10.5194/amt-15-7019-2022, 2022
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N2O5 is an important reservoir of atmospheric nitrogen, on whose interface reaction ambient particles can largely influence the fate of nitrogen oxides and air quality. In this study, we develop an approach to enable the reactions of N2O5 on ambient particles directly in a tube reactor, deriving the reaction rates with high accuracy by means of a chemistry model. Its successful application helps complement the data scarcity and to fill the knowledge gap between laboratory and field results.
Yubin Chen, Bin Yuan, Chaomin Wang, Sihang Wang, Xianjun He, Caihong Wu, Xin Song, Yibo Huangfu, Xiao-Bing Li, Yijia Liao, and Min Shao
Atmos. Meas. Tech., 15, 6935–6947, https://doi.org/10.5194/amt-15-6935-2022, https://doi.org/10.5194/amt-15-6935-2022, 2022
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In this study, we demonstrate that selective online measurements of cycloalkanes can be achieved using proton transfer reaction time-of-flight mass spectrometry with NO+ chemical ionization (NO+ PTR-ToF-MS), with fast response and low detection limits. Applications of this method in both urban air and emission sources will be shown.
Marsailidh M. Twigg, Augustinus J. C. Berkhout, Nicholas Cowan, Sabine Crunaire, Enrico Dammers, Volker Ebert, Vincent Gaudion, Marty Haaima, Christoph Häni, Lewis John, Matthew R. Jones, Bjorn Kamps, John Kentisbeer, Thomas Kupper, Sarah R. Leeson, Daiana Leuenberger, Nils O. B. Lüttschwager, Ulla Makkonen, Nicholas A. Martin, David Missler, Duncan Mounsor, Albrecht Neftel, Chad Nelson, Eiko Nemitz, Rutger Oudwater, Celine Pascale, Jean-Eudes Petit, Andrea Pogany, Nathalie Redon, Jörg Sintermann, Amy Stephens, Mark A. Sutton, Yuk S. Tang, Rens Zijlmans, Christine F. Braban, and Bernhard Niederhauser
Atmos. Meas. Tech., 15, 6755–6787, https://doi.org/10.5194/amt-15-6755-2022, https://doi.org/10.5194/amt-15-6755-2022, 2022
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Ammonia (NH3) gas in the atmosphere impacts the environment, human health, and, indirectly, climate. Historic NH3 monitoring was labour intensive, and the instruments were complicated. Over the last decade, there has been a rapid technology development, including “plug-and-play” instruments. This study is an extensive field comparison of the currently available technologies and provides evidence that for routine monitoring, standard operating protocols are required for datasets to be comparable.
Caroline C. Womack, Steven S. Brown, Steven J. Ciciora, Ru-Shan Gao, Richard J. McLaughlin, Michael A. Robinson, Yinon Rudich, and Rebecca A. Washenfelder
Atmos. Meas. Tech., 15, 6643–6652, https://doi.org/10.5194/amt-15-6643-2022, https://doi.org/10.5194/amt-15-6643-2022, 2022
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We present a new miniature instrument to measure nitrogen dioxide (NO2) using cavity-enhanced spectroscopy. NO2 contributes to the formation of pollutants such as ozone and particulate matter, and its concentration can vary widely near sources. We developed this lightweight (3.05 kg) low-power (<35 W) instrument to measure NO2 on uncrewed aircraft vehicles (UAVs) and demonstrate that it has the accuracy and precision needed for atmospheric field measurements.
Alexander Håland, Tomáš Mikoviny, Elisabeth Emilie Syse, and Armin Wisthaler
Atmos. Meas. Tech., 15, 6297–6307, https://doi.org/10.5194/amt-15-6297-2022, https://doi.org/10.5194/amt-15-6297-2022, 2022
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PTR-MS is widely used in atmospheric sciences for the detection of non-methane organic trace gases. The two most widely used types of PTR-MS instruments differ in their ion source and drift tube design. We herein present a new prototype PTR-MS instrument that hybridizes these designs and combines a conventional hollow cathode glow discharge ion source with a focusing ion–molecule reactor. We also show how this new instrument performs in detecting atmospheric amines.
Gustavo Britto Hupsel de Azevedo, Bill Doyle, Christopher A. Fiebrich, and David Schvartzman
Atmos. Meas. Tech., 15, 5599–5618, https://doi.org/10.5194/amt-15-5599-2022, https://doi.org/10.5194/amt-15-5599-2022, 2022
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Strong changes in pressure, temperature, and humidity occur when small scientific aircraft ascend through the atmosphere to measure carbon dioxide. These strong changes can produce errors in the carbon dioxide measurements. To avoid these errors, we present a low-cost and simple correction method. This low-complexity method allows more researchers to study atmospheric carbon dioxide, reducing entry barriers in this field.
Ilann Bourgeois, Jeff Peischl, J. Andrew Neuman, Steven S. Brown, Hannah M. Allen, Pedro Campuzano-Jost, Matthew M. Coggon, Joshua P. DiGangi, Glenn S. Diskin, Jessica B. Gilman, Georgios I. Gkatzelis, Hongyu Guo, Hannah A. Halliday, Thomas F. Hanisco, Christopher D. Holmes, L. Gregory Huey, Jose L. Jimenez, Aaron D. Lamplugh, Young Ro Lee, Jakob Lindaas, Richard H. Moore, Benjamin A. Nault, John B. Nowak, Demetrios Pagonis, Pamela S. Rickly, Michael A. Robinson, Andrew W. Rollins, Vanessa Selimovic, Jason M. St. Clair, David Tanner, Krystal T. Vasquez, Patrick R. Veres, Carsten Warneke, Paul O. Wennberg, Rebecca A. Washenfelder, Elizabeth B. Wiggins, Caroline C. Womack, Lu Xu, Kyle J. Zarzana, and Thomas B. Ryerson
Atmos. Meas. Tech., 15, 4901–4930, https://doi.org/10.5194/amt-15-4901-2022, https://doi.org/10.5194/amt-15-4901-2022, 2022
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Understanding fire emission impacts on the atmosphere is key to effective air quality management and requires accurate measurements. We present a comparison of airborne measurements of key atmospheric species in ambient air and in fire smoke. We show that most instruments performed within instrument uncertainties. In some cases, further work is needed to fully characterize instrument performance. Comparing independent measurements using different techniques is important to assess their accuracy.
Woohui Nam, Changmin Cho, Begie Perdigones, Tae Siek Rhee, and Kyung-Eun Min
Atmos. Meas. Tech., 15, 4473–4487, https://doi.org/10.5194/amt-15-4473-2022, https://doi.org/10.5194/amt-15-4473-2022, 2022
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We describe our vibration-resistant instrument for measuring ambient NO3, NO2, and H2O based on cavity-enhanced absorption spectroscopy. By simultaneous retrieval of H2O with the other species using a measured H2O absorption spectrum, direct quantifications among all species are possible without any pre-treatment for H2O. Our instrument achieves the effective light path to ~101.5 km, which allows the sensitive measurements of NO3 and NO2 as 1.41 pptv and 6.92 ppbv (1σ) in 1 s.
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Short summary
Unmanned aircraft could provide a cost-effective way to close gaps in the observation of the carbon cycle, provided that small yet accurate analysers are available. We have developed a COmpact Carbon dioxide analyser for Airborne Platforms (COCAP). During validation of its CO2 measurements in simulated and real flights we found a measurement error of 1.2 μmol mol−1 or better with no indication of bias. COCAP is a self-contained package that has proven well suited for operation on board UASs.
Unmanned aircraft could provide a cost-effective way to close gaps in the observation of the...
